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At least 127 records · Page 7

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DOE OSTI2023

4'-Deoxypyridoxine disrupts vitamin B 6 homeostasis in Escherichia coli K12 through combined inhibition of cumulative B 6 uptake and PLP-dependent enzyme activity

Pyridoxal 5'-phosphate (PLP) is the active form of vitamin B 6 and a cofactor for many essential metabolic processes such as amino acid biosynthesis and one carbon metabolism. 4’-deoxypyridoxine (4dPN) is a long known B 6 antimetabolite but its mechanism of action was not totally clear. By exploring different conditions in which PLP metabolism is affected in the model organism Escherichia coli K12, we showed that 4dPN cannot be used as a source of vitamin B 6 as previously claimed and that it is toxic in several conditions where vitamin B 6 homeostasis is affected, such as in a B 6 auxotroph or in a mutant lacking the recently discovered PLP homeostasis gene, yggS . In addition, we found that 4dPN sensitivity is likely the result of multiple modes of toxicity, including inhibition of PLP-dependent enzyme activity by 4’-deoxypyridoxine phosphate (4dPNP) and inhibition of cumulative pyridoxine (PN) uptake. These toxicities are largely dependent on the phosphorylation of 4dPN by pyridoxal kinase (PdxK).

59 BASIC BIOLOGICAL SCIENCES↗

DOE OSTI2025

Si content in methacrylamide-containing A- b -(B- r -C) block copolymers and its impact on reactive ion etching properties

Block copolymers (BCPs) of an A-block-(B-random-C) architecture have been explored as materials for nanolithography because the composition and chemistry of the random block enables modification of thermodynamic and wetting properties to meet manufacturing criteria. Here, in this study, A-b-(B-r-C) BCPs created by an amidation reaction of polystyrene-block-poly(pentafluorophenyl methacrylate) (PS-b-PPFMA) with controlled amounts of Si add insight to previous conclusions about the dual contributions of BCP chemistry and reactive ion etch (RIE) gas chemistry on etch properties. We focus on two RIE etch characteristics: organosilicon etch resistance in H 2 /N 2 plasma etching and enhanced removal of non-styrenic structures in an Ar/O 2 etch. Consistent with previous studies, higher amounts of Si result in greater etch resistance under H 2 /N 2 RIE, where at least ∼10 wt. % Si is necessary to exhibit sufficient etch resistance. By contrast, Ar/O 2 etching resulted in etch rates independent of Si content. We observe previously unreported surface roughening aligned with morphological domains during the H 2 /N 2 etch of modified PS-b-PPFMA BCPs. Limited in the amount of allowable Si to attain equal surface energy between blocks, these BCPs are further disqualified in forming a Si-containing mask. However, in an Ar/O 2 etch, the same BCPs exhibit suitable etch contrast and smooth domain structures, forming a uniform PS mask. Ultimately, this study uses the chemical flexibility of these materials to demonstrate the mechanisms of interactions between BCP and etch chemistry that must be considered to design effective materials for pattern transfer applications.

Eom, Christopher J. [University of Chicago, IL (Un↗

NASA NTRS1995

Theoretical Study of the B(sup 3) Sigma(sup -, sub u) - X(sup3)Sigma(sub g, sup -) and B"(sup 3)Pi(sub u) - X(sup 3)Sigma(sub g, sup -) Band Systems of S(sub 2)

Multireference configuration-interaction (MRCI) wavefunctions and potential energy curves have been calculated for the X(sup 3)Sigma(sub g,sup -), B(sup 3)Sigma(sub u, Sup -) and B"(sup 3)Pi((sub u) states of S(sub 2) using correlation consistent Gaussian basis sets. These wavefunctions are utilized to compute the the transition dipole moments of the B(sup 3)Sigma(sub g, sup -) - X(sup 3) Sigma(sub g, sup -) and B"(sup 3)Pi(sub u) - X(sup 3)Sigma(sub g, sup -) systems. Oscillator strengths, transition probabilities, and radiative lifetimes are computed for the X-B system and comparison is made with experimental data.

Pradhan, Atul D.↗

DOE OSTI2023

A study of $CP$ violation in the decays $B^±$ → [$K^+ K^-π^+π^-$]$_Dh^±$ ($h$ = $K, π$) and $B^±$ → [$π^+π^-π^+π^-$]$_Dh^±$

The first study of CP violation in the decay mode $B^±$ → [$K^+ K^-π^+π^-$]$_Dh^±$, with $h$ = $K, π$, is presented, exploiting a data sample of proton–proton collisions collected by the LHCb experiment that corresponds to an integrated luminosity of 9 fb -1 . The analysis is performed in bins of phase space, which are optimised for sensitivity to local CP asymmetries. CP-violating observables that are sensitive to the angle γ of the Unitarity Triangle are determined. The analysis requires external information on charm-decay parameters, which are currently taken from an amplitude analysis of LHCb data, but can be updated in the future when direct measurements become available. Measurements are also performed of phase-space integrated observables for $B^±$ → [$K^+ K^-π^+π^-$]$_Dh^±$ and $B^±$ → [$π^+π^-π^+π^-$]$_Dh^±$ decays.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

DOE OSTI2022

Cubic Crystal Structure Formation and Optical Properties within the Ag–B II –M IV –X (B II = Sr, Pb; M IV = Si, Ge, Sn; X = S, Se) Family of Semiconductors

Quaternary chalcogenide semiconductors are promising materials for energy conversion and nonlinear optical applications, with properties tunable primarily by varying the elemental composition and crystal structure. Here, we first analyze the connections among several cubic crystal structure types, as well as the orthorhombic Ag 2 PbGeS 4 -type structure, reported for select members within the Ag–B II –M IV –X (B II = Sr, Pb; M IV = Si, Ge, Sn; X = S, Se) compositional space. Focusing on the Ag–Pb–Si–S and Ag–Sr–Sn–S systems, we show that one structure type, with the formulas Ag 2 Pb 3 Si 2 S 8 and Ag 2 Sr 3 Sn 2 S 8 , is favored. We have prepared powder and single-crystal samples of Ag 2 Pb 3 Si 2 S 8 and Ag 2 Sr 3 Sn 2 S 8 , showing that each takes on the noncentrosymmetric cubic space group I$\bar{43}$d and is isostructural to the previously reported compound Ag 2 Sr 3 Ge 2 Se 8 . Through hybrid density functional theory calculations, these cubic compounds are demonstrated to be (quasi-)direct band gap semiconductors with high densities of states at the band maxima. Furthermore, the band-gap energies are measured by reflectance spectroscopy as 1.95(3) and 2.66(4) eV for Ag 2 Pb 3 Si 2 S 8 and Ag 2 Sr 3 Sn 2 S 8 , respectively. We further measure the optical properties and show the electronic band structures of three other isostructural A I –B II –M IV –X-type materials, i.e., Ag 2 Sr 3 Si 2 S 8 , Ag 2 Sr 3 Ge 2 S 8 , and Ag 2 Sr 3 Ge 2 Se 8 , showing that the band gaps can be predictably tuned by element substitution. Detailed visual analyses of the different structures and of their relationships with other members of the Ag–B II –M IV –X compositional family provide a basis for a broader understanding of the structure formation and optoelectronic properties within the quaternary chalcogenide semiconductor family.

14 SOLAR ENERGY↗

DOE OSTI2024

TOI-2374 b and TOI-3071 b: two metal-rich sub-Saturns well within the Neptunian desert

ABSTRACT We report the discovery of two transiting planets detected by the Transiting Exoplanet Survey Satellite (TESS), TOI-2374 b and TOI-3071 b, orbiting a K5V and an F8V star, respectively, with periods of 4.31 and 1.27 d, respectively. We confirm and characterize these two planets with a variety of ground-based and follow-up observations, including photometry, precise radial velocity monitoring and high-resolution imaging. The planetary and orbital parameters were derived from a joint analysis of the radial velocities and photometric data. We found that the two planets have masses of (57 ± 4) M⊕ or (0.18 ± 0.01) MJ, and (68 ± 4) M⊕ or (0.21 ± 0.01) MJ, respectively, and they have radii of (6.8 ± 0.3) R⊕ or (0.61 ± 0.03) RJ and (7.2 ± 0.5) R⊕ or (0.64 ± 0.05) RJ, respectively. These parameters correspond to sub-Saturns within the Neptunian desert, both planets being hot and highly irradiated, with Teq ≈ 745 K and Teq ≈ 1812 K, respectively, assuming a Bond albedo of 0.5. TOI-3071 b has the hottest equilibrium temperature of all known planets with masses between 10 and 300 M⊕ and radii less than 1.5 RJ. By applying gas giant evolution models we found that both planets, especially TOI-3071 b, are very metal-rich. This challenges standard formation models which generally predict lower heavy-element masses for planets with similar characteristics. We studied the evolution of the planets’ atmospheres under photoevaporation and concluded that both are stable against evaporation due to their large masses and likely high metallicities in their gaseous envelopes.

Hacker, Alejandro (ORCID:0009000994520181)↗

NASA NTRS2020

TOI-481 b and TOI-892 b: Two Long-period Hot Jupiters from the Transiting Exoplanet Survey Satellite

We present the discovery of two new 10 day period giant planets from the Transiting Exoplanet Survey Satellite mission, whose masses were precisely determined using a wide diversity of ground-based facilities. TOI-481 b and TOI-892 b have similar radii (0.99 ± 0.01 R(J) and 1.07 ± 0.02 R(J), respectively), and orbital periods (10.3311 days and 10.6266 days, respectively), but significantly different masses (1.53 ± 0.03 M(J) versus 0.95 ± 0.07 M(J), respectively). Both planets orbit metal-rich stars ([Fe/HG] = +0.26 ± 0.05 dex and [Fe/H] = +0.24 ± 0.05 for TOI-481 and TOI-892, respectively) but at different evolutionary stages. TOI-481 is a M(*) = 1.14 ± 0.02 Mꙩ, R(*) = 1.66 ± 0.02 Rꙩ G-type star (T(eff) = 5735 ± 72 K), that with an age of 6.7 Gyr, is in the turn-off point of the main sequence. TOI-892 on the other hand, is a F-type dwarf star (T(eff) = 6261 ± 80 K), which has a mass of M(*) = 1.28 ± 0.03 Mꙩ and a radius of R(*) = 1.39 ± 0.02 Rꙩ. TOI-481 b and TOI-892 b join the scarcely populated region of transiting gas giants with orbital periods longer than 10 days, which is important to constrain theories of the formation and structure of hot Jupiters.

Rafael Brahm↗

DOE OSTI2022

Precise determination of the $B^0_S - \bar {B}^0_S$ oscillation frequency

Mesons comprising a beauty quark and strange quark can oscillate between particle ($B^0_s$) and antiparticle ($\bar{B}^0_s$) flavour eigenstates, with a frequency given by the mass difference between heavy and light mass eigenstates, Δm s . Here we present a measurement of Δm s using $B^0_s$ → $D^–_sπ^+$ decays produced in proton–proton collisions collected with the LHCb detector at the Large Hadron Collider. The oscillation frequency is found to be Δm s = 17.7683 ± 0.0051 ± 0.0032 ps –1 , where the first uncertainty is statistical and the second is systematic. This measurement improves on the current Δm s precision by a factor of two. We combine this result with previous LHCb measurements to determine Δm s = 17.7656 ± 0.0057 ps –1 , which is the legacy measurement of the original LHCb detector.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

DOE OSTI2024

Search for the e + e − → η b ( 1 S ) ω and e + e − → χ b 0 ( 1 P ) ω processes at s = 10.745 GeV

We search for the e + e − → η b ( 1 S ) ω and e + e − → χ b 0 ( 1 P ) ω processes at a center-of-mass energy of 10.745 GeV, which is close to the peak of the ϒ ( 10753 ) state. We use data collected by the Belle II experiment during a special run, corresponding to an integrated luminosity of 9.8 fb − 1 . We reconstruct ω → π + π − π 0 decays and use the ω meson’s recoil mass to search for the signals. We do not find evidence for either process, and set upper limits on the corresponding Born-level cross sections of 2.5 pb and 7.8 pb, respectively, at the 90% confidence level. The χ b 0 ( 1 P ) ω limit is the result of a combination of this analysis and a previous search using full reconstruction. Published by the American Physical Society 2024

Astronomy & Astrophysics↗

DOE OSTI2025

Basis light-front quantization for the Λ b and Σ b baryons

Within the basis light-front quantization framework, we compute the masses and light-front wave functions of the Λ b baryon and its isospin triplet counterparts Σ b + , Σ b 0 , and Σ b − using a light-front effective Hamiltonian in the leading Fock sector. These wave functions are obtained as eigenstates of the effective Hamiltonian, which incorporates the one-gluon exchange interaction with fixed coupling and a three-dimensional confinement potential. With the quark masses and the couplings as adjustable parameters, the computed masses are set within the experimental range. The resulting predictions for their electromagnetic properties align well with other theoretical calculations. Additionally, the parton distribution functions (PDFs) of these baryons are obtained for the first time, with gluon and sea quark distributions dynamically generated through QCD evolution of the valence quark PDFs. Published by the American Physical Society 2025

Meng, Lingdi (ORCID:0009000096439904)↗

DOE OSTI2020

TOI-481 b and TOI-892 b: Two Long-period Hot Jupiters from the Transiting Exoplanet Survey Satellite

We present the discovery of two new 10 day period giant planets from the Transiting Exoplanet Survey Satellite mission, whose masses were precisely determined using a wide diversity of ground-based facilities. TOI-481 b and TOI-892 b have similar radii (0.99 ± 0.01 R{sub J} and 1.07 ± 0.02 R{sub J}, respectively), and orbital periods (10.3311 days and 10.6266 days, respectively), but significantly different masses (1.53 ± 0.03 M{sub J} versus 0.95 ± 0.07 M{sub J}, respectively). Both planets orbit metal-rich stars ([Fe/H] = +0.26±0.05 dex and [Fe/H] = +0.24±0.05 for TOI-481 and TOI-892, respectively) but at different evolutionary stages. TOI-481 is a M{sub ⋆} = 1.14 ± 0.02 M{sub ⊙}, R{sub ⋆} = 1.66 ± 0.02 R{sub ⊙} G-type star (T{sub eff} = 5735±72 K), that with an age of 6.7 Gyr, is in the turn-off point of the main sequence. TOI-892 on the other hand, is a F-type dwarf star (T{sub eff} = 6261±80 K), which has a mass of M{sub ⋆} = 1.28 ± 0.03 M{sub ⊙} and a radius of R{sub ⋆} = 1.39 ± 0.02 R{sub ⊙}. TOI-481 b and TOI-892 b join the scarcely populated region of transiting gas giants with orbital periods longer than 10 days, which is important to constrain theories of the formation and structure of hot Jupiters.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2021

TOI-954 b and K2-329 b: Short-period Saturn-mass Planets that Test whether Irradiation Leads to Inflation

We report the discovery of two short-period Saturn-mass planets, one transiting the G subgiant TOI-954 (TIC 44792534, V = 10.343, T = 9.78) observed in TESS sectors 4 and 5 and one transiting the G dwarf K2-329 (EPIC 246193072, V = 12.70, K = 10.67) observed in K2 campaigns 12 and 19. We confirm and characterize these two planets with a variety of ground-based archival and follow-up observations, including photometry, reconnaissance spectroscopy, precise radial velocity, and high-resolution imaging. Combining all available data, we find that TOI-954 b has a radius of 0.852{sub −0.062}{sup +0.053} R{sub J} and a mass of 0.174{sub −0.017}{sup +0.018} M {sub J} and is in a 3.68 day orbit, while K2-329 b has a radius of 0.774{sub −0.024}{sup +0.026} R{sub J} and a mass of 0.260{sub −0.022}{sup +0.020} M {sub J} and is in a 12.46 day orbit. As TOI-954 b is 30 times more irradiated than K2-329 b but more or less the same size, these two planets provide an opportunity to test whether irradiation leads to inflation of Saturn-mass planets and contribute to future comparative studies that explore Saturn-mass planets at contrasting points in their lifetimes.

47 OTHER INSTRUMENTATION↗

NASA NTRS1991

Spectral differences in the QSO pairs Q1634 + 267A,B and Q2345 + 007A,B and the gravitational lens interpretation

High S/N spectra of two candidate gravitational lens pairs, over the wavelength range 3150-7000 A at 4-6 A resolution are obtained in order to compare the emission line, continuum, and absorption line properties. The continuum shapes of Q1634 + 267A,B over the observed wavelength range agree remarkably well, and a constant multiplicative factor of 3.28 is found for the ratio A/B over the whole observed wavelength range. In agreement with previous investigations, it is found that the redshifts of the C III 1909 emission line are consistent with zero relative velocity shift and that the line profiles in the two images are identical. The continua of Q2345 + 007A and B match fairly well over the whole observed wavelength range if a constant scaling factor of 2.51 is used. Scaled difference spectra show that the Ly-alpha, NV, CIII, and Fe II emission lines are stronger relative to the continuum in Q2345 + 007B than in A. It is concluded that the pairs of images constituting Q1634 + 267A and B and Q2345 + 007A and B both result from gravitatinal lensing.

Steidel, Charles C.↗

NASA NTRS1995

Compendium of NASA data base for the global tropospheric experiment's Pacific Exploratory Mission West-B (PEM West-B)

This compendium describes aircraft data that are available from NASA's Pacific Exploratory Mission West-B (PEM West-B). PEM West is a component of the International Global Atmospheric Chemistry's (IGAC) East Asia/North Pacific Regional Study (APARE) project. Objectives of PEM West are to investigate the atmospheric chemistry of ozone over the northwest Pacific -- natural budgets and the impact of anthropogenic/continental sources; and to investigate sulfur chemistry -- continental and marine sulfur sources. The PEM West program encompassed two expeditions. PEM West-A was conducted in September 1991 during which the predominance of tropospheric air was from mid-Pacific (marine) regions, but (at times) was modified by Asian outflow. PEM West-B was conducted during February 1994, a period characterized by maximum Asian outflow. Results from PEM West-A and B are public domain. PEM West-A data are summarized in NASA TM 109177 (published February 1995). Flight experiments were based at Guam, Hong Kong, and Japan. This document provides a representation of NASA DC-8 aircraft data that are available from NASA Langley's Distributed Active Archive Center (DAAC). The DAAC includes numerous other data such as meteorological and modeling products, results from surface studies, satellite observations, and sonde releases.

Gregory, Gerald L.↗

NASA NTRS1995

Synthesis of Substituted 2,3,5,6-tetraarylbenzo(1,2-b:5,4-b')difurans

A series of substituted 2,3,5,6-tetraarylbenzo(l,2-b:5,4-b')difurans 1 was synthesized. This synthesis is based upon the photocyclization of 2,5-dibenzoylresorcinol dibenzyl ethers to the corresponding tetrahydrobenzo(1,2-b:5,4-b')difurans. Treatment of the photoproducts with methanesulfonyl chloride in pyridine afforded 1 in overall yields ranging from 30-72%. A number of these compounds have high fluorescence quantum yields (of phi(sub f) = 0.76-0.90), and their fluorescence spectra exhibit large solvatochromic shifts. These compounds may be suitable for use as fluorescent probes.

Abdul-Aziz, Mahmoud↗

NASA NTRS2000

Compendium of NASA Data Base for the Global Tropospheric Experiment's Pacific Exploratory Mission-Tropics B (PEM-Tropics B): DC-8 - Volume 1

This report provides a compendium of NASA aircraft data that are available from NASA's Global Tropospheric Experiment's (GTE) Pacific Exploratory Mission-Tropics B (PEM-Tropics B) conducted in March and April 1999. PEM-Tropics B was conducted during the southern-tropical wet season when the influence from biomass burning observed in PEM-Tropics A was minimal. Major deployment sites were Hawaii, Kiritimati (Christmas Island), Tahiti, Fiji, and Easter Island. The broad goals of PEM-Tropics B were to improved understanding of the oxidizing power of the atmosphere and the processes controlling sulfur aerosol formation and to establish baseline values for chemical species that are directly coupled to the oxidizing power and aerosol loading of the troposphere. The purpose of this document is to provide a representation of aircraft data that will be available in archived format via NASA Langley's Distributed Active Archive Center (DAAC) or are available through the GTE Project Office archive. The data format is not intended to support original research/analysis, but to assist the reader in identifying data that are of interest.

Scott, A. Donald, Jr.↗

NASA NTRS2000

Compendium of NASA Data Base for the Global Tropospheric Experiment's Pacific Exploratory Mission - Tropics B (PEM-Tropics B): P-3B - Volume 2

Scott, A. Donald, Jr.↗

DOE OSTI2024

Form factors for semileptonic B-decays with HISQ light quarks and clover b-quarks in Fermilab interpretation

We compute the vector, scalar, and tensor form factors for the $B\to \pi$, $B\to K$, and $B_s\to K$ amplitudes, which are needed to describe semileptonic $B$-meson decay rates for both the charged and neutral current cases. We use the highly improved staggered quark (HISQ) action for the sea and light valence quarks. The bottom quark is described by the clover action in the Fermilab interpretation. Simulations are carried out on $N_f = 2+1+1$ MILC HISQ ensembles at approximate lattice spacings from $0.15$ fm down to $0.057$ fm. We present blinded preliminary results for the form factors.

Jeong, Hwancheol↗