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NCERC Capabilities

National Criticality Experiments Research Center (NCERC), located at the Nevada Nuclear Security Site (NNSS) operated by Los Alamos National Laboratory, is our nation’s only general-purpose critical experiments facility and is one of only a few that remain operational throughout the world. NCERC Directly Contributes to Important National and International Missions and is Making Investments in Pipeline and the Facility for enduring capability and expanding missions. More detailed capabilities are described.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Characterizing novel Indium Phosphide pad detectors with focused X-ray beams and laboratory tests

Future tracking systems in High Energy Physics experiments will require large instrumented areas with low radiation length. Crystalline silicon sensors have been used in tracking systems for decades, but are difficult to manufacture and costly to produce for large areas. We are exploring alternative sensor materials that are amenable to fast fabrication techniques used for thin film devices. Indium Phosphide pad sensors were fabricated at Argonne National Lab using commercially available InP:Fe 2-inch mono-crystal substrates. Current-voltage and capacitance-voltage characterizations were performed to study the basic operating characteristics of a group of sensors. Micro-focused X-ray beams at Canadian Light Source and Diamond Light Source were used to study the response to ionizing radiation, and characterize the uniformity of the response for several devices. Electrical test results showed a high degree of performance uniformity between the 48 tested devices. X-ray test beam results showed good performance uniformity within tested devices after accounting for spatially-local defects and edge fields. As a result, this motivates further studies into thin film devices for future tracking detectors.

47 OTHER INSTRUMENTATION↗

LBNL-BELLA Center Monoenergetic Photon Source Experiments

This document outlines measurements made by Idaho National Laboratory (INL) staff at the Berkeley Lab Laser Accelerator (BELLA) Center. Measurements of a mono-energetic Thomson photon beam were made with various INL instruments. The photon beam was generated by a laser-plasma accelerator system. This project is referred to by the name Laser Wake. Key Lawrence Berkeley National Laboratory (LBNL) personnel involved include Liona Fan-Chiang, Cameron Geddes, Anthony Gonsalves, Robert Jacob, Tobias Ostermayr, and Hai-En Tsai.

46 - INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AN↗

Design and analysis of dudded fuel experiments at the National Ignition Facility

Recent experiments conducted at the National Ignition Facility (NIF) within the past 2 years have achieved the burning plasma state and exceeded the Lawson criterion for the first time in the laboratory. Here, we report on a set of experiments where the deuterium and tritium (DT) ice layers were replaced with dudded tritium, hydrogen, and deuterium (THD) fuel mixtures to remove the influence of alpha-heating on hot spot dynamics. The hot spot compression and yield in the absence of alpha particle self-heating were measured to assess the proximity of NIF implosions toward the ignition cliff. We find that the “burn-off” Lawson parameters χnoα inferred from the THD experiments are in good agreement with the inferences from postshot simulations of the DT-layered implosions. The THD for burning plasma shot N210307 yielded χnoα≈0.88±0.03 while the THD for ignition shot N210808 yielded χnoα≈1.04±0.04. These results also provide important context for the observed variability in the repeat attempts of ignition shot N210808 since implosions on the ignition cliff are expected to exhibit very large variations in the fusion yield from small changes in the initial conditions.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Internal Collaboration on Recent Nuclear Criticality Safety Assessments

Prevention of inadvertent criticality at facilities with large quantities of fissionable materials is one of the most important requirements those facilities grapple with. Given that criticality cannot be mitigated, only eliminated, a hard line must be taken on this requirement. The facilities and sites with the possibility of such an event must abide by a plethora of requirements, most stemming from the ANSI/ANS-8 series of consensus standards. One such standard, ANSI/ANS-8.19, Administrative Practices for Nuclear Criticality Safety, gives requirements and recommendations necessary for establishing a nuclear criticality safety program for a given facility or site. One of those requirements includes periodic assessments of the NCS program. To meet the assessment requirement, Los Alamos National Laboratory (LANL) conducts periodic assessments on individual facilities and overall programmatic health aspects. The teams developed to perform these assessments include people both inside and outside the LANL NCS program. Recently, the Nuclear Criticality Safety Division and the Critical Experiments Team of the Advanced Nuclear Technology Group established a collaboration to aid in fulfilling the assessment requirement.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Characterization of ceramic fuel powder packing fractions to support INFLUX

Triply periodic minimal surface (TPMS)-based structures show marked potential in novel nuclear reactor fuel designs, as their high surface area-to-volume ratio increases the efficiency of heat transfer out of the fuel, enabling safer, more innovative reactor designs. This milestone report addresses the role of dUO 2 powder processing route on the fill behavior of TPMS-based cladding shells to understand and advance the feasibility of manufacturing TPMS-based nuclear fuel forms. dUO 2 powder was processed through either a dry granulation route, varying consolidation pressure, or through milling, varying milling time, milling method and milled size distribution. The lowest tapped bulk densities (TBD), but best powder flowabilities, were obtained when testing unprocessed dUO 2 powder which was prone to self-agglomeration and formed low-density spheroids. The highest TBD and lowest flowabilities were obtained when using powder produced by hammer-milling dUO 2 powder to pass through a 200-mesh sieve, which led to particles with angular morphologies. Powder produced by dry granulation exhibited TBD that varied according to the consolidation pressure used to form the initial pellets and exhibited improved flowabilities when compared to hammer-milled material. Because of the large span of granule sizes formed as well as the irregular shape associated with the granules, a packing fraction of 0.69 was achieved, exceeding the analytical solution for random close packing of mono-sized spheres. TPMS polymer shells were loaded with unprocessed, granulated, and hammer-milled dUO 2 powders, and their qualitative packing behaviors were analyzed using x-ray computed tomography (xCT). TBDs calculated after loading TPMS polymer shells were 10-20% lower when compared to tapped bulk density measurements taken in a glass graduated cylinder, indicating a non-trivial impact on the tapped bulk density of either the TPMS channel size, TPMS channel surface material, powder cohesiveness, or a combination of the two parameters. A metallic zircaloy-4 TPMS shell will be loaded with hammer-milled dUO 2 powder upon receipt of the shell from Oak Ridge National Laboratory (ORNL) and shipped to Idaho National Labs (INL) for subsequent hot isostatic pressing (HIP) densification experiments.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Radiochemical capabilities for astrophysics experiments at the national ignition facility

The Nuclear and Radiochemistry Group at Lawrence Livermore National Laboratory (LLNL) has developed a suite of diagnostics and techniques that can be used for astrophysics experiments at the National Ignition Facility (NIF). Capabilities have been developed to add material to the outside of NIF hohlraum assemblies as well as to the interior of NIF target capsules or the fill gas. The ability to place very small amounts of material close to the NIF target enables activation with very large, short-pulse neutron fluxes. The Solid Radiochemistry Diagnostic can be used to collect solid debris from a NIF shot within 2 h of the execution of a shot, and this can be analyzed for radioactive signatures with or without post-shot chemical processing. The Radiochemical Analysis of Gaseous Samples diagnostic system can be used to collect gaseous products produced during a NIF shot. Capsule doping and radiochemical analysis capabilities at NIF will be discussed. The application of these techniques to astrophysical measurements will be discussed as well as some preliminary results.

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗

Cylindricity Sensitivity Thermal Model of the AGR-5/6/7 Experiment in the Advanced Test Reactor

The AGR-5/6/7 experiment is currently being irradiated in the Advanced Test Reactor (ATR) at the Idaho National Laboratory and is approximately 70% complete. Several fuel and material irradiation experiments have been planned for the U.S. Department of Energy Advanced Gas Reactor Fuel Development and Qualification Program, which supports the development and qualification of tristructural isotropic (TRISO) coated particle fuel for use in high-temperature gas-cooled reactors. The goals of these experiments are to provide irradiation performance data to support fuel process development, qualify fuel for normal operating conditions, support development of fuel performance models and codes, and provide irradiated fuel and materials for post-irradiation examination and safety testing. Originally planned and named as separate fuel experiments, but subsequently combined into a single test train, AGR-5/6/7 is testing low-enriched uranium oxycarbide TRISO fuel. The AGR-5/6/7 test train has 5 capsules with thermocouples and independent gas control mixtures. Unique to this paper is a sensitivity study concerning the cylindricity of the graphite holders containing the fuel compacts and their eccentricity in relation to the stainless-steel capsule walls. Each capsule has small nubs on the outside used for centering the graphite holder inside the stainless-steel capsule with a small gas gap used to control temperature. Due to machining tolerances of these nubs and vibration wearing the nubs down when the experiment is running in the reactor, the possibility exists that the holder may move around radially. Each capsule is equipped with several thermocouples placed at various radii and depths within each graphite holder. This paper will show the sensitivity of offsetting the graphite holder for various radii in 45-degree increments around the circle with the objective of minimizing the difference between the measured thermocouples and the modeled thermocouple temperatures. Separate gas mixtures of helium/neon are introduced into this gas gap between the holder and capsule wall and changed as necessary to maintain the desired thermocouple temperatures to keep the fuel compacts at constant temperature as the nuclear reactor conditions change. The goal of the sensitivity study is to find a radius and an angle to offset the holder from perfectly centered for each of the five capsules separately. The complex thermal model includes fission heating, gamma heating, radiation heat transfer, and heat transfer via conduction and radiation across the control gaps. Subroutines linked to the thermal model offer an easy method to offset the graphite holder from the capsule walls without remeshing the entire model.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Simulations of Sweeping Wave Propagation in a Boron Carbide Plate

In February 2020, experiments were conducted at Los Alamos National Laboratory measuring the propagation of a sweeping wave through a plate of boron carbide which was induced by detonating an adjacent charge of high explosive. Six such shots were red and in each case progress of the wave along the exposed surface of the plate was tracked using photon doppler velocimetry (PDV). In this report we discuss calculations performed using the Lagrangian hydrocode FLAG to model data taken from these experiments. We discuss the models chosen for the different experimental components, the choice of mesh (focusing on, both, two- and three-dimensional geometries), and compare the results from these calculations to experimentally-extracted PDV traces. Notably, we find that the PDV traces for this experiment are most faithfully reproduced using the full three-dimensional geometry, even when the mesh resolution for the three-dimensional calculations was significantly lower than the resolution for the corresponding two-dimensional calculations. We attribute this to the geometry of the experimental setup. Moreover, we find only negligible differences for the PDV traces obtained using the sesame table equation of state for boron carbide and the Gruneisen equation of state.

36 MATERIALS SCIENCE↗

Supporting data for "Frozen flume experiments indicate rapid permafrost riverbank erosion depends on bank roughness"

This dataset contains supporting files detailing five frozen flume experiments conducted at the Caltech Earth Surface Dynamics Laboratory to investigate rates of ablation-limited permafrost riverbank erosion under controlled conditions. Water flowed past a bank of saturated, frozen sand and ice and gradually eroded the bank by thawing pore ice and immediately entraining sand and washing it downstream. Experiments were scaled for flow hydraulics and heat transfer allowing comparisons between our results and natural permafrost riverbanks. For each experiment, we measured the initial and final sand bank topography using a Keyence laser scanner, water surface slope at 3-min intervals throughout the experiment using a Massa sonar scanner, bank erosion using 10-sec overhead timelapse imagery taken by an overhead camera, water and bank temperature using thermistors frozen into the sand bank and sampling at 2 Hz, and water discharge using an in-line flow meter. We include calibration data for the carriage (engineered by the Saint Anthony Falls Laboratory) used to make sonar and laser topography measurements. We also include calibration data for temperature sensors, water discharge measurements, and images of a regular grid placed in the flume to align overhead camera images with the carriage datum. Grain size analysis for the channel bed (gravel) was produced using a pebble count and bank sand was measured using a Camsizer X2. In addition to the five frozen experiments, we include sonar scans of water surface slope and Keyence scans of bed and bank topography for calibration experiments ran with an immobile gravel bank and bed.

54 ENVIRONMENTAL SCIENCES↗

AGC Experiment Status

AGC Experiment Status to include: History and status of the AGC-4, Review of the AGC experiment, AGC graphite grades and samples, The AGC-4 capsule and specimens, and HDG-1 and HDG-2. Description of the Experiment, AGC graphite grades and samples, AGC-1 Test Train, AGC-1 Test Train Design Features, New AGC Irradiation Schedule (2018) and update in schedule, Irradiation and disassembly history, present and future status, and shipment and initial PIE. Initial PIE strategy, recovered specimens, PIE results, and status of experiments.

11 - NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

HYBRID Modeling of DETAIL Experimental Facility

Idaho National Laboratory continues to be at the forefront of advanced reactor systems and integrated energy systems research. Through the Thermal Energy Distribution System (TEDS) and Microreactor Agile Non-nuclear Test Bed (MAGNET) experiments in the Dynamic Energy Transport and Innovation Laboratory (DETAIL) within the Engineering Systems Laboratory, a mix of digital and physical testing systems can explore the operation of thermally and electrically integrated systems. Modeling of these systems has been done using the HYBRID modeling repository of the Integrated Energy Systems program. DETAIL also contains high temperature steam electrolysis (HTSE) units to produce hydrogen and generate the load imposed on MAGNET and TEDS. The dynamic modeling capabilities within the IES program describe the DETAIL components as-built and can be used to evaluate controls, process flows, and overall system conditions.

08 HYDROGEN↗

Innovative Nuclear Materials Outboard-A Project Specimen Preparation Guide

The Innovative Nuclear Materials (INM) Program was recently established by the U.S. Department of Energy (DOE) to develop advanced material technologies for use in nuclear reactors. The INM program is presently focused on researching in-core non-fueled materials for application in fast spectrum nuclear reactors. The widespread deployment of fast reactors continues to be a prominent aspiration for advanced nuclear technology developers. However, companies working to license these reactors have no choice but to rely on historic material technologies since further optimization and advancement of these materials is impeded by the lack of fast neutron irradiation test facilities. INM-OA is a non-fueled drop-in experiment which will irradiate material specimens of interest to fast reactor applications. This experiment will be irradiated at Idaho National Laboratory (INL) in the Advanced Test Reactor (ATR) outboard-A (OA) position during normal and high temperature steady state (HTSS) cycles. It will include material specimens supplied by members of the INM program and will utilize a cadmium-lined basket to filter out incident thermal neutrons, thus simulating a faster neutron energy spectrum. Material specimens will undergo post-irradiation examination including microscopy and mechanical testing. In addition to absorption reactions, fast neutrons cause microstructural damage in materials by atom displacement, which can cause exacerbated changes in physical properties and behavior. Thus, the data obtained from the INM-OA experiment will be crucial for understanding the engineering-scale behavior of reactor materials. This document is intended for the Principal Investigators providing samples for this project. Topics included are a general description of the experiment, the irradiation experiment/capsule design, sample geometries, number of samples to be provided, documentation to be provided, a brief list potentially useful characterization methods that can be leveraged at INL, and other miscellaneous requirements specific to this project. This document is intended for informational use only.

innovative nuclear materials↗

Building a Simplistic Automatic Extruder: Instrument Development Opportunities for the Laboratory

This work presents an automatic extruder as a research experience for undergraduate students. The system offers a user-friendly approach to preparing vesicles, such as liposomes or polymersomes, with a defined size and polydispersity properties crucial for research in biology and macromolecules. It comprises two syringe pumps connected by a membrane filter. The setup is controlled by software. Compared to manual extrusion, this automated system provides advantages, such as precisely controlled variables. The project describes a tool to enhance undergraduate learning in science and engineering laboratories. Building an automatic extruder serves as a simplified model of a complex industrial process. It offers a clear advantage: automating a well-understood manual extrusion process. To make this project accessible, it is broken down into three manageable tasks: software development, hardware assembly, and testing procedures. This breakdown describes the software created, the hardware components used, and the testing procedures conducted for this project. All project data, including software code, testing data, and procedures, are freely available online. This allows undergraduate students to not only begin their own projects but also contribute to this educational instrument’s ongoing development.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Effect of magnetic field ripple on parallel electron transport during microwave plasma heating in the Proto-MPEX linear plasma device

The Prototype Material Plasma Exposure eXperiment (Proto-MPEX) is a linear plasma device located at Oak Ridge National Laboratory to develop the plasma source concept for the Materials Plasma Exposure eXperiment (MPEX). Recent experiments have demonstrated the heating of electrons in a high-density deuterium plasma (n e ~ 5 × 10 19 m -3 ) via electron Bernstein waves and source plasma production via helicon waves in this linear configuration. Moreover, experimental observations suggest that the magnetic ripple adversely affects the parallel transport of the heated electrons toward the target where material samples are to be exposed to the plasma. In order to understand the transport process during microwave application, a test-particle Monte-Carlo (MC) code has been developed that incorporates the effects of Coulomb collisions, magnetic mirror adiabatic trapping and electron cyclotron interaction via a quasilinear RF heating operator. MC calculations indicate that the absence of 2nd turning points along the trajectory of cyclotron heated electrons significantly reduces adiabatic trapping and maximizes power transport to the Target surface. Thermalization of cyclotron heating electrons is analyzed with the MC code and it is found that for conditions relevant to ProtoMPEX, a significant fraction of the absorbed heating power is coupled to the Target surface via ballistic fast electrons; however, under certain conditions, up to 60% of the absorbed RF power can be dissipated via thermalization of the fast electrons on the background plasma. Results are compared with experimental measurements. Finally, the implications of the results are discussed in the context of the upcoming MPEX device.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Beam characterization at NSRL for radiobiological experiments—phase 1

An experimental campaign was carried out at the NASA Space Radiation Laboratory to perform an additional, independent dosimetric characterization of the beams of protons, helium and carbon ions for radiobiological experiments. The campaign was undertaken by the request and with the support from the National Cancer Institute, U.S. In this initial phase, the goals were to obtain a first assessment of the dosimetric reproducibility of the beam control system, including analysis of spatial homogeneity and evaluation of ion beam contamination. They should facilitate the design of further experimental campaigns for beam characterization for radiobiological experiments. Measurements included reference dosimetry with comparison of in-house and external ionization chambers and electrometers, lateral-dose profile measurements in air, depth-dose profile in a water tank, evaluation of water equivalent thickness of a HDPE binary range shifter and estimation of impurities of the investigated helium-ion beam. The experiments and results are presented.

43 PARTICLE ACCELERATORS↗

Trigger Detection for the sPHENIX Experiment via Bipartite Graph Networks with Set Transformer

Trigger (interesting events) detection is crucial to high-energy and nuclear physics experiments because it improves data acquisition efficiency. It also plays a vital role in facilitating the downstream offline data analysis process. The sPHENIX detector, located at the Relativistic Heavy Ion Collider in Brookhaven National Laboratory, is one of the largest nuclear physics experiments on a world scale and is optimized to detect physics processes involving charm and beauty quarks. Furthermore, these particles are produced in collisions involving two proton beams, two gold nuclei beams, or a combination of the two and give critical insights into the formation of the early universe. This paper presents a model architecture for trigger detection with geometric information from two fast silicon detectors. Transverse momentum is introduced as an intermediate feature from physics heuristics. We also prove its importance through our training experiments. Each event consists of tracks and can be viewed as a graph. A bipartite graph neural network is integrated with the attention mechanism to design a binary classification model. Compared with the state-of-the-art algorithm for trigger detection, our model is parsimonious and increases the accuracy and the AUC score by more than 15%.

97 MATHEMATICS AND COMPUTING↗

NCERC-CL TREAT Free Field Characterization Foil Reaction Rate Results

This report summarizes the analysis and preliminary MCNP reaction rate modeling of free field characterization measurements performed in the Transient Reaction Test Facility (TREAT) at Idaho National Laboratory (INL) between 12/18/2023 and 2/22/2024. A series of seven irradiations were performed using the Big-BUSTER (Broad Use Specimen Transient Experiment Rig) core configuration. Foil sets including 19.5% LEU-Zr alloy wire, S, Au, Fe, Ni, Co, Ti, and Zr were deployed in each irradiation. Identical foil sets were supplied to Los Alamos National Laboratory (LANL), Lawrence Livermore National Laboratory (LLNL), and INL. All foils were supplied by INL. Additional details on the experiment can be found in [2]. The foil sets were shipped to the National Criticality Experiments Research Center Counting Laboratory (NCERC-CL) branch at LANL (NCERC-CL NISC) and were received on 3/25/2024. Additional details on receipt and counting are reported in [3]. All reactor dosimetry measurements were performed in adherence to the ASTM standards applicable to reactor dosimetry. Measured reaction rates from Au, Co, Fe, Ni, and Ti are reported. Select reaction rate ratios and simulated reaction rates and ratios are discussed. Reaction rates for all measured reaction products were modeled with MCNP 6.3.1 and a TREAT input deck supplied by Edward Lum. Neutron emission estimates calculated using the measured and simulated reaction rates show excellent agreement between the three fast-threshold n-p reactions with the percent differences being < 9% between the three reactions. The capture reactions had poorer, but still reasonable, agreement with < 20% percent differences between the neutron emission estimates of the three capture reactions. The percent difference between the fast-threshold and capture reactions is ∼ 100% for each reaction. This supports the TREAT model is not accurately modeling the neutron spectrum and additional measurements are required to characterize TREAT and match measurements to simulation.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗