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At least 1,153 records · Page 64
All sourcesNASA NTRSDOE OSTI
DOE OSTI2016

Role of target-substrate distance on the growth of CuInSe{sub 2} thin films by pulsed laser ablation technique

CuInSe{sub 2} thin films have been deposited on corning glass substrates by pulsed laser ablation technique. The chamber pressure and substrate temperature was maintained at 1 × 10{sup −6} torr and 550°C respectively during deposition of the films. The influence of target to substrate (T-S) distance on the structural and optical properties of thin films have been investigated by grazing incidence x-ray diffraction, Raman spectroscopy, scanning electron microscope and UV-Vis-NIR spectroscopy. The study reveals that thin films crystallized in a chalcopyrite structure with highly preferential orientation along (112) plane. Optimum T-S distance has been attained for the growth of thin films with large grain size. An intense Raman peak at 174 cm{sup −1} corresponding to dominant A{sub 1} vibration mode is gradually shifted to smaller wavenumber with the increase in T-S distance. The optical bandgap energy of the films was evaluated and found to vary with the T-S distance. The bandgap tailing was observed to obey the Urbach rule and the Urbach energy was also calculated for the films. Scanning electron micrographs depicts uniform densely packed grains and EDAX studies revealed the elemental composition of CuInSe{sub 2} thin films.

36 MATERIALS SCIENCE↗
DOE OSTI2016

The effects of electron thermal radiation on laser ablative shock waves from aluminum plasma into ambient air

The effect of electron thermal radiation on 7 ns laser ablative shock waves from aluminum (Al) plasma into an ambient atmospheric air has been numerically investigated using a one-dimensional, three-temperature (electron, ion, and radiation) radiation hydrodynamic code MULTI. The governing equations in Lagrangian form are solved using an implicit scheme for planar, cylindrical, and spherical geometries. The shockwave velocities (V{sub sw}) obtained numerically are compared with our experimental values obtained over the intensity range of 2.0 × 10{sup 10} to 1.4 × 10{sup 11 }W/cm{sup 2}. It is observed that the numerically obtained V{sub sw} is significantly influenced by the thermal radiation effects which are found to be dominant in the initial stage up to 2 μs depending on the input laser energy. Also, the results are found to be sensitive to the co-ordinate geometry used in the simulation (planar, cylindrical, and spherical). Moreover, it is revealed that shock wave undergoes geometrical transitions from planar to cylindrical nature and from cylindrical to spherical nature with time during its propagation into an ambient atmospheric air. It is also observed that the spatio-temporal evolution of plasma electron and ion parameters such as temperature, specific energy, pressure, electron number density, and mass density were found to be modified significantly due to the effects of electron thermal radiation.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2017

Use of 41Ar production to measure ablator areal density in NIF beryllium implosions

For the first time, 41Ar produced by the (n,ϒ) reaction from 40Ar in the beryllium shell of a DT filled Inertial Confinement Fusion capsule has been measured. Ar is co-deposited with beryllium in the sputter deposition of the capsule shell. Combined with a measurement of the neutron yield, the radioactive 41Ar then quantifies the areal density of beryllium during the DT neutron production. The measured 1.15 ± 0.17 × 10+8 atoms of 41Ar are 2.5 times that from the best post-shot calculation, suggesting that the Ar and Be areal densities are correspondingly higher than those calculated. Possible explanations are that (1) the beryllium shell is compressed more than calculated, (2) beryllium has mixed into the cold DT ice, or more likely (3) less beryllium is ablated than calculated. Since only one DT filled beryllium capsule has been fielded at NIF, these results can be confirmed and expanded in the future.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2017

The effect of electron transport on the characterization of x-ray free-electron laser pulses via ablation

The spatial intensity distribution of x-ray free-electron laser (XFEL) pulses in-focus is commonly characterized by performing ablative imprints in thin gold films on silica substrates. In many cases, the range of the electrons generated in the gold by x-ray absorption far exceeds the beam size, and so, it is not clear if the results of imprint studies are compromised by electron transport. Thermal conduction could further modify the energy density profile in the material. We used here a combination of Monte-Carlo transport and continuum models to quantify the accuracy of the imprint method for characterizing XFEL beam profiles. We found that for x-ray energies in the range of 1 to 10 keV, the actual and the measured beam diameters agree within 12% or better for beam diameters between 0.1 and 1 μm.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2019

Two mode coupling of the ablative Rayleigh-Taylor instabilities

In this work, the coupling and evolution of two-mode ablative Rayleigh-Taylor instability (ARTI) in two-dimensional geometry are studied via numerical simulations. We focus primarily on two scenarios: Coupling and bubble competition of a long and a short wavelength mode and of two short-wavelength modes. It is found that the long-wavelength modes tend to dominate in the nonlinear phase of the long-short coupling cases. The presence of the short-wavelength mode in the long-short cases enhances the total ARTI bubble vertex velocity. However, due to the formation of enclosed bubbles, this enhancement does not increase monotonically with the initial short-wavelength amplitude. Coupling of two short-wavelength modes forms a long-wavelength component which grows faster than each individual short-wavelength mode.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2019

Enhancing cylindrical compression by reducing plasma ablation in pulsed-power drivers

Warm dense matter, which can be found in planetary cores, is too dense to be described by plasma theory and too hot to be considered condensed matter. With no theory describing perfectly how such large quantum systems evolve at macroscopic scales, modeling planetary evolution is simply out of reach. While recent experiments using high power lasers and heavy ion beams have produced warm dense matter samples, they do not confine matter long enough to allow for bulk material properties to take hold, precluding the validation of any theories beyond electron-ion equilibration time. To this end, pulsed-power drivers are required. This approach allows experimentalists to probe macroscopic states of matter where bulk material properties are at equilibrium. High resolution numerical simulations show that a mega-ampere pulsed-power driver can generate macroscopic samples of warm dense matter, using direct magnetic compression, without any pusher. A thin coating, deposited onto the material just before the experiment, softens the density gradients responsible for plasma ablation. Starved of plasma outside the conductors, electrical currents are forced to flow along material surfaces, resulting in a very stable magnetic topology that yields homogeneous compression above 1 Mbar. Another key aspect is as follows: mega-ampere pulsed power systems are compact enough to be located next to existing high brilliance x-ray sources, which can probe best the properties of matter under extreme pressure.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2025

Magnetized ICF implosions: Ignition at low laser energy using designs with more ablator mass remaining

This paper is the first work to redesign a spherical ICF implosion to best utilize the benefits of applying an external magnetic field. The sub-ignition experiment N170601 is taken as the baseline design, which used 1.57 MJ of laser energy. The optimum magnetized design benefits from increasing the shell thickness by 14 μ m and decreasing the ice thickness by 18 μ m, resulting in a neutron yield of 8.9 × 10 17 . This is 34 × greater than the unmagnetized simulation of the same design, and 18.5 × the greatest unmagnetized simulation across all designs simulated. The resultant implosion velocity for the magnetized design is lower, which would also reduce ablation front instability growth. This design was found by using a simplified 1D magnetization model and then validated against full 2D extended-MHD capsule simulations with radiation asymmetries applied to correct the shape.

Walsh, Christopher A. [Lawrence Livermore National↗
DOE OSTI2016

Study of the formation of a microrelief on ZnSe- and CdSe-crystal surfaces ablated by excimer KrF-laser radiaton

One-dimensional gratings with a period of 0.5−2.3 μm are formed on the surfaces of CdSe and ZnSe crystals ablated by two interfering radiation beams of a nanosecond excimer KrF laser. Investigated are the dependences of the shape and depth of gratings on the energy density under irradiation by a single pulse, and on the number of pulses at a given energy density. The maximum grating depth is estimated as ∼0.57 of the period. By forming a one-dimensional grating with a period of 1.5 μm and a depth of 0.53 μm on the CdSe-crystal surface, this surface becomes antireflective at a wavelength of 4 μm. The surface reflectivity is reduced by 88 %. A possibility of forming two-dimensional gratings having periods of 1 and 1.5 μm is demonstrated. (paper)

77 NANOSCIENCE AND NANOTECHNOLOGY↗
DOE OSTI2024

Precision Polishing of Ablator Capsules via in situ Process Monitoring and Machine Learning–Based Optimization

In inertial confinement fusion (ICF) experiments seeking output gains of unity and beyond, the quality of the ablator capsule is paramount for minimizing the hydrodynamic mix that quenches the central hot spot. Defects in the form of foreign particles or missing mass on the surface and within the wall of the capsule are primary offenders. High-density carbon capsules made for ICF experiments at the National Ignition Facility are precision polished to achieve surface smoothness on the order of a few nanometers as well as to minimize isolated defects in the form of pits. Given the critical role of this process, we are developing smart manufacturing techniques with the goal of elevating the efficiency of this process. Our approach is to use MEMS (micro-electromechanical systems)–based sensors to capture the fine vibration signals generated during the polishing process and combine them with synchronized visual feedback as needed. Beyond using these sensors for process monitoring, we use specific deep learning methods to analyze the data and extract correlations with both the process parameters and the final performance of the polishing run. Here, in this work, we describe the multiple fronts we have explored in this regard and the results we have gotten so far. This approach promises to have the potential to ultimately provide real-time feedback that can be used to ensure the progress of the run as well as a means for faster optimization.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2015

DIRECT DETECTION OF COMPLEX ORGANIC PRODUCTS IN ULTRAVIOLET (Lyα) AND ELECTRON-IRRADIATED ASTROPHYSICAL AND COMETARY ICE ANALOGS USING TWO-STEP LASER ABLATION AND IONIZATION MASS SPECTROMETRY

As discovery of complex molecules and ions in our solar system and the interstellar medium has proliferated, several groups have turned to laboratory experiments in an effort to simulate and understand these chemical processes. So far only infrared (IR) and ultraviolet (UV) spectroscopy has been able to directly probe these reactions in ices in their native, low-temperature states. Here we report for the first time results using a complementary technique that harnesses two-step two-color laser ablation and ionization to measure mass spectra of energetically processed astrophysical and cometary ice analogs directly without warming the ices—a method for hands-off in situ ice analysis. Electron bombardment and UV irradiation of H{sub 2}O, CH{sub 3}OH, and NH{sub 3} ices at 5 K and 70 K led to complex irradiation products, including HCO, CH{sub 3}CO, formamide, acetamide, methyl formate, and HCN. Many of these species, whose assignment was also strengthened by isotope labeling studies and correlate with IR-based spectroscopic studies of similar irradiated ices, are important ingredients for the building blocks of life. Some of them have been detected previously via astronomical observations in the interstellar medium and in cometary comae. Other species such as CH{sub 3}CO (acetyl) are yet to be detected in astrophysical ices or interstellar medium. Our studies suggest that electron and UV photon processing of astrophysical ice analogs leads to extensive chemistry even in the coldest reaches of space, and lend support to the theory of comet-impact-induced delivery of complex organics to the inner solar system.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2016

Filamentation due to the Weibel instability in two counterstreaming laser ablated plasmas

Weibel-type filamentation instability was observed in the interaction of two counter streaming laser ablated plasma flows, which were supersonic, collisionless, and closely relevant to astrophysical conditions. The plasma flows were created by irradiating a pair of oppositely standing plastic (CH) foils with 1ns-pulsed laser beams of total energy of 1.7 kJ in two laser spots. Finally, with characteristics diagnosed in experiments, the calculated features of Weibel-type filaments are in good agreement with measurements.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2016

Behaviour of rippled shocks from ablatively-driven Richtmyer-Meshkov in metals accounting for strength

While numerous continuum material strength and phase transformation models have been proposed to capture their complex dependences on intensive properties and deformation history, few experimental methods are available to validate these models particularly in the large pressure and strain rate regime typical of strong shock and ramp dynamic loading. In the experiments and simulations we present, a rippled shock is created by laser-ablation of a periodic surface perturbation on a metal target. The strength of the shock can be tuned to access phase transitions in metals such as iron or simply to study high-pressure strength in isomorphic materials such as copper. Simulations, with models calibrated and validated to the experiments, show that the evolution of the amplitude of imprinted perturbations on the back surface by the rippled shock is strongly affected by strength and phase transformation kinetics. Increased strength has a smoothing effect on the perturbed shock front profile resulting in smaller perturbations on the free surface. Lastly, in iron, faster phase transformations kinetics had a similar effect as increased strength, leading to smoother pressure contours inside the samples and smaller amplitudes of free surface perturbations in our simulations.

36 MATERIALS SCIENCE↗
DOE OSTI2019

Laser ablation tomography for visualization of root colonization by edaphic organisms

Soil biota have important effects on crop productivity, but can be difficult to study in situ . Laser ablation tomography (LAT) is a novel method that allows for rapid, three-dimensional quantitative and qualitative analysis of root anatomy, providing new opportunities to investigate interactions between roots and edaphic organisms. LAT was used for analysis of maize roots colonized by arbuscular mycorrhizal fungi, maize roots herbivorized by western corn rootworm, barley roots parasitized by cereal cyst nematode, and common bean roots damaged by Fusarium . UV excitation of root tissues affected by edaphic organisms resulted in differential autofluorescence emission, facilitating the classification of tissues and anatomical features. Samples were spatially resolved in three dimensions, enabling quantification of the volume and distribution of fungal colonization, western corn rootworm damage, nematode feeding sites, tissue compromised by Fusarium , and as well as root anatomical phenotypes. Owing to its capability for high-throughput sample imaging, LAT serves as an excellent tool to conduct large, quantitative screens to characterize genetic control of root anatomy and interactions with edaphic organisms. Additionally, this technology improves interpretation of root–organism interactions in relatively large, opaque root segments, providing opportunities for novel research investigating the effects of root anatomical phenes on associations with edaphic organisms.

60 APPLIED LIFE SCIENCES↗
DOE OSTI2019

Kinetic simulations of fusion ignition with hot-spot ablator mix

Inertial confinement fusion fuel suffers increased x-ray radiation losses when carbon from the capsule ablator mixes into the hot-spot. Here, we present one- and two-dimensional ion Vlasov-Fokker-Planck simulations that resolve hot-spot self-heating in the presence of a localized spike of carbon mix, totalling 1.9% of the hot-spot mass. The mix region cools and contracts over tens of picoseconds, increasing its α particle stopping power and radiative losses. Furthermore, this makes a localized mix region more severe than an equal amount of uniformly distributed mix. There is also a purely kinetic effect that reduces fusion reactivity by several percent, since faster ions in the tail of the distribution are absorbed by the mix region. Radiative cooling and contraction of the spike induces fluid motion, causing neutron spectrum broadening. This artificially increases the inferred experimental ion temperatures and gives line of sight variations.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2023

Nonlinear ablative Rayleigh-Taylor instability: Increased growth due to self-generated magnetic fields

The growth rate of the nonlinear ablative Rayleigh-Taylor (RT) instability is enhanced by magnetic fields self-generated by the Biermann battery mechanism; a scaling for this effect with perturbation height and wavelength is proposed and validated with extended-magnetohydrodynamic simulations. The magnetic flux generation rate around a single RT spike is found to scale with the spike height. The Hall parameter, which quantifies electron magnetization, is found to be strongly enhanced for short-wavelength spikes due to Nernst compression of the magnetic field at the spike tip. Furthermore, the impact of the magnetic field on spike growth is through both the suppressed thermal conduction into the unstable spike and the Righi-Leduc heat flow deflecting heat from the spike tip to the base. Righi-Leduc is found to be the dominant effect for small Hall parameters, while suppressed thermal conduction dominates for large Hall parameters. These results demonstrate the importance of considering magnetic fields in all perturbed inertial confinement fusion hot spots.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2024

Microphysics of shock-grain interaction for inertial confinement fusion ablators in a fluid approach

Ablator materials used for inertial confinement fusion, such as high-density carbon (HDC) and beryllium, have grain structure which may lead to small-scale density nonuniformity and the generation of perturbations when the materials are shocked and compressed. Here, we use a combination of a linear theory of shock interaction with density nonuniformity [Velikovich et al., Phys. Plasmas 14, 072706 (2007)] and numerical simulations to study shock interaction with a model representation of HDC grains. While the shock-grain interaction is nonlinear, the linear theory shows some key features of the shock-grain interaction, which also hold for the (nonlinear) simulations. The postshock perturbations are made up of sonic reflections off of grain boundaries and vorticity deposition along them, with the latter dominating the perturbed energy content. The mean (per mass) postshock perturbed kinetic energy decreases with increasing grain size, but energy will be deposited at increasing spatial scale. From the perspective of the postshock perturbed energy, the detailed linear theory largely supports a proposed method [S. Davidovits et al., Phys. Plasmas 29, 112708 (2022)] for deresolving the grains (in a similar grains model) that treats the grains statistically. Finally, our simulation results highlight the influence of thermal conduction on the perturbation dynamics at grain scales.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2021

Evidence of Three-Dimensional Asymmetries Seeded by High-Density Carbon-Ablator Nonuniformity in Experiments at the National Ignition Facility

Inertial confinement fusion implosions must achieve high in-flight shell velocity, sufficient energy coupling between the hot spot and imploding shell, and high areal density ( ρ R = ∫ ρ d r ) at stagnation. Asymmetries in ρ R degrade the coupling of shell kinetic energy to the hot spot and reduce the confinement of that energy. In this study, we present the first evidence that nonuniformity in the ablator shell thickness ( ~ 0.5 % of the total thickness) in high-density carbon experiments is a significant cause for observed 3D ρ R asymmetries at the National Ignition Facility. These shell-thickness nonuniformities have significantly impacted some recent experiments leading to ρ R asymmetries on the order of ~ 25 % of the average ρ R and hot spot velocities of ~ 100 km / s . This work reveals the origin of a significant implosion performance degradation in ignition experiments and places stringent new requirements on capsule thickness metrology and symmetry.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2026

Ablating Pellets for Areal Density Symmetry Control in Indirectly Driven Inertial Confinement Fusion Target Designs

Asymmetry of the compressed fusion fuel configuration, as characterized by a variation in areal density, in inertial confinement fusion (ICF) implosions is a known performance limitation. While ignition has been achieved on the National Ignition Facility (NIF), implosion symmetry was not perfect, and subsequent experiments that have extended fusion performance still struggle with symmetry control and would, in principle, perform much better if the areal density uniformity of the fuel was improved by eliminating thin regions in the DT (Deuterium-Tritium) fuel that develop by the time of peak compression. In indirect drive (IDD), altering the time-dependent laser cone fraction and cross-beam energy transfer are the usual tactics for controlling implosion asymmetry in IDD target designs, but it may be that those tools have been pushed to their limits. In this Letter, we present a new tactic for controlling the implosion using satellite ablating pellets to manipulate the time-dependent x-ray field around an ICF capsule. In theory and in simulations the action of these pellets is quite effective at reducing the swing of x-ray drive from waist hot to pole hot, thus achieving a more one-dimensional fuel configuration at peak compression. Simulations show that a factor of ∼2 in yield performance can be obtained via this technique, when applied to past record implosions on the NIF. As a result, some speculative alternate uses of the proposed target concept are also mentioned in the conclusion of this Letter.

Implosion symmetry↗