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Results of South-East Flux Trap Dosimetry Measurements for the Advanced Test Reactor Critical Facility in support of Advanced Sensors and Instrumentation Development

Reactor dosimetry measurements are commonly used to validate simulation and modeling in nuclear reactor tests. Numerous standard dosimeter materials exist which are commonly utilized with sensitivities to different energy ranges of neutrons. At the Advanced Test Reactor (ATR), cobalt alloy and pure nickel wires are installed every cycle to monitor thermal- and fast-neutron fluence rates. However, there is growing interest in exploring less commonly used materials which are either more sensitive to different parts of the neutron energy spectrum or which can incorporate multiple activation paths in a single material. Epithermal and fast-neutron energies beyond the typical 1-MeV threshold are of particular interest. Two ATR-C Flux Runs took place during 2024; each flux run included supplemental dosimetry packages in the South-East Flux Trap (SEFT) Filler. The focus of the dosimetry package for flux run 23-4 was to test two novel dosimetry methods that can provide simultaneous thermal and threshold (fast) sensitivity in a single dosimeter wire. A selection of 3% Au in Cu alloyed wires were available that provided sensitivity to fast and thermal neutrons through 5 different reactions. Likewise, Fe offers multiple interaction pathways with sensitivity to both thermal and fast neutrons. The main question to be answered by these irradiations was if sufficient radioactivation would take place in the ATR-C SEFT during a nominal 20-minute irradiation at typical power levels (near 600Wth) to observe the threshold reactions that have smaller activation cross-sections than the thermal reactions without being saturated by interfering interactions and Compton continuum during the High-Purity Germanium (HPGe) measurements. The results from comparing the measurement results to anticipated activity levels provide confidence in our ability to activate both traditional and novel dosimetry materials in ATR-C, however not all the measured values matched with the predicted activities. This leaves further room for investigation both on the experimental and computational approaches for future irradiation experiments.

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Graphite for Advanced Nuclear Reactors: Deployment Readiness Review

Historically, graphite has been used in numerous reactor technologies, including research/test reactors and, commercially, in advanced gas reactors. These non-metallic materials can play a key role as internal core structures, reflectors, or neutron moderators, making them important for deployment of certain advanced reactor technologies. This report explores the industry readiness for graphite material deployment, documenting Codes and Standards applicable to their design, qualification, and manufacturing. Discussions also examine the manufacturing processes, aging/degradation, inspection techniques, and disposal options. The report covers the current status, documents gaps, and proposes some conclusions about approaches to managing some of the current gaps.

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Depletion Benchmark of the AFIP-7 Experiment in the Advanced Test Reactor

Reactor physics depletion benchmarks for low-enriched uranium fuel are limited in number. In particular, there is very limited data for LEU benchmarks for U-10Mo (Uranium-10% Molybdenum) plate fuel developed for use in U.S. high-performance research reactors (USHPRR). USHPRR includes the Advanced Test Reactor (ATR), Advanced Test Reactor Critical Facility (ATR-C), High Flux Isotope Reactor (HFIR), University of Missouri Research Reactor (MURR), Massachusetts Institute of Technology Reactor (MITR), and National Bureau of Standards Reactor (NBSR) at the National Institute of Science and Technology. These reactors are fueled with high-enriched uranium dispersed fuel in a silicon/aluminum matrix. In support of conversion to a HALEU fuel, qualification of U-10Mo formed into a monolithic foil is being performed. Fuel qualification involves irradiated fueled specimens in the ATR. The irradiation tests provide an opportunity to benchmark depletion capabilities of reactor physics codes in support of the ATR operation, as well as develop benchmarks that can be used by other institutions to benchmark other reactor physics codes. This report documents the development of a benchmark model of the irradiation of the ATR Full -size plate In center flux trap Position 7 (AFIP-7) experiment.

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Advanced Test Reactor Neutron Dosimetry Report - Cycle 175C: Results of Neutron Dosimetry Measurements for the Advanced Test Reactor Cycle 175C

Results of neutron dosimetry measurements in ATR for cycle 175C are presented. A single set of cobalt and nickel wires were installed in numerous irradiation locations for the duration of the cycle. The specific activity of these wire segments can be used in conjunction with the presented cycle history information to determine the thermal- and fast-neutron fluence rates for each irradiation position during the cycle using the referenced standard test methods.

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Potential Supply Chain and Cost Reduction Strategies for Advanced Nuclear Reactors

This milestone represents a level of effort to provide recommendations for a supply chain plan and establish relationships between advanced reactor companies and large companies in the oil & gas and chemical industries. It represents a starting point to develop the plan with options, general equipment lists, and rough associated cost estimates of major equipment and the associated systems needed. This effort will provide an opportunity to leverage the experience that oil & gas and chemicals companies possess in large capital equipment procurement, modularization, acquisition and installation. Potential supply chain solutions will be discussed and preliminary options for worldwide manufacturers will be elucidated. The goal of this effort will be to leverage the years of accumulated experience in the oil & gas and chemical industries in the area of capital equipment acquisition to understand the potential supply chain options and to reduce potential acquisition costs by optimizing the supply chain options for advanced nuclear reactor modularization, manufacturing and acquisition.

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Accident Progression and Source Term Demonstration Calculations for the Advanced Burner Test Reactor (ABTR)

As advanced reactor designers approach broad deployment of new reactor technologies and the associated applications, a critical milestone on this path includes licensing or authorization of these designs in the current regulatory environment. Commercial licensing and DOE authorization both consist of numerous aspects to not only certify the designed plant will operate as intended, but also related to confirmation of the safe operation of these facilities that comply with specific standards and requirements. To that end, domestic industry and regulators require toolsets and methods which can be used to confirm that advanced reactor designs not only align with expected performance during normal operation, but also a series of transient scenarios. These codes require a satisfactory validation basis, and in the absence of such a basis, code-to-code comparisons are often utilized as a surrogate to confirm model adequacy. To support this need for fast reactor technologies, a series of analyses using SAS4A/SASSYS- 1 and the Simplified Radionuclide Transport (SRT) code have been conducted for the Advanced Burner Test Reactor (ABTR). These analyses are expected to not only provide a baseline for transient and source term analyses of ABTR, but to also provide context for the key physics that determine evolution of specific transient scenarios in a sodium-cooled fast reactor (SFR). These codes are utilized for this work given their adoption in the SFR industry and by key SFR stakeholders.

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Conceptual Design of a Thermal–to-14-MeV Neutron Conversion Device for Use in the Advanced Test Reactor

Here, this paper details the conceptual design of a thermal-to-14-MeV neutron converter consisting of a mixture of lithium and deuterium in a blanket material. Such a device operates a two-step reaction, first generating tritons via thermal neutron absorption in the tritium breeding material, and in the second step, high-energy neutrons are produced either via deuterium-tritium fusion reaction or with tritium reacting with lithium. A thermal-to-14-MeV neutron converter significantly hardens the neutron spectrum by virtually removing thermal neutrons and adding a high-energy 14 MeV component to the neutron spectrum. While similar concepts have been previously proposed and tested in other reactors, the unique characteristics of the Advanced Test Reactor (ATR), namely its important thermal flux (up to $10^{15}$ n.cm$^{-2}$.s$^{-1}$) makes it markedly attractive for obtaining a very large fast neutron flux, usable for irradiation studies under neutron flux conditions prototypical of fusion reactors. The paper provides a description of a new computational scheme developed for handling the coupled neutron-triton transport mechanism using the Geant4 toolkit. Resulting neutron spectra and high-energy neutron yields are summarized for different irradiation positions and potential neutron breeder materials. Maximum predicted thermal-to-14-MeV neutron yields are on the order of $2.10^{-4}$, which is consistent with previous studies found in the literature. Thus, when placed inside the ATR, such a neutron converter will be providing the largest high-energy neutron source available for activation and irradiation studies of materials foreseen for use in fusion reactors. Future steps will involve qualifying the computational scheme using the ATR critical facility using activation foil measurements.

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A machine-learning-aided data recovery approach for predicting multi-material thermal behaviors in advanced test reactor capsules

Instrumented experiments conducted at test reactors are essential to the deployment of new advanced reactor systems. Designing new experiments and generating data on specific reactor conditions require significant investments in terms of both time and cost. Finite element analysis software can be used to create high-fidelity models of experiment environments in order to support the actual experiments, but computation time remains a concern in terms of applying outcomes to real-time usage of data (e.g., a digital twin [DT]). Here, the present research proposes a machine-learning (ML) aided approach to making temperature and displacement predictions based on the thickness of the outer gas gap on the experimental capsule used for in-pile demonstration of a novel new thermal conductivity probe in the Advanced Test Reactor (ATR). This capsule consisted of U10Zr fuel, a rodlet, sodium, and inner and outer capsules. Gas gaps existed between the fuel and the rodlet, and between the inner and the outer capsule. The learning data pertained to an experimental capsule's radial distributions of temperature and displacement, as obtained based on Abaqus and the physical features. For the first step of ML sequence, the temperature was predicted using three positional parameters. Next, the displacement was predicted using seven additional parameters. Each physical feature was normalized in order to be both nondimensional and standardized. The temperature and displacement predictions showed good agreement with the simulation results in all cases involving interpolation and extrapolation. Furthermore, data similarity enhancement increased the similarity between the training and the target data, thereby increasing the predictive accuracy of the ML models. In certain extrapolation cases involving limited original ML model accuracy, data similarity enhancement and data recovery was able to somewhat improve this accuracy.

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Test and Evaluation of Radiofrequency Tamper Indicating Devices for Remote Monitoring of Advanced/Small Modular Reactors

Advanced and small modular reactors (A/SMRs), due to their versatile nature, are likely to be used in remote locations to provide electrical power or other services in regions that are difficult to access or have limited transportation infrastructure. This will result in limited on-site staff, therefore driving A/SMR vendors to consider remote monitoring as a solution to support nuclear security. Maintaining Continuity of Knowledge (CoK) of nuclear material quantities and locations is vital to nuclear security, and remote monitoring of active tamper indicating devices (TIDs) has been well established as a component of International Atomic Energy Agency (IAEA) Safeguards since the early 2000s. Active TIDs, such as radiofrequency TIDs (RFTIDs), immediately alarm upon unauthorized access attempts, promoting timely detection. In contrast, passive TIDs require a surveillance regime and offer delayed detection. Active TIDs deter insiders and enable prompt detection of malicious acts. They can be used on nuclear material containers and controlled entry points like vaults and toolboxes. Therefore, the implementation of RFTIDs into security programs bolsters overall nuclear material control, and provides a visible deterrent, with primary efficacy in mitigating the insider threat and potentially allowing for Security by Design considerations. They are a strong candidate technology for maintaining nuclear security of A/SMRs but need to be evaluated for feasibility and implementation into the wider physical protection system.

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Assessment of Thin Plastic Scintillation Detectors for Beta-Particle Measurements at the Advanced Test Reactor Critical Facility

The Fission Wire Measurement System is a custom measurement system designed in the 1960s to measure the beta-particle activity of irradiated uranium-aluminum fission wires. This measurement is conducted to determine the fission rate profile of the Advanced Reactor Test Critical facility. The Advanced Test Reactor Critical facility is an open-pool, low-power test reactor used to qualify experiment configurations and verify core models prior to full-power experiment irradiations in the Advanced Test Reactor. Power distribution measurements in ATR-C use uranium-aluminum wires that are distributed throughout the core to validate simulation and modeling results. These measurements require from 340 to 1500 wires to be irradiated and measured within a 12-hour window. The system consists of 4 measurement channels and one reference channel, each with a 2-pi proportional gas flow detector and the measurement channels each have an automated sample changer. The gas flow detectors are of a custom design for this detector system that use methane gas with a large anode wire compared to modern proportional counters. These detectors, which are nearly 60 years old are irreplaceable. The measurements from these gas detectors are affected by the gas flow rate, atmospheric and line pressure, and are very sensitive to the applied high voltage. Recent improvements have been made to the control and data acquisition system, but the detectors have remained the same. The nature of the measurement of the fission product decay activity is such that the energy spectrum of the signal is changing with time. Thin, 250-um thick, plastic scintillators were commercially obtained as a potential replacement for the gas flow detectors. The original calibration of the uranium-aluminum fission wires was conducted in 1965 using a series of irradiations of gold foils and the wires in a well-characterized thermal neutron field. These measurements provided a time-dependent fission rate conversion factor from the gold foil data to calibrate the fission wires based on the response from the 2-pi proportional gas detectors. Transitioning to the new detectors requires qualification and testing. The sensitivity of the scintillators to changes in the energy spectrum of the fission wires and translation of the calibration factor have been completed. These measurements indicated that the sensitivity of the scintillators over time changes at a different rate than the sensitivity of the gas flow detectors. However, the inverse activity of measurements of both detector types is linear with time. Initial results indicate that the scintillator detectors will be a sufficient replacement for the gas detectors with minor adjustments to the fission rate conversion factor. Replacement of the detectors will improve the fission wire measurements and provide a more stable and reliable measurement system.

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Performance Investigation of High-temperature Latent Heat Storage for Integration with Advanced Nuclear Reactors

Integrating thermal energy storage (TES) with advanced nuclear reactors enhances the flexible use of nuclear energy, facilitating its expansion beyond conventional electricity generation. High-temperature TES, capable of storing heat above 400 degree C, emerges as a vital carbon-free energy solution for decarbonizing industrial sector, especially when combined with low-emission energy sources like advanced nuclear reactors. Idaho National Laboratory (INL) has recently developed a novel design for high-temperature latent heat storage system, called Heat pipe Integrated Thermal Battery (HITB), and efforts are underway to experimentally demonstrate the concept. HITB employs liquid-metal heat pipes to establish thermal linkage between TES and nuclear systems without direct fluid exchange, minimizing the potential risk of the integrated systems such as cross-contamination. HITB is designed to achieve high charging and discharging efficiency as well as high energy storage density by employing metal alloys as Phase Change Material (PCM). Initial proof-of-concept experiments are being undertaken using an aluminum alloy (Al59%-Mg35%-Zn6%). This paper discusses current progress of the HITB project at INL, seeking to develop high-temperature TES for versatile integration with advanced nuclear reactors, and shares insights from the performance evaluations via numerical modeling and analysis.

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Analytical and Performance-Based Evaluation Alternatives to Full-Scope, High-Fidelity Testbeds

One consequence the design and operational differences of advanced reactors is that integrated system validation (ISV) using full-scope, high-fidelity testbed might not be cost-justified or practical. The absence of traditional ISV may pose an issue for the conduct of safety evaluations since it may leave regulators without the information derived from this performance-based testing. The purpose of this research is to identify analytical and performance-based test and evaluation methods that are alternatives to full-scope, high-fidelity testbeds that have traditionally been used for ISV. We developed a method to test validation based on a multi-stage validation (MSV) framework. MSV is an approach to meeting validation objectives through incremental, successive validation activities beginning in the early stages of the design process and continuing through the later stages. MSV doesn't rely solely on late stage validation, rather it accommodates the use of a broad spectrum of analytical and performance-based information and a diversity of testbeds. In addition, MSV embraces the use of information from other types of evaluations and analyses.

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Benchmarking MCNP models to support gamma irradiation experiments

Seismic isolators and damping devices have been used for 30+ years to reduce seismic forces and deployed in 10,000+ structures, including bridges, buildings, and mission-critical infrastructure. Studies have shown that seismic isolation of nuclear power plants can reduce the seismic risk by several orders of magnitude and substantially reduce the overnight capital cost. Advanced reactor developers are considering seismic isolation as an integral design feature in their reactor design. It can either be deployed at the building level, isolating the entire reactor building, or at the component level, isolating individual pieces of safety-class equipment, such as a reactor vessel or a steam generator. For equipment isolation, located close to the reactor vessel, the seismic isolators and/or damping devices may be exposed to gamma and neutron radiation, with a possible effect on their mechanical properties which would affect the response of the isolated equipment under earthquake shaking. The Department of Energy, as part of its Nuclear Energy University Program (NEUP), in collaboration with the Idaho National Laboratory (INL), is funding a project at the University at Buffalo (UB) to investigate the effect of gamma radiation on the mechanical properties of various seismic protective devices. (When isolating equipment, the seismic protective devices will be located outside the reactor vessel where the neutron exposure will be insignificant.

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DOE ART-GCR Program Overview

To provide Advanced Reactor Technologies Gas-Cooled Reactor Program: Overview of ART-GCR and Graphite program objectives, status, and activities. Also Identify research areas and outcomes that will benefit stakeholders and clients (HTGR designers, suppliers, regulators, DOE-NE, etc.), and to Identify remaining R&D gaps and future needs.

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The Meaning of Risk for Safety, Security, and Safeguards in the Design of Advanced Nuclear Reactors

What is the meaning of risk as it applies to the design of advanced reactors in the disciplines of safety, security, and safeguards? How can we find common terminology for the concept of risk and how can we find interfaces between these disciplines? These are important questions that should be explored in order that they may be applied in an integrated manner for the most effective and efficient design approaches. Eliminating or minimizing risks is a key design driver that motivates and informs the development of nuclear reactors. For safety, risk is well understood and applied in Probabilistic Risk Assessments. For security, the risk-based concepts of vulnerability assessments and vital areas are all considered in designing security systems. For safeguards, the concept of risk is not formally defined, as it relates to the design and operation of nuclear reactors. International nuclear safeguards seek to reduce the risk of proliferation in the nuclear fuel cycle and as such the concept of risk does exist. Therefore, the current understanding of the “3S’ approach, which seeks to find the interfaces and conflicts between safety, security, and safeguards requires a thorough understanding of the role that the reduction of risk plays in all three disciplines. The intersection of risk for safety and security is now being developed as there is a strong correlation between reactor design and operations and their vulnerability to sabotage. The intersection of risk for security and safeguards has to date chiefly been focused on the nuclear material control and accounting systems, which are relied on by both the operator (State) and the IAEA. This paper explores the concept of risk in each of the three disciplines, how they interact, potential conflicts and interfaces , how these might be addressed and leveraged, and a notional framework for how this could be achieved.

Kovacic, Donald N

Depletion Analysis of a Generic Fast Spectrum Molten Salt Reactor Supporting Material Control and Accounting (Rev.1)

Advanced reactors are of interest for a variety of use scenarios, and there are numerous advanced reactor designs being considered, which includes molten salt reactors (MSRs). Depending on the design, advanced reactors may have more extensive material control and accounting (MC&A) processes than current Light Water Reactor (LWR) designs. This project evaluated the use of Monte Carlo simulations for generating information that could guide the development of MC&A approaches for MSRs. In particular, the current capabilities of MCNP version 6.3 internally coupled with CINDER’90 were assessed for a fast spectrum liquid fueled MSR with online fission product removal and refueling. The fission product removal and refueling was performed in batches, and a Python wrapper was developed to control the simulations and update the fuel composition.

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Dynamic response of a freely rotating butterfly valve in the advanced test reactor − dynamic coefficients modeling

Here, in evaluating the water hammer issue pertaining to the primary-coolant-regulating butterfly valve in the Advanced Test Reactor, the dynamic fluid body interaction (DFBI) approach was implemented in the analysis covered in Part I. Although DFBI modeling accurately and simultaneously solved the dynamic motion of the valve’s disk along with the flow field of the surrounding fluid, it shed little light on the reason behind such motion. For Part II, the reacting torque of the fluid on the disk was decomposed into representations of the dynamic coefficients in terms of stiffness, damping, and added mass. These were evaluated via simulations with steady-state static (stiffness), constant angular speed (damping), and variable angular speed (added mass) disks. Substituting the dynamic coefficients into Newton’s second law enabled the response trajectories to be obtained. Stable (by average) and unstable equilibrium positions and thrust tendencies of the valve were determined based on the stiffness coefficient (or static torque), the response amplitude was dampened or enlarged by the damping coefficient (minorly affected by added mass), and the response frequency was altered by the damping and added mass coefficients. Although the dynamic coefficient approach renders slightly different trajectories, due to the averaging effect of the torque in comparison to the DFBI method, the overall trend of the response aligns with the DFBI simulation, thus confirming the conclusion in Part I that a fix to the current butterfly valve is necessary.

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Characterization of MC&A for the Molten Salt Fuel Cycle

Advanced reactor developers are exploring diverse reactor designs, including molten salt reactors (MSRs). These advanced reactors are considered for wider applications and a range of deployment locations, including supporting the integration of renewable energy sources in the grid. There are three main types of MSRs: (1) reactors in which the fuel salt freely circulates within the core; (2) reactors with the fuel salt contained within vented fuel tubes; and (3) reactors that use molten salt solely as a coolant, with the fuel in a separate, solid form. In this document, the term MSR refers specifically to the first two types, which use fuel salt—special nuclear material (enriched uranium, plutonium, and 233 U) in chloride or fluoride form mixed with chloride- or fluoride-based carrier salt in a peritectic mixture—as the primary medium for fission. The composition of fuel salt, both at startup and for makeup or refueling, varies depending on the MSR design and the chosen fuel cycle approach, which can be either once-through or closed. For MSRs, a variety of fuel cycle approaches (e.g., U, U–Pu, U–Pu–TRU, U–Th, U–Pu–Th) are being considered. Fuel in MSRs is much different than traditional solid fuel, including its preparation. The uniqueness warrants investigation into characterizing fuel preparation processes, known as fuel salt synthesis . This effort characterized major fuel preparation and synthesis processes, identifying temperature, equipment, and environmental requirements for uranium-, plutonium-, and thorium-based fuel preparation and synthesis. Because MSR fuel salt synthesis facilities handle special nuclear material in loose, bulk form, a material control and accounting plan will be required for licensing from the US Nuclear Regulatory Commission or under the US Department of Energy authorization. This effort serves as a foundation to investigate material control and accounting approaches for synthesis facilities, including determining measurement points and techniques. Because several MSR developers are planning demonstration facilities in the coming years, this effort will support stakeholders with preparing or reviewing material control and accounting plans for providing assurance that all special nuclear material is accounted for at fuel salt synthesis facilities. This report was produced for Materials Protection, Accounting, and Control Technologies (MPACT) program under the US Department of Energy (DOE), Office of Nuclear Energy, Nuclear Fuel Cycle and Supply Chain.

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