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At least 1,099 records · Page 61
All sourcesNASA NTRSDOE OSTI
NASA NTRS2002

Photonic Bandgaps in Mie Scattering by Concentrically Stratified Spheres

The Mie formulation for homogeneous spheres is generalized to handle core/shell systems and multiple concentric layers in a manner that exploits an analogy with stratified planar systems, thereby allowing concentric multi-layered structures to be treated as photonic bandgap materials. Representative results from a Mie code employing this analogy demonstrate that photonic bands are present for periodic concentric spheres, though not readily apparent in extinction spectra. Rather, the periodicity simply alters the scattering profile, enhancing the ratio of backscattering to forward scattering inside the bandgap, whereas modification of the interference structure is evident in extinction spectra in accordance with the optical theorem

Smith, David D.↗
NASA NTRS2022

Aerosols Optical and Radiative Properties in Indonesia Based on AERONET Version 3

Heterogeneity in seasonal aerosol types due to different sources, local characteristics, and meteorology lead to different optical and radiative properties from one place to another. This study analyzes the long-term averages of aerosol optical and radiative properties obtained by the Aerosol Robotic Network (AERONET) version 3 at four sites in Indonesia representing fire prone areas (Palangka Raya, Pontianak, Jambi: 2012–2020), and urban-industrial (Bandung: 2009–2018). We examined the seasonal variation of aerosol optical depth (AOD), Angstrom Exponent (AE), Precipitable Water Vapor (PWV), and Single Scattering Albedo (SSA) combined with meteorological parameters at these Indonesian sites. Multiple clustering techniques from different relationships among various aerosol optical and radiative parameters was employed to further study the aerosol type in respect to different seasonality. The results exhibited a distinct seasonal pattern at all sites except Bandung, whereas AOD increased owing to forest and peat fire outbreaks during the dry season. The trend in AOD annual depicts an increase in Bandung as emission from urban/industrial increases episodically, while it depicts a decrease at the three biomass burning sites. As AOD increased, Palangka Raya, Pontianak, and Jambi exhibited wider ranges of observed AE (1.2–1.8) and high FMF (>0.8) in the dry burning period (June to October). On the other hand, Bandung has more aerosol distribution in the range of FMF values 0.6–1 and AE 1–1.6, compared with other sites, suggesting contribution of complex aerosol emission from different sources and likely due to the formation of secondary aerosol production from trace gases. Palangka Raya, Pontianak, and Jambi exhibited non-absorbing characteristics, as indicated by high SSA (>0.95), high FMF, and high EAE values (1.2–1.7) with no discrepancy in seasonal patterns, implying that biomass burning aerosols in Indonesia tend to cool the atmosphere with strong scattering rather than absorbing. At Bandung, aerosols mixed with slightly absorbing and non-absorbing aerosols owing to urban and industrial emissions. This study lays a foundation for further research on the contribution of aerosol radiative forcing to climate within the complex aerosol and cloud environments in Indonesia.

Aerosol optical depth↗
DOE OSTI2022

What is the iε for the S-matrix?

Can the S-matrix be complexified in a way consistent with causality? Since the 1960's, the affirmative answer to this question has been well-understood for 2→2 scattering of the lightest particle in theories with a mass gap at low momentum transfer, where the S-matrix is analytic everywhere except at normal-threshold branch cuts. We ask whether an analogous picture extends to realistic theories, such as the Standard Model, that include massless fields, UV/IR divergences, and unstable particles. Especially in the presence of light states running in the loops, the traditional iε prescription for approaching physical regions might break down, because causality requirements for the individual Feynman diagrams can be mutually incompatible. We demonstrate that such analyticity problems are not in contradiction with unitarity. Instead, they should be thought of as finite-width effects that disappear in the idealized 2→2 scattering amplitudes with no unstable particles, but might persist at higher multiplicity. To fix these issues, we propose an iε -like prescription for deforming branch cuts in the space of Mandelstam invariants without modifying the analytic properties. This procedure results in a complex strip around the real part of the kinematic space, where the S-matrix remains causal. In addition to giving a pedagogical introduction to the analytic properties of the perturbative S-matrix from a modern point of view, we illustrate all the points on explicit examples, both symbolically and numerically. Furthermore, to help with the investigation of related questions, we introduce a number of tools, including holomorphic cutting rules, new approaches to dispersion relations, as well as formulae for local behavior of Feynman integrals near branch points.

Anomalous thresholds↗
DOE OSTI2020

Cogeneration of hot electrons from multiple laser-plasma instabilities

Interactions of two plasmon decay (TPD) and side stimulated Raman scattering (SSRS) were studied using 3-D particle-in-cell simulations under ICF-relevant conditions for linearly and circularly polarized lasers. In the linear stage, SSRS took place under n e = 0.235n c and TPD dominated near the quarter-critical density surface and their growth rates agreed with theory. In the nonlinear stage, SSRS reduced TPD through pump depletion. Hot electrons were found to be first accelerated by the SSRS plasma waves and then by TPD plasma waves through a co-generation mechanism. Compared to the linearly polarized case with the same laser intensity, both SSRS and TPD were reduced due to the lower laser amplitude in the circularly-polarized case. As a result, a 30 percent decrease in hot electron flux was observed.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
NASA NTRS1983

Rotational CARS application to simultaneous and multiple-point temperature and concentration determination in a turbulent flow

Coherent anti-Stokes Raman scattering (CARS) from the pure rotational Raman lines of N2 is employed to measure the instantaneous (approximately 10 ns) rotational temperature of N2 gas at room temperature and below with good spatial resolution (0.2 x 0.2 x 3.0 cu mm). A broad bandwidth dye laser is used to obtain the entire rotational spectrum from a single laser pulse; the CARS signal is then dispersed by a spectrograph and recorded on an optical multichannel analyzer. A best fit temperature is found in several seconds with the aid of a computer for each experimental spectrum by a least squares comparison with calculated spectra. The model used to calculate the theoretical spectra incorporates the temperature and pressure dependence of the pressure-broadened rotational Raman lines, includes the nonresonant background susceptibility, and assumes that the pump laser has a finite linewidth. Temperatures are fit to experimental spectra recorded over the temperature range of 135 to 296 K, and over the pressure range of .13 to 15.3 atm.

Snow, J. B.↗
NASA NTRS1984

Rotational cars application to simultaneous and multiple-point temperature and concentration determination in a turbulent flow

Coherent Anti-stokes Raman Scattering (CARS) from the pure rotational Raman lines of N2 is employed to measure the instantaneous rotational temperature of N2 gas at room temperature and below with good spatial resolution. A broad-bandwidth dye laser is used to obtain the entire rotational spectrum from a signal laser pulse; the CARS signal is then dispersed by a spectrograph and recorded on an optical multichannel analyzer. A best-fit temperature is found in several seconds with the aid of a computer for each experimental spectrum by a least squares comparison with calculated spectra. The model used to calculate the theoretical spectra incorporates the temperature and pressure dependence of the pressure-broadened rotational Raman lines, includes the nonresonant background susceptibility, and assumes that the pump laser has a finite linewidth. Temperatures are fit to experimental spectra recorded over the temperature range of 135 to 296K, and over the pressure range of 0.13 to 15.3 atm. In addition to the spatially resolved single point work, we have used multipoint CARS to obtain information from many spatially resolved volume elements along a cylindrical line (0.1 x 0.1 x 2.0 mm). We also obtained qualitative information on the instantaneous species concentration and temperature at 20 spatially resolved volume elements (0.1 x 0.1 x 0.1 mm) along a line.

Snow, J. B.↗
NASA NTRS2008

Direct-View Multi-Point Two-Component Interferometric Rayleigh Scattering Velocimeter

This paper describes an instantaneous velocity measurement system based on the Doppler shift of elastically scattered laser light from gas molecules (Rayleigh scattering) relative to an incident laser. The system uses a pulsed laser as the light source, direct-viewing optics to collect the scattered light, an interferometer to analyze spectrally the scattered light mixed with the incident laser light, and a CCD camera to capture the resulting interferogram. The system is capable of simultaneous, spatially (approximately 0.2 mm(exp 3)) and temporally (approximately 40 ns) resolved, multiple point measurements of two orthogonal components of flow velocity in the presence of background scattered light, acoustic noise and vibrations, and flow particulates. Measurements in a large-scale axi-symmetric Mach 1.6 H2-air combustion-heated jet running at a flow sensible enthalpy specific to Mach 5.5 hypersonic flight are performed to demonstrate the technique. The measurements are compared with CFD calculations using a finite-volume discretization of the Favre-averaged Navier-Stokes equations (VULCAN code).

Bivolaru, Daniel↗
DOE OSTI2023

Study of charged particle production at high p T using event topology in pp, p–Pb and Pb–Pb collisions at $\sqrt{s_{NN}}=5.02$ TeV

This letter reports measurements which characterize the underlying event associated with hard scatterings at mid-pseudorapidity (|$η$| < 0.8) in pp, p–Pb and Pb–Pb collisions at centre-of-mass energy per nucleon pair, $\sqrt{s_{NN}}=5.02$ TeV. The measurements are performed with ALICE at the LHC. Different multiplicity classes are defined based on the event activity measured at forward rapidities. The hard scatterings are identified by the leading particle defined as the charged particle with the largest transverse momentum ($p_{T}$) in the collision and having 8 < $p_{T}$ < 15 GeV/c. The $p_{T}$ spectra of associated particles (0.5 < $p_{T}$ < 6 GeV/c) are measured in different azimuthal regions defined with respect to the leading particle direction: toward, transverse, and away. The associated charged particle yields in the transverse region are subtracted from those of the away and toward regions. The remaining jet-like yields are reported as a function of the multiplicity measured in the transverse region. The measurements show a suppression of the jet-like yield in the away region and an enhancement of high-$p_{T}$ associated particles in the toward region in central Pb–Pb collisions, as compared to minimum-bias pp collisions. These observations are consistent with previous measurements that used two-particle correlations, and with an interpretation in terms of parton energy loss in a high-density quark gluon plasma. These yield modifications vanish in peripheral Pb–Pb collisions and are not observed in either high-multiplicity pp or p–Pb collisions.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2024

Isotopic gamma lines for identification of shielding materials

Identifying the constituting materials of concealed objects is crucial in a wide range of sectors, such as medical imaging, geophysics, nonproliferation, national security investigations, and so on. Existing methods face limitations, particularly when multiple materials are involved or when there are challenges posed by scattered radiation and large areal mass. Here we introduce a novel brute-force statistical approach for material identification using high spectral resolution detectors, such as HPGe. The method relies upon updated semianalytic formulae for computing uncollided flux from source of gamma radiation, shielded by a sequence of nested spherical or cylindrical materials. These semianalytical formulae make possible rapid flux estimation for material characterization via combinatorial search through all possible combinations of materials, using a high-resolution HPGe counting detector. An important prerequisite for the method is that the geometry of the objects is known (for example, from X-ray radiography). We demonstrate the viability of this material characterization technique in several use cases with both simulated and experimental data in spherical geometry.

98 NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL P↗
DOE OSTI2022

Bio-inspired non self-similar hierarchical elastic metamaterials

Hierarchy provides unique opportunities for the design of advanced materials with superior properties that arise from architecture, rather than from constitutive material response. Contrary to the quasi-static regime, where the potential of hierarchy has been largely explored, its role in vibration mitigation and wave manipulation remains elusive. So far, the majority of the studies concerning hierarchical elastic metamaterials have proposed a self-similar repetition of a specific unit cell at multiple scale levels, leading to the activation of the same bandgap mechanism at different frequencies. On the contrary, here, we show that by designing non self-similar hierarchical geometries allows us to create periodic structures supporting multiple, highly attenuative and broadband bandgaps involving (independently or simultaneously) different scattering mechanisms, namely, Bragg scattering, local resonance and/or inertial amplification, at different frequencies. The type of band gap mechanism is identified and discussed by examining the vibrational mode shapes and the imaginary component of the wavenumber in the dispersion diagram of the unit cell. Finally, we also experimentally confirm this by performing measurements in the lowest frequency regime on a 3D printed structure. Hierarchical design strategies may find application in vibration mitigation for civil, aerospace and mechanical engineering.

36 MATERIALS SCIENCE↗
DOE OSTI2021

Constructive Quantum Interference in Photochemical Reactions

Interferences emerge when multiple pathways coexist together, leading toward the same result. Here, we report a theoretical study for a reaction scheme that leads to constructive quantum interference in a photoassociation (PA) reaction of a 87 Rb Bose–Einstein condensate where the reactant spin state is prepared in a coherent superposition of multiple bare spin states. This is achieved by changing the reactive scattering channel in the PA reaction. As the origin of coherent control comes from the spin part of the wavefunction, we show that it is sufficient to use radio frequency (RF) coupling to achieve the superposition state. We simulate the RF coupling on a quantum processor (IBMQ Lima), and our results show that interferences can be used as a resource for the coherent control of photochemical reactions. The approach is general and can be employed to study a wide spectrum of chemical reactions in the ultracold regime.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2022

Visualizing discrete Fermi surfaces and possible nodal-line to Weyl state evolution in ZrSiTe

Topological nodal line semimetals (TNLSMs) represent a quantum state of topological matter. When the crystal/time-reversal symmetry is broken, a nodal line state is expected to evolve into a Dirac semimetal, a Weyl semimetal, or other topological phases according to theoretical studies. Here, we report scanning tunneling microscopy (STM) based quasiparticle interference (QPI) measurements performed on the surface of TNLSM ZrSiTe single crystal. A discrete Fermi surface with multiple electron/hole pockets and the impurity-induced inter-/intra- pockets scatterings are directly visualized from QPI patterns. Moreover, the degenerated Dirac points at X point evolve into the pairs of Weyl nodes when Fe atoms are deposited, suggesting a possible phase transition from the nodal line to the Weyl state. The calculated band structures and the Weyl points by applying Zeeman splitting energies along x-direction, further confirm the existence of Weyl points in the Fe-doped ZrSiTe induced by the broken of time-reversal symmetry.

36 MATERIALS SCIENCE↗
DOE OSTI2022

Signatures of non-Loudon-Fleury Raman scattering in the Kitaev magnet 𝛽−Li 2 ⁢IrO 3

We investigate the magnetic excitations of the hyperhoneycomb Kitaev magnet 𝛽−Li 2 ⁢IrO 3 by means of inelastic Raman scattering. The spectra exhibit the coexistence of a broad scattering continuum and two sharp low-energy peaks at 2.5 and 3 meV, with a distinctive polarization dependence. While the continuum is suggestive of fractional quasiparticles emerging from a proximate quantum spin liquid phase, the sharp peaks provide the first experimental signature of the “non-Loudon- Fleury” one-magnon scattering processes proposed recently. The corresponding microscopic mechanism is similar to the one leading to the symmetric off-diagonal exchange interaction Γ (because it involves a combination of both direct and ligand-mediated exchange paths) but is otherwise completely unexpected within the traditional Loudon-Fleury theory of Raman scattering. Furthermore, the present experimental verification therefore calls for a drastic reevaluation of Raman scattering in similar systems with strong spin-orbit coupling and multiple exchange paths.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2024

RMCProfile7 : reverse Monte Carlo for multiphase systems

This work introduces a completely rewritten version of the programRMCProfile(version 7), big-box, reverse Monte Carlo modelling software for analysis of total scattering data. The major new feature ofRMCProfile7is the ability to refine multiple phases simultaneously, which is relevant for many current research areas such as energy materials, catalysis and engineering. Other new features include improved support for molecular potentials and rigid-body refinements, as well as multiple different data sets. An empirical resolution correction and calculation of the pair distribution function as a back-Fourier transform are now also available.RMCProfile7is freely available for download at https://rmcprofile.ornl.gov/.

Chemistry↗
DOE OSTI2021

Efficient loading of reduced data ensembles produced at ORNL SNS/HFIR neutron time-of-flight facilities

We present algorithmic improvements to the loading operations of certain reduced data ensembles produced from neutron scattering experiments at Oak Ridge National Laboratory (ORNL) facilities. Ensembles from multiple measurements are required to cover a wide range of the phase space of a sample material of interest. They are stored using the standard NeXus schema on individual HDF5 files. This makes it a scalability challenge, as the number of experiments stored increases in a single ensemble file. The present work follows up on our previous efforts on data management algorithms, to address identified input output (I/O) bottlenecks in Mantid, an open-source data analysis framework used across several neutron science facilities around the world. We reuse an in-memory binary-tree metadata index that resembles data access patterns, to provide a scalable search and extraction mechanism. In addition, several memory operations are refactored and optimized for the current common use cases, ranging most frequently from 10 to 180, and up to 360 separate measurement configurations. Results from this work show consistent speed ups in wall-clock time on the Mantid LoadMD routine, ranging from 19% to 23% on average, on ORNL production computing systems. The latter depends on the complexity of the targeted instrument-specific data and the system I/O and compute variability for the shared computational resources available to users of ORNL’s Spallation Neutron Source (SNS) and the High Flux Isotope Reactor (HFIR) instruments. Nevertheless, we continue to highlight the need for more research to address reduction challenges as experimental data volumes, user time and processing costs increase.

Godoy, William↗
DOE OSTI2022

60 GHz Outdoor Propagation Measurements and Analysis Using Facebook Terragraph Radios

The high attenuation of millimeter-wave (mmWave) would significantly reduce the coverage areas, and hence it is critical to study the propagation characteristics of mmWave in multiple deployment scenarios. In this work, we investigated the propagation and scattering behavior of 60 GHz mmWave signals in outdoor environments at a travel distance of 98 m for an aerial link (rooftop to rooftop), and 147 m for a ground link (light-pole to light-pole). Measurements were carried out using Facebook Terragraph (TG) radios. Results include received power, path loss, signal-to-noise ratio (SNR), and root mean square (RMS) delay spread for all beamforming directions supported by the antenna array. Strong line-of-sight (LOS) propagation exists in both links. We also observed rich multipath components (MPCs) due to edge scatterings in the aerial link, while only LOS and ground reflection MPCs in the other link.

60 GHz↗
DOE OSTI2024

Quantification of the Crack Evolution Process by Extracting Relevant Signal Components from Wave Propagation and Diffusive Transport Front Measurements

Wave propagation and diffusive transport phenomena in a geological rock sample undergoing crack evolution process are expected to interact with the mechanical discontinuities in the medium. The measurements of the signals associated with these phenomena can be used to assess and monitor the crack-driven micromechanical alterations in the rock. Different wave/diffusion phenomena, such as sonic propagation, pressure diffusion, and acoustic emission (AE), are sensitive to different elements of the mechanical discontinuities generated during the evolution of the crack clusters from initiation to coalescence. Sonic propagation, AE, and pressure diffusion monitoring have the potential to map the crack evolution because the transmitter-receiver arrays can be designed, arranged and tuned to (1) achieve maximum recovery of the scattered waveforms and travel times, (2) capture the later arrivals and multiple reflections, and (3) illuminate large rock volume. However, the structural/topological complexities of the mechanical discontinuities, complex distribution of the stress fields, complex mechanical alterations in media, and fluid redistribution in the crack system pose serious challenges for the detection and modeling of the crack evolution process (from here on, we will use the term ‘crack evolution process’ to mean that the crack evolution occurred under shallow crustal conditions). For purposes of accurately accounting such complexities and heterogeneities in the absence of reliable physical laws, simulation methods, and signal processing techniques, my early-career research proposal will develop and apply novel data-driven machine learning methods to: (1) extract signal components relevant to the various phases of crack evolution and (2) generate a 2D visual map of the crack evolution process.

58 GEOSCIENCES↗
NASA NTRS1991

A two-dimensional time domain near zone to far zone transformation

In a previous paper, a time domain transformation useful for extrapolating 3-D near zone finite difference time domain (FDTD) results to the far zone was presented. In this paper, the corresponding 2-D transform is outlined. While the 3-D transformation produced a physically observable far zone time domain field, this is not convenient to do directly in 2-D, since a convolution would be required. However, a representative 2-D far zone time domain result can be obtained directly. This result can then be transformed to the frequency domain using a Fast Fourier Transform, corrected with a simple multiplicative factor, and used, for example, to calculate the complex wideband scattering width of a target. If an actual time domain far zone result is required it can be obtained by inverse Fourier transform of the final frequency domain result.

Luebbers, Raymond J.↗