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Hadron spectroscopy of pseudoscalar and vector meson photoproduction using linearly polarised photons at CLAS

The field of hadron spectroscopy is informed by experiments which study excited states of the nucleon by detecting the decay products following excitation with a hadronic, leptonic or electromagnetic probe. Experiments using a polarised beam of photons provide an important contribution to the world data. This thesis describes the analysis of data from one such experiment, the CEBAF Large Acceptance Spectrometer at Jefferson Laboratory, Virginia, USA. In the experiment, an incident beam of electrons passes through a diamond radiator producing a linearly polarised photon beam of energy from 1.1 to 2.1 GeV on a liquid hydrogen target. The analysis method and results for two reaction channels are presented. In the first analysis, the polarisation observables {?, P, T, Ox, Oz} for the reaction ??? p ? K0 S ?+ are extracted simultaneously using likelihood sampling with Markov-Chain Monte-Carlo. The results are presented as angular distributions (cos ?K0S) for bins in photon energy E? for a total of 21 bins. The values extracted for T , Ox and Oz are a first measurement of these quantities for this reaction and the beam asymmetry (?) measurement supplements the one previous measurement for this quantity and extends the energy range over which it has been extracted. The measurement of the recoil polarisation, P, is consistent with previous measurements. In a second analysis, the spin density matrix elements (SDMEs) for ? p ? p ? are extracted using similar analysis techniques. The results are presented as angular distributions (cos ?? ) for bins in photon energy E? for a total of 24 bins. This work is the first to extract all nine SDMEs for the full angular range of the ? meson production. A comparison is made to the predictions of the Vector Meson Dominance (VMD) model and the results provide evidence for contributing processes other than VMD, particularly at more backward angles of the ? meson production. The data also indicate non-helicity conserving process in both the s-channel and the t-channel. The results from the first analysis have been passed to the Juelich-Bonn theory group and the effect of including the new data within their dynamical coupled channel model is described. Several nucleon resonances are affected and the impact on the pole positions, widths and photon decay amplitudes of the affected resonances is described.

Clark, Louise↗

Multimodal photon and neutron imaging devices with fast event-by-event multisampling readout and optimized particle type discrimination

A particle imaging method for distinguishing between types of incident particles, such as neutrons, photons, and alphas, and improving the position resolution of particle imaging devices with matrix readout. The method includes high frequency multisampling readout electronics that provides the sequences of multiple measurements for each detected event, resulting in recorded detailed waveform information describing the signals. Such detailed information is used to approximate each signal waveform with a parameterized function in which the extracted parameter sets determine the type of the incident particle in an optimized fashion. The detailed event-by-event multisampling information for each signal readout channel in the matrix readout of the radiation imaging devices improves and optimizes the position resolution for variable shapes of the signals. Such devices can be used in mixed radiation fields, creating a new class of multimodal photon and neutron imagers.

Degtiarenko, Pavel V.↗

GPS-Based Gamma Survey for Characterizing and Decommissioning NORM Sites - 20389

Gamma survey techniques are an especially powerful decommissioning tool at naturally occurring radioactive material (NORM) sites due to both the low cost to obtain data over a large spatial scale and the abundance of gamma emitters in the uranium and thorium decay series. Gamma surveys are executed by coupling a detector - most often a sodium iodide crystal - to a global positioning system (GPS), then reporting a location and gross gamma reading coincidentally to a data logger. Systems may be carried by workers or mounted to a car, all-terrain vehicle, or unmanned aerial system (UAS). The resulting data set provides a high-resolution but low precision map of the gamma radiation field over the area surveyed. Frequently this map is also correlated to soil concentrations of NORM radionuclides (most often, Ra-226) and/or exposure rate. Gamma survey parameters such as movement speed, transect spacing, and data logging frequency define the spatial resolution of the resulting surface, and can be optimized depending on the desired survey sensitivity. This paper examines gamma survey as a tool for decommissioning NORM sites and provides an overview of current gamma survey technology designed to improve the efficiency and effectiveness of the decommissioning process. Topics to be discussed in the paper include: - An overview of gamma survey systems, and the utility of different delivery vehicles depending on desired cost, desired spatial resolution, and site topography. - The influence of physical detector characteristics on detection sensitivity and survey planning. - The tradeoff between high-resolution and large spatial extent, but inherently uncertain data, and low-resolution, low spatial extent, but highly certain data, as well as the specific utility of each of these types of data during NORM facility decommissioning. - Confounding variables that may limit the utility of gamma survey at some sites (e.g., radon gas and spatial heterogeneity / hot spots), and methods to plan for and control these conditions. Results show that the confounding variables, such as radon and data output can greatly influence the overall data quality associated with the decommissioning process. In addition, the use of real-time and aerial survey platforms provides a method for ensuring proper spatial extent of the data. When applied thoughtfully, gamma survey is a powerful tool for detecting NORM radionuclides in the environment and a cost-effective technique for identifying areas requiring remediation. However, entities performing or using gamma survey as a decommissioning tool must be aware of both its advantages and its limitations before basing remediation or regulatory action on gamma survey results. (authors)

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Quantification and assessment of the atmospheric boundary layer height measured during the AWAKEN experiment by a scanning LiDAR

The atmospheric boundary layer (ABL) height plays a key role in many atmospheric processes as one of the dominant flow length scales. However, a systematic quantification of the ABL height over the entire range of scales (i.e., with periods ranging from one minute to one year) is still lacking in literature. In this work, the ABL height is quantified based on high-resolution measurements collected by a scanning pulsed Doppler LiDAR during the recent American WAKE experimeNt (AWAKEN) campaign. The high availability of ABL height estimates (≈2200 collected over one year and each of them based on 10-min averaged statistics) allows to robustly assess five different ABL height models, i.e., one for convective thermal conditions and four for stable conditions. Thermal condition is quantified by a stability parameter spanning three orders of magnitude and probed by near-ground 3D sonic anemometry. The free-atmosphere stability, quantified by the Brunt–Väisälä frequency, is both calculated from simultaneous radiosonde measurements and obtained from the best fit of two of the chosen ABL height models. Good agreement is found between the data and three of the chosen models, quantified by mean absolute errors on the ABL height between 281 and 585 m. Furthermore, the seasonal variability of the convective ABL height model parameters (−15% to +23% with respect to the year baseline) agrees with the variability of buoyancy-generated turbulence caused by the variation in solar radiation throughout the year.

17 WIND ENERGY↗

g -mode oscillations in hybrid stars: A tale of two sounds

We study the principal core g-mode oscillation in hybrid stars containing quark matter and find that they have an unusually large frequency range ( ≈ 200 - 600 Hz) compared to ordinary neutron stars or self-bound quark stars of the same mass. Theoretical arguments and numerical calculations that trace this effect to the difference in the behaviour of the equilibrium and adiabatic sound speeds in the mixed phase of quarks and nucleons are provided. We propose that the sensitivity of core g-mode oscillations to non-nucleonic matter in neutron stars could be due to the presence of a mixed quark-nucleon phase. Based on our analysis, we conclude that for binary mergers where one or both components may be a hybrid star, the fraction of tidal energy pumped into resonant g-modes in hybrid stars can exceed that of a normal neutron star by a factor of 2-3, although resonance occurs during the last stages of inspiral. A self-bound star, on the other hand, has a much weaker tidal overlap with the g-mode. The cumulative tidal phase error in hybrid stars, ΔΦ = 0.5 rad, is comparable to that from tides in ordinary neutron stars, presenting a challenge in distinguishing between the two cases. Furthermore, should the principal g-mode be excited to sufficient amplitude for detection in a postmerger remnant with quark matter in its interior, its frequency would be a possible indication for the existence of non-nucleonic matter in neutron stars.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Characterizing Shielded Special Nuclear Material by Neutron Capture Gamma-Ray Multiplicity Counting

We present a new neutron multiplicity counting analysis and measurement method for neutron-shielded fissile material using neutron-capture gamma rays. Neutrons absorbed in shielding produce characteristic gamma rays that preserve the otherwise lost neutron multiplicity signature. Neutron multiplicity counting provides estimates of fission parameters, such as neutron leakage multiplication, spontaneous fissioner (e.g. Pu-240) mass, and (α,n) ratio. Standard neutron multiplicity counting can incorporate the new neutron-capture gamma-ray multiplicity counting technique to characterize previously degenerate or intractable source configurations by maximizing the multiplicity signature. The new method decouples neutron source-detector interferences, such as reflection and thermalization time in the detector, that could improve measurements of the mean neutron lifetime. We also develop a detector prototype for the multiplicity counting of neutron-capture gamma rays and present detector design considerations, such as detection material and shielding, to optimize the detection of the 2.2 MeV hydrogen capture gamma ray. We simulate the prototype neutron- capture gamma-ray multiplicity counter against the BeRP ball in polyethylene shells to inform future measurements.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Measuring Black Hole Light Echoes with Very Long Baseline Interferometry

Light passing near a black hole can follow multiple paths from an emission source to an observer due to strong gravitational lensing. Photons following different paths take different amounts of time to reach the observer, which produces an echo signature in the image. The characteristic echo delay is determined primarily by the mass of the black hole, but it is also influenced by the black hole spin and inclination to the observer. In the Kerr geometry, echo images are demagnified, rotated, and sheared copies of the direct image and lie within a restricted region of the image. Echo images have exponentially suppressed flux, and temporal correlations within the flow make it challenging to directly detect light echoes from the total light curve. In this Letter, we propose a novel method to search for light echoes by correlating the total light curve with the interferometric signal at high spatial frequencies, which is a proxy for indirect emission. We explore the viability of our method using numerical general relativistic magnetohydrodynamic simulations of a near-face-on accretion system scaled to M87-like parameters. We demonstrate that our method can be used to directly infer the echo delay period in simulated data. An echo detection would be clear evidence that we have captured photons that have circled the black hole, and a high-fidelity echo measurement would provide an independent measure of fundamental black hole parameters. Our results suggest that detecting echoes may be achievable through interferometric observations with a modest space-based very long baseline interferometry mission.

79 ASTRONOMY AND ASTROPHYSICS↗

Capability Demonstration of a 3D CdZnTe Detector on a High-Altitude Balloon Flight

In collaboration between the University of Michigan and Los Alamos National Laboratory, a 3D position-sensing CdZnTe (CZT) detector prototype was built and integrated into a high-altitude balloon platform to evaluate its performance in a space-like mixed-radiation environment. The detector prototype, Orion Eagle, was designed to operate in near-vacuum environments without any temperature regulation. Orion Eagle was hand-launched from NASA’s Columbia Scientific Balloon Facility (CSBF) at Fort Sumner, NM on September 26, 2021, and successfully operated throughout a 9-hour flight, which reached 38.5 km in altitude. The flight met its objectives, successfully detecting atmospheric gamma rays and galactic cosmic rays, and raising the Technical Readiness Level from 4 to 6 for large-volume 3D CZT detector technology for space applications. Ionization tracks produced by charged particles create spatial signatures in the detector that are distinguishable from discrete gamma-ray interactions. Therefore, the 3D position-sensing capabilities using pixelated electrodes on a CZT detector can help enable discrimination of background charged particles from gamma-ray events without an anticoincidence shield. The potential for background rejection capability, ambient-temperature operation, gamma-ray coded-aperture and Compton imaging, and near High Purity Germanium (HPGe) energy resolution motivate the use of large-volume 3D CZT imaging spectrometers in future space missions.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Shipping regulations lead to large reduction in cloud perturbations

Global shipping accounts for 13% of global emissions of SO2, which, once oxidized to sulfate aerosol, acts to cool the planet both directly by scattering sunlight and indirectly by increasing the albedo of clouds. This cooling due to sulfate aerosol offsets some of the warming effect of greenhouse gasses and is the largest uncertainty in determining the change in the Earth’s radiative balance by human activity. Ship tracks—the visible manifestation of the indirect of effect of ship emissions on clouds as quasi-linear features—have long provided an opportunity to quantify these effects. However, they have been arduous to catalog and typically studied only in particular regions for short periods of time. Using a machine-learning algorithm to automate their detection we catalog more than 1 million ship tracks to provide a global climatology. We use this to investigate the effect of stringent fuel regulations introduced by the International Maritime Organization in 2020 on their global prevalence since then, while accounting for the disruption in global commerce caused by COVID-19. We find a marked, but clearly nonlinear, decline in ship tracks globally: An 80% reduction in SO x emissions causes only a 25% reduction in the number of tracks detected.

54 ENVIRONMENTAL SCIENCES↗

Noise suppression for MHD characterization with electron cyclotron emission imaging 1D technique

Significant noise suppression for magnetohydrodynamics (MHD) mode characterization in the spatial and spectral domain is achieved by processing two-dimensional (2D) electron cyclotron emission imaging (ECEI) data with a one-dimensional (1D) ECEI technique using a short time window ($1\;{\text{ms}}$). The technique is applied to detect toroidal Alfven eigenmodes (TAEs) in the temporal spectrum and fit their radial envelope using the data from the DIII-D tokamak W-band 2D ECEI system. Using the data length (time window) of only 1 ${\text{ms}}$, the 1D ECEI can clearly detect the TAEs (~100 ${\text{kHz}}$) on the spectrum, while similar spectrum quality requires ~10 ${\text{ms}}$ data length with the cross power spectrum between two midplane ECEI channels. The 1D ECEI technique also effectively avoids biased fitting when resolving the fine structure of the TAE's radial envelope. The radially spatial resolution of 1D ECEI is constrained by the finite ECE radiation volume of the ECEI receiver. Here, with forward radiation modeling, we find the DIII-D ECEI system can sensitively measure the even parity MHD activities, for which the mode width is >15 mm, and tearing modes (odd parity MHD activities), for which the island full width is >30 mm.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

X-ray-line coincidence photopumping in a potassium-chlorine mixed plasma

Exploiting the multiple long pulse capability and suite of x-ray diagnostics of the Orion laser, we have set out to explore line coincidence photopuming—the enhancement in population of an atomic level brought on by resonant absorption of x rays from a different emitting ion. Unlike previous work, the two ions are in the same plasma and so the experiment is an x-ray analog of the well-known Bowen resonance fluorescence mechanism that operates in astrophysical situations in the optical region. Herein, our measurements have shown enhanced fluorescence in a chlorine plasma, attributable to line coincident photopumping from co-mixed potassium ions. To detect this relatively low signal-to-noise phenomenon, the data from multiple shots are combined, and the statistical method of bootstrapping is used to assign a confidence value to the measured enhancement, resulting in an estimate of the enhancement of 39 ± 18 16 % compared to the null case, where no pumping occurs. The experimental results have been compared to coupled radiation-transport and radiation hydrodynamics simulations using the CRETIN code together with the NYM radiation hydrodynamics model and agreement has been found, with the simulations also predicting modest enhancement.

74 ATOMIC AND MOLECULAR PHYSICS↗

Validation of the Cloud_CCI (Cloud Climate Change Initiative) cloud products in the Arctic

The role of clouds in the Arctic radiation budget is not well understood. Ground-based and airborne measurements provide valuable data to test and improve our understanding. However, the ground-based measurements are intrinsically sparse, and the airborne observations are snapshots in time and space. Passive remote sensing measurements from satellite sensors offer high spatial coverage and an evolving time series, having lengths potentially of decades. However, detecting clouds by passive satellite remote sensing sensors is challenging over the Arctic because of the brightness of snow and ice in the ultraviolet and visible spectral regions and because of the small brightness temperature contrast to the surface. Consequently, the quality of the resulting cloud data products needs to be assessed quantitatively. In this study, we validate the cloud data products retrieved from the Advanced Very High Resolution Radiometer (AVHRR) post meridiem (PM) data from the polar-orbiting NOAA-19 satellite and compare them with those derived from the ground-based instruments during the sunlit months. The AVHRR cloud data products by the European Space Agency (ESA) Cloud Climate Change Initiative (Cloud_CCI) project uses the observations in the visible and IR bands to determine cloud properties. The ground-based measurements from four high-latitude sites have been selected for this investigation: Hyytiälä (61.84°N, 24.29°E), North Slope of Alaska (NSA; 71.32°N, 156.61°W), Ny-Ålesund (Ny-Å; 78.92°N, 11.93°E), and Summit (72.59°N, 38.42°W). The liquid water path (LWP) ground-based data are retrieved from microwave radiometers, while the cloud top height (CTH) has been determined from the integrated lidar–radar measurements. The quality of the satellite products, cloud mask and cloud optical depth (COD), has been assessed using data from NSA, whereas LWP and CTH have been investigated over Hyytiälä, NSA, Ny-Å, and Summit.

54 ENVIRONMENTAL SCIENCES↗

Characterization of PIPS detectors for measurement of radioxenon

The International Monitoring System arm of the Comprehensive Nuclear-Test-Ban Treaty Organization utilizes sampling of atmospheric radioxenon to scan the world for nuclear testing events. Current designs utilized in the field involve plastic scintillator cells run in coincidence with Sodium Iodide (NaI) or High Purity Germanium (HPGe) detectors. The use of plastic scintillators as electron detectors exhibit some issues in comparison to other materials. Silicon detectors are analyzed as an alternative to plastic scintillators for beta detection based on their higher energy resolution and lowered memory effect. A radioxenon detection setup was created with the intent of measuring radioxenon samples using coincidence counting between silicon and NaI detectors as well as silicon and HPGe. Finally, the absolute efficiency of both setups is calculated and compared.

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗

Blowing Snow at McMurdo Station, Antarctica During the AWARE Field Campaign: Surface and Ceilometer Observations

Blowing snow (BLSN) is an impactful process in cold climates, affecting regional thermodynamics, radiation properties, and the surface mass balance of snow. Though it has significant climatic impacts, the process is still poorly understood and not widely included in weather and climate models. In 2016, the AWARE Field Campaign saw the deployment of a large suite of in situ and remote sensing instruments to McMurdo Station, Antarctica allowing for investigation of BLSN. A ceilometer–based BLSN detection algorithm used elsewhere in Antarctica is applied to data from AWARE, yielding a BLSN frequency of 14.1% compared to 8.2% as detected by human observers. To increase confidence in detections, the algorithm is updated to have shorter temporal averaging and to include a variety of meteorological thresholds to limit false detections due to fog. Efforts to incorporate a laser disdrometer into the algorithm were unsuccessful. An unphysical dependence of particle size distributions on wind speed is found suggesting observations are problematic at wind speeds greater than 10 m s –1 . The revised algorithm detected a BLSN frequency of 7.4%, increasing agreement with human observations and confidence that the process is actively occurring at the observation site. Furthermore, these observations are put into context of a climatology of human observations of BLSN at McMurdo station from 2002–2018. An annual average of 8.0%–14.0% is estimated, with a total annual range of 3.4%–21.3%. Regardless of whether BLSN is observed by humans or instrument, the majority of cases at this location are associated with ongoing precipitation.

54 ENVIRONMENTAL SCIENCES↗

Electron cyclotron emission detection of neoclassical tearing modes for control for ITER

Successful operation of ITER requires control of magnetic instabilities including neoclassical tearing modes (NTMs) that can degrade confinement and lead to disruption. Low latency detection by electron cyclotron emission (ECE) diagnostics has been demonstrated in a few current experiments. Using a synthetic diagnostic, we demonstrate low latency NTM detection for ITER with plasmas described by ITER IMAS database scenarios and with realistic limitations imposed on the instrumentation by these high temperature scenarios. 2/1 NTMs are detected 430 ms after magnetic island seeding and before island locking. The radiometer configuration was optimized using simulation, and the smallest detectable island size was explored. Island sizes of ∼3 cm are detectable at the 2/1 surface. The simulated signals incorporate recent physics models for island growth and rotation, which show early locking and continued island growth after locking and before disruption. This work determines limits for ITER ECE spatial resolution imposed by relativistic broadening of channels, which informs hardware design. Real-time detection is demonstrated in hardware that is required by ITER, including on an NI PXI-7853R FPGA system. Development of a synthetic diagnostic and details of the hardware will be discussed.

Cyclotron radiation↗

Imaging of Calibrated Defects in Additively Manufactured Materials: Pulsed Thermal Tomography Nondestructive Examination of Additively Manufactured Reactor Materials and Components

Additive manufacturing (AM, or 3D printing) for commercial nuclear energy applications is an emerging method for cost-efficient manufacturing aimed at replacing aging nuclear reactor parts and reducing costs for new construction. Known material flaws in AM include low-density regions consisting of non-sintered powder, which have to be detected to ensure the safety of long-term performance nuclear reactor components. Currently, limited options are available for nondestructive evaluation (NDE), either during or post manufacturing. As a solution to NDE of AM, we are developing pulsed thermal imaging which is non-contact, one-sided, and scalable to arbitrary size and shape of the AM parts. Pulsed thermography (PT) system utilizes a high intensity flash lamp to rapidly heat surface of sample, and a high sensitivity fast-frame megapixel infrared (IR) camera to capture data of surface temperature variations. The acquired data cube consists of a stack of surface temperature images taken at different times. Information about material internal defects is extracted by analyzing the data cube. This report provides results of preliminary performance evaluation of pulsed thermal imaging capability in detection of imprinted flaws in AM metallic structures. The flaws were introduced into AM parts as imprinted hemispherical low density regions, consisting of trapped un-sintered metallic powder. Specimens for developed for this study consisted of AM stainless steel 316 and Inconel 718 plates. The diameters of imprinted defects varied from 1mm to 8mm, and their depths below the plate flat surface varied between 1mm and 6mm. Pulsed thermal tomography (PTT) processes the measured data cube to obtain 3D reconstructions of material effusivity using a unique inversion algorithm developed at Argonne. PTT has been previously used in imaging of similar size flat bottom hole (FBH) simulated defects in stainless steel 316 and Inconel 718 specimens. In the study involving AM specimens, PTT imaging results have shown that 1mm-diameter defects located 1mm and 2mm below the surface of specimens were detectable. Larger size defects were detectable at greater depth. We also explored an alternative approach to detection of material flaws in PT data cube, which is using neural learning-based approach to blind source separation. Detection of small material defects requires finding features in the data cube which have signal contrast levels approaching sensitivity limit of IR camera. In this study, an optimized Neural Learning based Blind Source Separation (NLBSS) algorithm, including Principal Component Analysis (PCA), and Independent Component Analysis (ICA) is demonstrated to automatically extract principal temporal and spatial features of thermography frames to enhance flaw detection. By using the NLBSS algorithm, material internal defects can be automatically detected. Furthermore, this processing approach compensates for experimental thermal imaging artifacts, such as noise and uneven heating. By merging artificial intelligence with phtotothermics, the NDE system detects internal calibrated defects of various sizes and depths in AM nuclear-grade metallic alloys.

36 MATERIALS SCIENCE↗

Nuclear Physics of Compact Binaries with GADGET

The research goal of this project was to experimentally constrain the thermonuclear rate of the 15 O(α, Υ) 19 Ne reaction, whose uncertainty has a strong influence on the modeling of astrophysical Type-I X-ray bursts on accreting neutron stars. To this end, Experiment 21072 was run in November 2022 at the Facility for Rare Isotope Beams using the GADGET II detection system. The limited scope and duration of this award included work in the year following the experiment: drafting a technical paper on the time projection chamber of the GADGET II detection system, and analysis of data from Experiment 21072. The award contributed to the education and development of the scientific and technical workforce by partially supporting one postdoctoral Research Associate who did this work.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Gravity as a Portal to Reheating, Leptogenesis and Dark Matter

Considering graviton as the only messenger that exists between the inflaton, the dark sector and the Standard Model (SM), we show, it is possible to simultaneously generate the observed relic density of dark matter (DM), the baryon asymmetry via leptogenesis, as well as successful reheating after inflation. Assuming the inflaton Φ oscillates in a monomial potential V(Φ) ∝ Φ k at the end of inflation, reheating via minimal gravitational interaction turns out to be excluded due to excessive production of gravitational wave (GW) energy density from inflation. We thus (a) extend the minimal model by considering a non-minimal gravitational contribution to radiation and (b)) propose an explanation for the PeV excess observed by IceCube, when the DM has an explicit Yukawa coupling to the SM leptong and Higgs. We also propose a novel scenario, where the gravitational production is a two-step process, through the production of a pair of scalars, that eventually decay into fermionic final states. Our framework gives rise to detectable primordial GW signal, that falls within the sensitivity of several proposed GW detectors.

Barman, Basabendu↗