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At least 1,117 records · Page 62

Pedestal origin and extrapolation of high-density small edge-localised-modes peak parallel energy fluence in ITER and SPARC

Experimental analysis and simulations with the BOUT++ code show that small edge-localised modes (ELMs) in reactor-relevant high-density regimes originate in a region close to the separatrix and only marginally perturb the pedestal structure. The measured divertor peak parallel energy fluence (ε ∥,peak ) for a database of small ELM scenarios in DIII-D and ASDEX Upgrade can be reproduced, within 40 % accuracy on average, if an ad hoc modification of the Eich peak parallel ELM energy fluence model is applied to account for the small ELM pedestal birth location. This allows for first-order extrapolation of small-ELM divertor ε ∥,peak to ITER and SPARC, resulting in values that satisfy the nominal melting threshold of tungsten monoblocks of 12 MJ m −2 . The findings reported in this study, both via modelling and direct measurements, constitute a step forward in assessing small ELMs in high edge-collisionality scenarios as a viable plasma regime for the operation of next-generation fusion machines.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Fast and Invertible Simplicial Approximation of Magnetic‐Following Interpolation for Visualizing Fusion Plasma Simulation Data

We introduce a fast and invertible approximation for fusion plasma simulation data represented as 2D planar meshes with connectivities approximating magnetic field lines along the toroidal dimension in deformed 3D toroidal spaces. Scientific variables (e.g., density and temperature) in these fusion data are interpolated following a complex magnetic-field-line-following scheme in the toroidal space represented by a cylindrical coordinate system. This deformation in the 3D space poses challenges for root-finding and interpolation. To this end, we propose a novel paradigm for visualizing and analyzing such data based on a newly developed algorithm for constructing a 3D simplicial mesh within the deformed 3D space. Our algorithm generates a tetrahedral mesh that connects the 2D meshes using tetrahedra while adhering to the constraints on node connectivities imposed by the magnetic field-line scheme. Specifically, we first divide the space into smaller partitions to reduce complexity based on the input geometries and constraints on connectivities. Then, we independently search for a feasible tetrahedralization of each partition, considering nonconvexity. We demonstrate our method with two X-Point Gyrokinetic Code (XGC) simulation datasets on the International Thermonuclear Experimental Reactor (ITER) and Wendelstein 7-X (W7-X), and use an ocean simulation dataset to substantiate broader applicability of our method. An open source implementation of our algorithm is available at https://github.com/rcrcarissa/DeformedSpaceTet.

Ren, Congrong [The Ohio State Univ., Columbus, OH ↗

Evaluations of Silicon Carbide Temperature Monitors

The effect of irradiation on materials properties is an important field of study for materials usage in both fission and fusion systems for energy production. Neutron flux and energy spectrums are well understood; however, the irradiation temperature can be more difficult to determine. Since the early 1960s, Silicon Carbide (SiC) has been used as a passive post-irradiation temperature monitor because the irradiation defects anneal out above the irradiation temperature. Irradiation temperature is determined by measuring a property change after isochronal annealing or during a continuously monitored annealing process. There are many properties that may be measured including electrical resistivity, bulk density, dimensions, thermal diffusivity, or lattice spacing. Electrical resistivity is accepted as a robust measurement technique; however, such method is time-consuming since the steps involved must be performed in a serial manner. The use of thermal expansion from continuous dilatometry is an automated process requiring minimal setup time. As part of a Nuclear Science User Facilities (NSUF) project, low dose silicon carbide monitors were irradiated in the BR2 material test reactor at SCK, Belgium, and were then evaluated at the Idaho National Laboratory (INL) High Temperature Test Laboratory (HTTL) to determine their peak temperature achieved during irradiation. The technical significance of this work was that the monitors were irradiated to a dose that was significantly less than recommended in published literature. This paper will discuss the evaluation processes available at HTTL and the performance of the low dose silicon carbide temperature monitors.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Nitridation of atomically smooth (111) diamond surfaces using a low temperature Penning plasma discharge

Diamond is a material with a wide band gap that can host a variety of isolated paramagnetic defects, called “color centers”1. These color centers have attractive optical and magnetic properties suitable for quantum applications including quantum computing, nanophotonics and quantum sensing. The most common one is the negatively charged nitrogen vacancy (NV) color center. For quantum sensing, it is desirable to reduce the distance between the NV center and the analyte by using shallow color centers in order to increase sensitivity. In this context, the diamond surface termination is especially critical. The appropriate surface termination is required to stabilize the color centers and mitigate surface magnetic noise. The nitrogen termination of diamond has been postulated as highly desirable for the NV color center. The goal of this project is to take advantage of an electron beam-generated ExB low temperature plasma developed by the Princeton Collaborative Low Temperature Plasma Research Facility (PCRF) at the Princeton Plasma Physics Laboratory (PPPL) to nitridate the surface of (100) diamond single crystals with minimal surface damage. In this reactor, the use of a magnetized plasma enables gentle processing of materials sensitive to ion damage. This is in strong contrast to radiofrequency plasma processing reactors which are known to etch and sputter the surface. XPS measurements indicate the incorporation of nitrogen and oxygen atoms at the surface in similar amounts. XAS measurements confirm the nitridation and indicate that the nitrogen termination is different from the nitrogen termination obtained using radiofrequency plasma treatment4. The combination of these results indicates the formation of amid species at the (100) diamond surface that are promising for the stabilization of NV centers for quantum sensing.

36 MATERIALS SCIENCE↗

FreeMHD: Validation and verification of the open-source, multi-domain, multi-phase solver for electrically conductive flows

The extreme heat fluxes in the divertor region of tokamaks may require an alternative to solid plasma-facing components, for the extraction of heat and the protection of the surrounding walls. Flowing liquid metals are proposed as an alternative, but raise additional challenges that require investigation and numerical simulations. Free surface designs are desirable for plasma-facing components, but steady flow profiles and surface stability must be ensured to limit undesirable interactions with the plasma. Previous studies have mainly used steady-state, 2D, or simplified models for internal flows and have not been able to adequately model free-surface liquid metal (LM) experiments. Therefore, FreeMHD has been recently developed as an open-source magnetohydrodynamics (MHD) solver for free-surface electrically conductive flows subject to a strong external magnetic field. The FreeMHD solver computes incompressible free-surface flows with multi-region coupling for the investigation of MHD phenomena involving fluid and solid domains. The model utilizes the finite-volume OpenFOAM framework under the low magnetic Reynolds number approximation. FreeMHD is validated using analytical solutions for the velocity profiles of closed channel flows with various Hartmann numbers and wall conductance ratios. Next, experimental measurements are then used to verify FreeMHD, through a series of cases involving dam breaking, 3D magnetic fields, and free-surface LM flows. These results demonstrate that FreeMHD is a reliable tool for the design of LM systems under free surface conditions at the reactor scale. Furthermore, it is flexible, computationally inexpensive, and can be used to solve fully 3D transient MHD flows.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Evaluating the carbon footprint of the integrated DBD‐plasma bi‐reforming unit via laboratory scale experiments and scaled‐up process modeling

Catalytic dielectric barrier discharge (DBD) plasma reactor experiments were performed in a tubular glass reactor with a 2 mm gap at 550°C to facilitate the reaction kinetics of steam added dry reforming or bireforming. The best specific energy input obtained was 11.2 eV/molecule feed at CO 2 :CH 4 :H 2 O of 4.5:1:4.5 ratio and gas hour space velocity (GHSV) = 432 h −1 . This value was used to design a conceptual process and assess the environmental impact of methane steam reforming-based H 2 production 18.4 kmol/h CO 2 emission processing into H 2 :CO = 2 syngas, with an emphasis on the carbon footprint.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Effects of frequency and pulse width on electron density, hydrogen peroxide generation, and perfluorooctanoic acid mineralization in a nanosecond pulsed discharge gas-liquid plasma reactor

Plasma electron density and temperature were characterized in a continuous flowing gas-liquid film reactor with argon carrier gas by time-resolved optical emission spectroscopy. The plasma parameters were studied as a function of time for varying pulse widths and frequencies. Pulse frequency was varied between 1 and 10 kHz at 16 kV (input voltage) and 40 ns (pulse width) using an Eagle Harbor Technologies, Inc. (EHT) power supply and 5–100 kHz using an Airity Technologies, LLC (AT) power supply. The pulse width was varied between 40 and 200 ns at 16 kV, 2 kHz with the EHT power supply. Optimal frequencies of 5 and 20 kHz were observed for peak electron density with EHT and AT power supplies, respectively. The peak electron density increased with increasing pulse width between 40 and 200 ns using the EHT power supply. Hydrogen peroxide exiting the reactor in the liquid phase increased with discharge power irrespective of the power supply or pulse parameters. Mineralization of 12.5, 50, and 200 ppm perfluorooctanoic acid (PFOA) dissolved in DI water to fluoride (F - ) correlated to the peak electron density. Glycerol, a liquid-phase hydroxyl radical scavenger, depleted hydrogen peroxide but did not affect PFOA mineralization. CO, a gas-phase hydroxyl radical scavenger, led to a reduction in the formation of F - production, suggesting hydroxyl radicals in the gas-liquid film play a necessary, but not singular, role in mineralization of PFOA.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Plasma-arc lamp high heat flux cycling exposure of neutron irradiated tungsten materials

Thick plate, unalloyed W was neutron irradiated in the High Flux Isotope Reactor (HFIR) at 550 °C to a fast fluence of 1.24 × 10 25 n m -2 E > 0.1 MeV (~0.24 dpa). Unirradiated and irradiated specimens of the material were high heat flux (HHF) tested in the Plasma Arc Lamp (PAL) facility. The PAL uses a high-power photon source to provide a broad and even heat distribution on the sample surface. To simulate on/off cycling of normal operating plasma, the samples were exposed to approximately 800 cycles at 4.73 MW m -2 absorbed heat flux (incident heat fluxes of 10.95 MW m -2 ). Additionally, after PAL exposure, slight changes were observed on the surfaces of the samples with SEM. The samples showed some annealing in the near surface polished region, but they were all below the damage threshold for cracking or other destructive features. The PAL has a large parameter space for future testing. The use of the HFIR and PAL to sequentially expose neutron irradiated samples to HHF will be a powerful tool for understanding materials behavior in a fusion-like environment.

36 MATERIALS SCIENCE↗

Prototype tests of the electromagnetic particle injector-2 for fast time response disruption mitigation in tokamaks

Predicting and controlling disruptions is an important and urgent issue for ITER. Some disruptions with a short warning time may be unavoidable. For these cases, a fast time response disruption mitigation method is essential. Experimental tests on a prototype system of a novel, rapid time-response disruption mitigation system being developed for tokamak-based reactors and as a backup option for ITER, referred to as the electromagnetic particle injector (EPI), have been able to verify the primary advantages of the concept. These are its ability to meet short warning time scales of <10 ms while attaining the projected high velocities for deep radiative payload penetration in reactor-scale plasmas. The EPI relies on an electromagnetic propulsion system. A metallic sabot is accelerated electromagnetically to the required velocities (>1 km s -1 ) within 2 ms, at which point it releases a radiative payload consisting of a shell pellet or well-defined microspheres. Initial experimental tests from the prototype system show attainment of over 600 m s -1 in about 1 ms. Finally, essential aspects of payload separation from the sabot and sabot capture have also been demonstrated at 200 m s -1 , and the method can be extended to over 2 km s -1 .

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Power balance analysis at the L-H transition in JET-ILW NBI-heated deuterium plasmas

The understanding of the physics underlying the L-H transition has strong implications for ITER experimental reactor and demonstration power plant (DEMO). In many tokamaks, including JET, it has been observed that, at a particular plasma density, n e,min , the power necessary to access H-mode P L-H is minimum. In the present work, L-H transitions of JET deuterium plasmas heated by neutral beam injection (NBI) are studied for the first time by means of a power balance analysis to characterize the main contributions in the transition, through integrated transport modelling. In the pulses analysed, we do observe a minimum of the L-H power threshold in density, indicating the presence of density branches and of n e,min . Electron and ion heat fluxes at the transition are estimated separately. The electron/ion equipartition power results in favour of the ions, as shown by QuaLiKiz quasilinear gyrokinetic simulations, which predict a larger ion transport that causes T e > T i . The resulting edge ion heat flux also shows a clear change of slope below n e,min , similarly to ASDEX-Upgrade (AUG) NBI pulses (Ryter et al 2014 Nucl. Fusion 54 083003). JET NBI data are compared to radio-frequency heated AUG and Alcator C-mod pulses (Schmidtmayr et al 2018 Nucl. Fusion 58 056003), showing a different trend of the power, coupled to ions at the L-H transition with respect to the linearity observed in the radio-frequency heated plasmas. Finally, the presence of n e,min and the role of the ion heat flux is discussed in the paper, although it seems it is not possible to explain the presence of a P L-H minimum in density by a critical ion heat flux and by the equipartition power for the JET NBI-heated plasmas analysed.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Comparing Sensor Fusion and Multimodal Chemometric Models for Monitoring U(VI) in Complex Environments Representative of Irradiated Nuclear Fuel

Optical sensors and chemometric models were leveraged for the quantification of uranium(VI) (0–100 μg mL –1 ), europium (0–150 μg mL –1 ), samarium (0–250 μg mL –1 ), praseodymium (0–350 μg mL –1 ), neodymium (0–1000 μg mL –1 ), and HNO 3 (2–4 M) with varying corrosion product (iron, nickel, and chromium) levels using laser fluorescence, Raman scattering, and ultraviolet–visible–near-infrared absorption spectra. In this paper, an efficient approach to developing and evaluating tens of thousands of partial least-squares regression (PLSR) models, built from fused optical spectra or multimodal acquisitions, is discussed. Each PLSR model was optimized with unique preprocessing combinations, and features were selected using genetic algorithm filters. The 7-factor D-optimal design training set contained just 55 samples to minimize the number of samples. The performance of PLSR models was evaluated by using an automated latent variable selection script. PLS1 regression models tailored to each species outperformed a global PLS2 model. PLS1 models built using fused spectra data and a multimodal (i.e., analyzed separately) approach yielded similar information, resulting in percent root-mean-square error of prediction values of 0.9–5.7% for the seven factors. Further, the optical techniques and data processing strategies established in this study allow for the direct analysis of numerous species without measuring luminescence lifetimes or relying on a standard addition approach, making it optimal for near-real-time, in situ measurements. Nuclear reactor modeling helped bound training set conditions and identified elemental ratios of lanthanide fission products to characterize the burnup of irradiated nuclear fuel. Leveraging fluorescence, spectrophotometry, experimental design, and chemometrics can enable the remote quantification and characterization of complex systems with numerous species, monitor system performance, help identify the source of materials, and enable rapid high-throughput experiments in a variety of industrial processes and fundamental studies.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Role of microtearing mode in DIII-D and future high- β p core plasmas

This paper provides modeling evidence for a new variant of microturbulence instability that regulates the electron thermal fluxes in the transport barrier region of DIII-D "high β p " discharges. This scenario is being investigated as a possible scenario for future steady-state reactors, and thus it is essential to understand the physics processes which govern its performance in order to confidently extrapolate to future devices. Additional analysis examining the extrapolation of this scenario to ITER shows that while the new microtearing mode identified here is unlikely to be unstable in that regime (due to increased temperatures and reduced collisionality), the large shift in magnetic axis (Shafranov shift) that arises in these plasmas may still favor stabilization of common ballooning instabilities which peak on the low field side, but destabilize electrostatic slab modes on the high field side.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Phase Contrast Imaging Diagnostic on DIII-D (1994-2007); Phase Contrast Imaging Diagnostic on DIII-D and Alcator C-Mod (2007-2010); Experimental Study of Waves, Turbulence and Transport, and Model Validation with Phase Contrast Imaging on DIII-D and Alcator C-Mod (2010-2012); Phase Contrast Imaging Diagnostic Upgrade on DIII-D for Measuring High-k Turbulence and Alfven modes (2021-2016); Phase Contrast Imaging Diagnostic Upgrade on DIII-D for Full Multi-Scale Measurements (2016-2020) (Final Report)

This report describes the first twenty-five years of development and use of the Phase Contrast Imaging (PCI) diagnostic for measuring plasma fluctuations on the DIII–D tokamak. One of the key challenges in moving tokamak technology forward to the stage of a nuclear reactor remains understanding how energy and particles are transported across the magnetic field by the action of turbulence and waves, and PCI provides a highly flexible and capable measurement of these fluctuations. The PCI diagnostic uses a laser beam to probe the plasma and optical filtering to produce an amplitude variation on a linear detector array which provides an image of the density waves in the plasma. The PCI covers an exceptional range in frequency and wavelength of the measured fluctuations, allowing observation of plasma-sized magnetohydrodynamic (MHD) modes and ion- and electron-scale turbulence. Modulation of the beam amplitude allows measurement of radio frequency (RF) waves.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

A scalable transformer model for real-time decision making in neutron scattering experiments

The U.S. Department of Energy's (DOE's) neutron research facilities at Oak Ridge National Laboratory (ORNL), including the High Flux Isotope Reactor (HFIR) and the Spallation Neutron Source (SNS), are a state-of-the-art neutron scattering facility that allows researchers to study the structure and dynamics of materials at the atomic scale. At the SNS, neutrons are measured using the time-of-flight (TOF) technique as they move through a neutron beamline to interact with a sample. Large volumes of neutron scattering data are collected and recorded in neutron event mode. Optimal productivity of the TOF instrument is limited due to the lack of real-time data analysis tools. The large amount of data generated by the experiments can be challenging to process and analyze in real time, particularly for experiments that require rapid feedback and adjustment of experimental parameters. The regular computer/workstation cannot keep up with the experiment speed to provide real-time feedback to adjust experimental parameters, so connecting the supercomputers available to the neutron facility is necessary to achieve real-time data analysis and experiment steering. To address this challenge, we exploit the Frontier supercomputer at Oak Ridge Leadership Computing Facility (OLCF) to train a scalable temporal fusion transformer model for real-time decision making of TOF neutron scattering experimentation. Here, in this paper, we present the results using Frontier to provide the processing power needed to rapidly process and analyze large volumes of single-crystal diffraction data collected at TOPAZ, a neutron time-of-flight Laue single-crystal diffractometer at the SNS.

97 MATHEMATICS AND COMPUTING↗

Identifying Regimes During Plasma Catalytic Ammonia Synthesis

Herein, we demonstrate that the performance of mesoporous silica SBA-15 and SBA-15-Ag during plasma ammonia synthesis depends on the plasma conditions. At high power, the mesoporous silica SBA-15 without Ag produces the largest amount of ammonia, but the addition of Ag provides a minor benefit at lower powers. Plasma conditions were analyzed through optical emission spectroscopy using N 2 , N 2 + , and NH molecular bands and H α line. Stark broadening of H α line was used to find electron density, and N 2 molecular bands were used to assess N 2 vibrational excitation, important for plasma nitrogen decomposition. At similar input conditions, reactors with SBA-15 have higher electron density and higher N 2 vibrational temperature. Consistent with higher electron density, SBA-15 reactors have stronger N 2 + emission intensity relative to the neutral N 2 . The addition of Ag results in higher N 2 rotational temperature, possibly due to localized heating. From the materials point of view, SBA-15 is a more robust catalyst with good surface area retention after plasma exposure due to the lack of local heating generated when a metal is in the structure. Furthermore, we identify two possible regimes during ammonia synthesis, a metal and a surface-plasma driven. At lower plasma densities, the addition of metal is beneficial, while at higher power and plasma density, the best performance is achieved without the aid of a metal catalyst.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Access and limits of RMP ELM suppression with n = 1 fields in DIII-D

This work reports on DIII-D experiments aimed at extending resonant magnetic perturbation (RMP) suppression of edge localized modes (ELMs) to n = 1 fields, where n is the toroidal mode number. Modeling of the 3D ideal MHD plasma response to the RMPs using the GPEC code is used to quantify edge and core resonant fluxes, guiding experimental strategies to increase plasma resilience against core error field penetration, optimize multicoil phasing, and explore higher q 95 operation. In DIII-D, ELM mitigation is regularly observed across a wide range of n = 1 RMP scenarios. A ∼100 ms phase of complete ELM suppression was achieved at q 95 ∼ 3.9 using an odd-parity coil configuration. The suppressed phase exhibited clear signatures of RMP ELM suppression, including the elimination of Dα spikes, increased pedestal rotation, enhanced magnetic response, and elevated broadband density turbulence. An optimized coil configuration for edge-to-core resonant flux did show increased edge resonance indicated by increased density pumpout, but did not yield RMP ELM suppression. At q 95 ∼ 5.1, a bifurcation to a grassy-like ELM regime occurred, while large type-I ELMs persisted. These results demonstrate progress in experimental access to n = 1 RMP ELM suppression in DIII-D, motivating further study for robust access. This work also highlights the potential role of 3D edge stability as well as rational surface alignment in RMP ELM suppression access, which has important implications for the use of low-n RMPs in future reactor-scale devices.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗