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DOE OSTI2025

Mock-Up Waveguide Loop Development toward a Half-Meter Scale Traveling-Wave SRF Cavity

Mock-up waveguide loop development toward a half-meter scale traveling-wave SRF cavity ABSTRACT = Traveling-Wave (TW) technology can push the accelerator field gradient of niobium SRF cavity to 70MV/m or higher beyond the fundamental limit of 50~60MV/m in Standing-Wave regime. The success of TW resonance excitation in a proof-of-principle 3-cell SRF cavity in 2K liquid helium encouraged to advance TW technologies necessary more for future accelerator-scale one. Fermilab has proposed a preliminary RF design of a half-meter scale TW cavity by considering the physical dimensions of existing SRF facilities and the lessons learned from the 3-cell. It consists of a 7-cell structure and a power feedback waveguide (WG) loop with new TW excitation and control schemes such as, double directional coupler and two WG tuners. Mock-up waveguide loop development was launched under Fermilab LDRD program to demonstrate those new RF schemes at a room temperature. Fabrication drawings of a mock-up loop were completed. More details and plans of the development will be presented.

Furuta, Fumio [Fermilab]↗

DOE OSTI2025

Scaling Up: Demonstrating Risk Reduction and Cost Compression for Commercial Heat Pump Water Heaters (CRADA 625) (Final Report)

This report is a final deliverable for project 81966: Scaling Up: Demonstrating Risk Reduction and Cost Compression for Commercial Heat Pump Water Heaters (CRADA 625) Commercial heat pump water heater (CHPWH) systems can significantly improve the energy efficiency of service water heating (SWH), aka domestic hot water (DHW), in commercial and multifamily buildings but have not yet achieved widespread adoption due to pricing, complexity, and perceived risk factors. The goal of this project – Scaling Up: Demonstrating Risk Reduction and Cost Compression for Commercial HPWHs (Scaling Up) – was to demonstrate and validate a holistic systems approach for CHPWHs that de-risks the technology, creating a reliable, cost-effective, and repeatable approach to CHPWH deployment.

32 ENERGY CONSERVATION, CONSUMPTION, AND UTILIZATI↗

DOE OSTI2025

Development of a bench-scale dissolution concept for the direct extraction of nuclear fuel

Current used nuclear fuel reprocessing efforts utilize a hydrometallurgical approach in which the UNF is dissolved in hot nitric acid followed by solvent extraction into an organic solvent to harvest target nuclides. Previous studies have shown that the dissolution and loading process could be combined into a single organic dissolution/extraction step, producing loaded organic in a single step process. This single step process also includes the advantage of selectively targeting key nuclides in the dissolution while leaving undesirable constituents as part of the undissolved solids. This process is referred to hereafter as direct extraction. Ongoing research from multiple national labs has proven the effectiveness of this technique at research scale. Therefore, potential methods to implement direct extraction at both bench and industrial scale have been developed. The key features of potential dissolver system designs were identified via the team at Pacific Northwest National Laboratory and several designs based on industrial counterparts were assessed for feasibility. This report summarizes the advantages and disadvantages of multiple methods, concluding with a path forward to create multiple unique dissolver designs. The first design will be a single stage recirculating eductor mixer. The second design recommendation is a stator rotor static mixing flow loop design. Each dissolver could be utilized separately, simultaneously, or in series to answer questions surrounding reaction kinetics including residence time, provide a proof of concept for targeted extractions of specific nuclides, and inform needs for industrial scale implementation

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

DOE OSTI2026

Development of large-scale, 3D Printed high temperature ceramic material

Through this collaborative effort, a new 3D printing platform for ceramics called laser-induced slip casting (LIS) was explored and developed for improving the processing and manufacture of silicon carbide (SiC), a high temperature ceramic material. This method prints layers of ceramic slips/slurries with subsequent selective-laser heating to dry each layer to build a 3D structure. The completed and dried part is then sintered. This manufacturing process is inherently lower cost than alternative ceramic printing methods such as binder jet technology or stereolithography when it comes to the feedstock material but is more expensive than robocasting or direct ink writing. However, it has the potential to make more controlled parts with less defects compared to robocasting. The largest cost is the heating source for the printer. With this technique, there is potential to make large ceramic parts in a near-net shape. Further, there is no known commercial manufacturing of 3D printed ceramics that creates a large range of different high-density ceramics at large scale. The goals and outcomes for the development of the new printing technology were: 1) assessing the technology with alumina by characterizing coupons, 2) printing and sintering of silicon carbide (SiC), and 3) characterization and properties testing of materials printed and a scale-up of SiC part(s). Through this collaborative project, it was sought to provide the best solution to achieving highly dense and near-net shaped ceramic parts at large scale and reduced cost. The goal was to produce high density sintered materials for applications in defense, energy generating systems, armor, and wear parts using 3D printing methods. Variables including powder particle sizes, dispersant molecular weights (MWs), binders, printing parameters, and post processing were explored as well as the characterization of the physical properties (add specifics here).

36 MATERIALS SCIENCE↗

DOE OSTI2025

Scale up production of carbon fibers from petroleum mesophase pitch

This work investigates the scale-up of pitch precursors for the carbon fiber market using mesophase pitch formulated and produced by Advanced Carbon Products Technologies’ (ACPT’s) patented mesophase pitch processing technology. Through use of its patented process, ACPT developed strategic materials by converting petroleum-based pitch into a high-value, low-cost, carbon-rich feedstock for carbon fiber and other materials critical to our national security. The team successfully developed processing criteria for the tailored mesophase pitch material that can be processed further into precursor and carbon fiber. Processability of the mesophase pitch into precursor and carbon fiber was demonstrated at scale. The resulting materials sequester the carbon that would otherwise be burned and released into the atmosphere, making this an environmentally friendly way to produce these materials in the United States.Pitch-based carbon fibers offer a promising pathway toward cost-effective, high-performance materials for structural and high-modulus composite applications; however, adoption has been limited by challenges in precursor processability and scale-up. In this work, tailored isotropic and mesophase petroleum-derived pitch materials were developed and evaluated for precursor and carbon fiber production through a collaborative effort between Oak Ridge National Laboratory (ORNL) and ACPT. Processing conditions were established at ORNL’s Carbon Fiber Technology Facility to enable stable melt-blowing of pitch-based precursors under continuous operation. Mesophase pitch precursor fibers were produced following oxidation and carbonization, corresponding to a diameter shrinkage of approximately 12%–13% and an estimated mass yield of about 75%–80%. Continuous melt-blowing steady-state operation was demonstrated over time, indicating robust process stability. Melt-blowing was achieved at throughput rates of approximately 20 lb/h⁻¹, validating the commercial viability of petroleum-derived pitch feedstocks for fiber production. Further studies are required to tailor carbon fiber microstructure and properties for specific composite applications.

99 GENERAL AND MISCELLANEOUS↗

DOE OSTI2022

Plasma Imaging, LOcal Measurement, and Tomographic Experiment (PILOT): A Mission Concept for Transformational Multi-Scale Observations of Mass and Energy Flow Dynamics in Earth’s Magnetosphere

We currently do not understand the fundamental physical processes that govern mass and energy flow through the Earth’s magnetosphere. Knowledge of these processes is critical to understanding the mass loss rate of Earth’s atmosphere, as well as for determining the role that a planetary magnetic field plays in atmospheric retention, and therefore habitability, for Earth-like planets beyond the solar system. Mass and energy flow processes are challenging to determine at Earth in part because Earth’s planetary magnetic field creates a complex “system of systems” composed of interdependent plasma populations and overlapping spatial regions that perpetually exchange mass and energy across a broad range of temporal and spatial scales. Further, the primary mass carrier in the magnetosphere is cold plasma (as cold as ~0.1 eV), which is invisible to many space-borne instruments that operate in the inner magnetosphere. The Plasma Imaging LOcal and Tomographic experiment (PILOT) mission concept, described here, provides the transformational multi-scale observations required to answer fundamental open questions about mass and energy flow dynamics in the Earth’s magnetosphere. PILOT uses a constellation of spacecraft to make radio tomographic, remote sensing, and in-situ measurements simultaneously, fully capturing cold plasma mass dynamics and its impact on magnetospheric systems over an unprecedented range of spatial and temporal scales. This article details the scientific motivation for the PILOT mission concept as well as a potential mission implementation.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2020

Multi-Scale Simulation of Wind Farm Performance during a Frontal Passage

Predicting the response of wind farms to changing flow conditions is necessary for optimal design and operation. Here in this work, simulation and analysis of a frontal passage through a utility scale wind farm is achieved for the first time using a seamless multi-scale modeling approach. A generalized actuator disk (GAD) wind turbine model is used to represent turbine–flow interaction, and results are compared to novel radar observations during the frontal passage. The Weather Research and Forecasting (WRF) model is employed with a nested grid setup that allows for coupling between multi-scale atmospheric conditions and turbine response. Starting with mesoscale forcing, the atmosphere is dynamically downscaled to the region of interest, where the interaction between turbulent flows and individual wind turbines is simulated with 10 m grid spacing. Several improvements are made to the GAD model to mimic realistic turbine operation, including a yawing capability and a power output calculation. Ultimately, the model is able to capture both the dynamics of the frontal passage and the turbine response; predictions show good agreement with observed background velocity, turbine wake structure, and power output after accounting for a phase shift in the mesoscale forcing. This study demonstrates the utility of the WRF-GAD model framework for simulating wind farm performance under complex atmospheric conditions.

17 WIND ENERGY↗

DOE OSTI2021

Mitigation of Gaseous Emissions from Stored Swine Manure with Biochar: Effect of Dose and Reapplication on a Pilot-Scale

Rural communities are affected by gaseous emissions from intensive livestock production. Practical mitigation technologies are needed to minimize emissions from stored manure and improve air quality inside barns. In our previous research, the one-time surficial application of biochar to swine manure significantly reduced emissions of NH3 and phenol. We observed that the mitigation effect decreased with time during the 30-day trials. In this research, we hypothesized that bi-weekly reapplication of biochar could improve the mitigation effect on a wider range of odorous compounds using a larger scale and longer trials. The objective was to evaluate the effectiveness of biochar dose and reapplication on mitigation of targeted gases (NH3, odorous, volatile organic compounds VOCs, odor, greenhouse gases (GHG)) from stored swine manure on a pilot-scale setup over 8-weeks. The bi-weekly reapplication of the lower biochar dose (2 kg/m2) showed much higher significant percentage reductions in emissions for NH3 (33% without and 53% with reapplication) and skatole (42% without and 80% with reapplication), respectively. In addition, the reapplication resulted in the emergence of a statistical significance to the mitigation effect for all other targeted VOCs. Specifically, for indole, the percentage reduction improved from 38% (p = 0.47, without reapplication) to 78% (p = 0.018, with reapplication). For phenol, the percentage reduction improved from 28% (p = 0.71, without reapplication) to 89% (p = 0.005, with reapplication). For p-cresol, the percentage reduction improved from 31% (p = 0.86, without reapplication) to 74% (p = 0.028, with reapplication). For 4-ethyl phenol, the percentage emissions reduction improved from 66% (p = 0.44, without reapplication) to 87% (p = 0.007, with reapplication). The one-time 2 kg/m2 and 4 kg/m2 treatments showed similar effectiveness in mitigating all targeted gases, and no statistical difference was found between the dosages. The one-time treatments showed significant percentage reductions of 33% and 42% and 25% and 48% for NH3 and skatole, respectively. The practical significance is that the higher (one-time) biochar dose may not necessarily result in improved performance over the 8-week manure storage, but the bi-weekly reapplication showed significant improvement in mitigating NH3 and odorous VOCs. The lower dosages and the frequency of reapplication on the larger-scale should be explored to optimize biochar treatment and bring it closer to on-farm trials.

Chen, Baitong (ORCID:0000000266071253)↗

DOE OSTI2020

Wake Statistics of Different-Scale Wind Turbines under Turbulent Boundary Layer Inflow

Subscale wind turbines can be installed in the field for the development of wind technologies, for which the blade aerodynamics can be designed in a way similar to that of a full-scale wind turbine. However, it is not clear whether the wake of a subscale turbine, which is located closer to the ground and faces different incoming turbulence, is also similar to that of a full-scale wind turbine. In this work we investigate the wakes from a full-scale wind turbine of rotor diameter 80 m and a subscale wind turbine of rotor diameter of 27 m using large-eddy simulation with the turbine blades and nacelle modeled using actuator surface models. The blade aerodynamics of the two turbines are the same. In the simulations, the two turbines also face the same turbulent boundary inflows. The computed results show differences between the two turbines for both velocity deficits and turbine-added turbulence kinetic energy. Such differences are further analyzed by examining the mean kinetic energy equation.

17 WIND ENERGY↗

DOE OSTI2024

Inflaton Decay in No-Scale Supergravity and Starobinsky-like Models

We consider the decay of the inflaton in Starobinsky-like models arising from either an R+R 2 theory of gravity or N = 1 no-scale supergravity models. If Standard Model matter is simply introduced to the R+R 2 theory, the inflaton (which appears when the theory is conformally transformed into the Einstein frame) couples to matter predominantly in Standard Model Higgs kinetic terms. This will typically lead to a reheating temperature of ~3 × 10 9 GeV. However, if the Standard Model Higgs is conformally coupled to curvature, the decay rate may be suppressed and vanishes for conformal coupling ζ = 1/6. Nevertheless, the inflaton decays through the conformal anomaly, leading to a reheating temperature of the order of 10 8 GeV. The Starobinsky potential may also arise in no-scale supergravity. In this case, the inflaton decays if there is a direct coupling of the inflaton to matter in the superpotential or to gauge fields through the gauge kinetic function. We also discuss the relation between the theories and demonstrate the correspondence between the no-scale models and the conformally coupled R+R 2 theory (with ζ = 1/6).

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2026

Recent progress in atomic-scale controlled plasma processing

Atomic-scale control in plasma processing is becoming increasingly critical for fabricating of advanced semiconductor devices, particularly as the industry shifts toward three-dimensional (3D) architectures and high-aspect-ratio (HAR) structures. This review presents a comprehensive overview of recent developments in atomic-scale controlled plasma processes, organized along two key directions: the hierarchical structure of plasma–surface interactions and the generational evolution of atomic layer processing (ALP) technologies. We examined the gas phase, where molecular design enables selective generation of ions and radicals; the boundary layer, where transport phenomena govern species delivery into nanoscale features, and the surface, where temperature-dependent reactions and cyclic processing determine etching selectivity and precision. Building on this foundation, we outline five generations of ALP—from thermal atomic layer deposition to transport-aware, temporally and structurally decoupled processes—highlighting the increasing sophistication of process control. The review further explores the transition from empirical recipe development to science-based, data-driven methodologies. By integrating quantum-chemical modeling, advanced diagnostics, and machine learning, we demonstrated how predictive models can link plasma species composition to process outcomes, enabling autonomous and adaptive control strategies. Finally, this review discusses the broader societal implications of plasma process innovation through the E4 quartet: energy and resource efficiency, environmental sustainability, evolutionary advancement, and educational promotion. These principles guide the development of sustainable and intelligent atomic-scale manufacturing technologies that are not only technically advanced but also socially responsible.

Ishikawa, Kenji [Nagoya Univ. (Japan)] (ORCID:0000↗

DOE OSTI2020

Meso-scale Instability Triggered by Dust Feedback in Dusty Rings: Origin and Observational Implications

High spatial resolution observations of protoplanetary disks by ALMA have revealed many substructures that are providing interesting constraints on disk physics as well as dust dynamics, both of which are essential for understanding planet formation. We carry out high-resolution, 2D global hydrodynamic simulations, including the effects of dust feedback, to study the stability of dusty rings. When the ring edges are relatively sharp and the dust surface density becomes comparable to the gas surface density, we find that dust feedback enhances the radial gradients of both the azimuthal velocity profile and the potential vorticity profile at the ring edges. This eventually leads to instabilities on meso-scales (spatial scales of several disk scale heights), causing dusty rings to be populated with many compact regions with highly concentrated dust densities. We also produce synthetic dust emission images using our simulation results and discuss the comparison between simulations and observations.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2022

The ALMaQUEST Survey. VII. Star Formation Scaling Relations of Green Valley Galaxies

We utilize the ALMA-MaNGA QUEnch and STar formation (ALMaQUEST) survey to investigate the kpc-scale scaling relations, presented as the resolved star-forming MS (rSFMS: Σ SFR versus Σ * ), the resolved Schmidt–Kennicutt relation (rSK: Σ SFR versus ${{\rm{\Sigma }}}_{{{\rm{H}}}_{2}}$), and the resolved molecular gas MS (rMGMS: ${{\rm{\Sigma }}}_{{{\rm{H}}}_{2}}$ versus Σ * ), for 11,478 star-forming and 1414 retired spaxels (oversampled by a factor of ~20) located in 22 GV and 12 MS galaxies. For a given galaxy type (MS or GV), the retired spaxels are found to be offset from the sequences formed by the star-forming spaxels on the rSFMS, rSK, and rMGMS planes, toward lower absolute values of sSFR, SFE, and ${f}_{{{\rm{H}}}_{2}}$ by ~1.1, 0.6, and 0.5 dex. The scaling relations for GV galaxies are found to be distinct from that of the MS galaxies, even if the analyses are restricted to the star-forming spaxels only. It is found that, for star-forming spaxels, sSFR, SFE, and ${f}_{{{\rm{H}}}_{2}}$ in GV galaxies are reduced by ~0.36, 0.14, and 0.21 dex, respectively, compared to those in MS galaxies. Therefore, the suppressed sSFR/SFE/f gas in GV galaxies is associated with not only an increased proportion of retired regions in GV galaxies but also a depletion of these quantities in star-forming regions. Finally, the reduction of SFE and ${f}_{{{\rm{H}}}_{2}}$ in GV galaxies relative to MS galaxies is seen in both bulge and disk regions (albeit with larger uncertainties), suggesting that, statistically, quenching in the GV population may persist from the inner to the outer regions.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2023

Core States of Neutron Stars from Anatomizing Their Scaled Structure Equations

Given an Equation of State (EOS) for neutron star (NS) matter, there is a unique mass–radius sequence characterized by a maximum mass ${M}_{\mathrm{NS}}^{\max}$ at radius $R$ max . We first show analytically that the ${M}_{\mathrm{NS}}^{\max}$ and $R$ max scale linearly with two different combinations of the NS central pressure $P$ $c$ and energy density $ε$ $c$ , by dissecting perturbatively the dimensionless Tolman–Oppenheimer–Volkoff (TOV) equations governing NS internal variables. The scaling relations are then verified via 87 widely used and rather diverse phenomenological as well as 17 microscopic NS EOSs with/without considering hadron–quark phase transitions and hyperons, by solving numerically the original TOV equations. The EOS of the densest NS matter allowed before it collapses into a black hole is then obtained. Using the universal ${M}_{\mathrm{NS}}^{\max}$ and $R$ max scalings and Neutron Star Interior Composition Explorer and XMM-Newton mass–radius observational data for PSR J0740+6620, a very narrow constraining band on the NS central EOS is extracted directly from the data for the first time, without using any specific input EOS model.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2024

Relativistic Alfvén Turbulence at Kinetic Scales

Abstract In a strongly magnetized, magnetically dominated relativistic plasma, Alfvénic turbulence can extend to scales much smaller than the particle inertial scales. It leads to an energy cascade somewhat analogous to inertial- or kinetic-Alfvén turbulent cascades existing in nonrelativistic space and astrophysical plasmas. Based on phenomenological modeling and particle-in-cell numerical simulations, we propose that the energy spectrum of such relativistic kinetic-scale Alfvénic turbulence is close to k −3 or slightly steeper than that due to intermittency corrections or Landau damping. We note the analogy of this spectrum with the Kraichnan spectrum corresponding to the enstrophy cascade in 2D incompressible fluid turbulence. Such turbulence strongly energizes particles in the direction parallel to the background magnetic field, leading to nearly one-dimensional particle momentum distributions. We find that these distributions have universal log-normal statistics.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2020

Linking large-scale circulation patterns to low-cloud properties

Abstract. The North Pacific High (NPH) is a fundamental meteorological feature present during the boreal warm season. Marine boundary layer (MBL) clouds, which are persistent in this oceanic region, are influenced directly by the NPH. In this study, we combine 11 years of reanalysis and an unsupervised machine learning technique to examine the gamut of 850 hPa synoptic-scale circulation patterns. This approach reveals two distinguishable regimes – a dominant NPH setup and a land-falling cyclone – and in between a spectrum of large-scale patterns. We then use satellite retrievals to elucidate for the first time the explicit dependence of MBL cloud properties (namely cloud droplet number concentration, liquid water path, and shortwave cloud radiative effect – CRESW) on 850 hPa circulation patterns over the northeast Pacific Ocean. We find that CRESW spans from −146.8 to −115.5 W m−2, indicating that the range of observed MBL cloud properties must be accounted for in global and regional climate models. Our results demonstrate the value of combining reanalysis and satellite retrievals to help clarify the relationship between synoptic-scale dynamics and cloud physics.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2021

Aerosol characteristics at the Southern Great Plains site during the HI-SCALE campaign

Abstract. Large uncertainties exist in global climate model predictions of radiative forcing due to insufficient understanding and simplified numerical representation of cloud formation and cloud–aerosol interactions. The Holistic Interactions of Shallow Clouds, Aerosols and Land Ecosystems (HI-SCALE) campaign was conducted near the DOE's Atmospheric Radiation Measurement (ARM) Southern Great Plains (SGP) site in north-central Oklahoma to provide a better understanding of land–atmosphere interactions, aerosol and cloud properties, and the influence of aerosol and land–atmosphere interactions on cloud formation. The HI-SCALE campaign consisted of two intensive observational periods (IOPs) (April–May and August–September, 2016), during which coincident measurements were conducted both on the G-1 aircraft platform and at the SGP ground site. In this study we focus on the observations at the SGP ground site. An Aerodyne high-resolution time-of-flight aerosol mass spectrometer (HR-ToF-AMS) and an Ionicon proton-transfer-reaction mass spectrometer (PTR-MS) were deployed, characterizing chemistry of non-refractory aerosol and trace gases, respectively. Contributions from various aerosol sources, including biogenic and biomass burning emissions, were retrieved using factor analysis of the AMS data. In general, the organic aerosols at the SGP site was highly oxidized, with oxygenated organic aerosol (OOA) identified as the dominant factor for both the spring and summer IOP though more aged in spring. Cases of isoprene-epoxydiol-derived secondary organic aerosol (IEPOX SOA) and biomass burning events were further investigated to understand additional sources of organic aerosol. Unlike other regions largely impacted by IEPOX chemistry, the IEPOX SOA at SGP was more highly oxygenated, likely due to the relatively weak local emissions of isoprene. Biogenic emissions appear to largely control the formation of organic aerosol (OA) during the HI-SCALE campaign. Potential HOM (highly oxygenated molecule) chemistry likely contributes to the highly oxygenated feature of aerosols at the SGP site, with impacts on new particle formation and global climate.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2022

Subgrid-scale horizontal and vertical variation of cloud water in stratocumulus clouds: a case study based on LES and comparisons with in situ observations

Abstract. Stratocumulus clouds in the marine boundary layer cover a large fraction of ocean surface and play an important role in the radiative energy balance of the Earth system. Simulating these clouds in Earth system models (ESMs) has proven to be extremely challenging, in part because cloud microphysical processes such as the autoconversion of cloud water into precipitation occur at scales much smaller than typical ESM grid sizes. An accurate autoconversion parameterization needs to account for not only the local microphysical process (e.g., the dependence on cloud water content qc and cloud droplet number concentration Nc) but also the subgrid-scale variability of the cloud properties that determine the process rate. Accounting for subgrid-scale variability is often achieved by the introduction of a so-called enhancement factor E. Previous studies of E for autoconversion have focused more on its dependence on cloud regime and ESM grid size, but they have largely overlooked the vertical dependence of E within the cloud. In this study, we use a large-eddy simulation (LES) model, initialized and constrained with in situ and surface-based measurements from a recent airborne field campaign, to characterize the vertical dependence of the horizontal variation of qc in stratocumulus clouds and the implications for E. Similar to our recent observational study (Zhang et al., 2021), we found that the inverse relative variance of qc, an index of horizontal homogeneity, generally increases from cloud base upward through the lower two-thirds of the cloud and then decreases in the uppermost one-third of the cloud. As a result, E decreases from cloud base upward and then increases towards the cloud top. We apply a decomposition analysis to the LES cloud water field to understand the relative roles of the mean and variances of qc in determining the vertical dependence of E. Our analysis reveals that the vertical dependence of the horizontal qc variability and enhancement factor E is a combined result of condensational growth throughout the lower portion of the cloud and entrainment mixing at cloud top. The findings of this study indicate that a vertically dependent E should be used in ESM autoconversion parameterizations.

54 ENVIRONMENTAL SCIENCES↗