Engineering Papers⌕ Search

SEARCH · Engineering Papers

Results for “BACKSCATTERING”

Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

Quote a phrase for an exact phrase match. Source license links do not imply unrestricted reuse.

At least 1,081 records · Page 60

TPSAS-NF1676L-13037-DND

Mineral dust has a significant and uncertain role in the direct aerosol radiative forcing of climate. Spaceborne lidars such as CALIOP help reduce these uncertainties through vertical profile measurements of aerosol optical properties. One current limitation to the accurate retrieval of aerosol extinction and optical depth from CALIOP is the assumed relationship between the aerosol extinction to aerosol backscatter (i.e. the extinction-to-backscatter ratio, also referred to here as the lidar ratio or Sa). This problem is especially acute at 1064 nm, where few estimates of the lidar ratio exist. This study uses a dataset of eight underflights of CALIOP during August 2010 by the NASA Langley Research Center airborne High Spectral Resolution Lidar (HSRL) to study Saharan dust transported across the Atlantic Ocean. The standard HSRL profile products include aerosol backscatter coefficients and depolarization ratios at both 532 nm and 1064 nm, and aerosol extinction coefficients (and therefore also lidar ratios) at 532 nm only. In this work, we further derive estimates of aerosol lidar ratios and extinction coefficients at 1064 nm via application of a two-wavelength technique that uses the 532 nm aerosol backscatter coefficients and the 1064 nm attenuated total backscatter profile. Summary statistics of the dust lidar ratio and depolarization at 532 nm and 1064 nm from these eight flights are presented. Implications for the CALIOP dust and polluted dust aerosol types and lidar ratio selection are discussed. In addition to the two-wavelength retrievals of lidar ratio at 1064 nm, a demonstration case of a 1064 nm lidar ratio retrieval over the ocean from CALIOP using the CloudSat measurement of surface scattering cross section as a constraint is presented (Josset et al, 2010).

Raymond R Rogers↗

Science Performance Comparison Between a Spaceborne HSRL and CALIOP

NASA operates airborne and spaceborne lidar systems to answer aerosol and cloud related science questions. NASA Langley Research Center has extensive experience operating lidar systems in both regimes. These include High Spectral Resolution Lidar (HSRL) systems, which have been operating on airborne systems,and CALIOP, the spaceborne elastic backscatter lidar system on board CALIPSO. In support of NASA’s ACCP Study Plan to address the Aerosol (A) and Cloud, Convection, and Precipitation (CCP) Designated Observables called out in the 2017 Earth Science Decadal Survey, LaRC is using lidar simulation tools to evaluate the performance of spaceborne systems using both the HSRL and elastic backscatter techniques. The LaRC high-fidelity simulator tool models both HSRL and elastic backscatter lidar systems by modeling the effects of the instrument specifications and producing backscatter signals generated from molecules, aerosols, clouds, ocean surface, and ocean subsurface. It derives the solar background signals from the scene specific aerosol and cloud characteristics, surface type, and sun elevation. The tool models both random and systematic uncertainties in the retrieved geophysical parameters. In this study, we will present simulated results that compare and contrast the performance of spaceborne HSRL systems to the performance of CALIOP. As recommended by the Decadal Study, ACCP is seeking advances over performance that has been achieved by A-Train. This study will provide a description of the HSRL and elastic backscatter techniques and demonstrate how and why the performance of these HSRL systems exceeds the performance of CALIOP.

Kathleen A Powell↗

Airborne HSRL Assessment of CALIOP Aerosol Extinction Retrievals Constrained by Column AOD

Current operational CALIOP aerosol extinction profile retrievals usually rely on accurately specifying the relationship between aerosol extinction and backscattering (i.e. lidar ratio). Uncertainties in the assigned lidar ratios are typically the largest source of systematic error (~30-50%) in the CALIOP retrievals of aerosol extinction, backscatter, and aerosol optical depth. Alternatively, column aerosol optical depth (AOD) can be used to solve the lidar equation and obtain column-equivalent lidar ratios and retrieve aerosol extinction profiles from the CALIOP attenuated backscatter profiles. These derived lidar ratios correspond to the aerosols in the altitude range from 0-7 km. We derive column-equivalent aerosol lidar ratios and aerosol extinction profiles from CALIOP attenuated backscatter profiles constrained using co-located column AODs provided by several instruments/techniques: Synergized Optical Depth of Aerosols (SODA), Ocean-Derived Column Optical Depths (ODCOD), MODIS (dark target), MODIS (Multi-Angle Implementation of Atmospheric Correction-MAIAC), and PARASOL (Generalized Retrieval of Aerosol and Surface Properties-GRASP). These various retrievals of AOD and the column-average aerosol lidar ratios and aerosol extinction profiles derived from CALIOP using these AOD constraints are evaluated using the extensive record of coincident and co-located airborne HSRL measurements of AOD, aerosol lidar ratio, and aerosol extinction profiles acquired during more than 140 HSRL underflights of CALIPSO since 2006. The HSRL technique allows for the independent measurement of extinction and backscatter without the need for external constraints or assumptions regarding the lidar ratios. Initial comparisons with these coincident HSRL aerosol extinction profiles show that the CALIOP aerosol extinction profiles retrieved using these various AOD constraints are generally in better agreement with the HSRL measurements than aerosol extinction profiles from the operational techniques. The quality of agreement depends on the accuracy and magnitude of the AOD constraint. We present these comparisons of AOD, column aerosol lidar ratio, and aerosol extinction profiles for each of the AOD constraints described above.

lidar↗

hsrl (01)

High-spectral-resolution lidar (HSRL) systems collect data about clouds and aerosols. These systems provide vertical profiles of optical depth, backscatter cross-section, depolarization, and backscatter phase function. All HSRL measurements are absolutely calibrated by reference to molecular scattering, which is measured at each point in the lidar profile. Like the Raman lidar, but unlike simple backscatter lidars such as the micropulse lidar, the HSRL can measure backscatter cross-sections and optical depths without prior assumptions about the scattering properties of the atmosphere. The depolarization observations also allow robust discrimination between ice and water clouds. In addition, rigorous error estimates can be computed for all measurements. A very narrow, angular field of view reduces multiple scattering contributions. The small field of view, coupled with a narrow optical bandwidth, nearly eliminates noise due to scattered sunlight. ARM operates two HSRL systems, one at the Barrow, North Slope of Alaska (NSA) site and the other in the second ARM Mobile Facility (AMF2), which is deployed at various locations on field campaigns.

54 ENVIRONMENTAL SCIENCES↗

Scattering of electromagnetic waves from a magnetized plasma column at oblique incidence

Scattering of electromagnetic waves from a magnetized plasma column is investigated using Maxwell's equations and applying boundary conditions. Backscattering cross section is evaluated by analytic solution of electric fields inside and outside of plasma column. Plots of backscattering cross section versus frequency, for the range up to J band, reveal two main peaks and two sidebands. Effects of plasma density and radius, as main parameters determining the characteristics of plasma column, on backscattering are discussed. Furthermore, the effect of electromagnetic wave incidence angle on backscattering of plasma column is included in the analysis. The influence of wave incidence angle and frequency, as well as, plasma density and radius on scattering pattern, which is an indicator of the distribution of scattered power in different azimuthal angles, is discussed.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

High-Spectral Resolution Lidar (HSRL) Instrument Handbook

High-spectral-resolution lidar (HSRL) systems provide vertical profiles of optical depth, backscatter cross-section, depolarization, and backscatter phase function. All HSRL measurements are calibrated by reference to molecular scattering, which is measured at each point in the lidar profile. Like the Raman lidar (RL), but unlike simple backscatter lidars such as the micropulse lidar (MPL), this enables the HSRL to measure backscatter cross-sections and optical depths without prior assumptions about the scattering properties of the atmosphere. The depolarization observations allow robust discrimination between ice and water clouds. Rigorous error estimates can be computed for all measurements. A very narrow angular field of view reduces multiple scattering contributions. The small field of view, coupled with a narrow optical bandwidth, nearly eliminates noise due to scattered sunlight. The laser transmitter is a diode-pumped, frequency-doubled Nd:YAG laser. Narrow-band, single-frequency operation is provided by injection seeding with a single-frequency, cw-diode-pumped diode laser. The main laser cavity is maintained in resonance with the seed laser by adjusting the cavity length to minimize the time between the Q-switch trigger and the emission of the laser pulse. The emission wavelength is tuned via temperature control of the seed laser crystal and is locked to line #1109 of the iodine absorption spectra. Locking is accomplished by minimizing the transmission through a 2-cm-long iodine absorption cell. Use of a high-repetition-rate laser and expansion of the transmitted beam through a 400-mm telescope reduces the transmitted energy density to eye-safe levels. It is possible to look directly into the output beam without hazard. The receiver and transmitter use the same afocal telescope, simplifying the maintenance of stable alignment of the transmitter and receiver although the angular FOV is only 100 μrad. The small FOV and the 4-kHz repetition rate also limit the near-field signal strength, making it possible to record continuous profiles that start at an altitude of ~100 m and extend to 30 km using photon counting detectors. The small FOV also suppresses multiple scattering contributions.

54 ENVIRONMENTAL SCIENCES↗

First beryllium capsule implosions on the National Ignition Facility

The first indirect drive implosion experiments using Beryllium (Be) capsules at the National Ignition Facility confirm the superior ablation properties and elucidate possible Be-ablator issues such as hohlraum filling by ablator material. Since the 1990s, Be has been the preferred Inertial Confinement Fusion (ICF) ablator because of its higher mass ablation rate compared to that of carbon-based ablators. This enables ICF target designs with higher implosion velocities at lower radiation temperatures and improved hydrodynamic stability through greater ablative stabilization. Recent experiments to demonstrate the viability of Be ablator target designs measured the backscattered laser energy, capsule implosion velocity, core implosion shape from self-emission, and in-flight capsule shape from backlit imaging. The laser backscatter is similar to that from comparable plastic (CH) targets under the same hohlraum conditions. Implosion velocity measurements from backlit streaked radiography show that laser energy coupling to the hohlraum wall is comparable to plastic ablators. The measured implosion shape indicates no significant reduction of laser energy from the inner laser cone beams reaching the hohlraum wall as compared with plastic and high-density carbon ablators. These results indicate that the high mass ablation rate for beryllium capsules does not significantly alter hohlraum energetics. In addition, these data, together with data for low fill-density hohlraum performance, indicate that laser power multipliers, required to reconcile simulations with experimental observations, are likely due to our limited understanding of the hohlraum rather than the capsule physics since similar multipliers are needed for both Be and CH capsules as seen in experiments.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Experimental and calculational investigation of laser-heated additive manufactured foams

Foam materials are starting to find application in laser-heated Hohlraums used to drive inertial confinement fusion implosions. Foams made using additive manufacturing (AM) techniques are now available and may have advantages over traditional chemical (aerogel) foams. Here, we present new experimental data on laser-heated AM foams. Samples of four different types of printed AM foams were heated using a single 527 nm laser beam at the Jupiter Laser Facility. The laser pulse was ∼180 J square pulse with an FWHM of 1.6 ns and a peak intensity of 3–4 × 1014 W/cm2. The foam densities ranged from 12 to 93 mg/cc (all supercritical for 527 nm light). We measured the backscattered light (power and spectrum), the transmitted light, side-on x-ray images, and the Ti K-shell emission that was used to infer the time-integrated temperature. The fraction of backscattered light was 6%–15% of the input laser energy. The pure carbon foam sample had less backscatter than a C8H9O3 foam of similar density, which was consistent with multi-fluid calculations that predicted less ion heating for the C8H9O3 foam. The level of backscatter and the thermal front speeds for the AM foams were similar to values measured for stochastic (aerogel) foams under similar conditions.

36 MATERIALS SCIENCE↗

SU-E-I-22: Dependence On Calibration Phantom and Field Area of the Conversion Factor Used to Calculate Skin Dose During Neuro-Interventional Fluoroscopic Procedures

Purpose: To determine the appropriate calibration factor to use when calculating skin dose with our real-time dose-tracking system (DTS) during neuro-interventional fluoroscopic procedures by evaluating the difference in backscatter from different phantoms and as a function of entrance-skin field area. Methods: We developed a dose-tracking system to calculate and graphically display the cumulative skin-dose distribution in real time. To calibrate the DTS for neuro-interventional procedures, a phantom is needed that closely approximates the scattering properties of the head. We compared the x-ray backscatter from eight phantoms: 20-cm-thick solid water, 16-cm diameter water-filled container, 16-cm CTDI phantom, modified-ANSI head phantom, 20-cm-thick PMMA, Kyoto-Kagaku PBU- 50 head, Phantom-Labs SK-150 head, and RSD RS-240T head. The phantoms were placed on the patient table with the entrance surface at 15 cm tube-side from the isocenter of a Toshiba Infinix C-arm, and the entrance-skin exposure was measured with a calibrated 6-cc PTW ionization chamber. The measurement included primary radiation, backscatter from the phantom and forward scatter from the table and pad. The variation in entrance-skin exposure was also measured as a function of the skin-entrance area for a 30x30 cm by 20-cm-thick PMMA phantom and the SK-150 head phantom using four different added beam filters. Results: The entranceskin exposure values measured for eight different phantoms differed by up to 12%, while the ratio of entrance exposure of all phantoms relative to solid water showed less than 3% variation with kVp. The change in entrance-skin exposure with entrance-skin area was found to differ for the SK-150 head compared to the 20-cm PMMA phantom and the variation with field area was dependent on the added beam filtration. Conclusion: To accurately calculate skin dose for neuro-interventional procedures with the DTS, the phantom for calibration should be carefully chosen since different phantoms can contribute different backscatter for identical exposure parameters. Research supported in part by Toshiba Medical Systems and NIH Grants R43FD0158401, R44FD0158402 and R01EB002873.

61 RADIATION PROTECTION AND DOSIMETRY↗

Feasibility study of a dual detector configuration concept for simultaneous megavoltage imaging and dose verification in radiotherapy

Purpose: To test the feasibility of a dual detector concept for comprehensive verification of external beam radiotherapy. Specifically, the authors test the hypothesis that a portal imaging device coupled to a 2D dosimeter provides a system capable of simultaneous imaging and dose verification, and that the presence of each device does not significantly detract from the performance of the other. Methods: The dual detector configuration comprised of a standard radiotherapy electronic portal imaging device (EPID) positioned directly on top of an ionization-chamber array (ICA) with 2 cm solid water buildup material (between EPID and ICA) and 5 cm solid backscatter material. The dose response characteristics of the ICA and the imaging performance of the EPID in the dual detector configuration were compared to the performance in their respective reference clinical configurations. The reference clinical configurations were 6 cm solid water buildup material, an ICA, and 5 cm solid water backscatter material as the reference dosimetry configuration, and an EPID with no additional buildup or solid backscatter material as the reference imaging configuration. The dose response of the ICA was evaluated by measuring the detector’s response with respect to off-axis position, field size, and transit object thickness. Clinical dosimetry performance was evaluated by measuring a range of clinical intensity-modulated radiation therapy (IMRT) beams in transit and nontransit geometries. The imaging performance of the EPID was evaluated quantitatively by measuring the contrast-to-noise ratio (CNR) and spatial resolution. Images of an anthropomorphic phantom were also used for qualitative assessment. Results: The measured off-axis and field size response with the ICA in both transit and nontransit geometries for both dual detector configuration and reference dosimetry configuration agreed to within 1%. Transit dose response as a function of object thickness agreed to within 0.5%. All IMRT test patterns and clinical IMRT beams had gamma pass rates of ≥98% at 2%/2 mm criteria. In terms of imaging performance, the measured CNR and spatial resolution (f{sub 50}) were 263.23 ± 24.85 and 0.4025 ± 1.25 × 10{sup −3} for dual detector configuration and 324 ± 26.65 and 0.4141 ± 1.14 × 10{sup −3} for reference imaging configuration, respectively. The CNR and spatial resolution were quantitatively worse in the dual detector configuration due to the additional backscatter. The difference in imaging performance was not visible in qualitative assessment of phantom images. Conclusions: Combining a commercially available ICA dosimetry device with a conventional EPID did not significantly detract from the performance of either device. Further improvements in imaging performance may be achieved with an optimized design. This study demonstrates the feasibility of a dual detector concept for simultaneous imaging and dosimetry in radiation therapy.

60 APPLIED LIFE SCIENCES↗

Aerosol Plume Detection Algorithm Based on Image Segmentation of Scanning Atmospheric Lidar Data

An image-processing algorithm has been developed to identify aerosol plumes in scanning lidar backscatter data. The images in this case consist of lidar data in a polar coordinate system. Each full lidar scan is taken as a fixed image in time, and sequences of such scans are considered functions of time. The data are analyzed in both the original backscatter polar coordinate system and a lagged coordinate system. The lagged coordinate system is a scatterplot of two datasets, such as subregions taken from the same lidar scan (spatial delay), or two sequential scans in time (time delay). The lagged coordinate system processing allows for finding and classifying clusters of data. The classification step is important in determining which clusters are valid aerosol plumes and which are from artifacts such as noise, hard targets, or background fields. These cluster classification techniques have skill since both local and global properties are used. Furthermore, more information is available since both the original data and the lag data are used. Performance statistics are presented for a limited set of data processed by the algorithm, where results from the algorithm were compared to subjective truth data identified by a human.

97 MATHEMATICS AND COMPUTING↗

Spectroradiometric monitoring for open outdoor culturing of algae and cyanobacteria

We assess the measurement of hyperspectral reflectance for the outdoor monitoring of green algae and cyanobacteria cultures with a multi-channel, fiber-coupled spectroradiometer. Reflectance data acquired over a four-week period are interpreted via numerical inversion of a reflectance model, in which the above-water reflectance is expressed as a quadratic function of the single backscattering albedo, dependent on the absorption and backscatter coefficients. The absorption coefficient is treated as the sum of component spectra consisting of the cultured species (green algae or cyanobacteria), dissolved organic matter, and water (including the temperature dependence of the water absorption spectrum). The backscatter coefficient is approximated as the scaled Hilbert transform of the culture absorption spectrum with a wavelength-independent vertical offset. Additional terms in the reflectance model account for the pigment fluorescence features and the water surface reflection of sunlight and skylight. For both the green algae and cyanobacteria, the wavelength-independent vertical offset of the backscatter coefficient is found to scale linearly with daily dry weight measurements, providing the capability for a non-sampling measurement of biomass in outdoor ponds. Other fitting parameters in the reflectance model are compared to auxiliary measurements and physics-based calculations. The magnitudes of the sunlight and skylight water-surface contributions derived from the reflectance model compare favorably with Fresnel reflectance calculations, while the reflectance-derived quantum efficiency of Chl-a fluorescence is found to be in agreement with literature values. To conlclude, the water temperature derived from the reflectance model exhibits excellent agreement with thermocouple measurements during the morning hours and highlights significantly elevated temperatures in the afternoon hours.

47 OTHER INSTRUMENTATION↗

Doppler Lidar (DL) Instrument Handbook

The Doppler lidar (DL) is an active remote sensing instrument that provides range- and time-resolved measurements of radial velocity and attenuated backscatter. The principle of operation is similar to radar in that pulses of energy are transmitted into the atmosphere; the energy scattered back to the transceiver is collected and measured as a time-resolved signal. From the time delay between each outgoing transmitted pulse and the backscattered signal, the distance to the scatterer is inferred. The radial or line-of-sight velocity of the scatterers is determined from the Doppler frequency shift of the backscattered radiation. The DL uses a heterodyne detection technique in which the return signal is mixed with a reference laser beam (i.e., local oscillator) of known frequency. An onboard signal processing computer then determines the Doppler frequency shift from the spectra of the heterodyne signal. The energy content of the Doppler spectra can also be used to determine attenuated backscatter.

99 GENERAL AND MISCELLANEOUS↗

Lidar Inter-Comparison Exercise Final Campaign Report

The objective of this IOP was to evaluate the performances of the new Leosphere R-MAN 510 lidar procured by the Australian Bureau of Meteorology, by testing it against the MPL and Raman lidars at the Darwin ARM site. This lidar is an eye-safe (355 nm), turn-key mini Raman lidar, which allows for the detection of aerosols and cloud properties, and the retrieval of particulate extinction profiles. To do so, the R-MAN 510 lidar has been operated at the Darwin ARM site, next to the MPL, Raman lidar, and Vaisala ceilometer for three months (from 20 January 2013 to 20 April 2013) in order to collect a good sample for statistical comparisons. The comparisons with the Raman lidar were not performed, since the Raman lidar attenuated backscatter and depolarization ratio product was not available. A new product has just been delivered to the ARM archive as a value-added product, hence this study will continue. Nevertheless we have developed software to match the different space and time resolutions of the other lidars and project the data onto a common grid to permit detailed comparison of the instruments’ performance and an enhanced analysis of clouds and aerosols through the use of composite data products, like the ratios of attenuated backscatters, attenuated scattering ratios and depolarization ratios. Comparisons between the MPL and R-MAN510 lidar data exhibit large differences in total attenuated backscatter at 355 and 532 nm, attenuated scattering ratios, and aerosol volume depolarization ratios. Differences in attenuated backscatter result mainly from the different relative contributions of scattering from molecules and particles at the different wavelengths, but there are some intriguing differences that will require further investigations. The differences in volume depolarization ratios are due to the much larger contribution of molecular returns to the volume depolarization ratio (5 times larger at 355 nm than at 532 nm). The R-MAN510 lidar is also found to be much less sensitive to daylight solar background illumination, which is greater at the visible wavelength than in the UV.

54 ENVIRONMENTAL SCIENCES↗

State of Modeling Symmetry in Hohlraums

Modeling radiation drive asymmetry is challenging problem whose agreement with data depends on the hohlraum gas fill density. Modeling to date uses the HYDRA code with crossbeam energy transfer (CBET) calculated separately, and backscattered light removed from the input laser. For high fill hohlraums (~>1 mg/cc), matching symmetry requires ad hoc adjustments to CBET during picket and peak of drive. For near-vacuum hohlraums, there is little CBET or backscatter, and drive is more waist-high than predicted. For intermediate fill densities (~0.6 mg/cc) there appears to be a region of small CBET and backscatter where symmetry is reasonably well modeled. A new technique where backscatter and CBET are done “inline” appears it could bring high fill simulations closer to data.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Understanding the optical properties of ambient sub- and supermicron particulate matter: results from the CARES 2010 field study in northern California

Abstract. Measurements of the optical properties (absorption, scattering and extinction) of PM1, PM2.5 and PM10 made at two sites around Sacramento, CA, during the June 2010 Carbonaceous Aerosols and Radiative Effects Study (CARES) are reported. These observations are used to establish relationships between various intensive optical properties and to derive information about the dependence of the optical properties on photochemical aging and sources. Supermicron particles contributed substantially to the total light scattering at both sites, about 50 % on average. A strong, linear relationship is observed between the scattering Ångström exponent for PM10 and the fraction of the scattering that is contributed by submicron particles (fsca, PM1) at both sites and with similar slopes and intercepts (for a given pair of wavelengths), suggesting that the derived relationship may be generally applicable for understanding variations in particle size distributions from remote sensing measurements. At the more urban T0 site, the fsca, PM1 increased with photochemical age, whereas at the downwind, more rural T1 site the fsca, PM1 decreased slightly with photochemical age. This difference in behavior reflects differences in transport, local production and local emission of supermicron particles between the sites. Light absorption is dominated by submicron particles, but there is some absorption by supermicron particles ( ∼ 15 % of the total). The supermicron absorption derives from a combination of black carbon that has penetrated into the supermicron mode and from dust, and there is a clear increase in the mass absorption coefficient of just the supermicron particles with increasing average particle size. The mass scattering coefficient (MSC) for the supermicron particles was directly observed to vary inversely with the average particle size, demonstrating that MSC cannot always be treated as a constant in estimating mass concentrations from scattering measurements, or vice versa. The total particle backscatter fraction exhibited some dependence upon the relative abundance of sub- versus supermicron particles; however this was modulated by variations in the median size of particles within a given size range; variations in the submicron size distribution had a particularly large influence on the observed backscatter efficiency and an approximate method to account for this variability is introduced. The relationship between the absorption and scattering Ångström exponents is examined and used to update a previously suggested particle classification scheme. Differences in composition led to differences in the sensitivity of PM2.5 to heating in a thermodenuder to the average particle size, with more extensive evaporation (observed as a larger decrease in the PM2.5 extinction coefficient) corresponding to smaller particles; i.e., submicron particles were generally more susceptible to heating than the supermicron particles. The influence of heating on the particle hygroscopicity varied with the effective particle size, with larger changes observed when the PM2.5 distribution was dominated by smaller particles.

54 ENVIRONMENTAL SCIENCES↗

A global study of hygroscopicity-driven light-scattering enhancement in the context of other in situ aerosol optical properties

The scattering and backscattering enhancement factors (ƒ(RH) and ƒ b (RH)) describe how aerosol particle light scattering and backscattering, respectively, change with relative humidity (RH). They are important parameters in estimating direct aerosol radiative forcing (DARF). In this study we use the dataset presented in Burgos et al. (2019) that compiles ƒ(RH) and ƒ b (RH) measurements at three wavelengths (i.e., 450, 550 and 700 nm) performed with tandem nephelometer systems at multiple sites around the world. We present an overview of ƒ(RH) and ƒ b (RH) based on both long-term and campaign observations from 23 sites representing a range of aerosol types. The scattering enhancement shows a strong variability from site to site, with no clear pattern with respect to the total scattering coefficient. In general, higher ƒ(RH) is observed at Arctic and marine sites, while lower values are found at urban and desert sites, although a consistent pattern as a function of site type is not observed. The backscattering enhancement ƒ b (RH) is consistently lower than ƒ(RH) at all sites, with the difference between ƒ(RH) and ƒ b (RH) increasing for aerosol with higher ƒ(RH). This is consistent with Mie theory, which predicts higher enhancement of the light scattering in the forward than in the backward direction as the particle takes up water. Our results show that the scattering enhancement is higher for PM 1 than PM 10 at most sites, which is also supported by theory due to the change in scattering efficiency with the size parameter that relates particle size and the wavelength of incident light. At marine-influenced sites this difference is enhanced when coarse particles (likely sea salt) predominate. For most sites, ƒ(RH) is observed to increase with increasing wavelength, except at sites with a known dust influence where the spectral dependence of ƒ(RH) is found to be low or even exhibit the opposite pattern. The impact of RH on aerosol properties used to calculate radiative forcing (e.g., single-scattering albedo, ω 0 , and backscattered fraction, b) is evaluated. The single-scattering albedo generally increases with RH, while b decreases. The net effect of aerosol hygroscopicity on radiative forcing efficiency (RFE) is an increase in the absolute forcing effect (negative sign) by a factor of up to 4 at RH = 90 % compared to dry conditions (RH < 40 %). Because of the scarcity of scattering enhancement measurements, an attempt was made to use other more commonly available aerosol parameters (i.e., ω 0 and scattering Ångström exponent, α sp ) to parameterize ƒ(RH). The majority of sites (75 %) showed a consistent trend with ω 0 (higher ƒ(RH = 85 %) for higher ω 0 ), while no clear pattern was observed between ƒ(RH = 85 %) and αsp. This suggests that aerosol ω 0 is more promising than α sp as a surrogate for the scattering enhancement factor, although neither parameter is ideal. Nonetheless, the qualitative relationship observed between ω 0 and ƒ(RH) could serve as a constraint on global model simulations.

54 ENVIRONMENTAL SCIENCES↗

Methodology for deriving the telescope focus function and its uncertainty for a heterodyne pulsed Doppler lidar

Doppler lidars provide two measured parameters, radial velocity and signal-to-noise ratio, from which winds and turbulent properties are routinely derived. Attenuated backscatter, which gives quantitative information on aerosols, clouds, and precipitation in the atmosphere, can be used in conjunction with the winds and turbulent properties to create a sophisticated classification of the state of the atmospheric boundary layer. Calculating attenuated backscatter from the signal-to-noise ratio requires accurate knowledge of the telescope focus function, which is usually unavailable. Inaccurate assumptions of the telescope focus function can significantly deform attenuated backscatter profiles, even if the instrument is focused at infinity. Here, we present a methodology for deriving the telescope focus function using a co-located ceilometer for pulsed heterodyne Doppler lidars. The method was tested with Halo Photonics StreamLine and StreamLine XR Doppler lidars but should also be applicable to other pulsed heterodyne Doppler lidar systems. The method derives two parameters of the telescope focus function, the effective beam diameter and the effective focal length of the telescope. Additionally, the method provides uncertainty estimates for the retrieved attenuated backscatter profile arising from uncertainties in deriving the telescope function, together with standard measurement uncertainties from the signal-to-noise ratio. The method is best suited for locations where the absolute difference in aerosol extinction at the ceilometer and Doppler lidar wavelengths is small.

54 ENVIRONMENTAL SCIENCES↗