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At least 1,099 records · Page 61

Gas transport across the low-permeability containment zone of an underground nuclear explosion

Understanding the nature of gas transport from an underground nuclear explosion (UNE) is required for evaluating the ability to detect and interpret either on-site or atmospheric signatures of noble gas radionuclides resulting from the event. We performed a pressure and chemical tracer monitoring experiment at the site of an underground nuclear test that occurred in a tunnel in Nevada to evaluate the possible modes of gas transport to the surface. The site represents a very well-contained, low gaspermeability end member for past UNEs at the Nevada National Security Site. However, there is very strong evidence that gases detected at the surface during a period of low atmospheric pressure resulted from fractures of extremely small aperture that are essentially invisible. Our analyses also suggest that gases would have easily migrated to the top of the high-permeability collapse zone following the detonation minimizing the final distance required for migration along these narrow fractures to the surface. This indicates that on-site detection of gases emanating from such low-permeability sites is feasible while standoff detection of atmospheric plumes may also be possible at local distances for sufficiently high fracture densities. Finally, our results show that gas leakage into the atmosphere also occurred directly from the tunnel portal and should be monitored in future tunnel gas sampling experiments for the purpose of better understanding relative contributions to detection of radioxenon releases via both fracture network and tunnel transport.

98 NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL P↗

Evaluation of subsurface transport processes of delayed gas signatures applicable to underground nuclear explosions

Radioactive gas signatures from underground nuclear explosions (UNEs) result from gas-migration processes occurring in the subsurface. The processes considered in this study either drive or retard upward migration of gases from the detonation cavity. The relative importance of these processes is evaluated by simulating subsurface transport in a dual-permeability medium for the multi-tracer Noble Gas Migration Experiment (NGME) originally intended to study some aspects of transport from a UNE. For this experiment, relevant driving processes include weak two-phase convection driven by the geothermal gradient, over pressuring of the detonation cavity, and barometric pumping while gas sorption, dissolution, radioactive decay, and usually diffusion represent retarding processes. From deterministic simulations we found that over-pressuring of the post-detonation chimney coupled with barometric pumping produced a synergistic effect amplifying the tracer-gas reaching the surface. Bounding simulations indicated that the sorption and dissolution of gases, tending to retard transport, were much smaller than anticipated by earlier laboratory studies. The NGME observations themselves show that differences in gas diffusivity have a larger effect on influencing upward transport than do the combined effects of tracer-gas sorption and dissolution, which is consistent with a Sobol’ sensitivity analysis. Both deterministic simulations and those considering parametric uncertainties of transport-related properties predict that the excess in concentration of SF 6 compared to 127 Xe as might be captured in small volumetric samples should be much smaller than the order-of-magnitude contrast found in the large-volume gas samples taken at the site. While extraction of large-volume subsurface gas samples is shown to be capable of distorting in situ gas compositions, the highly variable injection rate of SF 6 into the detonation cavity relative to that of 127 Xe at the start of the field experiment is the most likely explanation for the large difference in observed concentrations.

58 GEOSCIENCES↗

Direct observation of diamond formation in a shock-compressed high explosive

Understanding the formation timescale and structure of carbonaceous reaction products is critical for modeling the high-pressure equation-of-state of organic materials. We use the National Ignition Facility to shock-compress polycrystalline TATB (C 6 H 6 N 6 O 6 ) samples to ~70–130 GPa and ~4000–5500 K, employing in situ nanosecond X-ray diffraction to probe reaction products and velocimetry to measure transmitted compression wave profiles. Our diffraction data is consistent with the formation of diamond over timescales less than ~60 ns. This represents carbon condensation from a molecular explosive on timescales three times faster than previously reported and the earliest observation of diamond produced from reacting TATB. Reactive flow simulations with explicit chemistry reproduce the observed temporal structure within wave profiles to inform the distribution of P-T states. These findings provide direct evidence of ultrafast diamond formation in a reactive system at extreme conditions and provide new constraints for models of shock and detonation chemistry.

Clarke, Samantha M. [Lawrence Livermore National L↗

Radionuclide gas transport through nuclear explosion-generated fracture networks

Underground nuclear weapon testing produces radionuclide gases which may seep to the surface. Barometric pumping of gas through explosion-fractured rock is investigated using a new sequentially-coupled hydrodynamic rock damage/gas transport model. Fracture networks are produced for two rock types (granite and tuff) and three depths of burial. The fracture networks are integrated into a flow and transport numerical model driven by surface pressure signals of differing amplitude and variability. There are major differences between predictions using a realistic fracture network and prior results that used a simplified geometry. Matrix porosity and maximum fracture aperture have the greatest impact on gas breakthrough time and window of opportunity for detection, with different effects between granite and tuff simulations highlighting the importance of accurately simulating the fracture network. In particular, maximum fracture aperture has an opposite effect on tuff and granite, due to different damage patterns and their effect on the barometric pumping process. From stochastic simulations using randomly generated hydrogeologic parameters, normalized detection curves are presented to show differences in optimal sampling time for granite and tuff simulations. In conclusion, seasonal and location-based effects on breakthrough, which occur due to differences in barometric forcing, are stronger where the barometric signal is highly variable.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Three-dimensional simulations of turbulent convective mixing in ONe and CO classical nova explosions

Classical novae are thermonuclear explosions that take place in the envelopes of accreting white dwarfs in binary systems. The material piles up under degenerate conditions, driving a thermonuclear runaway. The energy released by the suite of nuclear processes operating at the envelope heats the material up to peak temperatures of ~(1-4) × 10 8 K. During these events, about 10 -3 -10 -7 M ⊙ , enriched in CNO and, sometimes, other intermediate-mass elements (e.g., Ne, Na, Mg, Al) are ejected into the interstellar medium. To account for the gross observational properties of classical novae (in particular, the high concentrations of metals spectroscopically inferred in the ejecta), models require mixing between the (solar-like) material transferred from the secondary and the outermost layers (CO- or ONe-rich) of the underlying white dwarf. Recent multidimensional simulations have demonstrated that Kelvin-Helmholtz instabilities can naturally produce self-enrichment of the accreted envelope with material from the underlying white dwarf at levels that agree with observations. However, the feasibility of this mechanism has been explored in the framework of CO white dwarfs, while mixing with different substrates still needs to be properly addressed. We performed three-dimensional simulations of mixing at the core-envelope interface during nova outbursts with the multidimensional code FLASH, for two types of substrates: CO- and ONe-rich. We also show that the presence of an ONe-rich substrate, as in “neon novae”, yields higher metallicity enhancements in the ejecta than CO-rich substrates (i.e., non-neon novae). Finally, a number of requirements and constraints for such 3D simulations (e.g., minimum resolution, size of the computational domain) are also outlined.

79 ASTRONOMY AND ASTROPHYSICS↗

High power laser coupling to carbon nano-tubes and ion Coulomb explosion

Linear and non linear interaction of laser with an array of carbon nanotubes is investigated. The ac conductivity of nanotubes, due to uneven response of free electrons in them to axial and transverse fields, is a tensor. The propagation constant for p-polarization shows resonance at a specific frequency that varies with the direction of laser propagation. It also shows surface plasmon resonance at ω=ω{sub p}/√(2), where ω{sub p} is the plasma frequency of free electrons inside a nanotube, assumed to be uniform plasma cylinder. The attenuation constant is also resonantly enhanced around these frequencies. At large laser amplitude, the nanotubes behave as thin plasma rods. As the electrons get heated, the nanotubes undergo hydrodynamic expansion. At an instant when plasma frequency reaches ω{sub p}=√(2)ω, the electron temperature rises rapidly and then saturates. For a Gaussian laser beam, the heating rate is maximum on the laser axis and falls off with the distance r from the axis. When the excursion of the electrons Δ is comparable or larger than the radius of the nanotube r{sub c}, the nanotubes undergo ion Coulomb explosion. The distribution function of ions turns out to be a monotonically decreasing function of energy.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Stability of imploding shocks generated by underwater electrical explosion of cylindrical wire array

The results of two-dimensional hydrodynamic simulations of the dynamics and stability of azimuthal non-uniformities in converging shock waves generated by an underwater explosion of a cylindrical wire array and their effect on the cumulation of energy in the vicinity of the converging axis are presented. It has been shown that in spite of the fact that such non-uniformities are always weakly unstable, for a broad range of experimentally relevant regimes these non-uniformities remain small and do not significantly affect the cumulation of energy. Only the non-uniformities with wavelengths comparable to the distance from the axis of convergence exhibit substantial growth that considerably attenuates the energy cumulation.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Laser induced neutron production by explosion of the deuterium clusters

The high energy deuterium ions serve as compact source of neutrons when fused with either deuterium or tritium atoms. In view of this, the explosion of the deuterium clusters under the influence of the laser pulse with intensity ranging from 10{sup 15} to 10{sup 19} W/cm{sup 2} is being studied along with the effect of the cluster radius and inter-cluster distance. The objective of this article is to study the efficiency of the deuterium cluster as a compact source of neutrons under various laser and cluster parameters. It is being observed that the cluster density (number of clusters per unit volume) is quite important to gain high neutron yield.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Chaos and turbulent nucleosynthesis prior to a supernova explosion

Three-dimensional (3D), time dependent numerical simulations of flow of matter in stars, now have sufficient resolution to be fully turbulent. The late stages of the evolution of massive stars, leading up to core collapse to a neutron star (or black hole), and often to supernova explosion and nucleosynthesis, are strongly convective because of vigorous neutrino cooling and nuclear heating. Unlike models based on current stellar evolutionary practice, these simulations show a chaotic dynamics characteristic of highly turbulent flow. Theoretical analysis of this flow, both in the Reynolds-averaged Navier-Stokes (RANS) framework and by simple dynamic models, show an encouraging consistency with the numerical results. It may now be possible to develop physically realistic and robust procedures for convection and mixing which (unlike 3D numerical simulation) may be applied throughout the long life times of stars. In addition, a new picture of the presupernova stages is emerging which is more dynamic and interesting (i.e., predictive of new and newly observed phenomena) than our previous one.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

The calculation of electron chemical potential and ion charge state and their influence on plasma conductivity in electrical explosion of metal wire

The electron chemical potential and ion charge state (average ion charge and ion distribution) are important parameters in calculating plasma conductivity in electrical explosion of metal wire. In this paper, the calculating method of electron chemical potential and ion charge state is discussed at first. For the calculation of electron chemical potential, the ideal free electron gas model and Thomas-Fermi model are compared and analyzed in terms of the coupling constant of plasma. The Thomas-Fermi ionization model, which is used to calculate ion charge state, is compared with the method based on Saha equation. Furthermore, the influence of electron degenerated energy levels and ion excited states in Saha equation on the ion charge state is also analyzed. Then the influence of different calculating methods of electron chemical potential and ion charge state on plasma conductivity is discussed by applying them in the Lee-More conductivity model.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Evolution and explosion of the most massive asymptotic giant branch star

The most massive asymptotic giant branch (AGB) stars can form a critical mass of ONe core at its center. The collapse of such a critical ONe core may end up as an Electron Capture Supernova (ECSN). We have accomplished a progenitor calculation for ECSN for the first time in more than two decades and have updated a pre-explosion structure for this model. Some details for ONe core formation and important mechanisms for the core contraction are shown. We discuss how the envelope mass loss affects the predicted existence of ECSN, and what physics is needed to model for a plausible structure of ECSN progenitor.

79 ASTRONOMY AND ASTROPHYSICS↗

Supernova explosion and black hole formation with hadron-quark phase transition

Hadronic matter undergoes a deconfinement transition to quark matter at high temperature and/or high density. It would be realized in collapsing cores of massive stars. The fates of core collapses are investigated for various cases. Equations of state including the hadron-quark phase transition with different values of bag constant are used. As a result, for the case with a small bag constant (i.e. the transition occurs at low density), the second bounce revives the shock wave leading to explosion for the model with 15 solar mass. The systematics on the bag constant is also studied for the black hole formation of a 40 solar mass progenitor.

79 ASTRONOMY AND ASTROPHYSICS↗

Production of {sup 44}Ti in neutrino-driven aspherical supernova explosions

We examine the synthesis of {sup 44}Ti in a neutrino-driven aspherical supernova (SN), focusing on reaction rates related to {sup 44}Ti and rotation of a progenitor. We have performed 2D hydrodynamic simulations of SN of a 15M{sub ⊙} progenitor, whose angular velocity is manually set to be a cylindrical distribution and have followed explosive nucleosynthesis in the ejecta. We find that the faster rates of {sup 40}Ca(α,γ){sup 44}Ti and the slower rate of {sup 44}Ti(α,p){sup 47}V lead to more massive ejection of {sup 44}Ti and {sup 56}Ni and larger ratios <{sup 44}Ti/{sup 56}Ni>. Faster rotation also results in more massive ejection of {sup 44}Ti and {sup 56}Ni. Ratios <{sup 44}Ti/{sup 56}Ni> are however independent from rotation. Large masses of {sup 44}Ti and large ratios observed in SN 1987A and Cas A (> 1O{sup −4}M{sub ⊙} and 1-2 respectively) are not realized in all the models.

79 ASTRONOMY AND ASTROPHYSICS↗

Supernova neutrinos and explosive nucleosynthesis

Core-collapse supernovae eject huge amount of flux of energetic neutrinos. We studied the explosive nucleosyn-thesis in supernovae and found that several isotopes {sup 7}Li, {sup 11}B, {sup 92}Nb, {sup 138}La and {sup 180}Ta as well as r-process nuclei are affected by the neutrino interactions. The abundance of these isotopes therefore depends strongly on the neutrino flavor oscillation due to the Mikheyev-Smirnov-Wolfenstein (MSW) effect. We discuss first how to determine the neutrino temperatures in order to explain the observed solar system abundances of these isotopes, combined with Galactic chemical evolution of the light nuclei and the heavy r-process elements. We then study the effects of neutrino oscillation on their abundances, and propose a novel method to determine the still unknown neutrino oscillation parameters, mass hierarchy and θ{sub 13}, simultaneously. There is recent evidence that SiC X grains from the Murchison meteorite may contain supernova-produced light elements {sup 11}B and {sup 7}Li encapsulated in the presolar grains. Combining the recent experimental constraints on θ{sub 13}, we show that our method sug-gests at a marginal preference for an inverted neutrino mass hierarchy. Finally, we discuss supernova relic neutrinos that may indicate the softness of the equation of state (EoS) of nuclear matter as well as adiabatic conditions of the neutrino oscillation.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Cost effective nanostructured copper substrates prepared with ultrafast laser pulses for explosives detection using surface enhanced Raman scattering

Ultrafast laser pulses induced surface nanostructures were fabricated on a copper (Cu) target through ablation in acetone, dichloromethane, acetonitrile, and chloroform. Surface morphological information accomplished from the field emission scanning electron microscopic data demonstrated the diversities of ablation mechanism in each case. Fabricated Cu substrates were utilized exultantly to investigate the surface plasmon (localized and propagating) mediated enhancements of different analytes using surface enhance Raman scattering (SERS) studies. Multiple utility of these substrates were efficiently demonstrated by collecting the SERS data of Rhodamine 6G molecule and two different secondary explosive molecules such as 5-amino-3-nitro-l,2,4-triazole and trinitrotoluene on different days which were weeks apart. We achieved significant enhancement factors of >10{sup 5} through an easily adoptable cleaning procedure.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Influence of insulating coating on aluminum wire explosions

Single wire explosions are widely used in understanding the early stages of z-pinch experiments. This paper presents a serial of experiments conducted on the pulse power generator with ∼1 kA peak current and ∼10 ns rising time in Xi'an Jiao Tong University. Polyimide coated aluminum wires and uncoated ones were tested under three different voltages to analyze the effect of insulating coating. Experimental results showed that insulating coating can increase the energy deposition 10%∼30% in aluminum wires by delaying the voltage collapse and raising the maximum load resistance. The substantial energy deposition resulted in about 20% faster expansion rates for coated wires. Experimental evidence that plasma channel shunts the current from the wire core was observed by streak camera and schlieren graphs. This paper also briefly discussed the influence of nonuniform coating on the morphology of wire expansion.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗