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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 1,153 records · Page 64
All sourcesNASA NTRSDOE OSTI
NASA NTRS2015

Progress Towards Improved Analysis of TES X-ray Data Using Principal Component Analysis

The traditional method of applying a digital optimal filter to measure X-ray pulses from transition-edge sensor (TES) devices does not achieve the best energy resolution when the signals have a highly non-linear response to energy, or the noise is non-stationary during the pulse. We present an implementation of a method to analyze X-ray data from TESs, which is based upon principal component analysis (PCA). Our method separates the X-ray signal pulse into orthogonal components that have the largest variance. We typically recover pulse height, arrival time, differences in pulse shape, and the variation of pulse height with detector temperature. These components can then be combined to form a representation of pulse energy. An added value of this method is that by reporting information on more descriptive parameters (as opposed to a single number representing energy), we generate a much more complete picture of the pulse received. Here we report on progress in developing this technique for future implementation on X-ray telescopes. We used an 55Fe source to characterize Mo/Au TESs. On the same dataset, the PCA method recovers a spectral resolution that is better by a factor of two than achievable with digital optimal filters.

Low-temperature detectors A[center dot] Transition↗
DOE OSTI2022

Studies of EC pre-ionization in DIII-D to support development of ITER plasma initiation

New experiments have been conducted at DIII-D to improve the physics understanding of plasma initiation assisted by electron cyclotron (EC) wave injection, allowing better extrapolation to ITER. This has been achieved by applying an EC pulse prior to start of the inductive plasma initiation (i.e. the generation of a loop voltage). A pre-plasma was formed during the EC pulse that was characterized in terms of the maximum density and temperature. Parametric scans were performed to study the influence of the EC injected power, EC injection angle, and pre-fill gas pressure on the pre-plasma creation process. These experiments showed that pre-ionized plasma of good quality can have a significant effect on the subsequent V loop induced plasma initiation process, i.e. a high density pre-plasma, increases the plasma current rise and speed at which ionization is achieved when the V loop is applied. Here, a good quality pre-plasma is one that achieved a significant degree of ionization, mainly obtained by providing sufficient ECH power in DIII-D of the order of 1 MW. It was found that a minimum EC power of 0.5 MW was required in DIII-D to create ionization, and this would scale to a minimum power of roughly 6.5 MW for ITER.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2020

Experimental demonstration of externally driven millimeter-wave particle accelerator structure

We report the experimental demonstration of a mm-wave electron accelerating structure powered by a high-power rf source. We demonstrate reliable coupling of an unprecedented rf power—up to 575kW into the mm-wave accelerator structure using a quasi-optical setup. This standing wave accelerating structure consists of a single-cell copper cavity and a Gaussian to TM 01 mode converter. The accelerator structure is powered by 110 GHz, 10-ns long rf pulses. These pulses are chopped from 3 microsecond pulses from a gyrotron oscillator using a laser-driven silicon switch. We show an unprecedented high gradient up to 230MV/m that corresponds to a peak surface electric field of more than 520 MV/m. We have achieved these results after conditioning the cavity with more than 100,000 pulses. We also report preliminary measurements of rf breakdown rates, which are important for understanding rf breakdown physics in the millimeter-wave regime. Furthermore, these results open up many frontiers for applications not only limited to the next generation particle accelerators but also x-ray generation, probing material dynamics, and nonlinear light-matter interactions at mm-wave frequency.

43 PARTICLE ACCELERATORS↗
DOE OSTI2023

Reactivity of radiolytically and photochemically generated tertiary amine radicals towards a CO 2 reduction catalyst

Homogeneous solar fuels photocatalytic systems often require several additives in solution with the catalyst to operate, such as a photosensitizer (PS), Brønsted acid/base, and a sacrificial electron donor (SED). Tertiary amines, in particular triethylamine (TEA) and triethanolamine (TEOA), are ubiquitously deployed in photocatalysis applications as SEDs and are capable of reductively quenching the PS’s excited state. Upon oxidation, TEA and TEOA form TEA •+ and TEOA •+ radical cations, respectively, which decay by proton transfer to generate redox non-innocent transient radicals, TEA • and TEOA • , respectively, with redox potentials that allow them to participate in an additional electron transfer step, thus resulting in net one-photon/two-electron donation. However, the properties of the TEA • and TEOA • radicals are not well understood, including their reducing powers and kinetics of electron transfer to catalysts. Herein, we have used both pulse radiolysis and laser flash photolysis to generate TEA • and TEOA • radicals in CH 3 CN, and combined with UV/Vis transient absorption and time-resolved mid-infrared spectroscopies, we have probed the kinetics of reduction of the well-established CO 2 reduction photocatalyst, fac-ReCl(bpy)(CO) 3 (bpy = 2,2'-bipyridine), by these radicals [k TEA• = (4.4 ± 0.3) × 10 9 M –1 s –1 and k TEOA• = (9.3 ± 0.6) × 10 7 M –1 s –1 ]. The ~50× smaller rate constant for TEOA • indicates, that in contrast to a previous assumption, TEA • is a more potent reductant than TEOA • (by ~0.2 V, as estimated using the Marcus cross relation). This knowledge will aid in the design of photocatalytic systems involving SEDs. Furthermore, we also show that TEA can be a useful radiolytic solvent radical scavenger for pulse radiolysis experiments in CH 3 CN, effectively converting unwanted oxidizing radicals into useful reducing equivalents in the form of TEA • radicals.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2022

Homogeneous, Micron-Scale High-Energy-Density Matter Generated by Relativistic Laser-Solid Interactions

Short-pulse, laser-solid interactions provide a unique platform for studying complex high-energy-density mat ter. We present the first demonstration of solid density, micron-scale keV plasmas uniformly heated by a high contrast, 400 nm laser at intensities up to 2×10 21 W/cm 2 . High-resolution spectral analysis of X-ray emission reveals uniform heating up to 3.0 keV over 1 µm depths. Particle-in-cell simulations indicate the production of a uniformly heated keV plasma to depths of 2 µm. The significant bulk heating and presence of highly-ionized ions deep within the target are attributed to the few MeV hot electrons that become trapped and undergo refluxing within the target sheath fields. In conclusion, these conditions enable the differentiation of atomic physics models such as ionization potential depression in high energy density environments.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
NASA NTRS1980

Ultrasonic spectrum analysis using frequency-tracked gated RF pulses

A new method of ultrasonic frequency analysis is introduced which employs frequency-tracked gated RF drive pulses rather than shock-excited broadband spikes to generate the ultrasonic waveform. The new technique, a variation of the sampled-continuous wave technique, eliminates problems associated with finite pulse widths of conventional methods. It is shown to yield correct ultrasonic wave velocity measurements of the sample irrespective of receiver gate width or position provided any portions of two successive echoes are gated simultaneously into the spectrum analyzer. The experimental observations are substantiated by a theoretical model based on the time-frequency domain formulation of ultrasonic frequency analysis.

Cantrell, J. H., Jr.↗
NASA NTRS1993

The solid state detector technology for picosecond laser ranging

We developed an all solid state laser ranging detector technology, which makes the goal of millimeter accuracy achievable. Our design and construction philosophy is to combine the techniques of single photon ranging, ultrashort laser pulses, and fast fixed threshold discrimination while avoiding any analog signal processing within the laser ranging chain. The all solid state laser ranging detector package consists of the START detector and the STOP solid state photon counting module. Both the detectors are working in an optically triggered avalanche switching regime. The optical signal is triggering an avalanche current buildup which results in the generation of a uniform, fast risetime output pulse.

Prochazka, Ivan↗
NASA NTRS2005

Vortex Rings Generated by a Shrouded Hartmann-Sprenger Tube

The pulsed flow emitted from a shrouded Hartmann-Sprenger tube was sampled with high-frequency pressure transducers and with laser particle imaging velocimetry, and found to consist of a train of vortices. Thrust and mass flow were also monitored using a thrust plate and orifice, respectively. The tube and shroud lengths were altered to give four different operating frequencies. From the data, the radius, velocity, and circulation of the vortex rings was obtained. Each frequency corresponded to a different length to diameter ratio of the pulse of air leaving the driver shroud. Two of the frequencies had length to diameter ratios below the formation number, and two above. The formation number is the value of length to diameter ratio below which the pulse converts to a vortex ring only, and above which the pulse becomes a vortex ring plus a trailing jet. A modified version of the slug model of vortex ring formation was used to compare the observations with calculated values. Because the flow exit area is an annulus, vorticity is shed at both the inner and outer edge of the jet. This results in a reduced circulation compared with the value calculated from slug theory accounting only for the outer edge. If the value of circulation obtained from laser particle imaging velocimetry is used in the slug model calculation of vortex ring velocity, the agreement is quite good. The vortex ring radius, which does not depend on the circulation, agrees well with predictions from the slug model.

DeLoof, Richard L.↗
DOE OSTI2023

Optimal gas cooling with minimal aero-opticaldistortion for next generation high-average-power lasers (Progress report, Year 2)

Next-generation lasers that combine high-peak-power ultrashort pulses with high repetition rates have the potential to efficiently deliver the high-average-power outputs required for inertial fusion energy generation, laser-based particle acceleration, and to generate compact secondary x- and 𝛾-ray radiation sources, among others. The combination of long gain length with high surface-to-volume ratio to remove residual heat makes gas-cooled multi-slab amplifier heads an inherently aperture- and average power scalable technology that enables this new class of solid-state lasers, and their thermal management becomes the most pressing technical challenge. As the index-of refraction depends on the gas density, heat removal from the slab surfaces unavoidably entails scattering of propagated light from regions of high temperature fluctuations. The requirement to maximize convective heat extraction from the gain medium under the constraint of minimum optical aberration of the beam renders amplifier slab cooling a technological challenge at the intersection of aero-optics, fluid-mechanics and heat transfer. The goal of this research is to leverage computational fluid dynamics and aero optics simulations of different levels of fidelity to devise a numerical modeling and optimization framework for gas-cooled multi-slab amplifiers. The project will be conducted in close collaboration with the Advanced Photon Technologies Group at Lawrence Livermore National Laboratory, where a gas-cooled test stand for laser materials and thermal management structures will be developed and installed. The final goal of the collaborative effort is to manufacture and benchmark a physical prototype of an numerically optimized amplifier head design. Measurement data on solid-state and thermo-optical distortions will be used for the validation of the numerical models. The key technical challenge in this multi-objective design problem is that of balancing optimal heat removal with minimal optical distortion. To facilitate computationally efficient design optimization and, at the same time, deepen our basic understanding of the interaction of light with turbulence, a complementary study that combines high and low-fidelity flow simulations and aero-optical models is proposed. Along the lines of these two objectives and solution strategies, the project is organized into two thrusts.

42 ENGINEERING↗
DOE OSTI2021

Bright, single helicity, high harmonics driven by mid-infrared bicircular laser fields

High-harmonic generation (HHG) is a unique tabletop light source with femtosecond-to-attosecond pulse duration and tailorable polarization and beam shape. Here, we use counter-rotating femtosecond laser pulses of 0.8 µm and 2.0 μm to extend the photon energy range of circularly polarized high-harmonics and also generate single-helicity HHG spectra. By driving HHG in helium, we produce circularly polarized soft x-ray harmonics beyond 170 eV—the highest photon energy of circularly polarized HHG achieved to date. In an Ar medium, dense spectra at photon energies well beyond the Cooper minimum are generated, with regions composed of a single helicity—consistent with the generation of a train of circularly polarized attosecond pulses. Finally, we show theoretically that circularly polarized HHG photon energies can extend beyond the carbon K edge, extending the range of molecular and materials systems that can be accessed using dynamic HHG chiral spectro-microscopies.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2025

Tailoring spectral properties for entangled photon generation

The linear intensity scaling of entangled two-photon absorption (ETPA) offers a fundamental mechanism to enable nonlinear optical spectroscopy and microscopy under a substantially lower excitation power than is currently feasible. However, the long data acquisition time and low signal-to-noise ratio in reported ETPA-based spectroscopic and microscopic studies prevent its widespread application. To gain the full potential of this novel quantum light approach, it is essential to optimize entangled photon generation for significantly enhanced ETPA responses. Here, we report a new quantum light source by combining entangled photon generation with free-space femtosecond pump-pulse shaping. Here, through measurements of singles and coincidence counts by varying the patterns applied to a spatial light modulator to control the spectral widths of the pump pulses, we reveal strong dependence of the singles and coincidence count rates as well as their ratios on the spectral widths of pump pulses. An optimal spectral width for the highest ratios between the coincidence photon and the signal or idler photon count rates is also determined. Identification of such optimal spectral widths for entangled photon generation in the presence of postgeneration spectral selection makes this quantum light source a promising choice for ETPA-based spectroscopy and imaging.

Photon pairs & parametric down-conversion↗
NASA NTRS2004

Membrane Vibration Analysis Above the Nyquist Limit with Fluorescence Videogrammetry

A new method for generating photogrammetric targets by projecting an array of laser beams onto a membrane doped with fluorescent laser dye has recently been developed. In this paper we review this new fluorescence based technique, then proceed to show how it can be used for dynamic measurements, and how a short pulsed (10 ns) laser allows the measurement of vibration modes at frequencies several times the sampling frequency. In addition, we present experimental results showing the determination of fundamental and harmonic vibration modes of a drum style dye-doped polymer membrane tautly mounted on a 12-inch circular hoop and excited with 30 Hz and 62 Hz sinusoidal acoustic waves. The projected laser dot pattern was generated by passing the beam from a pulsed Nd:YAG laser though a diffractive optical element, and the resulting fluorescence was imaged with three digital video cameras, all of which were synchronized with a pulse and delay generator. Although the video cameras are capable of 240 Hz frame rates, the laser s output was limited to 30 Hz and below. Consequently, aliasing techniques were used to allow the measurement of vibration modes up to 186 Hz with a Nyquist limit of less than 15 Hz.

Dorrington, Adrian A.↗
DOE OSTI2022

Non-premixed counterflow methane flames in DC/AC/NS electric fields

The response of counterflow diffusion flames to sub-breakdown DC and AC electric fields, as well as their superposition with ns pulse discharge waveforms, is studied in the plane-to-plane electrode geometry. Sub-breakdown DC and low-frequency AC electric fields cause the flame displacement toward the grounded electrode, in the direction of the applied field, indicating that the body force on the positive ions exceeds that on the electrons and negative ions. As the AC frequency increases, the flame response becomes less pronounced, due to the reduction of the electrohydrodynamic (EHD) body force impulse over the AC half-period. The electric field in the electrode gap is determined by ps Electric Field Induced Second Harmonic (E-FISH) generation, with absolute calibration using sub-breakdown ns pulses overlapped with the measured electric field waveform. The results show that the electric field distribution across the flame in the current saturation regime follows the Laplacian field. This indicates that the space charge density in the gap is too low to distort the applied DC or AC field, consistent with the kinetic modeling predictions. Combining a nanosecond pulse discharge with a sub-breakdown DC field generates a diffuse plasma across the entire gap. Time-resolved and spatially resolved measurements of the electric field in the discharge indicate the ionization wave propagation between the electrodes. The present results do not exhibit a detectable flame displacement enhancement by ns discharge pulses combined with a sub-breakdown field, observed previously. Kinetic modeling calculations show that the absence of this effect in the plane-to-plane geometry is due to the rapid plasma self-shielding. This indicates that alternative electrode geometries limiting the self-shielding would be more effective for the plasma / electric field enhanced flameholding and flame stabilization applications.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2020

Attosecond science based on high harmonic generation from gases and solids

Recent progress in high power ultrafast short-wave and mid-wave infrared lasers has enabled gas-phase high harmonic generation (HHG) in the water window and beyond, as well as the demonstration of HHG in condensed matter. In this Perspective, we discuss the recent advancements and future trends in generating and characterizing soft X-ray pulses from gas-phase HHG and extreme ultraviolet (XUV) pulses from solid-state HHG. Then, we discuss their current and potential usage in time-resolved study of electron and nuclear dynamics in atomic, molecular and condensed matters.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
NASA NTRS2008

Mitigating Photon Jitter in Optical PPM Communication

A theoretical analysis of photon-arrival jitter in an optical pulse-position-modulation (PPM) communication channel has been performed, and now constitutes the basis of a methodology for designing receivers to compensate so that errors attributable to photon-arrival jitter would be minimized or nearly minimized. Photon-arrival jitter is an uncertainty in the estimated time of arrival of a photon relative to the boundaries of a PPM time slot. Photon-arrival jitter is attributable to two main causes: (1) receiver synchronization error [error in the receiver operation of partitioning time into PPM slots] and (2) random delay between the time of arrival of a photon at a detector and the generation, by the detector circuitry, of a pulse in response to the photon. For channels with sufficiently long time slots, photon-arrival jitter is negligible. However, as durations of PPM time slots are reduced in efforts to increase throughputs of optical PPM communication channels, photon-arrival jitter becomes a significant source of error, leading to significant degradation of performance if not taken into account in design. For the purpose of the analysis, a receiver was assumed to operate in a photon- starved regime, in which photon counts follow a Poisson distribution. The analysis included derivation of exact equations for symbol likelihoods in the presence of photon-arrival jitter. These equations describe what is well known in the art as a matched filter for a channel containing Gaussian noise. These equations would yield an optimum receiver if they could be implemented in practice. Because the exact equations may be too complex to implement in practice, approximations that would yield suboptimal receivers were also derived.

Moision, Bruce↗
DOE OSTI2020

Accuracy of the duration estimates of ultrashort laser pulses using a single-shot second-order intensity autocorrelator

The accuracy of estimating the duration of single-cycle laser pulses with centre wavelengths of 910 and 780 nm is analysed using a single-shot second-order intensity autocorrelator. It is shown that estimates of the single-cycle pulse duration with an error of less than 5 % require the use of KDP crystals with a thickness of no more than 10 μm for the second harmonic generation. At the same time, to estimate the duration of a transform-limited pulse containing ten optical cycles, the crystal thickness can be up to 1 mm. In this case, at an optimum angle of convergence of the first-harmonic beams, the duration estimation error is less than 2 %. (paper)

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗