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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 1,207 records · Page 67
All sourcesNASA NTRSDOE OSTI
DOE OSTI2023

Calibration of the Solid‐State Nuclear Magnetic Resonance Search for Axion‐Like Dark Matter

Abstract Calibration of nuclear‐magnetic‐resonance‐based searches for axion‐like dark matter can be performed by free induction decay (FID) measurements. This manu‐ script describes FID experiments on several solid materials, motivated by the Cosmic Axion Spin Precession Experiment (CASPEr) program. Experiments with 207 Pb nuclear spins in ferroelectrics, lead magnesium niobate‐lead titanate (PbMg 1/3 Nb 2/3 O 3 ) (PbTiO 3 ) 1/3 (PMN‐PT) and lead zirconium titante PbZr 0.52 Ti 0.48 O 3 (PZT) are directly relevant to the CASPEr‐electric search for the electric dipole moment interaction of axion‐like dark matter. Experiments with 31 P nuclear spins in gadolinium‐doped hydroxypyromorphite Pb 4.95 Gd 0.05 (PO 4 ) 3 OH (HPM:Gd) are used for apparatus calibration. The measurements characterized the nuclear spin ensemble coherence time and the magnetic resonance detection sensitivity for these samples. Calibration is performed using small tip‐angle pulses.

Winter, Andrew J.↗
DOE OSTI2024

Relativistic Douglas–Kroll–Hess calculations of hyperfine interactions within first-principles multireference methods

A relativistic magnetic hyperfine interaction Hamiltonian based on the Douglas–Kroll–Hess (DKH) theory up to the second order is implemented within the ab initio multireference methods, including spin–orbit coupling in the Molcas/OpenMolcas package. This implementation is applied to calculate relativistic hyperfine coupling (HFC) parameters for atomic systems and diatomic radicals with valence s or d orbitals by systematically varying active space size in the restricted active space self-consistent field formalism with restricted active space state interaction for spin–orbit coupling. The DKH relativistic treatment of the hyperfine interaction reduces the Fermi contact contribution to the HFC due to the presence of kinetic factors that regularize the singularity of the Dirac delta function in the nonrelativistic Fermi contact operator. This effect is more prominent for heavier nuclei. As the active space size increases, the relativistic correction of the Fermi contact contribution converges well to the experimental data for light and moderately heavy nuclei. The relativistic correction, however, does not significantly affect the spin-dipole contribution to the hyperfine interaction. In addition to the atomic and molecular systems, the implementation is applied to calculate the relativistic HFC parameters for large trivalent and divalent Tb-based single-molecule magnets (SMMs), such as Tb(III)Pc2 and Tb(II)(CpiPr5)2 without ligand truncation using well-converged basis sets. In particular, for the divalent SMM, which has an unpaired valence 6s/5d hybrid orbital, the relativistic treatment of HFC is crucial for a proper description of the Fermi contact contribution. Even with the relativistic hyperfine Hamiltonian, the divalent SMM is shown to exhibit strong tunability of HFC via an external electric field (i.e., strong hyperfine Stark effect).

Chemistry↗
DOE OSTI2020

Effects of filling, strain, and electric field on the Néel vector in antiferromagnetic CrSb

CrSb is a layered antiferromagnet (AFM) with perpendicular magnetic anisotropy, a high Néel temperature, and large spin-orbit coupling (SOC), which makes it interesting for AFM spintronic applications. To elucidate the various mechanisms of Néel vector control, the effects of strain, band filling, and electric field on the magnetic anisotropy energy (MAE) of bulk and thin-film CrSb are determined and analyzed using density functional theory. The MAE of the bulk crystal is large (1.2 meV per unit cell). Due to the significant ionic nature of the Cr-Sb bond, finite slabs are strongly affected by end termination. Truncation of the bulk crystal to a thin film with one surface terminated with Cr and the other surface terminated with Sb breaks inversion symmetry, creates a large charge dipole and average electric field across the film, and breaks spin degeneracy, such that the thin film becomes a ferrimagnet. The MAE is reduced such that its sign can be switched with realistic strain, and the large SOC gives rise to an intrinsic voltage controlled magnetic anisotropy. A slab terminated on both faces with Cr remains a compensated AFM, but with the compensation occurring nonlocally between mirror-symmetric Cr pairs. In-plane alignment of the moments is preferred, the magnitude of the MAE remains large, similar to that of the bulk, and it is relatively insensitive to filling.

36 MATERIALS SCIENCE↗
DOE OSTI2021

Non-neutral plasma manipulation techniques in development of a high-capacity positron trap

Preliminary experiments have been performed toward the development of a multi-cell Penning–Malmberg trap for the storage of large numbers of positrons (≥10 10 e + ). We introduce the master-cell test trap and the diagnostic tools for first experiments with electrons. The usage of a phosphor screen to measure the z-integrated plasma distribution and the number of confined particles is demonstrated, as well as the trap alignment to the magnetic field ( B = 3.1 T) using the m = 1 diocotron mode. The plasma parameters and expansion are described along with the autoresonant excitation of the diocotron mode using rotating dipole fields and frequency chirped sinusoidal drive signals. We analyze the reproducibility of the excitation and use these findings to settle on the path for the next generation multi-cell test device.

Singer, M.↗
DOE OSTI2025

The HIBEAM instrument at the European spallation source

The European spallation source (ESS) will be the world’s brightest neutron source and will open a new intensity frontier in particle physics. The HIBEAM collaboration aims to exploit the unique potential of the ESS with a dedicated ESS instrument for particle physics which offers world-leading capability in a number of areas. The HIBEAM program includes the first search in thirty years for free neutrons converting to antineutrons and searches for sterile neutrons, ultralight axion dark matter and nonzero neutron electric charge. This paper outlines the capabilities, design, infrastructure, and scientific potential of the HIBEAM program, including its dedicated beamline, neutron optical system, magnetic shielding and control, and detectors for neutrons and antineutrons. Additionally, we discuss the long-term scientific exploitation of HIBEAM, which may include measurements of the neutron electric dipole moment and precision studies of neutron decays.

47 OTHER INSTRUMENTATION↗
DOE OSTI2018

An Analysis of Characteristics of Magnetostatic Waves Propagating in Nonhomogeneous Fields Across the Ferrospinel Film Thickness

The amplitude-frequency characteristics (AFCs) of magnetostatic waves in the films of magnesium-manganese ferrospinels with nanostructured inhomogeneities are discussed. A common effect, observed in the film AFCs under different process conditions, is the ‘oscillations of propagation’ of magnetostatic waves as a function of the frequency. The oscillation pattern is thought to depend on the inhomogeneous exchange parameters and the surface anisotropy constants. The wave instability is characterized by the resonant interaction of the dipole magnetostatic waves with the surface spin waves. It is shown that the ferrospinel films with periodic nanostructured inhomogeneities of 30–40 nm could be treated as magnon crystals. An inclusion of the inhomogeneity into consideration allows one to provide reasoning for the formation of the rejection bands within the range 9–12 GHz, whose frequencies correspond to Bragg frequencies.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2014

Theoretical structural and vibrational study of 5-trifluoromethyluracil. A comparison with uracil

In the present work, a comparative study on the structural and vibrational properties of the 5-trifluoromethyluracil (TFMU) derivative with those corresponding to uracil in gas and aqueous solution phases was performed combining the available H{sup 1}-NMR, C{sup 13}-NMR, F{sup 19}-NMR and FTIR spectra with Density Functional Theory (DFT) calculations. Three stable conformers were theoretically determined in both media by using the hybrid B3LYP/6-31G* method. The solvent effects were simulated by means of the self-consistent reaction field (SCRF) method employing the integral equation formalism variant (IEFPCM). Complete assignments of the vibrational spectra in both phases were performed combining the internal coordinates analysis and the DFT calculations with the Scaled Quantum Mechanics Force Field (SQMFF) methodology. The atomic charges, bond orders, solvation energies, dipole moments, molecular electrostatic potentials and force constants parameters were calculated for the three conformers of TFMU in gas phase and aqueous solution.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2015

Sub-terahertz spectroscopy reveals that proteins influence the properties of water at greater distances than previously detected

The initial purpose of the study is to systematically investigate the solvation properties of different proteins in water solution by terahertz (THz) radiation absorption. Transmission measurements of protein water solutions have been performed using a vector network analyser-driven quasi-optical bench covering the WR-3 waveguide band (0.220–0.325 THz). The following proteins, ranging from low to high molecular weight, were chosen for this study: lysozyme, myoglobin, and bovine serum albumin (BSA). Absorption properties of solutions were studied at different concentrations of proteins ranging from 2 to 100 mg/ml. The concentration-dependent absorption of protein molecules was determined by treating the solution as a two-component model first; then, based on protein absorptivity, the extent of the hydration shell is estimated. Protein molecules are shown to possess a concentration-dependent absorptivity in water solutions. Absorption curves of all three proteins sharply peak towards a dilution-limit that is attributed to the enhanced flexibility of protein and amino acid side chains. An alternative approach to the determination of hydration shell thickness is thereby suggested, based on protein absorptivity. The proposed approach is independent of the absorption of the hydration shell. The derived estimate of hydration shell thickness for each protein supports previous findings that protein-water interaction dynamics extends beyond 2-3 water solvation-layers as predicted by molecular dynamics simulations and other techniques such as NMR, X-ray scattering, and neutron scattering. According to our estimations, the radius of the dynamic hydration shell is 16, 19, and 25 Å, respectively, for lysozyme, myoglobin, and BSA proteins and correlates with the dipole moment of the protein. It is also seen that THz radiation can serve as an initial estimate of the protein hydrophobicity.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2016

Transducer selection and application in magnetoacoustic tomography with magnetic induction

As an acoustic receiver, transducer plays a vital role in signal acquisition and image reconstruction for magnetoacoustic tomography with magnetic induction (MAT-MI). In order to optimize signal acquisition, the expressions of acoustic pressure detection and waveform collection are theoretically studied based on the radiation theory of acoustic dipole and the reception pattern of transducer. Pressure distributions are simulated for a cylindrical phantom model using a planar piston transducer with different radii and bandwidths. The proposed theory is also verified by the experimental measurements of acoustic waveform detection for an aluminum foil cylinder. It is proved that acoustic pressure with sharp and clear boundary peaks can be detected by the large-radius transducer with wide bandwidth, reflecting the differential of the induced Lorentz force accurately, which is helpful for precise conductivity reconstruction. To detect acoustic pressure with acceptable pressure amplitude, peak pressure ratio, amplitude ratio, and improved signal to noise ratio, the scanning radius of 5–10 times the radius of the object should be selected to improve the accuracy of image reconstruction. This study provides a theoretical and experimental basis for transducer selection and application in MAT-MI to obtain reconstructed images with improved resolution and definition.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2020

Hilbert-Space Fragmentation from Strict Confinement

In this work, we study one-dimensional spin-1/2 models in which strict confinement of Ising domain walls leads to the fragmentation of Hilbert space into exponentially many disconnected subspaces. Whereas most previous works emphasize dipole moment conservation as an essential ingredient for such fragmentation, we instead require two commuting U(1) conserved quantities associated with the total domain-wall number and the total magnetization. The latter arises naturally from the confinement of domain walls. Remarkably, while some connected components of the Hilbert space thermalize, others are integrable by Bethe ansatz. We further demonstrate how this Hilbert-space fragmentation pattern arises perturbatively in the confining limit of $\mathbb{Z}_2$ gauge theory coupled to fermionic matter, leading to a hierarchy of timescales for motion of the fermions. This model can be realized experimentally in two complementary settings.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2019

Excitation and $\gamma$-decay coincidence measurements at the GRAF beamline for studies of pygmy and giant dipole resonances

Physical studies of electric dipole excitations in atomic nuclei e.g. the structure of pygmy dipole resonances and isovector giant dipole resonances are attracting much attention recently. In this article, we describe a technical development in the coincidence measurement of the excitation processes with the Grand Raiden high-resolution magnetic spectrometer and the γ-decay processes by the CAGRA and SCγ LLA efficient γ-detector arrays at the Research Center for Nuclear Physics at Osaka University. Specifically, we describe how we developed a new beamline (GRAF), for γ detection at the target position by placing the spectrometer at an angle of 4.5-19.0° and by transporting the primary beam to a well-shielded beam dump. Experimental conditions and representative data are shown for each of the two γ-detector arrays.

43 PARTICLE ACCELERATORS↗
DOE OSTI2018

Muon Beam Dynamics and Spin Dynamics in the g-2 Storage Ring

The goal of the new g-2 experiment at fermilab is a measurement of the anomalous magnetic moment of the muon, with uncertainty of less than 140 ppb. The experimental method is to store a beam of polarized muons in a storage ring with pure vertical dipole field and electrostatic focusing, and to measure the precession frequency. Control of the systematics depends on unprecedented knowledge of the details of the phase space of the muon distribution. That knowledge is derived from direct measurements with scintillating fiber detectors that are inserted into the muon beam for diagnostic measurements, traceback straw tube tracking chambers, as well as the calorimeters that measure energy, time and position of the decay positrons. The interpretation of the measurements depends on a detailed model of the storage ring guide field. This invited talk presents results of studies of the distribution from the commissioning run of the experiment.

43 PARTICLE ACCELERATORS↗
DOE OSTI2025

Search for the Muon EDM at Muon $g-2$

After 6 years of taking data, the Muon $g-2$ Experiment measured the anomalous magnetic moment of the muon $a_μ$ to a final precision of 127 ppb. In parallel to this analysis, it is possible to perform a measurement of the muon electric dipole moment (EDM) using the straw tracker detectors. In the Standard Model (SM) EDMs are predicted to be vanishingly small. A non-zero muon EDM would constitute physics beyond the SM (BSM) and be a source of charge-parity violation. The current limit on the muon EDM was set at the predecessor experiment at Brookhaven National Laboratory, giving $|d_\mu|<1.8\times10^{-19}\ e\cdot$cm Fermilab aims to improve this by an order of magnitude, which will help to constrain BSM theories. This poster will cover the importance, methodology, and status of this measurement.

Bailey, Lucy [University Coll. London]↗
DOE OSTI2019

Searches for Electric Dipole Moments—Overview of Status and New Experimental Efforts

Searches for permanent electric dipole moments (EDMs) of fundamental particles, atoms and molecules are promising experiments to constrain and potentially reveal beyond Standard Model (SM) physics. A non-zero EDM is a direct manifestation of time-reversal (T) violation, and, equivalently, violation of the combined operation of charge-conjugation (C) and parity inversion (P). Identifying new sources of CP violation can help to solve fundamental puzzles of the SM, e.g., the observed baryon-asymmetry in the Universe. Theoretical predictions for magnitudes of EDMs in the SM are many orders of magnitude below current experimental limits. However, many theories beyond the SM require larger EDMs. Experimental results, especially when combined in a global analysis, impose strong constraints on CP violating model parameters. Including an overview of EDM searches, I will focus on the future neutron EDM experiment at TRIUMF (Vancouver). For this effort, the TUCAN (TRIUMF Ultra Cold Advanced Neutron source) collaboration is aiming to build a strong, world leading source of ultra cold neutrons (UCN) based on a unique combination of a spallation target and a superfluid helium UCN converter. Another focus will be the search for an EDM of the diamagnetic atom 129 Xe using a 3 He comagnetometer and SQUID detection. The HeXeEDM collaboration has taken EDM data in 2017 and 2018 in the magnetically shielded room (BMSR-2) at PTB Berlin.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2019

New Limit on the Permanent Electric Dipole Moment of 129 Xe Using 3 He Comagnetometry and SQUID Detection

We report results of a new technique to measure the electric dipole moment of 129 Xe with 3 He comagnetometry. In this work, both species are polarized using spin-exchange optical pumping, transferred to a measurement cell, and transported into a magnetically shielded room, where SQUID magnetometers detect free precession in applied electric and magnetic fields. The result from a one week measurement campaign in 2017 and a 2.5 week campaign in 2018, combined with detailed study of systematic effects, is d A ( 129 Xe) = 1.4 ± 6.6 stat ± 2.0 syst ) × 10 –28 e cm. This corresponds to an upper limit of |d A ( 129 Xe)| < 1.4 × 10 –27 e cm (95% C.L.), a factor of 5 more sensitive than the limit set in 2001.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2013

Canted–Cosine–Theta Magnet (CCT)—A Concept for High Field Accelerator Magnets

Canted-Cosine-Theta (CCT) magnet is an accelerator magnet that superposes fields of nested and tilted solenoids that are oppositely canted. The current distribution of any canted layer generates a pure harmonic field as well as a solenoid field that can be cancelled with a similar but oppositely canted layer. The concept places windings within mandrel's ribs and spars that simultaneously intercept and guide Lorentz forces of each turn to prevent stress accumulation. With respect to other designs, the need for pre-stress in this concept is reduced by an order of magnitude making it highly compatible with the use of strain sensitive superconductors such as Nb 3 Sn or HTS. Intercepting large Lorentz forces is of particular interest in magnets with large bores and high field accelerator magnets like the one foreseen in the future high energy upgrade of the LHC. This paper describes the CCT concept and reports on the construction of CCT1 a "proof of principle" dipole.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2017

LINEAR LATTICE AND TRAJECTORY RECONSTRUCTION AND CORRECTION AT FAST LINEAR ACCELERATOR

The low energy part of the FAST linear accelerator based on 1.3 GHz superconducting RF cavities was successfully commissioned [1]. During commissioning, beam based model dependent methods were used to correct linear lattice and trajectory. Lattice correction algorithm is based on analysis of beam shape from profile monitors and trajectory responses to dipole correctors. Trajectory responses to field gradient variations in quadrupoles and phase variations in superconducting RF cavities were used to correct bunch offsets in quadrupoles and accelerating cavities relative to their magnetic axes. Details of used methods and experimental results are presented.

43 PARTICLE ACCELERATORS↗