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At least 1,135 records · Page 63

The good, the bad, and the ugly: Data-driven load profile discord identification in a large building portfolio

Reducing the overall energy consumption and associated greenhouse gas emissions in the building sector is essential for meeting our future sustainability goals. Recently, smart energy metering facilities have been deployed to enable monitoring of energy consumption data with hourly or subhourly temporal resolution. This unprecedented data collection has created various opportunities for advanced data analytics involving load profiles (e.g., building energy benchmarking programs, building-to-grid integration, and calibration of urban-scale energy models). These applications often need preprocessing steps to detect daily load profile discords, such as: 1) outliers due to system malfunctions (the bad) and 2) irregular energy consumption patterns, such as those resulting from holidays (the ugly) compared to normal consumption patterns (the good). However, current preprocessing methods predominantly focus on filtering using statistical threshold values, which fail to capture the contextual discords of daily profiles. In addition, discord detection algorithms in building research are often aimed at finding individual building-level discords, which are not suitable at a large scale. Thus, here, we develop a method for automated load profile discord identification (ALDI) in a large portfolio of buildings (more than 100 buildings). Specifically, ALDI 1) uses the matrix profile (MP) method to quantify the similarities of daily subsequences in time series meter data, 2) compares daily MP values with typical-day MP distributions using the Kolmogorov-Smirnov test, and 3) identifies daily load profile discords in a large building portfolio. We evaluate ALDI using the metering data of both an academic campus and a residential neighborhood. Our results demonstrate that ALDI efficiently discovers measurement errors by system malfunctions and low energy consumption days in the academic campus portfolio, and it detects unique load shape patterns likely driven by occupant behavior and extreme weather conditions in the residential neighborhood.

32 ENERGY CONSERVATION, CONSUMPTION, AND UTILIZATI↗

New developments and verification of fusion blanket simulation capabilities in the MOOSE framework

Multiphysics modeling capabilities have a crucial role to play in the accelerated deployment of fusion energy. To that end, we developed new multiphysics fusion blanket simulation capabilities in the Multiphysics Object-Oriented Simulation Environment (MOOSE). Firstly, we expanded on the existing capabilities of the previously published work, by coupling 3D tritium transport modeling capabilities using the Tritium Migration Analysis Program, version 8 (TMAP8) to an existing tool including thermal hydraulics, fully three-dimensional (3D) heat transfer, and loosely coupled neutronics analysis. Secondly, we performed a thorough verification of the new capabilities and increased testing code coverage to meet MOOSE’s software quality standards. The MOOSE framework follows a strict software quality assurance plan to be Nuclear Quality Assurance, Level 1 compliant. The new multiphysics fusion blanket simulation capabilities are now held to the same standard. Thirdly, to demonstrate MOOSE’s new fusion blanket modeling capabilities, we performed a fully integrated, multiphysics simulation of a 3D solid ceramic breeder blanket design. This proof-of-concept simulation provides the temperature and tritium distribution across the blanket. In conclusion, the combined efforts towards software quality and the development of multiphysics coupling capabilities provide an effective and reliable framework for modeling solid ceramic fusion blankets using MOOSE.

modeling and simulation↗

Cloud Optical Properties Over West Antarctica From Shortwave Spectroradiometer Measurements During AWARE

A shortwave spectroradiometer was deployed on the West Antarctic Ice Sheet (WAIS) as part of the U.S. Department of Energy Atmospheric Radiation Measurement (ARM) program ARM West Antarctic Radiation Experiment (AWARE). This instrument recorded 1-min averages of downwelling hemispheric spectral irradiance covering the wavelength range 350–2,200 nm with spectral resolution 3 and 10 nm for wavelengths shorter and longer than 1,000 nm, respectively. Using simultaneous micropulse lidar data to identify the thermodynamic phase of stratiform clouds, a radiative transfer algorithm is used here to retrieve optical depth and effective droplet (or particle) size for single-phase liquid water and ice water clouds. The AWARE campaign on the WAIS first sampled typical climatological conditions between 7 December 2015 and 9 January 2016 and then a much warmer air mass with more moisture associated with a surface melt event between 10 and 17 January 2016. Before the melt event most liquid cloud effective droplet radii were consistent with pristine polar maritime clouds (mode radius 13.5 μm) but showed a second local maximum in the distribution (at 8 μm) consistent with colder, moisture-limited conditions. Most ice clouds sampled occurred before the melt event (mode optical depth 4 and effective particle size 19 μm). During the melt event liquid water cloud optical depth nearly doubled (mode value increasing from 8 to 14). AWARE therefore sampled on the WAIS two cases relevant to climate model simulations: typical current climatological conditions, followed by warmer meteorology possibly consistent with future increasing surface melt scenarios.

54 ENVIRONMENTAL SCIENCES↗

Directed assembly of hybrid nanostructures using optically resonant nanotweezers

This represents the final report for this project. Over the course of the project we have made significant progress in photonically driven nano-assembly including: (1) demonstrating the first direct optical tweezer based manipulation of proteins, (2) the ability to apply optical angular torques to microtubuals and other rod-shaped microparticles, (3) direct assembly of hybrid nanostructures comprising of polymeric nanoparticles and carbon nanotubes and, (4) the ability to drive biological reactions (specifically protein aggregation) that are thermodynamically unfavorable by applying localized optical work. These advancements are described in the list of papers provided in section 2.0 of the below. Summary details are provided in prior year annual reports. We have two additional papers which will be submitted shortly based on the work done under this award. An updated publication list will be provided to the program manager when those are accepted. In this report, we report on a new advancement made in the final project year, which uses the nanotweezer technology to perform direct measurements of particle-surface interactions. Briefly, these measurements are important for characterizing the stability and behavior of colloidal and nanoparticle suspensions and current techniques are limited in their ability to measure piconewton scale interaction forces on sub-micrometer particles due to signal detection limits and thermal noise. In this project year we developed a new technique called “Nanophotonic Force Microscopy” which uses the localized region of exponentially decaying, near-field, light to confine small particles close to a surface. From the statistical distribution of the light intensity scattered by the particle the technique maps out the potential well of the trap and directly quantify the repulsive force between the nanoparticle and the surface. The major advantage of the technique is that it can measure forces and energy wells below the thermal noise limit, resolving interaction forces smaller than 1 pN on dielectric particles as small as 100 nm in diameter.

36 MATERIALS SCIENCE↗

Fundamental Studies of the Reforming of Oxygenated Compounds over Supported Metal Catalysts

The main objective of our research has been to elucidate fundamental concepts associated with controlling the activity, selectivity, and stability of bifunctional, metal-based heterogeneous catalysts for tandem reactions, such as liquid-phase conversion of oxygenated hydrocarbons derived from biomass. We have shown that bimetallic catalysts that combine a highly-reducible metal (e.g., platinum) with an oxygen-containing metal promoter (e.g., molybdenum) are promising materials for conversion of oxygenated hydrocarbons because of their high activity for selective cleavage for carbon-oxygen bonds. We have developed methods to stabilize metal nanoparticles against leaching and sintering under liquid-phase reaction conditions by using atomic layer deposition (ALD) to apply oxide overcoat layers. We have used controlled surface reactions to produce bimetallic catalysts with controlled particle size and controlled composition, with an important application being the selective conversion of biomass-derived molecules. The synthesis of catalysts by traditional methods may produce a wide distribution of metal particle sizes and compositions; and thus, results from spectroscopic and reactions kinetics measurements have contributions from a distribution of active sites, making it difficult to assess how the size and composition of the metal particles affect the nature of the surface, the active sites, and the catalytic behavior. Thus, we have developed methods to synthesize bimetallic nanoparticles with controlled particle size and controlled composition to achieve an effective link between characterization and reactivity, and between theory and experiment. We have also used ALD to modify supported metal catalysts by addition of promoters with atomic-level precision, to produce new bifunctional sites for selective catalytic transformations. We have used a variety of techniques to characterize the metal nanoparticles in our catalysts, including scanning transmission electron microcopy (STEM) to measure size and structure, energy dispersive X-ray spectroscopy (EDS) to measure atomic composition, X-ray absorption spectroscopy (XAS) to measure oxidation state and metal coordination, Fourier transform infrared spectroscopy (FTIR) to study adsorbed species, laser Raman spectroscopy to probe metal oxide promoters, and temperature programmed reaction/desorption to study the energetics of adsorption and desorption processes. We have studied our bimetallic catalysts for the selective cleavage of carbon-oxygen bonds, and we have studied the effects of adding metal oxide promoters to supported platinum and gold catalysts for water-gas shift (i.e., the production of hydrogen by reaction of carbon monoxide with water). We anticipate that the knowledge obtained from our studies will allow us to identify promising directions for new catalysts that show high activity, selectivity, and stability for important reactions, such as the conversion of biomass-derived oxygenated hydrocarbons to fuels and chemicals.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Assessing the Interactive Impacts of Energy Efficiency and Demand Response on Power System Costs and Emissions

Utilities are increasingly interested in integrating energy efficiency (EE) and demand response (DR) measures and technologies (as well as other distributed energy resources) as a strategic approach to improve their cost-effectiveness and performance. However, the specific EE and DR features that may be best integrated, the interplay between changing EE and DR resource potential, and resulting utility system impacts are not well understood. We quantify the impacts of EE and DR in isolation and in combination on bulk power system costs and emissions based on changes in generation expansion, transmission expansion, and dispatch patterns. The study methodology mimics utility resource planning and uses more novel techniques to select least-cost generation and transmission capacity from supply-and demand-side resources, as compared to more commonly used utility approaches that only consider supply-side resources. The results identify key EE and DR characteristics affecting each other’s power system value and the most valuable technologies and strategies that can be jointly deployed. We discuss implications for EE and DR cost-effectiveness frameworks, program design, and integrated resource planning.

32 ENERGY CONSERVATION, CONSUMPTION, AND UTILIZATI↗

High-Burnup BWR LOCA Burst Analysis Using High-Fidelity Multiphysics Simulations

The US nuclear industry is looking to improve on the operating economics of the current fleet of light-water reactors (LWRs). One way of achieving this is by operating fuel to higher burnup. In pressurized water reactors (PWRs), relaxing the current burnup limit will allow for cycle length extensions and power uprates; in boiling water reactors (BWRs) it may allow for improved fuel utilization and reduced feed assemblies, as well as more efficient power uprates and increased capacity factors that will support the Administration’s Executive Order to facilitate 5 GW of power uprates at existing nuclear facilities. However, one of the key limitations to operating fuel to higher burnup is the risk of fuel fragmentation, relocation, and dispersal (FFRD). Recognizing the high interest in extending burnup limits, the US Nuclear Regulatory Commission (NRC) has issued Draft Regulatory Guide DG-1434, which defines an approach that would be acceptable to the NRC for addressing FFRD risk. The approach defined will require better understanding of the phenomena leading to FFRD as well as best-estimate simulation methods to understand FFRD risk in high-burnup cores. The Nuclear Energy Advanced Modeling and Simulation program is supporting the FFRD industry challenge problem through development of state-of-the-art, high-fidelity modeling and simulation LWR analysis capabilities; namely, the BISON fuel performance code and the VERA core simulator software. These tools, along with the US NRC TRACE system analysis code, have been utilized for analysis of FFRD risk in both PWR and BWR cores in recent years. The work documented in this report addresses the lack of high-fidelity research for BWRs and builds on a previous activity where the framework has been applied to Cycles 16 through 18 of Limerick Unit 1, a BWR/4, with introduction of 8 high-burnup lead use assemblies (HBLUAs) that were representative of the 8 HBLUAs loaded into Limerick Unit 2 in 2021. VERA was used in this previous activity to model rod-by-rod depletion in these cycles, and its solution was used to initialize a TRACE simulation of a large-break loss-of-coolant accident (LBLOCA) at the end of Cycle 18. In the work documented in this report, the TRACE model was improved by refining the core mesh and utilizing a new feature that allows for capturing the full 3D VERA power distribution in the model. This allows for a more detailed solution for setting BISON boundary conditions. Furthermore, the solutions from VERA and TRACE were used to set up and perform BISON simulations of about 1,000 rods sampled from the core, including all burnup levels. Utilizing two cladding burst models, it was shown that no fuel rods were predicted to burst during the postulated LBLOCA transient. Additionally, a sensitivity study was performed by artificially increasing linear heat rate during the postulated LBLOCA to identify parameters that correlate with rod burst susceptibility. Burnup, fission gas release, and hoop strain were all found to be positively correlated with rod burst susceptibility. Small-break loss-of-coolant accident (SBLOCA) analyses were also performed; these analyses predicted cladding temperature increases that were bounded by the LBLOCA cladding temperatures for all small break sizes studied for this plant. However, future refinements to the plant response assumptions during the SBLOCA could impact the predicted cladding response. Finally, a benchmark study was performed between CTF and TRACE for LOCA conditions to better qualify CTF for BWR LOCA modeling.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

The creation of high-temperature superconducting cables of megawatt range in Russia

Urgent problems of the power industry in the 21st century require the creation of smart energy systems, providing a high effectiveness of generation, transmission, and consumption of electric power. Simultaneously, the requirements for controllability of power systems and ecological and resource-saving characteristics at all stages of production and distribution of electric power are increased. One of the decision methods of many problems of the power industry is the development of new high-efficiency electrical equipment for smart power systems based on superconducting technologies to ensure a qualitatively new level of functioning of the electric power industry. The intensive research and development of new types of electrical devices based on superconductors are being carried out in many industrialized advanced countries. Interest in such developments has especially increased in recent years owing to the discovery of so-called high-temperature superconductors (HTS) that do not require complicated and expensive cooling devices. Such devices can operate at cooling by inexpensive and easily accessible liquid nitrogen. Taking into account the obvious advantages of superconducting cable lines for the transmission of large power flows through an electrical network, as compared with conventional cables, the Federal Grid Company of Unified Energy System (JSC FGC UES) initiated a research and development program including the creation of superconducting HTS AC and DC cable lines. Two cable lines for the transmitted power of 50 MVA/MW at 20 kV were manufactured and tested within the framework of the program.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Search for dark matter decaying to two displaced muons produced in proton-proton collisions at 13 TeV with the CMS detector, and for dark photons produced in electron-positron fixed-target collisions at 500 MeV with the PADME detector

Two novel searches for dark matter using particle accelerators are presented. The first is a search for inelastically-coupled dark matter with the CMS detector at CERN, relying on 137 fb$^{-1}$ of proton-proton collision data collected at 13 TeV center-of-mass energy between 2016 and 2018. The search strategy exploits the striking signature expected of inelastic dark matter: a pair of displaced, soft, and narrow muons collimated with missing transverse momentum and recoiled off an initial-state radiation jet. This is the first search for inelastic dark matter at a hadron collider. The second experiment is PADME, a small-scale detector to search for dark photons located in Frascati, Italy. PADME seeks to detect the production of dark photons in positron-electron collisions with a stationary diamond target and a 500 MeV positron beam. The missing-mass technique employed in the experiment relies on constraining all four-momenta in the system except for the dark photon and lookin g for a bump in the resulting invariant mass distribution corresponding to the dark photon's mass. The projected sensitivity for both experiments is compared in the context of highlighting the need for a comprehensive experimental search program for dark matter. Both analyses expect first public results by the end of 2020.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Chefornak Energy Configuration Options: Energy Infrastructure Optimization to Reduce Fuel Cost and Dependence in Chefornak, Alaska

The U.S. Department of Energy is funding, through the Grid Modernization Program, the Alaska Microgrid Partnership (AMP), a multi-stakeholder collaborative comprised of national labs and Alaska based partners. The over-arching goal of AMP is to reduce the use of total imported fuel into communities to secure all energy services by at least 50% in Alaska's remote microgrids without increasing system lifecycle costs, while improving overall system reliability, security, and resilience. One goal of AMP is to investigate if a combination of Energy Efficiency (EE) and high contribution (from Renewable Energy (RE)) power systems can reduce total imported energy usage by 50% while lowering Life Cycle Costs (LCC) and improving reliability and resiliency. A techno-economic analysis was conducted for the community of Chefornak to investigate system architectures that could meet the goal of reducing imported fuel consumption by 50% or more.

24 POWER TRANSMISSION AND DISTRIBUTION↗

The ATLAS experiment software on ARM

With an increased dataset obtained during the Run 3 of the LHC at CERN and the even larger expected increase of the dataset by more than one order of magnitude for the HL-LHC, the ATLAS experiment is reaching the limits of the current data processing model in terms of traditional CPU resources based on x86_64 architectures and an extensive program for software upgrades towards the HL-LHC has been set up. The ARM architecture is becoming a competitive and energy efficient alternative. Some surveys indicate its increased presence in HPCs and commercial clouds, and some WLCG sites have expressed their interest. Chip makers are also developing their next generation solutions on ARM architectures, sometimes combining ARM and GPU processors in the same chip. Consequently it is important that the ATLAS software embraces the change and is able to successfully exploit this architecture. We report on the successful porting to ARM of the Athena software framework, which is used by ATLAS for both online and offline computing operations. Furthermore we report on the successful validation of simulation workflows running on ARM resources. For this we have set up an ATLAS Grid site using ARM compatible middleware and containers on Amazon Web Services (AWS) ARM resources. The ARM version of Athena is fully integrated in the regular software build system and distributed in the same way as other software releases. In addition, the workflows have been integrated into the HEPscore benchmark suite which is the planned WLCG wide replacement of the HepSpec06 benchmark used for Grid site pledges. In the overall porting process we have used resources on AWS, Google Cloud Platform (GCP) and CERN. A performance comparison of different architectures and resources will be discussed.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Multiphysics Simulations of MSRE with NEAMS Thermal Hydraulics Tools

This report documents the benchmarks being developed and simulations performed using tools and codes developed under the Nuclear Energy Advanced Modeling and Simulation (NEAMS) program, utilizing MSRE experimental data. In FY23, three main work scopes were investigated under the NEAMS MSR work package at ANL. The first scope investigated the Griffin-SAM coupling model for simulating the pump startup transient experiment of MSRE. The analyses start with a simple model (single-channel, single-lattice), gradually adding more details (multi-channel, full-core) into the model. The results show that the reactivity loss curve is very sensitive to the axial boundary conditions and the radial core discretization. The simple model can predict a similar reactivity trend as that of the more sophisticated model, which is likely due to error cancellation. Accurately modeling the axial boundary condition may further improve the reactivity trend but would require significant efforts to generate the mesh of the MSRE inlet and upper plenum. The core channel radial discretization for the Griffin-SAM coupled model also depends on the flow distribution. Given the complex geometry in the inlet plenum, the flow distribution needed to be calculated from CFD analysis, which was performed using the NekRS code. This analysis employed a MSRE CAD model developed by Copenhagen Atomics. The CAD model was disassembled to keep the inlet plenum region only, which was subsequently cleaned and modified so that the mesh generated is under the memory limit. The results are merged to a few radial regions to show that the flow rate is highest in the central region. This would be useful for future improvement of the Griffin-SAM coupling model of the MSRE core. The last task investigated is tritium transport modeling using the standalone SAM code. This task aimed to initiate the effort to demonstrate and validate the tritium transport model implemented in SAM. The preliminary investigation employed an MSRE model consisting of the primary loop. Three tritium transport pathways were examined including the retention in the graphite, the permeation through the HX tube wall, and the removal from the off-gas system. The results compare well with the MSRE data, but improvements are still needed on the initial conditions (i.e., the present state may not have reached equilibrium), the boundary conditions, the off-gas system modeling, and a better numerical strategy to reach the equilibrium state.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Bike and Scoot to Transit

In this project, we developed a micromobility first-mile service for customers to access public transit. We launched this service as a pilot in the Seattle area that incentivized transit customers to bike or scoot to transit. The objective was to learn how to integrate different micromobility services and provide a unified reward program. Our pilot was called “Bike and Scoot to Transit” and ran from November 2022 to September 2023. More than a dozen locations were selected near transit hubs and light rail/train stations as preferred parking locations. Trips ending at those locations were partially funded. The pilot supported 19,226 qualified trips and distributed $73,000 in total benefits for the participants of the pilot. This dataset was collected from our pilot, which includes the following: - Monthly data: Monthly trip and funding summaries. - Data summary: Data broken down based on the micromobility service provider and equipment. - Trip data: List of all trips recorded during the pilot. - Pricing models: Fees charged by micromobility service providers. ![bike to transit](bike-transit.png)

32 ENERGY CONSERVATION, CONSUMPTION, AND UTILIZATI↗

Costa - Introduction to 2015 Annual Report

In parallel with Sandia National Laboratories having two major locations (NM and CA), along with a number of smaller facilities across the nation, so too is the distribution of scientific, engineering and computing resources. As a part of Sandia’s Institutional Computing Program, CA site-based Sandia computer scientists and engineers have been providing mission and research staff with local CA resident expertise on computing options while also focusing on two growing high performance computing research problems. The first is how to increase system resilience to failure, as machines grow larger, more complex and heterogeneous. The second is how to ensure that computer hardware and configurations are optimized for specialized data analytical mission needs within the overall Sandia computing environment, including the HPC subenvironment. All of these activities support the larger Sandia effort in accelerating development and integration of high performance computing into national security missions. Sandia continues to both promote national R&D objectives, including the recent Presidential Executive Order establishing the National Strategic Computing Initiative and work to ensure that the full range of computing services and capabilities are available for all mission responsibilities, from national security to energy to homeland defense.

97 MATHEMATICS AND COMPUTING↗

Optimal Power Flow in DC Networks with Robust Feasibility and Stability Guarantees

With high penetrations of renewable generation and variable loads, there is significant uncertainty associated with power flows in DC networks such that stability and operational constraint satisfaction are of concern. Most existing DC network optimal power flow (DN-OPF) formulations assume exact knowledge of loading conditions and do not provide stability guarantees. Here, in contrast, this paper studies a DN-OPF formulation which considers both stability and operational constraint satisfaction under uncertainty. The need to account for a range of uncertainty realizations in this paper's robust optimization formulation results in a challenging semi-infinite program (SIP). The proposed solution algorithm reformulates this SIP into a computationally tractable problem by constructing a tight convex inner approximation of the stability set using sufficient conditions for the existence of a feasible and stable power flow solution. Optimal generator set-points are obtained by optimizing over the proposed convex stability set. The validity and effectiveness of the propose algorithm is demonstrated through various DC networks adapted from IEEE test cases.

24 POWER TRANSMISSION AND DISTRIBUTION↗

NSA Site Science: Use of ARM Observations from Northern Alaska to Evaluate and Improve Prediction Capabilities

The Arctic is warming at a rate nearly double that of the rest of the planet, leading to profound changes in atmospheric, oceanic, and ice processes. The U.S. Department of Energy's (DOE) Atmospheric Radiation Measurement (ARM) user facility has played a significant role in Arctic research, operating observatories in Alaska's North Slope for over 25 years. These observatories provide a rich, and wide-reaching dataset that offers insight into atmospheric processes in northern Alaska. This report details the results of a nine-year research project (2015–2024) supported by the DOE Atmospheric Systems Research (ASR) program, that leverages data from ARM’s deployment of observing facilities at Utqiaġvik (known as the North Slope of Alaska, or NSA, site) and Oliktok Point, Alaska. The project was conducted in two phases: - Phase 1 (2015–2019): Focused on understanding key atmospheric processes at Oliktok Point, including cloud formation, high-latitude precipitation, aerosol-cloud interactions, and cloud properties. - Phase 2 (2019–2024): Extended the research to the broader North Slope region, using data from both Oliktok Point and Utqiaġvik. Topics explored included surface energy budgets, atmospheric stability, ice nucleation processes, and microphysics in Arctic clouds. The project resulted in numerous research products, including 50 peer-reviewed publications and dissertations, 169 presentations, and 10 data products. These products cover a variety of topics, including: - Cloud Macro- and Microphysical Properties: Arctic clouds play a crucial role in energy transfer, and accurate representation in models is critical. The study explored cloud transitions, ice crystal shapes, and dual-wavelength radar data to understand ice crystal habits and size distributions. - Aerosol Properties and Processes: The team examined aerosol sources in the Arctic, including industrial emissions and natural sources. Observations showed significant spatial gradients in aerosol concentrations due to human activities and wildfire smoke. The influence of aerosols on cloud formation and the surface energy budget was also assessed. - Aerosol-Cloud Interactions: Research revealed that aerosols might suppress cloud ice production, affecting cloud radiative forcing and precipitation. The impact of local industrial emissions on cloud properties was also investigated. - Contextualizing the North Slope of Alaska in the context of the broader Arctic: To understand broader trends, the project evaluated large-scale circulation patterns and the influence of weather systems on the Arctic. Studies indicated that large-scale processes play a significant role in temperature patterns and the timing of snowmelt. - Advancing ARM Observational and Modeling Capabilities: The project developed new radar data products and advanced measurement techniques, including clutter mitigation and drizzle detection. Uncrewed aerial systems (UAS) and tethered balloon systems (TBS) were deployed to gather detailed atmospheric data. Additionally, the project supported 10 early career scientists, providing training and mentorship to undergraduate interns, graduate students, postdoctoral researchers, and early career researchers. These efforts contributed to the advancement of ARM research capabilities and fostered a new generation of scientists skilled in Arctic atmospheric research. Ultimately, this ASR-supported project has provided valuable insights into Arctic atmospheric processes and their broader climate implications. Recommendations for future work include continuing support for long-term observing at Arctic locations to foster additional research, further exploration of aerosol-cloud interactions and the potential impacts of enhanced industrialization of the Arctic, and expanded use of uncrewed systems to gather data in this remote and harsh environment. Additionally, the data products developed by this work, and the data products developed through the ARM infrastructure, leave a treasure-trove of additional information that should be explored for many years to come to gain additional insight into physical processes in the Arctic atmosphere that drive the rapid changes occurring in at high latitudes and their global impact.

58 GEOSCIENCES↗

Challenges of Maintaining Institutional Controls: Maintenance of an Alternate Water Supply- A Case Study - 19583

The US Department of Energy (DOE) cofunded an alternate water-supply system (AWSS) with the Indian Health Service that was installed in the vicinity of the former uranium mill site near Riverton, Wyoming, as one of the institutional controls (ICs) at the site. The AWSS was constructed in 1998 to supply drinking water to residents within the IC boundary in lieu of drinking untreated groundwater that could potentially be impacted by the contaminated shallow aquifer. The AWSS derives water from three source wells that pump groundwater from the sandstones of the Wind River Formation to a 3.8 x 106 liter (1,000,000 gallon) storage tank. Water from the storage tank is distributed throughout the AWSS service area by approximately 18 kilometers (11 miles) of PVC pipeline. The AWSS currently serves 103 residential customers and 1 commercial customer. DOE and the Northern Arapaho tribe (owner of the AWSS) have partnered over the years to address numerous challenges with the AWSS that included engineering assessments, scientific investigations, sampling support, a hydrant flushing program, and funding. Challenges with the AWSS have included the following: (1) Transmission pipe installed during initial construction did not have a pressure rating high enough to account for system pressure surges. (2) AWSS appurtenances were initially installed without accounting for the effects of corrosive soils on metal components. (3) Natural radium from the Wind River Formation groundwater builds up in the AWSS transmission pipes to levels above the primary drinking water standard because of the lack of a flushing program, dead-end lines, and low system demand. A 2-year study showed that a unidirectional hydrant-flushing program will control the radium buildup. (4) Aging system components including hydrants, valves, and pumps are nearing their effective lifespan and are in need of replacement. (5) With the addition of large commercial customers, demand on the system has increased since the initial installation of the system, and future growth in the area will continue to increase demand. (6) Additional connections and integration of the AWSS with an areawide water system in the near future will require changes to the current flushing plan and add additional complexity regarding areas of responsibility. (7) A well-organized financial and administrative infrastructure is not in place, and additional revenue is needed to operate, maintain, and improve the AWSS. To be a viable IC, the AWSS will require management, maintenance, and upgrades to provide safe drinking water until groundwater meets drinking water standards. Responsibilities and funding for maintaining the AWSS as a viable IC are the focus of current discussions, and decisions regarding responsibilities and funding will be formalized in future cooperative agreements and memoranda of understanding with the owners. (authors)

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Moderator design studies for a new neutron reference source based on the $\mathrm{D}$–$\mathrm{T}$ fusion reaction

The radioactive isotope Californium-252 ( 252 Cf) is relied upon internationally as a neutron calibration source for ionizing radiation dosimetry because of its high specific activity. The source may be placed within a heavy-water (D 2 O) moderating sphere to produce a softened spectrum representative of neutron fields common to commercial nuclear power plant environments, among others. Due to termination of the U.S. Department of Energy loan/lease program in 2012, the expense of obtaining 252 Cf sources has undergone a significant increase, rendering high output sources largely unattainable. On the other hand, the use of neutron generators in research and industry applications has increased dramatically in recent years. Neutron generators based on deuterium-tritium (D-T) fusion reaction provide high neutron fluence rates and, therefore, could possibly be used as a replacement for 252 Cf. To be viable, the 14.6 MeV D-T output spectrum must be significantly moderated to approximate common workplace environments. Here this paper presents the results of an effort to select appropriate moderating materials and design a configuration to reshape the primary neutron field toward a spectrum approaching that from a nuclear power plant workplace. A series of Monte-Carlo (MCNP) simulations of single layer high- and low-Z materials are used to identify initial candidate moderators. Candidates are refined through a similar series of simulations involving combinations of 2 to 5 different materials. The simulated energy distribution using these candidate moderators are rated in comparison to a target spectrum. Other properties, such as fluence preservation and/or enhancement, prompt gamma production and other characteristics are also considered.

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗