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At least 1,099 records · Page 61

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NASA NTRS1974

Fluid dynamic studies on scattering aerosol and its generation for application as tracer particles in supersonic flow measurements utilizing laser Doppler velocimeter

An experimental study on the particle-fluid interactions of scattering aerosols was performed using monodisperse aerosols of different particle sizes for the application of laser Doppler velocimeters in subsonic turbulence measurements. Particle response was measured by subjecting the particles to an acoustically excited oscillatory fluid velocity field and by comparing the ratio of particle velocity amplitude to the fluid velocity amplitude as a function of particle size and the frequency of oscillation. Particle velocity was measured by using a differential laser Doppler velocimeter. The test aerosols were fairly monodisperse with a mean diameter that could be controlled over the size range from 0.1 to 1.0 micron. Experimental results on the generation of a fairly monodisperse aerosol of solid particles and liquid droplets and on the aerosol response in the frequency range 100 Hz to 100 kHz are presented. It is indicated that a unit density spherical scatterer of 0.3 micron-diameter would be an optimum choice as tracer particles for subsonic air turbulence measurements.

Mazumder, M. K.↗

NASA NTRS1976

A thermoluminescent method for aerosol characterization

A thermoluminescent method has been used to study the interactions of aerosols with ozone. The preliminary results show that ozone reacts with many compounds found in aerosols, and that the thermoluminescence curves obtained from ozonated aerosols are characteristic of the aerosol. The results suggest several important applications of the thermoluminescent method: development of a detector for identification of effluent sources; a sensitive experimental tool for study of heterogeneous chemistry; evaluation of importance of aerosols in atmospheric chemistry; and study of formation of toxic, electronically excited species in airborne particles.

Long, E. R., Jr.↗

NASA NTRS1975

Preferential concentration of certain elements in smaller aerosols emitted from aircraft engines

Aerosols from aircraft engines were collected with an eight-stage cascade sampler for a period of 24 h. The aerosol samples from each stage were analyzed for their elemental composition using the proton-induced X-ray emission (PIXE) technique. Seventeen elements (Si, P, S, Cl, K, Ca, Ti, V, Fe, Ni, Cu, Zn, Br, Sr, Nb, Sn, and Pb) were positively identified and quantitated at each stage. Six elements (S, Ca, Fe, Zn, Sn, and Pb) showed a fractional concentration increase with decreasing aerosol size. Similar, but less well-defined, trends were also observed for V and Ni. Silicon and chlorine, on the other hand, showed an opposite trend. Neutron-activation analysis of bulk aerosol samples collected every 2 h over the same period showed a correlation between concentration of Si, Ca, V, Ti, Zn, Br, and Sn and the density of air traffic at the airport. Analysis of the aviation-fuel samples by PIXE indicates that major fractions of Pb, Sn, Br, Zn, Ni, Fe, V, Ca, and S observed in these aerosol studies come from the aircraft engine exhaust.

Jolly, R. K.↗

NASA NTRS1974

Generation and fluid dynamics of scattering aerosols in laser Doppler velocimetry

An experimental study on the particle-fluid interactions of scattering aerosols was performed using monodisperse aerosols of different particle sizes for the application of laser Doppler velocimeters in subsonic turbulence measurements. Particle response was measured by subjecting the particles to an acoustically excited flow field where the particle Reynolds numbers were controlled to simulate the corresponding values of fluid turbulence. The test aerosols were fairly monodisperse with a mean diameter that could be controlled over the size range from 0.1 to 1.0 micron. Experimental results on the generation of a fairly monodisperse aerosol of solid particles and liquid droplets and on the aerosol response in the frequency range 100 Hz to 100 kHz are presented. The present study indicates that a unit density spherical scatterer of 0.3 micron-diameter would be an optimum choice as tracer particles for subsonic air turbulence measurements.

Mazumder, M. K.↗

NASA NTRS1976

A kinetic study of the interaction between atomic oxygen and aerosols

This study was concerned with the effects of NH4Cl and (NH4)2SO4 aerosols on the kinetics of disappearance of atomic oxygen. Atomic oxygen was generated by a 2.45-GHz microwave discharge and the kinetics of disappearance measured in a fast flow system using NO2 titration. Values of the recombination coefficient for heterogeneous wall recombination were determined for clean, H2SO4-coated, and (NH4)2SO4-coated Pyrex to be 0.000050, 0.000020, and 0.000019, respectively. A rapid exothermic chemical reaction was found to occur between atomic oxygen and an NH4Cl wall coating; the products were NH3, NO, H2O, and HCl. The NH4Cl aerosol was generated by gas phase reaction of NH3 with HCl. The aerosol particles were approximately spherical and nearly monodisperse with a mean diameter of 1.6 plus or minus 0.2 micron. The rate constant for the disappearance of atomic oxygen in the presence of NH4Cl aerosol was measured. No significant decrease was observed in the rate of disappearance of atomic oxygen in the presence of an (NH4)2SO4 aerosol at a concentration of 285 mg per cu m.

Akers, F. I.↗

NASA NTRS1976

The aerosol distribution in Uranus' atmosphere - Interpretation of the hydrogen spectrum

New observations of Uranus' combined H2 spectrum have been obtained. An analysis, emphasizing the leverage provided by the S3(0) quadrupole line, leads to strong constraints on Uranus' bulk aerosol distribution with depth. Using an inhomogeneous model atmosphere program which includes Rayleigh scattering for gases and a 1 plus cos theta phase function for cloud layers, it is shown that Uranus' H2 spectrum implies a cloud layer (or dense aerosol) at a depth from 500 to 700 km-amagat H2. It also implies negligible aerosol scattering in the 280 to 450 km-amagat H2 region and a thin haze at 100 to 200 km-amagat H2 depths. The low albedo in very strong CH4 bands indicates that there is negligible aerosol scattering in Uranus' radiative zone. Hydrogen appears to be more abundant than the sum of all other atmospheric gases. The C/H ratio deep in Uranus' atmosphere is strongly enhanced over the solar value. Accurate limb-darkening measurements in and near strong CH4 bands would be effective in specifying Uranus' aerosol distribution in greater detail.

Trafton, L.↗

NASA NTRS1976

Non-dimensional groups in the description of finite-amplitude sound propagation through aerosols

Several parameters, which have fairly transparent physical interpretations, appear in the analytic description of finite-amplitude sound propagation through aerosols. Typically, each of these parameters characterizes, in some sense, either the sound or the aerosol. It also turns out that fairly obvious combinations of these parameters yield non-dimensional groups which, in turn, characterize the nature of the acoustic-aerosol interaction. This theme is developed in order to illustrate how a quick examination of such parameters and groups can yield information about the nature of the processes involved, without the necessity of extensive mathematical analysis. This concept is developed primarily from the viewpoint of sound propagation through aerosols, although complimentary acoustic-aerosol interaction phenomena are briefly noted.

Scott, D. S.↗

NASA NTRS1976

Monitoring stratospheric ozone and aerosols using orbiting photoelectric detectors

Application of slightly modified off-the-shelf automatic celestial navigation systems ('star trackers') is considered for the purposes of monitoring variations in the optical depth of the stratospheric aerosol and ozone layers. The basic principle of the technique is to observe stars from an orbiting station as they are occulted by the stratospheric aerosol layer. Since molecular and refraction extinction are directly calculable, total extinction measurements using a dual-sensor (S4 and S20) approach allows us to directly solve for ozone and aerosol extinction and look for correlations between these two parameters. The technique appears promising for remotely monitoring aerosol and ozone optical depth in the 15-25 km region over selected locations and is independently accurate if aerosol composition and relative size distribution are invariant.

Matloff, G. L.↗

NASA NTRS1978

Trace elemental characteristics of aerosols emitted from municipal incinerators

As part of a continuing investigation of high temperature combustion aerosols, elemental composition of size differentiated aerosols emitted from a local municipal incinerator was studied. Aerosols were aerodynamically separated into eight diameter groups ranging from 0.43 mm to 20 mm, collected, and analyzed by charged particle induced X-ray emission technique. On line data collection and reduction codes generated aerial densities for elements from Na to U with sensitivities in the ng/cu m range for most elements. From the total weights of aerosols collected per stage, their size distribution was determined to be bimodal, with one group centered at a diameter of 0.54 mm and the other at a diameter of 5.6 mm. Measured elemental concentrations in various size ranges indicate that K and S show a strong tendency to concentrate on aerosol surfaces. A weaker trend for surface preference was also observed for Mn and Ni, but other elements show no such trend.

Singh, J. J.↗

NASA NTRS1978

Albedo enhancement and perturbation of radiation balance due to stratospheric aerosols

The effect of stratospheric aerosols on the earth's monthly zonal radiation balance is investigated using a model layer consisting of 75% H2SO4, which is the primary constituent of the background aerosol layer. The reduction in solar energy absorbed by the earth-atmosphere system is determined through the albedo sensitivity, defined here as the change in albedo per unit mid-visible optical depth of the aerosol layer. The optically thin approximation is used in conjunction with the Henyey-Greenstein phase function for scattering to simplify computations. Satellite derived planetary albedos are used as the frame of reference about which the change in albedo is computed. An infrared radiative transfer model is used to estimate the increased greenhouse effect attributed to the aerosol layer. The infrared heating tends to compensate for the albedo effect in altering the radiation balance. The results indicate that the dominant influence of the thin model stratospheric aerosol layer is an increased reflection of solar energy all over the globe except for the polar-winter region, but the change in the radiation balance is seen to be uniform and small equatorwards of 50%.

HARSHVARDHAN↗

NASA NTRS1978

Post-volcanic stratospheric aerosol decay as measured by lidar

The paper summarizes and discusses results of lidar observations, at Hampton (Virginia), of the stratospheric aerosol vertical distribution for a period of 22 months (October 1974 to July 1976) after the volcanic eruption of the Volcan de Fuego in Guatemala. Data are presented in terms of lidar scattering ratio, vertically integrated aerosol backscattering, layer structure and location, and rawinsonde temperature profiles as a function of time. The results reveal a sudden increase in the stratospheric aerosol content after the volcanic eruption as well as its subsequent decline. There exists a high degree of correlation between the integrated aerosol backscattering and the tropopause height such that as one decreases the other increases and vice versa. Rapid decay of the stratospheric aerosol is found to occur over the late winter to early spring period.

Mccormick, M. P.↗

NASA NTRS1979

The investigation of advanced remote sensing techniques for the measurement of aerosol characteristics

Advanced remote sensing techniques and inversion methods for the measurement of characteristics of aerosol and gaseous species in the atmosphere were investigated. Of particular interest were the physical and chemical properties of aerosols, such as their size distribution, number concentration, and complex refractive index, and the vertical distribution of these properties on a local as well as global scale. Remote sensing techniques for monitoring of tropospheric aerosols were developed as well as satellite monitoring of upper tropospheric and stratospheric aerosols. Computer programs were developed for solving multiple scattering and radiative transfer problems, as well as inversion/retrieval problems. A necessary aspect of these efforts was to develop models of aerosol properties.

Deepak, A.↗

NASA NTRS1979

The NASA-Ames Research Center stratospheric aerosol model. 2. Sensitivity studies and comparison with observatories

Sensitivity tests were performed on a one-dimensional, physical-chemical model of the unperturbed stratospheric aerosols, and model calculations were compared with observations. The tests and comparisons suggest that coagulation controls the particle number mixing ratio, although the number of condensation nuclei at the tropopause and the diffusion coefficient at high altitudes are also important. The sulfur gas source strength and the aerosol residence time are much more important than the supply of condensation nuclei in establishing mass and large particle concentrations. The particle size is also controlled mainly by gas supply and residence time. In situ observations of the aerosols and laboratory measurements of aerosols, parameters that can provide further information about the physics and chemistry of the stratosphere and the aerosols found there are provided.

Toon, O. B.↗

NASA NTRS1979

Latitudinal variations of stratospheric aerosols

We have obtained stratospheric aerosols from tropical to northern latitudes using special collectors on U-2 aircraft during 1976 and 1977. Aerosols characterized by large numbers of small particles are found in the tropical zone suggesting this is a region of particle growth; whereas aerosols containing mostly larger particles are distributed throughout the Northern Hemisphere indicating a well-mixed, mature population. We find the aerosol layer extends from higher altitudes near the equator to lower ones toward the pole. Although this gradient suggests mature aerosols may leave the stratosphere at high latitudes, the data are, as yet, inconclusive. Comparisons of our data with those of other investigators using different instruments are generally encouraging, suggesting that if similar populations were sampled, the results would be similar. When our calculated sulfate mass mixing ratios are compared with those measured directly by others, we find better agreement is achieved if we assume more dilute sulfate and water mixtures than previously proposed.

Farlow, N. H.↗

NASA NTRS1980

Stratospheric aerosol modification by supersonic transport and space shuttle operations - Climate implications

The potential effects on stratospheric aerosols of supersonic transport emissions of sulfur dioxide gas and submicron soot granules, and space shuttle rocket emissions of aluminum oxide particulates are estimated. An interactive particle-gas model of the stratospheric aerosol layer is used to calculate changes due to exhaust emissions, and an accurate radiation transport model is employed to compute the effect of aerosol changes on the earth's average surface temperature. It is concluded that the release of large numbers of small particles (soot or aluminum oxide) into the stratosphere should not lead to a corresponding significant increase in the concentration of large, optically active aerosols, but that the increase in large particles is severely limited by the total mass of sulfate available to make large particles in situ, and by the rapid loss of small seed particles via coagulation. We find that a fleet of several hundred advanced supersonic aircraft operating daily at 20 km, or the launch of one space shuttle rocket per week, could produce roughly a 20% increase in the large-particle concentration of the stratosphere. We find, in addition, that aerosol increases of this magnitude would reduce the global surface temperature by less than 0.01 K.

Turco, R. P.↗

NASA NTRS1979

Formation and deposition of volcanic sulfate aerosols on Mars

The paper considers the formation and deposition of volcanic sulfate aerosols on Mars. The rate limiting step in sulfate aerosol formation on Mars is the gas phase oxidation of SO2 by chemical reactions with O, OH, and HO2; submicron aerosol particles would circuit Mars and then be removed from the atmosphere by gravitational forces, globally dispersed, and deposited over a range of equatorial and mid-latitudes. Volcanic sulfate aerosols on Mars consist of liquid droplets and slurries containing sulfuric acid; aerosol deposition on a global or hemispheric scale could account for the similar concentrations of sulfur within surficial soils at the two Viking lander sites.

Settle, M.↗

NASA NTRS1981

Measurements of the absorption coefficient of stratospheric aerosols

The absorption coefficients of stratospheric aerosols are measured using a variation on the integrating plate method. The technique is based on the decrease in the transparency of a substrate when an absorbing aerosol is deposited on it. A Lambert scatterer is placed behind the substrate to integrate forward scattered light and minimize the effect of scattering on the measurement. The low pressure in the stratosphere is used for the direct impaction of particles onto a narrow strip of opal glass. The eight samples collected had a median value of 4 x 10 to the -9th m with an uncertainty of + or - 5 x 10 to the -9th m. If this absorption is due to graphitic carbon, then its concentration is estimated at about 0.4 ng/cu m, or about 0.25% of the total aerosol mass concentration. Estimates of the aerosol scattering coefficients based on satellite extinction inversions result in an aerosol single-scattering albedo in the range of 0.96-1.0.

Ogren, J. A.↗

NASA NTRS1981

SAM 2 measurements of the polar stratospheric aerosol, volume 1: October to April 1979

Weekly averages of Antarctic and Arctic stratospheric aerosol data as well as corresponding temperature profiles for the time and place of each stratospheric aerosol measurement (SAM) II measurement during the first 6 months of satellite flight are presented. From the aerosol extinction profile data, contours of aerosol extinction as a function of altitude and longitude or time are plotted. Aerosol optical depths are calculated for each week. Polar stratospheric clouds at altitudes of about 22 km were observed during the Arctic winter at various times and locations. A representative sample of the first 6 months of data to be used in atmospheric and climatic studies is outlined.

Mccormick, M. P.↗