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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 1,081 records · Page 60
All sourcesNASA NTRSDOE OSTI
DOE OSTI2021

TNSL Overview

Thermal neutron scattering law (TNSL) data describe low-energy neutrons scattering off of bound materials, and can have a significant impact on modeling any system with slow neutrons, including nuclear reactors. Previous work to introduce TNSL data to neutron transport codes at LLNL focused on COG and TART [1], with the limitation that these codes require highly specialized data processing and formatting. We have recently increased efforts to process TNSL data with the central LLNL nuclear data processing code FUDGE, to be stored in the generalized nuclear database structure (GNDS) for use in any general transport code with the ability to read GNDS data. The first step in this effort is to verify that the TNSL processing with FUDGE yields results comparable to results obtained using the LANL nuclear data processing code NJOY. The next step is to verify the transport of thermal neutrons in Mercury (a Monte Carlo code) and Ardra (a deterministic code) against one another, as well as against the LANL Monte Carlo neutron transport code MCNP. This verification step has not been completed, due to a number of discrepancies between results obtained using differently processed data. There is ongoing effort to understand differences between FUDGE and NJOY. Finally, we map out our current capability to validate TNSL data against benchmark systems.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2023

Neutron inelastic scattering measurements on KCl and NaCl samples at the Dome

Precise and accurate measurements of neutron inelastic scattering cross sections are vital for both the LLNL national security mission and for scientific applications such as the nuclear spectroscopy of planetary bodies. In this work, initial measurements of relative cross sections were performed by irradiating KCl and NaCl samples with a DD neutron generator, a DT neutron generator, and a PuB source in building 262, the Dome. The measurements allowed the existing experimental setup to be benchmarked. Several improvements to the setup are suggested for future experiments.

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗
DOE OSTI2021

Application of Monte Carlo Algorithms to Cardiac Imaging Reconstruction

Monte Carlo algorithms have a growing impact on nuclear medicine reconstruction processes. One ofthe main limitations of myocardial perfusion imaging (MPI) is the effective mitigation of the scattering component,which is particularly challenging in Single Photon Emission Computed Tomography (SPECT). In SPECT,no timing information can be retrieved to locate the primary source photons. Monte Carlo methods allow anevent-by-event simulation of the scattering kinematics, which can be incorporated into a model of the imagingsystem response. This approach was adopted in the late Nineties by several authors, and recently took advantageof the increased computational power made available by high-performance CPUs and GPUs. These recent developmentsenable a fast image reconstruction with improved image quality, compared to deterministic approaches.Deterministic approaches are based on energy-windowing of the detector response, and on the cumulative estimateand subtraction of the scattering component. In this paper, we review the main strategies and algorithms tocorrect the scattering effect in SPECT and focus on Monte Carlo developments, which nowadays allow the threedimensionalreconstruction of SPECT cardiac images in a few seconds.

Pharmacology & Pharmacy↗
NASA NTRS2002

HST NICMOS Observations of the Polarization of NGC 1068

We have observed the polarized light at 2 microns in the center of NGC 1068 with HST (Hubble Space Telescope) NICMOS (Near Infrared Camera Multi Object Spectrometer) Camera 2. The nucleus is dominated by a bright, unresolved source, polarized at a level of 6.0 +/- 1.2% with a position angle of 122 degrees +/- 1.5 degrees. There are two polarized lobes extending tip to 8" northeast and southwest of the nucleus. The polarized flux in both lobes is quite clumpy, with the maximum polarization occurring in the southwest lobe at a level of 17% when smoothed to 0.23" resolution. The perpendiculars to the polarization vectors in these two lobes point back to the intense unresolved nuclear source to within one 0.076" Camera 2 pixel, thereby confirming that this source is the origin of the scattered light and therefore the probable AGN (Active Galactic Nuclei) central engine. Whereas the polarization of the nucleus is probably caused by dichroic absorption, the polarization in the lobes is almost certainly caused by scattering, with very little contribution from dichroic absorption. Features in the polarized lobes include a gap at a distance of about 1" from the nucleus toward the southwest lobe and a "knot" of emission about 5" northwest of the nucleus. Both features had been discussed by groundbased observers, but they are much better defined with the high spatial resolution of NICMOS. The northeast knot may be the side of a molecular cloud that is facing the nucleus, which cloud may be preventing the expansion of the northeast radio lobe at the head of the radio synchrotron-radiation-emitting jet. We also report the presence of two ghosts in the Camera 2 polarizers.

Simpson, Janet P.↗
DOE OSTI2020

Sample spinning to mitigate polarization artifact and interstitial-vacancy imbalance in ion-beam irradiation

Accelerator-based ion-beam irradiation has been widely used to mimic the effects of neutron radiation damage in nuclear reactors. However, ion radiation is most often monodisperse in the incoming ions’ momentum direction, leading to excessive polarization in defect distribution, while the scattering under neutron irradiation is often more isotropic and has less radiation-induced polarization. Mitigation of the excess-polarization as well as the damage non-uniformity artifact might be crucial for making the simulation of neutron radiation by ion-beam radiation more realistic. In this work, a general radiation polarization theory in treating radiation as external polar stimuli is established to understand the natural material responses in different contexts, and the possibility to correct the defect polarization artifact in ion-beam irradiation. Inspired by Magic Angle Spinning in Nuclear Magnetic Resonance, we present a precise sample spinning strategy to reduce the point-defect imbalance effect in ion-beam irradiation. It can be seen that with optimized surface inclination angle and the axis of sample rotation, the vacancy-interstitial population imbalance, as well as the damage profile non-uniformity in a designated region in the target are both reduced. It is estimated that sample spinning frequency on the order of kHz should be sufficient to scramble the ion momentum monodispersity for commonly taken ion fluxes and dose rates, which is experimentally feasible.

36 MATERIALS SCIENCE↗
DOE OSTI2023

Electron Scattering from 1-Methyl-5-Nitroimidazole: Cross-Sections for Modeling Electron Transport through Potential Radiosensitizers

In this study, we present a complete set of electron scattering cross-sections from 1-Methyl-5-Nitroimidazole (1M5NI) molecules for impact energies ranging from 0.1 to 1000 eV. This information is relevant to evaluate the potential role of 1M5NI as a molecular radiosensitizers. The total electron scattering cross-sections (TCS) that we previously measured with a magnetically confined electron transmission apparatus were considered as the reference values for the present analysis. Elastic scattering cross-sections were calculated by means of two different schemes: The Schwinger multichannel (SMC) method for the lower energies (below 15 eV) and the independent atom model-based screening-corrected additivity rule with interferences (IAM-SCARI) for higher energies (above 15 eV). The latter was also applied to calculate the total ionization cross-sections, which were complemented with experimental values of the induced cationic fragmentation by electron impact. Double differential ionization cross-sections were measured with a reaction microscope multi-particle coincidence spectrometer. Using a momentum imaging spectrometer, direct measurements of the anion fragment yields and kinetic energies by the dissociative electron attachment are also presented. Cross-sections for the other inelastic channels were derived with a self-consistent procedure by sampling their values at a given energy to ensure that the sum of the cross-sections of all the scattering processes available at that energy coincides with the corresponding TCS. This cross-section data set is ready to be used for modelling electron-induced radiation damage at the molecular level to biologically relevant media containing 1M5NI as a potential radiosensitizer. Nonetheless, a proper evaluation of its radiosensitizing effects would require further radiobiological experiments.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2020

Bulk and Nanocrystalline Cesium Lead-Halide Perovskites as Seen by Halide Magnetic Resonance

Lead-halide perovskites increasingly mesmerize researchers because they exhibit a high degree of structural defects and dynamics yet nonetheless offer an outstanding (opto)electronic performance on par with the best examples of structurally stable and defect-free semiconductors. This highly unusual feature necessitates the adoption of an experimental and theoretical mindset and the reexamination of techniques that may be uniquely suited to understand these materials. Surprisingly, the suite of methods for the structural characterization of these materials does not commonly include nuclear magnetic resonance (NMR) spectroscopy. The present study showcases both the utility and versatility of halide NMR and NQR (nuclear quadrupole resonance) for probing the structure and structural dynamics of CsPbX 3 (X = Cl, Br, I), in both bulk and nanocrystalline forms. The strong quadrupole couplings, which originate from the interaction between the large quadrupole moments of, e.g., the 35 Cl, 79 Br, and 127 I nuclei, and the local electric-field gradients, are highly sensitive to subtle structural variations, both static and dynamic. The quadrupole interaction can resolve structural changes with accuracies commensurate with synchrotron X-ray diffraction and scattering. It is shown that space-averaged site-disorder is greatly enhanced in the nanocrystals compared to the bulk, while the dynamics of nuclear spin relaxation indicates enhanced structural dynamics in the nanocrystals. The findings from NMR and NQR were corroborated by ab initio molecular dynamics, which point to the role of the surface in causing the radial strain distribution and disorder. These findings showcase a great synergy between solid-state NMR or NQR and molecular dynamics simulations in shedding light on the structure of soft lead-halide semiconductors.

36 MATERIALS SCIENCE↗
DOE OSTI2021

Effects of Al:Si and (Al + Na):Si ratios on the properties of the international simple glass, part I: Physical properties

Understanding composition-structure-property relationships of high-alumina nuclear waste glasses are important for vitrification of nuclear waste at the Hanford Site. Two series of glasses were designed, one with varying Al:Si ratios and the other with (Al+Na):Si ratios based on the International Simple Glass (ISG, a simplified nuclear waste model glass), with Al2O3 ranging from 0 to 23 mol % (0 to 32 wt. %). The glasses were synthesized and characterized using electron probe microanalysis, X-ray photoelectron spectroscopy, small angle X-ray scattering, high temperature oxide melt solution calorimetry, and infrared spectroscopy. Glasses were crystal free, and the lowest Na2O and Al2O3 glass formed an immiscible glass phase. Evolution of various properties - glass transition temperature, percentage of 4-coordinated B, enthalpy of glass formation - and infrared spectroscopy results indicate that structural effects differ based on the glass series.

Nuclear Waste Glass↗
DOE OSTI2024

Universal features of 2 → N scattering in QCD and gravity from shockwave collisions

A remarkable double-copy relation of Einstein gravity to QCD in Regge asymptotics is Γ μ ν = 1 2 C μ C ν − 1 2 N μ N ν , where Γ μ ν is the gravitational Lipatov vertex in the 2 → 3 graviton scattering amplitude, C μ its Yang-Mills counterpart, and N μ the QED bremsstrahlung vertex. In QCD, the Lipatov vertex is a fundamental building block of the BFKL equation describing the 2 → N scattering of gluons at high energies. Likewise, the gravitational Lipatov vertex is a key ingredient in a 2D effective field theory framework describing trans-Planckian 2 → N graviton scattering. We construct a quantitative correspondence between a semiclassical Yang-Mills framework for radiation in gluon shockwave collisions and its counterpart in general relativity. In particular, we demonstrate the Lipatov double copy in a dilute-dilute approximation corresponding to R S , L , R S , H ≪ b , where R S , L , R S , H are the respective emergent Schwarzchild radii generated in shockwave collisions and b is the impact parameter. We outline extensions of the correspondence developed here to the dilute-dense computation of gravitational wave radiation in the close vicinity of one of the black holes, the construction of graviton propagators in the shockwave background, and a renormalization group approach to compute 2 → N amplitudes that incorporates graviton Reggeization and coherent graviton multiple scattering. Published by the American Physical Society 2024

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2024

Heavy dark matter in white dwarfs: multiple-scattering capture and thermalization

We present an improved treatment for the scattering of heavy dark matter from the ion constituents of a white dwarf. In the heavy dark matter regime, multiple collisions are required for the dark matter to become gravitationally captured. Our treatment incorporates all relevant physical effects including the dark matter trajectories, nuclear form factors, and radial profiles for the white dwarf escape velocity and target number densities. Our capture rates differ by orders of magnitude from previous estimates, which have typically used approximations developed for dark matter scattering in the Earth. We also compute the time for the dark matter to thermalize in the center of the white dwarf, including in-medium effects such as phonon emission and absorption from the ionic lattice in the case where the star has a crystallized core. We find much shorter thermalization timescales than previously estimated, especially if the white dwarf core has crystallized. We illustrate the importance of our improved approach by determining the cross section required for accumulated asymmetric dark matter to self-gravitate.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
NASA NTRS1986

An X-ray heated wind in NGC 1068

Recent work published by Antonucci and Miller in 1985 has demonstrated the existence of a type 1 Seyfert nucleus inside the archetypical type 2 Seyfert galaxy NGC 1068. This nucleus is surrounded by an obscuring torus and is visible only by reflection from a warm electron scattering region on the torus's axis. Here it is shown that the warm region must be in a dynamic state and out of radiative equilibrium with the nuclear continuum. It is suggested that the source of this moving gas is the cold obscuring torus itself, and that the warm region is part of a wind driven by heating due to the central continuum. The obscuring torus may be an inner extension of the starburst region already known in NGC 1068. This model gives estimates of the temperature and optical depth of the electron scattering region consistent with the observed values. Variations in viewing angle and optical thickness in the torus may account for the range of observed properties in active galactic nuclei.

Krolik, J. H.↗
DOE OSTI2022

Partial muon capture rates in A = 3 and A = 6 nuclei with chiral effective field theory

Searches for neutrinoless-double beta decay rates are crucial in addressing questions within fundamental symmetries and neutrino physics. The rates of these decays depend not only on unknown parameters associated with neutrinos, but also on nuclear properties. In order to reliably extract information about the neutrino, one needs an accurate treatment of the complex many-body dynamics of the nucleus. Neutrinoless-double beta decays take place at momentum transfers on the order of 100 MeV/$c$ and require both nuclear electroweak vector and axial current matrix elements. Muon capture, a process in the same momentum transfer regime, has readily available experimental data to validate these currents. In this work, we present results of {\it ab initio} calculations of partial muon capture rates for $^3$He and $^6$Li nuclei using variational and Green's Function Monte Carlo computational methods. We estimate the impact of the three-nucleon interactions, the cutoffs used to regularize two-nucleon ($2N$) interactions, and the energy range of $2N$ scattering data used to fit these interactions.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
NASA NTRS2003

Expression of Prox1 defines regions of the avian otocyst that give rise to sensory or neural cells

The simple primordium of the inner ear (otocyst) differentiates into many cell types, including sensory neurons and hair cells. We examined expression of the divergent homeobox transcription factor, cProx1, during otocyst development in chickens. Nuclear cProx1 protein is not evident in the otic placode but emerges in the otic cup by stage 12. At stage 16, cProx1-positive nuclei are scattered continuously throughout the neuroepithelium, from anteroventral to posteromedial. These labeled cells are neural precursors; they express betaIII-tubulin and migrate to the cochleovestibular ganglion between stages 13 and 21. By stage 18, two areas develop a dense pattern of cProx1 expression in which every nucleus is labeled. These areas emerge at the anterior and posterior extremes of the band of scattered cProx1 expression and express the sensory markers cSerrate1 and Cath1 by stage 23. Four discrete patches of dense cProx1 expression appear by stage 23 that correspond to the future superior crista, lateral crista, saccular macula, and posterior crista, as confirmed by immunolabeling for hair cell antigen (HCA) by stage 29. The remaining sensory epithelia display a dense pattern of cProx1 expression and label for HCA by stage 29. In the basilar papilla, nuclear cProx1 expression is down-regulated in most hair cells by stage 37 and in many supporting cells by stage 40. Our findings show that regions of the otocyst that give rise to neurons or hair cells are distinguished by their relative density of cProx1-positive nuclei, and suggest a role for cProx1 in the genesis of these cell types.

NASA Discipline Developmental Biology↗
DOE OSTI2024

Chain extension epoxide polymerization to well‐defined block polymers using a N‐Al Lewis pair catalyst

Block polyethers comprised of poly(propylene oxide) (PPO) and poly(ethylene oxide) (PEG or PEO) segments form the basis of ABA-type PEO-b-PPO-b-PEO poloxamer materials. The inverse architecture with an internal hydrophilic PEO segment flanked by hydrophobic blocks can be difficult to prepare with control of architecture by use of traditional anionic polymerization. These oxyanionic polymerizations are plagued by chain-transfer-to-monomer side reactions that occur with substituted epoxides such as propylene oxide (PO). Herein, we report a new method for the preparation of block polymers through a controlled polymerization involving a N-Al Lewis adduct catalyst and an aluminum alkoxide macroinitiator. The Lewis pair catalyst was able to chain-extend commercial PEO macroinitiators to prepare di-, tri-, and pentablock polyethers with low dispersity and reasonable monomer tolerance. Chain extension was confirmed using size exclusion chromatography and diffusion ordered nuclear magnetic resonance spectroscopy. In conclusion, the resulting block polymers were additionally analyzed with small-angle X-ray scattering to correlate the morphology to molecular architecture.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2024

Renormalization group improved photon impact factors and the high energy virtual photon scattering

We perform the renormalization group improved collinear resummation of the photon-gluon impact factors. We construct the resummed cross section for virtual photon-photon (γ ∗ γ ∗ ) scattering which incorporates the impact factors and BFKL gluon Green’s function up to the next-to-leading logarithmic accuracy in energy. The impact factors include important kinematical effects which are responsible for the most singular poles in Mellin space at next-to-leading order. Further conditions on the resummed cross section are obtained by requiring the consistency with the collinear limits. Our analysis is consistent with previous impact factor calculations at NLO, apart from a new term proportional to C F that we find for the longitudinal polarization. Finally, we use the resummed cross section to compare with the LEP data on the γ ∗ γ ∗ cross section and with previous calculations. The resummed result is lower than the leading logarithmic approximation but higher than the pure next-to-leading one, and is consistent with the experimental data.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2023

Strange hadron collectivity in pPb and PbPb collisions

The collective behavior of K$_{S}^{0}$ and $Λ/ \overline{Λ}$ strange hadrons is studied by measuring the elliptic azimuthal anisotropy ($\mathcal{v}$ 2 ) using the scalar-product and multiparticle correlation methods. Proton-lead (pPb) collisions at a nucleon-nucleon center-of-mass energy $\sqrt{s_{NN}}$ = 8.16 TeV and lead-lead (PbPb) collisions at $\sqrt{s_{NN}}$ = 5.02 TeV collected by the CMS experiment at the LHC are investigated. Nonflow effects in the pPb collisions are studied by using a subevent cumulant analysis and by excluding events where a jet with transverse momentum greater than 20 GeV is present. The strange hadron $\mathcal{v}$ 2 values extracted in pPb collisions via the four- and six-particle correlation method are found to be nearly identical, suggesting the collective behavior. Comparisons of the pPb and PbPb results for both strange hadrons and charged particles illustrate how event-by-event flow fluctuations depend on the system size.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗