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At least 109 records · Page 6

Evaluation of refractory-metal-clad uranium nitride and uranium dioxide fuel pins after irradiation for times up to 10 450 hours at 990 C

The effects of some materials variables on the irradiation performance of fuel pins for a lithium-cooled space power reactor design concept were examined. The variables studied were UN fuel density, fuel composition, and cladding alloy. All pins were irradiated at about 990 C in a thermal neutron environment to the design fuel burnup. An 85-percent dense UN fuel gave the best overall results in meeting the operational goals. The T-111 cladding on all specimens was embrittled, possibly by hydrogen in the case of the UN fuel and by uranium and oxygen in the case of the UO2 fuel. Tests with Cb-1Zr cladding indicate potential use of this cladding material. The UO2 fueled specimens met the operational goals of less than 1 percent cladding strain, but other factors make UO2 less attractive than low-density UN for the contemplated space power reactor use.

Bowles, K. J.↗

High Spatial Resolution Mapping of Retained Fission Gas

Fission gas isotopic analysis provides quantitative high precision determination of irradiated nuclear fuel burnup, offers diagnostic value, and informs fuel performance models. A measurement capability has been developed at Idaho National Laboratory (INL) for the release of retained fission gas using a focused laser and static noble gas mass spectrometry (MS) analysis. This high resolution (10s microns spot size) capability was demonstrated using Xe implanted metal foils.

07 - ISOTOPES AND RADIATION SOURCES↗

POST-TEST EXAMINATIONS OF A LOCA SAMPLE FROM AN IRRADIATED HIGH-BURNUP PWR M5 FUEL ROD

A LOCA integral test with high burnup PWR M5 fuel rod was conducted in the Irradiated Fuel Examination Laboratory through the complete LOCA sequence: heating the LOCA sample to 300ºC and pressurizing the internal pressure to 8.27 MPa, heating at 5ºC/s from 300 to 1200ºC, holding in steam for 90s at 1200ºC, cooling at 3ºC/s to 800ºC, followed by water quench and rapid cooling to 100ºC. After LOCA testing, examinations, such as the fuel fragmentation analysis, burst and ballooning characterization, axial strain measurement, and microstructural examinations were performed. Metallographic examinations of an as-irradiated high burnup sample adjacent to the LOCA test sample revealed a bonding layer between the fuel and cladding. The posttest LOCA examinations indicates the corrosion layer formed during normal operations in the commercial reactor might provide a protection against the steam oxidation at high temperatures for test times performed in this work. The microstructure of the as-irradiated fuel is compared to the microstructure of the post-LOCA test fuel. Posttest LOCA examination on unirradiated post-tests Zr cladding samples was conducted, which served as baseline data for in cell testing with irradiated samples. The results obtained with irradiated PWR high burnup M5 fuel rad were compared to the LOCA test data obtained with irradiated BWR high burnup Zircaloy-2 fuel rod at Argonne national Laboratory.

Yan, Yong↗

High-Burnup LOCA Burst Susceptibility BISON Analysis in PWRs and BWRs

Accurately assessing high-burnup fuel behavior during loss-of-coolant accidents (LOCAs) is essential for understanding fuel fragmentation, relocation, and dispersal (FFRD) risks across the US light-water reactor fleet. This work updates previous Nuclear Energy Advanced Modeling and Simulation (NEAMS) Program multiphysics LOCA analyses for a pressurized water reactor (PWR) and a boiling water reactor (BWR) by incorporating recent model and material property advancements in the BISON fuel performance code, including a high-burnup structure (HBS) model, revised cladding burst criteria, and updated thermal–mechanical correlations. This update was needed to support ongoing industry initiatives and upcoming regulatory changes. Full-core, rod-resolved operating histories generated using Virtual Environment for Reactor Analysis (VERA) and system-level LOCA conditions obtained from TRACE were applied to statistically representative rod samples in BISON to evaluate burst behavior and FFRD susceptibility. These calculations used two cladding burst correlations and three fuel pulverization models so that the predictions of these models could be compared. The updated PWR simulations show markedly improved numerical stability as the number of crashed simulations decreased by 95% compared to the previous study, and hence higher confidence in results. The updated PWR simulations predicted cladding bursts exclusively among once-burned, high-power rods, with two different cladding burst models identifying the same burst-susceptible population. Resulting FFRD susceptibility estimates are significantly reduced compared with earlier studies, driven by cooler predicted fuel and plenum temperatures, lower hoop strains, and reduced fission gas release in the updated models. In contrast, none of the BWR rods were predicted to burst under either burst criterion, reaffirming minimal BWR FFRD susceptibility even with updated HBS and material models. Comparisons between the PWR and BWR end-of-cycle predictions are made. Comparison with prior work highlights significant shifts in PWR fuel performance metrics and confirmation of earlier BWR conclusions. Overall, the updated results underscore the importance of having high-resolution detailed modeling capability and continuously integrating evolving material models and physics into high-resolution multiphysics simulations. The unified assessment presented here strengthens confidence in predicting high-burnup LOCA behavior by improving agreement between different cladding burst correlations. These results also provide an improved foundation for future BISON model development, FFRD susceptibility calculations.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Status of the Fuel Fragment Dispersal Studies at Oak Ridge National Laboratory

During a loss-of-coolant accident, a nuclear fuel rods undergo balloon and burst. High burnup fuel is known to fragment and pulverize leading to the potential for the fuel to disperse through the burst opening either during the initial burst or following the burst during the reflood event. This milestone summarizes the design and assembly of a system to study dispersal in a postburst event. Surrogate fuel material (HfO 2 , tungsten, and yttria-stabilized zirconia [YSZ]) dispersing from as-burst loss-of-coolant accident (LOCA) test specimens was extensively investigated, along with dispersal of actual nuclear fuel following a LOCA Severe Accident Test Station (SATS) test.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Status of the Fuel Fragment Dispersal Studies at Oak Ridge National Laboratory

During a loss-of-coolant accident, a nuclear fuel rods undergo balloon and burst. High burnup fuel is known to fragment and pulverize leading to the potential for the fuel to disperse through the burst opening either during the initial burst or following the burst during the reflood event. This milestone summarizes the design and assembly of a system to study dispersal in a postburst event. Surrogate fuel material (HfO2, tungsten, and yttria-stabilized zirconia [YSZ]) dispersing from as-burst loss-of-coolant accident (LOCA) test specimens was extensively investigated, along with dispersal of actual nuclear fuel following a LOCA Severe Accident Test Station (SATS) test. Surrogate material tests spanned a variety of burst geometries, particle types, particle size distributions, and rod oscillation loadings (frequency and amplitude combinations).

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Update on Radiochemical Assessment of High Burnup Commercially Irradiated Fuel

This work documents an effort to collect burnup measurements on a high burnup rod, designated 6XV, and first cycle accident tolerant fuel (ATF) rod, designated 47I, to enable benchmarking of fuel performance codes and neutronics codes. In addition to measurements, Virtual Environment for Reactor Applications (VERA) full-core-depletion analysis was also performed for the rods that were experimentally analyzed to provide an opportunity for code validation. This effort focuses on collecting data from rods irradiated at Byron Generating Station and shipped to the Oak Ridge National Laboratory (ORNL) hot-cells. This data will also anchor non-destructive examination evaluations of burnup of the various fuel rods undergoing postirradiation examination (PIE) at ORNL. Previous PIE of these fuel rods provides some guidance on the burnup trend across the fuel. Axial gamma spectroscopy scans provide a measure of relative changes in burnup across a fuel pin. Mass spectrometry based burnup measurements performed for this work at specific axial locations in the fuel are fully quantitative. By combining the mass spectrometry data with the gamma scans it is possible to more quantitatively evaluate axial variations in burnup across the entire fuel pin [1]. The combined set of burnup evaluations will be made available to other organizations that have an interest in high burnup radiochemistry data for validation of neutronic simulations and source term evaluation such as the Nuclear Regulatory Commission (NRC).

Harp, Jason [Oak Ridge National Laboratory (ORNL),↗

Application of the bRapid fission matrix burnup methodology to the JSI TRIGA Mark II research reactor

The novel burnup methodology, bRAPID, of the RAPID code system has been applied to the TRIGA Mark II research reactor at the 'Jozef Stefan' Institute. This paper presents the first step in our goal for on-line determination of isotope inventory and burnup, that the RAPID code system with its Fission Matrix (FM) method enables. Burnup analysis of changes in FM coefficients due to TRIGA fuel burnup at different irradiation times and specific power distribution in the reactor core is presented. Our results demonstrate that primary contribution for changes of FM coefficients is the burnup of the destination s, while the spectrum differences, that arise due to fuel's core location, have negligible effect on FM coefficients. (authors)

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Fission Surface Power for the Exploration and Colonization of Mars

The colonization of Mars will require abundant energy. One potential energy source is nuclear fission. Terrestrial fission systems are highly developed and have the demonstrated ability to safely produce tremendous amounts of energy. In space, fission systems not only have the potential to safely generate tremendous amounts of energy, but could also potentially be used on missions where alternatives are not practical. Programmatic risks such as cost and schedule are potential concerns with fission surface power (FSP) systems. To be mission enabling, FSP systems must be affordable and programmatic risk must be kept acceptably low to avoid jeopardizing exploration efforts that may rely on FSP. Initial FSP systems on Mars could be "workhorse" units sized to enable the establishment of a Mars base and the early growth of a colony. These systems could be nearly identical to FSP systems used on the moon. The systems could be designed to be safe, reliable, and have low development and recurring costs. Systems could also be designed to fit on relatively small landers. One potential option for an early Mars FSP system would be a 100 kWt class, NaK cooled system analogous to space reactors developed and flown under the U.S. "SNAP" program or those developed and flown by the former Soviet Union ("BUK" reactor). The systems could use highly developed fuel and materials. Water and Martian soil could be used to provide shielding. A modern, high-efficiency power conversion subsystem could be used to reduce required reactor thermal power. This, in turn, would reduce fuel burnup and radiation damage .effects by reducing "nuclear" fuels and materials development costs. A realistic, non-nuclear heated and fully integrated technology demonstration unit (TDU) could be used to reduce cost and programmatic uncertainties prior to initiating a flight program.

Houts, Mike↗

Evaluating transient fission gas release in high burnup light water reactor fuel during loss of coolant accident conditions via new capabilities

In this work, the role of transient fission gas release (tFGR) in the cladding burst behavior of high burnup fuel during a loss-of-coolant accident (LOCA) in commercial light water reactors was further investigated via the use of a new apparatus. During the LOCA-related temperature ramps of high burnup fuel, the release of fission gases exceeds the steady-state release observed under normal operating conditions. An enhancement was made to the Oak Ridge National Laboratory Severe Accident Test Station (SATS) to probe the various factors influencing tFGR. Experiments were performed on commercially irradiated, zirconium-clad uranium dioxide fuel, and this paper details the design of the experimental setup, the initial test results, and the subsequent post-test analyses. Notably, the first test on high burnup fuel demonstrated a LOCA-relevant tFGR of 5.3% from an unpressurized fuel segment. The ultimate tFGR was 10.7% for beyond LOCA conditions. A follow-up test on similar fuel revealed a tFGR of 12.6% under comparable conditions. Microstructural analysis and an analysis of the released gas provide some insight regarding the source of tFGR in the fuel. Finally, a grain boundary bubble model may aid in the interpretation of the results and offer a guide for future work.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Sister Rod Destructive Examinations (FY2021) Appendix J: Leaching of High Burnup Used Nuclear Fuel in De-ionized Water

As a part of the DOE NE High Burnup Spent Fuel Data Project, Oak Ridge National Laboratory (ORNL) is performing destructive examinations (DEs) of high burnup (HBU) (>45 GWd/MTU) spent nuclear fuel (SNF) rods from the North Anna Nuclear Power Station operated by Dominion Energy. The SNF rods, called sister rods or sibling rods, are all HBU and include four different kinds of fuel rod cladding: standard Zircaloy-4 (Zirc-4), low-tin Zirc-4, ZIRLO, and M5. The leaching experiment was a part of a larger study by Yadukrishnan Sasikumar in defending his doctoral thesis at The Open University, School of Engineering and Innovation [13]. It utilized post-CIRFT Sister Rod test specimens that were slated for disposal. The leaching experiment aims to understand the trends in the radiolytic dissolution of High Burnup Spent Nuclear Fuel (SNF) when exposed to water (e.g., in-reactor or in-pool cladding failures). Specimens from a baseline M5-clad rod and a heat-treated M5 rod were cut from the fractured CIRFT specimens and placed in 100 mL de-ionized water for a period of 128 days. Both radial and axial sections were cut to provide different surface areas of fuel in contact with the leachate. During the four-month exposure period, aliquot samples of the leachate were analyzed gamma spectroscopy and inductively coupled plasma mass spectrometry (ICP-MS). The analysis quantified the amount of fuel leached into the solutions and provided individual isotopic release fractions (of 30+ isotopes) which were compared as a function of time and surface area of fuel exposed.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Identifying microstructures susceptible to pulverization in commercially irradiated high burnup UO2 under LOCA conditions

High burnup fuel fragmentation (HBFF) has been a concern in the nuclear industry for many years. When UO2 reaches and exceeds pellet average burnups around 55 GWd/tU, microstructural changes in the fuel pellet begin to occur that render the pellet susceptible to fine fragmentation under loss-of-coolant accident (LOCA) conditions. During a LOCA event, the cladding balloons and bursts, potentially releasing part of these fine fuel fragments into the reactor pressure vessel. This process is known as fuel fragmentation, relocation, and dispersal (FFRD). Presently, the US nuclear industry is developing a safety basis for FFRD with the goal of increasing burnups and pressurized water reactor cycle lengths. Increased cycle lengths would push the burnup limits of the fuel rods past the known threshold for HBFF susceptibility. In this work, the microstructural impact on HBFF was investigated by comparing the microstructures of as-irradiated rod segments to their post-LOCA tested counterparts. This investigation found that varied operational histories result in different microstructural evolutions across the pellet radius, which impacts the fragmentation behavior and radial location of the fragmentation. It is noted that regions with a high bubble density and a high density of grain boundaries fragment under LOCA-relevant conditions. In addition to the fragmentation that has been previously reported at the periphery of the fuel, fragmentation was also noted in the dark zone toward the fuel center. Analysis of the power histories of the fuel samples suggests that the dark zone forms in the central regions of the pellet between temperatures of approximately 740 and 960 °C.

McKinney, Casey [ORNL] (ORCID:0000000335383614)↗

Fracture behavior of irradiation induced nanocrystalline UO 2 studied by in-situ mechanical testing in transmission electron microscopy

Uranium Dioxide (UO 2 ) is widely used as a fuel in current light water reactors (LWRs). Upon accumulation of radiation damage, LWR UO 2 fuel pellets start to develop a different microstructure at the pellet periphery when fuel burnup exceeds 45–50 GWd/tHM. The resulting porous, nanocrystalline microstructure is one of the most prominent microstructural changes occurring in such fuel. Its fracture mechanisms, which causes fuel fine fragmentation, could impact safety limits when the cladding breaches. Direct measurements of these properties are challenging, therefore a surrogate obtained via ion irradiation can be used. In this study, multiple microcantilevers were fabricated by focused ion beam from both fresh UO 2 and UO 2 irradiated with 84 MeV Xe 26+ ions to a peak dose of 1357 displacements per atom (dpa). Further, the irradiation produced a pseudo high burnup structure approximately 2 µm below the surface. In-situ nano-mechanical bending tests were conducted to investigate the fracture behavior and the effect of the surrogate UO 2 high burnup structure on local fracture properties. Fresh UO 2 fuel was observed to fracture in transgranular mode without nucleation or movement of dislocations. However, the Xe-irradiated nanocrystalline microcantilevers fractured along the grain boundaries, with no influence from the pre-existing micro-cracks in the microcantilever. Fracture toughness for this type of surrogate high burnup UO 2 structure is reported for the first time in literature. Both the fracture stress and toughness show degradation for UO 2 as a result of Xe-irradiation.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

BISON-FIPD integration enhanced low-burnup SFR metallic fuel swelling model evaluation framework

Experiments indicated that metallic fuel in sodium-cooled fast reactors (SFRs) rapidly swells radially and axially at low burnup. Despite that, prior studies have been focused on describing high burnup axial fuel elongation. With recent conventional and non-conventional metallic fuel concepts being considered for license applications, understanding multidimensional fuel swelling at a wide range of burnup levels is important to fuel analysis and qualification activities. Here, we report the development and demonstration efforts of a low-burnup SFR metallic fuel swelling model evaluation framework using the BISON advanced fuel performance code. The framework leverages the Integral Fast Reactor (IFR) program X423 experiment data through the ongoing integration project to enable standardized and automated use of legacy metallic fuel irradiation data maintained in the SFR fuel irradiation and physics database (FIPD) for BISON metallic fuel model verification and validation. In conclusion, the performance of the framework was demonstrated using the two representative metallic fuel swelling model sets implemented in BISON, with a series of insights about future advanced swelling model development.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Advanced Electron Microscopy Characterization of the Fuel-Cladding Chemical Interaction Region in a High Burnup U-10Zr Fuel

To support the development of U-10Zr metallic fuel, advanced characterization techniques have been applied to the fuel-cladding chemical interaction (FCCI) region in a Na-bonded solid U-10Zr fuel cross-section that was irradiated to a burnup of ~13.1 at.% at the Fast Flux Test Facility. 17 phases were identified in the FCCI region through a combination of high-resolution scanning transmission electron microscopy (STEM), STEM based energy dispersive X-ray spectroscopy (STEM-EDS), and TEM based selective area electron diffraction (TEM-SAED) analysis. In this talk, we will also discuss the implications of results on metallic fuel FCCI by focusing on the formation of Zr rind, fission product migration, and HT-9 cladding integrality under the investigated thermal irradiation conditions. This work complements our previous study on the TEM characterization of the fuel region of this high burnup fuel sample and serves as scientific basis to support metallic fuel development and qualification.

11 - NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Estimation of post-burst vibration-induced fuel dispersal thresholds following LOCA-simulant testing

The nuclear industry intends to increase burnup past the regulatory limit of 62 GWd/MTU, and to be successful, the dispersal behavior of fragmented high-burnup fuel during loss-of-coolant accidents must be better understood. Part of this behavior is fuel fragmentation, relocation, and dispersal. This work reports on testing concerning the dispersal of fuel from rods following burst and pressure blowdown through the burst. The Fuel Relocation Induced by Accident Recovery (FRIAR) system was used to examine surrogate material and pre-burst cladding specimens to evaluate the effects of vibrational loading, mixture composition, and burst size on post-burst dispersal. Vibrational loading resulted in maximum dispersal around 15 Hz when the loading was performed with peak-to-peak oscillation amplitudes at 0.5 and 1 mm. Here, under this aggressive vibrational loading, dispersal was found to become significant as burst widths increased to approximately 5 mm and larger. However, below 4 mm widths, little material dispersed out of the opening, even at 1 mm amplitudes and for more dispersive mixtures (smaller average fragments). At and above 7 mm widths, dispersal was rapid for all mixtures. Finally, dispersal in the threshold region (4–5 mm wide bursts) strongly depended on the mixture. For mixtures with large fragments, dispersal was minimized to a few fragments, as the large fragments proved to be effective at minimizing dispersal. Conversely, mixtures with smaller fragments showed increased dispersal in this region.

Burst geometry↗

Computational Investigation of Fuel Dispersal Phenomena during Large-Break Loss of Coolant Accident in Light-Water Reactors

In the event of cladding rupture, which could occur in light water reactor fuel assemblies during a loss-of-coolant accident (LOCA), fuel particles, along with fission gases, can be expelled into the reactor core from the fractured fuel rod. This expulsion of fragmented fuel particles, referred as fuel dispersal, is the subject of investigation to evaluate the safety implications of increasing fuel burnup in light water reactors, with a specific focus on fuel fragmentation, relocation, and dispersal. Particle trajectories and the resulting mass distribution of the settled particles within the reactor pressure vessel can pose a long-term cooling challenge for the reactor core. The fuel dispersal phenomenon is significantly influenced by the ejection characteristics of the fuel fragments, as well as the size and shape of the cladding rupture and fuel rod depressurization history during LOCA transients. In this study, the transport of fuel particles within a scaled 5 × 5 lattice of a pressurized water reactor rod bundle geometry is modeled through a two-fluid Eulerian framework that treats the gas and solid phases as interpenetrating continua. The required boundary conditions are evaluated from the fuel performance code BISON in a postulated large-break LOCA scenario. The modeling framework considers solid fuel particles as granular matter, interacting with the gaseous dry steam phase and fission gases through the governing interfacial momentum and energy exchange between the gas and solid phases. The simulation results provide the volume fraction of the solids settled on the bottom surface of the fuel bundle, quantifying the deposition within the bundle geometry.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

DEMONSTRATION OF MULTI-PHYSICS EVALUATION OF FUEL ROD BURST PROBABILITY WITH BURNUP EXTENSION UNDER LBLOCA CONDITIONS

Extending the fuel discharge burnup level, e.g., from the current limit of rod averaged discharge burnup limit of 62 GWD/MT to a proposed new limit of 75 GWD/MT, can provide significant economic benefits to the current fleet of operating light water reactors (LWRs). It allows for longer operating cycles and improved resource utilization. The major economic gain of longer operating cycles is attributable to the increased capacity factor resulting from decreased refueling time as a fraction of total operating time, as well as fewer assemblies to be discharged for a given amount of energy produced. The main licensing challenges for higher burnup fuel are to ensure fuel rod safety under design basis accident conditions, especially under large-break loss-of-coolant accident (LBLOCA) and reactivity insertion accident (RIA). In this work, two-year cycle core design for a typical 4-loop pressurized water reactor (PWR) is performed with enrichment increased up to 6% and burnup extended to 75 GWD/MT. The fuel rod burst potential evaluations under large-break loss-of-coolant accident (LBLOCA) conditions are subsequently performed using the multi-physics best estimate plus uncertainty analysis framework LOTUS (LOCA Toolkit for the U.S. LWRs) and the preliminary results are presented.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗