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At least 1,099 records · Page 61

The Net Decay Time of Anomalies in Concentrations of Atmospheric Pollutants

This paper introduces a new parameter to characterize the random component in temporal variability of atmospheric pollutants and proposes a simple statistical technique for its evaluation. That parameter is the net decay time (or the time scale) of the local anomalies in concentrations of atmospheric pollutants, rather than the traditionally used chemical lifetimes of total amounts of the species. Using widely available data of hourly multi-year surface trace gas pollutant concentrations we demonstrate a simplified way to estimate the net decay time with an exponential approximation of lag-correlation functions. We assessed the decay times of fluctuations in observations of eight atmospheric pollutants (SO2, NO, NO2, NOy, O3, CO, NH3, and HNO3) at two urban sites and one cleaner rural site in the Eastern US. The time scales of temporal fluctuations (net decay times) vary from about one hour to slightly more than one day. These scales are generally much shorter in urban environments than in remote regions. We also compared day- and night-time observations in warm and cold seasons. At night in the cold season, time scales of fluctuations in atmospheric pollutants are usually the longest. Such estimates should be useful to air quality prediction, public health, and satellite remote sensing research communities.

air quality prediction↗

Does Orbital Angular Momentum Have Effect on Laser’s Scattering by Molecular Atmosphere?

Lasers with orbital angular momentum (OAM) have potential applications in communication technology, manipulation of particles, and remote sensing. Because of its unusual light-scattering properties, the OAM laser’s interaction with a molecular atmosphere must be studied to ensure that it is not lossy for communication or remote-sensing applications that involve its transmission through an atmospheric environment. In this study, the finite-difference time-domain (FDTD) method [21] is applied to calculate the light scattering of the purely azimuthal (the radial mode number is assumed to be zero) Laguerre-Gaussian (LG) beams with OAM by very small dielectric particles. Not like Lorentz-Mie solutions, the FDTD method can calculate for particles off the central axis of the LG beam. It is found that when the particles are very small, and the topological charge number of the OAM of a laser is not extremely large, the laser’s OAM has little effect on the scattering phase function. This suggests that Rayleigh theory can be applied directly to calculate the light scattering by atmospheric molecules. The transmission of a laser beam with OAM in a molecular atmosphere is not different from that of a regular Gaussian beam.

Molecular atmosphere↗

Atmospheric Correction Over Ocean for Hyperspectral Radiometers Using Multi-Angle Polarimetric Retrievals

We developed a fast and accurate POLYnomial based Atmospheric Correction (POLYAC) algorithm for hyperspectral radiometric measurements, which parameterizes the atmospheric path radiances using aerosol properties retrieved from co-located multi-wavelength Multi-Angle Polarimeter (MAP) measurements. This algorithm has been applied to co-located Spectrometer for Planetary Exploration (SPEX) airborne and Research Scanning Polarimeter (RSP) measurements, where SPEX airborne was used as a proxy of hyperspectral radiometers, and RSP as the MAP. The hyperspectral remote sensing reflectance obtained from POLYAC is accurate when compared to Aerosol Robotic Network (AERONET), and Visible Infrared Imaging Radiometer Suite (VIIRS) ocean color products. POLYAC provides a robust alternative atmospheric correction algorithm for hyperspectral or multi-spectral radiometric measurements for scenes involving coastal oceans and/or absorbing aerosols, where traditional atmospheric correction algorithms are less reliable.

ocean color↗

Decadal Changes in the Interannual Variability of Heat Waves in East Asia Caused by Atmospheric Teleconnection Changes

The heat wave in East Asia is examined by using empirical orthogonal function analysis to isolate dominant heat-wave patterns in the ground-based temperature observations over the Korean Peninsula and China and related large-scale atmospheric circulations obtained from the National Centers for Environmental Prediction–National Center for Atmospheric Research Reanalysis 1 during 1973–2012. This study focuses particularly on the interannual variability of heat waves and its decadal change. The analysis identifies two major atmospheric teleconnection patterns playing an important role in developing typical heat-wave patterns in East Asia—the Scandinavian (SCAND) and the circumglobal teleconnection (CGT) patterns, which exhibit a significant decadal change in the interannual variability in the mid-1990s. Before the mid-1990s, heat-wave occurrence was closely related to the CGT pattern, whereas the SCAND pattern is more crucial to explain heat-wave variability in the recent period. The stationary wave model experiments suggest an intensification of the SCAND pattern in the recent period driven by an increase in land–atmosphere interaction over Eurasia and decadal change in the dominant heat-wave patterns in East Asia.

heat wave patterns↗

Optimal Estimation Framework for Ocean Color Atmospheric Correction and Pixel-level Uncertainty Quantification

Ocean color remote sensing requires compensation for atmospheric scattering and absorption (aerosol, Rayleigh, and trace gases), referred to as atmospheric correction (AC). AC allows inference of parameters such as spectrally resolved remote sensing reflectance ( R rs )(λ) ; sr 1 ) at the ocean surface from the top-of-atmosphere reflectance. Often, the uncertainty of this process is not fully explored. Bayesian inference techniques provide a simultaneous AC and uncertainty assessment via a full posterior distribution of the relevant variables, given the prior distribution of those variables and the radiative transfer (RT) likelihood function. Given uncertainties in the algorithm inputs, the Bayesian framework enables better constraints on the AC process by using the complete spectral information compared to traditional approaches that use only a subset of bands for AC. This paper investigates a Bayesian inference research method (Optimal Estimation, OE) for ocean color AC by simultaneously retrieving atmospheric and ocean properties using all visible and near-infrared spectral bands. The OE algorithm analytically approximates the posterior distribution of parameters based on normality assumptions and provides a potentially viable operational algorithm with a reduced computational expense. We developed a Neural Network (NN) RT forward model look-up-table-based emulator to increase algorithm efficiency further and thus speed up the likelihood computations. We then applied the OE algorithm to synthetic data and observations from the MODerate resolution Imaging Spectroradiometer (MODIS) on NASA’s Aqua spacecraft. We compared the R rs )(λ) retrieval and its uncertainty estimates from the OE method with in-situ validation data from the SeaWiFS Bio-optical Archive and Storage System (SeaBASS) and Aerosol Robotic Network Ocean Color (AERONET-OC) datasets. The OE algorithm improved R rs )(λ) estimates relative to the NASA standard operational algorithm by improving all statistical metrics at 443, 555, and 667 nm. Unphysical negative R rs )(λ) , which often appear in complex water conditions, was reduced by a factor of 3. The OE-derived pixel-level R rs )(λ) uncertainty estimates were also assessed relative to in-situ data and were shown to have skill.

Atmospheric correction↗

Stratospheric Temperatures and Water Loss From Moist Greenhouse Atmospheres of Earth-Like Planets

A radiative-convective climate model is used to calculate stratospheric temperatures and water vapor concentrations for ozone-free atmospheres warmer than that of modern Earth. Cold, dry stratospheres are predicted at low surface temperatures, in agreement with recent 3D calculations. However, at surface temperatures above 350 K, the stratosphere warms and water vapor becomes a major upper atmospheric constituent, allowing water to be lost by photodissociation and hydrogen escape. Hence, a moist greenhouse explanation for loss of water from Venus, or some exoplanet receiving a comparable amount of stellar radiation, remains a viable hypothesis. Temperatures in the upper parts of such atmospheres are well below those estimated for a gray atmosphere, and this factor should be taken into account when performing inverse climate calculations to determine habitable zone boundaries using 1D models.

Astrobiology↗

Future Atmospheric Rivers and Impacts on Precipitation: Overview of the ARTMIP Tier2 High-Resolution Global Warming Experiment

Atmospheric rivers (ARs) are long, narrow synoptic scale weather features important for Earth’s hydrological cycle typically transporting water vapor poleward, delivering precipitation important for local climates. Understanding ARs in a warming climate is problematic because the AR response to climate change is tied to how the feature is defined. The Atmospheric River Tracking Method Intercomparison Project (ARTMIP) provides insights into this problem by comparing 16 atmospheric river detection tools (ARDTs) to a common dataset consisting of high resolution climate change simulations from a global atmospheric general circulation model. ARDTs mostly show increases in frequency and intensity, but the scale of the response is largely dependent on algorithmic criteria. Across ARDTs, bulk characteristics suggest intensity and spatial footprint are inversely correlated, and most focus regions experience increases in precipitation volume coming from extreme ARs. The spread of the AR precipitation response under climate change is large and dependent on ARDT selection.

Atmospheric Rivers↗

Warming Reduces the Efficacy of Wet Conditions to Moderate Extreme Heat and Atmospheric Aridity Across the Central Plains

In the literature, dry land surface conditions possess a well-established association with extreme heat and high atmospheric aridity, especially in regions that experience strong land-atmosphere feedbacks. However, few studies have examined whether global warming will impact the ability of wet conditions to constrain high temperatures and atmospheric aridity occurrences. Here we investigate how wet conditions, which we define using precipitation and soil moisture, constrain high temperature and high vapor pressure deficit during the warm season over the Central Plains in North America at different global warming levels (0-3 degrees K). Using a CMIP6 multi-model ensemble, we show that absolute changes in the maximum temperature distribution outweigh the historical cooling effect of high precipitation or soil moisture conditions, reducing the probability of non-extreme maximum temperatures under global warming. Strikingly, the conditional likelihood of non-extreme maximum temperatures falls from 97-98% at baseline conditions to 50-58% at 1 degree of global warming. Once 2 degrees of warming is reached, there is very little probability of constraining extreme maximum temperatures. On the other hand, high precipitation and high soil moisture are able to better retain the ability to constrain concurrent high vapor pressure deficit conditions – moving from 99% at baseline conditions to 81-91% at 1 degree of warming and 26-42% at 2 degrees of warming. With our results, we find that the extent of this retention is dependent on how individual models represent relative changes in the VPD distribution as temperatures warm. Overall, our results highlight the growing vulnerability of the Central North American region to warmer temperatures and drier atmospheric conditions, even during periods of high precipitation and soil moisture.

Extreme heat↗

PACE UV-VIS Polarimetric Remote Sensing of Atmosphere-Ocean Systems: Sensitivity to Variations in Brown Carbon

The NASA Plankton, Aerosol, Cloud, and ocean Ecosystem (PACE) mission, scheduled for launch in 2024, will carry two instruments that measure ultraviolet (UV) radiance emerging from the top of the atmosphere: the Ocean Color Instrument (OCI) and the Spectro-Polarimeter for Planetary Exploration (SPEXone) instrument. OCI will provide single-view, hyperspectral radiometric data, whereas SPEXone will provide multi-angle, multispectral polarimetric data. Together, these instruments will be the most advanced in NASA’s history for the combined observation of ocean color and atmospheric aerosols in the UV, and they will therefore provide unprecedented research opportunities for the ocean color and atmospheric aerosol communities. In particular, UV observations are best suited to retrieve properties of Colored Dissolved Organic Matter (CDOM) in the ocean, and of Brown Carbon (BrC) aerosols in the atmosphere. However, both CDOM and BrC exhibit very similar absorption spectra in the UV and the visible (VIS) spectrum; hence, care must be taken in accurately modeling these spectra for analyses of OCI and SPEXone measurements. In this presentation, we summarize a simple but highly accurate three-parameter model for complex refractive index spectra of BrC in the UV and VIS. We apply this model to simulations of PACE-like total and polarized multiangle radiance in the UV, and demonstrate that the impact of BrC and CDOM variations can be similar in total radiance, but is easy to distinguish in polarized radiance.

PACE↗

Moon to Mars (M2M): Exploration Atmosphere

As humans leave the bounds of Earth to explore the lunar surface and beyond, crew will don extravehicular activity (EVA) suits to learn more about these extraterrestrial environments, establish sustained presence, and perform needed upgrades and maintenance to their space vehicle and habitation systems. Spacefaring vehicle and habitation design will need to support these EVA excursions while ensuring crew health and safety. A crucial technological design advancement towards this goal is the use of a lower pressure exploration atmosphere (EA) that enables high efficiency EVA, rather than the sea level atmosphere of 14.7 psia, 21% oxygen (O 2 ) found on the International Space Station, Shuttle, and most other Russian and Chinese space vehicles and stations. Early space vehicles (Mercury through Apollo Programs) used a 5 psia, 100% O 2 environment, which eliminated the need for pre-EVA denitrogenation protocols, simplified the life support system to a single gas, and saved structural mass. For longer duration missions (Skylab), a diluent gas was added, changing the atmosphere to 5 psia, 70-74% O 2 to prevent atelectasis while remaining normoxic. As in-flight science became a top priority, Shuttle and ISS atmospheres were chosen to operate at sea level allowing for simpler ground-based study control conditions. Consequently this led to long pre-EVA denitrogenation protocols involving up to 4 hours of O 2 prebreathe because the EVA suit still operated at a low pressure of 4.3 psid. To increase operational efficiency, the Shuttle was retroactively certified to operate using 10.2 psia, 26.5% O 2 , reducing O 2 prebreathe time to 40-75 min. Current plans for M2M habitats on the Lunar surface require EVA, thus EA recommendation became 8 psia and 32% O 2 but was revised to 8.2 psia and 34% O 2 to decrease hypoxia exposure. Unfortunately, the benefits of EA in support of safe and efficient EVAs comes with the challenge of fire management in a higher-than-normal O 2 % environment. Although known for decades, the recommended forward work to address fire management has only recently begun. Current flammability tests include examining material propagation and ignition sources as well as fire mitigation processes to better understand these properties for proposed new EA environments. Fire safety, DCS risk, and mission design all contribute to the multifaceted parameters of EA. Thus while it is clear that EA is required to achieve the goals of future exploratory space missions, final specifications are still being evaluated for optimizing crew health and safety.

space atmosphere↗

The Atmosphere and Haze of Mars

The 'blue haze' is an absorbing smoke, dark as soot in reflection, red in transmission. Its currently accepted explanation by pure scattering (omnidirectional or forward) is untenable, as it would either increase the surface brightness of fall to obscure the surface details. The limb darkening of Mars is mainly the results of absorption by the smoke. The opacity of the Martian atmosphere increases from the red toward the violet. The extinction by the Martian atmosphere is greater than that by the terrestrial at all wavelengths, but only about 20 per cent of the Martian extinction is due to scattering. Dollfus' polarimeteric estimate, corrected for self-absorption, corresponds to a martian atmospheric pressure of 87 mm Hg. The photochemical breakup of carbon dioxide and the escape of oxygen must lead to considerable concentrations of carbon monoxide in the martian atmosphere.

HAZE↗

Estimation of microwave absorption in the Jupiter atmosphere

A procedure for estimating the microwave absorption loss of the Jupiter atmosphere is presented. Estimation of microwave absorption by planetary atmospheres involves two different investigative disciplines (1) the determination of an acceptable model of the atmosphere itself and (2) the determination of the microwave attenuation rate applicable to each different volume sample of the atmosphere, and the integration of this loss over the varying radio propagation path for any given entry trajectory to obtain the total loss.

Coombs, W. C.↗

Investigation of line-of-sight propagation in dense atmosphere, phase 3, part 1

The investigation of microwave absorption in the 1 to 10 GHz frequency band by the Jovian atmosphere has continued, and an estimate of the strength of signal fading at these frequencies due to layers of turbulence in Jupiter's atmosphere is given. The microwave absorption due to gaseous ammonia is estimated both in terms of a power loss in dB/km, and in total power loss in dB for slant-path communication with a probe at altitudes down to pressures of several tens of atmospheres. The graphs indicate a frequency-squared scaling of the absorption, and appreciable losses at altitudes where the pressure is several atmospheres. An estimate of turbulence strength is given. This may turn out to be quite crude considering the absence of any relevant data. A planetary scaling law which appears to hold reasonably well for Earth to Venus, is extrapolated to Jupiter. No reasonable modifications of the estimate can alter the conclusion that direct-path fading is negligible for pressure regimes up to 20 atm.

Dewolf, D. A.↗

Some aspects of remote atmospheric sensing by laser radar

An analysis has been made of some aspects of atmospheric sensing by laser radar spectroscopy. A discussion of the laser radar equation is presented which leads to methods for obtaining atmospheric information by spectroscopic means. Calculations are presented which investigate the potential of Doppler, Raman and differential absorption techniques. It is concluded that atmospheric measurements based upon Doppler and Raman approaches are restricted to qualitative studies at the present time primarily because of the limitations imposed by existing laser sources and detectors. It is probable that these limitations will be removed in the near future and it is recommended that exploratory experiments be continued. The differential absorption method for obtaining the spatial distribution of atmospheric gases is well developed for such gases as water vapor and oxygen where the basic laser frequency lies close to the center of the particular absorption line. Further investigation is recommended in the field of laser frequency shifting. Additional information is also required on the shape of the absorption line, particular in the region where the line reflects both pressure and Doppler broadening.

Schotland, R. M.↗

Radiometer for remote sounding of the upper atmosphere.

The pressure-modulated carbon dioxide radiometer is a new kind of instrument capable of making temperature soundings in the 40-80-km region of the earth's atmosphere. It is intended to be mounted on a polar-orbiting satellite, where it will give global coverage of the upper atmosphere in a region that is not well understood at present but that is, as rocket soundings show, clearly the seat of many interesting and vigorous phenomena. The new technique employs a cell containing carbon dioxide as a filter. The pressure and hence transmission of this cell is periodically modulated, resulting in the selection of thermal radiation from the strong lines in the spectrum of atmospheric carbon dioxide. This radiation originates at levels in the atmosphere where the pressure is low. The energy grasp of the device is large enough to give high sensitivity.

Taylor, F. W.↗

Planetary atmospheres.

Study of the composition of the atmospheres of the planets. Their wide variety is of interest in view of the fact that all nine planets were probably formed at the same time and out of the same chemically homogeneous mixture of gas and dust, i.e., the primitive solar nebula. The most likely explanation for this diversity in composition seems to be that the planetary atmospheres have undergone important evolutionary changes during their history of about 4.5 billion years. The early history of the earth's atmosphere is reviewed, as well as that of Venus and Mars. The most interesting aspect of Jupiter is that its present atmosphere seems to be composed of the same gases, hydrogen, methane, and ammonia, out of which the first living organisms are believed to have been synthesized on the earth.

Rasool, S. I.↗

Atmospheric waves and the ionosphere.

A review of evidence supporting the existence of atmospheric waves is presented, and a simple, theoretical approach for describing them is shown. Suggestions for gravity wave sources include equatorial and auroral electrojet, auroral and polar substorm heating, atmospheric jet streams, and large oceanic tides. There are reviewed previous studies dealing with the interaction between ionization and atmospheric waves believed to exist at ionospheric heights. These waves include acoustic waves, evanescent waves, and internal atmospheric gravity waves. It is explained that mode analysis, often employed when an increased number of layers is used for a more complete profile, is inapplicable for waves very close to a source.

Beer, T.↗

The bulk composition of Titan's atmosphere.

Consideration of the physical constraints for Titan's atmosphere leads to a model which describes the bulk composition of the atmosphere in terms of observable parameters. Intermediate-resolution photometric scans of both Saturn and Titan, including scans of the Q branch of Titan's methane band, constrain these parameters in such a way that the model indicates the presence of another important atmospheric gas, namely, another bulk constituent or a significant thermal opacity. Further progress in determining the composition and state of Titan's atmosphere requires additional observations to eliminate present ambiguities. For this purpose, particular observational targets are suggested.

Trafton, L.↗