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At least 1,135 records · Page 63

Revealing important nocturnal and day-to-day variations in fire smoke emissions through a multiplatform inversion

We couple airborne, ground-based, and satellite observations; conduct regional simulations; and develop and apply an inversion technique to constrain hourly smoke emissions from the Rim Fire, the third largest observed in California, USA. Emissions constrained with multiplatform data show notable nocturnal enhancements (sometimes over a factor of 20), correlate better with daily burned area data, and are a factor of 2–4 higher than a priori estimates, highlighting the need for improved characterization of diurnal profiles and day-to-day variability when modeling extreme fires. Constraining only with satellite data results in smaller enhancements mainly due to missing retrievals near the emissions source, suggesting that top-down emission estimates for these events could be underestimated and a multiplatform approach is required to resolve them. As a result, predictions driven by emissions constrained with multiplatform data present significant variations in downwind air quality and in aerosol feedback on meteorology, emphasizing the need for improved emissions estimates during exceptional events.

54 ENVIRONMENTAL SCIENCES↗

Assessment of future changes in water availability and aridity

Substantial changes in the hydrological cycle are projected for the 21st century, but these projections are subject to major uncertainties. In this context, the “dry gets drier, wet gets wetter” (DDWW) paradigm is often used as a simplifying summary. However, recent studies cast doubt on the validity of the paradigm and also on applying the widely used P-E (precipitation - evapotranspiration) metric over global land surfaces. Here we show in a comprehensive CMIP5-based assessment that projected changes in mean annual P - E are generally not significant, except for high-latitude regions showing wetting conditions until the end of the 21st century. Significant increases in aridity do occur in many subtropical and also adjacent humid regions. However, combining both metrics still shows that approximately 70% of all land area will not experience significant changes. Finally, based on these findings, we conclude that the DDWW paradigm is generally not confirmed for projected changes in most land areas.

54 ENVIRONMENTAL SCIENCES↗

The two-way relationship between ionospheric outflow and the ring current

It is now well established that the ionosphere, because it acts as a significant source of plasma, plays a critical role in ring current dynamics. However, because the ring current deposits energy into the ionosphere, the inverse may also be true: the ring current can play a critical role in the dynamics of ionospheric outflow. This study uses a set of coupled, first-principles-based numerical models to test the dependence of ionospheric outflow on ring current-driven region 2 field-aligned currents (FACs). A moderate magnetospheric storm event is modeled with the Space Weather Modeling Framework using a global MHD code (Block Adaptive Tree Solar wind Roe-type Upwind Scheme, BATS-R-US), a polar wind model (Polar Wind Outflow Model), and a bounce-averaged kinetic ring current model (ring current atmosphere interaction model with self-consistent magnetic field, RAM-SCB). Initially, each code is two-way coupled to all others except for RAM-SCB, which receives inputs from the other models but is not allowed to feed back pressure into the MHD model. The simulation is repeated with pressure coupling activated, which drives strong pressure gradients and region 2 FACs in BATS-R-US. It is found that the region 2 FACs increase heavy ion outflow by up to 6 times over the non-coupled results. The additional outflow further energizes the ring current, establishing an ionosphere-magnetosphere mass feedback loop. This study further demonstrates that ionospheric outflow is not merely a plasma source for the magnetosphere but an integral part in the nonlinear ionosphere-magnetosphere-ring current system.

58 GEOSCIENCES↗

Survey of radiation belt energetic electron pitch angle distributions based on the Van Allen Probes MagEIS measurements: Electron Pitch Angle Distributions

A statistical survey of electron pitch angle distributions (PADs) is performed based on the pitch angle-resolved flux observations from the Magnetic Electron Ion Spectrometer (MagEIS) instrument on board the Van Allen Probes during the period from 1 October 2012 to 1 May 2015. By fitting the measured PADs to a sin n α form, where α is the local pitch angle and n is the power law index, we investigate the dependence of PADs on electron kinetic energy, magnetic local time (MLT), the geomagnetic Kp index, and L shell. The difference in electron PADs between the inner and outer belt is distinct. In the outer belt, the common averaged n values are less than 1.5, except for large values of the Kp index and high electron energies. The averaged n values vary considerably with MLT, with a peak in the afternoon sector and an increase with increasing L shell. In the inner belt, the averaged n values are much larger, with a common value greater than 2. The PADs show a slight dependence on MLT, with a weak maximum at noon. A distinct region with steep PADs lies in the outer edge of the inner belt where the electron flux is relatively low. The distance between the inner and outer belt and the intensity of the geomagnetic activity together determine the variation of PADs in the inner belt. Finally, besides being dependent on electron energy, magnetic activity, and L shell, the results show a clear dependence on MLT, with higher n values on the dayside.

79 ASTRONOMY AND ASTROPHYSICS↗

Wet scavenging of soluble gases in DC3 deep convective storms using WRF-Chem simulations and aircraft observations

In this work, we examine wet scavenging of soluble trace gases in storms observed during the Deep Convective Clouds and Chemistry (DC3) field campaign. We conduct high-resolution simulations with the Weather Research and Forecasting model with Chemistry (WRF-Chem) of a severe storm in Oklahoma. The model represents well the storm location, size, and structure as compared with Next Generation Weather Radar reflectivity, and simulated CO transport is consistent with aircraft observations. Scavenging efficiencies (SEs) between inflow and outflow of soluble species are calculated from aircraft measurements and model simulations. Using a simple wet scavenging scheme, we simulate the SE of each soluble species within the error bars of the observations. The simulated SEs of all species except nitric acid (HNO 3 ) are highly sensitive to the values specified for the fractions retained in ice when cloud water freezes. To reproduce the observations, we must assume zero ice retention for formaldehyde (CH 2 O) and hydrogen peroxide (H 2 O 2 ) and complete retention for methyl hydrogen peroxide (CH 3 OOH) and sulfur dioxide (SO 2 ), likely to compensate for the lack of aqueous chemistry in the model. We then compare scavenging efficiencies among storms that formed in Alabama and northeast Colorado and the Oklahoma storm. Significant differences in SEs are seen among storms and species. More scavenging of HNO 3 and less removal of CH 3 OOH are seen in storms with higher maximum flash rates, an indication of more graupel mass. Graupel is associated with mixed-phase scavenging and lightning production of nitrogen oxides (NOx ), processes that may explain the observed differences in HNO 3 and CH 3 OOH scavenging.

54 ENVIRONMENTAL SCIENCES↗

Evaluation of the aerosol vertical distribution in global aerosol models through comparison against CALIOP measurements: AeroCom phase II results

The ability of 11 models in simulating the aerosol vertical distribution from regional to global scales, as part of the second phase of the AeroCom model intercomparison initiative (AeroCom II), is assessed herein and compared to results of the first phase. The evaluation is performed using a global monthly gridded data set of aerosol extinction profiles built for this purpose from the CALIOP (Cloud-Aerosol Lidar with Orthogonal Polarization) Layer Product 3.01. Results over 12 subcontinental regions show that five models improved, whereas three degraded in reproducing the interregional variability in Z α 0–6 km , the mean extinction height diagnostic, as computed from the CALIOP aerosol profiles over the 0–6 km altitude range for each studied region and season. While the models' performance remains highly variable, the simulation of the timing of the Z α 0–6 km peak season has also improved for all but two models from AeroCom Phase I to Phase II. The biases in Z α 0–6 km are smaller in all regions except Central Atlantic, East Asia, and North and South Africa. Most of the models now underestimate Z α 0–6 km over land, notably in the dust and biomass burning regions in Asia and Africa. At global scale, the AeroCom II models better reproduce the Z α 0–6 km latitudinal variability over ocean than over land. Hypotheses for the performance and evolution of the individual models and for the intermodel diversity are discussed. We also provide an analysis of the CALIOP limitations and uncertainties contributing to the differences between the simulations and observations.

54 ENVIRONMENTAL SCIENCES↗

Characterizing relative humidity with respect to ice in midlatitude cirrus clouds as a function of atmospheric state: RHI IN MIDLATITUDE CIRRUS

Midlatitude cirrus cloud macrophysical and microphysical properties have been shown in previous studies to vary seasonally and in various large-scale dynamical regimes, but relative humidity with respect to ice (RHI) within cirrus clouds has not been studied extensively in this context. Using a combination of radiosonde and millimeter-wavelength cloud radar data, we identify 1076 cirrus clouds spanning a 7 year period from 2004 to 2011. These data are separated into five classes using a previously published algorithm that is based largely on synoptic conditions. Using these data and classification scheme, we find that RHI in cirrus clouds varies seasonally. Variations in cirrus cloud RHI exist within the prescribed classifications; however, most of the variations are within the measurement uncertainty. Additionally, with the exception of nonsummer class cirrus, these variations are not statistically significant. We also find that cirrus cloud occurrence is not necessarily correlated with higher observed values of RHI. The structure of RHI in cirrus clouds varies more in thicker clouds, which follows previous studies showing that macrophysical and microphysical variability increases in thicker cirrus clouds.

54 ENVIRONMENTAL SCIENCES↗

A forward analysis on the applicability of tracer breakthrough profiles in revealing the pore structure of tight gas sandstone and carbonate rocks

Here, we explore tracer breakthrough profiles (TBP) as a macroscopic property to infer the pore-space topology of tight gas sandstone and carbonate rocks at the core scale. The following features were modeled via three-dimensional multiscale networks: microporosity within dissolved grains and pore-filling clay, cementation in the absence and presence of microporosity (each classified into uniform, pore-preferred, and throat-preferred modes), layering, vug, and microcrack inclusion. A priori knowledge of the extent and location of each process was assumed to be known. With the exception of an equal importance of macropores and pore-filling micropores, TBPs show little sensitivity to the fraction of micropores present. In general, significant sensitivity of the TBPs was observed for uniform and throat-preferred cementation. Layering parallel to the fluid flow direction had a considerable impact on TBPs whereas layering perpendicular to flow did not. Microcrack orientations seemed of minor importance in affecting TBPs.

58 GEOSCIENCES↗

Evaluating geothermal and hydrogeologic controls on regional groundwater temperature distribution

Described is a one-dimensional (1-D) analytic solution is developed for heat transport through an aquifer system where the vertical temperature profile in the aquifer is nearly uniform. The general anisotropic form of the viscous heat generation term is developed for use in groundwater flow simulations. The 1-D solution is extended to more complex geometries by solving the equation for piece-wise linear or uniform properties and boundary conditions. A moderately complex example, the Eastern Snake River Plain (ESRP), is analyzed to demonstrate the use of the analytic solution for identifying important physical processes. For example, it is shown that viscous heating is variably important and that heat conduction to the land surface is a primary control on the distribution of aquifer and spring temperatures. Use of published values for all aquifer and thermal properties results in a reasonable match between simulated and measured groundwater temperatures over most of the 300 km length of the ESRP, except for geothermal heat flow into the base of the aquifer within 20 km of the Yellowstone hotspot. Previous basal heat flow measurements (110 mW/m 2 ) made beneath the ESRP aquifer were collected at distances of > 50 km from the Yellowstone Plateau, but a higher basal heat flow of 150 mW/m 2 is required to match groundwater temperatures near the Plateau. As a result, the ESRP example demonstrates how the new tool can be used during preliminary analysis of a groundwater system, allowing efficient identification of the important physical processes that must be represented during more-complex 2-D and 3-D simulations of combined groundwater and heat flow.

58 GEOSCIENCES↗

Prolonged El Niño conditions in 2014-2015 and the rapid intensification of Hurricane Patricia in the eastern Pacific: EL NIÑO AND HURRICANE PATRICIA

Hurricane Patricia was the most intense tropical cyclone on record in the eastern North Pacific or Atlantic, reaching a peak intensity of 95 m s -1 only 30 hours after attaining hurricane status (33 m s -1 ). Here it is shown that exceptionally warm sea surface temperatures (SSTs), a deeper than normal thermocline, and strong near-surface salinity stratification all aided Patricia’s rapid intensifciation, combining to increase its Dynamic Potential Intensity by 10–21 m s -1 . Anomalous surface warming and thermocline deepening along Patricia’s track were driven by prolonged El Niño during 2014–15 and punctuated by the buildup to the extreme El Niño of 2015–16. In the region where Patricia intensified, SST was 1.5°C higher and sea surface height was 10 cm higher compared to conditions during the last extreme El Niño in 1997, emphasizing the extraordinary nature of the 2015 anomalies.

58 GEOSCIENCES↗

Anthropogenic warming impacts on California snowpack during drought

Sierra Nevada climate and snowpack is simulated during the period of extreme drought from 2011 to 2015 and compared to an identical simulation except for the removal of the twentieth century anthropogenic warming. Anthropogenic warming reduced average snowpack levels by 25%, with middle-to-low elevations experiencing reductions between 26 and 43%. In terms of event frequency, return periods associated with anomalies in 4 year 1 April snow water equivalent are estimated to have doubled, and possibly quadrupled, due to past warming. Here, we also estimate effects of future anthropogenic warmth on snowpack during a drought similar to that of 2011–2015. Further snowpack declines of 60–85% are expected, depending on emissions scenario. The return periods associated with future snowpack levels are estimated to range from millennia to much longer. Therefore, past human emissions of greenhouse gases are already negatively impacting statewide water resources during drought, and much more severe impacts are likely to be inevitable.

54 ENVIRONMENTAL SCIENCES↗

Foreshock wave interaction with the magnetopause: Signatures of mode conversion

Our previous hybrid simulation under a radial interplanetary magnetic field (IMF) and a supercritical solar wind Mach number has shown that foreshock compressional waves originated from the quasi–parallel (Q–∥) shock are mode converted to kinetic Alfvén waves (KAWs) at the Alfvén resonance surface of the subsolar magnetopause. In this paper, three–dimensional global dayside mode conversion is investigated for cases under various solar wind conditions using the global hybrid model. The global patterns and propagations of KAWs are distinguished and presented. Under a near–critical Mach number ( M A =3), KAW structures due to mode conversion exhibit a feature of broader excitation regions in the magnetopause boundary layer (MPBL) compared to supercritical Mach number ( M A =5) shocks. For cases with an oblique IMF with supercritical Mach numbers ( M A =5), the amplitude of magnetosheath compressional waves is larger at the quasi–parallel shock (Q–∥) than at the quasi–perpendicular (Q–⊥) shock. Downstream of the Q–∥ shock, there is a general trend that the perturbations of density ( N ) and magnetic field ( B ) change from predominantly in–phase in the magnetosheath to antiphase near the MPBL. While downstream of the Q–⊥ shock, an antiphase relation between N and B is dominant throughout the magnetosheath and magnetopause except near the shock transition. The compressional drivers are found to reach an extended region of the magnetopause due to the combined effects of wave propagation in the plasma frame and flow convection, leading to a broad region of mode conversion at the magnetopause. Subsequently, the resulting KAWs can be carried to the regions downstream of the Q–⊥ shock owing to the flow convection at the magnetopause. Furthermore the KAWs propagate poleward along the geomagnetic field lines and meanwhile are carried tailward by the ambient flows, and they are more intense in the downstream of Q–∥ shocks than downstream of Q–⊥ shocks.

79 ASTRONOMY AND ASTROPHYSICS↗

An ensemble of ocean reanalyses for 1815-2013 with sparse observational input

This paper describes a new eight-member ensemble of ocean reanalyses spanning nearly 200 years from 1815 to 2013 generated using the Simple Ocean Data Assimilation system with sparse observational input (SODAsi) to explore long-term changes in the oceans. The eight ensemble members assimilate surface temperature observations and use surface boundary conditions from an atmospheric reanalysis that is loosely coupled to the ocean reanalysis. In this work, both surface and subsurface quantities, such as dynamic height and heat content, show a broad spectrum of variability. Surface temperature trends from 1815 to 2013 are positive in most regions, with some important exceptions; the central Tropical Pacific, around Antarctica, and in the Gulf Stream and Kuroshio extension regions all show cooling trends. A near-global average shows warming of about 0.8°C over the full period, with most of the warming occurring after 1920. There is pronounced multidecadal variability in both the midlatitude and tropical oceans. In the North Atlantic Ocean, temperature variability is highly correlated with the meridional overturning stream function, with the largest correlation occurring when the stream function is advanced by 9 years. Trends of upper ocean heat content and dynamic height from the 1950s onward compare well with previously published values. Globally averaged heat content of the upper 700 m shows a nearly linear rise after the 1920s, requiring a net downward surface heat flux increase of 0.47 W m -2 into the ocean. This is close to published estimates of the increased flux required to explain the heat content increase from 1971 to 2010.

54 ENVIRONMENTAL SCIENCES↗

Turbulent mixing and removal of ozone within an Amazon rainforest canopy

Simultaneous profiles of turbulence statistics and mean ozone mixing ratio are used to establish a relation between eddy diffusivity and ozone mixing within the Amazon forest. A one–dimensional diffusion model is proposed and used to infer mixing time scales from the eddy diffusivity profiles. Data and model results indicate that during daytime conditions, the upper (lower) half of the canopy is well (partially) mixed most of the time and that most of the vertical extent of the forest can be mixed in less than an hour. During nighttime, most of the canopy is predominantly poorly mixed, except for periods with bursts of intermittent turbulence. Even though turbulence is faster than chemistry during daytime, both processes have comparable time scales in the lower canopy layers during nighttime conditions. Nonchemical loss time scales (associated with stomatal uptake and dry deposition) for the entire forest are comparable to turbulent mixing time scale in the lower canopy during the day and in the entire canopy during the night, indicating a tight coupling between turbulent transport and dry deposition and stomatal uptake processes. Because of the significant time of day and height variability of the turbulent mixing time scale inside the canopy, it is important to take it into account when studying chemical and biophysical processes happening in the forest environment. In conclusion, the method proposed here to estimate turbulent mixing time scales is a reliable alternative to currently used models, especially for situations in which the vertical distribution of the time scale is relevant.

54 ENVIRONMENTAL SCIENCES↗

Cloud and circulation feedbacks in a near‐global aquaplanet cloud‐resolving model

Abstract A near‐global aquaplanet cloud‐resolving model (NGAqua) with fixed meridionally varying sea‐surface temperature (SST) is used to investigate cloud feedbacks due to three climate perturbations: a uniform 4 K SST increase, a quadrupled‐CO 2 concentration, and both combined. NGAqua has a horizontal resolution of 4 km with no cumulus parameterization. Its domain is a zonally periodic 20,480 km‐long tropical channel, spanning 46°S–N. It produces plausible mean distributions of clouds, rainfall, and winds. After spin‐up, 80 days are analyzed for the control and increased‐SST simulations, and 40 days for those with quadrupled CO 2 . The Intertropical Convergence Zone width and tropical cloud cover are not strongly affected by SST warming or CO 2 increase, except for the expected upward shift in high clouds with warming, but both perturbations weaken the Hadley circulation. Increased SST induces a statistically significant increase in subtropical low cloud fraction and in‐cloud liquid water content but decreases midlatitude cloud, yielding slightly positive domain‐mean shortwave cloud feedbacks. CO 2 quadrupling causes a slight shallowing and a statistically insignificant reduction of subtropical low cloud fraction. Warming‐induced low cloud changes are strongly correlated with changes in estimated inversion strength, which increases modestly in the subtropics but decreases in the midlatitudes. Enhanced clear‐sky boundary layer radiative cooling in the warmer climate accompanies the robust subtropical low cloud increase. The probability distribution of column relative humidity across the tropics and subtropics is compared between the control and increased‐SST simulations. It shows no evidence of bimodality or increased convective aggregation in a warmer climate.

58 GEOSCIENCES↗

Projected Changes in the Asian‐Australian Monsoon Region in 1.5°C and 2.0°C Global‐Warming Scenarios

Abstract In light of the Paris Agreement, it is essential to identify regional impacts of half a degree additional global warming to inform climate adaptation and mitigation strategies. We investigate the effects of 1.5°C and 2.0°C global warming above preindustrial conditions, relative to present day (2006–2015), over the Asian‐Australian monsoon region (AAMR) using five models from the Half a degree Additional warming, Prognosis and Projected Impacts (HAPPI) project. There is considerable intermodel variability in projected changes to mean climate and extreme events in 2.0°C and 1.5°C scenarios. There is high confidence in projected increases to mean and extreme surface temperatures over AAMR, as well as more‐frequent persistent daily temperature extremes over East Asia, Australia, and northern India with an additional 0.5°C warming, which are likely to occur. Mean and extreme monsoon precipitation amplify over AAMR, except over Australia at 1.5°C where there is uncertainty in the sign of the change. Persistent daily extreme precipitation events are likely to become more frequent over parts of East Asia and India with an additional 0.5°C warming. There is lower confidence in projections of precipitation change than in projections of surface temperature change. These results highlight the benefits of limiting the global‐mean temperature change to 1.5°C above preindustrial, as the severity of the above effects increases with an extra 0.5°C warming.

54 ENVIRONMENTAL SCIENCES↗

Quantifying black carbon deposition over the Greenland ice sheet from forest fires in Canada

We identify an important Black Carbon (BC) aerosol deposition event that was observed in snow stratigraphy and dated to between 27 July 2013 – 2 August 2013. This event comprises a significant portion (~60%) of total deposition over a 10 month period (July 2013 – April 2014). Here we link this event to forest fires burning in Canada during summer 2013 using modeling and remote sensing tools. Aerosols were detected by both the CALIOP and MODIS instruments during transport between Canada and Greenland, confirming that this event involved emissions from forest fires in Canada. We use high-resolution regional chemical transport mod-eling (WRF-Chem) combined with high-resolution fire emissions (FINNv1.5) to study aerosol emissions, transport, and deposition during this event. The model accurately captures the timing of the BC deposition event and shows that the major contribution to deposition during this event is emissions originating from fires in Canada. However, the model under-predicts aerosol deposition compared to measurements at all sites by a factor of 2–100. Under-prediction of modeled BC deposition originates from uncertainties in fire emissions combined with uncertainties in aerosol scavenging by clouds. This study suggests that it is possible to describe the transport of an exceptional smoke event on regional and continental scales. Improvements in model descriptions of precipitation scavenging and emissions from wildfires are needed to correctly predict deposition, which is critical for determining the climate impacts of aerosols that originate from fires.

54 ENVIRONMENTAL SCIENCES↗

A Low Viscosity Lunar Magma Ocean Forms a Stratified Anorthitic Flotation Crust With Mafic Poor and Rich Units

Much of the lunar crust is monomineralic, comprising >98% plagioclase. The prevailing model argues the crust accumulated as plagioclase floated to the surface of a solidifying lunar magma ocean (LMO). Whether >98% pure anorthosites can form in a flotation scenario is debated. An important determinant of the efficiency of plagioclase fractionation is the viscosity of the LMO liquid, which was unconstrained. Here we present results from new experiments conducted on a late LMO-relevant ferrobasaltic melt. The liquid has an exceptionally low viscosity of 0.22 $+0.11\atop{-0.19}$to 1.45 $+0.46\atop{-0.82}$ Pa s at experimental conditions (1,300–1,600°C; 0.1–4.4 GPa) and can be modeled by an Arrhenius relation. Extrapolating to LMO-relevant temperatures, our analysis suggests a low viscosity LMO would form a stratified flotation crust, with the oldest units containing a mafic component and with very pure younger units. Old, impure crust may have been buried by lower crustal diapirs of pure anorthosite in a serial magmatism scenario.

58 GEOSCIENCES↗