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DOE OSTI2026

Prognostic simulations of mixed-phase clouds with model AC-1D v1.0: the impact of aerosol types and freezing parameterizations on ice crystal budgets

Mixed-phase clouds at high latitudes contribute to the uncertainty in predicting cloud feedbacks and climate sensitivity, mainly due to the complexity of microphysical processes that influence the partitioning between the supercooled liquid and ice phases, and hence, cloud radiative effects on regional scales. Particularly in Arctic mixed-phase clouds, the activation of ice-nucleating particles (INPs) from various aerosol populations remains a leading source of uncertainty. We developed an aerosol-cloud one-dimensional (AC-1D) model, which provides a novel framework to prognostically treat INP and ice crystal budgets while explicitly accounting for polydisperse and multicomponent aerosol that activate INPs following different freezing parameterizations. The AC-1D model is informed by large-eddy simulations to probe the impact of INP representation on predicted ice crystal number concentrations (N i ) and ice crystal budgets in mixed-phase Arctic stratus. We apply three immersion freezing (IMF) parameterizations, two time-independent (singular) and one time-dependent (classical nucleation theory), to predict the evolution of the INP reservoir and resulting ice crystal budget from polydisperse mineral dust, organic (humic-like substances), and sea spray aerosol particle size distributions. Our analysis focuses on how variations in aerosol number concentration and cloud system parameters such as cloud cooling rate, cloud-top entrainment rate, and ice crystal fall speed influence the INP reservoir and ice crystal budgets. Furthermore, this study investigates the competitive ice nucleation dynamics in mixed aerosol environments and provides a process-level quantification of the INP budget terms, which directly controls ice crystal budgets. For all studied case scenarios, the aerosol types and associated particle size distributions significantly impact INP and N i , and the choice between a time-dependent and a singular freezing description yields orders-of-magnitude differences in the predicted INP and N i over the 10 h simulation time, reflecting typical cloud lifetimes. Our results show that the influence of cloud cooling, INP entrainment, and sedimentation varies significantly depending on the chosen freezing parameterization. These findings underscore the critical need for robust IMF parameterizations and precise cloud system observations to enhance the accuracy of models in predicting mixed-phase cloud structure and evolution.

Arctic clouds↗

NASA NTRS2006

Using Microwave Limb Sounder Data to Validate Model Ice Fields

MLS IWC overall tends to be higher relative to ECMWF after considering MLS track sampling and sensitivity (cutoff application). Disagreement tends to be accentuated over Indian and Western Pacific Oceans and over tropical landmasses. Large disagreement occur at upper level at 147 hPa but small at lower levels at 215 and 316 hPa suggesting the need to investigate the strength of model large-scale circulation and physics associated with the IWC formation. Future work includes: Present MMF/ECMWF Comparisons at AGU/Baltimore Session on MMF/Cloud Resolving Modeling, GMAO/GSFC & at the WPac/Bejing/AGU in Tao's Cloud-Radiation Session. Write-up Results on ECMWF/MLS Comparisons for GRL. Continue with MLS vs ECMWF Water Vapor & Temperature comparisons - will seek more interaction with other MLS colleagues. Investigate the Development of Biases in ECMWF Forecasts - i.e. in the actual model. Work with GMAO-5 development team regarding their cloud microphysics performance. Integrate CloudSat into IWC Analyses.

cloud ice↗

NASA NTRS2003

Light Scattering by Gaussian Particles: A Solution with Finite-Difference Time Domain Technique

The understanding of single-scattering properties of complex ice crystals has significance in atmospheric radiative transfer and remote-sensing applications. In this work, light scattering by irregularly shaped Gaussian ice crystals is studied with the finite-difference time-domain (FDTD) technique. For given sample particle shapes and size parameters in the resonance region, the scattering phase matrices and asymmetry factors are calculated. It is found that the deformation of the particle surface can significantly smooth the scattering phase functions and slightly reduce the asymmetry factors. The polarization properties of irregular ice crystals are also significantly different from those of spherical cloud particles. These FDTD results could provide a reference for approximate light-scattering models developed for irregular particle shapes and can have potential applications in developing a much simpler practical light scattering model for ice clouds angular-distribution models and for remote sensing of ice clouds and aerosols using polarized light. (copyright) 2003 Elsevier Science Ltd. All rights reserved.

Sun, W.↗

NASA NTRSDate not supplied

Characterization of Large Drop Velocity in the NASA Icing Research Tunnel

This presentation presents experimental work conducted in the Icing Research Tunnel at NASA Glenn Research Center to characterize the velocity of large drops in the tunnel test section. Some icing spray clouds with large-sized drops were generated with Mod1 nozzles at low nozzle air pressure of 2 to 4 psig for various tunnel air speeds. Drop diameters and drop velocities were measured via high-resolution imaging with a Particle Imaging Particle Tracking Velocimetry probe developed by Artium Technologies. The probe was mounted at four different locations aligned with the centerline of the test section from near the end of the contraction to the constant height test section part of the tunnel. CFD analyses were performed. It showed that the probe head geometry affects the local air flow between the prongs and in front of the probe. Initial analysis of the air velocity data during the test also indicated that the probe mounting stand has blockage effect on the local tunnel air velocity measurement by a Pitot static probe affixed on the mounting plate. Those findings were later verified in the Icing Research Tunnel using a new Pitot probe design with a linear motion system to measure the local tunnel air velocity with and without the probe. As a result, additional drop trajectory simulations as airflow moving towards the probe head were run for a Langmuir-D 7-bin drop size distribution of a spray cloud with a nominally large value of medium volumetric diameter. The simulation results helped identify a critical drop-size threshold of 300 µm above which the velocities of larger drops are not affected by the adverse pressure gradient generated by the probe head due to their large drop inertia. From the dimensional analysis of the drop velocity measurement data obtained, it showed that at the tunnel test section reference location a generalized empirical correlation was developed for the non-dimensional drop velocity as a function of the non-dimensional corrected drop diameter independent of the actual spraybar pressure settings and the tunnel air speeds. The generalized curve-fit correlation showed that the drop velocity was universally asymptotic to about 86 percent of the corresponding tunnel air speed at the test section reference location for the largest drop diameter captured by the probe. Further evaluation of this correlation is recommended to assess its applicability for Supercooled Large Drop icing scaling applications in the Icing Research Tunnel.

SLD↗

NASA NTRSDate not supplied

Characterization of Large Drop Velocity in the NASA Icing Research Tunnel

This paper presents experimental work conducted in the Icing Research Tunnel at NASA Glenn Research Center to characterize the velocity of large drops in the test section. Some icing spray clouds with large drops were generated with Mod1 nozzles at low nozzle air pressure of 2 to 4 psig for various tunnel air speeds. Drop diameters and drop velocities were measured via high-resolution imaging with a Particle Imaging Particle Tracking Velocimetry probe developed by Artium Technologies. The probe was mounted at four different locations aligned with the centerline of the test section from near the end of the contraction to the constant height test section part of the tunnel. CFD analyses were performed. It showed that the probe head geometry affects the local air flow in the measurement area of the probe between the prongs and in front of the probe. Initial analysis of the air velocity data during the test also indicated that the probe mounting stand has blockage effect on the local tunnel air velocity measurement by a pitot-static probe affixed on the mounting plate next to the stand. Those findings were later verified in the Icing Research Tunnel using a new pitot-static probe design with a linear motion system to measure the local tunnel air velocity with and without the probe. As a result, additional drop trajectory simulations were performed with the airflow moving towards the probe head with a Langmuir-D 7-bin distribution cloud containing large drops. The simulation results helped identify a critical drop-size threshold of 300 μm above which the velocities of larger drops are negligibly affected by the adverse pressure gradient generated by the probe head due to their large drop inertia. From the dimensional analysis of the drop velocity measurement data obtained, it showed that at the tunnel test section reference location a generalized empirical correlation was developed for the non-dimensional drop velocity as a function of the non-dimensional corrected drop diameter independent of the actual spraybar pressure settings and the tunnel air speeds. The generalized curve-fit correlation showed that the drop velocity was universally asymptotic to about 86 percent of the corresponding tunnel air speed at the test section reference location for the largest drop diameter captured by the probe. Further evaluation of this correlation is recommended to assess its applicability for Supercooled Large Drop icing scaling applications in the Icing Research Tunnel.

SLD↗

NASA NTRS2019

Summary of the High Ice Water Content (HIWC) RADAR Flight Campaigns

NASA and the FAA conducted two flight campaigns to quantify onboard weather radar measurements with in-situ measurements of high concentrations of ice crystals found in deep convective storms. The ultimate goal of this research was to improve the understanding and develop onboard weather radar processing to detect regions of high ice water content ahead of an aircraft and enable tactical avoidance of the potentially hazardous conditions. Both High Ice Water Content (HIWC) RADAR campaigns utilized the NASA DC-8 Airborne Science Laboratory which was equipped with a Honeywell RDR-4000 weather radar and icing instruments to characterize the ice crystals clouds. The purpose of this paper is to summarize how these campaigns were conducted and highlight key results.

Aircraft icing↗

NASA NTRS2002

The Laboratory Production of Complex Organic Molecules in Simulated Interstellar Ices

Much of the volatiles in interstellar dense clouds exist in ices surrounding dust grains. Their low temperatures preclude most chemical reactions, but ionizing radiation can drive reactions that produce a suite of new species, many of which are complex organics. The Astrochemistry Lab at NASA-Ames studies the UV radiation processing of interstellar ice analogs to better identify the resulting products and establish links between interstellar chemistry, the organics in meteorites, and the origin of life on Earth. Once identified, the spectral properties of the products can be quantified to assist with the search for these species in space. Of particular interest are findings that UV irradiation of interstellar ice analogs produces molecules of importance in current living organisms, including quiriones, amphiphiles, and amino acids. Quinones play a variety of roles including electron transport and are used by all organisms. Studies show that quinones should be made wherever polycyclic aromatic hydrocarbons are irradiated in interstellar ices (Bernstein et al. 2001). Amphiphiles are also made when mixed molecular ices are irradiated. These amphiphiles self-assemble into membrane-walled vesicles when put in liquid water (Dworkin et al. 2001). Ice irradiation can also produce (Bernstein et al. 2002) and destroy amino acids (Ehrenfreund et al. 2001). Many of the same processes thought to make organics in space should yield products highly enriched in deuterium (D) (Sandford et al. 2001). The high D/H ratios in some interstellar species, and the knowledge that many of the organics in primitive meteorites are D-enriched, suggests that such linkages do exist. By using D as a tracer, we expect to learn more about the different chemical processes occurring in space and their relative importance in the production of different organic compounds and delivery to planetary surfaces.

Dworkin, Jason P.↗

NASA NTRS2002

The Laboratory Production of Complex Organic Molecules in Simulated Interstellar Ices

Dworkin, J. P.↗

NASA NTRS2003

Complex Organics from Laboratory Simulated Interstellar Ices

Many of the volatiles in interstellar dense clouds exist in ices surrounding dust grains. The low temperatures of these ices (T < 50 K) preclude most chemical reactions, but photolysis can drive reactions that produce a suite of new species, many of which are complex organics. We study the UV and proton radiation processing of interstellar ice analogs to explore links between interstellar chemistry, the organics in comets and meteorites, and the origin of life on Earth. The high D/H ratios in some interstellar species, and the knowledge that many of the organics in primitive meteorites are D-enriched, suggest that such links are plausible. Once identified, these species may serve as markers of interstellar heritage of cometary dust and meteorites. Of particular interest are our findings that UV photolysis of interstellar ice analogs produce molecules of importance in current living organisms, including quinones, amphiphiles, and amino acids. Quinones are essential in vital metabolic roles such as electron transport. Studies show that quinones should be made wherever polycyclic aromatic hydrocarbons are photolyzed in interstellar ices. In the case of anthracene-containing ices, we have observed the production of 9-anthrone and 9,10 anthraquinone, both of which have been observed in the Murchison meteorite. Amphiphiles are also made when mixed molecular ices are photolyzed. These amphiphiles self-assemble into fluorescent vesicles when placed in liquid water, as do Murchison extracts. Both have the ability to trap an ionic dye. Photolysis of plausible ices can also produce alanine, serine, and glycine as well as a number of small alcohols and amines. Flash heating of the room temperature residue generated by such experiments generates mass spectral distributions similar to those of IDPs. The detection of high D/H ratios in some interstellar molecular species, and the knowledge that many of the organics, such as hydroxy and amino acids, in primitive meteorites are D-enriched provides evidence for a connection between intact organic material in the interstellar medium and in meteorites. Thus, some of the oxidized aromatics, amphiphiles, amino acids, hydroxy acids, and other compounds found in meteorites may have had an interstellar ancestry and not solely a product of parent body aqueous alteration. Such compounds should also be targeted for searches of organics in cometary dust.

Dworkin, J. P.↗

NASA NTRS2019

Summary of the High Ice Water Content (HIWC) RADAR Flight Campaigns

NASA and the FAA (Federal Aviation Administration) conducted two flight campaigns to quantify onboard weather radar measurements with in-situ measurements of high concentrations of ice crystals found in deep convective storms. The ultimate goal of this research was to improve the understanding and develop onboard weather radar processing to detect regions of high ice water content ahead of an aircraft and enable tactical avoidance of the potentially hazardous conditions. Both High Ice Water Content (HIWC) RADAR campaigns utilized the NASA DC-8 Airborne Science Laboratory which was equipped with a Honeywell RDR-4000 weather radar and icing instruments to characterize the ice crystal clouds. The purpose of this paper is to summarize how these campaigns were conducted and highlight key results.

Airborne Radar↗

NASA NTRS2006

Percentage Contributions from Atmospheric and Surface Features to Computed Brightness Temperatures

Over the past few years, there has become an increasing interest in the use of millimeter-wave (mm-wave) and sub-millimeter-wave (submm-wave) radiometer observations to investigate the properties of ice particles in clouds. Passive radiometric channels respond to both the integrated particle mass throughout the volume and field of view, and to the amount, location, and size distribution of the frozen (and liquid) particles with the sensitivity varying for different frequencies and hydrometeor types. One methodology used since the 1960's to discern the relationship between the physical state observed and the brightness temperature (TB) is through the temperature weighting function profile. In this research, the temperature weighting function concept is exploited to analyze the sensitivity of various characteristics of the cloud profile, such as relative humidity, ice water path, liquid water path, and surface emissivity. In our numerical analysis, we compute the contribution (in Kelvin) from each of these cloud and surface characteristics, so that the sum of these various parts equals the computed TB. Furthermore, the percentage contribution from each of these characteristics is assessed. There is some intermingling/contamination of the contributions from various components due to the integrated nature of passive observations and the absorption and scattering between the vertical layers, but all in all the knowledge gained is useful. This investigation probes the sensitivity over several cloud classifications, such as cirrus, blizzards, light snow, anvil clouds, and heavy rain. The focus is on mm-wave and submm-wave frequencies, however discussions of the effects of cloud variations to frequencies as low as 10 GHz and up to 874 GHz will also be presented. The results show that nearly 60% of the TB value at 89 GHz comes from the earth's surface for even the heaviest blizzard snow rates. On the other hand, a significant percentage of the TB value comes from the snow in the cloud for 166, and 183 plus or minus 7 GHz for the heavy and medium snow rates. For submm-wave channels, there is no contribution from the surface because these channels cannot probe through clouds, nor normal water vapor amounts in clear air regions. This work is extremely valuable in physically-based retrieval algorithm development research.

Gail Skofronick-Jackson↗

NASA NTRS1986

Space Shuttle cloud detection and earth feature classification experiment

The Feature Identification and Location Experiment (FILE) that is being designed for the detection and classification of four primary earth features (water, vegetation, bare land, and the clouds-snow-ice class) is described. Consideration is given to the FILE classification technology concept and the FILE instrument, which will use two solid-state CCD cameras operating at 0.65 and 0.85-micron center frequency wavelengths, with the camera outputs being functions of the earth surface material radiance. The classification is based on camera output radiance ratio values. The preliminary analysis of the data collected on the STS 41-G mission is discussed. The results demonstrated the suitability of using the two-channel-ratio detection technology and a simple (y = mx) algorithm to autonomously classify the four earth surface features. The technology is especially attractive as a cloud sensor, where, in advance of or during a mission, a threshold value for cloud cover percentage can be programmed and/or adaptively modified for use in the control of other remote sensors.

Sivertson, W. E., Jr.↗

NASA NTRS2009

Cloud Imagers Offer New Details on Earth's Health

A stunning red sunset or purple sunrise is an aesthetic treat with a scientific explanation: The colors are a direct result of the absorption or reflectance of solar radiation by atmospheric aerosols, minute particles (either solid or liquid) in the Earth s atmosphere that occur both naturally and because of human activity. At the beginning or end of the day, the Sun s rays travel farther through the atmosphere to reach an observer s eyes and more green and yellow light is scattered, making the Sun appear red. Sunset and sunrise are especially colorful when the concentration of atmospheric particles is high. This ability of aerosols to absorb and reflect sunlight is not just pretty; it also determines the amount of radiation and heat that reaches the Earth s surface, and can profoundly affect climate. In the atmosphere, aerosols are also important as nuclei for the condensation of water droplets and ice crystals. Clouds with fewer aerosols cannot form as many water droplets (called cloud particles), and consequently, do not scatter light well. In this case, more sunlight reaches the Earth s surface. When aerosol levels in clouds are high, however, more nucleation points can form small liquid water droplets. These smaller cloud particles can reflect up to 90 percent of visible radiation to space, keeping the heat from ever reaching Earth s surface. The tendency for these particles to absorb or reflect the Sun s energy - called extinction by astronomers - depends on a number of factors, including chemical composition and the humidity and temperature in the surrounding air; because cloud particles are so small, they are affected quickly by minute changes in the atmosphere. Because of this sensitivity, atmospheric scientists study cloud particles to anticipate patterns and shifts in climate. Until recently, NASA s study of atmospheric aerosols and cloud particles has been focused primarily on satellite images, which, while granting large-scale atmospheric analysis, limited scientists ability to acquire detailed information about individual particles. Now, experiments with specialized equipment can be flown on standard jets, making it possible for researchers to monitor and more accurately anticipate changes in Earth s atmosphere and weather patterns.

Source record↗

NASA NTRS2021

Aerosol–Ice Formation Closure: A Southern Great Plains Field Campaign

Prediction of ice formation in clouds presents one of the grand challenges in the atmospheric sciences. Immersion freezing initiated by ice-nucleating particles (INPs) is the dominant pathway of primary ice crystal formation in mixed-phase clouds, where supercooled water droplets and ice crystals coexist, with important implications for the hydrological cycle and climate. However, derivation of INP number concentrations from an ambient aerosol population in cloud-resolving and climate models remains highly uncertain. We conducted an aerosol-ice formation closure pilot study using a field-observational approach to evaluate the predictive capability of immersion freezing INPs. The closure study relies on co-located measurements of the ambient size-resolved and single-particle composition and INP number concentrations. The acquired particle data serve as input in several immersion freezing parameterizations, that are employed in cloud-resolving and climate models, for prediction of INP number concentrations. We discuss in detail one closure case study in which a front passed through the measurement site, resulting in a change of ambient particle and INP populations. We achieved closure in some circumstances within uncertainties, but we emphasize the need for freezing parameterization of potentially missing INP types and evaluation of the choice of parameterization to be employed. Overall, this closure pilot study aims to assess the level of parameter details and measurement strategies needed to achieve aerosol-ice formation closure. The closure approach is designed to accurately guide immersion freezing schemes in models, and ultimately identify the leading causes for climate model bias in INP predictions.

ice formation↗

NASA NTRS1998

Observations of the north polar region of Mars from the Mars orbiter laser altimeter

Elevations from the Mars Orbiter Laser Altimeter (MOLA) have been used to construct a precise topographic map of the martian north polar region. The northern ice cap has a maximum elevation of 3 kilometers above its surroundings but lies within a 5-kilometer-deep hemispheric depression that is contiguous with the area into which most outflow channels emptied. Polar cap topography displays evidence of modification by ablation, flow, and wind and is consistent with a primarily H2O composition. Correlation of topography with images suggests that the cap was more spatially extensive in the past. The cap volume of 1.2 x 10(6) to 1.7 x 10(6) cubic kilometers is about half that of the Greenland ice cap. Clouds observed over the polar cap are likely composed of CO2 that condensed out of the atmosphere during northern hemisphere winter. Many clouds exhibit dynamical structure likely caused by the interaction of propagating wave fronts with surface topography.

Flight Experiment↗

DOE OSTI2024

Organisation of Diverse Mechanisms of Secondary Ice Production among Basic Convective and Stratiform Cloud-types

This 3-year DoE-funded joint project had the over-arching aim of understanding how ice is initiated in clouds of various types. Focus was given to processes of fragmentation of pre-existing ice, which can occur in positive feedback loops (‘ice multiplication’). A basic question to address was which fragmentation processes prevail in which basic cloud-types. The approach was to use cloud models and field observations, while pioneering our own lab observations of ice initiation to break the deadlock from the past lack of lab observations. Historically, the tendency of the cloud physics community to avoid doing lab observations has allowed a vast gap in knowledge about ice initiation to persist for decades. During the first part of the project, new formulations were created to treat two overlooked types of fragmentation of ice. First, sublimational breakup of ice was treated based on a theoretical formula that we fitted to a pooled dataset of lab observations published previously in the literature. Second, a new mode of fragmentation of freezing raindrops was treated, which involves a supercooled drop being hit by a more massive ice particle. Some of the secondary droplets from the impact freeze. This work was done at Manchester University by Co-I Connolly. Then during the second part, both formulations were implemented in our ‘aerosol-cloud model’ (AC). AC has a hybrid bin/bulk microphysics scheme, and now represents four processes of SIP. The accuracy of AC was evaluated for four cases typifying four basic cloud-types: slightly cold-based stratiform cloud and cold-, warm- and very warm-based convective clouds. We discovered that the warmth of cloud-base, especially in the tropics, promotes SIP processes of raindrop-freezing fragmentation and rime-splintering, and surprisingly, sublimational breakup too. It was found that breakup in ice-ice collisions is ubiquitous. Finally, a portable laboratory chamber was constructed at Lund and deployed in northern Sweden to observe breakup in graupel-snow collisions outdoors. This was seen to be even more prolific than treated in our 2018 formulation. Papers describing results are either published or soon to be published.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2021

KAZR Hydrometeor and Insect Masks

The Ka-band ARM zenith pointing radar (aka, KAZR) is so sensitive that it detects cloud particles and individual insects. While detecting insects with Ka-band radar is beneficial and desirable to advance radar entomology, this sensitivity can be detrimental to radar meteorology because insects could be interpreted as clouds or precipitation. For example, misclassifying insects as clouds has been a problem for the ARM Active Remote Sensing of Clouds (ARSCL) Value Added Product since its inception (Clothiaux et al. 2000). Based on cloud particle and insect radar scattering properties, an algorithm was developed that identifies clouds, raindrops, ice particles, and insects in KAZR co- and cross-polarimeteric Doppler velocity spectra. The algorithm produces affirmative masks in the KAZR native time and height resolution indicating time-height locations of hydrometeors and insects. The hydrometeor mask contains binary information (e.g., yes/no hydrometeor presence), and the insect mask includes a proxy for insect activity that increases when more insects are detected in the Doppler velocity spectra. The algorithm was developed using KAZR medium sensitivity mode (MD) observations and was applied to two summer seasons of KAZR observations at the Southern Great Plains (SGP) Central Facility: May-October 2018 and 2019. In the future, this data set will be expanded to include other KAZR operating modes and observations from other ARM field sites. Details of the algorithm and data set can be found in: Williams, C.R., K.L. Johnson, S.E. Giangrande, J. C. Hardin, R. Oktem, and D. M. Romps, 2021: Identifying Insects, Clouds, and Precipitation using Vertically Pointing Polarimetric Radar Doppler Velocity Spectra. Atmospheric Measurement Techniques, submitted 6-Feb-2021. https://amt.copernicus.org/preprints/amt-2021-27/#discussion.For more information on the ARSCL VAP, see Clothiaux, E. E., T. P. Ackerman, G. G. Mace, K. P. Moran, R. T. Marchand, M. A. Miller, and B. E. Martner, 2000; J. Appl. Meteor., 39, 645-665.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2021

New insights into ice multiplication using remote-sensing observations of slightly supercooled mixed-phase clouds in the Arctic

Significance During secondary ice events, ice particle number concentrations in mixed-phase clouds can increase by orders of magnitude with profound implications for the cloud evolution. However, characterization of secondary ice events in the natural environment has been a challenge for the community for decades. We show the long-term frequency of secondary ice events in Arctic supercooled clouds for temperatures warmer than − 10 ○ C, made possible by applying a remote-sensing technique to 6 y of data. Secondary ice events are found to occur preferentially in the presence of drizzle droplets, compared with the better-known rime-splintering process, causing up to a 1,000-fold enhancement in ice number concentration. These results provide critical insights for model parameterizations and future laboratory experiments.

54 ENVIRONMENTAL SCIENCES↗