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All sourcesNASA NTRSDOE OSTI
NASA NTRS2007

NASA Tech Briefs, January 2007

Topics covered include: Flexible Skins Containing Integrated Sensors and Circuitry; Artificial Hair Cells for Sensing Flows; Video Guidance Sensor and Time-of-Flight Rangefinder; Optical Beam-Shear Sensors; Multiple-Agent Air/Ground Autonomous Exploration Systems; A 640 512-Pixel Portable Long-Wavelength Infrared Camera; An Array of Optical Receivers for Deep-Space Communications; Microstrip Antenna Arrays on Multilayer LCP Substrates; Applications for Subvocal Speech; Multiloop Rapid-Rise/Rapid Fall High-Voltage Power Supply; The PICWidget; Fusing Symbolic and Numerical Diagnostic Computations; Probabilistic Reasoning for Robustness in Automated Planning; Short-Term Forecasting of Radiation Belt and Ring Current; JMS Proxy and C/C++ Client SDK; XML Flight/Ground Data Dictionary Management; Cross-Compiler for Modeling Space-Flight Systems; Composite Elastic Skins for Shape-Changing Structures; Glass/Ceramic Composites for Sealing Solid Oxide Fuel Cells; Aligning Optical Fibers by Means of Actuated MEMS Wedges; Manufacturing Large Membrane Mirrors at Low Cost; Double-Vacuum-Bag Process for Making Resin- Matrix Composites; Surface Bacterial-Spore Assay Using Tb3+/DPA Luminescence; Simplified Microarray Technique for Identifying mRNA in Rare Samples; High-Resolution, Wide-Field-of-View Scanning Telescope; Multispectral Imager With Improved Filter Wheel and Optics; Integral Radiator and Storage Tank; Compensation for Phase Anisotropy of a Metal Reflector; Optical Characterization of Molecular Contaminant Films; Integrated Hardware and Software for No-Loss Computing; Decision-Tree Formulation With Order-1 Lateral Execution; GIS Methodology for Planning Planetary-Rover Operations; Optimal Calibration of the Spitzer Space Telescope; Automated Detection of Events of Scientific Interest; Representation-Independent Iteration of Sparse Data Arrays; Mission Operations of the Mars Exploration Rovers; and More About Software for No-Loss Computing.

Source record↗
DOE OSTI2026

Picosecond measurements of plastic scintillator pulse shapes from gamma-ray interactions

An understanding of the pulse shape of organic scintillators can provide insight into scintillation mechanisms and inform the selection of the optimal detector material for a given application. Although the timing properties of organic scintillators have been extensively studied, significant discrepancies persist in reported rise and decay times. New plastic scintillating media have also been developed in recent years for which no literature data exist. The goal of this work is to provide high-precision measurements of the pulse shape of a suite of fast plastic organic scintillators from Eljen Technology—EJ-200, EJ-204, EJ-208, EJ-230, EJ-232, and EJ-232Q (with 0.5% benzophenone)—under excitation from $γ$-ray sources. The contributors to the system temporal resolution were quantified, and the dominant source of uncertainty was identified as the determination of the start time of a scintillation event. A pulse shape model was applied to the reconstructed temporal distributions, and rise and decay times were extracted and compared with manufacturer specifications. This work outlines a measurement approach to obtain the pulse shape of organic scintillators in response to $γ$-rays with temporal resolution on the order of tens of picoseconds, yielding data required for modeling plastic scintillator based detection systems for a range of applications.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2020

A variable X-ray chopper system for phase-sensitive detection in synchrotron X-ray scanning tunneling microscopy

An ultra-high-vacuum compatible X-ray chopper system has been designed, constructed and integrated into the XTIP beamline at the Advanced Photon Source at Argonne National Laboratory. The XTIP beamline can operate at soft X-ray energies from 400 eV to 1900 eV while providing a focused beam down to about 10 µm × 10 µm into the synchrotron X-ray scanning tunneling microscopy (SX-STM) endstation instrument. The X-ray chopper is a critical component for separating topographic information from chemical information in SX-STM through phase-sensitive current detection. Depending on the experimental needs, the modulation frequency can be controlled from 100 Hz to 10 kHz. In addition, the chopper system is fully bakeable and can achieve a base pressure of 10 -10 mbar. Facilities for active water cooling have been designed, but passive cooling through copper braids has been shown to be sufficient at standard chopping frequencies. Using an Fe/Al 2 O 3 /CoAl(111) sample, the separation of the SX-STM current into a chemical component and a stable feedback signal is demonstrated.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
NASA NTRS1993

Space Shuttle main engine OPAD: The search for a hardware enhanced plume

The process of applying spectroscopy to the Space Shuttle Main Engine (SSME) for plume diagnostics, as it exists today, originated at Marshall Space Flight Center in Huntsville, Alabama, and its implementation was assured largely through the efforts of Sverdrup AEDC, in Tullahoma, Tennessee. This team continues to lead and guide efforts in the plume diagnostics arena. The process, Optical Plume Anomaly Detection (OPAD), formed the basis for various activities in the development of ground-based systems as well as the development of in-flight plume spectroscopy. OPAD currently provides and will continue to provide valuable information relative to future systems definitions, instrumentation development, code validation, and data diagnostic processing. OPAD is based on the detection of anomalous atomic and molecular species in the SSME plume using two complete, stand-alone optical spectrometers. To-date OPAD has acquired data on 44 test firings of the SSME at the Technology Test Bed (TTB) at MSFC. The purpose of this paper will be to provide an introduction to the OPAD system by discussing the process of obtaining data as well as the methods of examining and interpreting the data. It will encompass such issues as selection of instrumentation correlation of data to nominal engine operation, investigation of SSME component erosion via OPAD spectral data, necessity and benefits of plume seeding, application of artificial intelligence (AI) techniques to data analysis, and the present status of efforts to quantify specie erosion utilizing standard plume and chemistry codes as well as radiative models currently under development.

Powers, W. T.↗
NASA NTRS1995

A search for fast gamma-ray pulsars with OSSE

Pulsar mode data from the Oriented Scintillation Spectrometer Experiment (OSSE) onboard the Compton Gamma Ray Observatory (CGRO), with time resolution between 125 microsecs and 8 ms, have been analyzed for the presence of short-period gamma-ray pulsations. Observations of known point sources (including SN 1987A, SN 1993J, GRO J0422+32, and several pulsars) and of regions where higher densities of pulsars are expected (including the Galactic center, the Galactic plane and arms, and the Large Magellanic Cloud) are included in the study. Both isolated pulsars and pulsars in close binary systems are searched for; in the latter case, the quadratic coherence recovery technique is used to correct for broadening of the pulsar signal from orbital motion. No new gamma-ray pulsars have been detected. Upper limits on the pulsed gamma-ray flux from isolated pulsars in the 50-210 keV energy range of OSSE are between 0.2 x 10(exp -3) and 2.0 x 10(exp -3) photons/s/sq cm for pulse periods between 250 microsecs and 0.5 s. Upper limits on the pulsed flux from binary pulsars are between 1.5 x 10(exp -3) and 6.4 x 10(exp -3) photons/s/sq cm for the same energy band and pulse period range. We estimate that, in the Galaxy, there are fewer than approximately 125 isolated pulsars similar to PSR B1509-58 with radiation peaks in the OSSE band but undetected in the radio and X-rays bands.

Hertz, P.↗
NASA NTRS2008

NASA Tech Briefs, June 2008

Topics covered include: Charge-Control Unit for Testing Lithium-Ion Cells; Measuring Positions of Objects Using Two or More Cameras; Lidar System for Airborne Measurement of Clouds and Aerosols; Radiation-Insensitive Inverse Majority Gates; Reduced-Order Kalman Filtering for Processing Relative Measurements; Spaceborne Processor Array; Instrumentation System Diagnoses a Thermocouple; Chromatic Modulator for a High-Resolution CCD or APS; Commercial Product Activation Using RFID; Cup Cylindrical Waveguide Antenna; Aerobraking Maneuver (ABM) Report Generator; ABM Drag_Pass Report Generator; Transformation of OODT CAS to Perform Larger Tasks; Visualization Component of Vehicle Health Decision Support System; Mars Reconnaissance Orbiter Uplink Analysis Tool; Problem Reporting System; G-Guidance Interface Design for Small Body Mission Simulation; DSN Scheduling Engine; Replacement Sequence of Events Generator; Force-Control Algorithm for Surface Sampling; Tool for Merging Proposals Into DSN Schedules; Micromachined Slits for Imaging Spectrometers; Fabricating Nanodots Using Lift-Off of a Nanopore Template; Making Complex Electrically Conductive Patterns on Cloth; Special Polymer/Carbon Composite Films for Detecting SO2; Nickel-Based Superalloy Resists Embrittlement by Hydrogen; Chemical Passivation of Li+-Conducting Solid Electrolytes; Organic/Inorganic Polymeric Composites for Heat-Transfer Reduction; Composite Cathodes for Dual-Rate Li-Ion Batteries; Improved Descent-Rate Limiting Mechanism; Alignment-Insensitive Lower-Cost Telescope Architecture; Micro-Resistojet for Small Satellites; Using Piezoelectric Devices to Transmit Power through Walls; Miniature Latching Valve; Apparatus for Sampling Surface Contamination; Novel Species of Non-Spore-Forming Bacteria; Chamber for Aerosol Deposition of Bioparticles; Hyperspectral Sun Photometer for Atmospheric Characterization and Vicarious Calibrations; Dynamic Stability and Gravitational Balancing of Multiple Extended Bodies; Simulation of Stochastic Processes by Coupled ODE-PDE; Cluster Inter-Spacecraft Communications; Genetic Algorithm Optimizes Q-LAW Control Parameters; Low-Impact Mating System for Docking Spacecraft; Non-Destructive Evaluation of Materials via Ultraviolet Spectroscopy; Gold-on-Polymer-Based Sensing Films for Detection of Organic and Inorganic Analytes in the Air; and Quantum-Inspired Maximizer.

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NASA NTRS2011

The 2010 May Flaring Episode of Cygnus X-3 in Radio, X-Rays, and gamma-Rays

In 2009, Cygnus X-3 (Cyg X-3) became the first microquasar to be detected in the GeV gamma-ray regime, via the satellites Fermi and AGILE. The addition of this new band to the observational toolbox holds promise for building a more detailed understanding of the relativistic jets of this and other systems. We present a rich dataset of radio, hard and soft X-ray, and gamma-ray observations of Cyg X-3 made during a flaring episode in 2010 May. We detect a approx.3-d softening and recovery of the X-ray emission, followed almost immediately by a approx.1-Jy radio flare at 15 GHz, followed by a 4.3sigma gamma-ray flare (E > 100 MeV) approx.1.5 d later. The radio sampling is sparse, but we use archival data to argue that it is unlikely the gamma-ray flare was followed by any significant unobserved radio flares. In this case, the sequencing of the observed events is difficult to explain in a model in which the gamma-ray emission is due to inverse Compton scattering of the companion star's radiation field. Our observations suggest that other mechanisms may also be responsible for gamma-ray emission from Cyg X-3.

Williams, Peter K. G.↗
NASA NTRS2018

Biosignature Anisotropy Modeled on Temperate Tidally Locked M-Dwarf Planets

A planet’s atmospheric constituents (e.g., O2, O3, H2Ov, CO2, CH4, and N2O) can provide clues to its surface habitability, and may offer biosignature targets for remote life detection efforts. The plethora of rocky exoplanets found by recent transit surveys (e.g., the Kepler mission) indicates that potentially habitable systems orbiting K- and M-dwarf stars may have very different orbital and atmospheric characteristics than Earth. To assess the physical distribution and observational prospects of various biosignatures and habitability indicators, it is important to understand how they may change under different astrophysical and geophysical configurations, and to simulate these changes with models that include feedbacks between different subsystems of a planet’s climate. Here we use a three-dimensional (3D) Chemistry–Climate model (CCM) to study the effects of changes in stellar spectral energy distribution (SED), stellar activity, and planetary rotation on Earth analogs and tidally locked planets. Our simulations show that, apart from shifts in stellar SEDs and UV radiation, changes in illumination geometry and rotation-induced circulation can influence the global distribution of atmospheric biosignatures. We find that the stratospheric day-to-nightside mixing ratio differences on tidally locked planets remain low (<20%) across the majority of the canonical biosignatures. Interestingly, however, secondary photosynthetic biosignatures (e.g., C2H6S) show much greater (∼67%) day-to-nightside differences, and point to regimes in which tidal locking could have observationally distinguishable effects on phase curve, transit, and secondary eclipse measurements. Overall, this work highlights the potential and promise for 3D CCMs to study the atmospheric properties and habitability of terrestrial worlds.

Chen, Howard↗
NASA NTRS2003

The Achromatic Light Curve of the Optical Afterglow of GRB 030226 at a Redshift of z Approximately 2

Abstract. We report on optical and near-infrared (NIR) follow-up observations of the afterglow of GRB 030226, mainly performed with the telescopes at ESO La Silla and Paranal, with additional data obtained at other places. Our first observations started 0.2 days after the burst when the afterglow was at a magnitude of R approximately equal to 19 . One week later the magnitude of the afterglow had fallen to R=25, and at two weeks after the burst it could no longer be detected (R > 26). Our VLT blueband spectra show two absorption line systems at redshifts z = 1.962 +/- 0.001 and at z = 1.986 +/- 0.001, placing the redshift of the burster close to 2. Within our measurement errors no evidence for variations in the line strengths has been found between 0.2 and 1.2 days after the burst. An overabundance of alpha-group elements might indicate that the burst occurred in a chemically young interstellar region shaped by the nucleosynthesis from type II supernovae. The spectral slope of the afterglow shows no signs for cosmic dust along the line of sight in the GRB host galaxy, which itself remained undetected (R > 26.2). At the given redshift no supernova component affected the light from the GRB afterglow, so that the optical transient was essentially only powered by the radiation from the GRB fireball, allowing for a detailed investigation of the color evolution of the afterglow light. In our data set no obvious evidence for color changes has been found before, during, or after the smooth break in the light curve approximately 1 day after the burst. In comparison with investigations by others, our data favor the interpretation that the afterglow began to develop into a homogeneous interstellar medium before the break in the light curve became apparent.

Klose, S.↗
NASA NTRS2012

The Use of the North Alabama Lightning Mapping Array (NALMA) in the Real-Time Operational Warning Environment During the March 2nd, 2012 Severe Weather Outbreak in Northern Alabama

The North Alabama Lightning Mapping Array (NALMA) is a three-dimensional very high frequency (VHF) detection network consisting of 11 sensors spread across north central Alabama and two sensors located in the Atlanta, Georgia region. The primary advantage of this network is that it detects total lightning, or the combination of both cloud-to-ground and intra-cloud lightning, instead of cloud-to-ground lightning alone. This helps to build a complete picture of storm evolution and development, and can serve as a proxy for storm updraft strength, particularly since intra-cloud lightning makes up the majority of all lightning in a typical thunderstorm. While the NALMA data do not directly indicate severe weather, they can indirectly indicate when a storm is strengthening (weakening) due to increases (decreases) in updraft strength, as the updraft is responsible for charging mechanisms within the storm. Data output are VHF radiation sources, which are produced during lightning breakdown processes. These sources are made into 2x2 km source density grids and are ported into the Advanced Weather Interactive Processing System (AWIPS) for National Weather Service (NWS) offices in Huntsville, AL, Nashville, TN, Morristown, TN, and Birmingham, AL, in near real-time. An increase in sources, or source densities, correlates to increased lightning activity and trends in updraft magnitude as long as the storm is within about 125 km of the center of the LMA network. Operationally, these data have been used at the Huntsville NWS office since early 2003 through a collaborative effort with NASA s Short-term Prediction Research and Transition (SPoRT) Center. Since then, total lightning observations have become an essential tool for forecasters during real-time warning operations. One of the operational advantages of the NALMA is the two-minute temporal resolution of the data. This provides forecasters with two to three updates during a typical volume scan of the WSR-88D radar.

White, Kristopher↗
NASA NTRS2019

Internal Electrostatic Discharge Testing of Inert Solid Rocket Motor Materials

Jupiter’s moon Europa is believed to have a global liquid-water ocean beneath its icy surface. As such, it is a highly interesting destination for explorers seeking signs of life outside of Earth. This interest has given rise to the Europa Lander Mission [Hand, et al., 2017]. The central goal of the Europa Lander Mission is to place a stationary lander on Europa and make surface and sub-surface measurements, dramatically improving understanding of this Jovian moon, and potentially detecting signs of life.Placing a lander on Europa will require multiple spacecraft elements deployed across a multi-year mission timeline. Some of the key elements include: a large payload capacity rocket, such as the Space Launch System (SLS), capable of providing direct Jupiter orbit insertion; a solar-powered carrier; a de-orbit system; a sky crane landing system; and, of course, the surface lander. A noteworthy fact is that the current design requires a large solid rocket motor to provide the necessary braking thrust for the de-orbit stage. While solid rocket motors have been used extensively by NASA during launch, in-space use has been limited. In addition to the normal challenges associated with a long-distance planetary mission, the Europa Lander Mission must also contend with the high-radiation environment associated with the Jovian system. The size of Jupiter, combined with its magnetic field strength, and rotation speed, result in a harsh radiation environment composed of high energy charged particles (ions and electrons) as well as high-temperature plasmas [de Soria-Santacruz Pich, 2016]. Due to this high-radiation environment, each component of the Europa Lander spacecraft must be evaluated to determine its radiation dose tolerance and its likelihood for experiencing electrostatic charging (and discharging). In general, metal components in a Jovian environment do not pose a concern for radiation degradation; in fact, metal structures and closeouts can act as radiation shielding for the more sensitive components. Charging of a metal component is only an issue if the component is not properly grounded to the spacecraft chassis. However, electrically insulating materials, such as polymers, are subject to radiation degradation as well as surface and internal charging, and therefore require extra scrutiny. The focus of this paper will be on the insulating materials that are commonly used inside solid rocket motors. The special application of a solid rocket motor used in space after a relatively long duration flight, combined with the high energy electron environment in the Jovian system, raises concerns about the possibility of significant charging and discharging leading to reduced performance.

Schneider, Todd A.↗
DOE OSTI2025

Origin of proton irradiation-induced deep acceptors in Al 0.70 Ga 0.30 N

Deep level defect introduction and carrier removal were characterized using steady-state photocapacitance (SSPC), deep level transient spectroscopy (DLTS) and lighted capacitance–voltage for proton irradiated n-type Al 0.70 Ga 0.30 N Schottky diodes grown by metal-organic vapor phase epitaxy on AlN-on-sapphire templates. SSPC observed deep levels in the as-grown diode with zero-phonon transition energies of 2.20, 2.65, 3.10, 3.40, and 4.65 eV relative to the conduction band minimum (E c ), and an additional deep level emerged at 1.20 eV with irradiation. Lighted capacitance–voltage measurements quantified the deep level concentration (N t ) of states detected by SSPC, and it was observed that N t increased with proton fluence only for the 1.2 and 4.65 eV levels. Carrier removal was much larger than the increase in N t of the 1.2 and 4.65 eV deep levels, suggesting that radiation-induced deep level compensators existed beyond what was detected with SSPC. DLTS detected additional, proton-induced deep acceptors at E c —0.55, 0.82, and 1.16 eV, the latter of which is likely the same 1.20 eV deep state observed by SSPC. The concentration of the E c —0.82 eV defect state was large enough to reconcile carrier removal with total deep level introduction. Comparing the E c —0.82 and 1.16 eV deep acceptor levels to previous experimental and theoretical reports suggests that their atomistic origins could be the nitrogen vacancy (V N ) and oxygen substituting on the nitrogen sub-lattice (O N ), respectively. This defect behavior contrasts starkly with GaN, where V N and O N are shallow donors, and demonstrates that the electronic properties of defects can evolve drastically within the AlGaN alloy system ranging from wide bandgap GaN to ultra-wide bandgap AlN.

Armstrong, Andrew Michael [Sandia National Laborat↗
NASA NTRS1994

Study of atmospheric parameters measurements using MM-wave radar in synergy with LITE-2

The Lidar In-Space Technology Experiment, (LITE), has been developed, designed, and built by NASA Langley Research Center, to be flown on the space shuttle 'Discovery' on September 9, 1994. Lidar, which stands for light detecting and ranging, is a radar system that uses short pulses of laser light instead of radio waves in the case of the common radar. This space-based lidar offers atmospheric measurements of stratospheric and tropospheric aerosols, the planetary boundary layer, cloud top heights, and atmospheric temperature and density in the 10-40 km altitude range. A study is being done on the use, advantages, and limitations of a millimeterwave radar to be utilized in synergy with the Lidar system, for the LITE-2 experiment to be flown on a future space shuttle mission. The lower atmospheric attenuation, compared to infrared and optical frequencies, permits the millimeter-wave signals to penetrate through the clouds and measure multi-layered clouds, cloud thickness, and cloud-base height. These measurements would provide a useful input to radiation computations used in the operational numerical weather prediction models, and for forecasting. High power levels, optimum modulation, data processing, and high antenna gain are used to increase the operating range, while space environment, radar tradeoffs, and power availability are considered. Preliminary, numerical calculations are made, using the specifications of an experimental system constructed at Georgia Tech. The noncoherent 94 GHz millimeter-wave radar system has a pulsed output with peak value of 1 kW. The backscatter cross section of the particles to be measured, that are present in the volume covered by the beam footprint, is also studied.

Andrawis, Madeleine Y.↗
NASA NTRS1998

Operational processing and cloud boundary detection from micro pulse lidar data

Micro Pulse Lidar (MPL) was developed at NASA Goddard Space Flight Center (GSFC) as the result of research on space-borne lidar techniques. It was designed to provide continuous, unattended observations of all significant atmospheric cloud and aerosol structure with a rugged, compact system design and the benefit of eye safety (Spinhirne 1993). The significant eye safety feature is achieved by using low pulse energies and high pulse repetition rates compared to standard lidar systems. MPL systems use a diode pumped 10 microj, 2500 Hz doubled Nd:YLF laser. In addition, a solid state Geiger mode avalanche photo diode (GAPD) photon counting detector is used allowing for quantum efficiencies approaching 70%. Other design features have previously been noted by Spinhirne (1995). Though a commercially available instrument, with nearly 20 systems operating around the world, the most extensive MPL work has come from those operated by the Atmospheric Radiation Measurement (ARM) (Stokes and Schwartz 1994) program. The diverse ability of the instrument relating to the measurement of basic cloud macrophysical structure and both cloud and aerosol radiative properties well suits the ARM research philosophy. MPL data can be used to yield many parameters including cloud boundary heights to the limit of signal attenuation, cloud scattering cross sections and optical thicknesses, planetary boundary layer heights and aerosol scattering profiles, including those into the stratosphere in nighttime cases (Hlavka et al 1996). System vertical resolution ranges from 30 m to 300 m (i.e. high and low resolution respectively) depending on system design. The lidar research group at GSFC plays an advisory role in the operation, calibration and maintenance of NASA and ARM owned MPL systems. Over the past three years, processing software and system correction techniques have been developed in anticipation of the increasing population of systems amongst the community. Datasets produced by three ARM-owned systems have served as the basis for this development. With two operating at the southern Great Plains Cloud and Radiation Testbed Site (SGP CART) since December 1993 and another at the Manus Island Atmospheric Radiation and Cloud Station (TWP ARCS) location in the tropical western Pacific since February 1997, the ARM archive contains over 4 years of observations. In addition, high resolution systems planning to come on-line at the North Slope, AK CART shortly with another scheduled to follow at the TWP ARCS-II will diversify this archive with more extensive observations.

Campbell, James R.↗
DOE OSTI2022

Radioxenon signatures of molten salt reactors

Developments of molten salt reactor (MSR) technologies are making rapid progress across the globe. These reactor designs involve properly controlling radionuclides through off-gas systems. This work examines radioxenon emissions and assesses treaty detection technology to be used for monitoring. This work also includes a sensitivity study with ORIGEN on the nuclear forensic signals possible from a MSR. Multiple Isotope Ratio Comparison (MIRC) plots are used to compare the ratios of radioxenon isotopes in an MSR to a highly enriched uranium (HEU) reactor. Finally, the results show that MSR emissions may significantly overlap with signals produced in a HEU reactor and that changing reactor operations or retaining emissions in an off-gas system can significantly shift the radioxenon signature away from the HEU pulse.

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗
DOE OSTI2022

A Strategy for NACS investment in Machine Learning

The Nuclear and Chemical Sciences (NACS) Division furnishes the expertise in the scientific areas of chemical, nuclear and isotopic sciences that are foundational in the Laboratory’s national security missions. This expertise is maintained and advanced through identification, development and application of state-of-the-art theoretical, computational and experimental methods and tools. Recent developments in artificial intelligence and machine learning (AI/ML) techniques enabled by advances in computing capabilities and widespread availability of powerful software implementations have made use of these techniques ubiquitous across both science and industry. While the scope of AI/ML applications is incredibly large and evolves very rapidly, the topics most relevant to NACS missions fall into the general category of detecting, categorizing or identifying features in large, complex datasets using either supervised or unsupervised learning. This covers both basic scientific data analysis and the development of efficient surrogate models of real-life technological systems, experimental detectors, or theoretical models. To remain at the forefront of its core scientific disciplines, NACS must both cultivate ML expertise as well as continuously explore applying this expertise to new problems or utilizing new methods. This document identifies the key areas where this support is critical and provides a strategy for investing in them.

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗
NASA NTRS2004

Clear Evidence for Fe-60 in Silicate from a Semarkona Chondrule

Fe-60 (t(sub 1/2) = 1.5 Ma) is key to understanding the sources of short-lived radionuclides in the early solar system because it is the only one among those known from meteoritic material that is produced only in stars [1]. Within the last year, it has become clear that Fe-60 was present in sulfides from primitive ordinary and enstatite chondrites in amounts sufficient to require a recent stellar input [2-5]. The sulfide data indicate an initial Fe-60/Fe-56 ratio for the early solar system of between approx. 3 10(exp -7) and approx. 1.6 10(exp -6) [2-4]. However, iron (and nickel?) in sulfides is easily mobilized by very mild heating [e.g., 6], so there is considerable uncertainty over the true initial ratio. To resolve this uncertainty, we have begun a search for evidence of Fe-60 in silicates from primitive chondrites. In olivine from type 3.0-3.1 ordinary chondrites, diffusive exchange of iron and magnesium has not occurred to any significant degree, and diffusive exchange in pyroxene is slower [7]. However, the relatively small elemental fractionation of iron from nickel in silicates, coupled with the fact that the daughter nuclide, Ni-60, makes up approx. 26 % of normal nickel, make detection of excesses of radiogenic Ni-60 very difficult. Fortunately, we have found a fine-grained radiating-pyroxene chondrule in Semarkona (LL3.0) with a very high Fe/Ni ratio that gives clear evidence of Fe-60.

Huss, G. R.↗
DOE OSTI2023

Colors of entangled two-photon absorption

Multiphoton absorption of entangled photons offers ways for obtaining unique information about chemical and biological processes. Measurements with entangled photons may enable sensing biological signatures with high selectivity and at very low light levels to protect against photodamage. In this paper, we present a theoretical and experimental study of the excitation wavelength dependence of the entangled two-photon absorption (ETPA) process in a molecular system, which provides insights into how entanglement affects molecular spectra. We demonstrate that the ETPA excitation spectrum can be different from that of classical TPA as well as that for one-photon resonant absorption (OPA) with photons of doubled frequency. These results are modeled by assuming the ETPA cross-section is governed by a two-photon excited state radiative linewidth rather than by electron-phonon interactions, and this leads to excitation spectra that match the observed results. Further, we find that the two-photon-allowed states with highest TPA and ETPA intensities have high electronic entanglements, with ETPA especially favoring states with the longest radiative lifetimes. These results provide concepts for the development of quantum light–based spectroscopy and microscopy that will lead to much higher efficiency of ETPA sensors and low-intensity detection schemes.

Science & Technology - Other Topics↗