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At least 109 records · Page 6

On the Spatial Distribution of High Velocity Al-26 Near the Galactic Center

We present results of simulations of the distribution of 1809 keV radiation from the decay of Al-26 in the Galaxy. Recent observations of this emission line using the Gamma Ray Imaging Spectrometer (GRIS) have indicated that the bulk of the AL-26 must have a velocity of approx. 500 km/ s. We have previously shown that a velocity this large could be maintained over the 10(exp 6) year lifetime of the Al-26 if it is trapped in dust grains that are reaccelerated periodically in the ISM. Here we investigate whether a dust grain velocity of approx. 500 km/ s will produce a distribution of 1809 keV emission in latitude that is consistent with the narrow distribution seen by COMPTEL. We find that dust grain velocities in the range 275 - 1000 km/ s are able to reproduce the COMPTEL 1809 keV emission maps reconstructed using the Richardson-Lucy and Maximum Entropy image reconstruction methods while the emission map reconstructed using the Multiresolution Regularized Expectation Maximization algorithm is not well fit by any of our models. The Al-26 production rate that is needed to reproduce the observed 1809 keV intensity yields in a Galactic mass of Al-26 of approx. 1.5 - 2 solar mass which is in good agreement with both other observations and theoretical production rates.

Sturner, Steven J.↗

Evaluation of Electron Tomography Capabilities for Shale Imaging

Despite the advantageous resolution of electron tomography (ET), reconstruction of three-dimensional (3D) images from multiple two-dimensional (2D) projections presents several challenges, including small signal-to-noise ratios, and a limited projection range. This study evaluates the capabilities of ET for thin sections of shale, a complex nanoporous medium. A numerical phantom with 1.24 nm pixel size is constructed based on the tomographic reconstruction of a Barnett shale. A dataset of 2D projection images is numerically generated from the 3D phantom and studied over a range of conditions. First, common reconstruction techniques are used to reconstruct the shale structure. The reconstruction uncertainty is quantified by comparing overall values of storage and transport metrics, as well as the misclassification of pore voxels compared to the phantom. We then select the most robust reconstruction technique and we vary the acquisition conditions to quantify the effect of artifacts. We find a strong agreement for large pores over the different acquisition workflows, while a wider variability exists for nanometer-scale features. Furthermore, the limited projection range and reconstruction are identified as the main experimental bottlenecks, thereby suggesting that sample thinning, advanced holders, and advanced reconstruction algorithms offer opportunities for improvement.

3D scanning transmission electron microscopy↗

Ancilla-entangling Floquet kicks for accelerating quantum algorithms

Quantum simulation with adiabatic annealing can provide insight into difficult problems that are impossible to study with classical computers. However, it deteriorates when the systems scale up due to the shrinkage of the excitation gap and thus places an annealing rate bottleneck for high success probability. Here, in this study, we accelerate quantum simulation using digital multiqubit gates that entangle primary system qubits with ancillary qubits. The practical benefits originate from tuning the ancillary gauge degrees of freedom to enhance the quantum algorithm's original functionality in the system registry. For simple but nontrivial short-ranged, infinite long-ranged transverse-field Ising models, and the hydrogen molecule model after qubit encoding, we show improvement in the time to solution by one hundred percent but with higher accuracy through exact state-vector numerical simulation in a digital-analog setting. The findings are further supported by time-averaged Hamiltonian theory.

97 MATHEMATICS AND COMPUTING↗

Site Suitability and Air Pollution Impacts of Composting Infrastructure for California’s Organic Waste Diversion Law

The emerging field of polaritonic chemistry explores the behavior of molecules under strong coupling with cavity modes. Despite recent developments in ab initio polaritonic methods for simulating polaritonic chemistry under electronic strong coupling, their capabilities are limited, especially in cases where the molecule also features strong electronic correlation. To bridge this gap, we have developed a novel method for cavity QED calculations utilizing the Density Matrix Renormalization Group (DMRG) algorithm in conjunction with the Pauli–Fierz Hamiltonian. Our approach is applied to investigate the effect of the cavity on the S0–S1 transition of n-oligoacenes, with n ranging from 2 to 5, encompassing 22 fully correlated π orbitals in the largest pentacene molecule. Our findings indicate that the influence of the cavity intensifies with larger acenes. Additionally, we demonstrate that, unlike the full determinantal representation, DMRG efficiently optimizes and eliminates excess photonic degrees of freedom, resulting in an asymptotically constant computational cost as the photonic basis increases.

54 ENVIRONMENTAL SCIENCES↗

Radiative transfer calculated from a Markov chain formalism

The theory of Markov chains is used to formulate the radiative transport problem in a general way by modeling the successive interactions of a photon as a stochastic process. Under the minimal requirement that the stochastic process is a Markov chain, the determination of the diffuse reflection or transmission from a scattering atmosphere is equivalent to the solution of a system of linear equations. This treatment is mathematically equivalent to, and thus has many of the advantages of, Monte Carlo methods, but can be considerably more rapid than Monte Carlo algorithms for numerical calculations in particular applications. We have verified the speed and accuracy of this formalism for the standard problem of finding the intensity of scattered light from a homogeneous plane-parallel atmosphere with an arbitrary phase function for scattering. Accurate results over a wide range of parameters were obtained with computation times comparable to those of a standard 'doubling' routine. The generality of this formalism thus allows fast, direct solutions to problems that were previously soluble only by Monte Carlo methods. Some comparisons are made with respect to integral equation methods.

Esposito, L. W.↗

Survey of Gravitationally lensed objects in HSC Imaging (SuGOHI). VIII. New galaxy-scale lenses from the HSC SSP

Abstract We conduct a search for galaxy-scale strong gravitational lens systems in Data Release 4 of the Hyper Suprime-Cam Subaru Strategic Program (HSC SSP), consisting of data taken up to the S21A semester. We select 103191 luminous red galaxies from the Baryon Oscillation Spectroscopic Survey (BOSS) sample that have deep multiband imaging from the HSC SSP and use the YattaLens algorithm to identify lens candidates with blue arc-like features automatically. The candidates are visually inspected and graded based on their likelihood of being a lens. We find eight definite lenses, 28 probable lenses, and 138 possible lenses. The new lens candidates generally have lens redshifts in the range 0.3 ≲ zL ≲ 0.9, a key intermediate redshift range to study the evolution of galaxy structure. Follow-up spectroscopy will confirm these new lenses and measure source redshifts to enable detailed lens modeling.

Astronomy & Astrophysics↗

Clustering of the Diffuse Infrared Light from the COBE DIRBE Maps: Power Spectrum Analysis and Excess Isotropic Component of Fluctuations - 3

The cosmic infrared background (CIB) radiation is the cosmic repository for energy release throughout the history of the universe. The spatial fluctuations of the CIB resulting from galaxy clustering are expected to be at least a few percent on scales of a degree, depending on the luminosity and clustering history of the early universe. Using the all-sky data from the COBE DIRBE instrument at wavelengths 1.25 - 100 microns we attempt to measure the CIB fluctuations. In the near-IR, foreground emission is dominated by small scale structure due to stars in the Galaxy. There we find a strong correlation between the amplitude of the fluctuations and Galactic latitude after removing bright foreground stars. Using data outside the Galactic plane (absolute value of b > 20 deg) and away from the center (90 deg < l < 270 deg) we extrapolate the amplitude of the fluctuations to cosec absolute value of b = 0. We find a positive intercept of delta.F(sub rms) = 15.5(sup +3.7, sub -7.0), 5.9(sup +1.6, sub -3.7), 2.4(sup +0.5, sub -0.9), 2.0(sup +0.25, sub -0.5) nW/sq m.sr at 1.25, 2.2, 3.5 and 4.9 microns respectively, where the errors are the range of 92% confidence limits. For color subtracted maps between band 1 and 2 we find the isotropic part of the fluctuations at 7.6(sup +1.2, sub -2.4) nW/sq m.sr. Based on detailed numerical and analytic models, this residual is not likely to originate from the Galaxy, our clipping algorithm, or instrumental noise. We demonstrate that the residuals from the fit used in the extrapolation are distributed isotropically and suggest that this extra variance may result from structure in the CIB. We also obtain a positive intercept from a linear combination of maps at 1.25 and 2.2 microns. For 2 deg < theta < 15 deg, a power-spectrum analysis yields limits of (theta/5 deg) x delta.F(sub rms)(theta) < 6, 2.5, 0.8, 0.5 nW/sq m.sr at 1.25, 2.2, 3.5 and 4.9 microns respectively. From 10 - 100 microns, the dominant foregrounds are emission by dust in the Solar system and the Galaxy. There the upper limits on the CIB fluctuations are below 1 nW/sq m.sr and are lowest (< equal 0.5 nW/sq m.sr) at 25 microns.

Kashlinsky, A.↗

Stress-dominated growth of two-dimensional materials on nonplanar substrates

Curved features are ubiquitous on solid surfaces, but the effect of surface curvatures on growth of two-dimensional (2D) materials has not yet been established. Using a newly developed method based on the Metropolis algorithm and taking graphene as a prototype, we find that a curved feature on substrates can result in a variety of topological defects in 2D materials. As the feature's size increases by just nanometers, the defects can vary from adatoms, dislocation pairs, and grain boundary scars to long-range grain boundaries, in contrast to previously reported defect-free modes of rigid colloidal crystals growing on spheres. We identify an important role of curvature-induced lattice stress in lowering the growth rate over the curved features and driving a plastic instability in the materials. When the feature's size increases to several nanometers, the stress effect is compromised by an enhanced effect of geodesic curvature, yielding long-range grain boundaries as a result of increased local growth rate on the feature with respect to that on flat regions. Here we further provide a ‘phase diagram’ of defects that helps to guide a rational choice of geometrical parameters of features towards the growth of high-quality 2D materials as well as controllable creation of topological defects.

36 MATERIALS SCIENCE↗

Autonomously Calibrating a Quadrupole Mass Spectrometer

A computer program autonomously manages the calibration of a quadrupole ion mass spectrometer intended for use in monitoring concentrations and changes in concentrations of organic chemicals in the cabin air of the International Space Station. The instrument parameters calibrated include the voltage on a channel electron multiplier, a discriminator threshold, and an ionizer current. Calibration is achieved by analyzing the mass spectrum obtained while sweeping the parameter ranges in a heuristic procedure, developed by mass spectrometer experts, that involves detection of changes in signal trends that humans can easily recognize but cannot necessarily be straightforwardly codified in an algorithm. The procedure includes calculation of signal-to-noise ratios, signal-increase rates, and background-noise-increase rates; finding signal peaks; and identifying peak patterns. The software provides for several recovery-from-error scenarios and error-handling schemes. The software detects trace amounts of contaminant gases in the mass spectrometer and notifies associated command- and-data-handling software to schedule a cleaning. Furthermore, the software autonomously analyzes the mass spectrum to determine whether the parameters of a radio-frequency ramp waveform are set properly so that the peaks of the mass spectrum are at expected locations.

Lee, Seungwon↗

Correlated Anion Disorder in Heteroanionic Cubic TiOF 2

Resolving anion configurations in heteroanionic materials is crucial for understanding and controlling their properties. For anion-disordered oxyfluorides, conventional Bragg diffraction cannot fully resolve the anionic structure, necessitating alternative structure determination methods. We have investigated the anionic structure of anion-disordered cubic (ReO 3 -type) TiOF 2 using X-ray pair distribution function (PDF), 19 F MAS NMR analysis, density functional theory (DFT), cluster expansion modeling, and genetic-algorithm structure prediction. Our computational data predict short-range anion ordering in TiOF 2 , characterized by predominant cis-[O 2 F 4 ] titanium coordination, resulting in correlated anion disorder at longer ranges. To validate our predictions, we generated partially disordered supercells using genetic-algorithm structure prediction and computed simulated X-ray PDF data and 19 F MAS NMR spectra, which we compared directly to experimental data. To construct our simulated 19 F NMR spectra, we derived new transformation functions for mapping calculated magnetic shieldings to predicted magnetic chemical shifts in titanium (oxy)fluorides, obtained by fitting DFT-calculated magnetic shieldings to previously published experimental chemical shift data for TiF 4 . We find good agreement between our simulated and experimental data, which supports our computationally predicted structural model and demonstrates the effectiveness of complementary experimental and computational techniques in resolving anionic structure in anion-disordered oxyfluorides. From additional DFT calculations, we predict that increasing anion disorder makes lithium intercalation more favorable by, on average, up to 2 eV, highlighting the significant effect of variations in short-range order on the intercalation properties of anion-disordered materials.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Component-to-Optimization Workflow Demonstration

This report aims to demonstrate workflow-generating algorithms for optimizing dispatch across a broad range of Integrated Energy System applications using the Framework for Optimization of Resources and Economics (FORCE) tool suite. The optimization is performed at two different time scales. In the coarse time scale, the optimization focuses on a class of energy sources and consumers and aims to find the optimal combinations and flows of energy based on real-time price data information. In the fine time scale, the optimization focuses on a specific thermal energy delivery system and aims to find the optimal setpoints of components in order to meet the energy demands from coarse-time-scale optimizations. In this demonstration, the coarse-scale optimization is implemented using the newly developed Dispatch Optimization Variable Engine (DOVE), while the fine-scale optimization used Optimization of Real-Time Capacity Allocation (ORCA).

29 ENERGY PLANNING, POLICY, AND ECONOMY↗

Preservation and Enhancement of the Spacewatch Data Archives

In March of 1998, the asteroid 1997 XF11 was announced to be potentially hazardous after being tracked over 90 days. A potential two year wait for confirming observations was shortened to under 24 hours because of the existence of archived photographic prediscovery images. Spacewatch was a pioneer in using CCD scanning and possesses a valuable digital archive of its scans. Unfortunately these data are aging on magnetic tape and will soon be lost. Since 1990, the Spacewatch project gathered some 1.5 Terabytes of scan data covering roughly 75,000 degrees of sky to a limiting magnitude of V = 21.5. The data have not yet been mined for all of their asteroids for scientific studies and orbit determination. Spacewatch's real-time motion detection program MODP was constrained by the computers of the era to use simplified image processing algorithms at a reduced efficiency. Jedicke and Herron estimated MODP's efficiency at finding asteroids to be approximately 60 percent to V=18 and improving somewhat thereafter. This lead to a substantial bias correction in their analyses. Larsen has developed a MODP replacement capable in excess of 90 percent efficiency in the same range and able to push a magnitude fainter in completeness. We propose a program of post-processing and re-archiving Spacewatch data. Our scans would be transferred from tape to CD-ROMs and converted to FITS images -- establishing a consistent data format and media for both past and future Spacewatch observations. Larsen's MODP replacement would mine these data for previously undetected motions, which would be made available to the Minor Planet Center and our ongoing asteroid population studies. A searchable observation record would be made generally available for prediscovery work. We estimate the net asteroid yield of this proposal is equivalent to three full years of Spacewatch operations.

Larsen, Jeffrey A.↗

Association between optically identified galaxy clusters and the underlying dark matter halos

Clusters of galaxies trace massive dark matter halos in the Universe, but they can include multiple halos projected along lines of sight. Here, we study the halos contributing to clusters using the Cardinal simulation, which mimics the Dark Energy Survey data. We use the red-sequence-based cluster finding algorithm redMaPPer as a case study. For each cluster, we identify the halos hosting its member galaxies, and we define the main halo as the one contributing the most to the cluster's richness ($λ$, the estimated number of member galaxies). At $z=0.3$, for clusters with $λ> 60$, the main halo typically contributes to $92\%$ of the richness, and this fraction drops to $67\%$ for $λ\approx 20$. Defining "clean" clusters as those with $\geq50\%$ of the richness contributed by the main halo, we find that $100\%$ of the $λ> 60$ clusters are clean, while $73\%$ of the $λ\approx 20$ clusters are clean. Three halos can usually account for more than $80\%$ of the richness of a cluster. The main halos associated with redMaPPer clusters have a completeness ranging from $98\%$ at virial mass $10^{14.6}~h^{-1}M_{\odot}$ to $64\%$ at $10^{14}~h^{-1}M_{\odot}$. In addition, we compare the inferred cluster centers with true halo centers, finding that $30\%$ of the clusters are miscentered with a mean offset $40\%$ of the cluster radii, in agreement with recent X-ray studies. These systematics worsen as redshift increases, but we expect that upcoming surveys extending to longer wavelengths will improve the cluster finding at high redshifts. Our results affirm the robustness of the redMaPPer algorithm and provide a framework for benchmarking other cluster-finding strategies.

79 ASTRONOMY AND ASTROPHYSICS↗

Measurements of Rainfall Rate, Drop Size Distribution, and Variability at Middle and Higher Latitudes: Application to the Combined DPR-GMI Algorithm

The Global Precipitation Measurement mission is a major U.S.–Japan joint mission to understand the physics of the Earth’s global precipitation as a key component of its weather, climate, and hydrological systems. The core satellite carries a dual-precipitation radar and an advanced microwave imager which provide measurements to retrieve the drop size distribution (DSD) and rain rates using a Combined Radar-Radiometer Algorithm (CORRA). Our objective is to validate key assumptions and parameterizations in CORRA and enable improved estimation of precipitation products, especially in the middle-to-higher latitudes in both hemispheres. The DSD parameters and statistical relationships between DSD parameters and radar measurements are a central part of the rainfall retrieval algorithm, which is complicated by regimes where DSD measurements are abysmally sparse (over the open ocean). In view of this, we have assembled optical disdrometer datasets gathered by research vessels, ground stations, and aircrafts to simulate radar observables and validate the scattering lookup tables used in CORRA. The joint use of all DSD datasets spans a large range of drop concentrations and characteristic drop diameters. The scaling normalization of DSDs defines an intercept parameter N(W), which normalizes the concentrations, and a scaling diameter D(m), which compresses or stretches the diameter coordinate axis. A major finding of this study is that a single relationship between N(W) and D(m), on average, unifies all datasets included, from stratocumulus to heavier rainfall regimes. A comparison with the N(W)–D(m) relation used as a constraint in versions 6 and 7 of CORRA highlights the scope for improvement of rainfall retrievals for small drops (D(m) < 1 mm) and large drops (D(m) > 2 mm). The normalized specific attenuation–reflectivity relationships used in the combined algorithm are also found to match well the equivalent relationships derived using DSDs from the three datasets, suggesting that the currently assumed lookup tables are not a major source of uncertainty in the combined algorithm rainfall estimates.

Viswanathan Bringi↗

Low-mass Active Galaxies in the SAMI Galaxy Survey with Spatially Resolved Spectroscopy

The smallest supermassive black holes (BHs), which provide constraints on BH seeds, reside in low-mass galaxies. Here, we present a systematic analysis of 990 low-mass galaxies in the SAMI Galaxy Survey to identify emission from accreting BHs using integral field spectroscopy (IFS). Employing a novel automated scoring algorithm based on spatially resolved narrow emission-line diagnostics, we find signatures of active galactic nuclei (AGNs) in 41 galaxies, as well as an additional 46 (less secure) candidates. The galaxies have stellar masses between 10 9.4 ≲ M ⋆ /M ⊙ ≲ 10 10 (down to 10 8.5 , including less secure candidates), redshifts z ≲ 0.06, and morphologies ranging from early-type ellipticals to late-type spirals. Our AGN fraction of 4% (9% if we include the less secure candidates) is significantly higher than those reported by studies using single-fiber spectroscopy (≲1%–2%). Indeed, our additional analysis of single-fiber spectra of the objects in our sample demonstrates that many of our AGN candidates detected via IFS are missed. This work highlights the advantages of IFS, especially the ability to capture extended or decentralized emission from accreting BHs.

79 ASTRONOMY AND ASTROPHYSICS↗

Towards Precision Photometric Type ia Supernova Cosmology With Machine Learning

The revolutionary discovery of dark energy and accelerating cosmic expansion was made with just 42 type Ia supernovae (SNe Ia) in 1999. Since then, large synoptic surveys, e.g., Dark Energy Survey (DES), have observed thousands more SNe Ia and the upcoming Rubin Legacy Survey of Space and Time (LSST) and Roman Space Telescope promise to deliver millions in the next decade. This unprecedented data volume can produce the required precision to unambiguously test concordance cosmology which could represent a monumental shift in our understanding of dark energy and its role in cosmic history. However, extracting a pure SN Ia sample with accurate redshifts for such a large dataset will be a challenge. Specifically, spectroscopic classification will not be possible for the vast majority of discovered objects, and only ~25% will have spectroscopic redshifts. This thesis presents a series of observational and methodological studies designed to address the questions associated with this new era of photometric SN Ia cosmology. First, we present a machine learning method for photometric classification of SNe, Supernova Classification with a COnvolutional Neural Network (SCONE). Photometric classification enables SNe with no spectroscopic information to be confidently categorized, and is a critical component of current and future analysis pipelines. SCONE achieves >99% accuracy distinguishing simulated SNe Ia from non-Ia SNe, and has been integrated into DES, LSST, and Roman analysis pipelines. We also demonstrate the efficacy of SCONE on early-time photometric classification, which will be vital for optimal allocation of spectroscopic resources. We show that SCONE can distinguish between 6 SN types with 75% accuracy on the night of initial discovery, comparable to results in the literature for full-phase SNe. Next, we study current methods for estimating SN Ia redshifts and propose a machine learning alternative that uses SN photometry alone to extract redshift information. Most SNe Ia inherit redshift information from their host galaxy, but the process of matching SNe to the correct host galaxy can be challenging. We systematically analyze the impact of incorrect redshifts from host galaxy mismatch on 5 years of DES SN data, and conclude that improved host matching or redshift estimation methods can reduce our systematic errors by ~10%. In response to this finding, we present a SN photometry-only method for estimating redshifts independent of host galaxy information, Photo-zSNthesis. We show that Photo-zSNthesis redshift estimates are accurate to within 2% across the full redshift range of LSST, a first in the literature. Finally, we focus on the robustness of machine learning (ML) algorithms for real-world and scientific applications. ML models generalize poorly beyond their training set and often experience severe performance degradation when deployed on new data. We demonstrate a general method for improving robustness that achieves new state-of-the-art results on astronomical object classification, wildlife identification, and tumor detection.

79 ASTRONOMY AND ASTROPHYSICS↗

Comparison of multiobjective optimization methods for the $\mathrm{LCLS-II}$ photoinjector

Particle accelerators are among some of the largest science experiments in the world and can consist of thousands of components with a wide variety of input ranges. These systems can easily become unwieldy optimization problems during design and operations studies. Starting in the early 2000s, searching for better beam dynamics configurations became synonymous with heuristic optimization methods in the accelerator physics community. Genetic algorithms and particle swarm optimization are currently the most widely used. These algorithms can take thousands of simulation evaluations to find optimal solutions for one machine prototype. For large facilities such as the Linac Coherent Light Source (LCLS) and others, this equates to a limited exploration of many possible design configurations. In this paper, the LCLS-II photoinjector is optimized with three optimization algorithms. All optimizations were started from both a uniform random and Latin hypercube sample. In all cases, the optimizations started from Latin hypercube samples outperformed optimizations started from uniform samples. All three algorithms were able to optimize the photoinjector, with the model-based methods approximating the Pareto front in fewer simulation evaluations. This work, in combination with previous optimization observations, indicates objective penalties have a strong impact on the efficiency of such methods. In general, we recommend heuristic methods for initial optimizations and model-based methods when information about the objective space is available.

43 PARTICLE ACCELERATORS↗

Fast Bayesian optimization of Needle-in-a-Haystack problems using zooming memory-based initialization (ZoMBI)

Abstract Needle-in-a-Haystack problems exist across a wide range of applications including rare disease prediction, ecological resource management, fraud detection, and material property optimization. A Needle-in-a-Haystack problem arises when there is an extreme imbalance of optimum conditions relative to the size of the dataset. However, current state-of-the-art optimization algorithms are not designed with the capabilities to find solutions to these challenging multidimensional Needle-in-a-Haystack problems, resulting in slow convergence or pigeonholing into a local minimum. In this paper, we present a Zooming Memory-Based Initialization algorithm, entitled ZoMBI, that builds on conventional Bayesian optimization principles to quickly and efficiently optimize Needle-in-a-Haystack problems in both less time and fewer experiments. The ZoMBI algorithm demonstrates compute time speed-ups of 400× compared to traditional Bayesian optimization as well as efficiently discovering optima in under 100 experiments that are up to 3× more highly optimized than those discovered by similar methods.

36 MATERIALS SCIENCE↗