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At least 109 records · Page 6

Augmented Monitoring and Condition Assessment Program for SNF Wet Storage Life Extension - 20489

Approximately 27 MTHM of spent nuclear fuel (SNF) owned and managed by the U.S. Department of Energy, Office of Environmental Management is stored in the L Basin at the Savannah River Site (SRS). This 'DOE SNF' is comprised of approximately 12,000 aluminum-clad, aluminum-based fuel assemblies (∼7 MTHM), and approximately 2000 non-aluminum fuel assemblies (∼20 MTHM). A program is in progress to perform Non-Destructive Examination (NDE) of the fuel and their storage containers to characterize the materials' condition, and to evaluate the effects of service to enable continued safe wet storage of the SNF. The Augmented Monitoring and Condition Assessment Program (AMCAP), a two-part program to develop and implement remote underwater Non-Destructive Examination of the aluminum SNF, and of the containers of the non-aluminum SNF, respectively, is aimed at the characterization and evaluation of corrosion degradation of aluminum fuel and container materials. The predominant design of the aluminum SNF (ASNF) stored in L Basin is the Materials Test Reactor (MTR) equivalent design, a plate fuel design. These SNF are stored in 5'' diameter tubes or 5'' x 5'' squares (called bundles) that are nominally 12' or up to 14' long. The SNF is de-bundled and inspected using a custom-designed MTR Fuel Inspection Table. The inspection table provides for indexed fuel positioning for a video camera examination with controlled lighting. A total of 10 of the SNF originating from foreign research and test reactors were selected for examination based on burnup, enrichment, and prior damage caused by service/storage history. A special inspection campaign of these 10 assemblies is in progress. The observed corrosion damage included minor to moderate attack from general corrosion, pitting, crevice, end grain and galvanic corrosion. Example results from the completed inspections are shown and discussed. The focus is a comparison of the as-received condition versus the as-found current storage condition that will serve to validate Water Chemistry and Corrosion Monitoring Programs. The non-aluminum SNF (NASNF) stored in L Basin are of diverse design that includes various geometries with claddings of stainless steel, Zircaloy, and Hastelloy. The fuel core materials include uranium alloys, oxides/mixed oxides, and carbides. These SNF materials, originating from early experimental and test reactors, are in various physical forms including single fuel elements and cut pieces. The fuel is stored in L Basin in various configurations including in direct bundled storage in aluminum tubes and in isolation cans that are in the bundles or in a larger over-size storage container (OSC). Concern with inside-out corrosion and the potential loss of configuration control and ability to handle the storage containers prompted the development of remote NDE methods that include visual and UT technologies to assess the condition of the containers. Candidate stored materials were selected for a special inspection campaign; the development of the NDE methods for the inspection for galvanic, crevice and sediment-induced corrosion (inside-out) are discussed. A summary of the SNF storage in L Basin at the SRS, and an overview of the AMCAP to enable continued safe storage of DOE SNF are described. (authors)

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

BISON: A Finite Element-Based Nuclear Fuel Performance Code

BISON is a finite element-based nuclear fuel performance code applicable to a variety of fuel forms including light water reactor fuel rods, TRISO particle fuel, and metallic rod and plate fuel. It is a multiphysics fuel analysis tool that solves fully-coupled thermomechanical problems. BISON is based on MOOSE and can efficiently solve problems using standard workstations or very large high-performance computers in a variety of different dimensions, including full 3D, 2D-RZ axisymmetric, layered axisymmetric 1D, and spherically symmetric 1D systems. It is developed by a team of scientists and engineers at Idaho National Laboratory and by collaborators. The development of BISON is supported by various funding agencies, principally the United States Department of Energy.

11 - NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

(Oxy)hydroxides Formed on Aluminum Fuel Materials After Irradiation and Long-Term Wet Storage - 20354

The aluminum cladding of research-reactor fuel experiences general corrosion when in contact with water during in-reactor service and post-discharge wet storage, resulting in the formation of adherent aluminum (oxy)hydroxide films. These (oxy)hydroxides contain chemically-bound water that poses challenges for extended dry storage due to the risk of thermal or radiolytic decomposition releasing free water and/or hydrogen and oxygen gases. This study describes characterization of the (oxy)hydroxides present on several aluminum materials used in reactor operation and subsequently stored wet in the L-Basin storage facility at the Savannah River Site (SRS) for an extended period. Characterization data providing insight into the loading, composition, and morphology of (oxy)hydroxides to be expected on service-exposed aluminum cladding provides valuable benchmarks for designing adequate drying and dry-storage approaches. This work is part of a broader investigation to address knowledge gaps and technical data needs for dry storage of aluminum-clad spent nuclear fuel (ASNF), which included in-lab growth of (oxy)hydroxide films on aluminum alloy substrates to investigate formation behavior, investigation of drying methods to remove existing (oxy)hydroxides from ASNF cladding, and measurement of radiolytic yield of hydrogen from (oxy)hydroxide powders and films. In this study, (oxy)hydroxide films were characterized for three aluminum-alloy materials used in reactors and subsequently stored wet for up to approximately 40 years in L-Basin at SRS: one cropping from a Missouri University Research Reactor (MURR) fuel element (Al-6061 alloy), one cropping from a Universal Sleeve Housing (USH) (Al-6063 alloy), and one Mark-16B fuel assembly (either Al-6061 or Al- 6063). The USH and Mark-16B were used in SRS production reactors. Characterization of the as-received (oxy)hydroxides included scanning electron microscopy (SEM) in both plan-view and cross-section to characterize the (oxy)hydroxide layer's morphology, thickness, and structure. X-ray diffraction (XRD) was used to identify the chemical composition and distinguish between the various aluminum (oxy)hydroxides known to form under reactor and storage conditions. XRD analysis revealed both bayerite (Al(OH)3) and boehmite (AlOOH) on the surface of the MURR and USH samples, as well as bayerite, boehmite, and gibbsite (another Al(OH)3 polymorph) on the surface of the Mark-16B sample. The aluminum trihydroxides, bayerite and gibbsite, are typically associated with corrosion in low-temperature (<80 deg. C) water, while boehmite is expected to form at higher water temperature (>80 deg. C). The presence of bayerite on the USH, which is believed to have operated close to 90 deg. C, suggests that boehmite formed during in-reactor exposure was not protective against further hydroxide growth in low-temperature wet storage. Cross-section scanning electron microscopy (SEM) showed total (oxy)hydroxide layer thicknesses of ∼5- 10 μm for the MURR and ∼5-15 μm for the Mark-16B. The thickness of the USH's (oxy)hydroxide layer was indiscernible by the current mounting and imaging method, despite plan-view SEM and XRD confirming the presence of an (oxy)hydroxide layer. (authors)

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Application of FREMES to Characterize and Sort Soil During Site Remediation - 20182

During decommissioning of buildings and the related release of nuclear sites, large amounts of bulk materials such as soil must be measured for clearance. These measurements are required to demonstrate that for example potentially contaminated soil is below the respective radiological limits. Doing so also helps to minimize the amount of bulk material which has to be disposed of as nuclear waste. NUKEM Technologies Engineering Services GmbH (NUKEM) applies their FREMES technology in a project at the former fuel element factory of FBFC International at Dessel, Belgium. The purpose is to measure and check for potential contamination within the excavated soil. The project started in 2017 with design and procurement of the necessary equipment. In October 2017 the FREMES system was installed at the site. After installation and an extensive test program the FREMES facility went fully into operation in July 2018. Original foreseen to measure between 4.000 and 8.000 tons of material, it has currently (mid 2019) measured 23.600 tons. It is expected that another 5.000 tons still have to be measured before the project successfully ends. (authors)

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Aluminum Spent Fuel Performance in Dry Storage Task 4 Aluminum Oxide Sampling of ATR Dry Stored Fuel

Milestone report on sampling of long-term dry-stored ATR spent fuel elements. It describes tooling, sample acquisition methods and analysis of the aluminum oxide samples by scanning electron microscopy, thermogravimetric analysis, X-ray diffraction and transmission electron microscopy. The observations provide input to projections on controls necessary for maintaining the integrity of the fuel during extended interim storage.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

SCALE Modeling of the Fast Spectrum Heat Pipe Reactor

As part of the severe accident analysis collaboration with Sandia National Laboratories (SNL) and the Nuclear Regulatory Commission (NRC), SCALE models were developed for a fast-spectrum heat pipe reactor. These models were based on the Idaho National Laboratory (INL) Design A concept, which is an alternative design to the Los Alamos National Laboratory (LANL) Special Purpose Reactor (SPR), also known as the Megapower reactor. The model contains 1,134 heat pipes, surrounded by hexagonal fuel elements, with a potassium working fluid; the fuel is UO 2 with 19.75 wt% 235 U enrichment. The model contains axial beryllium oxide (BeO) reflectors above and below the active fuel region along with a radial alumina reflector containing 12 B 4 C control drums. The center of the core is left unfueled to make room for two shutdown control rods, one annular and one solid. The active region of the core was discretized into twenty axial and five radial zones to analyze spatial variations in power and burnup. Infinite lattice unit cell sensitivity studies were used to perform verification between the SCALE and INL models. The eigenvalue results agreed well with the reported results to within roughly 50 percent mille (pcm). Full-core model verification was performed by analyzing system eigenvalues with differing configurations of control drum and shutdown rod positions. These full core results all had eigenvalue differences less than 310 pcm. Control drum and shutdown rod worths were also compared, with differences of 3.2% or less. Using the verified model, the isotopic inventory and decay heat, as well as temperature feedback coefficients, were calculated and provided to SNL as input to the MELCOR severe accident code to analyze potential releases from this class of reactor. The results of the MELCOR analysis are provided in a different report.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

The STAT7 Code for Statistical Propagation of Uncertainties in Steady State Thermal Hydraulics Analysis of Plate Fueled Reactors

The STAT7 software was developed to perform steady-state thermal hydraulic analyses. Application of the software is for non-power research and test reactors, including conversion to low-enriched uranium fuel of U.S. High-Performance Research Reactors such as MITR-II. Since it can be necessary to repeat analysis during fuel reloading, STAT7 accommodates flexibility in analyzing many realistic aspects of reactor fuel management. STAT7 uses a Monte Carlo approach to model common fabrication parameters and other key reactor analysis uncertainties required for research and test reactor thermal hydraulic analyses. These safety calculations are ultimately intended to protect against high fuel plate temperatures due to critical heat flux or departure from nucleate boiling or onset of flow instability; but additional margin is obtained by basing the limiting safety settings on avoiding onset of nucleate boiling. STAT7 can simultaneously analyze all of the axial nodes of all of the fuel plates and all of the coolant channels for one lateral stripe of a fuel element. The stripes run the length of the fuel, from the bottom to the top. Power splits are calculated for each axial node of each plate to determine how much of the power goes out each face of the plate. By running STAT7 multiple times, full core analysis can be performed by analyzing the margin to onset of nucleate boiling and onset of flow instability for each axial node of each stripe of each plate of each element in the core.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

The HRA/Solarium Project: Feedback Based on 20 Years of Experience in Treatment of Medium Level Waste - 20185

Since the 1980's the management of the historical site of Mol has been transferred to the National Agency for Radioactive Waste and Enriched Fissile Materials (ONDRAF/NIRAS). Belgoprocess is entrusted by ONDRAF/NIRAS with the operational waste management and site remediation. One of the major challenges has been the characterization, treatment and conditioning of approximately 200 m{sup 3} of medium level waste. These waste packages were stored in poor conditions in storage vaults ('HRA') or concrete containers ('Solarium'). They have been produced in various research programs and reactor operations at the Belgian nuclear energy research centre SCK.CEN, isotope production, decontamination and dismantling operations from the 1960's up to the 1980's. Despite the limited volume, this historical waste consists of a great variation of waste characteristics and waste configurations. To tackle these liabilities, a new processing facility was built in the 1990's to allow safe transfers, handling, characterization and treatment of these packages. Also some auxiliary facilities have been built to deal with the by-products, like emptied concrete containers. The engineering of the installation, safety procedures and (characterization) methodology that has been developed generically have been proved to be successful. Nevertheless, the specific nature of some items made it necessary to organize a step-by-step treatment in distinct campaigns in which some relevant extra (safety) measures had to be taken into account. This dynamic approach made it possible to process a great variety of waste types in order to to ensure that this legacy is no longer left for subsequent generations. After about 20 years of operations, there has been a great build-up of experience and feed-back concerning the waste management of these specific waste streams. Some cases will be highlighted to specify the approach followed for treatment of e.g.: - Na/NaK containing equipment; - spent radioactive sources; - fuel element residues; - medium level waste originating from activation experiments; - radium bearing medium level waste originating from Ac-227 production research. (authors)

07 ISOTOPE AND RADIATION SOURCES↗

The STAT7 Code for Statistical Propagation of Uncertainties In Steady-State Thermal Hydraulics Analysis of Plate-Fueled Reactors

STAT7 was written to automate many of the steady-state thermal hydraulic safety calculations for the MIT research reactor, both for conversion of the reactor from highly enriched uranium fuel to low-enriched uranium fuel and for future fuel re-loads after the conversion. A Monte-Carlo statistical propagation approach is used to treat uncertainties in important parameters in the analysis. These safety calculations are ultimately intended to protect against high fuel plate temperatures due to critical heat flux or departure from nucleate boiling or onset of flow instability; but additional margin is obtained by basing the limiting safety settings on avoiding onset of nucleate boiling. STAT7 can simultaneously analyze all of the axial nodes of all of the fuel plates and all of the coolant channels for one stripe of a fuel element. The stripes run the length of the fuel, from the bottom to the top. Power splits are calculated for each axial node of each plate to determine how much of the power goes out each face of the plate. By running STAT7 multiple times, full core analysis can be performed by analyzing the margin to ONB for each axial node of each stripe of each plate of each element in the core.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Codisposal Waste Package Loading Options for DOE SNF and HLW PPT

The U.S. Department of Energy (DOE) is responsible for managing spent nuclear fuel (SNF) that is currently in, or will in the future come into, its possession. DOE must continue to safely store that SNF, transport it to an interim storage site or a repository, and dispose of it. These fuels come from a wide range of reactor types with various cladding materials and enrichments. Many of these reactors, now decommissioned, had unique design features, such as core configuration, fuel element and assembly geometry, moderator and coolant materials, operational characteristics, and neutron spatial and spectral properties, resulting in a large diversity of reactor and fuel designs. Because of the wide variety and conditions of SNF, a robust DOE Standard Canister was proposed that would confine radionuclides and preclude moderator. The DOE Standard Canister had four variations: 3.05-meter (10-foot) or 4.57-meter (15-foot) length, and 45.7-cm (18-inch) or 61.0-cm (24-inch) diameter. For ultimate disposal in the Yucca Mountain Repository, these canisters were to be grouped with 61.0-cm (24-inch) diameter high level waste (HLW) canisters in a 2.13-meter (84-inch) diameter co-disposal waste package. The smaller 45.7-cm (18-inch) diameter DOE Standard Canister could be placed in the middle of five HLW canisters. The larger 61.0-cm (24-inch) diameter DOE Standard Canister would take the place of one of the five HLW canisters on the outer ring in the co-disposal waste package. No DOE Standard Canisters have been loaded. A preliminary evaluation has estimated the number of elements of a fuel type that can fit into the different sizes of the DOE Standard Canister, but no definitive loading configuration has been selected. Changing the loading configuration could impact the number of loadable DOE Standard Canisters and the number of co-disposal waste packages needed for eventual disposition. This paper conveys the ranges of DOE Standard Canisters and HLW canisters that may be produced under certain conditions. It also examines the differences in the estimated number of co-disposal waste packages produced for eventual disposal when using different loading strategies in the DOE Standard Canister for Advanced Test Reactor (ATR), Peach Bottom, and High Flux Isotope Reactor (HFIR) SNF. Changing the loading configurations of ATR, Peach Bottom, and HFIR SNF slightly impacted the number of co-disposal waste packages that may be needed for ultimate disposal. The change in loading configuration was more impactful when a different canister was used, as opposed to varying the number of elements that could fit inside the same size canister. In one case, a reduction of co-disposal waste packages could be achieved by allowing mixing of short HLW canisters with long DOE Standard Canisters. The main conclusion from this analysis is that the ratio between HLW canisters and DOE Standard Canisters will drive the total number of co-disposal waste packages. If too many HLW canisters (i.e., more than five times the number of 18-inch DOE standard canisters) or DOE Standard Canisters are produced, some co-disposal waste packages may not have all positions filled. A co-disposal waste package may be filled with all HLW with no DOE Standard Canister, or a co-disposal waste package could be filled with a single DOE Standard Canister. A ratio that does not closely align to optimum could allow for the design of waste packages that hold just HLW canisters or just DOE SNF canisters.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Co-Disposal Waste Package Loading Options for DOE SNF and HLW - 20331

The U.S. Department of Energy (DOE) is responsible for managing spent nuclear fuel (SNF) that is currently in, or will in the future come into, its possession. DOE must continue to safely store that SNF, transport it to an interim storage site or a repository, and dispose of it. These fuels come from a wide range of reactor types with various cladding materials and enrichments. Many of these reactors, now decommissioned, had unique design features, such as core configuration, fuel element and assembly geometry, moderator and coolant materials, operational characteristics, and neutron spatial and spectral properties, resulting in a large diversity of reactor and fuel designs. Because of the wide variety and conditions of SNF, a robust DOE Standard Canister was proposed that would confine radionuclides and preclude moderator. The DOE Standard Canister had four variations: 3.05-meter (10-foot) or 4.57-meter (15-foot) length, and 45.7-cm (18-inch) or 61.0-cm (24-inch) diameter. For ultimate disposal in the Yucca Mountain Repository, these canisters were to be grouped with 61.0-cm (24-inch) diameter high level waste (HLW) canisters in a 2.13-meter (84-inch) diameter co-disposal waste package. The smaller 45.7-cm (18-inch) diameter DOE Standard Canister could be placed in the middle of five HLW canisters. The larger 61.0-cm (24-inch) diameter DOE Standard Canister would take the place of one of the five HLW canisters on the outer ring in the co-disposal waste package. No DOE Standard Canisters have been loaded. A preliminary evaluation has estimated the number of elements of a fuel type that can fit into the different sizes of the DOE Standard Canister, but no definitive loading configuration has been selected. Changing the loading configuration could impact the number of loadable DOE Standard Canisters and the number of co-disposal waste packages needed for eventual disposition. This paper conveys the ranges of DOE Standard Canisters and HLW canisters that may be produced under certain conditions. It also examines the differences in the estimated number of co-disposal waste packages produced for eventual disposal when using different loading strategies in the DOE Standard Canister for Advanced Test Reactor (ATR), Peach Bottom, and High Flux Isotope Reactor (HFIR) SNF. Changing the loading configurations of ATR, Peach Bottom, and HFIR SNF slightly impacted the number of co-disposal waste packages that may be needed for ultimate disposal. The change in loading configuration was more impactful when a different canister was used, as opposed to varying the number of elements that could fit inside the same size canister. In one case, a reduction of co-disposal waste packages could be achieved by allowing mixing of short HLW canisters with long DOE Standard Canisters. The main conclusion from this analysis is that the ratio between HLW canisters and DOE Standard Canisters will drive the total number of co-disposal waste packages. If too many HLW canisters (i.e., more than five times the number of 18-inch DOE standard canisters) or DOE Standard Canisters are produced, some co-disposal waste packages may not have all positions filled. A co-disposal waste package may be filled with all HLW with no DOE Standard Canister, or a co-disposal waste package could be filled with a single DOE Standard Canister. A ratio that does not closely align to optimum could allow for the design of waste packages that hold just HLW canisters or just DOE SNF canisters. (authors)

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Specification of EBR-II Laser Profilometry Data

All laser profilometry data stored in FIPD were originally measured using the element laser profilometer system in HFEF/N. The irradiated fuel elements or pins were scanned by a laser beam to measure the outer diameter with position mapping of the spacer wire. The normal operation and data collection were performed automatically with HFEF/N Data Acquisition and Process Control System (DAPCS). With the digital control system, measured laser profilometry data were recorded in digital form on magnetic tapes, different from the analog contact profilometry data recorded by strip-chart record sheets. Two documents contained most of the important details about laser profilometry measurements. The first one is the operational manual of the laser profilometer (title: Element laser profilometer (ELP) operation and maintenance manual, HFEF/N OMM 4329, DOC. NO. W0171-0149-ES-01). This manual provides: (1) description of laser profilometer including the functions of each component (transceiver, retroreflector, clamping guide, shielding enclosure, electronic controller, etc.); (2) step-by-step guidance for calibrations, operations and measurements; and (3) maintenance procedures and other details of the element laser profilometer. Since first issued on 12/1/1986, several revisions/changes of the manual were developed to update the measurement accuracies and other factors for the laser profilometer system. The second document is a publicly accessible conference article titled “the element laser profilometer system in HFEF/N.” This article summarizes important functions and parameters of the laser profilometer. The range of measurements and the uncertainties reported in the article were consistent with the values reported in the operational manual.

42 ENGINEERING↗

Metallic Coating of Cerium Oxide Microspheres

The ability to remove heat is paramount to nuclear fuel performance and longevity. Retaining fission product and separating fuel from reactor coolant and the environment is also necessary to prevent radiological contamination. Conventional nuclear fuel for commercial light water reactors and radioisotope power systems (RPS) is composed of oxide powders pressed into a pellet (cm-scale) and then sealed into a metal cladding to confine the fuel. What typical fuels lack is a method to surround each particle of nuclear fuel in metal, thus providing a more intimate protection layer for accident tolerance and boosting the thermal extraction from the fuel element. In such a way, metal-coated fuel particles increase heat extraction efficiency over clad-pellet designs while increasing the accident tolerance of the fuel. Metal oxide microspheres have wide-ranging applications, including the realm of fuels for nuclear reactors and RPS. Microspheres of uranium oxide/uranium carbide, mixed uranium/plutonium oxides, transuranics, and thorium fuels have been extensively studied. Pacific Northwest National Laboratory has also demonstrated the production of 238 PuO 2 microspheres for RPS applications. Metal-coated oxide microsphere fuels may also be attractive for other applications such as nuclear thermal rockets, future nuclear reactor designs, and catalysts.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Simplifying the Advanced Test Reactor LOWE Element Test Series

The Advanced Test Reactor (ATR) is one of six remaining high performance research reactors in the United States scheduled to be converted from 93% high-enriched uranium (HEU) fuel to 19.75% low-enriched uranium (LEU) fuel as part of the Department of Energy (DOE), National Nuclear Security Administration (NNSA), Office of Material Management and Minimization (MMM) reactor conversion efforts(1). The specific LEU fuel element design for the ATR is called the Low Enriched (LOWE) element. A series of fuel qualification tests are scheduled to occur over the next decade before the ATR is fully converted. In addition to several experiments of demonstration plates, a series of Element Tests (ETs) are planned for conversion, in which full sized LOWE elements are placed in ATR driver positions. The purpose of these ETs was generally to sequentially increase the amount of LEU and core power to full power, therefore creating a representative safety profile in which LEU could operate for the duration of the ATR lifetime. The planned element tests were (2): ET-1: one LOWE element at low power for once cycle ET-2: ~8 LOWE elements at low/medium power for multiple cycles, and ET-3: >8 LOWE elements for a full lobe of elements at high power for multiple cycles. Given recent improvements in modeling fidelity, scheduling considerations, and an opportunity to combine later ETs, the LEU conversion program successfully defined the operational requirements for the “ET-ATR” test, which combines the needed information collected from ET-2 and ET-3 into a single test.

42 ENGINEERING↗

Metallic Fuel Performance Code Requirements for the Versatile Test Reactor Project

Metallic nuclear fuels have been proposed for use in several emerging nuclear reactor designs, and a number of codes have been developed to model these fuels and assess their performance. Qualification of these metallic nuclear fuels will ultimately require monitored irradiation of lead test assemblies, but the use of fuel performance codes can reduce the uncertainty associated with these efforts by quantifying uncertainties and estimating margins to failure ahead of time. In this work, metallic fuel performance code requirements are defined for the Versatile Test Reactor (VTR) project using input from the Experimental Breeder Reactor II functional requirements, operational requirements, and design criteria. This work focuses on the thermomechanical responses and irradiation behaviors of metallic fuel elements that are representative of the proposed VTR driver fuel design concepts. As such, many of the code requirements and physics/modeling discussions in this work are expected to be broadly applicable to metallic fuel applications outside of the VTR project.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Sensitivity of UO 2 fuel performance to microstructural evolutions driven by dilute additives

Use of dilute additives to nuclear fuel is being considered to increase the security of commercial fuel management through traceability of fabricated fuel elements. Taggants, as additives are denoted when included for traceability purposes, may also improve fuel performance, as demonstrated in Cr-containing uranium dioxide as described in the literature, and they may also improve fuel safety. In fact, studies have shown that some additives affect fuel material properties such as grain size and density after sintering. Given the possible range of elements that could be used as additives, the impact of such fuel property variations on the fuel’s thermomechanical behavior becomes relevant. These effects can be evaluated through a sensitivity study of standard fuel models to analyze changes in these properties using a fuel performance code. In this work, the BISON code is being used to investigate these effects through a 2D axisymmetric model of smeared UO 2 fuel pellets and ZIRLO® cladding under realistic pressurized water reactor core irradiation conditions. Here, randomly sampled densities and grain sizes within specified ranges are used as input parameters in the simulations, and several fuel model-related outputs are evaluated. The thermomechanical response of the cladding is also addressed in this study. The simultaneous variation of both input parameters offers a more comprehensive path to identify key sensitivities. Outputs explored include temperature, fission gas release, creep, and radial stress. Results show that although most of these outputs are sensitive to grain size to a certain extent, density mainly affects fuel temperature and elastic strain. Furthermore, sensitivities can vary depending on the radial position within the fuel pellet.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Review of the Technical Basis for Properties and Fuel Performance Data Used in HEU to LEU Conversion Analysis for U-10Mo Monolithic Alloy Fuel

This report provides the technical basis for properties and fuel performance data used in conversion analysis for U.S. High Performance Research Reactors (USHPRR) that will convert from highly enriched uranium (HEU) to low-enriched uranium (LEU) using a new U-10Mo monolithic alloy fuel that is being qualified. The conditions that the fuel experiences changes between an HEU and LEU fuel element design due to many causes, including the density of the fuel, the presence of U-238 resonant absorber, changes to the plate and coolant channel dimensions, and changes in fuel management due to reactivity or optimization. These types of changes have been documented in operational and safety analyses conducted for conversions over decades for over 70 reactors. These conversions have all, or almost all, required recalculation of safety-related values as well as establishing operational characteristics of the core, including power distribution, reactor core power level, and cycle length between required fuel management. An overall objective of conversion is to change the reactor core design as little as possible while maintaining the reactors’ scientific, isotope production, medical, and engineering missions.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗