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At least 1,189 records · Page 66

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DOE OSTI2021

An Efficient Bifunctional Air Electrode for Reversible Protonic Ceramic Electrochemical Cells

One of the main bottlenecks that limits the performance of reversible protonic ceramic electrochemical cells (R-PCECs) is the sluggish kinetics of the oxygen reduction and evolution reactions (ORR and OER). Here, the significantly enhanced ORR and OER kinetics and stability of a conventional La 0.6 Sr 0.4 Co 0.2 Fe 0.8 O 3-δ (LSCF) air electrode by an efficient catalyst coating of barium cobaltite (BCO) is reported. The polarization resistance of a BCO-coated LSCF air electrode at 600 oC is 0.16 Ω cm 2 , about 30% of that of the bare LSCF air electrode under the same conditions. Further, a R-PCEC with the BCO-coated LSCF air electrode shows exceptional performance in both fuel cell (maximum power density of 1.16 W cm -2 at 600 ºC) and electrolysis (current density of 1.80 A cm -2 at 600 ºC at 1.3 V) modes. Finally, the performance enhancement is attributed mainly to the facilitated rate of oxygen surface exchange.

32 ENERGY CONSERVATION, CONSUMPTION, AND UTILIZATI↗

DOE OSTI2022

Enabling Extreme Fast-Charging: Challenges at the Cathode and Mitigation Strategies

We report charging lithium-ion batteries (LiBs) in 10 to 15 min via extreme fast-charging (XFC) is important for the widespread adoption of electric vehicles (EVs). Lately, the battery research community has focused on identifying XFC bottlenecks and determining novel design solutions. Like other LiB components, cathodes can present XFC bottlenecks, especially when considering long-term battery life. Therefore, it is necessary to develop a comprehensive understanding of how XFC conditions degrade LiB cathodes. The present article reviews relevant cathode-focused studies and summarizes the current understanding regarding cathode performance and aging issues under XFC conditions. Dominant aging modes and mechanisms are identified at different length-scales with electrochemical correlations for LiNi x Mn y Co z O 2 (NMC)-based cathodes. A range of electrochemical techniques and models provide key insights into cathode performance and life issues. A suite of multimodal and multiscale microscopy and X-ray techniques is surveyed to quantify chemical, structural, and crystallographic NMC-cathode degradation. Cathode cycle-life is scaled to equivalent EV miles to illustrate how cathode degradation translates to real-world scenarios and quantifies cathode-related bottlenecks that hinder XFC adoption. Finally, the article discusses several cathode cycle-life aging mitigation strategies with example case studies and identifies remaining challenges.

25 ENERGY STORAGE↗

DOE OSTI2020

Keratin-derived functional carbon with superior charge storage and transport for high-performance supercapacitors

In this work, we report a scalable method to synthesize hierarchically porous, hetero-atom doped activated carbon nanosheet from waste biomass-human hair, and demonstrates the use of this carbon as an ultra-high performance electrode material for supercapacitor applications. Microscopic analyses reveal that sheet size ranges from 50 to 200 nm having a thickness of 15–27 nm. As-synthesized, carbon nanosheets possess a hierarchical porous structure having a specific surface area of 1548 m 2 g -1 . Heteroatom concentration (nitrogen, oxygen, and sulfur) of around 25% is confirmed from XPS analysis. Therefore, the novel interconnected hierarchical porous nanosheets structure enables fast adsorption and transportation of ions during electrochemical processes. Also, the abundant chemically available electroactive heteroatom species in the material enhance the wettability of ions and contribute to pseudocapacitance. The electrochemical analyses through cyclic voltammetry and galvanostatic charge-discharge measurements in 6 M KOH reveal the quasi-EDLC behavior of the activated carbons due to the presence of heteroatoms. A reprensentative KOH activated carbon shows an excellent specific capacitance value of 999 F g -1 at a current density of 1 A g -1 . Furthermore, the symmetrically assembled two-electrode device also delivers a maximum energy density of 32 W h Kg -1 at a power density of 325 W Kg -1 . In addition, excellent cyclic stability of 98% capacitance retention is observed after 10,000 continuous GCD cycles even at a high current density of 5 A g -1 . Symmetric flexible supercapacitor device using KOH-PVA-K3FeCN6 as redox gel polymer electrolyte shows a synergistic specific capacitance of 145 mF cm -1 at a current density of 0.8 mA cm -1 exhibiting very less deviation in bending mode. Therefore, this waste biomass derived heteroatom doped hierarchical porous carbon nanosheets can be a promising material for cost-effective high- performance supercapacitor.

42 ENGINEERING↗

DOE OSTI2020

Simulation of MHD instabilities with fluid runaway electron model in M3D- C 1

Runaway electrons are generated in a tokamak during the start up, during normal operation and during a plasma disruption. During a disruption, runaway electrons can be accelerated to high energies, potentially damaging the first wall. To predict the consequences of runaway generation during a disruption, it is necessary to consider resonant interactions of runaways with the bulk plasma. Here we consider the interactions of runaways on low mode number tearing modes. We have developed a fluid runaway electron model for the 3D MHD code M3D-C1[Jardin,et al. J Comput. Sci Discovery 6 014002 (2012)]. To benchmark, we have reproduced the MHD linear tearing mode results (with runaway electrons) in a circular cylinder presented in previous analytic studies[[Helander, P., et al, Phys. Plasmas 14 144102 (2007)] and extended here with a numerical eigenvalue calculation. Furthermore, we find that the low mode number tearing mode has a rotation caused by the MHD - runaways interaction, and the toroidal current scale length is much smaller with runaways than that for without and decreases as the runaway speed increases.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

DOE OSTI2023

Measurement of the branching fractions for Cabibbo-suppressed decays D + → K + K - π + π 0 and D ( s ) + → K + π - π + π 0 at Belle

We present measurements of the branching fractions for the singly Cabibbo-suppressed decays and , and the doubly Cabibbo-suppressed decay , based on of data recorded by the Belle experiment at the KEKB e + ⁢e - collider. We measure these modes relative to the Cabibbo-favored modes D + → K - ⁢π + ⁢π + ⁢π 0 and D$^{+}_{s}$ → K + ⁢K -⁢ π + ⁢π 0 . Our results for the ratios of branching fractions are $\mathscr{B}$⁡(D + →K + ⁢K -⁢ π + ⁢π 0 )/$\mathscr{B}$⁡(D + → K - ⁢π + ⁢π + ⁢π 0 ) =(11.32±0.13±0.26)%, $\mathscr{B}$⁡(D + →K + π - ⁢π + ⁢π 0 )/$\mathscr{B}$(D + →K -⁢ π + ⁢π + ⁢π 0 ) =(1.68±0.11±0.03)%, and $\mathscr{B}$⁡(D$^{+}_{s}$ → K + ⁢π - π + ⁢π 0 )/$\mathscr{B}$⁡(D$^{+}_{s}$ → K + ⁢K - π + π 0 ) =(17.13±0.62±0.51)%, where the uncertainties are statistical and systematic, respectively. The second value corresponds to (5.83 ±0.42) ×tan 4 ⁡θ C , where θ C is the Cabibbo angle; this value is larger than other measured ratios of branching fractions for a doubly Cabibbo-suppressed charm decay to a Cabibbo-favored decay. Multiplying these results by world average values for $\mathscr{B}$⁡(D + → K - ⁢π + ⁢π + ⁢π 0 ) and $\mathscr{B}$⁡(D$^{+}_{s}$ → K + ⁢K - π + π 0 ) yields $\mathscr{B}$( + →K + ⁢K -⁢ π + ⁢π 0 ) = (7.08±0.08±0.16±0.20)×10 -3 , $\mathscr{B}$⁡(D + → K +⁢ π - π + ⁢π 0 ) =(1.05±0.07±0.02±0.03)×10 -3 , and $\mathscr{B}$⁡(D$^{+}_{s}$ → K + ⁢π - π + ⁢π 0 ) =(9.44±0.34±0.28±0.32)×10 -3 , where the third uncertainty is due to the branching fraction of the normalization mode. The first two results are consistent with, but more precise than, the current world averages. The last result is the first measurement of this branching fraction.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

DOE OSTI2024

Photonic Crystal Surface Emitting GaSb-Based Type-I Quantum Well Diode Lasers

The GaSb-based epitaxially regrown monolithic diode PCSELs operating near 2 μm at room temperature in continuous wave regime and generating 30 mW of output power from 200 μm diameter aperture have been designed and fabricated. Here, the devices demonstrated CW threshold current density of about 500 A/cm 2 . The laser output power was enhanced thanks to increased buried void area fill-factor in the photonic crystal layer with multiple voids per unit cell. The PCSEL generated ultra-low divergence donut shape beams at the currents near threshold. At higher injection currents, the device brightness was limited by excitation of the higher order lateral modes. Generation of the vector-vortex beams of different types by different band edge states of the buried photonic crystal was observed.

77 NANOSCIENCE AND NANOTECHNOLOGY↗

DOE OSTI2022

FFTF Acceptance and Startup Testing for GAIN

The Fast Flux Test Facility (FFTF) is the most recent liquid metal reactor (LMR) to be designed, constructed, and operated by the U.S. Department of Energy (DOE). The 400-MWt sodium-cooled, fast-neutron flux reactor plant was designed for irradiation testing of nuclear reactor fuels and materials for liquid metal fast breeder reactors. Following the demise of the breeder reactor program in the United States, FFTF continued to play a key role in providing a test bed for demonstrating performance of advanced fuel designs and demonstrating operation, maintenance, and safety of advanced liquid metal reactors. FFTF operations ceased in April 1992 after a determination by DOE that no combination of proposed missions was financially feasible over a ten-year period. The reactor is currently deactivated and in a long-term surveillance and maintenance (S&M) mode. This report provides information on the extensive and rigorous process that was used to conduct turnover from construction followed by acceptance and startup testing of the FFTF. This paper is in support of the Gateway for Accelerated Innovation in Nuclear (GAIN), which provides the nuclear energy community with access to the technical, regulatory, and financial support necessary to move new or advanced nuclear reactor designs toward commercialization while ensuring the continued safe, reliable, and economic operation of the existing nuclear fleet. The information obtained from the design, startup, and operation of the FFTF provides valuable insight for follow-on reactor projects, such as the Versatile Test Reactor (VTR), in the areas of plant system and component design, component fabrication, fuel design and performance, prototype testing, site construction, reactor startup and operations, and reactor deactivation and decommissioning (D&D). The focus of this report is on the process used to startup the FFTF and to ensure that operations could be conducted efficiently and safely. A reference section is provided of documents detailing the successful turnover and testing process implemented for startup of the reactor and its supporting systems. The documents listed can be retrieved upon request and are believed useful for future reactor startup endeavors.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

DOE OSTI2022

High-Efficiency Quantum Dot Lasers as Comb Sources for DWDM Applications

The trend of data center transceivers is to increase bandwidth while simultaneously decreasing their size, power consumption, and cost. While data center links have previously relied on vertical-cavity surface-emitting lasers (VCSELs) or in-plane lasers using coarse wavelength division multiplexing (WDM) to encode data, recently, dense WDM (DWDM) has moved to the forefront for next-generation links. Several approaches exist as light sources for DWDM links; DFB arrays, nonlinear microcombs, and semiconductor mode-locked lasers (MLLs). This paper focuses on quantum dot MLLs (QDMLLs), which currently offer the best efficiency, simplicity, and size. The efficiency of optical combs generated by QDMLLs is analyzed in depth in this study.

Dumont, Mario (ORCID:000000023956612X)↗

NASA NTRS1971

Nonvolatile read/write memory element - A concept

Bidirectional MOS driver, integrated with diode matrix reduces fuse read current to only that of junction leakage and transient MOS gate charging current. No current, except junction leakage current, flows in unaddressed cells. Current required to drive MOS gate flows through unfused branch only during read mode.

Cricchi, J. R.↗

NASA NTRS1972

Comets: Scientific data and missions; Proceedings of the Tucson Comet Conference, University of Arizona, Tucson, Ariz., April 8, 9, 1970.

Current knowledge of comets is surveyed, and comet-rendezvous mission constraints, opportunities, modes, and spacecraft capabilities are discussed. Attention is given to cometary nuclei, infrared measurements of comets, the nature and origin of the cometary head, L-alpha photometry of Comet Bennett, Types I and II tails, comet spectra and orbits, and evidence from stream meteoroids. Some scientific criteria for a cometary mission are considered. Individual items are announced in this issue.

Kuiper, G. P.↗

NASA NTRS1980

Absolute line strengths in nu4, /C-12/H4 - A dual-beam diode laser spectrometer with sweep integration

A tunable diode laser spectrometer with several unique features has been developed for use in the middle IR. The all-reflective optical system has a dual-beam configuration before the dispersive mode selector to eliminate transit-angle errors at the calibration etalon. By maintaining separated beams through the mode selector, beam combiner losses are avoided. Averaging successive sweeps of the current-modulated laser permits stable reproducible spectral integrations, eliminating etalon thermal errors and producing high photometric sensitivity. Line strengths have been measured using this instrument for eleven transitions in nu4 of (C-12)H4. These include R0 and R1 and nine P-branch transitions in the 1202-1263-per cm range. Techniques for measuring strengths with a diode laser are discussed.

Jennings, D. E.↗

NASA NTRS1984

Characteristics of a microwave plasma disk ion source

This letter describes an ion source using a cylindrical microwave cavity operating in a hybrid mode associated with the TE(211) empty cavity mode. The design principles and associated electrical systems are also discussed. Extracted beam current versus accelerating voltage, and specific energy versus extracted beam current are displayed over the range of flow rates 20-80 sccm and absorbed powers 80-150 W. The results show the feasibility of this concept. The ion source has many potential uses such as space propulsion, material processing, and neutral beam ion sources.

Asmussen, J.↗

NASA NTRS1985

Atmospheric refractivity corrections in satellite laser ranging

Atmospheric refraction can cause significant errors in satellite laser ranging (SLR) systems. There are two techniques which can be used to correct for these errors. Atmospheric models based upon surface measurements of pressure, temperature, and relative humidity have been shown by ray tracing to be accurate to within a few centimeters at 20 deg elevation angle. The residual errors in the models are thought to be primarily caused by horizontal gradients in the refractivity. Although models have been developed to predict the gradient effects, initial studies show that they can be sensitive to local topographic effects. Atmospheric turbulence can introduce random fluctuations in the refractivity, but only introduces centimeter level errors at elevation angles below 10 deg. Pulsed two-color ranging systems can directly measure the atmospheric delay in satellite ranging. These systems require mode-locked multiple-frequency lasers and streak-camera-based receivers and currently appear capable of measuring the atmospheric delay with an accuracy of 0.5 cm or better.

Abshire, J. B.↗

NASA NTRS1987

Control considerations for high frequency, resonant, power processing equipment used in large systems

Addressed is a class of resonant power processing equipment designed to be used in an integrated high frequency (20 KHz domain), utility power system for large, multi-user spacecraft and other aerospace vehicles. It describes a hardware approach, which has been the basis for parametric and physical data used to justify the selection of high frequency ac as the PMAD baseline for the space station. This paper is part of a larger effort undertaken by NASA and General Dynamics to be sure that all potential space station contractors and other aerospace power system designers understand and can comfortably use this technology, which is now widely used in the commercial sector. In this paper, we will examine control requirements, stability, and operational modes; and their hardware impacts from an integrated system point of view. The current space station PMAD system will provide the overall requirements model to develop an understanding of the performance of this type of system with regard to: (1) regulation; (2) power bus stability and voltage control; (3) source impedance; (4) transient response; (5) power factor effects, and (6) limits and overloads.

Mildice, J. W.↗

NASA NTRS1987

Control considerations for high frequency, resonant, power processing equipment used in large systems

Mildice, J. W.↗

NASA NTRS1988

High-resolution detectors for imaging and spectroscopy at ultraviolet and soft X-ray wavelengths

The Multi-Anode Microchannel Arrays (MAMAs) are a family of pulse-counting imaging array detectors designed specifically for astrophysical investigations in space. The MAMAs have a number of unique performance characteristics which make them particularly suitable for imaging and spectroscopy at ultraviolet and soft X-ray wavelengths. First, they employ 'solar blind' photocathodes eliminating the 'red leak' problem associated with solid state arrays such as the CCDs. Second, they operate with zero readout noise, yielding photon-statistics limited signals. Third, they utilize a random readout technique and can determine both the location of a detected photon and also its arrival time to an accuracy of the order of 100 ns. This paper gives an overview of the construction, mode of operation, and performance characteristics of the MAMA detectors and describes the current status of the development program.

Timothy, J. G.↗

NASA NTRS1990

Magnetohydrodynamic modeling of the solar corona

The ideal and resistive magnetohydrodynamic (MHD) model is used to examine the dynamics and structure of the solar corona. When the coronal magnetic field is deformed by photospheric flow it can evolve to states that become unstable to ideal MHD modes. The nonlinear evolution of these instabilities can lead to the generation of current sheets, field line reconnection, and energy release. The disruption of an arcade field and the kinking of coronal loops is described. The braiding of the large-scale coronal field by convective photospheric motions develops fine-scale structure in the magnetic field and leads to the development of intense current filaments. The resistive dissipation of these currents can provide an efficient coronal heating mechanism.

Mikic, Zoran↗

NASA NTRS1990

Formally specifying the logic of an automatic guidance controller

The following topics are covered in viewgraph form: (1) the Penelope Project; (2) the logic of an experimental automatic guidance control system for a 737; (3) Larch/Ada specification; (4) some failures of informal description; (5) description of mode changes caused by switches; (6) intuitive description of window status (chosen vs. current); (7) design of the code; (8) and specifying the code.

Guaspari, David↗