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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 1,207 records · Page 67
All sourcesNASA NTRSDOE OSTI
NASA NTRS1991

An experimental study of curved mixing layers: Flow visualization using volume rendering

The existence and importance of large-scale spanwise vortical structures for 2-D straight mixing layers has been well documented in the last decade. Computer models and simulations have sought to reproduce these vortical structures associated with the Kelvin-Helmholtz (K-H) instability mode which is due to the shear per se. Secondary streamwise vortical structures for the same flows were also seen experimentally and have recently been given importance in computational efforts. Curved mixing layers can be characterized as stable (the high-speed stream is placed on the outside of the longitudinal bend), leading to a suppression of the Taylor-Gortler (T-G) instability, and unstable (high-speed stream on the inside of the bend), leading to an enhancement of the T-G instability. The T-G instability is associated with the centripetal acceleration that the curvature imparts. Thus, curvature superimposed on 2-D shear layer flows provides a way for studying the importance of streamwise vorticity, its competition with spanwise vorticity, and changes to entrainment and mixing. Furthermore, the outcome of the competition of a relatively enhanced or suppressed T-G instability with the K-H instability offers the possibility of achieving passive mixing enhancement. As a first step in understanding the competition between the K-H and the T-G instabilities and the resulting changes to the structure of the flow, highly resolved visualizations of the flow structure for the stable and the unstable configurations are provided. The straight layer is also visualized for comparison with earlier works.

Karasso, Paris S.↗
DOE OSTI2023

Structure–function relationships for squid skin-inspired wearable thermoregulatory materials

Wearable thermoregulatory technologies have attracted widespread attention because of their potential for impacting individual physiological comfort and for reducing building energy consumption. Within this context, the study of materials and systems that can merge the advantageous characteristics of both active and passive operating modes has proven particularly attractive. Accordingly, our laboratory has drawn inspiration from the appearance-changing skin of Loliginidae (inshore squids) for the introduction of a unique class of dynamic thermoregulatory composite materials with outstanding figures of merit. Herein, we demonstrate a straightforward approach for experimentally controlling and computationally predicting the adaptive infrared properties of such bioinspired composites, thereby enabling the development and validation of robust structure–function relationships for the composites. Our findings may help unlock the potential of not only the described materials but also comparable systems for applications as varied as thermoregulatory wearables, food packaging, infrared camouflage, soft robotics, and biomedical sensing.

Liu, Panyiming (ORCID:0000000242223670)↗
DOE OSTI2021

Evolution of Metastable Phases During Mg Metal Corrosion: An In Situ Cryogenic X-ray Photoelectron Spectroscopy Study

Magnesium and its alloys are potential structural materials candidates for a wide variety of applications due to their high strength-to-weight ratio. However, ductility and poor corrosion resistance under ambient environmental conditions are the bottleneck for industrial deployment. Designing passivation layers and/or corrosion resistant alloys requires fundamental understanding of the corrosion process. The traditional ex-situ spectroscopic measurements of polycrystalline metal surface with ubiquitous surface impurities and grain boundaries only provided an indistinct view of the corrosion process. To clearly distinguish the mechanism and sequence of corrosion process, we employed in-situ cryo-based x-ray photoelectron spectroscopy (XPS) measurements on Mg single crystal surface exposed to aqueous salt solution. Clean Mg (0001) surfaces were exposed to pure D2O and NaCl aqueous solution (5 wt% NaCl+95 wt% D2O). The interfacial reactions were studied using multimodal analysis including XPS, x-ray diffraction (XRD) and scanning electron microscopy (SEM). In contrast to previous studies, our experiments demonstrated the formation of magnesium chloride hydroxide hydrate during aqueous salt corrosion processes. Evidence of metastable ClO* radicals were also found during the initial aqueous salt solution exposure.

Shutthanandan, Vaithiyalingam↗
NASA NTRS1993

LIF measurements of scalar mixing in turbulent shear layers

The structure of shear layer flows at high Reynolds numbers remains a very interesting problem. Straight mixing layers have been studied and yielded information on the probability density function (pdf) of a passive scalar across the layer. Konrad and Koochesfahani & Dimotakis measured the pdf of the mixture fraction for mixing layers of moderate Reynolds numbers, each about 25,000 (Re based on velocity difference and visual thickness). Their measurements showed a 'non-marching' pdf (central hump which is invariant from edge to edge across the layer), a result which is linked to the visualizations of the spanwise Kelvin-Helmholtz (K-H) instability mode, which is the primary instability for plane shear layer flows. A secondary instability mode, the Taylor-Gortler (T-G) instability, which is associated with streamwise vortical structures, has also been observed in shear layers. Image reconstruction by Jimenez et al. and volume renderings by Karasso & Mungal at low Re numbers have demonstrated that the K-H and the T-G instability modes occur simultaneously in a non-mutually destructive way, evidence that supports the quasi two-dimensional aspect of these flows and the non-marching character of the pdf at low Reynolds numbers. At higher Re numbers though, the interaction of these two instability modes is still unclear and may affect the mixing process. In this study, we perform measurements of the concentration pdf of plane mixing layers for different operating conditions. At a speed ratio of r = U(sub 1)/U(sub 2) = 4:1, we examine three Reynolds number cases: Re = 14,000, Re = 31,000, and Re = 62,000. Some other Re number cases' results, not presented in detail, are invoked to explain the behavior of the pdf of the concentration field. A case of r = 2.6:1 at Re = 20,000 is also considered. The planar laser-induced fluorescence technique is used to yield quantitative measurements. The different Re are obtained by changing the velocity magnitudes of the two streams. The question of resolution of these measurements is addressed. In order to investigate the effects of the initial conditions on the development and the structure of the mixing layer, the boundary layer on the high-speed side of the splitter plate is tripped. The average concentration and the average mixed fluid concentration are also calculated to further understand the changes in the shear layer for the different cases examined.

Karasso, Paris S.↗
NASA NTRS1982

The composition and vertical structure of the lower cloud deck on Venus

Excluding the insertion of a probe into the lower Venus atmosphere, the only means of examining the atmospheric properties below the upper cloud layer are by passive or active radio techniques. Particularly, in a radio occultation experiment, the amplitude and Doppler data of a signal which has been refracted by the dense Venus atmosphere provide temperature, pressure, atmospheric density, cloud mass content, and some information about the cloud composition. The Venus orbiting spacecraft Pioneer Venus has provided radio occultation data for more than two years. The present investigation has the primary goal to use the absorption coefficient profiles derived from the radio occultation experiment to determine the mass content and composition of the Venusian lower deck. Attention is given to an experiment description, liquid content calculations, the mass content equation, the subtraction of gaseous absorbers, dielectric constant measurements, the concentration profile, the spherical shell model, and mass content profiles for all orbits.

Cimino, J.↗
DOE OSTI2019

Purification of Gas and Liquid Streams Using Composite Sorbents Embedded in a Polyacrylonitrile Matrix

As new sorbents are developed for purifying gases or liquids via physisorption and/or chemisorption processes, the objective is typically to increase the specific surface area (SSA) to maximize the available binding sites for capturing various species of interest. One downfall to making a sorbent more porous is that it often leads to a product that is fragile or friable and can be damaged (resulting in unwanted powders), thus imposing process limitations. Techniques can be used to enhance the mechanical integrity of a sorbent, including heat treatments or pelletization with extrusion or granulation processes, but these can result in collapsed, unavailable pore structures within the sorbent, which decreases the diffusivity and eventually reduces the capacities of target species. An alternative approach for improving the mechanical integrity of the sorbent is to bind it (or encapsulate it) within a porous matrix that passively holds the sorbent in place. Typically, this approach leads to a decrease in sorption efficiency on the basis of starting sorbent mass, because the active sorbent is diluted by the binding matrix material and the active surfaces of the sorbent are somewhat obscured by the binding matrix; however, it comes with the advantage that the active sorbent is held in place and better protected from disintegrating during operation. One approach to securing the active sorbent is to embed it in a macroporous, passive polyacrylonitrile (PAN) matrix to create a composite sorbent. When optimized, the PAN matrix is highly porous and allows for gaseous or aqueous media transport through the product, providing adequate binding site access between the active sorbent and the species of interest. Including a polymer in the composite sorbent limits the maximum operating temperature, above which the composite sorbent incurs loss of structural integrity (e.g., decomposes) and/or reduction in SSA. Composite sorbents have been demonstrated with sulfide aerogels (SnS-PAN) for capturing I2(g), hydrogen mordenite (HZ-PAN) and silver-exchanged mordenite (AgZ-PAN) for capturing Kr and Xe, nanoparticle metal oxides (Nano-Composite Arsenic Sorbent, or N-CAS) for removing arsenic from water, ammonium molybdophosphate (AMP-PAN) for removing cesium-137 (137Cs) from aqueous nuclear waste streams, and The Phosphate Sponge (TPS) composite, which is being used to remove inorganic/ortho-phosphates in water treatment processes to mitigate introduction to the environment, which impedes toxic algae bloom formations. This chapter provides details on production of these materials along with options to optimize the synthesis process. It also includes experimental techniques to characterize products and assess their performance.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2016

Programmable shape transformation of elastic spherical domes

We investigate mismatch strain driven programmable shape transformation of spherical domes and report the effects of different geometric and structural characteristics on dome behavior in response to applied mismatch strain. We envision a bilayer dome design where the differential swelling of the inner layer with respect to the passive outer layer in response to changes in dome surroundings (such as the introduction of an organic solvent) introduces mismatch strain within the bilayer system and causes dome shape transformation. Finite element analysis reveals that, in addition to snap-through, spherical domes undergo bifurcation buckling and eventually gradual bending to morph into cylinders with increasing mismatch strain. Besides demonstrating how the snap-through energy barrier depends on the spherical dome shape, our analysis identifies three distinct groups of dome geometries based on their mismatch strain-transformed configuration relationships. Our experiments with polymer-based elastic bilayer domes that exhibit differential swelling in organic solvents qualitatively confirm the finite element predictions. We establish that, in addition to externally applied stimuli (mismatch strain), bilayer spherical dome morphing can be tuned and hence programmed through its geometry and structural characteristics. Incorporation of an elastic instability mechanism such as snap-through within the framework of stimuli-responsive functional devices can improve their response time which is otherwise controlled by diffusion. Furthermore, our proposed design guidelines can be used to realize deployable, multi-functional, reconfigurable, and therefore, adaptive structures responsive to a diverse set of stimuli across multiple length scales.

36 MATERIALS SCIENCE↗
DOE OSTI2017

Avoiding Complications in Bone and Soft Tissue Ablation

As with percutaneous ablation of tumors in the liver, lungs, and kidneys, ablation of bone and non-visceral soft tissue tumors carries risk, primarily from collateral damage to vital structures in proximity to the target tumor. Certain risks are of particular interest when ablating bone and non-visceral soft tissue tumors, namely neural or skin injury, bowel injury, fracture, and gas embolism from damaged applicators. Ablation of large volume tumors also carries special risk. Many techniques may be employed by the interventional radiologist to minimize complications when treating tumors in the musculoskeletal system. These methods include those to depict, displace, or monitor critical structures. Thus, measures to provide thermoprotection may be active, such as careful ablation applicator placement and use of various displacement techniques, as well as passive, including employment of direct temperature, radiographic, or neurophysiologic monitoring techniques. Cementoplasty should be considered in certain skeletal locations at risk of fracture. Patients treated with large volume tumors should be monitored for renal dysfunction and properly hydrated. Finally, ablation applicators should be cautiously placed in the constrained environment of intact bone.

62 RADIOLOGY AND NUCLEAR MEDICINE↗
DOE OSTI2016

Infrared absorption of hydrogen-related defects in ammonothermal GaN

Polarization controlled Fourier transform infrared (FTIR) absorption measurements were performed on a high quality m-plane ammonothermal GaN crystal grown using basic chemistry. The polarization dependence of characteristic absorption peaks of hydrogen-related defects at 3000–3500 cm{sup −1} was used to identify and determine the bond orientation of hydrogenated defect complexes in the GaN lattice. Majority of hydrogen was found to be bonded in gallium vacancy complexes decorated with one to three hydrogen atoms (V{sub Ga}-H{sub 1,2,3}) but also hydrogenated oxygen defect complexes, hydrogen in bond-center sites, and lattice direction independent absorption were observed. Absorption peak intensity was used to determine a total hydrogenated V{sub Ga} density of approximately 4 × 10{sup 18} cm{sup −3}, with main contribution from V{sub Ga}-H{sub 1,2}. Also, a significant concentration of electrically passive V{sub Ga}-H{sub 3} was detected. The high density of hydrogenated defects is expected to have a strong effect on the structural, optical, and electrical properties of ammonothermal GaN crystals.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2018

Passive wavelength tuning and multichannel photonic coupling using monolithically integrated vertical microresonators on ridge waveguides

The passive tuning of the resonant coupling wavelength in a SiN x vertical microring coupler (VμRC) monolithically integrated on a ridge waveguide by engineering the structural parameters of the VμRCs is experimentally demonstrated and theoretically verified. Multi-channel photonic coupling is achieved by integrating two different VμRCs on a single ridge waveguide. This work represents here a critical step to 3D photonic integration using VμRCs.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2021

Twisted bilayer graphene. I. Matrix elements, approximations, perturbation theory, and a k · p two-band model

We investigate the twisted bilayer graphene (TBG) model of Bistritzer and MacDonald (BM) [Bistritzer and MacDonald, Proc. Natl. Acad. Sci. 108, 12233 (2011)] to obtain an analytic understanding of its energetics and wave functions needed for many-body calculations. We provide an approximation scheme for the wave functions of the BM model, which first elucidates why the BM K M -point centered original calculation containing only four plane waves provides a good analytical value for the first magic angle (θ M ≈ 1°). The approximation scheme also elucidates why most of the many-body matrix elements in the Coulomb Hamiltonian projected to the active bands can be neglected. By applying our approximation scheme at the first magic angle to a Γ M -point centered model of six plane waves, we analytically understand the reason for the small Γ M -point gap between the active and passive bands in the isotropic limit w 0 = w 1 . Furthermore, we analytically calculate the group velocities of the passive bands in the isotropic limit, and show that they are almost doubly degenerate, even away from the Γ M point, where no symmetry forces them to be. Furthermore, moving away from the Γ M and K M points, we provide an explicit analytical perturbative understanding as to why the TBG bands are flat at the first magic angle, despite the first magic angle is defined by only requiring a vanishing K M -point Dirac velocity. We derive analytically a connected “magic manifold” w 1 = $2\sqrt{1 + w^{2}_{0}}$ $-\sqrt{2 + 3w^2_0}$, on which the bands remain extremely flat as w 0 is tuned between the isotropic (w 0 = w 1 ) and chiral (w 0 = 0) limits. We analytically show why going away from the isotropic limit by making w 0 less (but not larger) than w 1 increases the Γ M -point gap between the active and the passive bands. Finally, by perturbation theory, we provide an analytic Γ M point k ∙ p two-band model that reproduces the TBG band structure and eigenstates within a certain w 0 , w 1 parameter range. Further refinement of this model are discussed, which suggest a possible faithful representation of the TBG bands by a two-band Γ M point k ∙ p model in the full w 0 , w 1 parameter range.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2021

Reliability Analysis of Large-Area, Low Pressure-Assisted Silver Sintering for Medium-Voltage Power Modules

Multi-layer insulating ceramic substrates can enable medium-voltage (MV) power modules with reduced peak electric field. This benefit is particularly important for MV silicon carbide (SiC) MOSFETs due to their higher operating voltages. Large-area, low-pressure assisted silver sintering is a potential solution for bonding substrates to create a multi-layer structure. The voiding content and defect density of the bond used to create the multi-layer substrate stack-up is critical to the reliability of the power module and the thermal performance, as this bond is in the primary path for heat dissipation in the power module structure. Here, samples of two-layer direct bonded aluminum (DBA) stacks have been fabricated and subjected to thermal cycling to analyze their reliability. Passive thermal cycling from -40 degrees C to 200 degrees C was performed. Cross-sections were cut at pre-determined intervals and imaged with Scanning Electron Microscopy (SEM). After 1000 thermal cycles, adhesive failures are observed between the sintered silver and the DBA surface. Cross-sections were cut and imaged via optical microscope and SEM. Thermal analyzer measurements are recorded on a 10-kV SiC power module utilizing the sintered DBA substrate stacks.

30 DIRECT ENERGY CONVERSION↗
DOE OSTI2022

MELCOR Accident Progression and Source Term Demonstration Calculations for a FHR

MELCOR is an integrated thermal hydraulics, accident progression, and source term code for reactor safety analysis that has been developed at Sandia National Laboratories for the United States Nuclear Regulatory Commission (NRC) since the early 1980s. Though MELCOR originated as a light water reactor (LWR) code, development and modernization efforts have expanded its application scope to include non-LWR reactor concepts. Current MELCOR development efforts include providing the NRC with the analytical capabilities to support regulatory readiness for licensing non-LWR technologies under Strategy 2 of the NRC's near- term Implementation Action Plans. Beginning with the Next Generation Nuclear Project (NGNP), MELCOR has undergone a range of enhancements to provide analytical capabilities for modeling the spectrum of advanced non-LWR concepts. This report describes the generic plant model developed to demonstrate MELCOR capabilities to perform fluoride-salt-cooled high-temperature reactor (FHR) safety evaluations. The generic plant model is based on publicly-available FHR design information. For plant aspects (e.g., reactor building leak rate and details of the cover-gas system) that are not described in the FHR references, the analysts made assumptions needed to construct a MELCOR full-plant model. The FHR model uses a TRi-structural ISOtropic (TRISO)-particle fuel pebble-bed reactor with a primary system rejecting heat to two coiled tube air heat ex changers. Three passive direct reactor auxiliary cooling systems provide heat removal to supplement or replace the emergency secondary system heat removal during accident conditions. Surrounding the reactor vessel is a low volume reactor cavity that insulates the reactor with fire bricks and thick concrete walls. A refractory reactor liner system provides water cooling to reduce the concrete wall temperatures. Example calculations are performed to show the plant response and MELCOR capabilities to characterize a range of accident conditions. The accidents selected for evaluation consider a range of degraded and failed modes of operation for key safety functions providing reactivity control, the primary system decay heat removal and also a piping leak of the line to the coolant drain tank.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗
DOE OSTI2021

Multiphysics simulations of a steady-state lower hybrid current drive antenna for the FSNF

The Fusion Nuclear Science Facility (FNSF) is a proposed tokamak reactor with the mission to investigate operation of a fusion reactor in a nuclear environment. The high neutron fluence component of the FNSF mission requires steady-state operation for extremely long pulses (t_{pulse} ∼ months) at full power. Plasma sustainment and current drive will be critical components of a successful FNSF. COMSOL Multiphysics software is used for combined radiofrequency (RF) and thermal simulations of the lower hybrid current drive (LHCD) antenna system. These simu- lations consider the resistive RF losses in the antenna including realistic surface roughness and a range of potential materials. The thermal analysis adds volumetric nuclear heating, plasma heat flux on leading edges, and electromagnetic radiation from the plasma to the RF heating calculated by COMSOL. Additional neutronics calculations have been performed to determine the impact of these antenna designs on activated waste disposal for the materials considered. The simulations show that it is technically feasible to implement a fully-active multi-junction (FAM) rather than a passive-active multi-junction (PAM) style of antenna if the septum between adjacent waveguides is sufficiently wide and the thermal conductivity of the structural material is sufficiently high. The FAM has the benefit of higher achievable power density with respect to the PAM, which results in a more compact antenna with potentially lower impact on neutron shielding and tritium breeding. These considerations point to tungsten rather than steel as the preferred structural material in constructing the antenna.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
NASA NTRS1970

The integration of remote sensing data into global weather prediction, wave forecasting, and ocean circulation computer based systems

Data from infrared imaging systems and satellite infrared spectrometer (SIRS) for determining sea surface temperature and the atmospheric structure in cloudless areas over the oceans are discussed. Although some interpretations differ, it is clear that simultaneous measurements of radar sea return and passive microwave temperature will provide estimates of the wind speed, and perhaps wind direction, over the oceans, especially in cloudless areas, for a wide range of wind speeds. The problem of integrating the data that would be obtained by a spacecraft, especially one with a combination radar-radiometer, into global analysis procedures for meteorological, wave, and oceanographic predictions is described.

Pierson, W. J., Jr.↗
NASA NTRS1980

Heat-rejection design for large concentrating solar arrays

This paper considers the effect of heat rejection devices (radiators) on the performance and cost of large concentrating solar arrays for space application. Overall array characteristics are derived from the weight, cost, and performance of four major components; namely primary structure, optics/secondary structure, radiator, and solar panel. An ideal concentrator analysis is used to establish general cost and performance trends independent of specific array design. Both passive and heat-pipe radiation are evaluated, with an incremental cost-of-power approach used in the evaluation. Passive radiators are found to be more cost effective with silicon than with gallium arsenide (GaAs) arrays. Representative concentrating arrays have been evaluated for both near-term and advanced solar cell technology. Minimum cost of power is achieved at geometric concentration ratios in the range 2 to 6.

French, E. P.↗
NASA NTRS1980

Development of simplified process for environmentally resistant cells

This report describes a program to develop a simple, foolproof, all vacuum solar cell manufacturing process which can be completely automated and which results in medium efficiency cells which are inherently environmentally resistant. All components of the completed cells are integrated into a monolithic structure with no material interfaces. The exposed materials (SI, Al2O3, Al, Ni) are all resistant to atmospheric attack and the junction, per se, is passivated to prevent long term degradation. Such cells are intended to be incorporated into a simple module consisting basically of a press formed metallic superstructure with a separated glass cover for missile, etc., protection.

King, W. J.↗