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All sourcesNASA NTRSDOE OSTI
DOE OSTI2024

Quantifying the impacts of marine aerosols over the southeast Atlantic Ocean using a chemical transport model: implications for aerosol–cloud interactions

The southeast Atlantic region, characterized by persistent stratocumulus clouds, has one of the highest uncertainties in aerosol radiative forcing and significant variability across climate models. In this study, we analyze the seasonally varying role of marine aerosol sources and identify key uncertainties in aerosol composition at cloud-relevant altitudes over the southeast Atlantic using the GEOS-Chem chemical transport model. We evaluate simulated aerosol optical depth (AOD) and speciated aerosol concentrations against those collected from ground observations and aircraft campaigns such as LASIC, ORACLES, and CLARIFY, conducted during 2017. The model consistently underestimates AOD relative to AERONET, particularly at remote locations like Ascension Island. However, when compared with aerosol mass concentrations from aircraft campaigns during the biomass burning period, it performs adequately at cloud-relevant altitudes, with a normalized mean bias (NMB) between -3.5 % (CLARIFY) and -7.5 % (ORACLES). At these altitudes, in the model, organic aerosols (63 %) dominate during the biomass burning period, while sulfate (41 %) prevails during austral summer, when dimethylsulfide (DMS) emissions peak in the model. Our findings indicate that marine sulfate can account for up to 69 % of total sulfate during the high-DMS period. Sensitivity analyses indicate that refining DMS emissions and oxidation chemistry may increase sulfate aerosol produced from marine sources, highlighting that there remains large uncertainty as to the role of DMS emissions in the marine boundary layer. Additionally, we find marine primary organic aerosol emissions may substantially increase total organic aerosol concentrations, particularly during austral summer. This study underscores the imperative need to refine marine emissions and their chemical transformations, as aerosols from marine sources are a major component of total aerosols at cloud-relevant altitudes and may impact uncertainties in aerosol radiative forcing over the southeast Atlantic.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2025

Mid-Atlantic US observations of radiocarbon in CO 2 : fossil and biogenic source partitioning and model evaluation

Accurately quantifying regional anthropogenic CO 2 fluxes is fundamental to improving our understanding of the carbon cycle and for creating effective carbon mitigation policies, and the radiocarbon to total carbon ratio in atmospheric CO 2 (Δ 14 CO 2 ) is a robust tracer of fossil fuel CO 2 that can discriminate between biogenic and fossil fuel CO 2 sources. NASA's Atmospheric Carbon and Transport-America (ACT-America) airborne mission between 2016 and 2019 aimed to improve the accuracy of regional greenhouse gas flux estimates, through refining our understanding and characterization of fluxes and flux uncertainties in models. Δ 14 CO 2 observations from 26 flights are presented for examining seasonal CO 2 source partitioning in the Mid-Atlantic USA. Observed variability in boundary layer CO 2 at timescales ranging from intra-day to seasonal was largely driven by biogenic CO 2 (CO 2bio ) variability that ranged from −19.7 ppm in summer to 16.2 ppm in fall, while fossil fuel CO 2 (CO 2ff ) variability remained at 3.3±2.0 ppm. Carbonyl sulfide uptake was well-correlated with CO 2bio uptake, and examining this relationship, as well as that between CO 2 and CO 2bio variability reinforces the seasonal extent of gross primary productivity response throughout ACT-America. We use airborne Δ 14 CO 2 flask sampling alongside in situ carbon monoxide measurements to calculate high-frequency CO 2ff and evaluate the magnitude and diurnal variability of modeled CO 2ff , deducing likely transport errors in an example flight. Although ACT-America CO 2ff signals were attenuated due to the broad source regions sampled, results illustrate the value of Δ 14 CO 2 sampling and observation-based methodologies for regional CO 2 flux attribution, evaluation and improvement of modeled CO 2 .

Baier, Bianca C. [National Oceanic and Atmospheric↗
DOE OSTI2025

Application of PRIM for understanding patterns in carbon dioxide model-observation differences

Reducing uncertainties in regional carbon balances requires a better understanding of CO 2 transport in synoptic weather systems. Here, we apply the Patient Rule Induction Method (PRIM), a data-mining method to identify high-density regions for a target-class within an input parameter space, to airborne observations of potential temperature, wind speed, water vapor mixing ratio, and CO 2 dry mol fraction gathered during the Atmospheric Carbon and Transport (ACT)-America Summer 2016 and Winter 2017 campaigns. ACT observations were targeted at expert-designated cases of fair weather and near-frontal warm and cold sector air at atmospheric boundary-layer, lower-, and higher free tropospheric levels (ABL, LFT, and HFT, respectively). We investigate atmospheric characteristics of these pre-defined cases and associated CO 2 model-observation-differences in the mesoscale WRF-Chem model. PRIM results separate winter- and summertime observations as well as observations from ABL, LFT, and HFT with enrichment factors of 4.0–20.5 inside the PRIM box compared to the entire dataset but cannot distinguish between near-frontal warm and cold sector observations in the higher free troposphere. Analyzing of the parameter space constrained by PRIM, we find that large magnitude model observation differences preferentially associated with times when atmospheric conditions are less typical. This association suggests that PRIM could provide a useful tool for isolating atmospheric conditions with large-magnitude and non-Gaussian CO 2 -residuals for targeted transport model evaluation and to potentially improve inversion results during synoptically active periods.

Gerken, Tobias [James Madison Univ., Harrisonburg,↗
DOE OSTI2025

The diurnal susceptibility of subtropical clouds to aerosols

The diurnal susceptibility of clouds and their radiative properties to aerosols is examined during their Lagrangian transition from subtropical stratocumulus to shallow cumulus regimes. Using large-eddy simulations, we analyze the six-day evolution of an air mass along a 3800 km observed trajectory from the coast of Peru toward the equator. Pristine and polluted scenarios are simulated with forcing imposed from weather reanalysis. The polluted scenario exhibits stronger diurnal variations in cloud water, cloud fraction, and albedo, with enhanced nighttime entrainment and suppressed precipitation. The overall response of cloud properties and outgoing shortwave radiation to droplet number concentration follows a distinct diurnal pattern: strong positive cloud adjustments dominate at night and in the morning, while weak negative adjustments prevail in the afternoon. This cycle is driven by the competition between precipitation suppression, which enhances cloud water and coverage, and entrainment drying, which depletes them. In polluted conditions, enhanced entrainment leads to a deeper and more decoupled boundary layer that cannot be sustained by surface fluxes in the afternoon, resulting in negative cloud adjustments. The enhanced entrainment rate under polluted conditions is caused by the reduced sedimentation of cloud and precipitation water from the entrainment zone. While the Twomey effect dominates the diurnal average albedo response, the diurnal variation in the competing cloud adjustments lead to a near-neutral net susceptibility in the afternoon, highlighting the critical role of diurnally varying processes in aerosol-cloud interactions.

Geosciences↗
DOE OSTI2025

Regime-based aerosol–cloud interactions from CALIPSO-MODIS and the Energy Exascale Earth System Model version 2 (E3SMv2) over the Eastern North Atlantic

This study investigates aerosol-cloud interactions in marine boundary layer (MBL) clouds using an advanced deep-learning-driven synoptic-regime-based framework, combining satellite data (CALIPSO vertically resolved aerosol extinction and MODIS cloud properties) with 1° nudged Energy Exascale Earth System Model version 2 (E3SMv2) simulation over the Eastern North Atlantic (ENA; ∼10°×10°, 2006–2014). The E3SMv2 captures observed seasonal variations in cloud droplet number concentrations (N d ) and liquid water path (LWP), though it systematically underestimates N d . We then partition ENA meteorology into four synoptic regimes (Pre-Trough, Post-Trough, Ridge, Trough) via a deep-learning clustering of ERA5 reanalysis fields, enabling regime-dependent aerosol-cloud interactions analyses. Both satellite and E3SMv2 exhibit an inverted-V LWP-N d relationship. In Post-Trough and Ridge regimes, the satellite shows stronger negative LWP-N d sensitivities than in Pre-Trough regime. The Trough regime displays a muted satellite LWP response. In comparison, the model predicts more exaggerated LWP responses across regimes, with LWP increasing too quickly at low N d and decreasing more sharply at high N d , especially in Pre-Trough and Trough regimes. These exaggerated model LWP sensitivities may stem from uncertainties in representing drizzle processes, entrainment, and turbulent mixing. As for N d susceptibility to aerosols, N d increases with MBL aerosol extinction in both datasets, but the simulated aerosol-cloud interactions appear oversensitive to meteorological conditions. Overall, E3SMv2 better captures aerosol effects under regimes that favor stratiform clouds (Post-Trough, Ridge), but performance deteriorates for regimes with deeper, dynamically complex clouds (Trough), highlighting the need for improved representations of those cloud processes in climate models.

Environmental sciences↗
DOE OSTI2025

Tropospheric aerosols over the western North Atlantic Ocean during the winter and summer deployments of ACTIVATE 2020: life cycle, transport, and distribution

The Aerosol Cloud meTeorology Interactions oVer the western ATlantic Experiment (ACTIVATE) is a NASA mission to characterize aerosol–cloud interactions over the western North Atlantic Ocean (WNAO). Such characterization requires understanding of life cycle, composition, transport pathways, and distribution of aerosols over the WNAO. This study uses the GEOS-Chem model to simulate aerosol distributions and properties that are evaluated against aircraft, ground-based, and satellite observations during the winter and summer field deployments in 2020 of ACTIVATE. Transport in the boundary layer (BL) behind cold fronts was a major mechanism for the North American continental outflow of pollution to the WNAO in winter. Turbulent mixing was the main driver for the upward transport of sea salt within and ventilation out of BL in winter. The BL aerosol composition was dominated by sea salt, which increased in the summer, followed by organics and sulfate. Aircraft in situ aerosol measurements provided useful constraints on wet scavenging in GEOS-Chem. The model generally captured observed features such as continental outflow, land–ocean gradient, and mixing of anthropogenic aerosols with sea salt. Model sensitivity experiments with elevated smoke injection heights to the mid-troposphere (versus within BL) better reproduced observations of smoke aerosols from the western US wildfires over the WNAO in the summer. Model analysis suggests strong hygroscopic growth of sea salt particles and their seeding of marine BL clouds over the WNAO (< 35° N). Future modeling efforts should focus on improving parameterizations for aerosol wet scavenging, implementing realistic smoke injection heights, and applying high-resolution models that better resolve vertical transport.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2025

African dust transported to Barbados in the wintertime lacks indicators of chemical aging

The chemical processing (“aging”) of mineral dust is thought to increase dust light-scattering efficiency, cloud droplet activation, and nutrient solubility. However, the extent of African dust aging during long-range transport to the western Atlantic is poorly understood. Here, we explore African dust aging in wintertime samples collected from Barbados when dust is transported at lower altitudes. Ion chromatography (IC) analysis indicates that the mass concentrations of bulk nitrate, sulfate, and oxalate increase, relative to background conditions, when African dust reaches Barbados after transatlantic transport, indicating dust aging. However, aerosol mixing-state analysis from computer-controlled scanning electron microscopy with energy dispersive X-ray spectroscopy (CCSEM/EDX) indicates that approximately 67 % of dust particles are internally mixed with sea salt, while only about 26 % of dust particles contain no internally mixed components. SEM/EDX elemental mapping and time-of-flight secondary ion mass spectrometry (TOF-SIMS) reveals that within internally mixed dust and sea salt particles, only sea salt components contain signs of aging as indicated by the loss of chloride and acquisition of nitrate and/or sulfate. Our results suggest that chemical aging may only modestly increase the solubility of nutrients in African dust during long-range transport. Because most dust that we measured was internally mixed with sea salt, chemical aging is not necessarily required to increase the hygroscopicity of dust, at least in the lower boundary layer. Further, our findings have implications for understanding the release of halogens from sea salts, which may be enhanced in internally mixed dust and sea salt particles.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2025

Magnitude and timescale of liquid water path adjustments to cloud droplet number concentration perturbations for nocturnal non-precipitating marine stratocumulus

Cloud liquid water path (L) adjusts to perturbations in cloud droplet number concentration (N) over time. We explore the magnitude and timescale of this adjustment in nocturnal non-precipitating marine stratocumuli using large eddy simulations of baseline conditions and aerosol seeding experiments for 22 meteorological conditions. The results confirm that the L adjustment (δL) slope (k) is more negative for simulation pairs with relatively low N and less negative for high N. Overall, k is unlikely to be lower than −0.4 within 24 h of seeding start, meaning the L adjustment is unlikely to fully offset the brightening due to the Twomey effect. After seeding, the δL becomes increasingly negative, which can be characterized by an exponential convergence. This evolution is governed by a short timescale around 5 h and lasts for around 8–12 h. It is driven by the feedback between entrainment, L, and boundary layer (BL) turbulence. Other processes, including radiation, surface fluxes, and subsidence, respond to the seeding weakly. This short timescale is insensitive to the amount of seeding, making the evolution of δL and some other deviations similar for different seeding amounts after appropriate scaling. The timescale of k evolution is closely related to the δL timescale and hence also short, while it could also be affected by the δN evolution. The results are most relevant to conditions where seeding is applied to a large area of marine stratocumulus in well-mixed and overcast BL where shear is not a primary source of turbulence.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2025

Aerosol impacts on isolated deep convection: findings from TRACER

This study focuses on quantifying the conditional relationship between aerosol and convective precipitation properties of isolated deep convective clouds (DCCs) in the Houston–Galveston region, after adjusting for confounding effects. We leverage comprehensive ground-based observations from the TRacking Aerosol Convection interactions ExpeRiment (TRACER) to estimate aerosol effects on convective echo top height (ETH), intensity, and area separately. Our results show that greater aerosol number concentrations generally have a limited impact on these convective properties, showing relationships consistent with the possibility of both invigoration and suppression effects. Under certain conditions, where ultrafine particles are abundant, aerosols exhibit a positive effect on ETH, increasing it by about 1 km. However, it is inevitable to consider measurement uncertainties and the limitations of temporal and spatial resolution in the data, as these factors can further contribute to uncertainties in our estimates. In DCCs associated with sea breezes, the estimated aerosol effects on DCCs are found to be more pronounced. However, this heightened effect could be attributed to the exclusion of key confounders such as boundary layer updrafts in the analysis.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2026

Impact on cloud properties of reduced-sulphur shipping fuel in the Eastern North Atlantic

The global reduction in shipping fuel sulphur that culminated in 2020 with an ∼ 80 % reduction has created a large-scale natural experiment on the role of aerosol-cloud interaction (ACI) in the climate system. We compare observations from the Atmospheric Radiation Measurement program's Eastern North Atlantic site (ARM-ENA; 39.1° N, 28.0° W) during two June to September periods: 2016–2018 (pre-2020) and 2021–2023 (post-2020). We find a significant (∼ 15 %) decrease in cloud condensation nuclei concentrations post-2020, which resulted in a decrease in cloud droplet number (N d ) and an increase in effective radius (r e ) of marine boundary layer clouds. However, cloud liquid water path (LWP) increased post-2020. The increase in LWP offset the increase in r e , resulting in insignificant changes to optical depth. MODIS and CERES data in the vicinity of ENA during these periods produce similar results also with negligible change in albedo and optical depth. Regional cloud occurrence declined in line with changes in the large-scale meteorology. Our results highlight the complex interplay of factors that modulate cloud feedbacks in the Eastern North Atlantic.

Mace, Gerald G. [Univ. of Utah, Salt Lake City, UT↗
DOE OSTI2026

Evaluation of UKESM aerosol size and composition using ATom measurements indicates missing marine aerosol formation mechanisms

Atmospheric aerosols influence climate through their interactions with radiation and clouds, yet large uncertainties remain in their simulation by global models. This study evaluates the United Kingdom Earth System Model version 1.1 (UKESM1.1) using global-scale aircraft observations from the Atmospheric Tomography (ATom) mission, focusing on aerosol lifecycle processes in the remote marine atmosphere. We assess model performance in simulating aerosol precursor vapours, number size distributions, chemical composition, and environmental conditions. Several process improvements are tested, including sulfuric acid-ammonia nucleation, ammonium nitrate scheme, methanesulfonic acid condensation, and low-temperature isoprene-derived secondary organic aerosol formation. Model biases differ significantly between the upper troposphere (UT) and the marine boundary layer (MBL). In the UT, UKESM1.1 overestimates nucleation and Aitken mode particles while underestimating accumulation mode, indicating insufficient growth. In the MBL, the model overestimates primary aerosols (e.g. seasalt) and precursor gases but underestimates nucleation and Aitken mode particles, even after incorporating updated nucleation and ammonium nitrate scheme. The persistence of low aerosol number concentrations, despite overestimated precursors, suggests missing formation pathways likely involving other species such as iodine, amines, and organic vapours. These limitations result in an unbalanced cloud condensation nuclei budget that over-relies on primary emissions. Sensitivity tests reveal that model outputs are strongly influenced by dimethyl sulfide emissions and vapour condensation schemes. Our results highlight the need for future model development to prioritise mechanistic representation of currently missing aerosol sources, rather than relying on empirical tuning, to improve aerosol-climate interaction estimates.

He, Xu-Cheng [Univ. of Cambridge (United Kingdom);↗
DOE OSTI2026

Emerging low-cloud feedback and adjustment in global satellite observations

From mid-2003 to mid-2024, a global decrease in low-cloud amount enhanced the absorption of solar radiation by 0.22±0.07 W m −2 per decade (±1σ range), accelerating the energy imbalance trend during that period (0.44 W m −2 per decade). Through controlling factor analysis, here we show that the low-cloud trend is due to a combination of cloud feedback and adjustments to greenhouse gases and aerosols (respectively 0.09±0.02, 0.05±0.03, and 0.03±0.03 W m −2 per decade), which jointly account for 74 % of the trend. The contribution of natural climate variability is weak but uncertain (0.01±0.08 W m −2 per decade), owing to a poorly constrained trend in boundary-layer inversion strength. Importantly, the observed low-cloud radiative trend lies well within the range of values simulated by contemporary global climate models under conditions close to present day. Any systematic model error in the representation of present-day global energy imbalance trends is thus likely to originate in processes unrelated to low clouds.

Geosciences↗
DOE OSTI2026

A robust aerosol impact on clouds along the subtropical to tropical transition

Marine clouds undergo a transition from subtropical stratocumulus (Sc) to shallow cumulus (Cu) and eventually to deep convective (DC) systems as air masses advect from the subtropics towards the deep tropics. How aerosols modulate this Lagrangian cloud evolution remains largely uncertain. Here we use both 5 years of satellite observations mapped along 8 d Lagrangian trajectories and complementary large-eddy simulations from 9 initiation locations across the Northeast Pacific, Southeast Pacific, and Southeast Atlantic. This Lagrangian framework allows us to quantify the aerosol effect and its co-variability with meteorological conditions on cloud microphysics, macrophysics, and top-of-atmosphere radiation through the full Sc-Cu-DC transition. We show that increasing aerosol concentrations leads to deeper and more reflective clouds throughout this cloud transition. Examining the thermodynamic evolution along the trajectory indicates a well-known trend: enhanced moistening near the boundary-layer top and lower free troposphere under polluted conditions, suggesting that part of the co-variability between aerosol and meteorological conditions may be internally driven. The agreement between model simulations and satellite data alongside the multi-basin coherence of the results indicates that aerosols systematically amplify cloud depth and reflectivity during the subtropical–to–tropical cloud transition.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2020

Methodology for deriving the telescope focus function and its uncertainty for a heterodyne pulsed Doppler lidar

Doppler lidars provide two measured parameters, radial velocity and signal-to-noise ratio, from which winds and turbulent properties are routinely derived. Attenuated backscatter, which gives quantitative information on aerosols, clouds, and precipitation in the atmosphere, can be used in conjunction with the winds and turbulent properties to create a sophisticated classification of the state of the atmospheric boundary layer. Calculating attenuated backscatter from the signal-to-noise ratio requires accurate knowledge of the telescope focus function, which is usually unavailable. Inaccurate assumptions of the telescope focus function can significantly deform attenuated backscatter profiles, even if the instrument is focused at infinity. Here, we present a methodology for deriving the telescope focus function using a co-located ceilometer for pulsed heterodyne Doppler lidars. The method was tested with Halo Photonics StreamLine and StreamLine XR Doppler lidars but should also be applicable to other pulsed heterodyne Doppler lidar systems. The method derives two parameters of the telescope focus function, the effective beam diameter and the effective focal length of the telescope. Additionally, the method provides uncertainty estimates for the retrieved attenuated backscatter profile arising from uncertainties in deriving the telescope function, together with standard measurement uncertainties from the signal-to-noise ratio. The method is best suited for locations where the absolute difference in aerosol extinction at the ceilometer and Doppler lidar wavelengths is small.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2021

Ground-based temperature and humidity profiling: combining active and passive remote sensors

Abstract. Thermodynamic profiles in the planetary boundary layer (PBL) are important observations for a range of atmospheric research and operational needs. These profiles can be retrieved from passively sensed spectral infrared (IR) or microwave (MW) radiance observations or can be more directly measured by active remote sensors such as water vapor differential absorption lidars (DIALs). This paper explores the synergy of combining ground-based IR, MW, and DIAL observations using an optimal-estimation retrieval framework, quantifying the reduction in the uncertainty in the retrieved profiles and the increase in information content as additional observations are added to IR-only and MW-only retrievals. This study uses ground-based observations collected during the Perdigão field campaign in central Portugal in 2017 and during the DIAL demonstration campaign at the Atmospheric Radiation Measurement Southern Great Plains site in 2017. The results show that the information content in both temperature and water vapor is higher for the IR instrument relative to the MW instrument (thereby resulting in smaller uncertainties) and that the combined IR + MW retrieval is very similar to the IR-only retrieval below 1.5 km. However, including the partial profile of water vapor observed by the DIAL increases the information content in the combined IR + DIAL and MW + DIAL water vapor retrievals substantially, with the exact impact vertically depending on the characteristics of the DIAL instrument itself. Furthermore, there is a slight increase in the information content in the retrieved temperature profile using the IR + DIAL relative to the IR-only; this was not observed in the MW + DIAL retrieval.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2021

Undersizing of aged African biomass burning aerosol by an ultra-high-sensitivity aerosol spectrometer

The ultra-high-sensitivity aerosol spectrometer (UHSAS) differs from most other optical particle spectrometers by using a high-power infrared (IR) laser to detect small particles and reduce the sizing ambiguity due to the non-monotonicity of scattering with particle size. During the NASA ORACLES project (ObseRvations of Aerosols above CLouds and their intEractionS) over the southeast Atlantic Ocean, the UHSAS clearly undersized particles in the biomass burning plume extending from southern Africa. Since the horizontal and vertical extent of the plume was vast, the NASA P-3B research aircraft often flew through a fairly uniform biomass burning plume for periods exceeding 30 min, sufficient time to explore the details of the UHSAS response by selecting single particle sizes with a differential mobility analyzer (DMA) and passing them to the UHSAS. This was essentially an in-flight calibration of the UHSAS using the particles of interest. Two modes of responses appeared. Most particles were undersized by moderate amounts, ranging from not at all for 70 nm aerosols to 15 % for 280 nm particles. Mie scattering calculations show that composition-dependent refractive index of the particles cannot explain the pattern. Heating of brown carbon or tarballs in the beam causing evaporation and shrinking of the particles is the most plausible explanation, though mis-sizing due to non-sphericity cannot be ruled out. A small fraction (10 %–30 %) of the particles were undersized by 25 % to 35 %. Those were apparently the particles containing refractory black carbon. Laboratory calibrations confirm that black carbon is drastically undersized by the UHSAS, because particles heat to their vaporization point and shrink. A simple empirical correction equation was implemented that dramatically improves agreement with DMA distributions between 100 and 500 nm. It raised the median particle diameter by 18 nm, from 163 to 181 nm, during the August 2017 deployment and by smaller amounts during deployments with less intense pollution. Calculated scattering from UHSAS size distributions increased by about 130 %, dramatically improving agreement with scattering measured by nephelometers. The correction is only valid in polluted instances; clean marine boundary layer and free troposphere aerosols behaved more like the calibration spheres. We were unable to directly test the correction between 500 and 1000 nm, though aerodynamic particle sizer (APS) data appear to show that the correction is poor at the largest diameters, which is no surprise as the composition of those particles is likely to be quite different than that of the accumulation mode. This adds to the evidence that UHSAS data must be treated cautiously whenever the aerosol may absorb infrared light. Similar corrections may be required whenever brown carbon aerosol is present.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2022

The DataHawk2 uncrewed aircraft system for atmospheric research

Abstract. The DataHawk2 (DH2) is a small, fixed-wing, uncrewed aircraft system, or UAS, developed at the University of Colorado (CU) primarily for taking detailed thermodynamic measurements of the atmospheric boundary layer. The DH2 weighs 1.7 kg and has a wingspan of 1.3 m, with a flight endurance of approximately 60 min, depending on configuration. In the DH2's most modern form, the aircraft carries a Vaisala RSS-421 sensor for pressure, temperature, and relative humidity measurements, two CU-developed infrared temperature sensors, and a CU-developed fine-wire array, in addition to sensors required to support autopilot function (pitot tube with pressure sensor, GPS receiver, inertial measurement unit), from which wind speed and direction can also be estimated. This paper presents a description of the DH2, including information on its design and development work, and puts the DH2 into context with respect to other contemporary UASs. Data from recent field work (MOSAiC, the Multidisciplinary drifting Observatory for the Study of Arctic Climate) is presented and compared with radiosondes deployed during that campaign to provide an overview of sensor and system performance. These data show good agreement across pressure, temperature, and relative humidity as well as across wind speed and direction. Additional examples of measurements provided by the DH2 are given from a variety of previous campaigns in locations ranging from the continental United States to Japan and northern Alaska. Finally, a look toward future system improvements and upcoming research campaign participation is given.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2023

Estimating turbulent energy flux vertical profiles from uncrewed aircraft system measurements: exemplary results for the MOSAiC campaign

This study analyzes turbulent energy fluxes in the Arctic atmospheric boundary layer (ABL) using measurements with a small uncrewed aircraft system (sUAS). Turbulent fluxes constitute a major part of the atmospheric energy budget and influence the surface heat balance by distributing energy vertically in the atmosphere. However, only few in situ measurements of the vertical profile of turbulent fluxes in the Arctic ABL exist. The study presents a method to derive turbulent heat fluxes from DataHawk2 sUAS turbulence measurements, based on the flux gradient method with a parameterization of the turbulent exchange coefficient. This parameterization is derived from high-resolution horizontal wind speed measurements in combination with formulations for the turbulent Prandtl number and anisotropy depending on stability. Measurements were taken during the MOSAiC (Multidisciplinary drifting Observatory for the Study of Arctic Climate) expedition in the Arctic sea ice during the melt season of 2020. For three example cases from this campaign, vertical profiles of turbulence parameters and turbulent heat fluxes are presented and compared to balloon-borne, radar, and near-surface measurements. The combination of all measurements draws a consistent picture of ABL conditions and demonstrates the unique potential of the presented method for studying turbulent exchange processes in the vertical ABL profile with sUAS measurements.

54 ENVIRONMENTAL SCIENCES↗