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At least 1,117 records · Page 62
All sourcesNASA NTRSDOE OSTI
NASA NTRS2023

Observations Suggest That North African Dust Absorbs Less Solar Radiation Than Models Estimate

Desert dust accounts for a large fraction of shortwave radiation absorbed by aerosols, which adds to the climate warming produced by greenhouse gases. However, it remains uncertain exactly how much shortwave radiation dust absorbs. Here, we leverage in-situ measurements of dust single-scattering albedo to constrain absorption at mid-visible wavelength by North African dust, which accounts for approximately half of the global dust. We find that climate and chemical transport models overestimate North African dust absorption aerosol optical depth (AAOD) by up to a factor of two. This occurs primarily because models overestimate the dust imaginary refractive index, the effect of which is partially masked by an underestimation of large dust particles. Similar factors might contribute to an overestimation of AAOD retrieved by the Aerosol Robotic Network, which is commonly used to evaluate climate and chemical transport models. The overestimation of dust absorption by models could lead to substantial biases in simulated dust impacts on the Earth system, including warm biases in dust radiative effects.

Atmospheric science↗
DOE OSTI2024

Burning conditions and transportation pathways determine biomass-burning aerosol properties in the Ascension Island marine boundary layer

African biomass-burning aerosol (BBA) in the southeast Atlantic Ocean (SEA) marine boundary layer (MBL) is an important contributor to Earth’s radiation budget yet its representation remains poorly constrained in regional and global climate models. Data from the Layered Atlantic Smoke Interactions with Clouds (LASIC) field campaign on Ascension Island (-7.95° N, -14.36° E) detail how fire source regions (burning conditions and fuel type), transport pathways, and longer-term chemical processing affect the chemical, microphysical, and optical properties of the BBA in the remote MBL between June and September of 2017. Ten individual plume events characterize the seasonal evolution of BBA characteristics. Inefficient burning conditions, determined by the mass ratio of refractory black carbon to above-background carbon monoxide (rBC:ΔCO), enhance organic- and sulfate-rich aerosol concentrations in June–July. In contrast, the heart of the burning season exhibited higher rBC:ΔCO values indicative of efficient burning conditions, correlating with more rBC-enriched BBA. Toward the end of the burning season, a mix of burning conditions results in increased variation of the BBA properties. The BBA transit to Ascension Island was predominantly through slow-moving pathways in the MBL and lower free troposphere (FT), facilitating prolonged chemical transformations through heterogeneous and aqueous phase processes. Heterogeneous oxidation can persist for up to 10 days, resulting in a considerable decrease in organic aerosol (OA) mass. OA to rBC mass ratios (OA:rBC) in the MBL between 2 and 5 contrast to higher values of 5 to 15 observed in the nearby FT. Conversely, early-season aqueous-phase processes primarily contributed to aerosol oxidation and some aerosol production, but not appreciable aerosol removal. These two chemical processes yield more light-absorbing BBA in the MBL than in the FT and explain the notably low scattering albedo at 530 nm (SSA 530 ) values (< 0.80) at Ascension Island. This study establishes a robust correlation between SSA 530 and OA:rBC across both MBL and FT, underscoring the dependency of optical properties on chemical composition. These findings highlight how the interplay between chemical composition and atmospheric processing can be improved in global and regional climate models. Questions remain on the mixing of aerosols with different pathway histories, and on what accounts for the doubling of the mass absorption coefficient in the boundary layer.

54 ENVIRONMENTAL SCIENCES↗
NASA NTRS2022

Analysis of the MODIS Above-Cloud Aerosol Retrieval Algorithm Using MCARS

The Multi-sensor Cloud and Aerosol Retrieval Simulator (MCARS) presently produces synthetic radiance data from Goddard Earth Observing System version 5 (GEOS-5) model output as if the Moderate Resolution Imaging Spectroradiometer (MODIS) was viewing a combination of atmospheric column inclusive of clouds, aerosols and a variety of gases and land/ocean surface at a specific location. In this paper we use MCARS to study the MODIS Above-Cloud AEROsol retrieval algorithm (MOD06ACAERO). MOD06ACAERO is presently a regional research algorithm able to retrieve aerosol optical thickness over clouds, in particular absorbing biomass burning aerosols overlying marine boundary layer clouds in the Southeastern Atlantic Ocean. The algorithm’s ability to provide aerosol information in cloudy conditions makes it a valuable source of information for modeling and climate studies n an area where current clear sky-only operational MODIS aerosol retrievals effectively have a data gap between the months of June and October. We use MCARS for a verification and closure study of the MOD06ACAERO algorithm. The purpose of this study is to develop a set of constraints a model developer might use during assimilation of MOD06ACAERO data. Our simulations indicate that the MOD06ACAERO algorithm performs well for marine boundary layer clouds in the SE Atlantic provided some specific screening rules are observed. For the present study, a combination of five simulated MODIS data granules was used for a dataset of 13.5 million samples with known input conditions. When pixel retrieval uncertainty was less than 30%, optical thickness of the underlying cloud layer was greater than 4 and scattering angle range within the cloud bow was excluded, MOD06ACAERO retrievals agreed with the underlying ground truth (GEOS-5 cloud and aerosol profiles used to generate the synthetic radiances) with a slope of 0.913, offset of 0.06, and RMSE=0.107. When only near-nadir pixels were considered (view zenith angle within +/-20 degrees) the agreement with source data further improved (0.977, 0.051 and 0.096 respectively). Algorithm closure was examined using a single case out of the five 38 used for verification. For closure, the MOD06ACAERO code was modified to use GEOS-5 temperature and moisture profiles as ancillary. Agreement of MOD06ACAERO retrievals with source data for the closure study had a slope of 0.996 with offset -0.007 and RMSE of 0.097 at pixel uncertainty level of less than 40%, illustrating the benefits of high-quality ancillary atmospheric data for such retrievals.

MODIS↗
NASA NTRS2001

Assessment of the Contribution of the Atmosphere to Uncertainties in Normalized Water-Leaving Radiance: A Combined Modeling and Data Analysis Approach

Our research for the Sensor Intercomparison and Merger for Biological and Interdisciplinary Oceanic Studies (SIMBIOS) program has been focused on modeling and simulation studies as well as the development of atmospheric correction algorithms. Based on our original proposal and discussions at the SIMBIOS team meetings and workshops, the objectives of our research can be summarized as follows: (1) Use our radiative transfer model for the coupled atmosphere-ocean system to simulate the radiation field at arbitrary levels and in any desired direction in the atmosphere and ocean so as to provide a firm connection between the signal received by the satellite sensor and by a sensor looking down into the water column just above the surface and just below it; (2) Use the simulations to quantify the influence of atmospheric aerosols on the water-leaving radiance, and to quantify the error in the water-leaving radiance as a function of uncertainties in the aerosol optical properties, mass loading and vertical extent; (3) Use the model simulations in conjunction with validation measurements taken by other SIMBIOS investigators (for satellite overpasses) to assess our understanding of the radiative transfer process in the coupled atmosphere-ocean column, and to examine the extent to which the model provides a realistic prediction of simultaneously measured in situ water-leaving radiance and the radiance received by the satellite sensor; (4) Modify and improve an existing atmospheric correction algorithm, based on the work above, as needed by constructing new look-up tables that include scattering by ocean particles; and (5) Carry out approaches to developing an atmospheric correction algorithm for ocean color imagery with strongly absorbing aerosols.

Stamnes, Knut↗
NASA NTRS1975

Instrumentation for measurements of solar irradiance and atmospheric optical properties

The Active Cavity Radiometer (ACR), an accurate absolute pyrheliometer, has been developed for measurements of total solar irradiance. It has been used to discover a -2.2% error in the International Pyrheliometric Scale and to make measurements in balloon flight experiments yielding a solar constant value of 136.6 (+ or - 0.7) mW/sq cm. New ACRs are being developed to monitor the total output of solar optical radiation in balloon, satellite and space shuttle experiments with long-term absolute uncertainty of + or - 0.1% or less. In a separate program, instrumentation for the measurement of the scattering and extinction of solar radiation by the atmosphere is being constructed to provide data for modeling atmospheric aerosol content. The aerosol models will facilitate computation of radiative transfer effects yielding quantitative net fluxes useful in evaluating the climatological impact of aerosols.

Willson, R. C.↗
NASA NTRS2000

What we Hope to Learn about Global Mineral Dust Aerosols from EOS Multi-Angle Imaging SpectroRadiometer (MISR)

On global scales, just a few broad atmospheric aerosol compositional groups are commonly observed. Of these, "mineral dust" is the only group which both contains non-spherical particles, and typically has size distributions with enough large particles for particle shape to affect its visible-light-scattering properties. The MISR instrument is scheduled for launch into a 10:30 AM sun-synchronous, polar orbit aboard the EOS Terra satellite in 1999. MISR will measure the upwelling visible radiance from Earth in 4 spectral bands centered at 446, 558, 672, and 866 nm, at each of 9 emission angles spread out in the forward and aft directions along the flight path at +/-70.5 deg, +/-60.0 deg, +/-45.6 deg, +/-26.1deg, and nadir. Over a period of 7 minutes, as the spacecraft flies along, a 360 km wide swath of Earth will successively be viewed by each of the cameras, allowing MISR to sample a very large range of scattering angles; in mid latitudes, the instrument will observe scattering angles between about 60 deg and 160 deg. Global coverage will be acquired about once in 9 days at the equator; the nominal mission lifetime is 6 years. The distinction in single scattering phase function between natural distributions of spherical and randomly oriented, non-spherical particles, with a broad range of aspect ratios, shows up strongly for scattering angles ranging from about 90 deg to near 180 deg. For non-spherical particle distributions, single scattering phase functions tend to be much flatter in this region than for spherical particles. Since MISR samples the relevant range of scattering angles very well, we expect to be able to make critical distinctions between natural distributions of spherical and randomly oriented, non-spherical particles with MISR data. We anticipate that the new multiangle, multispectral data from MISR will also contain other information about particle properties, a major step beyond current spacecraft remote sensing retrievals, which obtain aerosol optical depth based on entirely assumed particle microphysical properties. According to simulations over cloud-free, calm ocean, for pure particles with natural ranges of optical depth, particle size, and indices of refraction, MISR should retrieve column optical depth for all but the darkest particles, to an uncertainty of at most 0.05 or 20%, whichever is larger, even if the particle properties are poorly known. For one common particle type, soot, constraints on the optical depth over dark ocean are very poor. The simulated measurements also should allow us to separate two to four compositional groups based on indices of refraction, and to identify three to four distinct size groups between 0.1 and 2.0 microns characteristic radius at most latitudes. The technique is most sensitive to particle microphysical properties in the "accumulation mode" sizes. where particle scattering undergoes the transition from Rayleigh to large-particle regimes for the MISR wavelengths. Based on these results, we expect to distinguish air masses containing different aerosol types, routinely and globally, with multiangle remote sensing data. Such data complements in situ and field data, which can provide details about aerosol size and composition locally that are needed to assess the radiative effects of aerosols quantitatively. Both field data and correlations in space and time with likely source and sink regions will also be helpful in developing a global picture of mineral dust aerosol budgets. Further work on the expected sensitivity of MISR to natural mixtures of pure particles, including climatologically likely mineral dust components, is currently underway.

Kahn, Ralph↗
NASA NTRS1992

Multi-wavelength Airborne Lidar Intercomparisons of Aerosol and Cirrus Backscatter over the Pacific Ocean

Airborne CO2 and Nd:YAG lidar instruments were flown on the NASA DC-8 research aircraft during two extended missions over the Pacific. The objectives during these flights were to characterize aerosol backscatter levels at infrared wavelengths in relatively pristine regions of the troposphere, and to observe cloud effects on lidar signals. In addition, the three wavelength Nd:YAG data were processed using independent temperature profile information, in order to deduce the Rayleigh scattering component of the total backscatter at each wavelength. The data can be used to better understand the capabilities of various airborne or Earth-orbiting lidar designs to provide backscatter information from aerosols and clouds, or to provide Doppler or DIAL information from aerosol and cloud backscatter.

Menzies, Robert T.↗
NASA NTRSDate not supplied

Multi-angle Imaging SpectroRadiometer

MISR views the sunlit Earth simultaneously at nine widely spaced angles and provides ongoing global coverage with high spatial detail. Its imagery is carefully calibrated to provide accurate measures of the brightness, contrast, and color of reflected sunlight. MISR provides new types of information for scientists studying Earth's climate, such as the regional and global distribution of different types of atmospheric particles and aerosols. The change in reflection at different view angles provides the means to distinguish aerosol types, cloud forms, and land surface cover. Combined with stereoscopic techniques, this enables construction of 3-D cloud models and estimation of the total amount of sunlight reflected by Earth's diverse environments. MISR was built for NASA by the Jet Propulsion Laboratory (JPL) in Pasadena, California. It is part of NASA's first Earth Observing System (EOS) spacecraft, the Terra spacecraft, which was launched into polar orbit from Vandenberg Air Force Base on December 18, 1999. MISR has been continuously providing data since February 24, 2000. [Mission Objectives] The MISR instrument acquires systematic multi-angle measurements for global monitoring of top-of-atmosphere and surface albedos and for measuring the shortwave radiative properties of aerosols, clouds, and surface scenes in order to characterize their impact on the Earth's climate. The Earth's climate is constantly changing -- as a consequence of both natural processes and human activities. Scientists care a great deal about even small changes in Earth's climate, since they can affect our comfort and well-being, and possibly our survival. A few years of below-average rainfall, an unusually cold winter, or a change in emissions from a coal-burning power plant, can influence the quality of life of people, plants, and animals in the region involved. The goal of NASA's Earth Observing System (EOS) is to increase our understanding of the climate changes that are occurring on our planet, and the reasons for these changes, so we are better equipped to anticipate and prepare for the future. The MISR instrument is a part of EOS. Its role is to measure the amount of sunlight scattered in different directions under natural conditions. These measurements will help quantify the amount of solar energy that heats the Earth's surface and atmosphere, and the changes that occur in them over the lifetime of the MISR instrument. From the MISR observations, we are also learning more about those components of the Earth's environment that scatter sunlight: particles in the atmosphere, the planet's surface, and clouds. MISR monitors changes in surface reflection properties, in atmospheric aerosol content and composition, and in cloudiness. Scientists use these data to study land use changes, air pollution, volcanic eruptions, as well as processes such as desertification, deforestation, and soil erosion. As part of the EOS program, computer models that predict future climate will be improved by the results of these studies. [Temporal_Coverage: Start_Date=2000-02-24; Stop_Date=] [Spatial_Coverage: Southernmost_Latitude=-90; Northernmost_Latitude=90; Westernmost_Longitude=-180; Easternmost_Longitude=180].

Diner, David J.↗
DOE OSTI2022

Pan-Arctic seasonal cycles and long-term trends of aerosol properties from 10 observatories

Even though the Arctic is remote, aerosol properties observed there are strongly influenced by anthropogenic emissions from outside the Arctic. This is particularly true for the so-called Arctic haze season (January through April). In summer (June through September), when atmospheric transport patterns change, and precipitation is more frequent, local Arctic sources, i.e., natural sources of aerosols and precursors, play an important role. Over the last few decades, significant reductions in anthropogenic emissions have taken place. At the same time a large body of literature shows evidence that the Arctic is undergoing fundamental environmental changes due to climate forcing, leading to enhanced emissions by natural processes that may impact aerosol properties. In this study, we analyze 9 aerosol chemical species and 4 particle optical properties from 10 Arctic observatories (Alert, Kevo, Pallas, Summit, Thule, Tiksi, Barrow/Utgiavik, Villum, and Gruvebadet and Zeppelin Observatory – both at Ny-Ålesund Research Station) to understand changes in anthropogenic and natural aerosol contributions. Variables include equivalent black carbon, particulate sulfate, nitrate, ammonium, methanesulfonic acid, sodium, iron, calcium and potassium, as well as scattering and absorption coefficients, single scattering albedo and scattering Ångström exponent. First, annual cycles are investigated, which despite anthropogenic emission reductions still show the Arctic haze phenomenon. Second, long-term trends are studied using the Mann–Kendall Theil–Sen slope method. We find in total 41 significant trends over full station records, i.e., spanning more than a decade, compared to 26 significant decadal trends. The majority of significantly declining trends is from anthropogenic tracers and occurred during the haze period, driven by emission changes between 1990 and 2000. For the summer period, no uniform picture of trends has emerged. Twenty-six percent of trends, i.e., 19 out of 73, are significant, and of those 5 are positive and 14 are negative. Negative trends include not only anthropogenic tracers such as equivalent black carbon at Kevo, but also natural indicators such as methanesulfonic acid and non-sea-salt calcium at Alert. Positive trends are observed for sulfate at Gruvebadet. No clear evidence of a significant change in the natural aerosol contribution can be observed yet. However, testing the sensitivity of the Mann–Kendall Theil–Sen method, we find that monotonic changes of around 5 % yr –1 in an aerosol property are needed to detect a significant trend within one decade. This highlights that long-term efforts well beyond a decade are needed to capture smaller changes. It is particularly important to understand the ongoing natural changes in the Arctic, where interannual variability can be high, such as with forest fire emissions and their influence on the aerosol population. To investigate the climate-change-induced influence on the aerosol population and the resulting climate feedback, long-term observations of tracers more specific to natural sources are needed, as well as of particle microphysical properties such as size distributions, which can be used to identify changes in particle populations which are not well captured by mass-oriented methods such as bulk chemical composition.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2025

Explosive Soot Challenge (Final Report)

This project assembled a broad ensemble of modeling and experimentation tools to study the morphological and optical properties of detonation soots in explosive fireballs. A gram-scale hemispherical high explosive was studied in a low-pressure controlled environment using in-situ experimentation with diffusely illuminated visible absorption spectroscopy, particle sizing through light scattering techniques, and post-test collections with subsequent morphological analysis. Hydrocode modeling was performed to replicate the detonation flow observations, and subsequent aerosol kinetics models provided particle size distributions and extinction coefficients from the hydrocode results. Experimentally observed soot morphologies agreed with expectation from the literature - a bimodal distribution was found, brought upon by the particles growing to a size where their inertia and fluid wakes are non-negligible. The aerosol kinetics model did not replicate the observed bimodal size distribution for lack of a coagulation kernel to represent the behavior. To recover particulate optical properties, a spectrally resolved absorption spectroscopy method termed Spectral diffuse back-illuminated extinction imaging (SBI-EI) was developed and implemented on two explosive types. Inverting the absorption spectra using a Kramers-Kronig consistent method yielded the complex index of refraction for the soots produced by the explosives. This method resulted in an unrealistic index of refraction for one of the two explosives, and this is suspected to be due to the model neglecting scattering brought upon by the large particle sizes observed. In addition to the core work, three additional studies were performed in parallel. These investigated the impact of scattering on diffuse absorption spectroscopy, studied how soots oxidate and sublimate in a well-controlled shock tube, and laid the theoretical groundwork for a new collision kernel to replicate the bimodal size distribution from the observations. Summaries of these efforts are included at the end of this report.

45 MILITARY TECHNOLOGY, WEAPONRY, AND NATIONAL DEF↗
NASA NTRS1978

Determination of aerosol content in the atmosphere from LANDSAT data

The author has identified the following significant results. A large set of LANDSAT 2 data, obtained at San Diego, showed excellent linear relationships, particularly for MSS 5 and MSS 6, between the radiance over the ocean and the atmospheric aerosol content. Two other data points obtained at Adrigole, Ireland, representing a different ocean and a different ground truth instrument, showed very good agreement with the San Diego data. It appeared that the technique could be used for global monitoring of the atmospheric aerosol content over the oceans. Results obtained at several inland bodies of water showed that MSS 4, MSS 5, and MSS 6 cannot be used due to the effect of water pollution generally present. However, the LANDSAT 1 results suggested that MSS 7, which operates at longer wavelengths, was not very sensitive to water pollution, and might be useful for inland measurements of aerosol content. Use of the longer wavelength would also minimize the effects of adjacent high albedo land, since atmospheric scattering was reduced at longer wavelengths.

Griggs, M.↗
NASA NTRS1986

Laser remote sensing of the atmosphere

A guide to the extant literature concerning remote sensing of the atmosphere by laser-based devices is presented, with emphasis on surveys of the field as well as the most important recent results. Topics surveyed include measurements of aerosol constituents using lidar, the differential absorption lidar technique, the use of laser long-path differential absorption, Raman scattering techniques, and fluorescence lidar techniques. Special attention is given to measuring wind velocity using CO2 heterodyne lidar systems.

Grant, William B.↗
NASA NTRS1988

A continued program of planetary study

This program conducts solar system research in support of NASA missions and of general astronomical interest. Investigations of the composition, physical characteristics, and changes in solar system bodies are conducted primarily utilizing facilities of McDonald Observatory, but also utilizing various space vehicles where appropriate. The first detection of 2 micrometer II2 emission from Jupiter's southern auroral zone was made. Previous detection of northern auroral emission from Jupiter's H2 S(1) quadrupole line at 2.12 micrometer was confirmed. Unlike the previously known 8 micrometer aurorae, this phenomenon can not be thermal in origin. Analysis of Raman scattering in the blue and ultraviolet spectrum of Uranus (200 to 500 Angstroms) show that there must be absorbing aerosol particles in the upper 10 mbar region of the atmosphere. Spectra of Pluto-Charon in and out of eclipse in the red and near IR were obtained. These data confirm that CH4 is confined to Pluto and absent on Charon.

Smith, Harlan↗
NASA NTRS1993

Comparisons of downwelling radiation to model predictions based on groundbased measurements during FIRE 1991

Surface radiation measurements and simultaneous ground-based measurements of the atmosphere during the FIRE'91 cirrus field experiment provided an opportunity to identify crucial measurements and parameterization deficiencies in current cloud-radiation models. Comparisons between measured and calculated broadband surface fluxes with only a small data subset already reveal these needs: accurate humidity and aerosol vertical profiles for clear cases, accurate vertical extinction profiles and dimensions for clouds, and understanding of the (solar) scattering properties of cirrus.

Kinne, S.↗
NASA NTRS1997

Absorption and scattering properties of the Martian dust in the solar wavelengths

A new wavelength-dependent model of the single-scattering properties of the Martian dust is presented. The model encompasses the solar wavelengths (0.3 to 4.3 micrometers at 0.02 micrometer resolution) and does not assume a particular mineralogical composition of the particles. We use the particle size distribution, shape, and single-scattering properties at Viking Lander wavelengths presented by Pollack et al. [1995]. We expand the wavelength range of the aerosol model by assuming that the atmospheric dust complex index of refraction is the same as that of dust particles in the bright surface geologic units. The new wavelength-dependent model is compared to observations taken by the Viking Orbiter Infrared Thermal Mapper solar channel instrument during two dust storms. The model accurately matches afternoon observations and some morning observations. Some of the early morning observations are much brighter than the model results. The increased reflectance can be ascribed to the formation of a water ice shell around the dust particles, thus creating the water ice clouds which Colburn et al. [1989], among others, have predicted.

Atmosphere/analysis↗
NASA NTRS2011

EPIC Radiance Simulator for Deep Space Climate ObserVatoRy (DSCOVR)

The Deep Space Climate ObserVatoRy (DSCOVR) is a planned space weather mission for the Sun and Earth observations from the Lagrangian L1 point. Onboard of DSCOVR is a multispectral imager EPIC designed for unique observations of the full illuminated disk of the Earth with high temporal and 10 km spatial resolution. Depending on latitude, EPIC will observe the same Earth surface area during the course of the day in a wide range of solar and view zenith angles in the backscattering view geometry with the scattering angle of 164-172 . To understand the information content of EPIC data for analysis of the Earth clouds, aerosols and surface properties, an EPIC radiance Simulator was developed covering the UV -VIS-NIR range including the oxygen A and B-bands (A=340, 388, 443, 555, 680, 779.5, 687.7, 763.3 nm). The Simulator uses ancillary data (surface pressure/height, NCEP wind speed) as well as MODIS-based geophysical fields such as spectral surface bidirectional reflectance, column water vapor, and properties of aerosols and clouds including optical depth, effective radius, phase and cloud top height. The original simulations are conducted at 1 km resolution using the look-up table approach and then are averaged to 10 km EPIC radiances. This talk will give an overview of the EPIC Simulator with analysis of results over the continental USA and northern Atlantic.

Lyapustin, Alexei↗
NASA NTRS2021

Observation of absorbing aerosols above clouds over the South-East Atlantic Ocean from the geostationary satellite SEVIRI - Part 2: Comparison with MODIS and aircraft measurements from the CLARIFY-2017 field campaign

To evaluate the SEVIRI retrieval for aerosols above clouds presented in Part 1 of the companion paper, the algorithm is applied over the south-east Atlantic Ocean during the CLARIFY-2017 field campaign period. The first step of our analysis compares the retrieved aerosol and cloud properties against equivalent products from the MODIS MOD06ACAERO retrieval (Meyer et al., 2015). While the correlation between the two satellite retrievals of the above-cloud aerosol optical thickness (AOT) is good (R = 0.78), the AOT retrieved by SEVIRI is 20.3 % smaller than that obtained from the MODIS retrieval. This difference in AOT is attributed mainly to the more absorbing aerosol model assumed for the SEVIRI retrieval compared to MODIS. The underlying cloud optical thickness (COT) derived from the two satellites is in good agreement (R = 0.90). The cloud droplet effective radius (CER) retrieved by SEVIRI is consistently smaller than MODIS by 2.2 µm, which is mainly caused by the use of different spectral bands of the satellite instruments. In the second part of our analysis, we compare the forecast water vapour profiles used for the SEVIRI atmospheric correction as well as the aforementioned aerosol and cloud products with in situ measurements made from the Facility for Airborne Atmospheric Measurements (FAAM) aircraft platform during the CLARIFY-2017 campaign. Around Ascension Island, the column water vapour used to correct the SEVIRI signal is overestimated by 3.1 mm in the forecast compared to that measured by dropsondes. However, the evidence suggests that the accuracy of the atmospheric correction improves closer to the African coast. Consistency is observed between the SEVIRI above-cloud AOT and in situ measurements (from cavity ring-down spectroscopy instruments) when the measured single-scattering albedo is close to that assumed in the retrieval algorithm. On the other hand, the satellite retrieval overestimates the AOT when the assumed aerosol model is not absorbing enough. Consistency is also found between the cloud properties retrieved by SEVIRI and the CER measured by a cloud droplet probe and the liquid water path derived from a microwave radiometer. Despite the instrumental limitations of the geostationary satellite, the consistency obtained between SEVIRI, MODIS and the aircraft measurements demonstrates the ability of the retrieval in providing additional information on the temporal evolution of the aerosol properties above clouds.

absorbing aerosols↗
NASA NTRS2010

MISR Global Aerosol Product Assessment by Comparison with AERONET

A statistical approach is used to assess the quality of the MISR Version 22 (V22) aerosol products. Aerosol Optical Depth (AOD) retrieval results are improved relative to the early post- launch values reported by Kahn et al. [2005a], varying with particle type category. Overall, about 70% to 75% of MISR AOD retrievals fall within 0.05 or 20% AOD of the paired validation data, and about 50% to 55% are within 0.03 or 10% AOD, except at sites where dust, or mixed dust and smoke, are commonly found. Retrieved particle microphysical properties amount to categorical values, such as three groupings in size: "small," "medium," and "large." For particle size, ground-based AERONET sun photometer Angstrom Exponents are used to assess statistically the corresponding MISR values, which are interpreted in terms of retrieved size categories. Coincident Single-Scattering Albedo (SSA) and fraction AOD spherical data are too limited for statistical validation. V22 distinguishes two or three size bins, depending on aerosol type, and about two bins in SSA (absorbing vs. non-absorbing), as well as spherical vs. non-spherical particles, under good retrieval conditions. Particle type sensitivity varies considerably with conditions, and is diminished for mid-visible AOD below about 0.15 or 0.2. Based on these results, specific algorithm upgrades are proposed, and are being investigated by the MISR team for possible implementation in future versions of the product.

Kahn, Ralph A.↗