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At least 1,081 records · Page 60
All sourcesNASA NTRSDOE OSTI
DOE OSTI2015

METHANOL IN THE STARLESS CORE, TAURUS MOLECULAR CLOUD-1

To explore the formation mechanisms of gas phase CH{sub 3}OH in cold starless cores, we have conducted high spectral resolution observations toward the cyanopolyyne peak of Taurus Molecular Cloud-1 (TMC-1 CP) with the IRAM 30 m telescope, the Green Bank Telescope, and the Nobeyama 45 m telescope. The spectral lines of CH{sub 3}OH toward TMC-1 CP are found to have a double-peaked profile separated by 0.5 km s{sup −1}. Since the double-peaked profile is observed for {sup 13}CH{sub 3}OH, it is not due to optical depth and/or self-absorption effects. The spectral line profile of CH{sub 3}OH is much different from those of C{sup 34}S, C{sub 3}S, and HC{sub 7}N observed toward this source. The H{sub 2} densities of the emitting region of CH{sub 3}OH for the blueshifted and redshifted components are derived to be (1.7 ± 0.5) × 10{sup 4} cm{sup −3} and (4.3 ± 1.2) × 10{sup 4} cm{sup −3}, respectively. These densities are similar to or slightly lower than those found for the other molecules. These results suggest a chemical differentiation between CH{sub 3}OH and the other molecules, which has indeed been confirmed by mapping observations of the CH{sub 3}OH and C{sup 34}S lines. These results are consistent with the general idea that CH{sub 3}OH is formed on dust grains and is liberated into the gas phase by non-thermal desorption. The grain-surface origin of CH{sub 3}OH is further confirmed by the CH{sub 3}OH/{sup 13}CH{sub 3}OH ratio. Weak shocks caused by accreting diffuse gas to the TMC-1 filament, photoevaporation caused by cosmic-ray induced UV radiation, and the desorption of excess reaction energy in the formation of CH{sub 3}OH on dust grains are discussed for the desorption mechanisms.

79 ASTRONOMY AND ASTROPHYSICS↗
NASA NTRS2018

Changes in Earth’s Energy Budget during and after the “Pause” in Global Warming: An Observational Perspective

This study examines changes in Earth’s energy budget during and after the global warming “pause” (or “hiatus”) using observations from the Clouds and the Earth’s Radiant Energy System. We find a marked 0.83±0.41 Wm−2 reduction in global mean reflected shortwave (SW) top-of-atmosphere (TOA) flux during the three years following the hiatus that results in an increase in net energy into the climate system. A partial radiative perturbation analysis reveals that decreases in low cloud cover are the primary driver of the decrease in SW TOA flux. The regional distribution of the SW TOA flux changes associated with the decreases in low cloud cover closely matches that of sea-surface temperature warming, which shows a pattern typical of the positive phase of the Pacific Decadal Oscillation. Large reductions in clear-sky SW TOA flux are also found over much of the Pacific and Atlantic Oceans in the northern hemisphere. These are associated with a reduction in aerosol optical depth consistent with stricter pollution controls in China and North America. A simple energy budget framework is used to show that TOA radiation (particularly in the SW) likely played a dominant role in driving the marked increase in temperature tendency during the post-hiatus period.

Norman G Loeb↗
NASA NTRS2017

Mitigating Satellite-Based Fire Sampling Limitations in Deriving Biomass Burning Emission Rates: Application to WRF-Chem Model over the Northern sub-Saharan African Region

Largely used in several independent estimates of fire emissions, fire products based on MODIS sensors aboard the Terra and Aqua polar-orbiting satellites have a number of inherent limitations, including (a) inability to detect fires below clouds, (b) significant decrease of detection sensitivity at the edge of scan where pixel sizes are much larger than at nadir, and (c) gaps between adjacent swaths in tropical regions. To remedy these limitations, an empirical method is developed here and applied to correct fire emission estimates based on MODIS pixel level fire radiative power measurements and emission coefficients from the Fire Energetics and Emissions Research (FEER) biomass burning emission inventory. The analysis was performed for January 2010 over the northern sub-Saharan African region. Simulations from WRF-Chem model using original and adjusted emissions are compared with the aerosol optical depth (AOD) products from MODIS and AERONET as well as aerosol vertical profile from CALIOP data. The comparison confirmed an 30-50% improvement in the model simulation performance (in terms of correlation, bias, and spatial pattern of AOD with respect to observations) by the adjusted emissions that not only increases the original emission amount by a factor of two but also results in the spatially continuous estimates of instantaneous fire emissions at daily time scales. Such improvement cannot be achieved by simply scaling the original emission across the study domain. Even with this improvement, a factor of two underestimations still exists in the modeled AOD, which is within the current global fire emissions uncertainty envelope. Plain Language Summary Polar-orbiting satellites sensors, such as MODIS, have limitations in detecting fires under clouds or when viewing angles are large or in the gaps among satellites' different ground swaths. Here we developed an empirical method to mitigate the effect of these limitations in fire emission estimate. The method is applied to a fire emission inventory (FEER) based on MODIS. We show that, with our method, the adjusted emission inventory improves WRF-Chem simulation of smoke transport and distribution.

emissions properties↗
NASA NTRS1997

Radiative Closure Experiments at a Cloud-Free Desert Site, Nevada, as Part of MISR Algorithm Validation

Radiative closure experiments involving a comparison between surface-measured spectral irradiance and the surface irradiance calculated according to a radiative transfer code at a desert site in Nevada under clear skies, yield the result that agreement between the two requires presence of an absorbing aerosol component with an imaginary refractive index equal to 0.03 and a 50:50 mix by optical depth of small and large particles with log-normal size distributions.

MISR experiment field observations calibration dat↗
NASA NTRS2022

Tracking the 2022 Hunga Tonga-Hunga Ha'Apai Aerosol Cloud in the Upper and Middle Stratosphere Using Space-Based Observations

On 15 January 2022, the submarine Hunga Tonga volcanic eruption lofted materials high into the upper stratosphere, reaching a record-breaking altitude of ~58 km, unprecedented in the satellite observations era. Within two weeks, the bulk of the injected material circulated the globe between 20 – 30 km altitude, as observed by satellite instruments. We estimate that the stratospheric aerosol optical depth (sAOD) is the largest since the Pinatubo eruption and is at least twice as great as the sAOD after the 2015 Calbubo eruption despite the similar SO 2 injection from that eruption. We use space-based observations to monitor the Hunga-Tonga volcanic plume evolution and transport at different altitudes as it circulates the globe. While the main aerosol layer remains trapped in the tropical pipe, small parts have already made it to both the northern and southern hemisphere poles by April, which is almost certain to influence this year's ozone hole.

Atmospheric science↗
NASA NTRS1985

SAM 2 measurements of the polar stratospheric aerosol, volume 5

The Stratospheric Aerosol Measurement (SAM) 2 sensor is aboard the Earth-orbiting Nimbus 7 spacecraft providing extinction measurements of the Antarctic and Arctic stratospheric aerosol with a vertical resolution of 1 km. Representative examples and weekly averages of aerosol data and corresponding temperature profiles for the time and place of each SAM 2 mesurement (Oct. 1980 through Apr. 1981) are presented. Contours of aerosol extinction as a function of altitude and longitude or time are plotted and weekly aerosol optical depths are calculated. Seasonal variations and variations in space (altitude and longitude) for both polar regions are easily seen. Stratospheric optical depths are 0.002 to 0.003 for the Antarctic region and 0.005 to 0.006 at the beginning to 0.002 to 0.003 at the end of the time period for the Arctic region. The Northern Hemisphere values are quite large due mainly to the eruption of Mount St. Helens (46.2 deg N, 122.2 deg W) in May 1980. Polar stratospheric clouds at altitudes of about 20 km were observed during the Arctic winter. A ready-to-use format containing a representative sample of the fifth 6 months of data to be used in atmospheric and climatic studies is presented.

Mccormick, M. P.↗
NASA NTRS1986

Multiband far-infrared observations of the NGC 6334 complex

Multiband far-infrared (20-155 microns) observations of the large H II region/molecular cloud complex NGC 6334 are presented. The observations were performed simultaneously in four bands with effective wavelengths 21, 42, 71, and 134 microns. Eight far-infrared sources were detected which cover the range from sources with little of no continuum radio emission to well-developed H II regions. Maps of dust temperature and far-infrared optical depth of the complex are presented which reveal large-scale variations in the color temperature and optical depth. Star formation in the complex is discussed and it is concluded that a Rayleigh-Taylor instability generated by the gravitational attraction of the galactic plane can explain the regular separation of the far-IR sources.

Loughran, L.↗
NASA NTRS1990

Radiative heating rates in the tropical monsoon environment - A case study

A study designed to investigate the radiative impact of high clouds through a combination of modeling and data analysis is presented. A series of high-altitude survey flights was conducted utilizing a NASA Ames ER-2 aircraft carrying a nadir-viewing narrow field-of-view radiometer, with channels at 6.5 and 10.5 microns. The two intensities obtained by this radiometer can be employed to deduce optical depth as described by Liou et. al. (1990).

Heffernan, C. M.↗
NASA NTRS2015

Comparison of GFED3, QFED2 and FEER1 Biomass Burning Emissions Datasets in a Global Model

Biomass burning contributes about 40% of the global loading of carbonaceous aerosols, significantly affecting air quality and the climate system by modulating solar radiation and cloud properties. However, fire emissions are poorly constrained in models on global and regional levels. In this study, we investigate 3 global biomass burning emission datasets in NASA GEOS5, namely: (1) GFEDv3.1 (Global Fire Emissions Database version 3.1); (2) QFEDv2.4 (Quick Fire Emissions Dataset version 2.4); (3) FEERv1 (Fire Energetics and Emissions Research version 1.0). The simulated aerosol optical depth (AOD), absorption AOD (AAOD), angstrom exponent and surface concentrations of aerosol plumes dominated by fire emissions are evaluated and compared to MODIS, OMI, AERONET, and IMPROVE data over different regions. In general, the spatial patterns of biomass burning emissions from these inventories are similar, although the strength of the emissions can be noticeably different. The emissions estimates from QFED are generally larger than those of FEER, which are in turn larger than those of GFED. AOD simulated with all these 3 databases are lower than the corresponding observations in Southern Africa and South America, two of the major biomass burning regions in the world.

biomass burning↗
NASA NTRS2017

Remote Sensing of Multiple Cloud Layer Heights Using Multi-Angular Measurements

Cloud top height (CTH) affects the radiative properties of clouds. Improved CTH observations will allow for improved parameterizations in large-scale models and accurate information on CTH is also important when studying variations in freezing point and cloud microphysics. NASAs airborne Research Scanning Polarimeter (RSP) is able to measure cloud top height using a novel multi-angular contrast approach. For the determination of CTH, a set of consecutive nadir reflectances is selected and the cross-correlations between this set and co-located sets at other viewing angles are calculated for a range of assumed cloud top heights, yielding a correlation profile. Under the assumption that cloud reflectances are isotropic, local peaks in the correlation profile indicate cloud layers. This technique can be applied to every RSP footprint and we demonstrate that detection of multiple peaks in the correlation profile allow retrieval of heights of multiple cloud layers within single RSP footprints. This paper provides an in-depth description of the architecture and performance of the RSPs CTH retrieval technique using data obtained during the Studies of Emissions and Atmospheric Composition, Clouds and Climate Coupling by Regional Surveys (SEAC(exp. 4)RS) campaign. RSP retrieved cloud heights are evaluated using collocated data from the Cloud Physics Lidar (CPL). The method's accuracy associated with the magnitude of correlation, optical thickness, cloud thickness and cloud height are explored. The technique is applied to measurements at a wavelength of 670 nm and 1880 nm and their combination. The 1880-nm band is virtually insensitive to the lower troposphere due to strong water vapor absorption.

Sinclair, Kenneth↗
DOE OSTI2018

First forcing estimates from the future CMIP6 scenarios ofanthropogenic aerosol optical properties and an associated Twomeyeffect

We present the first forcing interpretation of the future anthropogenic aerosol scenarios of CMIP6 with the simple plumes parameterisation MACv2-SP. The nine scenarios for 2015 to 2100 are based on SO 2 and NH 3 emissions for use in CMIP6 (Riahi et al., 2017; Gidden et al., in prep.). We use the emissions to scale the observationally informed anthropogenic aerosol optical properties and the associated effect on the cloud albedo of present-day (Fiedler et al., 2017; Stevens et al., 2017) into the future. The resulting scenarios in MACv2-SP are then ranked according to their strength in forcing magnitude and spatial asymmetries. Almost all scenarios show a decrease in anthropogenic aerosol by 2100 with a range of 108 % to 36 % of the anthropogenic aerosol optical depth in 2015. We estimate the spread in the radiative forcing associated with the scenarios in the mid-2090s by performing ensembles of simulations with the atmosphere-only configuration of MPI-ESM1.2. MACv2-SP herein translates the CMIP6 emission scenarios for inducing aerosol forcing. With the implementation in our model, we obtain forcing estimates for both the shortwave instantaneous (RF) and effective radiative forcing (ERF) relative to 1850. Here, ERF accounts for rapid atmospheric adjustments and natural variability internal to the model. The spread for the mid-2090s is −0.20 to −0.57 Wm −2 (−0.15 to −0.54 Wm −2 ) for RF (ERF) of anthropogenic aerosol, associated with uncertainty in the emission pathway alone, i.e., the mid-2090s forcing ranges from 33–95% (30–108%) of the mid-2000s RF (ERF). We find a larger ERF spread of −0.15 to −0.92 Wm −2 , when we additionally consider uncertainty in the magnitude of the Twomey effect. The year-to-year standard deviations around 0.3 Wm −2 associated with natural variability highlights the necessity for averaging over sufficiently long time periods for estimating ERF, in contrast to RF that is typically well constrained after simulating just one year. The scenario interpretation of MACv2-SP will be used within the framework of CMIP6 and other cutting-edge scientific endeavours.

60 APPLIED LIFE SCIENCES↗
DOE OSTI2019

Chemical Imaging of Atmospheric Organic Particles in the Southern Great Plains Field Campaign Report

The main goal of this field project was to characterize the chemical and physical properties of atmospheric particles representative of the Southern Great Plains (SGP) environment to establish a relationship between the composition of aerosol particles and their atmospheric impacts. The specific research efforts were focused on in-depth microscopy studies of chemical and physical properties of atmospheric organic particles collected at the U.S. Department of Energy’s Atmospheric Radiation Measurement (ARM) SGP observatory. An array of novel molecular-level characterization and chemical imaging approaches were used to characterize chemical composition of particles and elucidate fundamental processes governing their atmospheric aging, evolution of chemical composition, optical properties, cloud formation ability, and implications for particle-cloud interactions – the most challenging problems relevant to predictive understanding of aerosol effects on climate.(1, 2) Atmospheric particles consist of a complex mixture of organic compounds with a wide range of molecular structures, morphologies, physical properties, and chemical reactivity. The chemical composition, morphology, and phase state of atmospheric particles are of crucial importance for understanding the formation and reaction mechanisms of particles, their atmospheric evolution, and their impact on climate. It is of great interest to understand how the chemical and morphological particle microstructure affects their physicochemical properties such as chemical reactivity, thermodynamics of gas-particle partitioning, phase separations inside individual particles, hygroscopicity, optical properties, and ability to form liquid droplets (cloud condensation nuclei) and ice crystals (ice nuclei) in clouds. The phase state of organic particles, which yet remains poorly understood, plays a key role in their physicochemical properties and has important implications in various atmospheric processes. Fundamental understanding of these physicochemical properties and their possible evolution in time requires advanced analytical approaches for chemical imaging of particles with a resolution on the scale of 10-100 nm.(3) Comprehensive characterization of the size-dependent chemical composition of individual particles collected at the site was carried out using advanced molecular-level characterization and imaging approaches to identify their possible sources and to correlate to their climatic properties.

Southern Great Plains, aerosols, HI-SCALE field ca↗
NASA NTRS2011

An Accuracy Assessment of the CALIOP/CALIPSO Version 2/Version 3 Daytime Aerosol Extinction Product Based on a Detailed Multi-Sensor, Multi-Platform Case Study

The Cloud Aerosol LIdar with Orthogonal Polarization (CALIOP), on board the CALIPSO platform, has measured profiles of total attenuated backscatter coefficient (level 1 products) since June 2006. CALIOP s level 2 products, such as the aerosol backscatter and extinction coefficient profiles, are retrieved using a complex succession of automated algorithms. The goal of this study is to help identify potential shortcomings in the CALIOP version 2 level 2 aerosol extinction product and to illustrate some of the motivation for the changes that have been introduced in the next version of CALIOP data (version 3, released in June 2010). To help illustrate the potential factors contributing to the uncertainty of the CALIOP aerosol extinction retrieval, we focus on a one-day, multi-instrument, multiplatform comparison study during the CALIPSO and Twilight Zone (CATZ) validation campaign on 4 August 2007. On that day, we observe a consistency in the Aerosol Optical Depth (AOD) values recorded by four different instruments (i.e. spaceborne MODerate Imaging Spectroradiometer, MODIS: 0.67 and POLarization and Directionality of Earth s Reflectances, POLDER: 0.58, airborne High Spectral Resolution Lidar, HSRL: 0.52 and ground-based AErosol RObotic NETwork, AERONET: 0.48 to 0.73) while CALIOP AOD is a factor of two lower (0.32 at 532 nm). This case study illustrates the following potential sources of uncertainty in the CALIOP AOD: (i) CALIOP s low signal-to-noise ratio (SNR) leading to the misclassification and/or lack of aerosol layer identification, especially close to the Earth s surface; (ii) the cloud contamination of CALIOP version 2 aerosol backscatter and extinction profiles; (iii) potentially erroneous assumptions of the aerosol extinction-to-backscatter ratio (Sa) used in CALIOP s extinction retrievals; and (iv) calibration coefficient biases in the CALIOP daytime attenuated backscatter coefficient profiles. The use of version 3 CALIOP extinction retrieval for our case study seems to partially fix factor (i) although the aerosol retrieved by CALIOP is still somewhat lower than the profile measured by HSRL; the cloud contamination (ii) appears to be corrected; no particular change is apparent in the observation-based CALIOP Sa value (iii). Our case study also showed very little difference in version 2 and version 3 CALIOP attenuated backscatter coefficient profiles, illustrating a minor change in the calibration scheme (iv).

Kacenelenbogen, M.↗
DOE OSTI2022

Gas and Cosmic-Ray Properties in the MBM 53, 54, and 55 Molecular Clouds and the Pegasus Loops Revealed by H i Line Profiles, Dust, and Gamma-Ray Data

In studying the interstellar medium (ISM) and Galactic cosmic rays (CRs), uncertainty of the interstellar gas density has always been an issue. To overcome this difficulty, we used a component decomposition of the 21 cm H i emission line and used the resulting gas maps in an analysis of γ-ray data obtained by the Fermi Large Area Telescope (LAT) for the MBM 53, 54, and 55 molecular clouds and the Pegasus loop. We decomposed the ISM gas into intermediate-velocity clouds, narrow-line and optically thick H i, broad-line and optically thin H i, CO-bright H 2 , and CO-dark H 2 using detailed correlations with the H i line profiles from the HI4PI survey, the Planck dust-emission model, and the Fermi-LAT γ-ray data. We found the fractions of the optical depth correction to the H i column density and CO-dark H 2 to be nearly equal. We fitted the CR spectra directly measured at/near the Earth and the measured γ-ray emissivity spectrum simultaneously. We obtained a spectral break in the interstellar proton spectrum at ~7 GeV, and found that the γ-ray emissivity normalization agrees with the AMS-02 proton spectrum within 10%, relaxing the tension with the CR spectra previously claimed.

79 ASTRONOMY AND ASTROPHYSICS↗
NASA NTRS1989

A study of the stellar population in the Lynds 1641 dark cloud - A possible dense cluster associated with IRAS 05338-0624

Sensitive images obtained at 1.6 and 2.2 microns reveal a possible dense cluster of stars associated with IRAS 05338-0624 and located within an optically thick molecular core; the visual extinction suffered by cluster members ranges from 7 to 40 mag. A circular region of diameter 70 arcsec (0.16 pc at a distance of 480 pc) contains 20 stellar objects or semistellar knots. Assuming that the depth of the region is comparable to its projected size leads to an estimated stellar density of 6800/cu pc. The ratio of stellar to molecular material contained within the core must lie between 4 percent and 43 percent. It is likely that this cluster will emerge from its parent core as a bound group.

Strom, Karen M.↗
NASA NTRS2012

Exploring the Longwave Radiative Effects of Dust Aerosols

Dust aerosols not only affect air quality and visibility where they pose a significant health and safety risk, but they can also play a role in modulating the energy balance of the Earth-atmosphere system by directly interacting with local radiative fields. Consequently, dust aerosols can impact regional climate patterns such as changes in precipitation and the evolution of the hydrological cycle. Assessing the direct effect of dust aerosols at the solar wavelengths is fairly straightforward due in part to the relatively large signal-to-noise ratio in broadband irradiance measurements. The longwave (LW) impacts, on the other hand, are rather difficult to ascertain since the measured dust signal level (10 Wm-2) is on the same order as the instrumental uncertainties. Moreover, compared to the shortwave (SW), limited experimental data on the LW optical properties of dust makes it a difficult challenge for constraining the LW impacts. Owing to the strong absorption features found in many terrestrial minerals (e.g., silicates and clays), the LW effects, although much smaller in magnitude compared to the SW, can still have a sizeable impact on the energetics of the Earth-atmosphere system, which can potentially trigger changes in the heat and moisture surface budgets, and dynamics of the atmosphere. The current endeavor is an integral part of an on-going research study to perform detailed assessments of dust direct aerosol radiative effects (DARE) using comprehensive global datasets from NASA Goddards mobile ground-based facility (cf. http://smartlabs.gsfc.nasa.gov/) during previous field experiments near key dust source regions. Here we examine and compare the results from two of these studies: the 2006 NASA African Monsoon Multidisciplinary Activities and the 2008 Asian Monsoon Years. The former study focused on transported Saharan dust at Sal Island (16.73N, 22.93W), Cape Verde along the west coast of Africa while the latter focused on Asian dust at Zhangye China (39.082N, 100.276E), a semi-arid region between the Taklimakan and Gobi deserts. NASA Goddards Giovanni system is used to help map out the spatial distribution of retrieved aerosol optical depths across the latter desert regions. 1-D radiative transfer model constrained by local measurements, including spectral photometry/interferometry and lidar for characterizing the spatiotemporal variability in dust properties and atmospheric conditions, is employed to evaluate the local instantaneous LW DARE of dust both at the surface and at the top of the atmosphere along with heating rate profiles for cloud-free atmospheres. The efficiency in LW DARE and its significance relative to the diurnally averaged SW effects are explored and compared in both studies. Found to be non-negligible, LW DARE is an important component in the study of regional climate variation with important implications for more detailed global assessments.

Hansell, Richard A., Jr.↗
DOE OSTI2015

The NH{sub 3} hyperfine intensity anomaly in high-mass star-forming regions

Anomalous ammonia (NH{sub 3}) spectra, exhibiting asymmetric hyperfine satellite intensity profiles in the (J,K) = (1, 1) inversion transition, have been observed in star-forming regions for over 35 years. We present a systematic study of this “hyperfine intensity anomaly” (HIA) toward a sample of 334 high-mass star forming regions: 310 high-mass (≳100 M{sub ⊙}) clumps and 24 infrared dark clouds. The HIA is ubiquitous in high-mass star forming regions. Although LTE excitation predicts that the intensity ratios of the outer satellites and inner satellites are exactly unity, for this sample the ensemble average ratios are 0.812 ± 0.004 and 1.125 ± 0.005, respectively. We have quantified the HIA and find no significant relationships between the HIA and temperature, line width, optical depth, and the stage of stellar evolution. The fact that HIAs are common in high-mass star-forming regions suggests that the conditions that lead to HIAs are ubiquitous in these regions. A possible link between HIAs and the predictions of the competitive accretion model of high-mass star formation is suggested; however, the expected trends of HIA strength with clump evolutionary stage, rotational temperature, and line width for evolving cores in competitive accretion models are not found. Thus, the exact gas structures that produce HIAs remain unknown. Turbulent gas structures are a possible explanation, but the details need to be explored.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2020

Using CESM-RESFire to understand climate–fire–ecosystem interactions and the implications for decadal climate variability

Large wildfires exert strong disturbance on regional and global climate systems and ecosystems by perturbing radiative forcing as well as the carbon and water balance between the atmosphere and land surface, while short- and long-term variations in fire weather, terrestrial ecosystems, and human activity modulate fire intensity and reshape fire regimes. The complex climate–fire–ecosystem interactions were not fully integrated in previous climate model studies, and the resulting effects on the projections of future climate change are not well understood. Here we use the fully interactive REgion-Specific ecosystem feedback Fire model (RESFire) that was developed in the Community Earth System Model (CESM) to investigate these interactions and their impacts on climate systems and fire activity. We designed two sets of decadal simulations using CESM-RESFire for present-day (2001–2010) and future (2051–2060) scenarios, respectively, and conducted a series of sensitivity experiments to assess the effects of individual feedback pathways among climate, fire, and ecosystems. Our implementation of RESFire, which includes online land–atmosphere coupling of fire emissions and fire-induced land cover change (LCC), reproduces the observed aerosol optical depth (AOD) from space-based Moderate Resolution Imaging Spectroradiometer (MODIS) satellite products and ground-based AErosol RObotic NETwork (AERONET) data; it agrees well with carbon budget benchmarks from previous studies. We estimate the global averaged net radiative effect of both fire aerosols and fire-induced LCC at –0.59±0.52 W m –2 , which is dominated by fire aerosol–cloud interactions (–0.82±0.19 W m –2 ), in the present-day scenario under climatological conditions of the 2000s. The fire-related net cooling effect increases by ~170 % to –1.60±0.27 W m –2 in the 2050s under the conditions of the Representative Concentration Pathway 4.5 (RCP4.5) scenario. Such considerably enhanced radiative effect is attributed to the largely increased global burned area (+19 %) and fire carbon emissions (+100 %) from the 2000s to the 2050s driven by climate change. The net ecosystem exchange (NEE) of carbon between the land and atmosphere components in the simulations increases by 33 % accordingly, implying that biomass burning is an increasing carbon source at short-term timescales in the future. High-latitude regions with prevalent peatlands would be more vulnerable to increased fire threats due to climate change, and the increase in fire aerosols could counter the projected decrease in anthropogenic aerosols due to air pollution control policies in many regions. We also evaluate two distinct feedback mechanisms that are associated with fire aerosols and fire-induced LCC, respectively. On a global scale, the first mechanism imposes positive feedbacks to fire activity through enhanced droughts with suppressed precipitation by fire aerosol–cloud interactions, while the second one manifests as negative feedbacks due to reduced fuel loads by fire consumption and post-fire tree mortality and recovery processes. These two feedback pathways with opposite effects compete at regional to global scales and increase the complexity of climate–fire–ecosystem interactions and their climatic impacts.

54 ENVIRONMENTAL SCIENCES↗