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At least 1,189 records · Page 66
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NASA NTRS1983

The sun-weather connection - Sudden stratospheric warmings correlated with sudden commencements and solar proton events

It has been found that a strong correlation exists between sudden stratospheric warmings and sudden commencements of geomagnetic activity. This correlation follows a 22-yr cycle. The sudden warmings of the lower stratosphere occur near the north magnetic pole over Siberia and the Pacific, although occasionally they do occur over North America. A mechanism explaining how the solar wind ultimately affects the surface weather through its selective interaction with the middle atmosphere is outlined.

Neubauer, L.↗
NASA NTRS1983

Observation of wave-wave interactions in the stratosphere

Data from the LIMS instrument for January 1979 are used to provide further evidence for the often observed vacillation between the amplitudes of waves 1 and 2 in the stratosphere. The vacillation is shown to result primarily from nonlinear wave-wave interactions within the stratosphere. Two ways of interpreting nonlinearity are discussed. In the first, the basic state is defined to include large amplitude waves as well as the mean zonal wind. A forced wave propagates with respect to this asymmetric basic state, which can lead to changes in the conventional zonal wavenumber measured at one latitude. The other view of nonlinearity, interaction of wave with the zonal flow and with other wavenumbers are considered separately. Wave-wave interactions among waves 1, 2 and 3 are calculated. The derivation and computation of wave-wave interaction terms in the potential enstrophy balance are given. The observations indicate that enstrophy transfer among waves can be substantial even when the amplitude of one of the contributing waves is small. The computed enstrophy balance also demonstrates that wave-wave interactions can have a large effect on the interaction of waves with the mean flow.

Smith, A. K.↗
NASA NTRS1983

Nitric oxide in the upper stratosphere - Measurements and geophysical interpretation

A rocket-borne parachute-deployed chemiluminescence instrument has obtained seven new measurements of atmospheric nitric oxide for altitudes between 30 and 50 km at mid-latitudes. These results, when combined with profiles measured by an earlier version of the instrument, cover all four seasons and provide a more comprehensive picture of upper stratospheric nitric oxide than has been available previously. At the highest altitudes studied, the vertical gradient in mixing ratio displays positive and negative values during different observations, with the largest values tending to appear at the greatest heights in summer. Examination of the differences among the profiles, which exceed a factor of 3 near the stratopause, suggests that they arise from the action of transport processes which carry air into the mid-latitude upper stratosphere from regions of the atmosphere that contain widely different odd-nitrogen abundances.

Harvath, J. J.↗
NASA NTRS1984

A measurement of stratospheric HO2 by ground-based millimeter-wave spectroscopy

Stratospheric perhydroxyl (HO2) was measured by using a sensitive mm-wave receiver to obtain spectroscopic line profiles of three rotational emission lines in the vicinity of 265.8 GHz. The observations were carried out over four days in September-October 1982 at Mauna Kea, Hawaii and yield good agreement with the column density and vertical distribution predicted above 35 km by three representative two-dimensional photochemical models employing JPL 82-57 reaction rates and chemistry. Contrasts between current theoretical predictions and previous observations by Anderson et al. (1981) are pointed out for HO2 in the 28 to 37-km range, along with the difficulty of joining the latter with the present measurements through a monotonically varying vertical profile for HO2. A possible explanation involving strong temporal and spatial variation in stratospheric water vapor content is suggested.

De Zafra, R. L.↗
NASA NTRS1984

Measurements of stratospheric NO2 from the Solar Mesosphere Explorer satellite. I - An overview of the results

The visible light spectrometer on board the Solar Mesosphere Explorer spacecraft measures stratospheric NO2 in the 20-40 km altitude region and provides accurate daytime NO2 density profiles with nearly complete latitudinal coverage over an extended period of time. The instrument and data analysis are discussed in detail, and NO2 results for winter/spring 1982 are presented and compared to current theoretical models. Agreement with other measurements is good, and comparison with NOx models indicates that although the overall agreement is acceptable, improvements in the models are required before good agreement is reached at all latitudes. The data indicate that NO2 has a strong memory of the physical conditions present in the stratosphere over a time period of several days.

Mount, G. H.↗
NASA NTRS1984

In situ measurement of stratospheric nitric oxide using a balloon-borne tunable diode laser spectrometer

The stratospheric mixing ratio of nitric oxide at an altitude of 36 km has been measured using a balloon-borne tunable diode laser (TDL) instrument operating in the 5.2-micron wavelength region. Currently the instrument operates with two TDLs, and the capability exists to measure four stratospheric species simultaneously: NO, NO2, O3, and H2O. During the NO measurements reported here, the second TDL operating near 6.2 microns was used to monitor water vapor concentration in the vicinity of the gondola by observing the 1889.57 per cm line absorption in the reference channel path length (1 m).

Webster, C. R.↗
NASA NTRS1984

Diurnal variation of stratospheric chlorine monoxide - A critical test of chlorine chemistry in the ozone layer

Ground-based observations of a mm-wave spectral line at 278 GHz have yielded stratospheric chlorine monoxide column density diurnal variation records which indicate that the mixing ratio and column density of this compound above 30 km are about 20 percent lower than model predictions based on 2.1 parts/billion of total stratospheric chlorine. The observed day-to-night variation is, however, in good agreement with recent model predictions, both confirming the existence of a nighttime reservoir for chlorine and verifying the predicted general rate of its storage and retrieval.

Solomon, P. M.↗
NASA NTRS1984

Measurements of stratospheric bromine

From 1974 to 1977, molecules containing acidic bromine were sampled in the stratosphere by using tetrabutyl ammonium hydroxide impregnated filters. Sampling was accomplished by WB-57F aircraft and high-altitude balloons, spanning latitudes from the equator to 75 deg N and altitudes up to 36.6 km. Analytical results are reported for 4 years of measurements and for laboratory simulations that determined the filter collection efficiencies for a number of brominated species. Mass mixing ratios for the collected bromine species in air average about 27 pptm in the stratosphere. Seasonal variability seems to be small.

Sedlacek, W. A.↗
NASA NTRS1984

Stratospheric ozone changes during the first year of SBUV observations

Synoptic analyses of solar backscattered ultraviolet (SBUV) ozone data have been performed on a daily basis for the first year of Nimbus 7 operation, November 1978 through October 1979, at the standard pressure levels: 30, 10, 5, 2, 1, and 0.4 mbar. By combining these data with the daily NMC meteorological analyses of temperature and geostrophic wind at the same levels, elements of the ozone-temperature relationship as well as the horizontal eddy transports are examined. In particular, the existence of an upper stratospheric high-latitude ozone minimum in winter is discussed, and the eddy fluxes are found to play a significant role in this feature, mainly associated with stratospheric warming pulses. At the same time, monthly average quantities are examined, and standing eddy components are related.

Nagatani, R. M.↗
NASA NTRS1983

Stratospheric species measurements with tunable diode laser absorption spectroscopy

A balloon-borne instrument for stratospheric research has been developed with the capability to simultaneously measure several chemically related species in situ, for a full diurnal cycle. The instrument utilizes tunable infrared diode lasers (TDLs) to provide the radiation in selected wavelength regions for sensitive absorption spectroscopy over a one-km round-trip path. The TDL radiation is directed to a remote retroreflector which is lowered 500 m below the instrument gondola. A HeNe laser and co-aligned TV camera with CID imaging are used for retroreflector tracking. Currently the instrument operates with two TDLs, and the capability exists to measure four stratospheric species: NO, NO2, O3, and H2O. The number of operating TDLs can be expanded to four, resulting in the possibility of measuring several additional trace species.

Menzies, R. T.↗
NASA NTRS1984

Sulphur-rich volcanic eruptions and stratospheric aerosols

Data from direct measurements of stratospheric optical depth, Greenland ice-core acidity, and volcanological studies are compared, and it is shown that relatively small but sulfur-rich volcanic eruptions can have atmospheric effects equal to or even greater than much larger sulfur-poor eruptions. These small eruptions are probably the most frequent cause of increased stratospheric aerosols. The possible sources of the excess sulfur released in these eruptions are discussed.

Rampino, M. R.↗
NASA NTRS1984

A model of the radiative properties of the El Chichon stratospheric aerosol layer

An accurate multiple-scattering model has been employed to examine the effect of an aerosol layer at 25 mb, corresponding to the El Chichon observations, on the reflection, transmission and absorption of radiation by the stratosphere as a function of latitude, optical thickness and aerosol size distribution. Results are presented and parameterized for each of two wavelength intervals in the shortwave region and 17 wavelength intervals in the longwave region for three models of the aerosol size distribution. They include one model representing the unperturbed stratospheric aerosol plus two models based on measurements of the El Chichon aerosol size distribution. In addition to models of the radiative properties of the aerosol layer, a simple model of the latitudinal distribution of aerosol optical thickness as a function of time is developed, based on diffusive transport in latitude and exponential decay in time. These parameterizations for solar and infrared radiation, together with the dispersion model, permit climate models to account for the evolution of an aerosol size distribution from post-volcanic conditions to background conditions.

King, M. D.↗
NASA NTRS1984

Utilization of SAGE aerosol profiles in the analysis of Mauna Loa stratospheric lidar data

A systematic approach to analyzing lidar data collected at NOAA's Mauna Loa Observatory (MLO) was developed which relies on parameters derived from SAGE satellite extinction profile measurements to verify boundary conditions applied to analysis. The approach also provides a means of assessing the uncertainties associated with the various inputs, so that the accuracy of the analysis of the MLO lidar data is available. The stratosphere during the 1980 to 1981 period was only mildly perturbed and could be easily represented by the SAMII/SAGE background aerosol model. The MLO lidar observations collected during this period provided stratospheric optical depths with uncertainties ranging between 15% and 25%. Uncertainties in the aerosol optical model contribute errors of 3% to 4% in the computed optical depths. Most of the optical depth uncertainty is associated with the calibration assumption in which no marked improvement can be expected.

Fernald, F. G.↗
NASA NTRS1985

Measurement of Elements in the Stratosphere

Balloon-borne winch system; stratospheric free radicals; stratospheric sounding; copper vapor lasers; ozone measurement; NO2 analysis; chlorine chemistry; trace elements; and ClO observations are discussed.

Anderson, J. G.↗
NASA NTRS1984

Numerical experiments with a general circulation model concerning the distribution of ozone in the stratosphere

The distribution of ozone below 60 km altitude has been simulated in two experiments employing a nine-layer quasi-geostrophic spectral model and linear parameterization of ozone photochemistry, the first of which included thermal and orographic forcing of the planetary scale waves, while the second omitted it. The first experiment exhibited a high latitude winter ozone buildup which was due to a Brewer-Dodson circulation forced by large amplitude (planetary scale) waves in the winter lower stratosphere. Photochemistry was also found to be important down to lower altitudes (20 km) in the summer stratosphere than had previously been supposed.

Kurzeja, R. J.↗
NASA NTRS1984

An upper limit for stratospheric hydrogen peroxide

It has been postulated that hydrogen peroxide is important in stratospheric chemistry as a reservoir and sink for odd hydrogen species, and for its ability to interconvert them. The present investigation is concerned with an altitude dependent upper limit curve for stratospheric hydrogen peroxide, taking into account an altitude range from 21.5 to 38.0 km for January 23, 1983. The data employed are from balloon flight No. 1316-P, launched from the National Scientific Balloon Facility (NSBF) in Palestine, Texas. The obtained upper limit curve lies substantially below the data reported by Waters et al. (1981), even though the results are from the same latitude and are both wintertime measurements.

Chance, K. V.↗
NASA NTRS1985

Detection of atomic oxygen and further line assignments in the far-infrared stratospheric spectrum

Recent progress in high-resolution measurement of sub-millimeter and far-infrared emission in the stratosphere is reviewed. Attention is given to the results of recent balloon measurements of the minor stratospheric constituents in the spectral range 40-190 per cm. Emission spectra are presented for HCl; HF; and OH. Emission spectra were also obtained for atomic oxygen; hydrobromic acid; and hydroperoxyl radical. The possibility of detecting HO2 and H2O2 in the far-infrared is also briefly discussed.

Carli, B.↗
NASA NTRS1984

A balloon-borne microwave limb sounder for stratospheric measurements

The balloon-borne microwave limb sounder (BMLS) measures atmospheric thermal emission from millimeter wavelength spectral lines to determine vertical profiles of stratospheric species. The instrument flown to date operates at 205 GHz to measure ClO, O3, and H2O2. A 63 GHz radiometer will be added to test the technique for determining tangent point pressure from the MLS experiment on the upper atmosphere research satellite (UARS). Many additional species could also be measured by the BMLS. A radiometer at 270 GHz would provide measurements of HO2, NO2, HNO3, N2O, O-16O-18O-16, and HCN. With this addition, the BMLS can test the current theory of O3 photochemical balance in the upper stratosphere.

Waters, J. W.↗