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At least 1,153 records · Page 64

SAIL Supermicron Bioaerosol (SSB) Field Campaign Report

The Surface Atmosphere Integrated Field Laboratory (SAIL) Supermicron Bioaerosol (SSB) study was designed to complement the larger Atmospheric Radiation Measurement (ARM) SAIL science goals to understand aerosol processes and aerosol-cloud interactions in the Colorado River’s East River Watershed Basin. Supermicron aerosol, particles larger than one micron in diameter, and bioaerosols, primary particles containing biological material, are important for understanding atmospheric processes and sources within high mountainous terrain. For example, they can interact with clouds and the water cycle such as by serving as nuclei for cloud droplets and ice crystals that can eventually result in precipitation events. These particles can also be recycled back to the surface via wet and dry deposition, where they can alter plant and microbial growth and/or be reemitted again, forming a positive feedback loop within the Earth system known as bioprecipitation.

54 ENVIRONMENTAL SCIENCES↗

The Connected Isotopic Water Cycle in the Community Earth System Model Version 1

Because of the pervasive role of water in the Earth system, the relative abundances of stable isotopologues of water are valuable for understanding atmospheric, oceanic, and biospheric processes, and for interpreting paleoclimate proxy reconstructions. Isotopologues are transported by both largescale and turbulent flows, and the ratio of heavy to light isotopologues changes due to fractionation that can accompany condensation and evaporation processes. Correctly predicting the isotopic distributions requires resolving the relationships between largescale ocean and atmospheric circulation and smallerscale hydrological processes, which can be accomplished within a coupled climate modeling framework. Here we present the water isotopeenabled version of the Community Earth System Model version 1 (iCESM1), which simulates global variations in water isotopic ratios in the atmosphere, land, ocean, and sea ice. In a transient Last Millennium simulation covering the 850-2005 period, iCESM1 correctly captures the latetwentiethcentury structure of δ(exp 18)O and δD over the global oceans, with more limited accuracy over land. The relationship between salinity and seawater δ(exp 18)O is also well represented over the observational period, including interbasin variations. We illustrate the utility of coupled, isotopeenabled simulations using both Last Millennium simulations and freshwater hosing experiments with iCESM1. Closing the isotopic mass balance between all components of the coupled model provides new confidence in the underlying depiction of the water cycle in CESM, while also highlighting areas where the underlying hydrologic balance can be improved. The iCESM1 is poised to be a vital community resource for ongoing model development with both modern and paleoclimate applications.

Brady, E.↗

Land Processes Can Substantially Impact the Mean Climate State

Terrestrial processes influence the atmosphere by controlling land-to-atmosphere fluxes of energy, water, and carbon. Prior research has demonstrated that parameter uncertainty drives uncertainty in land surface fluxes. However, the influence of land process uncertainty on the climate system remains underexplored. Here, we quantify how assumptions about land processes impact climate using a perturbed parameter ensemble for 18 land parameters in the Community Earth System Model version 2 under preindustrial conditions. We find that an observationally-informed range of land parameters generate biogeophysical feedbacks that significantly influence the mean climate state, largely by modifying evapotranspiration. Global mean land surface temperature ranges by 2.2°C across our ensemble (σ = 0.5°C) and precipitation changes were significant and spatially variable. Our analysis demonstrates that the impacts of land parameter uncertainty on surface fluxes propagate to the entire Earth system, and provides insights into where and how land process uncertainty influences climate.

54 ENVIRONMENTAL SCIENCES↗

Precipitation Recycling

The water cycle regulates and reflects natural variability in climate at the regional and global scales. Large-scale human activities that involve changes in land cover, such as tropical deforestation, are likely to modify climate through changes in the water cycle. In order to understand, and hopefully be able to predict, the extent of these potential global and regional changes, we need first to understand how the water cycle works. In the past, most of the research in hydrology focused on the land branch of the water cycle, with little attention given to the atmospheric branch. The study of precipitation recycling which is defined as the contribution of local evaporation to local precipitation, aims at understanding hydrologic processes in the atmospheric branch of the water cycle. Simply stated, any study on precipitation recycling is about how the atmospheric branch of the water cycle works, namely, what happens to water vapor molecules after they evaporate from the surface, and where will they precipitate?

Eltahir, Elfatih A. B.↗

Investigation of the daytime lunar atmosphere for lunar synthesis program

Synthesis studies of the daytime lunar atmoshere were directed toward improved understanding of fundamental lunar atmospheric dynamics and the relationship of the detectable atmosphere to physical processes of the lunar surface and interior. The primary source of data is the Apollo 17 lunar surface mass spectrometer. The Ar40 is radiogenic and its escape rate from the lunar atmosphere requires release of a significant fraction (about 8%) of the argon produced from the decay of K40 within the moon. Furthermore the process of argon release from the solid moon is time varying and related to seismic activity. Most of the helium on the moon is due to release of implanted solar wind alpha particles from the regolith.

Hodges, R. R., Jr.↗

Use of satellite soundings and imagery for nowcasting and very-short-range forecasting

Examples of GOES-East satellite imagery and sounding channel information are used to show how atmospheric behavior in the vicinity of intense mesoscale weather events can be analyzed. Mesoscale spatial and temporal information on atmospheric thermal structure and moisture distribution can be determined using satellite sounding and multispectral image data. Clouds and cloud patterns in a satellite image or animated series of images represent the integrated effect of ongoing dynamic and thermodynamic processes in the atmosphere. When information from satellite data is combined with radar, surface and upper air observations, important processes in storm development can be better understood.

Purdom, J. F. W.↗

Over three decades, and counting, of near-surface turbulent flux measurements from the Atmospheric Radiation Measurement (ARM) user facility

Processes mediating the coupling of terrestrial, aquatic, biospheric, and atmospheric systems influence weather, climate, and ecosystem dynamics via transfer of energy, momentum, water, and carbon (or other species). These exchange processes are quantified by measurements of near-surface turbulent fluxes. Understanding processes at these interfaces provides insight toward understanding and predicting current and future states within the Earth system. The Atmospheric Radiation Measurement (ARM) user facility has been conducting measurements of near-surface turbulent fluxes since the early 1990s at long-term fixed locations and shorter-term mobile deployments across the Earth. ARM has utilized two established methods for conducting these measurements: energy balance Bowen ratio (EBBR) and eddy covariance (EC). Primary measurements from the former include sensible and latent heat flux, while the latter also measures fluxes of momentum and carbon (primarily carbon dioxide, with methane fluxes measured at two locations to date). The EBBR systems have been deployed at 22 locations, and, to date, the EC systems have been deployed at over 50 sites, with plans for additional novel site locations in the future. Herein, the history, evolution, and key aspects of these instrument systems are documented, along with information on data quality assurance and post-processing, as well as best use practices. Additionally, three data validation experiments were recently conducted, and their key findings are summarized. Finally, ancillary datasets acquired by ARM, which can contextualize and aid interpretation of the near-surface turbulent flux measurements, are discussed. The datasets described herein include the eddy correlation flux measurement system: 30ECOR (https://doi.org/10.5439/1879993, Sullivan et al., 1997), 30QCECOR (https://doi.org/10.5439/1097546, Gaustad, 2003), ECORSF (https://doi.org/10.5439/1494128, Sullivan et al., 2019a), and associated AmeriFlux and Methane Value-Added Product, AMCMETHANE (https://doi.org/10.5439/1508268, Billesbach, 2011); the energy balance Bowen ratio system: 30EBBR (https://doi.org/10.5439/1023895, Sullivan et al., 1993) and 30BAEBBR (https://doi.org/10.5439/1027268, Gaustad and Xie, 1993); and the carbon dioxide flux measurement system: CO2FLX (https://doi.org/10.5439/1287574, https://doi.org/10.5439/1287575, https://doi.org/10.5439/1287576, Koontz et al., 2015a, b, c; https://doi.org/10.5439/1989774, https://doi.org/10.5439/1989776, https://doi.org/10.5439/1992202, Biraud and Chan, 2002a, b, c). These data can be found by searching the above data stream names at https://adc.arm.gov/discovery/#/results/ (last access: 8 September 2025).

Sullivan, Ryan C. [Argonne National Laboratory (AN↗

Atmospheric microphysical experiments on an orbital platform

The Zero-Gravity Atmospheric Cloud Physics Laboratory is a Shuttle/Spacelab payload which will be capable of performing a large range of microphysics experiments. This facility will complement terrestrial cloud physics research by allowing many experiments to be performed which cannot be accomplished within the confines of a terrestrial laboratory. This paper reviews the general Cloud Physics Laboratory concept and the experiment scope. The experimental constraints are given along with details of the proposed equipment. Examples of appropriate experiments range from three-dimensional simulation of the earth and planetary atmosphere and of ocean circulation to cloud electrification processes and the effects of atmospheric pollution materials on microphysical processes.

Eaton, L. R.↗

Chemistry and spectroscopy of the Jovian atmosphere

A comprehensive review is given of the chemistry and spectroscopic studies of the Jovian atmosphere. Thermochemical equilibrium models for determining atmospheric composition are considered along with possible disequilibrating processes, and studies of the photochemistry of H2, CH4, NH3, H2S, and PH3 using the modeling methods are summarized. It is shown that photodissociation and advection are the major disequilibrating processes in Jupiter's atmosphere, that lightning and charged-particle bombardment are relatively minor factors in the planet's bulk chemistry, and that the existence of living organisms on the planet is highly improbable. Spectroscopic investigations of Jupiter are discussed, emphasizing recent observations of absorption bands due to CH4, NH3, H2, He, and D. Spectroscopic abundance determinations are examined for H2, HD, CH4, CH3D, NH3, C2H6, C2H2, and PH3. Upper limits are given for the abundances of several unobserved gases in the visible atmosphere, including H2S, HCl, SiH4, benzene, purines, pyrimidines, and their derivatives.

Prinn, R. G.↗

Model atmospheres, predicted spectra, and colors

Theoretical models of stellar atmospheres and the process of forming a spectrum are reviewed with particular reference to the spectra of B stars. In the case of classical models the stellar atmosphere is though to consist of plane parallel layers of gas in which radiative and hydrostatic equilibrium exists. No radiative energy is lost or gained in the model atmosphere, but the detailed shape of the spectrum is changed as a result of the interactions with the ionized gas. Predicted line spectra using statistical equilibrium local thermodynamic equilibrium (LTE), and non-LTE physics are compared and the determination of abundances is discussed. The limitations of classical modeling are examined. Models developed to demonstrate what motions in the upper atmosphere will do to the spectrum and to explore the effects of using geometries different from plane parallel layer are reviewed. In particular the problem of radiative transfer is addressed.

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The nitrogen cycle: Atmosphere interactions

Atmospheric interactions involving the nitrogen species are varied and complex. These interactions include photochemical reactions, initiated by the absorption of solar photons and chemical kinetic reactions, which involve both homogeneous (gas-to-gas reactions) and heterogeneous (gas-to-particle) reactions. Another important atmospheric interaction is the production of nitrogen oxides by atmospheric lightning. The nitrogen cycle strongly couples the biosphere and atmosphere. Many nitrogen species are produced by biogenic processes. Once in the atmosphere nitrogen oxides are photochemically and chemically transformed to nitrates, which are returned to the biosphere via precipitation, dry deposition and aerosols to close the biosphere-atmosphere nitrogen cycle. The sources, sinks and photochemistry/chemistry of the nitrogen species; atmospheric nitrogen species; souces and sinks of nitrous oxide; sources; sinks and photochemistry/chemistry of ammonia; seasonal variation of the vertical distribution of ammonia in the troposphere; surface and atmospheric sources of the nitrogen species, and seasonal variation of ground level ammonia are summarized.

Levine, J. S.↗

Upper Atmosphere Research Satellite (UARS): A program to study global ozone change

A general overview of NASA's Upper Atmosphere Research Satellite (UARS) program is presented in a broad based informational publication. The UARS will be responsible for carrying out the first systematic, comprehensive study of the stratosphere and will furnish important new data on the mesosphere and thermosphere. The UARS mission objectives are to provide an increased understanding of energy input into the upper atmosphere; global photochemistry of the upper atmosphere; dynamics of the upper atmosphere; coupling among these processes; and coupling between the upper and lower atmosphere. These mission objectives are briefly described along with the UARS on-board instrumentation and related data management systems.

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Dimensional analysis of acoustically propagated signals

Traditionally, long term measurements of atmospherically propagated sound signals have consisted of time series of multiminute averages. Only recently have continuous measurements with temporal resolution corresponding to turbulent time scales been available. With modern digital data acquisition systems we now have the capability to simultaneously record both acoustical and meteorological parameters with sufficient temporal resolution to allow us to examine in detail relationships between fluctuating sound and the meteorological variables, particularly wind and temperature, which locally determine the acoustic refractive index. The atmospheric acoustic propagation medium can be treated as a nonlinear dynamical system, a kind of signal processor whose innards depend on thermodynamic and turbulent processes in the atmosphere. The atmosphere is an inherently nonlinear dynamical system. In fact one simple model of atmospheric convection, the Lorenz system, may well be the most widely studied of all dynamical systems. In this paper we report some results of our having applied methods used to characterize nonlinear dynamical systems to study the characteristics of acoustical signals propagated through the atmosphere. For example, we investigate whether or not it is possible to parameterize signal fluctuations in terms of fractal dimensions. For time series one such parameter is the limit capacity dimension. Nicolis and Nicolis were among the first to use the kind of methods we have to study the properties of low dimension global attractors.

Hansen, Scott D.↗

Winds from cool stars

Spectral observations of cool stars enable study of the presence and character of winds and the mass loss process in objects with effective temperatures, gravities, and atmospheric compositions which differ from that of the Sun. A wealth of recent spectroscopic measurements from the Hubble Space Telescope, and the Extreme Ultraviolet Explorer complement high resolution ground-based measures in the optical and infrared spectral regions. Such observations when combined with realistic semi-empirical atmospheric modeling allow us to estimate the physical conditions in the atmospheres and winds of many classes of cool stars. Line profiles support turbulent heating and mass motions. In low gravity stars, evidence is found for relatively fast (approximately 200 km s(exp -1)), warm winds with rapid acceleration occurring in the chromosphere. In some cases outflows commensurate with stellar escape velocities are present. Our current understanding of cool star winds will be reviewed including the implications of stellar observations for identification of atmospheric heating and acceleration processes.

Dupree, A. K.↗

Data Information for Global Change Studies: NASA's Distributed Active Archive Centers and Cooperating Data Centers

The Earth Observing System (EOS) is an integral part of the National Aeronautics and Space Administration's (NASA's) Earth Science Enterprise (ESE). ESE is a long-term global change research program designed to improve our understanding of the Earth's interrelated processes involving the atmosphere, oceans, land surfaces, and polar regions. Data from EOS instruments and other Earth science measurement systems are useful in understanding the causes and processes of global climate change and the consequences of human activities. The EOS Data and Information System (EOSDIS) provides a structure for data management and user services for products derived from EOS satellite instruments and other NASA Earth science data. Within the EOSDIS framework, the Distributed Active Archive Centers (DAACs) have been established to provide expertise in one or more Earth science disciplines. The DAACs and cooperating data centers provide data and information services to support the global change research community. Much of the development of the DAACs has been in anticipation of the enormous amount of data expected from EOS instruments to be launched within the next two decades. Terra, the EOS flagship launched in December 1999, is the first of a series of EOS satellites to carry several instruments with multispectral capabilities. Some data products from these instruments are now available from several of the DAACs. These and other data products can be ordered through the EOS Data Gateway (EDG) and DAAC-specific online ordering systems.

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Evaluation of Convective Transport in the GEOS-5 Chemistry and Climate Model

The NASA Goddard Earth Observing System (GEOS-5) Chemistry and Climate Model (CCM) consists of a global atmospheric general circulation model and the combined stratospheric and tropospheric chemistry package from the NASA Global Modeling Initiative (GMI) chemical transport model. The subgrid process of convective tracer transport is represented through the Relaxed Arakawa-Schubert parameterization in the GEOS-5 CCM. However, substantial uncertainty for tracer transport is associated with this parameterization, as is the case with all global and regional models. We have designed a project to comprehensively evaluate this parameterization from the point of view of tracer transport, and determine the most appropriate improvements that can be made to the GEOS-5 convection algorithm, allowing improvement in our understanding of the role of convective processes in determining atmospheric composition. We first simulate tracer transport in individual observed convective events with a cloud-resolving model (WRF). Initial condition tracer profiles (CO, CO2, O3) are constructed from aircraft data collected in undisturbed air, and the simulations are evaluated using aircraft data taken in the convective anvils. A single-column (SCM) version of the GEOS-5 GCM with online tracers is then run for the same convective events. SCM output is evaluated based on averaged tracer fields from the cloud-resolving model. Sensitivity simulations with adjusted parameters will be run in the SCM to determine improvements in the representation of convective transport. The focus of the work to date is on tropical continental convective events from the African Monsoon Multidisciplinary Analyses (AMMA) field mission in August 2006 that were extensively sampled by multiple research aircraft.

Pickering, Kenneth E.↗

Atmospheric corrections for satellite water quality studies

Variations in the relative value of the blue and green reflectances of a lake can be correlated with important optical and biological parameters measured from surface vessels. Measurement of the relative reflectance values from color film imagery requires removal of atmospheric effects. Data processing is particularly crucial because: (1) lakes are the darkest objects in a scene; (2) minor reflectance changes can correspond to important physical changes; (3) lake systems extend over broad areas in which atmospheric conditions may fluctuate; (4) seasonal changes are of importance; and, (5) effects of weather are important, precluding flights under only ideal weather conditions. Data processing can be accomplished through microdensitometry of scene shadow areas. Measurements of reflectance ratios can be made to an accuracy of plus or minus 12%, sufficient to permit monitoring of important eutrophication indices.

Piech, K. R.↗

Cirrus Susceptibility to Changes in Ice Nuclei: Physical Processes, Model Uncertainties, and Measurement Needs

One of the proposed concepts for mitigating the warming effect of increasing greenhouse gases is seeding cirrus cloud with ice nuclei (IN) in order to reduce the lifetime and coverage of cold cirrus that have a net warming impact on the earth's surface. Global model simulations of the net impact of changing upper tropospheric IN have given widely disparate results, partly as a result of poor understanding of ice nucleation processes in the current atmosphere, and partly as a result of poor representation of these processes in global models. Here, we present detailed process-model simulations of tropical tropopause layer (TTL) transport and cirrus formation with ice nuclei properties based on recent laboratory nucleation experiments and field measurements of aerosol composition. The model is used to assess the sensitivity of TTL cirrus occurrence frequency and microphysical properties to the abundance and efficacy of ice nuclei. The simulated cloud properties compared with recent high-altitude aircraft measurements of TTL cirrus and ice supersaturation. We find that abundant effective IN (either from glassy organic aerosols or crystalline ammonium sulfate with concentrations greater than about 100/L) prevent the occurrences of large ice concentration and large ice supersaturations, both of which are clearly indicated by the in situ observations. We find that concentrations of effective ice nuclei larger than about 50/L can drive significant changes in cirrus microphysical properties and occurrence frequency. However, the cloud occurrence frequency can either increase or decrease, depending on the efficacy and abundance of IN added to the TTL. We suggest that our lack of information about ice nuclei properties in the current atmosphere, as well as uncertainties in ice nucleation processes and their representations in global models, preclude meaningful estimates of climate impacts associated with addition of ice nuclei in the upper troposphere. We will briefly discuss the key field measurements needed to constrain ice nucleation processes.

Jensen, Eric↗