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NASA NTRSDate not supplied

Satellite-Assisted Particulate Matter (SAPM) for the Models, In situ, and Remote sensing of Aerosols (MIRA) Working Group

Models, In situ, and Remote sensing of Aerosols (MIRA) is an international working group that aims to foster collaborations amongst these three major aerosol specialties. It consists of a collection of interdisciplinary and independently funded projects/topics with clearly-defined goals. Currently there are four MIRA topic areas, including Satellite-Assisted Particulate Matter (SAPM), which is focused specifically on fine particulate matter (PM2.5). The study of PM2.5 is important due to its significant contribution to air pollution and resultant, adverse human health effects. The goal of the SAPM topic group is to conduct and provide intercomparisons of various methods and techniques to obtain surface PM2.5 estimates assisted by satellite remote sensors, global aerosol models, and in situ aerosol measurements. Some benefits of space-based/model-assisted PM2.5 retrievals include providing PM2.5 approximations in regions with poor in situ ground station coverage and a means for assessing spatial/temporal PM2.5 variations on regional and/or global scales. Furthermore, benefits of spaceborne lidar/model-assisted PM2.5 retrievals include providing nighttime PM2.5 estimates and characterization of near-surface aerosol vertical structure. SAPM is seeking international datasets of mass scattering/absorption coefficient and aerosol hygroscopic properties for different aerosol species, as well as ground-based in situ PM2.5 measurements. In this poster presentation, we give an overview of SAPM, and show results from three recent/ongoing PM2.5 studies. These efforts involve deriving surface PM2.5 concentrations from two spaceborne lidars, the Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) and Cloud-Aerosol Transport System (CATS), and investigating key variables that impact the estimation of PM2.5 from model simulated aerosol optical depth (AOD) using the Goddard Earth Observing System (GEOS) model.

Travis D. Toth↗
NASA NTRSDate not supplied

Impact of Size Distribution Assumption on PM2.5 Simulation

Aerosol particles, especially those with diameter that is smaller than 2.5um, i.e. PM2.5, have detrimental impact on public health. As a regulated criteria air pollutant, PM2.5 is monitored by ground networks using various instruments. At the same time aerosol assimilation modeling system is developed to simulate the aerosol distribution with continuous global coverage. In this study we compared the PM2.5 simulated by NASA’s MERRA-2 modeling system with the measurements made at US Embassy sites around the globe on diurnal cycle, monthly average, and interannual variabilities. We focused the comparison in the places that are significantly impacted by the desert dust. Simulations based on both aerodynamic and geometric diameters are compared with available measurements. Aerodynamic diameter assumption shows better model-observation agreements over several dust belt stations.

Qian Tan↗
NASA NTRS2024

Spacecraft Maximum Allowable Concentrations for Airborne Contaminants: Revision C

The enclosed table lists official Spacecraft Maximum Allowable Concentrations (SMACs) for selected airborne contaminants. They are based upon experiments conducted at standard pressure and oxygen environments and may or may not be applicable to altered atmospheres. The values listed in this summary document are applicable only to ambient conditions at standard temperature and oxygen (14.7 psi and 21% O2 at 25°C). These are guideline values set by the National Aeronautics and Space Administration (NASA)/Johnson Space Center (JSC) Toxicology Group in cooperation with the National Research Council Committee on Toxicology (NRCCOT), through publication in the peer- reviewed scientific literature, or NASA Technical Memoranda. Based on documented guidance (NRC, 1992; NRC, 2016), NASA has established SMACs for 58 chemical compounds that are particularly relevant to atmospheric contamination of the International Space Station (ISS) and targets of Exploration. Some long-term limits (1000-days) have also been established to support manned deep-space exploration. Summaries of these SMACs are presented in tabular form as part of this publication. This document provides a tabular summary of values that have been previously established based on guidelines established by NASA and the National Research Council’s Committee on Toxicology and vetted and published through the NRCCOT and/or non-NASA scientific literature and NASA Technical Memoranda. Short‐term (1‐ and 24‐hour) SMACs apply to off‐nominal situations, such as accidental releases aboard a spacecraft. These limits permit risk of minor, reversible effects, such as mild mucosal irritation. In contrast, the long‐term SMACs are set to fully protect healthy crewmembers from adverse effects resulting from continuous exposure to specific air pollutants for up to 1000 days. Because allergic reactions or chemical idiosyncrasy to certain airborne pollutants are very difficult to predict, crewmembers with allergies or unusual sensitivity to trace pollutants may not be afforded complete protection, even when long‐term SMACs are not exceeded.

SMACs↗
NASA NTRSDate not supplied

Satellite-Assisted Particulate Matter (SAPM) for the Models, In situ, and Remote Sensing of Aerosols (MIRA) Working Group

Models, In situ, and Remote sensing of Aerosols (MIRA) is an international working group that provides a forum for collaborations amongst these three atmospheric aerosol communities. MIRA consists of a collection of interdisciplinary and independently funded Topic/Project groups with clear goals and generally characterized by requests for additional scientific data. The Satellite-Assisted Particulate Matter (SAPM) Topic group focuses on the study of fine particulate matter (PM2.5), as it is a major contributor to air pollution and negatively impacts human health. Our group aims to provide intercomparisons of various methods and techniques for estimating surface PM2.5 assisted by satellite remote sensors (passive and active), global aerosol models, and in situ aerosol measurements. The overall motivation of our work is to enhance PM2.5 coverage beyond in situ ground stations, which can be limited. In this presentation, we provide an overview of various PM2.5 estimation approaches by current SAPM team members, as each approach has its own strengths and limitations. One approach uses near-surface aerosol extinction retrievals from the spaceborne Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) and an assumed value of mass extinction efficiency to derive PM2.5 concentrations (Toth et al 2019). A study using this method found a promising agreement (R=0.60; slope=0.89) with U.S. Environmental Protection Agency (EPA) in situ PM2.5 measurements over the contiguous United States (CONUS) for a 12-year (2007-2018) period (Toth et al 2022). In a different approach combining spaceborne lidar and a model, the Cloud Aerosol Transport System (CATS) lidar and Goddard Earth Observing System (GEOS) model are blended in an ensemble variational assimilation scheme to retrieve aerosol extinction and convert speciated mass concentrations to total PM2.5. A recent study (Matus et al in prep.) found agreement within 2 μg/m3 over the CONUS on the 2016 annual mean when compared to EPA ground-based measurements. Another study explored trends in city aerosol optical depth (AOD) from a spaceborne passive remote sensor, Moderate Resolution Imaging Spectroradiometer (MODIS), and found that these trends agree well with trends in city surface PM2.5, which provides confidence in the use of city AOD for city PM2.5 trend studies (Vohra et al 2021). In a follow-on study, steep and significant trends (~2.5 to 7.8% a-1) in AOD are found for several South Asian cities (e.g., Bangalore and Hyderabad), suggesting rapid growth in PM2.5 (Vohra et al 2022). Also in this presentation, we report results on our current collective SAPM study of India, a country that exhibits high levels of PM2.5 pollution. We show the temporal (i.e., seasonal) and spatial variability of PM2.5 over India using the CALIOP and CATS+model approaches, comparisons between the estimated PM2.5 from the retrieval schemes, and validation with in situ PM2.5 ground-based observations from the Central Pollution Control Board in India. This region provides us with an excellent case study to test our PM2.5 retrievals in heavily polluted scenes and over a complex and varying topography. The SAPM Topic group actively seeks international participants/collaborators in our group, including those working with in situ aerosol measurements (e.g., ACTRIS). We are interested in aerosol datasets in order to either improve our PM2.5 estimates from various approaches (e.g., using in situ mass scattering/absorption coefficient and aerosol hygroscopic properties for various aerosol species) and/or validate the PM2.5 estimates (e.g., using in situ ground-based PM2.5 concentrations).

Travis D Toth↗
NASA NTRSDate not supplied

Providing Satellite-Assisted Particulate Matter (SAPM) Estimates for the Models, In situ, and Remote sensing of Aerosols (MIRA) Working Group

The Models, In situ, and Remote sensing of Aerosols (MIRA) Working Group is an international forum that promotes collaboration amongst researchers of these three atmospheric aerosol communities. MIRA currently consists of a collection of five interdisciplinary and independently funded Topic groups with focused goals and generally involve requests for additional scientific datasets. Participants of the MIRA Satellite-Assisted Particulate Matter (SAPM) Topic group study particulate matter with diameters smaller than 2.5 microns (PM2.5), because of its substantial role in air pollution and the resulting negative impacts on human health. SAPM seeks to provide intercomparisons of different methods and techniques for obtaining surface PM2.5 proxies using spaceborne passive and active remote sensors, aerosol models, and in situ observations. The ultimate motivation of SAPM is to provide greater PM2.5 coverage than in situ ground stations, which are limited in some areas of the contiguous United States and large regions throughout the globe. In this poster presentation, we provide an overview of the PM2.5 estimation techniques applied by current SAPM team members, as well as the strengths and limitations of each technique. These approaches include spaceborne lidar (Cloud-Aerosol Lidar with Orthogonal Polarization) only, combined spaceborne lidar (Cloud Aerosol Transport System) and a model (Goddard Earth Observing System), and using aerosol optical depth (AOD) from a spaceborne passive remote sensor (Moderate Resolution Imaging Spectroradiometer) to explore city trends in AOD and relate those to city trends in PM2.5. Also in this poster presentation, we highlight results of our SAPM study of India, a country characterized by high levels of PM2.5 concentrations. We show the temporal and spatial variability of PM2.5 over India derived using various approaches and validation with ground-based in situ PM2.5 observations. The SAPM Topic group actively seeks additional collaborators, including those working with in situ aerosol measurements, and is interested in aerosol datasets to improve and/or validate the PM2.5 estimates.

Travis D Toth↗
NASA NTRSDate not supplied

Developing Satellite-Assisted Particulate Matter (SAPM) Estimates over India for the MIRA Working Group

The Models, In Situ, and Remote Sensing of Aerosols (MIRA) Working Group is an international collective that encourages collaboration among researchers from these three atmospheric aerosol communities. MIRA currently comprises five interdisciplinary and independently funded Topic Groups, each with specific goals, and involves requests for additional scientific datasets. The Satellite-Assisted Particulate Matter (SAPM) Topic Group, as part of MIRA, focuses on studying particulate matter smaller than 2.5 microns in diameter (PM2.5) due to its significant contribution to air pollution and its harmful effects on human health. While the annual mean PM2.5 levels are typically low (~5-15 μg/m³) across most of the contiguous United States (CONUS), other countries experience much higher concentrations (e.g., India). SAPM aims to compare different methods and techniques for obtaining surface PM2.5 proxies using spaceborne passive and active remote sensors, aerosol models, and in situ measurements. Ultimately, SAPM aims to provide more extensive coverage of PM2.5 concentrations than what is currently available from in situ ground stations, which are limited in some parts of the CONUS and large regions worldwide. Current SAPM members are exploring PM2.5 estimation techniques using active sensors. This presentation offers an overview of these techniques and highlights the strengths and limitations of each approach. These techniques include 1) spaceborne lidar (CALIOP: Cloud-Aerosol Lidar with Orthogonal Polarization) alone, and 2) a combination of spaceborne lidar (CATS: Cloud Aerosol Transport System) and a global aerosol transport model (GEOS: Goddard Earth Observing System). Additionally, we present a case study featuring our SAPM research in India, a country with high levels of PM2.5 concentrations (i.e., state-level annual means of ~100-200 μg/m³). Consistent spatial patterns in PM2.5 over India are found from the in situ data, CALIOP-based, and CATS/model-based methods, with the highest concentrations found in northern India near New Delhi. The gridded PM2.5 analysis yields high R values between in situ and CATS/model (~0.7) and between in situ and CALIOP nighttime (~0.9), as well as good agreement between CATS/model and CALIOP nighttime PM2.5 estimates (R = ~0.8 and slope = ~0.9). For current and future efforts, the SAPM Topic Group is actively seeking new collaborators, especially those working with in situ aerosol measurements, and is interested in acquiring additional aerosol datasets to improve and validate the PM2.5 proxies.

Travis D Toth↗
DOE OSTI2020

DIGITAL APPLICATIONS USING REAL-TIME VEHICLE EXHAUST INFORMATION

Vehicle emission is a major source of air pollution that causes a significant number of deaths globally. It has a profound impact on energy and the environment as well. The existing vehicle emission monitoring system is unable to help mitigating the pollution properly and therefore, requires precise real-time pollution measurement. The purpose of this paper is to discuss novel applications using the real-time measurement of pollutants from a vehicle tailpipe where exhaust gases enter the environment. Today, it is possible to measure such emission due to the emergence of affordable digital technologies such as the Internet of Things (IoT), wireless connectivity, cloud platform, and artificial intelligence. This paper discusses how digital technologies can be used for real-time monitoring of NOx gas as a measure of vehicle emission and predictive analytics applications. A description of data collection and pre-processing methodologies, actual collected data, and an approach to identify patterns between inputs such as vehicle speed and altitude and output such as NOx emission are included. Applying a simple neural network has produced promising results and is a first step towards developing predictive applications.

Digital, Vehicle Exhaust, IoT, AI, 1.4.2, Predicti↗
DOE OSTI2021

AFLEET: ASSESS THE IMPACTS OF CONVENTIONAL AND ALTERNATIVE FUEL VEHICLES

The Alternative Fuel Life-Cycle Environmental and Economic Transportation (AFLEET) tool, developed by researchers at Argonne National Laboratory for the U.S. Department of Energy (DOE) Clean Cities coalition network, estimates the environmental and economic costs and benefits of alternative fuel and advanced vehicles. Using simple inputs, AFLEET lets fleet managers estimate and compare petroleum use, greenhouse gas emissions (GHGs), air pollutant emissions, and cost of ownership for conventional and alternative fuel vehicles (AFVs).

Burnham, Andrew↗
DOE OSTI2021

Enrichments of Anaerobic Selenium Oxyanion Reducers from FGD Wastewater Effluent

Flue gas desulfurization systems (FGD) mitigate air pollutants from coal fired power plants. However, such systems produce wastewater that contains other pollutants such as mercury, arsenic, nitrogen, and selenium that must be removed before the water is released back into the environment. Selenium is of interest because chronic low doses of selenium (ng/L) can cause detrimental ecological consequences. Biological treatment can be utilized to remove selenium from FGD wastewater, but the microorganisms involved in this process and environment within the FGD effluent have not been well studied. This study identifies the microorganisms in selenate-enriched and selenite-enriched FGD effluent that can reduce selenium oxyanions to elemental selenium. Knowing more about these organisms can lead to an eventual optimization in the biological removal of selenium species in these wastewaters.

Sarkar, Preom↗
DOE OSTI2023

Environmental and Social Justice Implications of a Circular Plastics Economy

A consideration of environmental justice (EJ) and social justice (SJ) is critical to minimize the impacts of technology deployment on local communities. SJ and EJ impacts occur in specific geographic locations but can cover a wide range of effects (e.g., air pollution, access to clean water, jobs, wages, and education), making it challenging to determine which metrics are appropriate to evaluate and which data are required. Thus, there is currently a gap in the analysis community's ability to provide useful and universal EJ and SJ metrics for emerging technologies. Here, we present a draft framework for evaluating the human health, local environment, and job implications of processes that are at an early or middle technology readiness level (TRL). Using a case study on enzymatic polyethylene terephthalate (PET) recycling (middle TRL), we demonstrate how to qualitatively and quantitatively assess these EJ and SJ metrics for a circular economy context and how to communicate the results in a manner beneficial to both researchers and local communities.

circular economy↗
DOE OSTI2023

Electrifying Education: Insights into Charging Electric School Buses in the United States

School buses (SBs) have historically been a source of both greenhouse gas emissions and local air pollutants have negative health impacts for students and others living nearby. Battery electric SBs (ESBs) are a promising emerging technology for decarbonizing student transport, however, ESB adoption in the U.S. remains at an early stage (approximate 1.1%) with many outstanding uncertainties. In this study, we take inventory of the current SB stock within U.S. states and observe real-world SB operating profiles to better understand the potential battery range requirements, daily charging opportunities, and charging infrastructure needs for ESBs.

ADVANCED PROPULSION SYSTEMS↗
DOE OSTI2023

Environmental and Social Justice Considerations in a Circular Economy

A consideration of environmental justice (EJ) and social justice (SJ) is critical to minimize the impacts of technology deployment on local communities. SJ and EJ impacts occur in specific geographic locations but can cover a wide range of effects (e.g., air pollution, access to clean water, jobs, wages, and education), making it challenging to determine which metrics are appropriate to evaluate and which data are required for qualitative or quantitative analysis. This issue is only exacerbated when the technology in question is at an early technology readiness level (TRL) without community specific data. Here, we present a framework for evaluating the human health, local environment, and job implications of processes that are at early to middle TRLs. Using a case study on enzymatic polyethylene terephthalate (PET) recycling (middle TRL), we demonstrate how to qualitatively and quantitatively assess these EJ and SJ metrics for a circular economy context and how to communicate the results in a manner beneficial to both researchers and local communities.

circular economy↗
DOE OSTI2023

Enabling a Sustainable Future: Zero-Emission Vehicles Cost Analysis to Inform Decarbonization Pathways

Despite being only 5% of vehicles on the road, medium- and heavy-duty vehicles (MHDVs) are the second largest contributor to transportation emissions (21%) and a major source of local air pollution disproportionally affecting disadvantaged communities. This talk summarizes a cost analysis for zero emissions vehicles (battery electric EVs and hydrogen fuel cell FCEVs) for all medium and heavy duty applications, ranging from large pick-up trucks, to delivery vans, buses, and heavy trucks. Results show that with continued improvements in vehicle and fuel technologies (in line with U.S. Department of Energy targets and vetted with industry), zero-emission vehicles (ZEVs) can reach total-cost-of-driving parity with conventional diesel vehicles by 2035 for all medium- and heavy-duty (MD/HD) vehicle classes without incentives. Assuming economics drives adoption, ZEV sales could reach 42% of all MD/HD trucks by 2030, reflecting lower combined vehicle purchase and operating costs (using real-world payback periods). Two technological solutions - battery electric vehicles (BEVs) and fuel cell electric vehicles (FCEVs) - are viable in multiple market segments, offering alternative pathways for decarbonization: a) BEVs tend to become cost-competitive for smaller trucks before 2030 and for short-haul (<500-mile) heavy trucks before 2035. b) Hydrogen FCEVs tend to become cost-competitive for long-haul (>500-mile) heavy trucks by 2035. Results are very sensitive to technology improvement trajectories, adoption decision-making, and uncertain assumptions about future freight demand, logistics, and vehicle use explored in multiple scenarios.

ADVANCED PROPULSION SYSTEMS,ENERGY PLANNING, POLIC↗
DOE OSTI2024

SAE Government-Industry - Heavy-Duty Policy: Panel Discussion (G203)

Medium- and heavy-duty vehicles are 21% of US transportation greenhouse gas (GHG) emissions and a major source of air pollution. In this talk to present some results exploring how the total cost of driving (TCD) of zero-emission vehicles (ZEVs), including battery electric vehicles and hydrogen fuel cell electric vehicles (EVs and FCEVs), could evolve under alternative scenarios. Results show that with continued improvements in vehicles and fuels, ZEVs can rapidly become viable, potentially reaching TCD parity or better compared to diesel vehicles by 2035 for all market segments. For heavy long-haul trucks, EVs become competitive on a TCD basis at charging costs below $0.18/kWh, while FCEVs become competitive on a TCD basis at hydrogen costs below $5/kg. A full transition to ZEV sales by 2035 results in 65% emissions reductions by 2050 compared to 2019 without supportive policies. Incentives such as the Inflation Reduction Act vehicle purchase credits further accelerate ZEV TCD competitiveness with major adoption opportunities over the next five years.

ADVANCED PROPULSION SYSTEMS,DIRECT ENERGY CONVERSI↗
DOE OSTI2024

Optimum Operation of Microgrid Systems that Employ PV Solar and Battery Systems

On a global scale, over 1.3 billion lack access to electricity (85% in rural areas), and approximately 2.8 billion people rely on traditional biomass for cooking. The World Health Organization estimates that household air pollution from inefficient stoves causes more premature deaths than malaria, tuberculosis, and HIV/AIDS. Increasing demand for energy has led to dramatic increases in emissions. The need for reliable electricity and limiting emissions drives research on Resilient Hybrid Energy Systems (RHESs), which provide cleaner energy by combining wind, solar, and biomass energy with traditional fossil energy, increasing production efficiency and reliability and reducing generating costs and emissions. Microgrids have been shown as an efficient means of implementing RHESs, with some focused mainly on reducing the environmental impact of electric power generation. The technical challenges of designing, implementing, and applying microgrids involve conducting a cradle-to-grave Life Cycle Analysis (LCA) to evaluate these systems’ environmental and economic performance under diverse operating conditions to evaluate resiliency. A sample RHES was developed and used to demonstrate the implementation in rural applications, where the system can provide reliable electricity for heating, cooling, lighting, and pumping clean water. The model and findings can be utilized by other regions around the globe facing similar challenges.

Nagapurkar, Prashant↗
DOE OSTI2024

Sustainable Port Operations: Powered by NREL

Seaports are vital economic hubs that allow the United States to compete on a global scale. But the heavy vehicles and cargo equipment that enable their operations also emit harmful air pollutants and greenhouse gas emissions. For nearly two decades, National Renewable Energy Laboratory (NREL) researchers have worked toward comprehensive seaport decarbonization. They fuse world-class analysis with deep vehicle and transportation systems knowledge to guide strategic deployment of low- and zero-emissions vehicles, charging and refueling infrastructure, and grid improvements. Together, these capabilities can enable sustainable port operations. This fact sheet outlines major seaport and airport decarbonization capabilities across the laboratory, including: fleet research, energy data, and insights for decarbonization; comprehensive hydrogen infrastructure deployment; optimized charging through grid integration; strategic blueprinting for clean, optimized technology deployment; and integrating diversity, equity, inclusion, and accessibility considerations into decarbonization efforts.

ADVANCED PROPULSION SYSTEMS,ENERGY CONSERVATION, C↗
DOE OSTI2024

Biofuels Production and Development in the United States

Addressing transportation emissions will require a combination of policy interventions, technological innovations, and behavioral changes. To decrease transportation-related carbon emissions, we recommend transitioning to cleaner and more efficient transport, expanding public transportation, and promoting sustainable urban planning. Transitioning to biofuels in the U.S. transportation sector presents a host of environmental, economic, and strategic advantages. Environmentally, biofuels offer a promising avenue for reducing greenhouse gas (GHG) emissions compared to conventional fossil fuels. Biofuels produce fewer harmful emissions, such as particulate matter and nitrogen oxides, compared to conventional fuels, thereby improving local air quality, and reducing health risks associated with air pollution. The U.S. government issued a "Sustainable Aviation Fuel (SAF) Grand Challenge" to promote the development of SAF and address the decarbonization of commercial aviation. The targets are to expand current domestic SAF production to 3 billion gallons per year by 2030, and then to 35 billion gallons by 2050, while achieving life cycle GHG reduction of at least 50% relative to fossil Jet A. The United States' biofuel production capacity rose to 23.8 billion gallons per year in 2023, a growth of more than 1.7 billion gallons since 2022. Ethanol nameplate capacity has reached 17.8 billion gallons per year since 2023, the ethanol production is 15.6 billion gallons in 2023 as capped by EPA regulation. Biodiesel production capacity stands at 2.1 billion gallons, and renewable diesel capacity is now 3.9 billion gallons. This newsletter keeps you informed on the state of biofuels in the United States, policy and regulations, technology advancements, and environmental and social impacts.

biodiesel↗
DOE OSTI2023

Cloud Atlas: An Interactive Apparatus for Air Quality Awareness

This paper introduces a research project of a kinetic apparatus that translates collected air quality data to users. The kinetic mechanical skeleton is embedded with processors and electronics, and constantly changes its form according to air quality data collected online via a web crawler. By translating invisible environmental conditions, such as air quality data into morphological, colorful, and acoustic changes for the device, the participants can be aware of the phenomenon of air pollution in real time. The interac- tions between participants' movements and the changes of the device imply how human behaviors can affect the state of the atmosphere. As a result, the device evokes public awareness and participation in environmental issues through tangible experiences. This research aims to explore a new kind of responsive architecture that acts as a medium between invisible environments and inhabitants.

Zhao, Xiaoxiao↗