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At least 1,135 records · Page 63

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NASA NTRS1979

Efficiency of aerosol collection on wires exposed in the stratosphere

The theory of inertial impaction is briefly presented. Stratospheric aerosol research experiments were performed duplicating Wong et al. experiments. The use of the curve of inertial parameters vs particle collection efficiency, derived from Wong et al., was found to be justified. The results show that stratospheric aerosol particles of all sizes are collectible by wire impaction technique. Curves and tables are presented and used to correct particle counts for collection efficiencies less than 100%.

Lem, H. Y.↗

NASA NTRS1979

The stratosphere: Present and future

The present status of stratospheric science is discussed. The three basic elements of stratospheric science-laboratory measurements, atmospheric observations, and theoretical studies are presented along with an attempt to predict, with reasonable confidence, the effect on ozone of particular anthropogenic sources of pollution.

Hudson, R. D.↗

NASA NTRS1979

A sensitivity analysis of volcanic aerosol dispersion in the stratosphere

A computer sensitivity analysis was performed to determine the uncertainties involved in the calculation of volcanic aerosol dispersion in the stratosphere using a 2 dimensional model. The Fuego volcanic event of 1974 was used. Aerosol dispersion processes that were included are: transport, sedimentation, gas phase sulfur chemistry, and aerosol growth. Calculated uncertainties are established from variations in the stratospheric aerosol layer decay times at 37 latitude for each dispersion process. Model profiles are also compared with lidar measurements. Results of the computer study are quite sensitive (factor of 2) to the assumed volcanic aerosol source function and the large variations in the parameterized transport between 15 and 20 km at subtropical latitudes. Sedimentation effects are uncertain by up to a factor of 1.5 because of the lack of aerosol size distribution data. The aerosol chemistry and growth, assuming that the stated mechanisms are correct, are essentially complete in several months after the eruption and cannot explain the differences between measured and modeled results.

Butler, C. F.↗

NASA NTRS1979

Some aspects of stratospheric chemical response to solar particle precipitations. I - Potential roles of N2/A3Sigma/ and ion-chemistry

Large amounts of long lived N2(A3Sigma) are created by the energy degradation of precipitating solar particles. Laboratory data suggest that in the stratosphere N2(A3Sigma) are efficiently converted into N2O. Through reactions with O(1D), N2O may gradually release NO and thereby influence the long term aspects of stratospheric chemical response. During the daytime, negative ions may transform an active NO(x) into an inactive HNO3. At night both negative and positive ion chemistry generate HO(x). Omission of ionic chemistry results in considerable underestimation of O3 depletion during the initial phases of solar particle events, and thereby introduces significant error in the estimation of the nature of the prompt response.

Prasad, S. S.↗

NASA NTRS1979

Sulfur and halogen chemistry of the stratosphere and of volcanic eruption plumes

The major eruption of Volcan de Fuego caused an enhancement of 1.6 x 10 to the 9 kg of SO4(-) in the stratosphere 6 months after the eruption. Measurable changes in nitric acid vapor and particulate chloride were not observed. Subsequent data suggests that HCl was not injected into the stratosphere. The first simultaneous measurement of halogen and sulfur content of gases and particles in explosive eruption plumes is reported. The average percents of elements in particles were sulfur, 2.5 + or - 2.1; chlorine, 18 + or - 12; and fluorine, 38 + or - 29. The average molecular ratio of HCl/SO2 and HCl/HF were 0.41 + or - 0.26 and 14 + or - 12 in the Guatemalan eruption plumes.

Lazrus, A. L.↗

NASA NTRS1980

Numerical simulation of sudden stratospheric warmings

The paper presents a mechanistic, quasi-geostrophic, semi-spectral model with a self-consistent calculation of the mean zonal flow fields used to numerically simulate sudden stratospheric warmings generated by a single zonal harmonic (m) planetary wave. The development of a warming depends on the strength of the westerly winds in the lower stratosphere, and the growth rate of a m=2 warming is accelerated during the westerly zonal wind phase of the quasi-biennial oscillation. An m=1 warming is characterized by oscillation of wave amplitude and mean flow from resonantly trapped, westward, propagating planetary waves moving in and out of phase with the tropospherically forced stationary planetary wave. An m=2 critical level develops in the equatorial region and advances poleward, and its warming is characterized by a sudden intensification after an initially slow growth in contrast to slowly developing m=1 warmings.

Schoeberl, M. R.↗

NASA NTRS1980

High-altitude-resolution stratospheric measurements with the Arecibo 2380-MHz radar

The 2380-MHz planetary radar of the Arecibo Observatory and the 30-m interferometer antenna at Higuialles, Puerto Rico, have been instrumented as a bistatic radar for stratospheric turbulence research studies. The average power of the transmitter is 400 kW, and it uses the 300-m Arecibo spherical reflector. A vertical resolution of 30 m has been achieved by means of a novel continuous pseudorandom phase coding scheme. Preliminary results obtained with the system are presented. The thickness and internal structure of turbulent stratospheric layers have been resolved for the first time. The potential of the instrument in assessing the role of turbulence in the vertical transport of tracers, contaminants, and momentum is discussed.

Woodman, R. F.↗

NASA NTRS1980

Stratospheric H2O

The present state of our knowledge and understanding of H2O in the stratosphere is reviewed. This reveals continuing discrepancies between observations and expectations following from the Brewer-Dobson hypothesis of stratospheric circulation. In particular, available observations indicate unexplained upward and poleward directed H2O gradients immediately downstream from the tropical tropopause and variable vertical gradients above 20 km which generally disagree with those expected from oxidation of CH4.

Ellsaesser, H. W.↗

NASA NTRS1981

Energetics of a sudden stratospheric warming simulated with a three-dimensional, spectral, quasi-geostrophic model

The energetics of a three dimensional, quasi-geostrophic simulation of a sudden stratospheric warming which developed spontaneously during an annual cycle simulation are described. Daily values of the stratospheric temperatures, zonal winds, heating rates, energies, and energy conversions are discussed and compared with those for observed warmings. It is shown that, like observed warmings, the simulated warming was preceded by an increased vertical flux of eddy kinetic energy from the troposphere and the polar heating resulted because of the strong convergence of the horizontal, eddy heat flux which was only partially balanced by adiabatic and diabatic cooling. There is a significant similarity between the energetics of the simulated and observed warmings. In addition, the warming was spontaneous and the model did not develop a major warming in each winter of the simulation. These facts suggest that this model may be useful for studying not only the warming process but also the conditions that favor its development.

Haggard, K. V.↗

NASA NTRS1981

Measurement of HO2 and other trace gases in the stratosphere using a high resolution far infrared spectrometer at 28 Km

A progress report and data analyses from the December 1980 flight are presented. The following areas are covered: (1) computer analysis of the flight spectra to obtain phase corrected, normalized sums of spectra for retrieval of atmospheric profiles; (2) study of atmospheric HF, HCl, and H2O; (3) stratospheric H2O2 and HOCl; (4) laboratory spectroscopy of HOCl; and (5) design study of a new balloon gondola. The majority of the flight data were taken in the low background mode, i.e., one input to the spectrometer looking at the sky and the other looking at a LN2 temperature blackbody. An analysis of HF stratospheric measurements was undertaken in conjunction with the HF analysis. High quality spectra showing the HOCl q-branches under optically thin conditions were also obtained.

Traub, W. A.↗

NASA NTRS1980

A model of Saturn's seasonal stratosphere at the time of the Voyager encounters

A polar-equatorial climate model by Cess and Cladwell (1979) is extended to all latitudes of Saturn. Modifications for solar absorption within the stratosphere are made in the extension to intermediate latitudes. The latitudinally and temporally variable effects of sunlight absorption by the rings of Saturn are included in the model. Temperature-latitude profiles for several levels within the Saturn stratosphere are presented for January 1981, which should be directly comparable with Saturn Voyager observations in November 1980 and August 1981. Temperature-pressure profiles for latitudes +30 degrees and -25 degrees are provided, which correspond to the planned points at which radio equipment aboard Voyager II will produce occultation observations.

Carlson, B. E.↗

NASA NTRS1980

Carbon dioxide measurements in the stratosphere

A mass spectrometer experiment for the analysis of minor constituents in the stratosphere has been flown successfully four times from Palestine, Texas on board a balloon gondola. The carbon dioxide mixing ratio, which shows unexpectedly large variations in the stratosphere, reached 400 ppm in one particular night flight. This is about 20% higher than the ground value. Evidence is presented that the experiment performed well during each of the balloon flights. The isotopic ratio C-12/C-13 was measured and found in good agreement with previous air analyses showing a depletion of C-13.

Mauersberger, K.↗

NASA NTRS1981

Trace element composition of the Mount St. Helens plume - Stratospheric samples from the 18 May eruption

Atmospheric particulate material collected from the stratosphere in the plume of the 18 May 1980 eruption of the Mount St. Helens volcano was quite similar in composition to that of ash that fell to the ground in western Washington. However, there were small but significant differences in concentrations of some elements with altitude, indicating that the stratospheric material was primarily produced from fresh magma, not fragments of the mountain.

Vossler, T.↗

NASA NTRS1981

Effects of meteoric debris on stratospheric aerosols and gases

Characterizations of meteoric dust height and size distributions are obtained using Hunten's calculations of meteor ablation and recondensation rates. The contribution of meteor residues to aerosol composition, the role of meteoric dust as condensation nuclei, and the effects of meteor debris on aerosol size distributions are quantified, and particle surface areas are estimated. The potential importance of heterogeneous chemistry for stratospheric trace gases is discussed. The interaction between H2SO4 vapor and meteor metal vapors is investigated. It is concluded that meteoric particles may dominate the natural stratospheric aerosols at small (less than .01 micron radius) and large (greater than 1 micron radius) sizes under normal conditions.

Turco, R. P.↗

NASA NTRS1981

Chlorine oxide in the stratospheric ozone layer Ground-based detection and measurement

Stratospheric chlorine oxide, a significant intermediate product in the catalytic destruction of ozone by atomic chlorine, has been detected and measured by a ground-based 204 GHz, millimeter-wave receiver. Data taken at latitude 42 deg N on 17 days between January 10 and February 18, 1980 yield an average chlorine oxide column density of approximately 1.05 x 10 to the 14th/sq cm or approximately 2/3 that of the average of eight in situ balloon flight measurements (excluding the anomalously high data of July 14, 1977) made over the past four years at 32 deg N. Less chlorine oxide below 35 km and a larger vertical gradient than predicted by theoretical models of the stratospheric ozone layer are found.

Parrish, A.↗

NASA NTRS1980

Galilean satellite eclipse studies. II - Jovian stratospheric and tropospheric aerosol content

Aerosol profiles of the Jovian stratosphere and troposphere are presented using the Galilean satellite eclipse technique. The aerosol content is tenuous and varies with altitude, increasing rapidly with downward passage through the tropopause. The data indicate the presence of some aerosols of undetermined structure above the tropopause. An extended haze distribution is proposed, but the possibility that the stratospheric aerosol resides in a thin layer is not excluded.

Smith, D. W.↗

NASA NTRS1981

Measurement of stratospheric sulfur constituents

New measurements of mixing ratios of OCS in the lower stratosphere at midlatitude (Northern California) and high-latitude (Alaska) locations are reported which are in essential agreement with previous results. Weak signals due to stratospheric SO2 have been detected, and the estimated mixing ratios ranged from 36 to 51 pptv at altitudes 15.2 to 20.3 km. A very weak signal observed in the analysis is thought to be due to CS2 and, if this identification is correct, an upper limit concentration is estimated to be 1 pptv.

Inn, E. C. Y.↗

NASA NTRS1981

Measurements of the absorption coefficient of stratospheric aerosols

The absorption coefficients of stratospheric aerosols are measured using a variation on the integrating plate method. The technique is based on the decrease in the transparency of a substrate when an absorbing aerosol is deposited on it. A Lambert scatterer is placed behind the substrate to integrate forward scattered light and minimize the effect of scattering on the measurement. The low pressure in the stratosphere is used for the direct impaction of particles onto a narrow strip of opal glass. The eight samples collected had a median value of 4 x 10 to the -9th m with an uncertainty of + or - 5 x 10 to the -9th m. If this absorption is due to graphitic carbon, then its concentration is estimated at about 0.4 ng/cu m, or about 0.25% of the total aerosol mass concentration. Estimates of the aerosol scattering coefficients based on satellite extinction inversions result in an aerosol single-scattering albedo in the range of 0.96-1.0.

Ogren, J. A.↗