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NASA NTRS1991

Molecular dynamics of phenol at the liquid-vapor interface of water

Results of molecular dynamics calculations on phenol at the water liquid-vapor interface are presented. The density profile of the center of mass of phenol exhibits a maximum 1 A from the Gibbs surface toward the vapor phase, indicating that the molecule is surface-active. Changes in the profile caused by the interface extend 6 A from the Gibbs surface into the liquid, significantly more than change in the density profile of water. The most probable orientation of the solute at the surface is such that its symmetry axis is perpendicular to the interface with the OH substituent pointing toward the liquid. An additional simulation with benzene shows that this molecule at the surface most often adopts orientations parallel to the interface. Deeper in the liquid all the solutes are preferentially ordered perpendicular to the surface. In the interfacial region the orientational preferences of the solute are primarily determined by cavity formation needed to accommodate the hydrophobic portion of the dissolved molecule.

Pohorille, Andrew↗

NASA NTRS1991

Temperature sensitivity of differential absorption lidar measurements of water vapor in the 720-nm region

Recently measured properties of water vapor (H2O) absorption lines have been used in calculations to evalute the temperature sensitivity of differential absorption lidar (Dial) H2O measurements. This paper estimates the temperature sensitivity of H2O lines in the 717-733-nm region for both H2O mixing ratio and number density measurements, and discusses the influence of the H2O line ground state energies E-double-prime, the H2O absorption linewidths, the linewidth temperature dependence parameter, and the atmospheric temperature and pressure variations with altitude and location on the temperature sensitivity calculations. Line parameters and temperature sensitivity calculations for 67 H2O lines in the 720-nm band are given which can be directly used in field experiments. Water vapor lines with E-double-prime values in the 100-300/cm range were found to be optimum for Dial measurements of H2O number densities, while E-double-prime values in the 250-500/cm range were found to be optimum for H2O mixing ratio measurements.

Browell, Edward V.↗

NASA NTRS1990

In-situ atmospheric water-vapor retrieval in support of AVIRIS validation

A comparison is made between two ground-based atmospheric water-vapor measurement techniques, each of which uses data from a solar-pointing radiometer. One technique uses visible wavelength channels to retrieve aerosol loading, surface pressure readings for Rayleigh scattering analyses, and the 0.94 micron channel to extract water vapor from the residual of total versus scattering opacity. The other technique requires only the ratio of channels centered at 0.94 and 0.87 micron. Results are given for the April 13, 1989 AVIRIS in-flight calibration.

Bruegge, Carol J.↗

NASA NTRS1991

Quantification of vapor screen analysis

The traditionally qualitative method of vapor screening is applied to the task of gathering quantitative density measurements in supersonic flows. Quantitative density information for flow around a two-dimensional biconvex airfoil at Mach 2.8 is extracted from digitized images of vapor screens by assuming a linear relation between particle density and scattering intensity. Intensity readings are calibrated through known conditions in the free stream and at the airfoil bow shock. The experimental results are compared to densities generated by a Euler code and determined to have errors of less than ten percent.

Benedict, Lance H.↗

NASA NTRS1991

Retrieval of atmospheric water vapor profiles using radiometric measurements at 183 and 90 GHz

The algorithm developed by Wilheim (1990) dealt with the retrieval of water-vapor profiles from microwave radiometric measurements, even in the presence of clouds. This algorithm was tested using radiometric measurements at frequencies near 90 and 183 GHz; the results show that the retrieved water-vapor profiles were in general agreement with those derived from radiosonde data. In particular, retrieval over both land and ocean surfaces generated clouds at locations that could be verified from satellite photographs. The algorithm did not perform well where there were surface fronts. These clouds possibly contained ice particles as well as precipitating snow, which the algorithm was not expected to handle.

Lutz, Robert↗

NASA NTRS1991

A nuclear driven metallic vapor MHD coupled with MPD thrusters

Nuclear energy as a source of power for space missions, represents an enabling technology for advanced and ambitious space applications. Nuclear fuel in a gaseous or liquid form has been configured as a promising and practical candidate in this regard. The present study investigates and performs a feasibility analysis of an innovative concept for space power generation and propulsion. The system embodies a conceptual nuclear reactor with an MHD generator and coupled to MPD thrusters. The reactor utilizes liquid uranium in droplet form as fuel and superheated metallic vapor as the working fluid. This ultrahigh temperature vapor core reactor brings forward varied and challenging technical issues, and it has been addressed to in this paper. A parametric study of the conceived system has been performed in a qualitative and quantitative manner. Preliminary results show enough promise for further indepth analysis of this novel system.

Anghaie, Samim↗

NASA NTRS1990

Vapor-screen technique applied to a delta-wing aircraft

Recently, the vapor-screen technique has been applied to a delta-wing aircraft (F-106B) during both subsonic 1-g and transonic high-g flights. Selected subsonic vapor-screen images are presented which show the benefits of digital enhancement. Among the major findings are that multiple, corotating vortices exist up to 20-deg angle of attack, and the measured flight core location is not well predicted by theory. Planned extensions for this work are also discussed.

Lamar, John E.↗

NASA NTRS1991

Effect of Liquid Surface Turbulent Motion on the Vapor Condensation in a Mixing Tank

The effect of liquid surface motion on the vapor condensation in a tank mixed by an axial turbulent jet is numerically investigated. The average value (over the interface area) of the root-mean-squared (rms) turbulent velocity at the interface is shown to be linearly increasing with decreasing liquid height and increasing jet diameter for a given tank size. The average rms turbulent velocity is incorporated in Brown et al. (1990) condensation correlation to predict the condensation of vapor on a liquid surface. The results are in good agreement with available condensation data.

Lin, C. S.↗

NASA NTRS1992

Study of optical techniques for the Ames unitary wind tunnels. Part 2: Light sheet and vapor screen

Light sheet and vapor screen methods have been studied with particular emphasis on those systems that have been used in large transonic and supersonic wind tunnels. The various fluids and solids used as tracers or light scatters and the methods for tracing generation have been studied. Light sources from high intensity lamps and various lasers have been surveyed. Light sheet generation and projection methods were considered. Detectors and location of detectors were briefly studied. A vapor screen system and a technique for location injection of tracers for the NASA Ames 9 by 7 foot Supersonic Wind Tunnel were proposed.

Lee, George↗

NASA NTRS1992

Vapor crystal growth studies of single crystals of mercuric iodide (3-IML-1)

A single crystal of mercuric iodide (HgI2) will be grown during the International Microgravity Lab. (IML-1) mission. The crystal growth process takes place by sublimation of HgI2 from an aggregate of purified material, transport of the molecules in the vapor from the source to the crystal, and condensation on the crystal surface. The objectives of the experiment are as follow: to grow a high quality crystal of HgI2 of sufficient size so that its properties can be extensively analyzed; and to study the vapor transport process, specifically the rate of diffusion transport at greatly reduced gravity where convection is minimized.

Vandenberg, Lodewijk↗

NASA NTRS1992

An atlas of upper tropospheric radiances observed in the 6 to 7-micrometer water vapor band using TOVS data from the NOAA weather satellites during 1979-1991

This document is a pictorial atlas of the Earth's radiance emitted in the 6 to 7 micro-m water vapor band. At these wavelengths, the infrared brightness temperature corresponds to the layer-average temperature of the top few millimeters of water vapor in the atmosphere. At low altitudes, bright regions are dry slots in the upper troposphere. The satellite observations were obtained from NOAA's cloud and angle corrected measurements made by a series of polar orbiting TOVS (TIROS Operational Vertical Sounder) instruments flown from 1979 to 1991. TOVS 6.7 micro-m and 7.2 micro-m channels were converted to a single brightness temperature that simulates a high altitude channel near '6.5' micro-m. For climatological studies, the daily '6.5' micro-m overpass data were gridded to a cartesian projection with 5 by 5 degree horizontal resolution between 40 degrees N and 40 degrees S latitude. This atlas presents greyscale images of the '6.5' micro-m brightness fields for every day in every month for 13 years. The mean brightness for each of the 12 months for 13 years is presented to display interannual variability, and the annual cycle of 12 monthly means is summarized on a single page. Statistical summaries are presented from other investigations in progress.

Chesters, Dennis↗

NASA NTRS1992

BELINDA: Broadband Emission Lidar with Narrowband Determination of Absorption. A new concept for measuring water vapor and temperature profiles

We present a new concept for differential absorption lidar measurements of water vapor and temperature profiles. The idea is to use one broadband emission laser and a narrowband filter system for separation of the 'online' and 'offline' return signals. It is shown that BELINDA offers improvements as to laser emission shape and stability requirements, background suppression, and last and most important a significant reduction of the influence of Rayleigh scattering. A suitably designed system based on this concept is presented, capable of measuring water vapor or temperature profiles throughout the planetary boundary layer.

Theopold, F. A.↗

NASA NTRS1992

Investigations on atomic-vapor-filter high-spectral-resolution lidar for temperature measurements

The temperature measurement by the analysis of Rayleigh scattered laser radiation with atomic vapor filters is investigated in both theory and laboratory experiments. Synthetic air is irradiated with a cw dye laser at 283 nano-meters, and the backscattered spectrum is analyzed with two lead vapor cells in one oven. Temperature measurements are carried out, and the effect of different parameters on the accuracy is investigated. Important aspects for the realization of a lidar are given.

Voss, E.↗

NASA NTRS1992

Vaporizing particle velocimeter

A velocimeter measures flow characteristics of a flow traveling through a chamber in a given direction. Tracer particles are entrained in the flow and a source of radiant energy produces an output stream directed transversely to the chamber, having a sufficient intensity to vaporize the particles as they pass through the output stream. Each of the vaporized particles explodes to produce a shock wave and a hot core, and a flow visualization system tracks the motion of the hot cores and shock waves to measure the velocity of each tracer particle and the temperature of the flow around the tracer.

Weinstein, Leonard M.↗

NASA NTRS1991

An evaluation of water vapor radiometer data for calibration of the wet path delay in very long baseline interferometry experiments

The internal consistency of the baseline-length measurements derived from analysis of several independent VLBI experiments is an estimate of the measurement precision. The paper investigates whether the inclusion of water vapor radiometer (WVR) data as an absolute calibration of the propagation delay due to water vapor improves the precision of VLBI baseline-length measurements. The paper analyzes 28 International Radio Interferometric Surveying runs between June 1988 and January 1989; WVR measurements were made during each session. The addition of WVR data decreased the scatter of the length measurements of the baselines by 5-10 percent. The observed reduction in the scatter of the baseline lengths is less than what is expected from the behavior of the formal errors, which suggest that the baseline-length measurement precision should improve 10-20 percent if WVR data are included in the analysis. The discrepancy between the formal errors and the baseline-length results can be explained as the consequence of systematic errors in the dry-mapping function parameters, instrumental biases in the WVR and the barometer, or both.

Kuehn, C. E.↗

NASA NTRS1992

Effects of buoyancy-driven flow and thermal boundary conditions on physical vapor transport

A 2D numerical model was developed in order to ascertain if reduced gravity conditions are beneficial to physical vapor transport (PVT) and to determine its tolerance limits to residual accelerations. This was solved using the PHOENICS finite-volume code. Reduction of gravitational accelerations to less than 0.1 g0 was found to be sufficient to suppress buoyancy-driven convection to an extent that diffusion was the dominant transport mode, whence a greater uniformity in the growth rate could be obtained. It is shown that a uniform temperature gradient on the ampoule walls causes the vapor to be supersaturated throughout the ampoule, potentially resulting in undesirable nucleation at the walls. A 'hump' in the wall temperature profile can be used to avoid this. The prevailing transport conditions determine the size of the hump needed.

Nadarajah, Arunan↗

NASA NTRS1992

The slant path atmospheric refraction calibrator - An instrument to measure the microwave propagation delays induced by atmospheric water vapor

The water vapor-induced propagation delay experienced by a radio signal traversing the atmosphere is characterized by the Slant Path Atmospheric Refraction Calibrator (SPARC), which measures the difference in the travel times between an optical and a microwave signal propagating along the same atmospheric path with an accuracy of 15 picosec or better. Attention is given to the theoretical and experimental issues involved in measuring the delay induced by water vapor; SPARC measurements conducted along a 13.35-km ground-based path are presented, illustrating the instrument's stability, precision, and accuracy.

Walter, Steven J.↗

NASA NTRS1992

Vapor-liquid equilibrium thermodynamics of N2 + CH4 - Model and Titan applications

A thermodynamic model is presented for vapor-liquid equilibrium in the N2 + CH4 system, which is implicated in calculations of the Titan tropospheric clouds' vapor-liquid equilibrium thermodynamics. This model imposes constraints on the consistency of experimental equilibrium data, and embodies temperature effects by encompassing enthalpy data; it readily calculates the saturation criteria, condensate composition, and latent heat for a given pressure-temperature profile of the Titan atmosphere. The N2 content of condensate is about half of that computed from Raoult's law, and about 30 percent greater than that computed from Henry's law.

Thompson, W. R.↗