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At least 1,099 records · Page 61
All sourcesNASA NTRSDOE OSTI
NASA NTRS1973

Lunar rocks as meteoroid detectors

About 5000 microcraters on seven lunar rocks recovered during the Apollo 12 mission have been systematically studied using a stereomicroscope. Based on comparisons with laboratory cratering experiments, at least 95 percent of all millimeter sized craters observed were formed by impacts in which the impact velocity exceeded 10 km/s. The dynamics of particle motion near the moon and the distribution of microcraters on the rocks require an extralunar origin for these impacting particles. The microcrater population on at least one side of all rocks studied was in equilibrium for millimeter sized craters; i.e., statistically, craters a few millimeters in diameter and smaller were being removed by the superposition of new craters at the same rate new craters were being formed. The population of craters on such a surface is directly related to the total population of particles impacting that surface. Crater size distribution data together with an experimentally determined relationship between the crater size and the physical parameters of the impacting particle, yield the mass distribution of interplanetary dust at 1 AU.

Hartung, J. B.↗
NASA NTRS1998

Global Retrieval of Cloud Particle Size and Optical Thickness Using ISCCP Data

The primary thrust of this investigation is to develop an algorithm to retrieve cloud particle sizes using ISCCP data. The research under this grant has been successful in obtaining initial results of global distribution of ice-particle sizes. Further research about possible problems caused by nonsphericity of ice particle sizes is currently underway. An algorithm of retrieving ice-cloud particle sizes using ISCCP CX data has been developed. The first survey of ice-particle size in a near-global scale has been completed. Comparison with in situ measurements of ice crystal sizes during FIRE I shows good agreement. The initial results show that the global mean size of ice crystals (De) is about 60 micron. This result is consistent with the range of in situ measurements all over the world if definitions of effective particle size are unified (see next section). The survey also shows that there is no distinct difference of ice-particle sizes between continental and maritime ice-clouds. There are many different definitions of effective particle size used in ice-cloud research. Simple comparisons between values of in situ measurement and satellite remote sensing are misleading and may lead to incorrect conclusions. We reviewed different definitions of effective particle sizes used in the literature and compared their relative magnitudes.

Welch, Ronald M.↗
NASA NTRS2018

Sedimentation Efficiency of Condensation Clouds in Substellar Atmospheres

Condensation clouds in substellar atmospheres have been widely inferred from spectra and photometric variability. Up until now, their horizontally averaged vertical distribution and mean particle size have been largely characterized using models, one of which is the eddy diffusion-sedimentation model from Ackerman and Marley that relies on a sedimentation efficiency parameter, f(sub sed), to determine the vertical extent of clouds in the atmosphere. However, the physical processes controlling the vertical structure of clouds in substellar atmospheres are not well understood. In this work, we derive trends in f(sub sed) across a large range of eddy diffusivities (K (sub zz) ), gravities, material properties, and cloud formation pathways by fitting cloud distributions calculated by a more detailed cloud microphysics model. We find that f(sub sed) is dependent on K (sub zz), but not gravity, when K (sub zz) is held constant. f(sub sed) is most sensitive to the nucleation rate of cloud particles, as determined by material properties like surface energy and molecular weight. High surface energy materials form fewer, larger cloud particles, leading to large f(sub sed) (>1), and vice versa for materials with low surface energy. For cloud formation via heterogeneous nucleation, f(sub sed) is sensitive to the condensation nuclei flux and radius, connecting cloud formation in substellar atmospheres to the objects' formation environments and other atmospheric aerosols. These insights could lead to improved cloud models that help us better understand substellar atmospheres. For example, we demonstrate that f(sub sed) could increase with increasing cloud base depth in an atmosphere, shedding light on the nature of the brown dwarf L/T transition.

brown dwarfs; planets and satellites: atmospheres↗
NASA NTRS1982

Time variations of aerosols in the stratosphere following Mount St. Helens eruptions

Samples of stratospheric aerosols collected with U-2 aircraft for several months following the first three major eruptions of Mount St. Helens were analyzed for ash and liquid acid content. Ash grain sizes and compositions vary depending on collection altitude, location within the drifting cloud, and days following their injection. s computers Size distributions of ash particles vary with altitude. Generally small particles are depleted more rapidly at low altitudes (12 km) than at higher altitudes (17-18 km). Although samples collected 1 day after the first eruption of May 18, 1980, were dry, flow marks on the aircraft indicated parts of the cloud contained heavy acid concentrations. Indeed, all other samples obtained within 1 to 4 days after later eruptions (May 25 and June 12, 1980) were covered with copious amounts of liquid acid. Proportions of liquid to ash varied considerably depending on sampling location and cloud age. Because the acid-coated ash globules were large, they rapidly fell from the stratosphere until, by late June 1980, only a residue of acid droplets remained. Size distributions and concentrations of these droplets varied considerably.

Farlow, N. H.↗
NASA NTRS1996

An Experimental Study of Atmospheric Homogeneous Nucleation: Cluster Growth and Gas-Particle Reactions of H2SO4

The work proposed on this project included both field and laboratory studies. The laboratory studies were to consist of measurements of H2SO4 uptake and evaporation from aerosols of varying chemical composition, while the field component would include measurements of H2SO4 and other compounds which would be conducted as part of a large field campaign. By chance, the opportunity to conduct such an H2SO4/aerosol/ultrafine particle study in conjunction with an OH intercomparison/photochemistry study became available very early in this project (September 1993). This study was conducted at Caribou, Colorado in conjunction with several other groups from NCAR, NOAA and a number of universities. Our group measured OH, H2SO4, SO2, and H20, while Dr. McMurfy's group measured ultrafine particles, and total particle number and size distribution. In addition measurements of HO2/RO2, O3, NO, NO2, NO(y) CO, hydrocarbons, CH2O, and other chemical compounds and meteorological parameters were performed by the other participants and a new laser oblation/mass spectrometry technique was also employed by the NOAA Aeronomy Laboratory to study aerosol composition. The study of aerosol production and growth in conjunction with photochemical measurements is highly advantageous because particle growth precursors such as H2SO4.or MSA are formed by OH initiated sulfur oxidation. The large number of hydrocarbon measurements included in this study were also important in understanding particle growth.

Eisele, F. L.↗
NASA NTRS2003

Sunlight Transmission through Desert Dust and Marine Aerosols: Diffuse Light Corrections to Sun Photometry and Pyrheliometry

Desert dust and marine aerosols are receiving increased scientific attention because of their prevalence on intercontinental scales and their potentially large effects on Earth radiation and climate, as well as on other aerosols, clouds, and precipitation. The relatively large size of desert dust and marine aerosols produces scattering phase functions that are strongly forward- peaked. Hence, Sun photometry and pyrheliometry of these aerosols are more subject to diffuse-light errors than is the case for smaller aerosols. Here we quantify these diffuse-light effects for common Sun photometer and pyrheliometer fields of view (FOV), using a data base on dust and marine aerosols derived from (1) AERONET measurements of sky radiance and solar beam transmission and (2) in situ measurements of aerosol layer size distribution and chemical composition. Accounting for particle non-sphericity is important when deriving dust size distribution from both AERONET and in situ aerodynamic measurements. We express our results in terms of correction factors that can be applied to Sun photometer and pyrheliometer measurements of aerosol optical depth (AOD). We find that the corrections are negligible (less than approximately 1% of AOD) for Sun photometers with narrow FOV (half-angle eta less than degree), but that they can be as large as 10% of AOD at 354 nm wavelength for Sun photometers with eta = 1.85 degrees. For pyrheliometers (which can have eta up to approximately 2.8 degrees), corrections can be as large as 16% at 354 nm. We find that AOD correction factors are well correlated with AOD wavelength dependence (hence Angstrom exponent). We provide best-fit equations for determining correction factors from Angstrom exponents of uncorrected AOD spectra, and we demonstrate their application to vertical profiles of multiwavelength AOD.

Russell, P. B.↗
NASA NTRS1977

Application of modified Twomey techniques to invert lidar angular scatter and solar extinction data for determining aerosol size distributions

Polarization properties of the angularly scattered laser light from a volume of air are used to determine the size distribution of the aerosol particles within the volume by the use of appropriate inversion techniques. Similar techniques are employed to determine a mean size distribution of the particulates within a vertical column through the atmosphere from determinations of the aerosol optical depth as a function of wavelength. In both of these examples, a modification of an inversion technique originally described by Twomey has been employed. Details of this method are presented as well as results from actual measurements employing bistatic lidar and solar radiometer.

Herman, B. M.↗
NASA NTRS1976

Diffuse band extinction and polarization in core-mantle grains

Diffuse band shapes in both extinction and polarization are calculated for interstellar core-mantle particles for varying size distributions of mantle thickness. It is shown that no matter whether the source of the bands is in the silicate cores or the accreted icy mantles, the polarization shapes are highly asymmetric for all mantle thicknesses. The extinction-band shapes are significantly less asymmetric, although the effect is clearly present. The only apparent possibility for producing symmetric band shapes in the dust grains is in very small bare particles in interstellar space which, if they are aligned and produce the 2200-A band, must exhibit a strong polarization effect in this region.

Greenberg, J. M.↗
NASA NTRS1986

Measurements of precipitating atmosphere by the MU radar

Sensitive VHF Doppler radars have the capability to detect echoes from precipitation particles as well as refractive index irregularities. Researchers used the middle and upper (MU) atmosphere radar at Shigaraki, Japan for tropospheric observations of precipitating atmosphere. They detected precipitation motions simultaneously with the ambient air motion and showed the capabilities of the MU radar in investigating mesoscale structures of meteorological phenomena such as air precipitation motions within a cold frontal system. More recently, a direct method for deducing the drop size distribution of precipitation particles was developed using Doppler spectra of the MU radar. This method is free from errors inherent in conventional measurements using microwave Doppler spectra. Meteorological microwave radar data are also utilized for monitoring vertical and horizontal structures of precipitation.

Wakasugi, K.↗
NASA NTRS1985

A review of contamination issues associated with an orbiting Space Station external environment

Techniques for measuring, modeling, and limiting the effluent contamination of external spacecraft and instrument surfaces are reviewed, with an emphasis on their application to the Space Station. The major factors addressed by contamination studies are outlined; typical contamination sources are characterized; the critical measurement parameters are defined (molecular column density, background spectral intensity from UV to IR, particle size and velocity distribution, molecular deposition on ambient and cryogenic surfaces, molecular return flux for gaseous species, particulate deposition on surfaces, and optical-surface degradation); and measurement instrumentation is described. Contamination limits for quiescent operation periods of the Space Station are proposed, including column density 10 to the 11th/sq cm for H2O + CO2, 10 to the 13th/sq cm for O2 + N2, and 10 to the 10th/sq cm for other species; particle release no greater than 15-micron particle/orbit/0.00001 sr FOV for a 1-m telescope, and surface deposition 4 pg/sq cm sec for 298-K surfaces and 10 pg/sq cm sec for 4-K surfaces.

Smith, A. C.↗
DOE OSTI2021

Simultaneous imaging of two-phase velocities in particle-laden flows by two-color optical phase discrimination

In this Letter, we present a particle image/tracking velocimetry (PIV/PTV) technique for simultaneous velocity measurement of both fluid and particle phases, adopting newly developed optical phase discrimination methods and novel optical particles. Spherical acrylic (PMMA) particles of diameter ∼ <#comment/> O ( 100 µ <#comment/> m ) were used as the particle phase, while fine B A M : E u 2 + phosphors of diameter ∼ <#comment/> O ( 1 µ <#comment/> m ) were used as the fluid tracer. Under Nd:YAG 355 nm laser excitation, both the laser-induced fluorescence (LIF) from PMMA and laser-induced phosphorescence (LIP) from B A M : E u 2 + provided sufficiently strong signals for PIV imaging with two non-intensified cameras and were clearly separable for phase discrimination using spectral filters and temporal profiles. The advantages of the PIV/PTV method include the relatively low cost of B A M : E u 2 + phosphors, high sphericity and narrow size distribution of PMMA particles with LIF emission, and direct optical discrimination eliminating artifacts, while requiring much less computational capacity for PIV/PTV processing of complex particle-laden flows.

Bi, Xiaopeng (ORCID:0000000190847325)↗
DOE OSTI2020

The Role of Ice Splintering on Microphysics of Deep Convective Clouds Forming Under Different Aerosol Conditions: Simulations Using the Model With Spectral Bin Microphysics

Observations during the Ice in Clouds Experiment-Tropical (ICE-T) field experiment show that the ice particles concentration in a developing deep convective clouds at the level of T = -15 °C reached about 500 L -1 , that is, many orders higher than that of ice-nucleating particle. To simulate microphysics of these clouds, the 2-D Hebrew University Cloud model (HUCM) with spectral bin microphysics was used in which two main types of ice multiplication mechanisms were included in addition to the Hallet-Mossop mechanism. In the first ice multiplication mechanism ice splinters form by drop freezing and drop-ice collisions. Ice multiplication of this type dominates during developing stage of cloud evolution, when liquid water content is significant. At later stage when clouds become nearly glaciated, ice crystals are produced largely by ice splintering during ice-ice collisions (the second ice multiplication mechanism). Simulations show that droplet size distributions, as well as size distributions of ice particles, agree well with the measurements during ICE-T. Simulations with different cloud condensation nuclei concentrations show the existence of the “optimum” cloud condensation nuclei concentration (or droplet concentration), at which concentration of ice splinters reaches maximum. In these simulations ice nucleation caused by the direct formation of ice crystals upon ice-nucleating particles, as well as the Hallett-Mossop process, has a negligible contribution to the ice crystal concentration.

54 ENVIRONMENTAL SCIENCES↗
NASA NTRS1982

The Halley dust model

The properties of dust ejecta from Comet Halley are studied on the basis of (a) evidence from the comet's past apparitions and (b) analogy with recent, physically similar comets. Specifically discussed are the light curve and spectrum, discrete phenomena in the head, the physical properties of the nucleus (size, albedo, rotation, surface temperature, and morphology), and an interaction between the nucleus and dust atmosphere. Also reviewed are constraints on the size and mass distributions of dust particles, information on submicron-size and submillimeter-size grains from the comet's dust tail and antitail, and the apparent existence of more than one particle type. Similarities between the jet patterns of Halley and the parent comet of the Perseid meteor stream are depicted, and effects of the surface heterogeneity (discrete active regions) on the dust flow are assessed. Current dust models for Halley are summarized and the existence of short-term variations in the dust content in the comet's atmosphere is suggested.

Sekanina, Z.↗
DOE OSTI2023

Understanding and control of Zener pinning via phase field and ensemble learning

Zener pinning refers to the dispersion of fine particles which influences grain size distribution via movement of grain boundaries in a polycrystalline material. Grain size distribution in polycrystals has a significant impact on their properties including physical, chemical, mechanical, and optical to name a few. We explore the use of Phase-field modeling and machine-learning techniques to understand and improve the control of grain size distribution via Zener pinning in polycrystalline materials. We develop a machine learning model that determines the relative importance of various parameters to exercise microstructure control via Zener pinning. Our workflow combines high-throughput phase-field simulations and machine learning to address the computational bottlenecks associated with large-scale simulations as well as identify features necessary for microstructure control in polycrystals. A random forest (RF) regression model was developed to predict grain sizes based on five Phase-field model parameters, achieving an average prediction error of 0.72 nm for the training data and 1.44 nm for the test data. The importance of the input parameters is analyzed using the SHapley Additive exPlanations (SHAP) approach which reveals that diffusivity, volume fraction, and particle diameter are the most important parameters in determining the final grain size. These findings will allow us to select the best second-phase particles, optimize grain size distributions and thus design microstructures with the desired properties. The developed method is a highly versatile and generalizable approach that can be used to assess the combined effects of individual features in the presence of multiple variables.

36 MATERIALS SCIENCE↗
NASA NTRS1992

Extinction and scattering in the Orion Nebula - Comparison of optical and VLA 21 centimeter studies

We have compared VLA 21 cm continuum maps of M42 with extinction-corrected H-beta images and found that much of M42 has an excess of H-beta surface brightness. This is interpreted as reflection by particles lying close to the principal ionization front. Comparison of column densities of H I near M42 and extinction (C(H-beta)) indicates an excellent area-by-area correlation, establishing that most of the extinction in M42 arises in the neutral lid that lies on the near side of the nebula. A more quantitative comparison of (C(H-beta)) and N(H I), the column density, is consistent with this conclusion and indicates a dust scattering cross section per hydrogen atom that is similar to the value for the general interstellar medium. The usual model for extinction in the Trapezium region is that it occurs very near the stars and produces an anomalous reddening curve through modification of the nature or size distribution of the particles. These new results question the basic assumptions and conclusions of that model.

O'Dell, C. R.↗
DOE OSTI2021

Towards replacing physical testing of granular materials with a Topology-based Model

In the study of packed granular materials, the performance of a sample (e.g., the detonation of a high-energy explosive) often correlates to measurements of a fluid flowing through it. The “effective surface area,” the surface area accessible to the airflow, is typically measured using a permeametry apparatus that relates the flow conductance to the permeable surface area via the Carman-Kozeny equation. This equation allows calculating the flow rate of a fluid flowing through the granules packed in the sample for a given pressure drop. However, Carman-Kozeny makes inherent assumptions about tunnel shapes and flow paths that may not accurately hold in situations where the particles possess a wide distribution in shapes, sizes, and aspect ratios, as is true with many powdered systems of technological and commercial interest. To address this challenge, we replicate these measurements virtually on micro-CT images of the powdered material, introducing a new Pore Network Model based on the skeleton of the Morse-Smale complex. Pores are identified as basins of the complex, their incidence encodes adjacency, and the conductivity of the capillary between them is computed from the cross-section at their interface. We build and solve a resistive network to compute an approximate laminar fluid flow through the pore structure. Here, we provide two means of estimating flow-permeable surface area: (i) by direct computation of conductivity, and (ii) by identifying dead-ends in the flow coupled with isosurface extraction and the application of the Carman-Kozeny equation, with the aim of establishing consistency over a range of particle shapes, sizes, porosity levels, and void distribution patterns.

36 MATERIALS SCIENCE↗
NASA NTRS2012

Improvement of Aerosol Optical Depth Retrieval from MODIS Spectral Reflectance over the Global Ocean Using New Aerosol Models Archived from AERONET Inversion Data and Tri-axial Ellipsoidal Dust Database

New over-ocean aerosol models are developed by integrating the inversion data from the Aerosol Robotic Network (AERONET) sun/sky radiometers with a database for the optical properties of tri-axial ellipsoid particles. The new aerosol models allow more accurate retrieval of aerosol optical depth (AOD) from the Moderate Resolution Imaging Spectroradiometer (MODIS) in the case of high AOD (AOD greater than 0.3). The aerosol models are categorized by using the fine-mode fraction (FMF) at 550 nm and the singlescattering albedo (SSA) at 440 nm from the AERONET inversion data to include a variety of aerosol types found around the globe. For each aerosol model, the changes in the aerosol optical properties (AOPs) as functions of AOD are considered to better represent aerosol characteristics. Comparisons of AODs between AERONET and MODIS for the period from 2003 to 2010 show that the use of the new aerosol models enhances the AOD accuracy with a Pearson coefficient of 0.93 and a regression slope of 0.99 compared to 0.92 and 0.85 calculated using the MODIS Collection 5 data. Moreover, the percentage of data within an expected error of +/-(0.03 + 0.05xAOD) is increased from 62 percent to 64 percent for overall data and from 39 percent to 51 percent for AOD greater than 0.3. Errors in the retrieved AOD are further characterized with respect to the Angstrom exponent (AE), scattering angle, SSA, and air mass factor (AMF). Due to more realistic AOPs assumptions, the new algorithm generally reduces systematic errors in the retrieved AODs compared with the current operational algorithm. In particular, the underestimation of fine-dominated AOD and the scattering angle dependence of dust-dominated AOD are significantly mitigated as results of the new algorithm's improved treatment of aerosol size distribution and dust particle nonsphericity.

aerosol optical depth↗