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At least 1,081 records · Page 60
All sourcesNASA NTRSDOE OSTI
DOE OSTI2021

Dimensionality effects on multicomponent ionic transport and surface complexation in porous media

Coulombic interactions between charged species in pore water and at surface/solution interfaces are of pivotal importance for multicomponent reactive transport in porous media. In this study, we investigate the impact of domain dimensionality on electrostatically coupled dispersion and surface-solution reactions during transport of acidic plumes and major ions in porous media. Column and quasi two-dimensional flow-through experiments were performed, with identical silica porous media and under the same advection-dominated conditions. Equal mass fluxes of different electrolyte solutions (i.e., HCl - pH ~ 2.8, NaBr - 100 mM, HCl - pH ~ 2.8 plus NaBr - 100 mM) were continuously injected in the 1-D and 2-D experiments and breakthrough curves of pH and major ions were measured at the outlet of the domains. The presence of pronounced ionic strength gradients in the transverse direction in the 2-D setup caused distinct retardation and transport behaviors of protons and major ions which were not observed in the one-dimensional column experiments. Furthermore, in the cases of salt electrolytes injection, considerably enhanced release of H + (>61%) from the quartz surface was observed in the multidimensional system compared to the one-dimensional setup. Reactive transport modeling was performed to reproduce the experimental outcomes and to analyse the coupling between transport processes, based on the Nernst-Planck formulation of diffusive/dispersive fluxes and on surface complexation reactions at the solid-solution interface. Electrostatic interactions between Na + , B – , and H + , and deprotonation of the quartz surface upon the formation of sodium outer-sphere complexes, are the primary controllers of the spatial and temporal features displayed by the pH and major ions measurements. The reactive transport simulations allowed us to interpret the experimental observations, to visualize the distribution and spatio-temporal evolution of dissolved and solid species, to identify a spatially heterogeneous zonation of Coulombic interactions with distinct behavior at the fringe and core of the injected plumes in the multidimensional setup, and to quantify the different components of the Nerst-Planck fluxes of the charged solutes. This study demonstrates that the domain dimensionality directly affects electrostatic interactions between charged aqueous species in the pore water and surface complexation reactions at the solid-solution interface. The non-trivial effects of dimensionality on multicomponent ionic transport result in a significantly different behavior in 1-D and 2-D systems.

58 GEOSCIENCES↗
DOE OSTI2022

Method to account for natural fracture induced elastic anisotropy in geomechanical characterization of shale gas reservoirs

Shale has been usually recognized as a transverse isotropic (TI) medium in conventional geomechanical log interpretation due to its laminated nature. However, when natural fractures exist in the shale rock, additional elastic anisotropy is introduced, converting laminated Shale to an orthorhombic (OB) medium. Previous studies illustrate that neglecting the natural fracture induced anisotropy in shale geomechanical log interpretation could lead to inaccurate evaluations of elastic moduli and in-situ stresses. In this paper, a new method is developed to account for the natural fracture induced anisotropy in geomechanical log interpretation based upon the TI acoustic model developed by the author and a characterization technique of elastic wave anisotropy (Sayers, 1991). The new OB model incorporates the four acoustic log data inputs and five modeling constraints in a nonlinear optimization algorithm to solve for the nine independent stiffness coefficients of an OB rock, and further to solve for the geomechanical properties and in-situ stress profiles in an OB formation. The new method was validated with a Marcellus Gas Shale field case. Both the new OB model and the conventional TI model were applied to interpret the minimum horizontal stress profile for the same formation. By comparing the results, the OB model is more robust than the TI from two aspects. First, the average stress magnitude predicted by the OB model is closer to the one measured by the Diagnostic Fracture Injection Test (DFIT). Second, the OB model predicts a more obvious stress barrier between the lower Marcellus and upper Onondaga Limestone than the TI model does. Finally, the predicted stress barrier is consistent with the observation of the microseismic events of a horizontal well drilled and completed nearby, which reveals that no hydraulic fracture propagates downward through the bottom boundary of Marcellus Shale into the underlying Onondaga Limestone.

03 NATURAL GAS↗
DOE OSTI2023

Equibiaxial flexural strength determination of UO 2 using a ball-on-ring test

To increase nuclear fuel performance and reliability, their mechanical properties require an accurate and statistically relevant assessment. Biaxial flexural strength tests provide an alternative to bend bar techniques for assessing mechanical behavior; namely, the transverse rupture strength (TRS) of ceramic samples. Biaxial test samples require simple geometries and minimal surface preparation, reducing fabrication costs and handling hazards. This study investigated the TRS of polycrystalline UO 2 fuel forms at room temperature using a ball-on-ring test fixture. Here, pellets were fabricated from UO 2 powder using conventional powder processing and sintering techniques. The TRS and Weibull parameters were obtained through Weibull statistics on over 60 UO 2 samples tested under equibiaxial flexure. The larger sample size in this study enabled a more robust Weibull statistical analysis than alternative test methods, which may not capture the stochastic failure of typical ceramics. Furthermore, two different loading ball diameters were employed to assess the impact of contact damage on fracture strength. While Hertzian contact damage was observed with the smaller loading ball, the fracture strength remained unaffected. A fracture analysis of the tested UO 2 samples indicated a mixture of intergranular and transgranular fracture that transitions to transgranular fracture with increasing distance from the fracture origin. The characteristic strength of the combined data sets was determined to be 148 MPa, and the Weibull modulus was determined to be 9.1. The TRS values and Weibull parameters were close to values found in the literature for alternative testing techniques using samples with similar microstructure and density. The findings in this study validate the ball-on-ring method used to obtain the TRS of UO 2 with a sample geometry more representative of nuclear fuels. Additionally, experimental TRS results from this study can be implemented in modeling codes to predict fuel performance, which is critical to fuel burnup extension and advanced nuclear fuel technologies.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2025

Statistical fracture behavior of doped UO 2 using a ball-on-ring equibiaxial flexure test method

Metal oxide dopants, such as titanium and chromium oxides, have garnered considerable attention for their potential to increase grain size (≥ 30 µm) in UO 2 fuel, purportedly enhancing fission gas retention during reactor operation. Fuel performance is significantly impacted by fuel fracture behavior, so it is important to understand the effects of enhanced grain size and dopant content on UO 2 fuel fracture. UO 2 pellets were doped with 0.1 wt% TiO 2 and 0.3 wt% Cr 2 O 3 to alter density and grain size. Inductively coupled plasma mass spectroscopy measured dopant levels pre- and post-sintering. X-ray diffraction revealed lattice changes and microstrain via Rietveld refinement. Field emission scanning electron microscopy determined grain sizes of approximately 30 µm for TiO 2 doping and 7 µm for Cr 2 O 3 doping. Transverse rupture strength tests were performed on over 30 samples per dataset to obtain characteristic strength and Weibull modulus. Results indicate no statistical difference in fracture strength between 0.1 wt% TiO 2 doped UO 2 and undoped UO 2 , while 0.3 wt% Cr 2 O 3 doped UO 2 exhibited a 20% decrease in fracture strength. Doped UO 2 samples also showed reduced Weibull modulus compared to undoped UO 2 , suggesting increased scatter in fracture strength. This study's findings suggest that titanium and chromium oxide doping in UO 2 , regardless of grain size, induce residual stresses, decreasing fracture strength and increasing variability in fracture behavior.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2023

ECCE unpolarized TMD measurements

For this work, we performed feasibility studies for various measurements that are related to unpolarized TMD distribution and fragmentation functions for the ECCE detector proposal. The processes studied include semi-inclusive Deep inelastic scattering (SIDIS) where single hadrons (pions and kaons) were detected in addition to the scattered DIS lepton. The single hadron cross sections and multiplicities were extracted as a function of the DIS variables x and Q 2 , as well as the semi-inclusive variables z, which corresponds to the momentum fraction the detected hadron carries relative to the struck parton and P T , which corresponds to the transverse momentum of the detected hadron relative to the virtual photon. The expected statistical precision of such measurements is extrapolated to accumulated luminosities of 10 fb –1 and potential systematic uncertainties are approximated given the deviations between true and reconstructed yields. The expected uncertainties are then used to obtain the expected impact on the related TMD distribution and fragmentation functions. We find that the ECCE detector proposal fulfills the physics requirements on these channels as detailed in the EIC Yellow Report.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2024

Measurement of the Z boson invisible width at $\sqrt{s}=13$ TeV with the ATLAS detector

A measurement of the invisible width of the Z boson using events with jets and missing transverse momentum is presented using 37 fb -1 of 13 TeV proton–proton data collected by the ATLAS detector in 2015 and 2016. The ratio of Z → inv to Z → ℓℓ events, where inv refers to non-detected particles and ℓ is either an electron or a muon, is measured and corrected for detector effects. Events with at least one energetic central jet with p T ≥ 110 GeV are selected for both the Z → inv and Z → ℓℓ final states to obtain a similar phase space in the ratio. The invisible width is measured to be 506 ± 2 (stat.) ± 12 (syst.) MeV and is the single most precise recoil-based measurement. The result is in agreement with the most precise determination from LEP and the Standard Model prediction based on three neutrino generations.

13000 GeV-cms↗
DOE OSTI2026

Kinematic and dynamical origins of mean-p T fluctuations in heavy-ion collisions

Event-by-event fluctuations of the mean transverse momentum (mean-p T ) provide a sensitive probe of collective dynamics beyond single-particle spectra and anisotropic flow. We present a systematic study of mean-p T fluctuation observables using a Bayesian-calibrated multistage hydrodynamic framework, including quantitative comparisons to RHIC measurements and model-based investigations of beam-energy and kinematic-acceptance effects. The experimental definitions employed by the STAR and ALICE Collaborations are implemented explicitly and found to yield consistent results within controlled limits. We study the centrality and beam-energy dependence of the observable, its sensitivity to key soft-sector ingredients, and the impact of the kinematic p T acceptance. By introducing scaled-p T cuts, we demonstrate that a part of the apparent energy dependence arises from kinematic projection effects, while the remaining trends reflect genuine collective dynamics. Our results establish mean-p T fluctuations as a nontrivial and independent validation of calibrated hydrodynamic descriptions of the quark–gluon plasma.

Event-by-event correlations↗
DOE OSTI2026

Unpolarized GPDs at small x and non-zero skewness

We study the small-x asymptotics of unpolarized generalized parton distributions (GPDs) and generalized transverse momentum distributions (GTMDs). Unlike the previous works in the literature, we consider the case of non-zero (but small) skewness while allowing for non-linear contributions to the evolution equations. We first show that unpolarized GPDs and GTMDs at small x are related to the eikonal dipole amplitude N, whose small-x evolution is given by the BK/JIMWLK evolution equations, and to the odderon amplitude $\mathscr{O}$, whose evolution is also known in the literature. We then show that the effect of non-zero skewness ξ ≠ 0 is to modify the value of the evolution parameter (rapidity) in the arguments for the dipole amplitudes N and $\mathscr{O}$ from Y = ln(1/x) to Y = ln min{1/|x|, 1/|ξ|}.

Generalized parton distributions (GPDs)↗
DOE OSTI2022

Physically and chemically smooth cesium-antimonide photocathodes on single crystal strontium titanate substrates

The performance of x-ray free electron lasers and ultrafast electron diffraction experiments is largely dependent on the brightness of electron sources from photoinjectors. Here, the maximum brightness from photoinjectors at a particular accelerating gradient is limited by the mean transverse energy (MTE) of electrons emitted from photocathodes. For high quantum efficiency (QE) cathodes like alkali-antimonide thin films, which are essential to mitigate the effects of non-linear photoemission on MTE, the smallest possible MTE and, hence, the highest possible brightness are limited by the nanoscale surface roughness and chemical inhomogeneity. In this work, we show that high QE Cs 3 Sb films grown on lattice-matched strontium titanate (STO) substrates have a factor of 4 smoother, chemically uniform surfaces compared to those traditionally grown on disordered Si surfaces. We perform simulations to calculate roughness induced MTE based on measured topographical and surface-potential variations on the Cs 3 Sb films grown on STO and show that these variations are small enough to have no consequential impact on the MTE and, hence, the brightness.

43 PARTICLE ACCELERATORS↗
DOE OSTI2025

Characterization of Cs 3 Sb photocathodes at cryogenic temperatures

Here, we report measurements of quantum efficiency (QE) and mean transverse energy (MTE) from Cs 3 Sb photocathodes in a wide range of photon energies at both room and cryogenic temperatures. Our measurements show a strong temperature dependence of MTE even at photon energies well above threshold, indicating the presence of strong inelastic scattering of excited electrons during transport before emission into vacuum. We also demonstrate a cathode cooling method that largely preserves the QE while reducing MTE, allowing us to achieve MTEs as low as 58 meV with 3% QE in green light from Cs 3 Sb photocathodes. Our results are crucial for producing brighter electron beams for various photoinjector applications like ultrafast electron diffraction and microscopy, x-ray free-electron lasers, and particle colliders.

36 MATERIALS SCIENCE↗
DOE OSTI2020

Electronic nematicity in Sr 2 RuO 4

We have measured the angle-resolved transverse resistivity (ARTR), a sensitive indicator of electronic anisotropy, in high-quality thin films of the unconventional superconductor Sr 2 RuO 4 grown on various substrates. The ARTR signal, heralding the electronic nematicity or a large nematic susceptibility, is present and substantial already at room temperature and grows by an order of magnitude upon cooling down to 4 K. In Sr 2 RuO 4 films deposited on tetragonal substrates the highest-conductivity direction does not coincide with any crystallographic axis. In films deposited on orthorhombic substrates it tends to align with the shorter axis; however, the magnitude of the anisotropy stays the same despite the large lattice distortion. These are strong indications of actual or incipient electronic nematicity in Sr 2 RuO 4 .

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2023

Infinite neural network quantum states: entanglement and training dynamics

We study infinite limits of neural network quantum states (∞-NNQS), which exhibit representation power through ensemble statistics, and also tractable gradient descent dynamics. Ensemble averages of entanglement entropies are expressed in terms of neural network correlators, and architectures that exhibit volume-law entanglement are presented. The analytic calculations of entanglement entropy bound are tractable because the ensemble statistics are simplified in the Gaussian process limit. A general framework is developed for studying the gradient descent dynamics of neural network quantum states (NNQS), using a quantum state neural tangent kernel (QS-NTK). For ∞-NNQS the training dynamics is simplified, since the QS-NTK becomes deterministic and constant. An analytic solution is derived for quantum state supervised learning, which allows an ∞-NNQS to recover any target wavefunction. Numerical experiments on finite and infinite NNQS in the transverse field Ising model and Fermi Hubbard model demonstrate excellent agreement with theory. ∞-NNQS opens up new opportunities for studying entanglement and training dynamics in other physics applications, such as in finding ground states.

quantum state supervised learning↗
DOE OSTI2026

Collins-Soper kernel and reduced soft function in lattice QCD

We evaluate the Collins-Soper kernel and the reduced soft function in lattice QCD, incorporating 𝒪⁡(𝛼 𝑠 ) matching corrections. The calculation relies on the evaluation of the quasitransverse momentum–dependent wave function with asymmetric staple-shaped quark bilinear operators and four-point meson form factors. These quantities are computed nonperturbatively using two 𝑁 𝑓 =2 + 1 + 1 twisted-mass fermion ensembles with the same lattice spacing of 𝑎 = 0.093 fm: the first ensemble has a lattice size of 24 3 × 48 and a pion mass of 346 MeV, and the second one has a lattice size of 32 3 × 64 and a pion mass of 261 MeV. The Collins-Soper kernel and the soft function are needed for the determination of the transverse momentum–dependent parton distribution functions.

Lattice QCD↗
DOE OSTI2020

Moments of nucleon isovector structure functions in 2+1+1-flavor QCD

We present results on the isovector momentum fraction, $\langle x \rangle_{u–d}$ , helicity moment, $\langle x \rangle_{Δ u–Δd}$ , and the transversity moment, $\langle x \rangle_{δu–δd}$, of the nucleon obtained using nine ensembles of gauge configurations generated by the MILC Collaboration using 2 + 1 + 1 -flavors of dynamical highly improved staggered quarks. The correlation functions are calculated using the Wilson-Clover action, and the renormalization of the three operators is carried out nonperturbatively on the lattice in the RI'–MOM scheme. The data have been collected at lattice spacings a ≈ 0.15 , 0.12, 0.09, and 0.06 fm and $M_π$ ≈ 310 , 220, and 135 MeV, which are used to obtain the physical values using a simultaneous chiral-continuum-finite-volume fit. The final results, in the $\overline{\text{MS}}$ scheme at 2 GeV, are $\langle$ x $\rangle$ u – d = 0.173 ( 14 ) ( 07 ) , $\langle x \rangle_{Δu–Δd}$ = 0.213 ( 15 ) ( 22 ) , and $\langle x \rangle_{δu–δd}$ = 0.208 ( 19 ) ( 24 ) , where the first error is the overall analysis uncertainty and the second is an additional systematic uncertainty due to possible residual excited-state contributions. These results are consistent with other recent lattice calculations and phenomenological global fit values.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2020

First Measurement of Λ c Baryon Production in Au + Au Collisions at s N N = 200 GeV

Herein we report on the first measurement of the charmed baryon Λ c ± production at midrapidity ( | y | < 1 ) in Au + Au collisions at s NN = 200 GeV collected by the STAR experiment at the Relativistic Heavy Ion Collider. The Λ c / D 0 [denoting ( Λ c + + Λ c - ) / ( D 0 + D ¯ 0 ) ] yield ratio is measured to be 1.08 ± 0.16 ( stat ) ± 0.26 ( sys ) in the 0%–20% most central Au + Au collisions for the transverse momentum ( p T ) range 3 < p T < 6 GeV / c . This is significantly larger than the pythia model calculations for p + p collisions. The measured Λ c / D 0 ratio, as a function of p T and collision centrality, is comparable to the baryon-to-meson ratios for light and strange hadrons in Au + Au collisions. Model calculations including coalescence hadronization for charmed baryon and meson formation reproduce the features of our measured Λ c / D 0 ratio.

13000 GeV-cms/nucleon↗
DOE OSTI2026

Eikonal spin-dependent odderon and gluon Sivers function of a proton and its small-𝑥 evolution

The matrix element in the proton of the eikonal Odderon operator, with a helicity flip, has been shown to correspond to the dipole gluon Sivers function. We employ a three quark light-front model of the proton to determine the Sivers function at moderately small 𝑥 0 ∼ 0.1 and transverse momentum 𝑘 ⊥ ≲ 1 GeV. The model light-cone (LC) wave function predicts the properties of 𝑥⁢𝑓$^{⊥⁢𝑔}_{1⁢𝑇⁡}$(𝑥,𝑘 ⊥ ) such as its overall magnitude, the position of its peak in 𝑘 ⊥ , and its behavior at small 𝑘 ⊥ . We then compute numerically the Balitsky-Fadin-Kuraev-Lipatov anomalous dimension characterizing the power-law tail at 𝑘 ⊥ ≳ 1.5 GeV of the gluon Sivers function at small (but preasymptotic) LC momentum fractions 𝑥 ∼ 𝑥 0 ⁢𝑒 −1/𝛼 𝑠 : 𝑥⁢𝑓$^{⊥⁢𝑔}_{1⁢𝑇⁡}$⁡(𝑥,𝑘 ⊥ ) ∼ 𝑘$^{−3.3}_{⊥}$.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2025

Measurements of source emittance and beam coherence properties of the upgraded Advanced Photon Source

The Advanced Photon Source (APS) has been upgraded with a multi-bend achromat lattice, achieving significantly reduced electron beam emittance and enhanced X-ray coherence. Precise characterization of these properties is essential for optimizing beamline performance and enabling new experiments that take full advantage of the upgraded source. We report on measurements of source size and transverse coherence properties using grating interferometry at two beamlines: the APS 3-ID-B undulator beamline and the 1-BM-B bending magnet beamline. The results confirm the world-record horizontal emittance of the upgraded APS below 30 pm rad and validate the theoretical design parameters. We further investigate the impact of optical aberrations and mechanical vibrations at the 12-ID-C beamline on coherence preservation. These measurements establish a benchmark for future beamline enhancements and demonstrate the effectiveness of grating interferometry for high-precision beam characterization. Our findings provide critical insights into synchrotron beam dynamics, coherence degradation mechanisms, and strategies for optimizing beamline X-ray optics at next-generation light sources.

Advanced Photon Source↗
DOE OSTI2025

SEM Grid Testing at NLCTA in BeamNetUS Program

We report on the performance of a secondary electron monitor (SEM) grid used to measure the transverse profile of an MeV range electron beam at SLAC National Accelerator Laboratory’s Next Linear Collider Test Accelerator (NLCTA) facility. When inserted into the path of the electron beam, secondary electron emission results in a measurable current on the wires that make up the grid. We present measurements using this technique to reconstruct the beam profile. The SEM grid was designed and manufactured by a team of undergraduate students at Harvey Mudd College (HMC) and was tested at SLAC’s NLCTA facility in collaboration with NCLTA staff as part of the BeamNetUS program. Developed for real-time diagnostics of MeV-range electron beams, this SEM grid has potential applications in both industrial and medical contexts.

43 PARTICLE ACCELERATORS↗