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At least 1,153 records · Page 64
All sourcesNASA NTRSDOE OSTI
NASA NTRS1986

Effects of test facility contaminants on supersonic hydrogen-air diffusion flames

Results are presented from an analytical assessment of the effects of NO and H2O in air on the ignition and reaction of hydrogen. Three flow models of the burning process were used, each including a 32 reaction chemistry mechanism. These models were a plug flow reactor to determine ignition and reaction times; a well-stirred reactor to assess flame stability or blow-off; and a parabolic Navier-Stokes code to examine the diffusion flame combustion. The diffusion flame was computed for a cold supersonic H2 jet coaxial with a supersonic air stream at a static temperature of 1100 K and a pressure of 1 atmosphere.

Rogers, R. Clayton↗
NASA NTRS1986

Effects of test facility contaminants on supersonic hydrogen-air diffusion flames

Results are presented from an analytical assessment of the effects of NO and H2O in air on the ignition and reaction of hydrogen. Three flow models of the burning process were used, each including a 32 reaction chemistry mechanism. These models were a plug flow reactor to determine ignition and reaction times; a well-stirred reactor to assess flame stability or blow-off, and a parabolic Navier Stokes code to examine the diffusion flame combustion. The diffusion flame was computed for a cold supersonic H2 jet coaxial with a supersonic air stream at a static temperature of 1100 K and a pressure of 1 atmosphere.

Rogers, R. Clayton↗
NASA NTRS1987

Opposed jet burner studies of effects of CO, CO2, and N2 air-contaminants on hydrogen-air diffusion flames

The blowoff/restore characteristics for jets of various H2/N2 mixtures opposed to jets of air contaminated by N2, CO, and CO2 have been determined using a counterflow diffusion flame formed by a tubular opposed jet burner. Both blowoff and restore limits are found to be sensitive to fuel and air composition. Empirically derived variations in the limits of the average mass flux of incoming H2 with percent contaminant, at fixed incoming fuel and H2/O2 inputs, are used to quantify the effects of oxygen dilution, flame augmentation, and flame retardation by N2, CO, and CO2 contaminants. The implications of the results are discussed.

Guerra, Rosemary↗
NASA NTRS1988

Modeling of hydrogen-air diffusion flame

The present research objective is to determine the effects of contaminants on extinction limits of simple, well defined, counterflow Hydrogen 2-air diffusion flames, with combustion at 1 atmosphere. Results of extinction studies and other flame characterizations, with appropriate mechanistic modeling (presently underway), will be used to rationalize the observed effects of contamination over a reasonably wide range of diffusion flame conditions. The knowledge gained should help efforts to anticipate the effects of contaminants on combustion processes in Hydrogen 2-fueled scramjets.

Isaac, Kakkattukuzhy↗
NASA NTRS1989

Modeling of hydrogen-air diffusion flame

An analytical and computational study of opposed jet diffusion flame for the purpose of understanding the effects of contaminants in the reactants and thermal diffusion of light species on extinction and reignition of diffusion flames is in progress. The methodologies that have been attempted so far are described. Results using a simple, one-step reaction for the hydrogen-air counterflow diffusion flame are presented. These results show the correct trends in the profiles of chemical species and temperature. The extinction limit can be clearly seen in the plot of temperature vs. Damkohler number.

Isaac, K. M.↗
NASA NTRS1989

Determination of combustion gas temperatures by infrared radiometry in sooting and nonsooting flames

Flame temperatures in nonsooting and sooting environments were successfully measured by radiometry for pre-mixed propane-oxygen laminar flames stabilized on a water-cooled, porous sintered-bronze burner. The measured temperatures in the nonsooting flames were compared with fine-wire thermocouple measurements. The results show excellent agreement below 1700 K, and when the thermocouple measurements were corrected for radiation effects, the agreement was good for even higher temperatures. The benefits of radiometry are: (1) the flow is not disturbed by an intruding probe, (2) calibration is easily done using a blackbody source, and (3) measurements can be made even with soot present. The theory involved in the radiometry measurements and the energy balance calculations used to correct the thermocouple temperature measurements are discussed.

Lyons, Valerie J.↗
NASA NTRS1989

A study of the propagation, dynamics, and extinguishment of cellular flames using microgravity techniques

The characteristics of premixed gas flames in mixtures with low Lewis numbers, free of natural convection effects, were investigated and found to be dominated by diffusive-thermal instabilities. For sufficiently reactive mixtures, cellular structures resulting from these instabilities were observed and found to spawn new cells in regular patterns. For less reactive mixtures, cells formed shortly after ignition but did not spawn new cells; instead these cells evolved into a flame structure composed of stationary, apparently stable spherical flamelets. As a result of these phenomena, well-defined flammability limits were not observed. The experimental results are found to be in qualitative agreement with a simple analytical model based on the interaction of heat release due to chemical reaction, differential diffusion of thermal energy and mass, flame front curvature, and heat losses due to gas radiation.

Ronney, Paul D.↗
NASA NTRS1989

Opposed jet diffusion flames of nitrogen-diluted hydrogen vs air - Axial LDA and CARS surveys; fuel/air rates at extinction

An experimental study of H-air counterflow diffusion flames (CFDFs) is reported. Coaxial tubular opposed jet burners were used to form dish-shaped CFDFs centered by opposing laminar jets of H2/N2 and air in an argon bath at 1 atm. Jet velocities for extinction and flame restoration limits are shown versus input H2 concentration. LDA velocity data and CARS temperature and absolute N2, O2 density data give detailed flame structure on the air side of the stagnation point. The results show that air jet velocity is a more fundamental and appropriate measure of H2-air CFDF extinction than input H2 mass flux or fuel jet velocity. It is proposed that the observed constancy of air jet velocity for fuel mixtures containing 80 to 100 percent H2 measure a maximum, kinetically controlled rate at which the CFDF can consume oxygen in air. Fuel velocity mainly measures the input jet momentum required to center an H2/N2 versus air CFDF.

Pellett, G. L.↗
NASA NTRS1989

A Theoretical Study of Propagation and Extinction of Nonsteady Spherical Flame Fronts

Freely propagating expanding spherical flame fronts are studied analytically using the method of activation energy asymptotics. Effects of Lewis number (Le), curvature, heat loss, and thermal expansion on propagation rates and extinction conditions are examined. The behavior of spherical flame fronts is found to be determined primarily by the values of Le and a heat-loss parameter. Results are compared to recent experimental observations of spherical flame fronts in mixtures near the flammability limits; for Le less than 1, it is found that many of the features of these experimental results are described by the analysis presented here. For Le greater than 1, however, unrealistic dynamic behavior is predicted due to the nature of diffusive-thermal instabilities under these conditions.

Ronney, P. D.↗
NASA NTRS1989

Analysis of opposed jet hydrogen-air counter flow diffusion flame

A computational simulation of the opposed-jet diffusion flame is performed to study its structure and extinction limits. The present analysis concentrates on the nitrogen-diluted hydrogen-air diffusion flame, which provides the basic information for many vehicle designs such as the aerospace plane for which hydrogen is a candidate as the fuel. The computer program uses the time-marching technique to solve the energy and species equations coupled with the momentum equation solved by the collocation method. The procedure is implemented in two stages. In the first stage, a one-step forward overal chemical reaction is chosen with the gas phase chemical reaction rate determined by comparison with experimental data. In the second stage, a complete chemical reaction mechanism is introduced with detailed thermodynamic and transport property calculations. Comparison between experimental extinction data and theoretical predictions is discussed. The effects of thermal diffusion as well as Lewis number and Prandtl number variations on the diffusion flame are also presented.

Ho, Y. H.↗
NASA NTRS1990

Cellular structure of lean hydrogen flames in microgravity

Detailed, time-dependent, two-dimensional numerical simulations of premixed laminar flames have been used to study the initiation and subsequent development of cellular structures in lean hydrogen-air flames. The model includes detailed hydrogen-oxygen combustion with 24 elementary reactions of eight reactive species and a nitrogen diluent, molecular diffusion of all species, thermal conduction, viscosity, and convection. This model has been used to study the nonlinear evolution of cellular flame structure and shows that cell splitting, as observed in experiments, can be predicted numerically for sufficiently reactive mixtures. The structures that evolved also resembled the cellular structures observed in experiments. The present study shows that the 'cell-split limit' postulated from experimental observations is an intrinsic property of the mixture and that external factors such as heat losses are not necessary to cause this limit.

Patnaik, G.↗
NASA NTRS1990

UV Raman spectroscopy of H2-air flames excited with a narrowband KrF laser

Raman spectra of H2 and H2O in flames excited by a narrowband KrF excimer laser are reported. Observations are made over a porous-plug, flat-flame burner reacting H2 in air, fuel-rich with nitrogen dilution to control the temperature, and with an H2 diffusion flame. Measurements made from UV Raman spectra show good agreement with measurements made by other means, both for gas temperature and relative major species concentrations. Laser-induced fluorescence interferences arising from OH and O2 are observed in emission near the Raman spectra. These interferences do not preclude Raman measurements, however.

Shirley, John A.↗
NASA NTRS1991

Counterflow diffusion flames of hydrogen, and hydrogen plus methane, ethylene, propane, and silane vs. air - Strain rates at extinction

Five coaxial tubular opposed jet burners (OJBs) with tube diameter D(T) of 1.8-10 mm and 5 mm conical nozzles were used to form dish-shaped counterflow diffusion flames centered by opposing laminar jets of nitrogen and hydrocarbon-diluted H2 versus air in an argon-purged chamber at 1 atm. Area-averaged air jet velocities at blowoff of the central flame, U(air), characterized extinction of the airside flame as functions of input H2 concentration on the fuelside. A master plot of extensive U(air) data at blowoff versus D(T) shows that U(air) varies linearly with D(T). This and other data sets are used to find that nozzle OJB results for U(air)/diameter average 4.24 + or - 0.28 times larger than tubular OJB results for the same fuel compositions. Critical radial velocity gradients consistent with one-dimensional stagnation point boundary theory and with plug flow inputs are estimated. The results compare favorably with published numerical results based only on potential flow.

Pellett, G. L.↗
NASA NTRS1991

Two-dimensional imaging of molecular hydrogen in H2-air diffusion flames using two-photon laser-induced fluorescence

The use of a tunable ArF laser at 193.26 nm to record simultaneous single-laser-shot, planar images of molecular hydrogen and hot oxygen in a turbulent H2-air diffusion flame. Excitation spectra of fuel and oxidant-rich flame zones confirm a partial overlap of the two-photon H2 and single-photon O2 Schumann-Runge absorption bands. UV Rayleigh scattering images of flame structure and estimated detection limits for the H2 two-photon imaging are also presented.

Lempert, W.↗
NASA NTRS1991

Laser-based measurements of OH in high pressure CH4/air flames

Narrow-linewidth laser absorption measurements are reported from which mole fraction and temperature of OH are determined in high-pressure (1-10 atm), lean CH4/air flames. These measurements were made in a new high pressure combustion facility which incorporates a traversable flat flame burner, providing spatially and temporally uniform combustion gases at pressures up to 10 am. A commercially avialable CW ring dye laser was used with an intracavity doubling crystal to provide near-UV single mode output at approximately 306 nm. The UV beam was rapidly scanned over 120 GHz (0.1 sec scan duration) to resolve the absorption lineshape of the A-X (0,0) R1(7)/R1(11) doublet of the OH radical. From the doublet's absorption lineshape, the temperature was determined; and from peak absorption, Beer's Law was employed to find the mole fraction of OH. These data were obtained as a function of height above the flame at various pressures.

Battles, B. E.↗
NASA NTRS1991

A study of hydrogen diffusion flames using PDF turbulence model

The application of probability density function (pdf) turbulence models is addressed in this work. For the purpose of accurate prediction of turbulent combustion, an algorithm that combines a conventional CFD flow solver with the Monte Carlo simulation of the pdf evolution equation has been developed. The algorithm has been validated using experimental data for a heated turbulent plane jet. The study of H2-F2 diffusion flames has been carried out using this algorithm. Numerical results compared favorably with experimental data. The computuations show that the flame center shifts as the equivalence ratio changes, and that for the same equivalence ratio, similarity solutions for flames exist.

Hsu, Andrew T.↗
NASA NTRS1991

A study of hydrogen diffusion flames using PDF turbulence model

The application of probability density function (pdf) turbulence models is addressed. For the purpose of accurate prediction of turbulent combustion, an algorithm that combines a conventional computational fluid dynamic (CFD) flow solver with the Monte Carlo simulation of the pdf evolution equation was developed. The algorithm was validated using experimental data for a heated turbulent plane jet. The study of H2-F2 diffusion flames was carried out using this algorithm. Numerical results compared favorably with experimental data. The computations show that the flame center shifts as the equivalence ratio changes, and that for the same equivalence ratio, similarity solutions for flames exist.

Hsu, Andrew T.↗
NASA NTRS1991

Opposed Flow Flame Spread in Normal, Enhanced and Reduced Gravity

Experimental and theoretical aspects of opposed-flow flame spread over solid fuels are presented with emphasis on the microgravity environments of spacecraft. For high opposing flow velocities, spread rate decreases with increasing velocity eventually leading to flame blowoff due to kinetic effects. At low opposing flow velocities, where diffusional effects are slowed and radiation becomes important, flame spread rate increases with increasing flow velocity. Extinction at low velocities is due to radiative effects. Modeling efforts that include radiation, both solid surface radiation and gas-phase radiation, predict qualitatively the experimental trends observed. Computationally, gas-phase radiation is conveniently included in solution of the conservation equations by employing a Plank mean absorption coefficient, a fraction of radiation that is fed back to the surface, and a shape function that describes the radiative flux distribution along the surface.

Altenkirch, Robert A.↗