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At least 1,153 records · Page 64
All sourcesNASA NTRSDOE OSTI
NASA NTRS2017

The Footprints of 16 Year Trends of Arctic Springtime Cloud and Radiation Properties on September Sea Ice Retreat

The most prominent September Arctic sea ice decline over the period of 2000–2015 occurs over the Siberian Sea, Laptev Sea, and Kara Sea. The satellite observed and retrieved sea ice concentration (SIC) and cloud/radiation properties over the Arctic (70°–90°N) have been used to investigate the impact of springtime cloud and radiation properties on September SIC variation. Positive trends of cloud fractions, cloud water paths, and surface downward longwave flux at the surface over the September sea ice retreat areas are found over the period of 1 March to 14 May, while negative trends are found over the period of 15 May to 28 June. The spatial distributions of correlations between springtime cloud/radiation properties and September SIC have been calculated, indicating that increasing cloud fractions and downward longwave flux during springtime tend to enhance sea ice melting due to strong cloud warming effect. Surface downward and upward shortwave fluxes play an important role from May to June when the onset of sea ice melting occurs. The comparison between linearly detrended and nondetrended of each parameter indicates that significant impact of cloud and radiation properties on September sea ice retreat occurs over the Chukchi/Beaufort Sea at interannual time scale, especially over the period of 31 March to 29 April, while strongest climatological trends are found over the Laptev/Siberian Sea.

Arctic sea ice trend↗
NASA NTRS2012

Climate Impacts of Ice Nucleation

Several different ice nucleation parameterizations in two different General Circulation Models (GCMs) are used to understand the effects of ice nucleation on the mean climate state, and the Aerosol Indirect Effects (AIE) of cirrus clouds on climate. Simulations have a range of ice microphysical states that are consistent with the spread of observations, but many simulations have higher present-day ice crystal number concentrations than in-situ observations. These different states result from different parameterizations of ice cloud nucleation processes, and feature different balances of homogeneous and heterogeneous nucleation. Black carbon aerosols have a small (0.06 Wm(exp-2) and not statistically significant AIE when included as ice nuclei, for nucleation efficiencies within the range of laboratory measurements. Indirect effects of anthropogenic aerosols on cirrus clouds occur as a consequence of increasing anthropogenic sulfur emissions with different mechanisms important in different models. In one model this is due to increases in homogeneous nucleation fraction, and in the other due to increases in heterogeneous nucleation with coated dust. The magnitude of the effect is the same however. The resulting ice AIE does not seem strongly dependent on the balance between homogeneous and heterogeneous ice nucleation. Regional effects can reach several Wm2. Indirect effects are slightly larger for those states with less homogeneous nucleation and lower ice number concentration in the base state. The total ice AIE is estimated at 0.27 +/- 0.10 Wm(exp-2) (1 sigma uncertainty). This represents a 20% offset of the simulated total shortwave AIE for ice and liquid clouds of 1.6 Wm(sup-2).

Gettelman, Andrew↗
DOE OSTI2022

High concentrations of ice: Investigations using polarimetric radar observations combined with in situ measurements and cloud modeling (Final Report)

This DOE-funded joint project had the over-arching goal of understanding the reasons for observed size distributions of ice particles in cold clouds. Its approach involves the use of cloud models and field observations by radar and aircraft of real storms. The project addresses three major research objectives: (1) Utilize a novel polarimetric radar technique to retrieve size distributions and amounts of ice from radar data collected during the previous DOE ARM field campaigns; (2) Evaluate the results of ice microphysical retrievals using available in situ aircraft measurements and other remote sensors (e.g., vertically pointing cloud radars and wind profilers); (3) Improve the treatment of microphysical processes leading to cloud glaciation and ice multiplication in numerical cloud models. The study was performed by three research organizations: University of Oklahoma, The Hebrew University of Jerusalem, Israel, and Lund University, Sweden. The Israel and Swedish partners were funded by the sub-awards from the University of Oklahoma. Cloud modeling studies have been performed by the research teams at The Hebrew University of Jerusalem (HUJ) and Lund University to identify the origins of high concentrations of cloud ice in areas of high ice water content (HIWC). The Hebrew University Cloud Model (HUCM) with full spectral bin microphysics and the Lund University aerosol-cloud (AC) model with a hybrid bin / bulk microphysics scheme complementing HUCM were utilized for simulations. Both research teams had particular focus on secondary ice production (SIP) as one of the possible sources of enhanced ice concentration. The HUJ group suggested a novel concept of ice multiplication during droplet freezing. It is assumed that splintering and droplet fragmentation during droplet freezing takes place because of dendritic growth within a supercooled drop. The resulting simulations of SIP generated small ice in concentrations exceeding hundreds per liter similar to what was observed in the HIWC regions of the tropical storms. The Lund team explored the SIP mechanisms such as breakup of ice particles due to ice-ice collisions and ice sublimation that are expected to dominate the continental storms. They also quantified the impact of homogeneous nucleation of cloud droplets on the total number concentration of ice at very low temperatures near the tops of the clouds. Additionally, the Lund AC model is able to simulate the effect of aerosols of various types (including biological) on the cloud life cycle and the corresponding ice production. The HUCM / AC model was used to simulate one of the “golden” cases of the DOE MC3E campaign on 20 May 2011. The model output was converted into the fields of polarimetric radar variables using the polarimetric radar forward operator developed at the University of Oklahoma and compared with radar observations and in situ microphysical measurements onboard research aircraft. It was demonstrated that specific differential phase KDP is the best radar parameter to identify the HIWC areas and quantify the corresponding ice parameters. For the first time, the shape of the vertical profile of KDP was realistically reproduced by the cloud model with the KDP maximum in the dendritic growth layer (DGL) centered at the -15°C isotherm. The University of Oklahoma team has developed a methodology for polarimetric radar retrievals of such microphysical parameters of ice as ice water content (IWC), mean volume diameter (Dm), and total number concentration (Nt) of ice particles. These retrievals have been validated using in situ aircraft measurements during 6 field campaigns and proved to be quite robust and reliable. This allowed to build the first climatology of the vertical profiles of polarimetric radar variables and retrieved microphysical parameters for the three types of weather systems: continental MCSs, maritime MCSs, and tropical cyclones / hurricanes (Hu and Ryzhkov 2022). The data were collected by a multitude of the WSR-88D radars in 13 continental and 10 maritime MCSs and 11 landfalling hurricanes. The HIWC areas were identified within the examined storms and the corresponding “HIWC statistics” was compared with the “background” one without HIWC. An overarching conclusion of the study is that maritime tropical storms (MCSs and hurricanes) are characterized by smaller size ice in higher concentration compared to the continental MCSs. High ice water content in the HIWC areas is primarily caused by a strong jump in a number concentration of ice particles rather than the increase of their size compared to the “background” environment. This may point to the homogeneous nucleation of excessive amounts of supercooled droplets and / or secondary ice production as the possible origins of HIWC. Such a climatology provides a good observational reference for the modelers to evaluate the performance of their models. As an example, the in-depth analysis of the 20 May 2011 MC3E case shows that the advanced cloud models developed in the course of this study still tend to underestimate the number concentration of ice in the HIWC areas although they succeed in reproducing realistically looking vertical profiles of IWC and Nt. The results of the project research are summarized in 13 journal papers.

54 ENVIRONMENTAL SCIENCES↗
NASA NTRS2018

An Investigation of Glaciated Cloud Capabilities in the NASA Glenn Icing Research Tunnel

In 2015 the FAA added Appendix D to Part 33 engine certification requirements that included Mixed Phase and Ice Crystal Icing to aircraft engine certification. Replicating the ice crystal environment that is seen in nature has proven to be a challenge, which multiple engine ground testing facilities and icing wind tunnels have achieved to varying degrees. The Icing Research Tunnel (IRT) at NASA Glenn has always been focused on super-cooled liquid water to produce FAA Part 23 and Part 25 regulations, targeting Appendix C and lately also Appendix O. However, due to a growing interest in the field of ice crystals and the high cost of operating engine icing facilities, the IRT staff have recently completed testing using the Multi-Element Sensor (also known as the multi-wire) to measure glaciated cloud conditions. Results indicate that turning off the heat to the nozzle air and water supply can create a stable, fully glaciated cloud in the test section for a small range of conditions: drop-size distribution values below 20 microns (median volumetric diameter), air temperatures as warm as -7 deg C, and airspeeds between 100 and 250 knots. These tests also revealed how varying the total temperature, airspeed, nozzle air pressure, and nozzle water pressure affect the glaciation of the IRT cloud.

ice water content↗
NASA NTRS1997

Ice Nucleation Processes in Upper Tropospheric Wave-Clouds Observed During SUCCESS

We have compared in situ measurements near the leading-edges of wave-clouds observed during the SUCCESS experiment with numerical modeling of ice nucleation. Observations of high supersaturations with respect to ice (\geq 150\%) near the leading edge of a very cold wave cloud (T < --60^\circC) are consistent with recent theoretical and laboratory studies suggesting that large supersaturations are required to homogeneously freeze sulfate aerosols. Also, the peak ice crystal number densities observed in this cloud (about 4cm -3/sup>) are consistent with the number densities calculated in our model. The consistency between model results (using homogeneous freezing and the observations indicates that the number density of effective heterogeneous ice nuclei must be no more than about 2 cm -3 . In the warmer wave-cloud (T (approx.)eq --37^\circC) relatively large ice number densities were observed (20--40 cm -3 . Our model calculations suggest that these large number densities are only possible if liquid droplets were activated at the cloud leading-edge, followed by subsequent homogeneous freezing. If sulfate aerosols had frozen before liquid droplets could be activated, then the peak ice crystal number density should have been less than 10 cm -3 .

Jensen, E. J.↗
NASA NTRS1978

Airborne measurements of cloud forming nuclei and aerosol particles at Kennedy Space Center, Florida

Results of airborne measurements of the sizes and concentrations of aerosol particles, ice nuclei, and cloud condensation nuclei that were taken at Kennedy Space Center, Florida, are presented along with a detailed description of the instrumentation and measuring capabilities of the University of Washington airborne measuring facility (Douglas B-23). Airborne measurements made at Ft. Collins, Colorado, and Little Rock, Arkansas, during the ferry of the B-23 are presented. The particle concentrations differed significantly between the clean air over Ft. Collins and the hazy air over Little Rock and Kennedy Space Center. The concentrations of cloud condensation nuclei over Kennedy Space Center were typical of polluted eastern seaboard air. Three different instruments were used to measure ice nuclei: one used filters to collect the particles, and the others used optical and acoustical methods to detect ice crystals grown in portable cloud chambers. A comparison of the ice nucleus counts, which are in good agreement, is presented.

Radke, L. F.↗
NASA NTRS1993

Comment on porosities of ice films used to simulate stratospheric cloud surfaces

Reference is made to a recent article by Hanson and Ravishankara (HR) containing data on the reaction probabilities of N2O5 and ClONO2 on ice films of varying thickness. In accordance with their interpretation of the observations, no correction for internal diffusion was needed and, thus, by implication, their films were effectively nonporous. Here, it is argued that vapor deposited films can be highly porous and that porous films do not always show a large increase in reactivity or uptake capacity with thickness. It is pointed out that the assumptions made by HR are responsible for the poor fit of their data.

Keyser, Leon F.↗
NASA NTRS2016

The Relationships Between Insoluble Precipitation Residues, Clouds, and Precipitation Over California's Southern Sierra Nevada During Winter Storms

Ice formation in orographic mixed-phase clouds can enhance precipitation and depends on the type of aerosols that serve as ice nucleating particles (INP). The resulting precipitation from these clouds is a viable source of water, especially for regions such as the California Sierra Nevada. Thus, a better understanding of the sources of INP that impact orographic clouds is important for assessing water availability in California. This study presents a multi-site, multi-year analysis of single particle insoluble residues in precipitation samples that likely influenced cloud ice and precipitation formation above Yosemite National Park. Dust and biological particles represented the dominant fraction of the residues (64% on average). Cloud glaciation, determined using GOES satellite observations, not only depended on high cloud tops (greater than 6.2 km) and low temperatures (less than -26 C), but also on the composition of the dust and biological residues. The greatest prevalence of ice-phase clouds occurred in conjunction with biologically-rich residues and mineral dust rich in calcium, followed by iron and aluminosilicates. Dust and biological particles are known to be efficient INP, thus these residues are what likely influenced ice formation in clouds above the sites and subsequent precipitation quantities reaching the surface during events with similar meteorology. The goal of this study is to use precipitation chemistry information to gain a better understanding of the potential sources of INP in the south-central Sierra Nevada, where cloud-aerosol-precipitation interactions are under-studied and where mixed-phase orographic clouds represent a key element in the generation of precipitation and thus the water supply in California.

Creamean, Jessie M.↗
NASA NTRS2016

Derivation of Physical and Optical Properties of Midlatitude Cirrus Ice Crystals for a Size-Resolved Cloud Microphysics Model

Single-crystal images collected in mid-latitude cirrus are analyzed to provide internally consistent ice physical and optical properties for a size-resolved cloud microphysics model, including single-particle mass, projected area, fall speed, capacitance, single-scattering albedo, and asymmetry parameter. Using measurements gathered during two flights through a widespread synoptic cirrus shield, bullet rosettes are found to be the dominant identifiable habit among ice crystals with maximum dimension (Dmax) greater than 100μm. Properties are therefore first derived for bullet rosettes based on measurements of arm lengths and widths, then for aggregates of bullet rosettes and for unclassified (irregular) crystals. Derived bullet rosette masses are substantially greater than reported in existing literature, whereas measured projected areas are similar or lesser, resulting in factors of 1.5-2 greater fall speeds, and, in the limit of large Dmax, near-infrared single-scattering albedo and asymmetry parameter (g) greater by approx. 0.2 and 0.05, respectively. A model that includes commonly imaged side plane growth on bullet rosettes exhibits relatively little difference in microphysical and optical properties aside from approx. 0:05 increase in mid-visible g primarily attributable to plate aspect ratio. In parcel simulations, ice size distribution, and g are sensitive to assumed ice properties.

asymmetry↗
NASA NTRS2018

Implementation of a Comprehensive Ice Crystal Formation Parameterization for Cirrus and Mixed-Phase Clouds in the EMAC Model (Based on MESSy 2.53)

A comprehensive ice nucleation parameterization has been implemented in the global chemistry-climate model EMAC to realistically represent ice crystal number concentrations. The parameterization of Barahona and Nenes (2009, hereafter BN09) allows the treatment of ice nucleation, taking into account the competition for water vapour between homogeneous and heterogeneous nucleation and pre-existing ice crystals in cold clouds. Furthermore, the influence of chemically-heterogeneous, polydisperse aerosols is considered via multiple ice nucleating particle spectra, which are included in the parameterization to compute the heterogeneously formed ice crystals. BN09 has been implemented to operate both in the cirrus and in the mixed-phase regimes. Compared to the standard EMAC results, BN09 produces fewer ice crystals in the upper troposphere but higher ice crystal number concentrations in the middle troposphere, especially in the Northern Hemisphere where ice nucleating mineral dust particles are relatively abundant. The comparison with a climatological data set of aircraft measurements shows that BN09 used in the cirrus regime improves the model results and, therefore, is recommended for future EMAC simulations.

EMAC↗
NASA NTRS2010

Improving the Representation of Snow Crystal Properties Within a Single-Moment Microphysics Scheme

As computational resources continue their expansion, weather forecast models are transitioning to the use of parameterizations that predict the evolution of hydrometeors and their microphysical processes, rather than estimating the bulk effects of clouds and precipitation that occur on a sub-grid scale. These parameterizations are referred to as single-moment, bulk water microphysics schemes, as they predict the total water mass among hydrometeors in a limited number of classes. Although the development of single moment microphysics schemes have often been driven by the need to predict the structure of convective storms, they may also provide value in predicting accumulations of snowfall. Predicting the accumulation of snowfall presents unique challenges to forecasters and microphysics schemes. In cases where surface temperatures are near freezing, accumulated depth often depends upon the snowfall rate and the ability to overcome an initial warm layer. Precipitation efficiency relates to the dominant ice crystal habit, as dendrites and plates have relatively large surface areas for the accretion of cloud water and ice, but are only favored within a narrow range of ice supersaturation and temperature. Forecast models and their parameterizations must accurately represent the characteristics of snow crystal populations, such as their size distribution, bulk density and fall speed. These properties relate to the vertical distribution of ice within simulated clouds, the temperature profile through latent heat release, and the eventual precipitation rate measured at the surface. The NASA Goddard, single-moment microphysics scheme is available to the operational forecast community as an option within the Weather Research and Forecasting (WRF) model. The NASA Goddard scheme predicts the occurrence of up to six classes of water mass: vapor, cloud ice, cloud water, rain, snow and either graupel or hail.

Molthan, Andrew L.↗
NASA NTRS1972

On radiational cooling computations in clouds.

Expressions are derived for the cooling or heating rates for clouds in which the condensed phase is either ice or water. Values are computed for ice and water clouds over a reasonable temperature range for pressures of 1000, 500, and 200 mb. The importance is shown of adequately allowing for the latent load in computations of radiative cooling or heating rates based on measurements of radiative divergence in clouds. It is shown that, other things being equal, the effect of the latent load is always greatest at low levels and higher temperatures.

Knollenberg, R. G.↗
NASA NTRS2000

New Multispectral Cloud Retrievals from MODIS

The Moderate Resolution Imaging Spectroradiometer (MODIS) was developed by NASA and launched onboard the Terra spacecraft on December 18, 1999. It achieved its final orbit and began Earth observations on February 24, 2000. MODIS scans a swath width sufficient to provide nearly complete global coverage every two days from a polar-orbiting, sun-synchronous, platform at an altitude of 705 km, and provides images in 36 spectral bands between 0.415 and 14.235 micrometers with spatial resolutions of 250 m (2 bands), 500 m (5 bands) and 1000 m (29 bands). These bands have been carefully selected to enable advanced studies of land, ocean, and atmospheric processes. In this paper I will describe the various methods being used for the remote sensing of cloud properties using MODIS data, focusing primarily on the MODIS cloud mask used to distinguish clouds, clear sky, heavy aerosol, and shadows on the ground, and on the remote sensing of cloud optical properties, especially cloud optical thickness and effective radius of cloud drops and ice crystals. Results will be presented of MODIS cloud properties both over the land and over the ocean, showing the consistency in cloud retrievals over various ecosystems used in the retrievals. The implications of this new observing system on global analysis of the Earth's environment will be discussed.

Platnick, Steven↗
DOE OSTI2024

Effect of Aggregation and Molecular Size on the Ice Nucleation Efficiency of Proteins

Aerosol acts as ice-nucleating particles (INPs) by catalyzing the formation of ice crystals in clouds at temperatures above the homogeneous nucleation threshold (-38 °C). In this study, we show that the immersion mode ice nucleation efficiency of the environmentally relevant protein, ribulose-1,5-bisphosphate carboxylase/oxygenase (RuBisCO), occurs at temperatures between -6.8 and -31.6 °C. Further, we suggest that this range is controlled by the RuBisCO concentration and protein aggregation. The warmest median nucleation temperature (-7.9 ± 0.8 °C) was associated with the highest concentration of RuBisCO (2 × 10 –1 mg mL –1 ) and large aggregates with a hydrodynamic diameter of ~10 3 nm. We investigated four additional chemically and structurally diverse proteins, plus the tripeptide glutathione, and found that each of them was a less effective INP than RuBisCO. Ice nucleation efficiency of the proteins was independent of the size (molecular weight) for the five proteins investigated in this study. In contrast to previous work, increasing the concentration and degree of aggregation did not universally increase ice nucleation efficiency. RuBisCO was the exception to this generalization, although the underlying molecular mechanism determining why aggregated RuBisCO is such an effective INP remains elusive.

54 ENVIRONMENTAL SCIENCES↗
NASA NTRSDate not supplied

The effects of preconditioning on the summer sea ice thickness evolution during MOSAiC

The central role of sea ice within the Arctic climate system is clear, as is the importance of sea ice properties in the Arctic Ocean’s evolution and response to climate change. Less clear is how the history of the sea ice floe (in winter and spring) precondition the summer thickness evolution. Accurate accounting for the collective influences of processes that affect the summer sea ice thickness evolution is necessary for determining sea ice survivability and the rate of future sea ice loss. In this study, we use a satellite-derived sea ice parcel database co-located with the MOSAiC floe to explore the factors that precondition the summer sea ice thickness evolution. First. we compare the >500 collocated satellite-tracked sea ice parcels that intersected the MOSAiC drift track with observations to evaluate the satellite-derived surface energy budget and surface properties, finding agreement with correlations >0.9. Approximately 60% of the satellite tracked parcels survived the summer melt season. Secondly, we explore the spread in sea ice thickness and survivability across the satellite-tracked parcels, finding contributions from spring/summer surface albedo evolution, surface temperature, clouds, and parcel sea ice concentration. The satellite tracked sea ice parcel analysis provides insights into the spatial coherence of the factors that influence sea ice thickness evolution.

Arctic↗
NASA NTRS2018

TPSAS-NF1676L-30397-DND

Arctic low clouds strongly affect the Arctic surface energy budget, and through this impact influence rest of the Arctic climate system: namely surface and atmospheric temperature, sea ice extent and thickness, and the atmospheric circulation. Arctic clouds are in turn influenced by the Arctic climate system creating the potential for cloud-climate feedbacks. We quantify the influence of atmospheric state on the surface cloud radiative effect (CRE) and the covariability between surface CRE and sea ice concentration (SIC) using instantaneous, active remote sensing satellite footprint data from the NASA A-Train. First, the results indicate significant differences in the surface CRE when stratified by atmospheric state. Second, a statistically insignificant covariability is found between CRE and SIC for most atmospheric regimes. Third, we find a statistically significant increase in the surface longwave CRE at with decreased SIC in fall. Specifically, a +3-5 W m 2 larger longwave CRE is found over footprints with 0% versus 100% SIC. Because systematic changes of 1 W m 2 are sufficient to explain the observed reductions in Arctic sea ice, our results (1) indicate a potentially significant amplifying sea ice-cloud feedback that could delay fall freeze-up influencing sea ice variability under certain atmospheric conditions and (2) suggest that a small change in the frequency of atmosphere states may yield a larger Arctic cloud feedback than any cloud response to sea ice.

Patrick Taylor↗
NASA NTRSDate not supplied

TPSAS-NF1676L-30631-DND

Arctic low clouds strongly affect the Arctic surface energy budget, and through this impact influence rest of the Arctic climate system: namely surface and atmospheric temperature, sea ice extent and thickness, and the atmospheric circulation. Arctic clouds are in turn influenced by the Arctic climate system creating the potential for cloud-climate feedbacks. We quantify the influence of atmospheric state on the surface cloud radiative effect (CRE) and the covariability between surface CRE and sea ice concentration (SIC) using instantaneous, active remote sensing satellite footprint data from the NASA A-Train. First, the results indicate significant differences in the surface CRE when stratified by atmospheric state. Second, a statistically insignificant covariability is found between CRE and SIC for most atmospheric regimes. Third, we find a statistically significant increase in the surface longwave CRE at with decreased SIC in fall. Specifically, a +3-5 W m^-2 larger longwave CRE is found over footprints with 0% versus 100% SIC. Because systematic changes of 1 W m^-2 are sufficient to explain the observed reductions in Arctic sea ice, our results (1) indicate a potentially significant amplifying sea ice-cloud feedback that could delay fall freeze-up influencing sea ice variability under certain atmospheric conditions and (2) suggest that a small change in the frequency of atmosphere states may yield a larger Arctic cloud feedback than any cloud response to sea ice.

Patrick Taylor↗