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At least 1,225 records · Page 68

Stable dielectric charge distributions from field enhancement of secondary mission

The emission of secondary electrons from dielectrics subject to numerous effects of electric field which are experimentally difficult to control is discussed. Measurements are reported using pulse techniques such that local fields do not build to significant levels, but measurements with fields present are also of interest. A specific series of measurements under controlled conditions are described and their implications in terms of fields, magnitude and angle, near the dielectric surface were examined. The measurements were made for a charged fluorinated-ethylene-propylene surface near a grounded aluminum half-round resting on the surface. The geometry produced a stable surface-charge gradient being controlled by a strongly enhanced secondary emission for which a model is constructed. Observations of surface flashovers under various conditions confirm the predictions of some scaling exercises.

Robinson, J. W.↗

Modeling the Gas Flux From a Jupiter-Class Comet Nucleus

Sublimation and gas flux of volatile ices from porous bodies in the Solar System are important, observable phenomena. Surface erosion and dust build-up on a comet nucleus and coma formation are processes attributable to the flux of sublimating gases. Our computer simulations focus on the gas flux from volatile, icy components in the surface layer of a porous, Jupiter-class comet in order to investigate the relationship of the observed relative molecular abundances in the coma with those in then nucleus. We compare results from one-dimensional and two-dimensional models.

Jupiter Comet↗

Transient evolution of basal drag during glacier slip

Glacier slip is usually described using steady-state sliding laws that relate drag, slip velocity and effective pressure, but where subglacial conditions vary rapidly transient effects may influence slip dynamics. Here we use results from a set of laboratory experiments to examine the transient response of glacier slip over a hard bed to velocity perturbations. The drag and cavity evolution from lab experiments are used to parameterize a rate-and-state drag model that is applied to observations of surface velocity and ice-bed separation from the Greenland ice sheet. The drag model successfully predicts observed lags between changes in ice-bed separation and sliding speed. These lags result from the time (or displacement) required for cavities to evolve from one steady-state condition to another. In comparing drag estimates resulting from applying rate-and-state and steady-state slip laws to transient data, we find the peaks in drag are out of phase. This suggests that in locations where subglacial conditions vary on timescales shorter than those needed for cavity adjustment transient slip processes control basal drag.

Glacier↗

Inland and Near Shore Water Profiles Derived from the High Altitude Multiple Altimeter Beam Experimental Lidar (MABEL)

The Advanced Topographic Laser Altimeter System (ATLAS) on the Ice, Cloud, and Land Elevation Satellite (ICESat-2) mission is a six beam, low energy, high repetition rate, 532 nm laser transmitter with photon counting detectors. Although designed primarily for detecting height changes in icecaps, sea ice and vegetation, the polar-orbital satellite will observe global surface water during its designed three year life span, including inland water bodies, coasts, and open oceans. In preparation for the mission, an ICESat-2 prototype or the Multiple Altimeter Beam Experimental Lidar (MABEL), was built and flown on high altitude aircraft experiments over a range of inland and near-shore targets. The purpose was to test the ATLAS concept and to provide a database for developing an algorithm that detects along track surface water height and light penetration under a range of atmospheric and water conditions. The current analysis examines the datasets of three MABEL transects observed from 20 km above ground of coastal and inland waters conducted in 2012 and 2013. Transects ranged from about 2 to 12 km in length and included the middle Chesapeake Bay, the near shore Atlantic coast at Virginia Beach, and Lake Mead. Results indicate MABEL's high capability for retrieving surface water height statistics with a mean height precision of approximately 5-7 cm per 100m segment length. Profiles of attenuated subsurface backscatter, characterized using a Signal to Background Ratio written in Log10 base, or LSBR0, were observed over a range of 1.3 to 9.3 meters depending on water clarity and atmospheric background. Results indicate that observable penetration depth, although primarily dependent on water properties, was greatest when solar background rate was low. Near shore bottom reflectance was detected only at the Lake Mead site down to maximum of 10 m under a clear night sky and low turbidity of approximately 1.6 Nephelometric Turbidity Units (NTU). The overall results suggest that the feasibility of retrieving operational surface water height statistics from space-based photon counting systems such as ATLAS is very high for resolutions down to about 100m, even in partly cloudy conditions. The capability to observe subsurface backscatter profiles is achievable but requires much longer transects of several hundreds of meters.

Topographic↗

Distribution and Variation of the Surface Sensible Heat Flux Over the Central and Eastern Tibetan Plateau: Comparison of Station Observations and Multireanalysis Products

Surface sensible heat fluxes (SH) over Tibetan Plateau (TP) dictate the seasonal conversion, onset and maintenance of the Asian monsoon. Spatiotemproal variability in SH over central and eastern TP (CETP) from reanalysis products (i.e., JRA55, ERA-Interim, NCEP1, and NCEP2) and derived using bulk transfer approximations applied to observations is characterized for all seasons during 1980–2015 and is diagnosed in the context of two important drivers of variability: wind speed and land-air temperature difference (Tg-Ta). In the climatological mean, SH from observations increases from east to west and exhibits obvious seasonality with highest value in spring and lowest in winter. Declines in SH prior to 2000 as manifest in the observations appears to have resulted from changes in wind speeds, and the subsequent recovery is attributable to increases in both wind speeds and air-surface temperature gradients. The intercomparison shows that ERA-Interim exhibits greatest accord with observations in terms of the climatological distribution and seasonality, and all reanalyses exhibit some aspects of the temporal variability and long-term trends as manifest in the observations. However, the root causes of the long-term variability in SH as manifest in the reanalysis products are not consistent with inferences derived from the observations.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

An Integrative Model for Soil Biogeochemistry and Methane Processes: I. Model Structure and Sensitivity Analysis

Abstract Environmental changes are anticipated to generate substantial impacts on carbon cycling in peatlands, affecting terrestrial‐climate feedbacks. Understanding how peatland methane (CH 4 ) fluxes respond to these changing environments is critical for predicting the magnitude of feedbacks from peatlands to global climate change. To improve predictions of CH 4 fluxes in response to changes such as elevated atmospheric CO 2 concentrations and warming, it is essential for Earth system models to include increased realism to simulate CH 4 processes in a more mechanistic way. To address this need, we incorporated a new microbial‐functional group‐based CH 4 module into the Energy Exascale Earth System land model (ELM) and tested it with multiple observational data sets at an ombrotrophic peatland bog in northern Minnesota. The model is able to simulate observed land surface CH 4 fluxes and fundamental mechanisms contributing to these throughout the soil profile. The model reproduced the observed vertical distributions of dissolved organic carbon and acetate concentrations. The seasonality of acetoclastic and hydrogenotrophic methanogenesis—two key processes for CH 4 production—and CH 4 concentration along the soil profile were accurately simulated. Meanwhile, the model estimated that plant‐mediated transport, diffusion, and ebullition contributed to ∼23.5%, 15.0%, and 61.5% of CH 4 transport, respectively. A parameter sensitivity analysis showed that CH 4 substrate and CH 4 production were the most critical mechanisms regulating temporal patterns of surface CH 4 fluxes both under ambient conditions and warming treatments. This knowledge will be used to improve Earth system model predictions of these high‐carbon ecosystems from plot to regional scales.

58 GEOSCIENCES↗

Climatological perspectives, oceanographic and meteorological, on variability in the subtropical convergence zone in the northwestern Atlantic

The large-scale climatological environment of the Frontal Air-Sea Interaction Experiment (FASINEX) is described, with emphasis on the largest scales. Both long-term and annual sea surface temperature (SST) variability is discussed; a climatology of the west-central North Atlantic, derived from various sets of data obtained during the intensive phases of January-March, is presented, and the meteorological and oceanographic context for FASINEX is thus established. Surface marine observations and SST variability are discussed, and the marine meteorology of the FASINEX area is examined in terms of the surface pressure and winds, the sea-air temperature difference, and the cloud cover. Near 28 deg N in February is found to be a favorable time and place to observe large mean temperature gradients and downward Ekman pumping. The large-scale processes that set up the favorable environment for frontal activity are not limited to the winter months.

Hanson, Howard P.↗

Snow Grain Size Retrieval over the Polar Ice Sheets with the Ice, Cloud and Land Elevation Satellite (ICESat) Observations

Snow grain size is an important parameter for cryosphere studies. As a proof of concept, this paper presents an approach to retrieve this parameter over Greenland, East and West Antarctica ice sheets from surface reflectances observed with the Geoscience Laser Altimeter System (GLAS) onboard the Ice, Cloud, and land Elevation Satellite (ICESat) at 1064 nanometers. Spaceborne lidar observations overcome many of the disadvantages in passive remote sensing, including difficulties in cloud screening and low sun angle limitations; hence tend to provide more accurate and stable retrievals. Results from the GLAS L2A campaign, which began on 25 September and lasted until 19 November, 2003, show that the mode of the grain size distribution over Greenland is the largest (approximately 300 microns) among the three, West Antarctica is the second (220 microns) and East Antarctica is the smallest (190 microns). Snow grain sizes are larger over the coastal regions compared to inland the ice sheets. These results are consistent with previous studies. Applying the broadband snow surface albedo parameterization scheme developed by Garder and Sharp (2010) to the retrieved snow grain size, ice sheet surface albedo is also derived. In the future, more accurate retrievals can be achieved with multiple wavelengths lidar observations.

ice↗

Construction of a model of the Venus surface and its use in processing radar observations

An algorithm is described for constructing the model of the Venus surface as an expansion in spherical functions. The relief expansion coefficients were obtained up to the coefficient S sub 99. The surface picture representation is given according to this expansion. The surface model constructed was used for processing radar observations. The use of the surface model allows improved agreement between the design and measured values of radar ranges.

Borodin, V. A.↗

Inland and Near-Shore Water Profiles Derived from the High-Altitude Multiple Altimeter Beam Experimental Lidar (MABEL)

The Advanced Topographic Laser Altimeter System (ATLAS) on the Ice, Cloud, and Land Elevation Satellite (ICESat-2) mission is a six beam, low energy, high repetition rate, 532-nanometer laser transmitter with photon counting detectors. Although designed primarily for detecting height changes in ice caps, sea ice, and vegetation, the polar-orbiting satellite will observe global surface water during its designed three-year life span, including inland waterbodies, coasts, and open oceans. In preparation for the mission, an ICESat-2 prototype, the Multiple Altimeter Beam Experimental Lidar (MABEL), was built and flown on high-altitude aircraft experiments over a range of inland and near-shore targets. The purpose was to test the ATLAS concept and to provide a database for developing an algorithm that detects along track surface water height and light penetration under a range of atmospheric and water conditions. The current analysis examines the data sets of three MABEL transects observed from 20 kilometers above ground of coastal and inland waters conducted in 2012 and 2013. Transects ranged from about 2 to 12 kilometers in length and included the middle Chesapeake Bay, the near-shore Atlantic coast at Virginia Beach, and Lake Mead. Results indicate MABEL's high capability for retrieving surface water height statistics with a mean height precision ofapproximately 5-7 centimeters per 100-meter segment length. Profiles of attenuated subsurface backscatter, characterized using a Signal to Background Ratio written in Log10 base, or LSBR (sub 0), were observed over a range of 1.3 to 9.3 meters, depending on water clarity and atmospheric background. Results indicate that observable penetration depth, although primarily dependent on water properties, was greatest when the solar background rate was low. Near-shore bottom reflectance was detected only at the Lake Mead site down to a maximum of 10 meters under a clear night sky and low turbidity of approximately 1.6 Nephelometric Turbidity Units (NTU). The overall results suggest that the feasibility of retrieving operational surface water height statistics from space-based photon counting systems such as ATLAS is very high for resolutions down to about 100 meters, even in partly cloudy conditions. The capability to observe subsurface backscatterprofiles is achievable but requires much longer transects of several hundreds of meters.

inland↗

Crystal orientation effects on helium ion depth distributions and adatom formation processes in plasma-facing tungsten

We present atomistic simulations that show the effect of surface orientation on helium depth distributions and surface feature formation as a result of low-energy helium plasma exposure. We find a pronounced effect of surface orientation on the initial depth of implanted helium ions, as well as a difference in reflection and helium retention across different surface orientations. Our results indicate that single helium interstitials are sufficient to induce the formation of adatom/substitutional helium pairs under certain highly corrugated tungsten surfaces, such as (1 1 1)-orientations, leading to the formation of a relatively concentrated layer of immobile helium immediately below the surface. The energies involved for helium-induced adatom formation on (1 1 1) and (2 1 1) surfaces are exoergic for even a single adatom very close to the surface, while (0 0 1) and (0 1 1) surfaces require two or even three helium atoms in a cluster before a substitutional helium cluster and adatom will form with reasonable probability. This phenomenon results in much higher initial helium retention during helium plasma exposure to (1 1 1) and (2 1 1) tungsten surfaces than is observed for (0 0 1) or (0 1 1) surfaces and is much higher than can be attributed to differences in the initial depth distributions alone. The layer thus formed may serve as nucleation sites for further bubble formation and growth or as a source of material embrittlement or fatigue, which may have implications for the formation of tungsten “fuzz” in plasma-facing divertors for magnetic-confinement nuclear fusion reactors and/or the lifetime of such divertors.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Epitaxial ZnO/LiNbO{sub 3}/ZnO stacked layer waveguide for application to thin-film Pockels sensors

We produced slab waveguides consisting of a LiNbO{sub 3} (LN) core layer that was sandwiched with Al-doped ZnO cladding layers. The ZnO/LN/ZnO stacked layers were grown on sapphire C-planes by electron cyclotron resonance (ECR) plasma sputtering and were subjected to structural, electrical, and optical characterizations. X-ray diffraction confirmed that the ZnO and LN layers were epitaxial without containing misoriented crystallites. The presence of 60°-rotational variants of ZnO and LN crystalline domains were identified from X-ray pole figures. Cross-sectional transmission electron microscopy images revealed a c-axis orientated columnar texture for LN crystals, which ensured operation as electro-optic sensors based on optical anisotropy along longitudinal and transversal directions. The interfacial roughness between the LN core and ZnO bottom layers as well as that between the ZnO top and the LN core layers was less than 20 nm, which agreed with surface images observed with atomic force microscopy. Outgrowth of triangular LN crystalline domains produced large roughness at the LN film surface. The RMS roughness of the LN film surface was twice that of the same structure grown on sapphire A-planes. Vertical optical transmittance of the stacked films was higher than 85% within the visible and infrared wavelength range. Following the approach adopted by Teng and Man [Appl. Phys. Lett. 56, 1734 (1990)], ac Pockels coefficients of r{sub 33} = 24-28 pm/V were derived for c-axis oriented LN films grown on low-resistive Si substrates. Light propagation within a ZnO/LN/ZnO slab waveguide as well as within a ZnO single layer waveguide was confirmed. The birefringence of these waveguides was 0.11 for the former and 0.05 for the latter.

36 MATERIALS SCIENCE↗

Magnetic dichroism in the Kondo insulator SmB 6

Samarium hexaboride (${\mathrm{SmB}}_{6}$) is a purported topological Kondo insulator, with theory predicting that the experimentally observed metallic surface states manifest from a topologically nontrivial insulating bulk band structure. The insulating bulk itself is driven by strong correlations, and both bulk and surface are known to host compelling magnetic and electronic phenomena. We employed here x-ray absorption spectroscopy and x-ray magnetic circular dichroism at the Sm ${M}_{4,5}$ edges to probe the surface and bulk magnetic properties of ${\mathrm{Sm}}^{2+}$ and ${\mathrm{Sm}}^{3+}$ within ${\mathrm{SmB}}_{6}$. We observed an unexpected antialignment to the applied field of the ${\mathrm{Sm}}^{3+}$ magnetic dipole moment below $T=75$ K and of the total orbital moment of samarium below 30 K. The total bulk magnetization at 2 K is, however, positive and driven by ${\mathrm{Sm}}^{2+}$ Van Vleck susceptibility as well as 1% paramagnetic impurities with ${{\mu}}_{\mathrm{eff}}=5.2(1){{\mu}}_{\mathrm{B}}$. This indicates the diamagneticlike ${\mathrm{Sm}}^{3+}$ magnetism is only a portion of the net magnetization, partially offsetting the response of paramagnetic impurities known within the bulk.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

In-situ measurement of the rate of U-235 fission induced by lunar neutrons

The depth profile of the neutron-induced fission rate of U-235 was directly measured to a depth of 350 g/sq cm by the Apollo 17 Lunar Neutron Probe Experiment. The fission rate rises sharply from the surface to a broad maximum from 110 to 160 g/sq cm and drops off at greater depths. The shape of the theoretical depth profile of Lingenfelter et al (1972) fits the measured capture rates well at all depths. The absolute magnitude of the experimental fission rates are (11 plus or minus 17)% lower than those calculated theoretically. The excellent agreement between theory and experiment implies that conclusions drawn previously by interpreting lunar sample data with the theoretical capture rates will not require revision. In particular, lunar surface processes, rather than uncertainties in the capture rates, are required to explain the relatively low neutron fluences observed for surface soil samples compared to the fluences expected for a uniformly mixed regolith.

Woolum, D. S.↗

Periodic striations on beryllium and tungsten surfaces by indirect femtosecond laser irradiation

Femtosecond laser pulses with λ = 800 nm were focused in air at one atmosphere and in deuterium (D) at low pressure. Submicron periodic structures were observed on surfaces made of Be, W and a mixture of Be-W immersed in these gases and placed nearly parallel with the laser beam, at 300 μm from the focal spot. In air, no structures were observed on Be. For the Be-W mixture, the periodic structures were uniform and parallel when formed in D but irregular in air. In this last case the striations were organized into small patches of 1 to 2 μm in size.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Correlating Nb-SRF Surface Processing with Evolution of Surface Electronic States

The few nanometers of the surface exposed to RF field plays a major role in defining the RF performance of superconducting cavities. Over the past two decades, several pioneering surface treatment and processing methods have emerged, enabling remarkable improvements in cavity performance by simultaneously achieving high Q with increasing Eacc. These processing methods include: thermal treatment under ultra-high vacuum (UHV) conditions across lo¬¬¬¬¬¬¬w-, mid-, and high-temperature ranges and high temperature treatments under controlled N2 atmosphere. These processes also produce distinct surface oxide configurations with different valence states, thicknesses, and uniformity, as well as different oxygen concentration profiles in bulk Nb. In this work, we are trying to understand how do surface-processing methods and the resulting oxide/oxygen profiles affect the electronic structure of surface and the mechanism of superconductivity? With the help of Fermilab’s in-house X-ray photoemission facility and, in collaboration with the synchrotron-based angle-resolved photoemission (ARPES) facility at Argonne National Laboratory, we are investigating how the valence band structure and density of states (DoS) near the Fermi level modify with different surface treatments. Our observations show that different surface-processing methods lead to distinct evolutions of the valence-band states near the Fermi level during the superconducting transition. This behavior suggests variations in Nb-O orbital hybridizations and points towards the possibility of different underlying mechanisms of superconductivity governed by the surface chemistry and oxide configuration. We also correlate these distinct superconducting mechanisms with RF cavity performance, specifically focusing on measured surface resistance, the nature of the Q-slope, and quench fields observed in SRF measurements. These results will enable us to identify the potential limiting factors and relevant controllable parameters that can be further optimized to improve the performance of SRF cavities.

Tripathi, Malvika [Fermilab]↗

Description and evaluation of tropospheric chemistry and aerosols in the Community Earth System Model (CESM1.2)

The Community Atmosphere Model (CAM), version 5, is now coupled to extensive tropospheric and stratospheric chemistry, called CAM5-chem, and is available in addition to CAM4-chem in the Community Earth System Model (CESM) version 1.2. The main focus of this paper is to compare the performance of configurations with internally derived "free running" (FR) meteorology and "specified dynamics" (SD) against observations from surface, aircraft, and satellite, as well as understand the origin of the identified differences. We focus on the representation of aerosols and chemistry. All model configurations reproduce tropospheric ozone for most regions based on in situ and satellite observations. However, shortcomings exist in the representation of ozone precursors and aerosols. Tropospheric ozone in all model configurations agrees for the most part with ozonesondes and satellite observations in the tropics and the Northern Hemisphere within the variability of the observations. Southern hemispheric tropospheric ozone is consistently underestimated by up to 25%. Differences in convection and stratosphere to troposphere exchange processes are mostly responsible for differences in ozone in the different model configurations. Carbon monoxide (CO) and other volatile organic compounds are largely underestimated in Northern Hemisphere mid-latitudes based on satellite and aircraft observations. Nitrogen oxides (NO x ) are biased low in the free tropical troposphere, whereas peroxyacetyl nitrate (PAN) is overestimated in particular in high northern latitudes. The present-day methane lifetime estimates are compared among the different model configurations. These range between 7.8 years in the SD configuration of CAM5-chem and 8.8 years in the FR configuration of CAM4-chem and are therefore underestimated compared to observational estimations. We find that differences in tropospheric aerosol surface area between CAM4 and CAM5 play an important role in controlling the burden of the tropical tropospheric hydroxyl radical (OH), which causes differences in tropical methane lifetime of about half a year between CAM4-chem and CAM5-chem. In addition, different distributions of NO x from lightning explain about half of the difference between SD and FR model versions in both CAM4-chem and CAM5-chem. Remaining differences in the tropical OH burden are due to enhanced tropical ozone burden in SD configurations compared to the FR versions, which are not only caused by differences in chemical production or loss but also by transport and mixing. For future studies, we recommend the use of CAM5-chem configurations, due to improved aerosol description and inclusion of aerosol–cloud interactions. However, smaller tropospheric surface area density in the current version of CAM5-chem compared to CAM4-chem results in larger oxidizing capacity in the troposphere and therefore a shorter methane lifetime.

54 ENVIRONMENTAL SCIENCES↗

Triton's surface-atmosphere energy balance

A model encompassing the turbulent transfer of sensible heat as well as insolation, reradiation, and latent heat transport is presently used to investigate the energetics of the surface-atmosphere system of Triton. Under the assumption of a physically plausible range of heat transfer coefficients, the atmospheric temperature 1 km above the surface is found to be 1-3 K hotter than the Triton surface. The observed N2 frosts must have an emissivity lower than unity in order to match a frost temperature at the surface of about 38 K.

Stansberry, John A.↗