Engineering Papers⌕ Search

SEARCH · Engineering Papers

Results for “radionuclide”

Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

Quote a phrase for an exact phrase match. Source license links do not imply unrestricted reuse.

At least 1,243 records · Page 69

Local and exotic components of primitive meteorites, and their origin

The chemical and isotopic compositions of chondrites and their implications for chondrite origins are considered, reviewing the results of recent theoretical and experimental investigations. Numerical data are compiled in tables and graphs and discussed in detail. Consideration is given to the properties and classifications of chondrites; components of local origin in the matrix, chondrules, Ca-Al-rich inclusions, and carbon and organic matter; exotic components such as O-16-enriched dust, nucleosynthetic anomalies, and extinct radionuclides; and isotopic anomalies of volatiles such as C, N, and the noble gases. The implications of the chondrite data for the stony fraction of comet nuclei are briefly indicated.

Anders, E.↗

Thermal metamorphism

Most chondrites have experienced thermal metamorphism, resulting in changes in texture, mineralogy and possibly chemical composition. The physical conditions for metamorphism range from approximately 400 to 1000 C at low lithostatic pressure. Metamorphism may have resulted from decay of short-lived radionuclides, electromagnetic induction or accretion of hot materials. Several thermal models for chondrite parent bodies have been proposed. The least metamorphosed type-3 chondrites probably carry the most information about the early solar system, but even these have been affected to some degree by thermal processing.

Mcsween, Harry Y., Jr.↗

Iodine-xenon dating

The most readily and widely studied of the extinct radionuclides in meteorites is I-129, and there is an extensive data base for meteorite chronology based on this isotope, but also significant uncertainty about how to interpret many of the data. If the data are interpreted as a straightforward chronology, a time span is inferred for most meteorite classes that appears too long for the events being dated to have taken place in the nebula.

Swindle, T. D.↗

Age of Allan Hills 82102, a meteorite found inside the ice

The terrestrial age of a meteorite that was recovered from below the surface of Antarctic ice is reported, and it is argued that this represents a measurement of the age of the ice itself. The cosmogenic radionuclides Be-10, C-14, Al-26, Cl-36, and Mn-53 are measured in the meteorite and Be-10 and Cl-36 in the ice. A terrestrial age of 11,000 yr is obtained for the meteorite, which suggests that the snow accumulation area where it fell was only a few tens of km away.

Nishiizumi, K.↗

Cosmogenic nuclides in cometary materials: Implications for rate of mass loss and exposure history

As planned, the Rosetta mission will return to earth with a 10-kg core and a 1-kg surface sample from a comet. The selection of a comet with low current activity will maximize the chance of obtaining material altered as little as possible. Current temperature and level of activity, however, may not reliably indicate previous values. Fortunately, from measurements of the cosmogenic nuclide contents of cometary material, one may estimate a rate of mass loss in the past and perhaps learn something about the exposure history of the comet. Perhaps the simplest way to estimate the rate of mass loss is to compare the total inventories of several long-lived cosmogenic radionuclides with the values expected on the basis of model calculations. Although model calculations have become steadily more reliable, application to bodies with the composition of comets will require some extension beyond the normal range of use. In particular, the influence of light elements on the secondary particle cascade will need study, in part through laboratory irradiations of volatile-rich materials. In the analysis of cometary data, it would be valuable to test calculations against measurements of short-lived isotopes.

Herzog, G. F.↗

Evolution of carbonaceous chondrite parent bodies: Insights into cometary nuclei

It is thought that cometary samples will comprise the most primitive materials that are able to be sampled. Although parent body alteration of such samples would not necessarily detract from scientists' interest in them, the possibility exists that modification processes may have affected cometary nuclei. Inferences about the kinds of modifications that might be encountered can be drawn from data on the evolution of carbonaceous chondrite parent bodies. Observations suggest that, of all the classes of chondrites, these meteorites are most applicable to the study of comets. If the proportion of possible internal heat sources such as Al-26 in cometary materials are similar to those in chondrites, and if the time scale of comet accretion was fast enough to permit incorporation of live radionuclides, comets might have had early thermal histories somewhat like those of carbonaceous chondrite parent bodies.

Mcsween, Harry Y., Jr.↗

Measurements of long-lived cosmogenic nuclides in returned comet nucleus samples

Measurements of long lived cosmic ray produced radionuclides have given much information on the histories and rates of surface evolution for meteorites, the Moon and the Earth. These nuclides can be equally useful in studying cometary histories and post nebular processing of cometary surfaces. The concentration of these nuclides depends on the orbit of the comet (cosmic ray intensity changes with distance from the sun), the depth of the sampling site in the comet surface, and the rate of continuous evolution of the surface (erosion rate of surface materials). If the orbital parameters and the sampling depth are known, production rates of cosmogenic nuclides can be fairly accurately calculated by theoretical models normalized to measurement on lunar surface materials and meteoritic samples. Due to the continuous evaporation of surface materials, it is expected that the long lived radioactivities will be undersaturated. Accurate measurements of the degree of undersaturation in nuclides of different half-lives allows for the determination of the rate of surface material loss over the last few million years.

Nishiizumi, K.↗

Requirements and designs for Mars Rover RTGs

A typical Rover mission, its requirements, the environment it imposes on the radionuclide thermoelectric generator (RTG), and a design approach for making the RTG operable in such an environment are described. Specific RTG designs for various thermoelectric element alternatives are presented. The results of studies show that current multifoil-insulated GPHS (general-purpose heat source) RTG and Mod-RTG designs can be modified to operate in an environment with an external atmosphere (e.g., Mars). This can be done while the helium generated by the fuel's alpha decay is vented to the external atmosphere. The use of novel selective vents and high-capacity getters is not required. The Rover RTGs can be built from standard, proven GPHS modules and standard SiGe unicouples or SiGe/GaP multicouples, using demonstrated thermoelectric material performance parameters. Rover's 500-W power requirement can be satisfied with two 250-W or four 125-W RTGs, whose sizes are compatible with currently envisaged Rover designs. An auxiliary cooling loop (e.g., water and antifreeze) will be required to cool the RTG while it is within the Rover's aeroshell during launch and transit to Mars.

Schock, A.↗

Low Be-10 and Al-26 contents of ureilites - Production at meteoroid surfaces

The Be-10 contents of 22 ureilites and the Al-26 contents of 18 ureilites are reported. When corrected for exposure age, where known, and for composition, the results give production rate, P that are on average 20 percent lower than values typical of other meteorite classes. This depression of production rates, the weak correlations of both P26 and P10 with Ne-22/Ne-21 and the generally high He-3/Ne-21 and Ne-22/Ne-21 ratios in urelities all suggest that many of the samples occupied near-surface locations in their parent meteoroids. A reduced flux of cosmic rays does not by itself explain the elevated Ne-22/Ne-21 ratios and appears inconsistent with a proposed source for ureilites in the inner asteroid belt. Cosmogenic radionuclide data do not support the tentative pairing of ALHA 78019 with ALHa 78262 proposed on the basis of mineralogical similarities. The high Al-26 content of LEW 85440 may be the result of irradiation by solar cosmic rays.

Aylmer, D.↗

Proceedings of a Workshop on Cosmogenic Nuclide Production Rates

Abstracts of reports from the proceedings are presented. The presentations were divided into discussion topics. The following general topic areas were used: (1) measured cosmogenic noble gas and radionuclide production rates in meteorite and planetary surface samples; (2) cross-section measurements and simulation experiments; and (3) interpretation of sample studies and simulation experiments.

Englert, Peter A. J.↗

The pre- and post-accretion irradiation history of cometary ices

Comets Halley and Wilson exhibited similar 3.4 micron emission features at approx. 1 AU from the Sun. A simple model of thermal emission from organic grains fits the feature, provides optical depths in good agreement with spacecraft measurements, and explains the absence of longer-wavelength organic features as due to spectral heliocentric evolution (Chyba and Sagan, 1987). The model utilizes transmission spectra of organics synthesized in the laboratory by irradiation of candidate cometary ices; the authors have long noted that related gas-phase syntheses yield polycyclic aromatic hydrocarbons, among other organic residues (Sagan et al., 1967). The authors previously concluded (Chyba and Sagan, 1987) that Halley's loss of several meters' depth with each perihelion passage, combined with the good fit of the Halley 3.4 micron feature to that of comet Wilson (Allen and Wickramasinghe, 1987), argues for the primordial - but not necessarily interstellar - origin of cometary organics. The authors examine the relative importance to the formation of organics of the variety of radiation environments experienced by comets. They conclude that there is at present no compelling reason to choose any of three contributing mechanisms (pre-accretion UV, pre-accretion cosmic ray, and post-accretion radionuclide processing) as the most important.

Chyba, Christopher↗

Surface activation of Concorde by Be-7

Activation analysis of two airframe parts from Concorde aircraft has identified the presence of Be-7, a nuclide which was found by other investigators to have been collected on the forward edge of the Long Duration Exposure Facility (LDEF) structure. The results of the Concorde analysis indicate that this phenomenon is very much a surface effect, and that the areal densities of the Be-7 are comparable to those found for LDEF. The collection of Be-7 by the aircraft must be greater than in the case of LDEF (since the duration for which Concorde is accumulating the nuclide is shorter) and is of the order of 1.9 to 40 nuclei sq cm/s, depending upon assumptions made regarding the efficiency of the process which removes the radionuclide.

Truscott, P. R.↗

The Cl-36 in the stratosphere

Initial measurements of the cosmogenic radionuclide, Cl-36, in the lower stratosphere were made by accelerator mass spectrometry. Samples were obtained using the large volume LASL air sampling pods on a NASA WB-57F aircraft. Untreated (for collection of particulates only) and tetrabutyl ammonium hydroxide treated (for collection of particulates and HCl) IPC-1478 filters were flown on three flights in the lower stratosphere. Chlorine (Cl) and Cl compounds are important trace constituents for stratospheric chemistry, in particular with respect to O3 destruction. Stratospheric Cl chemistry has recently received increased attention with the observation of strong O3 depletion in the Antarctic winter vortex and in the weaker and more complex Arctic winter vortices. Cosmogenic (Cl-36) is produced by spallation reactions from Ar mainly in the stratosphere, and has had several applications as a geochemical tracer. The large amounts of Cl-36 introduced by nuclear weapon testing have been removed from the stratosphere by now, and measurements in the stratosphere to obtain cosmogenic production rates and concentration distributions is now possible. The use of cosmogenic Cl-36 as a tracer for stratospheric Cl chemistry and for stratospheric/tropospheric exchange processes is investigated. A first attempt to determine stratospheric and tropospheric production rates, the partitioning of Cl-36 among particulate and gaseous Cl compounds, and the respective inventories and removal rates is being made. Results from a flight at 13.7 km, 30-33 degrees N, 97-107 degrees W, and from a second flight at 17.7 km, 43-45-36 degrees N, 92-94 degrees W, for the untreated and treated filters respectively are presented.

Deck, Bruce↗

Profiles of alpha 13 C and alpha D in methane from the lower stratosphere

Methane is an important greenhouse gas of biogenic and anthropogenic origin for which global budgets are being constructed from a variety of data. One approach to the global methane budget is the use of the stable isotopes C-13 and D, and the radionuclide C-14 as tracers. The authors measured the isotopic composition of methane from various sources and in tropospheric air for a number of locations. Here, the authors report on the isotopic composition of methane from the lower stratosphere. Measurements of this concentration in the stratosphere can yield estimates for the kinetic isotope effects in the methane destruction reactions. These effects have to be known for quantitative isotopic methane budgets.

Wahlen, Martin↗

Medium and high-energy neutrino physics from a lunar base

Neutrino astronomy at high energy levels conducted from the moon is treated by considering 'particle astronomy' as a part of physics and the moon as a neutrino detector. The ability to observe the Galactic center is described by means of a 1-1000 TeV 'window' related to the drop in flux of atmospheric neutrinos from the earth. The long-baseline particle physics which are described in terms of a lunar observatory are found to be possible exclusively from a lunar station. The earth's neutrinos can be eliminated for the observations of astrophysical sources, and other potential areas of investigation include neutrino oscillation and the moon's interior. Neutrino exploration of the earth-moon and antineutrino radionuclide imaging are also considered. The moon is concluded to be a significantly more effective orbital platform for the study of neutrino physics than orbiting satellites developed on earth.

Wilson, Thomas L.↗

Analysis of surfaces from the LDEF A0114, phase 4

Progress made from 1 Mar. to 31 Aug. 1991 is presented. The work concentrated on profilometry measurements of eroded and corroded sample surfaces, optical transmission measurements, analysis of the pinhole camera, and x-ray photoelectron spectroscopic (XPS) analysis of some samples. The following papers are presented: (1) observation of Be-7 on the surface of the Long Duration Exposure Facility (LDEF) Spacecraft; (2) measurement of the passive attitude control performance of a recovered spacecraft; (3) effects on LDEF exposed copper flim and bulk; (4) measurements of erosion characteristics for metal and polymer surfaces using profilometry; (5) the interactions of atmospheric cosmogenic radionuclides with spacecraft surfaces; (6) pinhole cameras as sensors for atomic oxygen in orbit; and (7) interaction of atomic oxygen with solid surfaces in low earth orbit- results from LDEF experiment A0114.

Gregory, John C.↗

Surface activation of Concorde by Be-7

Activation analysis of two airframe components from the Concorde aircraft has identified the presence of Be-7, a nuclide found by other investigators that was deposited on the forward edge of the Long Duration Exposure Facility (LDEF) structure. The results of the Concorde analysis indicate that this phenomenon is very much a surface effect, and that the areal densities of the Be-7 are comparable to those found for LDEF. The collection of Be-7 by the aircraft must be greater than in the case of LDEF (since duration for which Concorde is accumulating the nuclide is shorter) and is of the order of 1.2 to 41 nuclei/sq cm(-)s(exp -1) depending upon assumptions made regarding the altitude at which collection becomes appreciable, and the efficiency of the process which removes the radionuclide.

Truscott, P. R.↗

How Mars lost its atmosphere

There is a widespread suspicion that Mars thin atmosphere is in some way attributable to the planet's size. Another possibility is that the atmosphere was never degassed or outgassed in the first place. I prefer escape. Hydrodynamic escape (vigorous thermal escape) and impact erosion (expulsion of atmosphere by impacts) are two processes that should have been operative early. Although in principle hydrodynamic escape could have shrunk Mars atmosphere a hundredfold while leaving the composition of the remnant atmosphere nearly unaltered, very high escape fluxes are required. The implicated escape mechanism must have been efficient, nearly non-fractionating, and vastly more potent for Mars than for Earth or Venus. Impact erosion is an appealing candidate. Noble gases are the obvious first test. Noble gases are the most volatile elements and so are the most likely to have been affected by impact erosion and the easiest to address quantitatively. Xenon in particular imposes three constraints on how Mars lost its atmosphere: (1) the very low abundance of nonradiogenic Xe abundance of nonradiogenic Xe compared to Earth, Venus, and likely meteoritic sources; (2) its nonradiogenic isotopes distinct from likely meteoritic sources; and (3) the relatively high absolute abundance of radiogenic daughter of the extinct radionuclide I-129 (half-life 17 Myr). In impact erosion, the first two become constraints on the composition, mass distribution, and orbital elements of the impactors. The third requires that Mars lost its nonradiogenic Xe early, probably before it was 100 Myr old. Impact erosion can explain Mars by any of three stories. (1) Mars in unlikely. In a sort of planetary brinkmanship, impact erosion almost removed the entire atmosphere but was arrested just in time. (2) Martian noble gases are cometary and cometary Xe is as isotopically mass fractionated as Martian and terrestrial Xe. This is most easily accomplished if a relatively thick geochemically controlled CO2 atmosphere protected trace atmophiles against escape. (3) Mars was indeed stripped of its early atmosphere but a small remnant was safely stored in the regolith, later released as a byproduct of water mobilization.

Zahnle, Kevin↗