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All sources NASA NTRS DOE OSTI

DOE OSTI2025

Solid-state platform for cooperative quantum dynamics driven by correlated emission

While traditionally regarded as an obstacle to quantum coherence, recent breakthroughs in quantum optics have shown that the dissipative interaction of a qubit with its environment can be leveraged to protect quantum states and synthesize many-body entanglement. Inspired by this progress, here we set the stage for the—as yet uncharted—exploration of analogous cooperative phenomena in hybrid solid-state platforms. We develop a comprehensive formalism for the quantum many-body dynamics of an ensemble of solid-state spin defects interacting with the magnetic field fluctuations of a common solid-state reservoir. Our framework applies to any solid-state reservoir whose fluctuating spin, pseudospin, or charge degrees of freedom generate magnetic fields. To understand whether correlations induced by dissipative processes can play a relevant role in a realistic experimental setup, we apply our model to a qubit array interacting via the spin fluctuations of a ferromagnetic bath. Our results show that the low-temperature collective relaxation rates of the qubit ensemble can display clear signatures of super- and subradiance, i.e., forms of cooperative dynamics traditionally achieved in atomic ensembles. We find that the solid-state analog of these cooperative phenomena is robust against spatial disorder in the qubit ensemble and thermal fluctuations of the magnetic reservoir, providing a route for their feasibility in near-term experiments. Finally, our work lays the foundation for a multiqubit approach to quantum sensing of solid-state systems and the direct generation of many-body entanglement in spin-defect ensembles. Furthermore, we discuss how the tunability of solid-state reservoirs opens up novel pathways for exploring cooperative phenomena in regimes beyond the reach of conventional quantum optics setups.

NV centers↗

DOE OSTI2022

On the theory of nonhomogeneous nonequilibrium superconductivity in 2D systems with massless fermions

Here we analyze static and nonequilibrium superconducting properties of a 2D relativistic-like model system with local electron-electron interaction, Rashba spin-orbit interaction αR in presence of time-dependent in-plane magnetic field H(t). It is shown that similar to the 2D case with ordinary massive quasiparticle dispersion ε(k)~|k| 2 at large fields, such a system demonstrates a nonhomogeneous superconducting stripe phase with the order parameter Δ(r)=Δ(0)cos(2[μ B B×r]n/$\hbarυ_F$) (B is the magnetic induction, υF is the Fermi velocity, n is the normal to the plane, μ B is the Bohr magneton, and αR$\ll$υF) where the stripes are oriented along the B direction. In the considered system, the inter-stripe period L and the magnitude of the magnetic field B are related by a universal relation BL=$\hbarυ_F$/μ B ≃0.714∙10 -4 Tm. Contrary to the case of massive quasiparticles, where the condition α R ~υ F can be, in principle, satisfied by increasing α R or by charge doping (Fermi velocity decreasing), in a relativistic-like system, where υF is doping-independent and one-two orders of magnitude larger than typical Fermi velocity in the “standard” 2D systems, the stripe phase can be the ground state at a rather low doping level. We also analyzed the nonequilibrium properties of the system with a focus on the melting of the stripe order (when the magnetic field is quenched to a lower value) and stripe dynamics (when the field is rotated by 90° degrees) and found several notable results. In particular, it was shown that the stripe domains melt according to law R~1$\sqrt{t}$ at initial times, while at longer times they shrink exponentially. In the case of the flipped magnetic field, the stripe orientation gradually turns from x- to y-direction, and the intermediate “crossed-stripe” phase takes place during times of order of picoseconds. Such a crossed phase is built of periodic superconducting bubbles that potentially may have applications in modern ultrafast superconducting technologies.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

DOE OSTI2022

Determination of Multimode Motional Quantum States in a Trapped Ion System

Trapped atomic ions are a versatile platform for studying interactions between spins and bosons by coupling the internal states of the ions to their motion. Measurement of complex motional states with multiple modes is challenging, because all motional state populations can only be measured indirectly through the spin state of ions. Here we present a general method to determine the Fock state distributions and to reconstruct the density matrix of an arbitrary multimode motional state. Further, we experimentally verify the method using different entangled states of multiple radial modes in a five-ion chain. This method can be extended to any system with Jaynes-Cummings-type interactions.

74 ATOMIC AND MOLECULAR PHYSICS↗

DOE OSTI2023

Decay rates of almost strong modes in Floquet spin chains beyond Fermi's Golden Rule

The stability and dynamics of almost strong zero and π modes in weakly nonintegrable Floquet spin chains are investigated. Such modes can also be viewed as localized Majorana modes at the edge of a topological superconductor. Perturbation theory in the strength of integrability breaking interaction J z is employed to estimate the decay rates of these modes, and compared to decay rates obtained from exact diagonalization. Here, the structure of the perturbation theory and thus the lifetime of the modes is governed by the conservation of quasienergy modulo 2π/T, where T is the period of the Floquet system. If there are 4n – 1 bulk excitations whose quasienergies add up to zero (or π/T for a π mode), one obtains a decay channel of the Majorana mode with a decay rate proportional to $J$$^{2n}_{z}$. Thus the lifetime is sensitively controlled by the width of the single-particle Floquet bands. For regimes where the decay rates are quadratic in J z , an analytic expression for the decay rate in terms of an infinite temperature autocorrelation function of the integrable model is derived, and shown to agree well with exact diagonalization.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

NASA NTRS2020

Timing of the Accreting Millisecond Pulsar IGR J17591-2342: Evidence of Spin-down during Accretion

We report on the phase-coherent timing analysis of the accreting millisecond X-ray pulsar IGR J17591–2342, using Neutron Star Interior Composition Explorer (NICER) data taken during the outburst of the source between 2018 August 15 and 2018 October 17. We obtain an updated orbital solution of the binary system. We investigate the evolution of the neutron star spin frequency during the outburst, reporting a refined estimate of the spin frequency and the first estimate of the spin frequency derivative ( ˙ν ∼ −7 × 10−14 Hz s−1), confirmed independently from the modelling of the fundamental frequency and its first harmonic. We further investigate the evolution of the X-ray pulse phases adopting a physical model that accounts for the accretion material torque as well as the magnetic threading of the accretion disc in regions where the Keplerian velocity is slower than the magnetosphere velocity. From this analysis we estimate the neutron star magnetic field Beq = 2.8(3) × 108 G. Finally, we investigate the pulse profile dependence on energy finding that the observed behaviour of the pulse fractional amplitude and lags as a function of energy is compatible with the down-scattering of hard X-ray photons in the disc or the neutron star surface.

A Sanna↗

NASA NTRS1976

Cost competitive space transportation system for geostationary payloads

A geostationary satellite system designer will have a number of launch vehicles to consider in the system designs for the 1980s. The Space transportation System (the shuttle orbiter plus upper stage) offers the opportunity for lower system cost in comparison with the expendable launch vehicles. An analysis of a spin stabilized solid rocket motor stage has demonstrated the feasibility of this upper stage concept. A cost competitive Space Transportation System (STS) for geostationary payloads is made possible by achievement of the STS cost goals, multiple launch from the STS orbiter, and a user-provided spin stabilized upper stage.

Jones, C. R.↗

DOE OSTI2026

One-Step Relativistic Driven Similarity Renormalization Group Multireference Perturbation Theory

We present an efficient implementation of a one-step relativistic second-order multireference perturbation theory based on the multireference driven similarity renormalization group (MR-DSRG) using the exact two-component (X2C) Hamiltonian, which we denote X2C-DSRG-MRPT2. We show that the X2C-DSRG-MRPT2 method can accurately capture spin–orbit coupling (SOC) effects in the electronic structure of strongly correlated systems containing elements across the periodic table. We further demonstrate that the X2C-DSRG-MRPT2 method, through its variational treatment of SOC effects, can yield spin–orbit splittings with mean absolute percentage errors consistently below 7% with respect to experimental values for systems containing up to sixth row elements. With its modest computational scaling (fourth power in system size for the perturbative step) and high accuracy, X2C-DSRG-MRPT2 provides a promising avenue for the routine treatment of relativistic effects in strongly correlated molecular systems.

Hamiltonians↗

DOE OSTI2021

String Phase in an Artificial Spin Ice

Abstract One-dimensional strings of local excitations are a fascinating feature of the physical behavior of strongly correlated topological quantum matter. Here we study strings of local excitations in a classical system of interacting nanomagnets, the Santa Fe Ice geometry of artificial spin ice. We measured the moment configuration of the nanomagnets, both after annealing near the ferromagnetic Curie point and in a thermally dynamic state. While the Santa Fe Ice lattice structure is complex, we demonstrate that its disordered magnetic state is naturally described within a framework of emergent strings. We show experimentally that the string length follows a simple Boltzmann distribution with an energy scale that is associated with the system’s magnetic interactions and is consistent with theoretical predictions. The results demonstrate that string descriptions and associated topological characteristics are not unique to quantum models but can also provide a simplifying description of complex classical systems with non-trivial frustration.

36 MATERIALS SCIENCE↗

DOE OSTI2024

Photo-induced non-collinear interlayer RKKY coupling in bulk Rashba semiconductors

Abstract The interplay between light-matter, spin-orbit, and magnetic interactions allows the investigation of light-induced magnetic phenomena that are otherwise absent without irradiation. We present our analysis of light-driven effects on the interlayer exchange coupling mediated by a bulk Rashba semiconductor in a magnetic multilayer. The collinear magnetic exchange coupling mediated by the photon-dressed spin-orbit coupled electrons of BiTeI develops light-induced oscillation periods and displays new decay power laws, both of which are enhanced with an increasing light-matter coupling. For magnetic layers with non-collinear magnetization, we find a non-collinear magnetic exchange coupling uniquely generated by light-driving of the multilayer. As the non-collinear magnetic exchange coupling mediated by the photon-dressed electrons of BiTeI is unique to the irradiated system and it is enhanced with increasing light-matter coupling, this effect offers a promising platform of investigation of light-driven effects on magnetic phenomena in spin-orbit coupled systems. In this platform, light properties, such as its intensity, can serve as external knobs for inducing non-collinear couplings of the interlayer exchange and for modulating the collinear couplings. Both of these effects signify the photo-generated modification in the spin textures of spin-orbit coupled electrons in BiTeI.

Physics↗

DOE OSTI2022

Nematic superconductivity in a one-dimensional system of massless fermions

The superconducting properties of the one-dimensional model of “relativistic” fermions with attraction generated by antiferromagnetic (Heisenberg) pair superexchange spin interaction are studied. Namely, we demonstrate that such a pairing in this system takes place in the nematic channel, with extended s-wave symmetry, where the attraction between fermions mostly takes place when the fermions occupy the nearest sites. It is demonstrated, that the zero-temperature properties of such a system are rather different from the “standard” case of superconductivity with local attraction. For instance, the order parameter has an unusual helical momentum dependence, ∼e −ika ⁠, where a is the lattice parameter and the dependence of the gap on doping has a bell shape, qualitatively similar to cuprate high-T c superconductors. Finally, the smooth transition from the overlapping pair to the local pair regime (or BCS–BEC crossover) in the nematic phase takes place at much lower values of doping as compared to the local pairing case, i.e., the “relativistic 1D” nematic superconductor is much less “friendly” to the local pairs. In conclusion, we also discuss the possible relation of the properties of this model to the superconducting properties of twisted graphene.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

NASA NTRS1974

Automatic spacecraft detumbling by internal mass motion

In the operation of future manned space vehicles, there will always be a finite probability that an accident will occur which results in uncontrolled tumbling of a craft. Hard docking by a manned rescue vehicle is not acceptable because of the hazardous environment to which rescue crewmen would be exposed and excessive maneuvering accelerations during docking operations. A movable-mass control concept, which is activated upon initiation of tumbling and is autonomous, can convert tumbling motion into simple spin. The complete equations of motion for an asymmetric rigid spacecraft containing a movable mass are presented, and appropriate control law and system parameters are selected to minimize kinetic energy, resulting in simple spin about the major principal axis. Simulations indicate that for a large space station experiencing a collision, which results in tumbling, a 1% movable mass is capable of stabilizing motion in 2 hr.

Edwards, T. L.↗

NASA NTRS1988

A spin and deployment mechanism

The spin ejector was developed as a simple and reliable mechanism to spin and deploy small payloads from an Earth orbiting platform. It is one component of a complete system for retaining a payload during vehicle ascent, releasing the payload for deployment, deploying the payload, and securing the payload canister after deployment. The complete system was designed, fabricated and qualified for flight in just over a year, with the flight article delivered to the launch site in October 1987. The complete system is briefly described, and then the focus in on the deployment mechanism (spin ejector) design concept and test program.

Preston, David W.↗

DOE OSTI2023

Optically Active Spin Defects in Few-Layer Thick Hexagonal Boron Nitride

Optically active spin defects in hexagonal boron nitride (hBN) are promising quantum systems for the design of two-dimensional quantum sensing units offering optimal proximity to the sample being probed. In this Letter, we first demonstrate that the electron spin resonance frequencies of boron vacancy centers ($V$$^{–}_{B}$) can be detected optically in the limit of few-atomic-layer thick hBN flakes despite the nanoscale proximity of the crystal surface that often leads to a degradation of the stability of solid-state spin defects. We then analyze the variations of the electronic spin properties of $V$$^{–}_{B}$ centers with the hBN thickness with a focus on (i) the zero-field splitting parameters, (ii) the optically induced spin polarization rate and (iii) the longitudinal spin relaxation time. Furthermore, this Letter provides important insights into the properties of $V$$^{–}_{B}$ centers embedded in ultrathin hBN flakes, which are valuable for future developments of foil-based quantum sensing technologies.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

NASA NTRS1977

Fluid interaction with spinning toroidal tanks

An experimental study was conducted to evaluate propellant behavior in spinning torroidal tanks that could be used in a retropropulsion system of an advanced outer-planet Pioneer orbiter. Information on propellant slosh and settling and on ullage orientation and stability was obtained. The effects of axial acceleration, spin rate, spin-rate change, and spacecraft wobble, both singly and in combination, were evaluated using a one-eighth scale transparent tank in one-g and low-g environments. Liquid loadings ranged from 5% to 96% full. The impact of a surface tension acquisition device was assessed by comparison with bare-tank results. The testing simulated the behavior of the fluorine/hydrazine and nitrogen textroxide/monomethylhydrazine propellants. Results are presented that indicate that no major fluid behavior problems would be encountered with any of the four propellants in the toroidal tanks of a spin-stabilized orbiter spacecraft.

Fester, D. A.↗

DOE OSTI2025

Spin Squeezing with Itinerant Magnetic Dipoles

Entanglement can improve the measurement precision of quantum sensors beyond the shot noise limit. Neutral atoms, the basis of some of the most precise and accurate optical clocks and interferometers, do not naturally exhibit the all-to-all interactions traditionally used to generate such entangled states. On the other hand, these systems exhibit exceedingly high degrees of experimental control over parameters such as temperature, spatial entropy, and itinerancy. In this work, we investigate spin squeezing in a highly coherent itinerant system of neutral atoms with magnetic dipole-dipole interactions. We achieve 7.1 dB of metrologically useful squeezing using finite-range spin-exchange interactions in an erbium quantum gas microscope, and we demonstrate that introducing atomic motion, realizing a dipolar 𝑡−𝐽 model, protects the spin sector coherence at low fillings, significantly improving the achievable spin squeezing in a 2D dipolar system. This work’s protocol can be implemented with most neutral atoms, opening the door to quantum-enhanced metrology in other itinerant dipolar systems, such as molecules or optical lattice clocks, and serves as a novel method for studying itinerant quantum magnetism with long-range interactions.

Atomic, optical & lattice clocks↗

DOE OSTI2026

Dynamical correlations and nonequilibrium sum rules in photodoped Hubbard ladders

Using matrix product state techniques we study the nonequilibrium dynamical response of the half-filled Hubbard ladder when subject to an optical pump. Optical pumping offers a way of producing and manipulating new strongly correlated phenomena by suppressing existing magnetic correlations. The ladder allows the effects of pump directionality to be investigated, and compared to a single chain it has strong spin-charge coupling and a fully gapped excitation spectrum, promising different nonequilibrium physics. We compute time-dependent correlations, including the nonequilibrium dynamical structure factors for spin and charge. By deriving a combined spin-charge sum rule that applies both in and out-of-equilibrium, we show that spectral weight is pumped directly from the antiferromagnetic spin response into a low energy 𝜔 ∼ 0 charge response below the Mott gap. The transfer of weight is pump direction dependent: pumping directed along the legs disrupts magnetic correlations more than pumping in the rung-direction, even if the post-pump energy density is similar. The charge correlation length is dramatically enhanced by the pump, whilst the spin correlations are most strongly suppressed at nearest- and next-nearest-neighbor spacings. After the pump the system is in a nonthermal correlated metallic state, with gapless charge excitations and approximately equal spin and charge correlation lengths, emphasizing the importance of treating these degrees of freedom on an equal footing in nonequilibrium systems.

36 MATERIALS SCIENCE↗

DOE OSTI2024

Higher-order topological corner and bond-localized modes in magnonic insulators

We theoretically investigate a two-dimensional decorated honeycomb lattice framework to realize a second-order topological magnon insulator (SOTMI) phase featuring distinct corner-localized modes. Here, our study emphasizes the pivotal role of spin-magnon mapping in characterizing bosonic topological properties, which exhibit differences from their fermionic counterparts. We employ a symmetry indicator topological invariant to identify and characterize this SOTMI phase, particularly for systems respecting time-reversal and rotational symmetry. Using a spin model defined on a honeycomb lattice geometry, we demonstrate that introducing “kekulé” type distortions yields a topological phase. In contrast, “antikekulé” distortions result in a nontopological magnonic phase. The presence of kekulé distortions manifests in two distinct topologically protected bosonic corner modes—an intrinsic and a pseudo, based on the specific edge terminations. On the other hand, antikekulé distortions give rise to Tamm/Shockley type bond-localized boundary modes, which are nontopological and reliant on particular edge termination. We further investigate the effects of random out-of-plane exchange anisotropy disorder on the robustness of these bosonic corner modes. The distinction between SOTMIs and their fermionic counterparts arises due to the system-specific magnonic onsite energies, a crucial feature often overlooked in prior literature. Our study unveils exciting prospects for engineering higher-order topological phases in magnon systems and enhances our understanding of their unique behavior within decorated honeycomb lattices.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

DOE OSTI2025

Diagrammatic Monte Carlo Approach to Real‐frequency Response Functions and the Spin‐Fermion Model of Hot Spots (Final Report)

This three‐year research project was focused on two outstanding condensed matter problems (i) Real‐frequency response functions in Coulomb systems at finite temperature, and Fermi surface (FS) reconstruction in the Spin-Fermion (SF) model. The uniform electron gas (jellium) model, describing electrons interacting via long‐range Coulomb forces on positive neutralizing background, is fundamentally important both for understanding the physics of correlated electrons and for formulation of the time‐dependent density functional theory (TDDFT). The spin-fermion model has found a wide range of applications in the physics of cuprates and iron‐based superconductors to explain the “strange metal" behavior and to suggest a possible pairing mechanism for high‐temperature superconductivity. The project’s goals were development and application of the Diagrammatic Monte Carlo (DiagMC) techniques for solving the above problems.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗