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At least 1,117 records · Page 62

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NASA NTRS1978

Interactions of simultaneous perturbations of stratospheric photochemistry

The combined effects of two specific ozone perturbation mechanisms are examined. The need to look back to predictions of the near past as well as the future as a means of testing model results is emphasized. The two perturbations examined are that due to chlorofluoromethane (CFM) release and that due to the air pollutants CO and nitrogen oxide. A steady-state model is used to investigate the characteristics of the stratospheric-tropospheric photochemical system for differing levels of CO and nitrogen oxide fluxes at the ground and for simultaneously changing the stratospheric from CFM release. Two basic scenarios chosen to illustrate the competing effects of the two types of perturbation use the time-dependence for chlorine radical buildup calculated for constant continued release of CFM's.

Butler, D. M.↗

NASA NTRS1978

The Limb Infrared Monitor of the Stratosphere (LIMS) experiment

The Limb Infrared Monitor of the Stratosphere is used to obtain vertical profiles and maps of temperature and the concentration of ozone, water vapor, nitrogen dioxide, and nitric acid for the region of the stratosphere bounded by the upper troposphere and the lower mesosphere.

Russell, J. M.↗

NASA NTRS1979

The NASA-Ames Research Center stratospheric aerosol model. 2. Sensitivity studies and comparison with observatories

Sensitivity tests were performed on a one-dimensional, physical-chemical model of the unperturbed stratospheric aerosols, and model calculations were compared with observations. The tests and comparisons suggest that coagulation controls the particle number mixing ratio, although the number of condensation nuclei at the tropopause and the diffusion coefficient at high altitudes are also important. The sulfur gas source strength and the aerosol residence time are much more important than the supply of condensation nuclei in establishing mass and large particle concentrations. The particle size is also controlled mainly by gas supply and residence time. In situ observations of the aerosols and laboratory measurements of aerosols, parameters that can provide further information about the physics and chemistry of the stratosphere and the aerosols found there are provided.

Toon, O. B.↗

NASA NTRS1978

Stratospheric composition balloon, aircraft and rocket-borne experiments, 28-30 September 1977 (systems, instruments, trajectories, supporting measurements)

The STRATCOM (STRATospheric COMposition) is a long term multipurpose program for integrated, correlated measurements of stratospheric parameters related to composition, thermodynamics, and radiative balance. Balloon 8-b, carrying a solar-pointing grating infrared spectrometer, two CO2 thermal emission radiometers and two in-situ air temperature sensors was launched at 1251 MST on 28 September 1977 to float at an altitude of 39 km from 1521 MST with the instruments making measurements at that altitude through the time of sunset at 1822 MST. Balloon 8-a lifted a payload consisting of four UV filter photometers, two UV spectrometers, two chemiluminescent ozonesondes, dasibi ozone monitor, 14 tube cryogenic sampler, two aluminum oxide H2O sensors, four air temperature sensors, atmospheric pressure sensor, infrared and visible pyranometers, downward-looking camera, blunt-kryton lamp-Gerdien condenser probe, three component anemometer, balloon apex-plate payload and three parachute-borne dropsondes.

Ballard, H. N.↗

NASA NTRS1978

Statistical sampling analysis for stratospheric measurements from satellite missions

Earth orbiting satellite experiments can be designed to measure stratospheric constituents such as ozone by utilizing remote sensing techniques. Statistical analysis techniques, mission simulation and model development have been utilized to develop a method for analyzing various mission/sensor combinations. Existing and planned NASA satellite missions such as Nimbus-4 and G, and Stratospheric Aerosol and Gas Experiment-Application Explorer Mission (SAGE-AEM) have been analyzed to determine the ability of the missions to adequately sample the global field.

Drewry, J. W.↗

NASA NTRS1978

Long period time variations of ozone in the lower stratosphere

Observations of total ozone at a number of stations in the Northern Hemisphere show an increase during the period 1961-1970 followed by a decrease of ozone during the 1970's, at least at many stations in Central Europe. It is well known that total ozone is highly correlated with ozone in the lower stratosphere. Analysis of the trends of ozone based on data derived from balloon-borne ozonesondes during the period 1967-75 at four stations in Central Europe shows that most of the ozone variations occurred in the lower stratosphere with relatively little contribution from tropospheric changes or those above the ozone peak. Possible meteorological origins of these decade type variations will be discussed.

London, J.↗

NASA NTRS1978

SSTs, nitrogen fertiliser and stratospheric ozone

A recently revised model of the stratosphere is used to show that a substantial enhancement in the ozone layer could accompany worldwide SST fleet operations and that water vapor may be an important factor in SST assessments. Revised rate coefficients for various ozone-destroying reactions are employed in calculations which indicate a slight increase in the total content of stratospheric ozone for modest-sized fleets of SSTs flying below about 25 km. It is found that water-vapor chemical reactions can negate in large part the NOx-induced ozone gains computed below 25 km and that increased use of nitrogen fertilizer might also enhance the ozone layer.

Turco, R. P.↗

NASA NTRS1978

Thermal response to ozone fluctuations of the stratosphere

Correlations between stratospheric meteorological parameters and ozone amount are examined in terms of radiation absorption by ozone. Fluctuations of ozone concentration at subtropic latitudes in summer are analyzed on the assumption that local temperature is governed entirely by radiative equilibrium. The analysis suggests that the fluctuations of mean monthly temperature and ozone are not only correlated, but also follow the order-of-magnitude values expected if ozone heating dominates the temperatures. Most direct control of ozone on temperature exists in the lowest parts of the stratosphere.

Stanulonis, S. F.↗

NASA NTRS1978

On the mean meridional mass motions of the stratosphere and mesosphere

Using a simplified, approximate 'Lagrangian-mean' dynamical formulation, the mean meridional mass circulation of the stratosphere and mesosphere is discussed. Under solstice conditions, it is shown that this Lagrangian-mean circulation may be inferred, as a first approximation, from the Eulerian-mean diabatic heating. Diabatic heating rates for the solstices, originally derived by Murgatroyd and Goody (1958), result in Lagrangian-mean rising motion at the tropical tropopause, subsidence across the extra-tropical tropopause, and a very strong summer-to-winter pole flow in the mesosphere. This circulation is exactly that obtained by Murgatroyd and Singleton (1961) for the solstices. Those authors, however, attempted to identify this circulation as the Eulerian-mean motion, and were later criticized for their neglect of the meridional eddy heat flux in the calculation, which proved to be extremely important in the winter hemisphere. The present study, nevertheless, indicates that Murgatroyd and Singleton's circulation may in fact be representative of actual air parcel motions in the stratosphere and mesosphere.

Dunkerton, T.↗

NASA NTRS1978

Stratospheric trace gas sampling with chemical absorption filters

Recent interest in stratospheric chemistry, sparked in part by the suggested roles of atomic chlorine (Cl) and nitrogen oxides (NOx) in the catalytic destruction of ozone (O3), has made sampling and measurement of trace constituents above the tropopause highly desirable. An ongoing research program in the In Situ Studies Project at the National Center for Atmospheric Research carries out aircraft and balloon-borne stratospheric chemical sampling at regular intervals by using chemically impregnated filters to collect particles and reactive gases.

Bonelli, J. E.↗

NASA NTRS1979

Latitudinal variations of stratospheric aerosols

We have obtained stratospheric aerosols from tropical to northern latitudes using special collectors on U-2 aircraft during 1976 and 1977. Aerosols characterized by large numbers of small particles are found in the tropical zone suggesting this is a region of particle growth; whereas aerosols containing mostly larger particles are distributed throughout the Northern Hemisphere indicating a well-mixed, mature population. We find the aerosol layer extends from higher altitudes near the equator to lower ones toward the pole. Although this gradient suggests mature aerosols may leave the stratosphere at high latitudes, the data are, as yet, inconclusive. Comparisons of our data with those of other investigators using different instruments are generally encouraging, suggesting that if similar populations were sampled, the results would be similar. When our calculated sulfate mass mixing ratios are compared with those measured directly by others, we find better agreement is achieved if we assume more dilute sulfate and water mixtures than previously proposed.

Farlow, N. H.↗

NASA NTRS1979

Inversion of stratospheric aerosol and gaseous constituents from spacecraft solar extinction data in the 0.38-1.0-micron wavelength region

The paper discusses a possible data retrieval technique for the spaceborne Stratospheric Aerosol and Gas Experiment (SAGE). The SAGE instrument has four radiometric channels located at selected intervals in the 0.38-1.0-micron wavelength range. A data reduction procedure is described for minimization of experimental errors on the basis of a detailed simulation of the measurement sequence. An efficient and accurate inversion method is then used for the retrieval of all the constituent vertical profiles. Also, the effects of horizontally inhomogeneous distributions of the constituent vertical profiles are studied based on available data of their global distributions. A simple horizontally inhomogeneous model of stratospheric aerosol and ozone is employed to estimate the perturbation on the retrieval accuracies.

Chu, W. P.↗

NASA NTRS1979

Large-scale motion in the Venus stratosphere

To examine a postulate that the horizontal momentum exchanges in the Venusian stratosphere are quasi-nondivergent, the properties of two-dimensional turbulence on a slowly rotating sphere in a high-resolution, one-level numerical model are investigated. It is concluded that the forcing which maintains the stratospheric flow is weak and influences the dynamics far less than the inertial effects. Consequently, the behavior resembles that of vorticity-conserving, two-dimensional flows. On a slowly rotating planet like Venus, such flows are dominated by solid-body rotation and by a planetary wave of unit zonal wavenumber - this wave corresponds to the observed Y-shaped UV feature. Although these largest scales of motion stand out, the dynamic balances of the flow are fundamentally nonlinear, in contrast to the quasi-linear Rossby wave regime on rapidly rotating planets.

Rossow, W. B.↗

NASA NTRS1979

A one-dimensional model describing aerosol formation and evolution in the stratosphere. I - Physical processes and mathematical analogs. II - Sensitivity studies and comparison with observations

A new time-dependent one-dimensional model of the stratospheric sulfate aerosol layer is developed. The model treats atmospheric photochemistry and aerosol physics in detail and includes the interaction between gases and particles explicitly. It is shown that the numerical algorithms used in the model are quite precise. Sensitivity studies and comparison with observations are made. The simulated aerosol physics generates a particle layer with most of the observed properties. The sensitivity of the calculated properties to changes in a large number of aeronomic aerosol parameters is discussed in some detail. The sensitivity analysis reveals areas where the aerosol model is most uncertain. New observations are suggested that might help resolve important questions about the origin of the stratospheric aerosol layer.

Turco, R. P.↗

NASA NTRS1979

Predissociation of nitric oxide in the mesosphere and stratosphere

Absorption of solar photons by nitric oxide in the wavelength ranges 181.3-183.5 and 189.4-191.6 nm leads to predissociation of the molecule in the mesosphere and upper stratosphere. Molecular oxygen controls the penetration of the required solar irradiance via absorption in the Schumann-Runge bands, while attenuation due to ozone becomes significant in the upper stratosphere. The calculation of the nitric oxide dissociation rate is complicated by the need to include all rotational fine structure in both the NO and O2 cross sections. The dissociation rate computed here for the upper mesosphere is a factor of 3.6 less than that reported in past work when currently accepted values of the oscillator strengths and solar irradiance are used. In addition, improved molecular parameters describing the O2 cross section predict less attenuation of the dissociation rate with decreasing altitude than results previously available.

Frederick, J. E.↗

NASA NTRS1979

Spatial-frequency response of the Limb Infrared Monitor of the Stratosphere /LIMS/ radiometer

The Limb Infrared Monitor of the Stratosphere (LIMS), an experiment on the Nimbus-7 satellite, is designed to scan the earth's limb vertically and measure spectral emission profiles of trace atmospheric gases believed to be important in processes controlling the stratospheric ozone distribution. Experiment objectives are reviewed and several analyses and measurements are described which were performed to determine the adequacy of the system for satisfying these objectives. Adequate spatial-frequency response for all the spectral channels is required to provide, through inversion of the measured limb-radiance profiles, important information about the temperature, structure, and composition of the atmosphere. From the LIMS design-model data, the MTF was calculated for the optical system, the detector field mask, the electronics, and the overall system, for each channel. The signal output performance of the instrument was predicted from the system MTF data model input radiance data for each channel. MTF measurements made on the flight sensor confirmed the analytical results. The predictions indicate that the instrument can satisfy the basic measurement objectives of the experiment.

Wilson, R. G.↗

NASA NTRS1979

Perturbation of the zonal radiation balance by a stratospheric aerosol layer

The effect of stratospheric aerosols on the earth's monthly zonal radiation balance is investigated using a model layer consisting of 75% H2SO4, the primary constituent of the background aerosol layer. The reduction in solar energy absorbed by the earth-atmosphere system is determined through the albedo sensitivity, and the optically thin approximation is used in conjunction with the Henyey-Greenstein phase function for scattering. An infrared radiative transfer model is used to estimate the increased greenhouse effect from the aerosol layer, and the infrared heating compensates for the albedo effect in altering the radiation balance. The results indicate that the dominant influence of the thin model stratospheric aerosol layer is an increased reflection of solar energy all over the globe except for the polar-winter region, but the change in the radiation balance is uniform and small equatorward of 50 deg.

Harshvardhan, MR.↗

NASA NTRS1979

Satellite studies of the stratospheric aerosol

The potential climatological and environmental importance of the stratospheric aerosol layer has prompted interest in measuring the properties of this aerosol. This paper reports on two recently deployed NASA satellite systems (SAM II and SAGE) that are monitoring the stratospheric aerosol. The satellite orbits obtain nearly global coverage. The instruments mounted in the spacecraft are sun photometers that measure solar intensity at specific wavelengths as it is moderated by atmospheric particulates and gases during each sunrise and sunset encountered by the satellites. Latitudinal, longitudinal, and temporal variations in the aerosol layer are evaluated. The satellite systems are being validated by a series of ground truth experiments using airborne and ground lidar, balloon-borne dustsondes, aircraft-mounted impactors, and other correlative sensors. The SAM II and SAGE satellite systems, instrument characteristics, and mode of operation are described; the methodology of the experiments is outlined; and the ground truth experiments are discussed. Preliminary results from these measurements are presented.

Mccormick, M. P.↗