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At least 1,099 records · Page 61
All sourcesNASA NTRSDOE OSTI
NASA NTRS2011

Coupling Between Waveguide-Fed Slot Arrays

Coupling between two waveguide-fed planar slot arrays has been investigated using full-wave analysis. The analysis employs the method-of-moments solution to the pertinent coupled integral equations for the aperture electric field of all slots. In order to compute coupling between two arrays, the input port of the first array is excited with a TE(sub 10) mode wave while the second one is match-terminated. After solving the moment method matrix equations, the aperture fields of all slots are obtained and thereby the TE(sub 10) mode wave received at the input port of the second array is determined. Coupling between two arrays is the ratio of the wave amplitude arriving in the second array port to the incident wave amplitude at the first array port. The coupling mechanism has been studied as a function of spacing between arrays in different directions, e.g. the electric field plane, the magnetic field plane, and the diagonal plane. Computed coupling values are presented for different array geometries. This work is novel since it provides a good understanding of coupling between waveguide-fed slot arrays as a function of spacing and orientation for different aperture distributions and array architectures. This serves as a useful tool for antenna design engineers and system engineers.

Rengarajan, Sembiam↗
DOE OSTI2020

One Electron Multiple Proton Transfer in Model Organic Donor–Acceptor Systems: Implications for High-Frequency EPR

EPR spectroscopy is an important spectroscopic method for identification and characterization of radical species involved in many biological reactions. The tyrosyl radical is one of the most studied amino acid radical intermediates in biology. Often in conjunction with histidine residues, it is involved in many fundamental biological electron and proton transfer processes, such as in the water oxidation in photosystem II. As biological processes are typically extremely complicated and hard to control, molecular bio-mimetic model complexes are often used to clarify the mechanisms of the biological reactions. In this work, we present theoretical calculations to investigate the sensitivity of magnetic resonance parameters to proton-coupled electron transfer events, as well as conformational substates of the molecular constructs which mimic the tyrosine-histidine (Tyr-His) pairs found in a large variety of proteins. Upon oxidation of the phenol, the Tyr analog, these complexes can perform not only one-electron one-proton transfer (EPT), but also one-electron two-proton transfers (E2PT). It is shown that in aprotic environment the g X -components of the electronicg-tensor are extremely sensitive to the first proton transfer from the phenoxyl oxygen to the imidazole nitrogen (EPT product), leading to a significant increase of the g X -value of up to 0.003, but are not sensitive to the second proton transfer (E2PT). In the latter case, the change of the g X -value is much smaller (ca. 0.0001), which is too small to be distinguished even by high-frequency EPR. The 14 N hyperfine values are also too similar to allow differentiation between the different protonation states in EPT and E2PT. The magnetic resonance parameters were also calculated as a function of the rotation angles around single bonds. It was demonstrated that rotation of the phenoxyl group results in large positive changes (> 0.001) in the g X -values. Analysis of the data reveals that the main source of these changes is related to the strength of the H-bond between phenoxyl oxygen and the proton(s) on N 1 and N 2 positions of the imidazole.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
NASA NTRS2023

Electron Acceleration and Heating during Magnetic Reconnection in the Earth's Quasi-parallel Bow Shock

We perform a 2.5-dimensional particle-in-cell simulation of a quasi-parallel shock, using parameters for the Earth's bow shock, to examine electron acceleration and heating due to magnetic reconnection. The shock transition region evolves from the ion-coupled reconnection dominant stage to the electron-only reconnection dominant stage, as time elapses. The electron temperature enhances locally in each reconnection site, and ion-scale magnetic islands generated by ion-coupled reconnection show the most significant enhancement of the electron temperature. The electron energy spectrum shows a power law, with a power-law index around 6. We perform electron trajectory tracing to understand how they are energized. Some electrons interact with multiple electron-only reconnection sties, and Fermi acceleration occurs during multiple reflections. Electrons trapped in ion-scale magnetic islands can be accelerated in another mechanism. Islands move in the shock transition region, and electrons can obtain larger energy from the in-plane electric field than the electric potential in those islands. These newly found energization mechanisms in magnetic islands in the shock can accelerate electrons to energies larger than the achievable energies by the conventional energization due to the parallel electric field and shock drift acceleration. This study based on the selected particle analysis indicates that the maximum energy in the nonthermal electrons is achieved through acceleration in ion-scale islands, and electron-only reconnection accounts for no more than half of the maximum energy, as the lifetime of sub-ion-scale islands produced by electron-only reconnection is several times shorter than that of ion-scale islands.

Solar magnetic reconnection↗
DOE OSTI2022

Coherent helicity-dependent spin-phonon oscillations in the ferromagnetic van der Waals crystal CrI3

Abstract The discovery of two-dimensional systems hosting intrinsic magnetic order represents a seminal addition to the rich landscape of van der Waals materials. CrI 3 is an archetypal example, where the interdependence of structure and magnetism, along with strong light-matter interactions, provides a new platform to explore the optical control of magnetic and vibrational degrees of freedom at the nanoscale. However, the nature of magneto-structural coupling on its intrinsic ultrafast timescale remains a crucial open question. Here, we probe magnetic and vibrational dynamics in bulk CrI 3 using ultrafast optical spectroscopy, revealing spin-flip scattering-driven demagnetization and strong transient exchange-mediated interactions between lattice vibrations and spin oscillations. The latter yields a coherent spin-coupled phonon mode that is highly sensitive to the driving pulse’s helicity in the magnetically ordered phase. Our results elucidate the nature of ultrafast spin-lattice coupling in CrI 3 and highlight its potential for applications requiring high-speed control of magnetism at the nanoscale.

36 MATERIALS SCIENCE↗
DOE OSTI2026

Proximity Magnetism in Mn(Bi,Sb) 2 Te 4 –(Bi,Sb) 2 Te 3 /MnTe Natural Heterostructures

Magnetic topological insulators and their heterostructures provide significant opportunities to couple band topology with a nontrivial spin configuration for enhanced spintronic device performance, as well as designing magnetoelectric systems and functionalities. We find that Mn interdiffusion from MnTe when interfaced with (Bi,Sb) 2 Te 3 stabilizes as self-organized Mn(Bi,Sb) 2 Te 4 septuple lamellae among alternating (Bi,Sb) 2 Te 3 quintuple layers, as observed using scanning transmission electron microscopy and depth-sensitive polarized neutron reflectometry. We further demonstrate a valuable combination of magnetic and topological orders in these naturally formed Mn(Bi,Sb) 2 Te 4 –(Bi,Sb) 2 Te 3 heterostructures, which are exchange-coupled with MnTe. Magnetotransport experiments and quantum magnetism simulations reveal that, above its own Néel temperature T N ∼ 20 K, Mn(Bi,Sb) 2 Te 4 mediates the exchange field leading to an anomalous Hall effect at the (Bi,Sb) 2 Te 3 /MnTe interface, with an enhanced interfacial T N exceeding 200 K, approaching that of the bulk MnTe. This magnetic interface, in turn, allows a robust and deterministic spin–orbit torque switching without an external magnetic field at a low critical current density of 3 × 10 5 A cm –2 . The antiferromagnetically coupled architecture of Mn(Bi,Sb) 2 Te 4 –(Bi,Sb) 2 Te 3 /MnTe, featuring magnetic and topological proximity effects across a chalcogenide backbone, is rich in fundamental interface physics and holds the potential for practical applications in spintronics.

magnetic topological insulator↗
DOE OSTI2025

Magneto-optical Evidence of the Tilting Effect in Coupled Weyl Bands

Theories have revealed the universality of the band tilting effect in topological Weyl semimetals (WSMs) and its implications for the material physical properties. However, the experimental identification of tilted Weyl bands remains less explored. Here, we report the magneto-optical evidence of the tilting effect in WSM niobium phosphide. Specifically, we observe Landau level transitions with rich features that are well reproduced within a model of coupled tilted Weyl points. Our analysis indicates that the tilting effect relaxes the selection rules and leads to transitions that would otherwise be forbidden in the non-tilt case. Additionally, we observe unconventional interband transitions with flat and negative magnetic field dispersions, highlighting the importance of coupling between Weyl points. Our results not only emphasize the significance of the tilting effect in the optical responses of WSMs but also demonstrate magneto-optics as an effective tool for probing the tilting effect in electronic band structures.

77 NANOSCIENCE AND NANOTECHNOLOGY↗
DOE OSTI2022

NaCo 2 (SeO 3 ) 2 (OH): competing magnetic ground states of a new sawtooth structure with 3d 7 Co 2+ ions

While certain magnetic sublattices have long been known theoretically to give rise to emergent physics via competing magnetic interactions and quantum effects, finding such configurations in real materials is often deeply challenging. Here we report the synthesis and characterization of a new such material, NaCo 2 (SeO 3 ) 2 (OH) which crystallizes with a highly frustrated sublattice of sawtooth Co 2+ chains. Single crystals of NaCo 2 (SeO 3 ) 2 (OH) were synthesized using a low-temperature hydrothermal method. X-ray single crystal structure analysis reveals that the material crystallizes in orthorhombic space group of Pnma (no. 62). Its crystal structure exhibits one-dimensional chains of corner-sharing isosceles triangles that are made of two crystallographically distinct 3d 7 Co 2+ sites (Co(1) and Co(2)). The chains run along the b-axis and are interconnected via [SeO 3 ] groups to form a three-dimensional structure mediating super-exchange interactions. The temperature dependent magnetization data show a ferromagnetic-like (FM) transition at 11 K (T 1 ) followed by an antiferromagnetic (AFM) transition at about 6 K (T 2 ). Neutron-powder diffraction measurements reveal that at T 1 = 11 K only the Co(2) site orders magnetically, forming ferromagnetic zigzag chains along the b-axis. Below T 2 = 6 K, both Co(1) and Co(2) sites order in a nearly orthogonal configuration, with Co(1) moments lying inside the plane of the sawtooth chain while Co(2) moments cant out of the plane. The canting of the magnetic moments leads to a net ferromagnetic component along b-axis, parallel to the chain direction. The ordered moments are fully compensated in the ac-plane. Inelastic neutron scattering measurements reveal crystal field excitations that are consistent with the presence of a spin–orbital entangled pseudo-spin state J eff = 1/2 for the Co 2+ ions. Low-energy spin-wave excitations are observed below the second magnetic transition. The analysis of powder excitation spectrum suggests complex exchange interactions that go beyond a Heisenberg Hamiltonian model with nearest neighbor couplings. Our results demonstrate the richness of the magnetic properties of sawtooth-type structures and encourage the study of similar structures with different oxyanion groups.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2026

Magnetism and magnetoelastic effect in the two-dimensional van der Waals multiferroic CuCrP 2 ⁢S 6

Here, we report a magnetic and neutron diffraction study on the ground state magnetism and field evolution of single-crystal van der Waals multiferroic CuCrP 2 ⁢S 6 . The ordered moments align along the 𝑏 axis in the "𝐴-type" antiferromagnetic configuration with a spin-flop transition along the same direction. Field application along 𝑎 introduces a smooth transition to a fully polarized ferromagnetic state via in-plane spin rotation. These findings resolve the ambiguity of the ground state magnetization direction in CuCrP 2 ⁢S 6 and uncover its field responses, providing a firm basis for future magnetoelectric study. A magnetoelastic coupling effect connecting the interlayer spacing and the magnetic order was further revealed, highlighting the out-of-plane strain as an effective control knob for tuning magnetism both in this system and in related van der Waals magnets.

Guo, Jiasen [Oak Ridge National Laboratory (ORNL),↗
NASA NTRS2003

A 10 Kelvin Magnet for Space-Flight ADRs

Future NASA missions will include detectors cooled by adiabatic demagnetization refrigerators (ADRs) coupled with mechanical cryocoolers. A lightweight, low-current 10 Kelvin magnet would allow the interface between these devices to be at temperatures as high as 10 Kelvin, adding flexibility to the instrument design. We report on the testing of a standard-technology Nb3Sn magnet and the development of a lightweight, low-current 10 Kelvin magnet. We also discuss the outlook for flying a 10 Kelvin magnet as part of an ADR system.

Tuttle, James↗
DOE OSTI2025

Solenoidal Fields from Permanent Magnets for a Polarized Electron Preinjector

This technical note describes the design of a compact focusing solenoid constructed from permanent bar magnets, intended for the low-energy section of a spin-polarized electron injector. Typically, quadrupole triplets provide appropriate focusing for the low-energy spin rotator section; however, their large footprint precludes the insertion of sufficient beam diagnostics. The primary motivation of this study is to provide beam focusing while preserving the vertical spin orientation of the electron beam. We propose a solenoidal field composed of multiple permanent magnets arranged to naturally yield a zero longitudinal magnetic field integral ($\int B_zdz = 0$). This design serves as a compact, passive, and non-coupling alternative to traditional quadrupole triplets. We present the magnet arrangement, field calculation methodology, spin tracking simulations using space charge codes, and calculations demonstrating that the required field strength is achievable.

43 PARTICLE ACCELERATORS↗
NASA NTRS1976

Microscale 'Alfven waves' in the solar wind at 1 AU

Data obtained by IMP 1 about interplanetary plasma and magnetic-field fluctuations on a scale of one hour are analyzed. It is found that linearly and circularly polarized Alfven waves were rarely present. Fluctuations having most of the characteristics of large-amplitude 'Alfven waves' and which were observed to be moving away from the sun nearly along the magnetic-field direction are shown not to have been pure transverse Alfven waves since they were accompanied by nonzero fluctuations in the magnetic-field intensity. It is suggested that the fluctuations may have been nonlinear elliptically polarized Alfven waves coupled to the fast mode and moving through a magnetic field that is nonuniform on a scale not exceeding about 0.01 AU.

Burlaga, L. F.↗
DOE OSTI2021

Nitride-Oxide-Metal Heterostructure with Self-Assembled Core–Shell Nanopillar Arrays: Effect of Ordering on Magneto-Optical Properties

Magneto-optical (MO) coupling incorporates photon-induced change of magnetic polarization that can be adopted in ultrafast switching, optical isolators, mode convertors, and optical data storage components for advanced optical integrated circuits. However, integrating plasmonic, magnetic, and dielectric properties in one single material system poses challenges since one natural material can hardly possess all these functionalities. Here, co-deposition of a three-phase heterostructure composed of a durable conductive nitride matrix with embedded core–shell vertically aligned nanopillars, is demonstrated. Additionally, the unique coupling between ferromagnetic NiO core and atomically sharp plasmonic Au shell enables strong MO activity out-of-plane at room temperature. Further, a template growth process is applied, which significantly enhances the ordering of the nanopillar array. The ordered nanostructure offers two schemes of spin polarization which result in stronger antisymmetry of Kerr rotation. The presented complex hybrid metamaterial platform with strong magnetic and optical anisotropies is promising for tunable and modulated all-optical-based nanodevices.

36 MATERIALS SCIENCE↗
DOE OSTI2022

Electron transport in a collisional plasma with multiple ion species in the presence of a magnetic field

The classical work of Braginskii [Zh. Eksp. Teor. Fiz. 33, 459 (1957)] published almost 65 years ago was the first to provide a complete, closed fluid description of a weakly coupled, fully ionized, collisional plasma immersed in a magnetic field. While this fact is not widely known or appreciated, the Braginskii expressions for the electron transport coefficients can under- or overestimate the said coefficients by up to a factor of two for the electron Hall parameter of order unity (with the Hall parameter being proportional to the electron gyro-frequency over the electron–ion collision frequency) and can provide incorrect Hall-parameter scalings for its large values. Starting with the work of Epperlein and Haines [Phys. Fluids 29, 1029 (1986)], several papers attempted to correct the Braginskii electron results with varying degrees of success. Herein, we present our own effort with a hope to finally put this problem to rest.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2025

Room-temperature in-plane ferromagnetism in Co-substituted Fe 5 GeTe 2 investigated by magnetic x-ray spectroscopy and microscopy

The exploration of two-dimensional (2D) van der Waals ferromagnets has revealed intriguing magnetic properties with significant potential for spintronics applications. In this study, we examine the magnetic properties of Co-doped Fe 5 GeTe 2 using x-ray photoemission electron microscopy (XPEEM) and x-ray magnetic circular dichroism (XMCD), complemented by density functional theory calculations. Our XPEEM measurements reveal that the Curie temperature (T c ) of a bilayer of (Co x Fe 1-x ) 5-δ GeTe 2 (with x = 0.28) reaches ∼300 K—a notable enhancement over most 2D ferromagnets in the ultrathin limit. Interestingly, the T c shows only a small dependence on film thickness (bulk T c ≈ 340 K), in line with the observed in-plane (IP) magnetic anisotropy and robust IP exchange coupling. XMCD measurements indicate that the spin moments for both Fe and Co are significantly reduced compared to the theoretical values. These insights highlight the potential of Co-doped Fe 5 GeTe 2 for stable, high-temperature ferromagnetic applications in 2D materials.

(Co0.28Fe0.72)5GeTe2↗
DOE OSTI2021

Imbalanced spin coupling in the copper hexamer compounds A 2 Cu 3 O(SO 4 ) 3 ( A 2 = Na 2 , NaK, K 2 )

The minerals A 2 Cu 3 O(SO 4 ) 3 (A 2 = Na 2 ,NaK,K 2 ) constitute quantum spin systems with copper hexamers as basic structural units. Strong intrahexamer spin couplings give rise to an effective triplet ground state. Weak interhexamer spin couplings are responsible for two-dimensional long-range magnetic order in the (b,c) plane below 3.0 < T c < 4.7K. We investigated the magnetic excitations at T = 1.5 K by inelastic neutron scattering (INS). Furthermore, the INS technique was based on the observation of wave vector dependent slices in reciprocal space in order to selectively probe the magnetic signals in different Brillouin zones with different weight. Due to the imbalance of the spin couplings, the data analysis relies on a model in which the interhexamer spin couplings are treated perturbatively on top of the exact S = 1 ground state. The interhexamer spin couplings turn out to be ferromagnetic.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2021

Topological Hall effect in magnetic topological insulator films

Geometric Berry phase can be induced either by spin–orbit coupling, giving rise to the anomalous Hall effect in ferromagnetic materials, or by chiral spin texture, such as skyrmions, leading to the topological Hall effect. Recent experiments have revealed that both phenomena can occur in topological insulator films with magnetic doping, thus providing us with an intriguing platform to study the interplay between these two phenomena. In this work, we report on a numerical simulation of the anomalous Hall and topological Hall effects in a four-band model that can properly describe the quantum well states in the magnetic topological insulator films by combining Landauer–Büttiker formula and the iterative Green’s function method. Our numerical results suggest that spin–orbit coupling in this model plays a different role in the quantum transport in the clean and disordered limits. In the clean limit, spin–orbit coupling mainly influences the longitudinal transport but does not have much effect on topological Hall conductance. In the disordered limit, the longitudinal transport is determined by disorder scattering and spin–orbit coupling is found to affect strongly the topological Hall conductance. Here, this sharp contrast unveils a dramatic interplay between spin–orbit coupling and disorder effect in topological Hall effect in magnetic topological insulator systems.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2020

SU(3) Topology of Magnon-Phonon Hybridization in 2D Antiferromagnets

Magnon-phonon hybrid excitations are studied theoretically in a two-dimensional antiferromagnet with an easy axis normal to the plane. In this work, we show that two magnon bands and one phonon band are intertwined by the magnetoelastic coupling through a nontrivial SU(3) topology, which can be intuitively perceived by identifying a skyrmion structure in the momentum space. Our results are insensitive to lattice details and generally applicable to two-dimensional antiferromagnets. We show this by developing a continuum theory as the long-wavelength approximation to the tight-binding model. The theoretical results can be probed by measuring the thermal Hall conductance as a function of the temperature and the magnetic field. We envision that the magnetoelastic coupling in antiferromagnets can be a promising venue in search of various topological excitations, which cannot be found in magnetic or elastic models alone.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
NASA NTRS2013

External Magnetic Field Reduction Techniques for the Advanced Stirling Radioisotope Generator

Linear alternators coupled to high efficiency Stirling engines are strong candidates for thermal-to-electric power conversion in space. However, the magnetic field emissions, both AC and DC, of these permanent magnet excited alternators can interfere with sensitive instrumentation onboard a spacecraft. Effective methods to mitigate the AC and DC electromagnetic interference (EMI) from solenoidal type linear alternators (like that used in the Advanced Stirling Convertor) have been developed for potential use in the Advanced Stirling Radioisotope Generator. The methods developed avoid the complexity and extra mass inherent in data extraction from multiple sensors or the use of shielding. This paper discusses these methods, and also provides experimental data obtained during breadboard testing of both AC and DC external magnetic field devices.

Thermoelectric Power Generation↗