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NASA NTRS2004

Sensitivity of Simulated Warm Rain Formation to Collision and Coalescence Efficiencies, Breakup, and Turbulence: Comparison of Two Bin-Resolved Numerical Models

Numerical models that resolve cloud particles into discrete mass size distributions on an Eulerian grid provide a uniquely powerful means of studying the closely coupled interaction of aerosols, cloud microphysics, and transport that determine cloud properties and evolution. However, such models require many experimentally derived paramaterizations in order to properly represent the complex interactions of droplets within turbulent flow. Many of these parameterizations remain poorly quantified, and the numerical methods of solving the equations for temporal evolution of the mass size distribution can also vary considerably in terms of efficiency and accuracy. In this work, we compare results from two size-resolved microphysics models that employ various widely-used parameterizations and numerical solution methods for several aspects of stochastic collection.

Fridlind, Ann↗

NASA NTRS1985

Convergence acceleration for a three-dimensional Euler/Navier-Stokes zonal approach

A fast diagonal algorithm is coupled with a zonal approach to solve the three-dimensional Euler/Navier-Stokes equations. Transonic viscous solutions are obtained on a 150,000 point mesh for a NACA 0012 wing. The new computational approach yields a speedup by as much as a factor of 40 over the standard Beam-Warming algorithm/zonal method originally coded. A three-order-of-magnitude drop in the L2-norm of the residual requires approximately 500 iterations, which takes about 45 min of CPU time on a Cray-XMP. The numerically computed solutions are in good agreement with experimental results. Effects on convergence rate owing to increasing the zonal boundary overlap regions, different stretching distributions in the viscous regions, and different CFL values are also explored.

Flores, J.↗

NASA NTRS1990

Implications of the IRAS data for galactic gamma ray astronomy and EGRET

Using the results of gamma-ray, millimeter wave and far surveys of the galaxy, logically consistent picture of the large scale distribution of galactic gas and cosmic rays was derived, tied to the overall processes of stellar birth and destruction on a galactic scale. Using the results of the IRAS far-infrared survey of te galaxy, the large scale radial distributions of galactic far-infrared emission independently was obtained for both the Northern and Southern Hemisphere sides of the Galaxy. The dominant feature in these distributions was found to be a broad peak coincident with the 5 kpc molecular gas cloud ring. Evidence was found for spiral arm features. Strong correlations are evident between the large scale galactic distributions of far-infrared emission, gamma-ray emission and total CO emission. There is particularly tight correlation between the distribution of warm molecular clouds and far-infrared emission on a galactic scale. The 5 kpc ring was evident in existing galactic gamma-ray data. The extent to which the more detailed spiral arm features are evident in the more resolved EGRET (Energetic Gamma-Ray Experimental Telescope) data will help to determine more precisely the propagation characteristics of cosmic rays.

Stecker, Floyd W.↗

NASA NTRS1992

Soil nitrogen cycling and nitrous oxide flux in a Rocky Mountain Douglas-fir forest - Effects of fertilization, irrigation and carbon addition

Nitrous oxide fluxes and soil nitrogen transformations were measured in experimentally-treated high elevation Douglas-fir forests in northwestern New Mexico. On an annual basis, forests that were fertilized with 200 kg N/ha emitted an average of 0.66 kg/ha of N2O-N, with highest fluxes occurring in July and August when soils were both warm and wet. Control, irrigated, and woodchip treated plots were not different from each other, and annual average fluxes ranged from 0.03 to 0.23 kg/ha. Fertilized soil mineralized 277 kg/ha per year in contrast to 18 kg/ha per year in control plots. Relative recovery of (N-15)H4-N applied to soil in laboratory incubations was principally in the form of NO3-N in the fertilized soils, while recovery was mostly in microbial biomass-N in the other treatments. Fertilization apparently added nitrogen that exceeded the heterotrophic microbial demand, resulting in higher rates of nitrate production and higher nitrous oxide fluxes. Global inputs of nitrogen into forests are not currently contributing significantly to the increasing concentrations of nitrous oxide in the atmosphere.

Matson, Pamela A.↗

NASA NTRS1980

Theoretical and experimental investigations of upper atmosphere dynamics

A brief overview of the significant contributions made to the understanding of the dynamics of the Earth's upper atmosphere is presented, including the addition of winds and diffusion to the semi-empirical Global Reference Atmospheric Model developed for the design phase of the Space Shuttle, reviews of turbulence in the lower thermosphere, the dynamics of the equatorial mesopause, stratospheric warming effects on mesopause level dynamics, and the relevance of these studies to the proposed Middle Atmosphere Program (1982-85). A chronological bibliography, with abstracts of all papers published, is also included.

Roper, R. G.↗

NASA NTRS1992

Soil nitrogen cycling and nitrous oxide flux in a Rocky Mountain Douglas-fir forest - Effects of fertilization, irrigation and carbon addition

Nitrous oxide fluxes and soil nitrogen transformations were measured in experimentally-treated high elevation Douglas-fir forests in northwestern New Mexico, USA. On an annual basis, forests that were fertilized with 200 kg N/ha emitted an average of 0.66 kg/ha of N2O-N, with highest fluxes occurring in July and August when soils were both warm and wet. Control, irrigated, and woodchip treated plots did not differ, and annual average fluxes ranged from 0.03 to 0.23 kg/ha. Annual net nitrogen mineralization and nitrate production were estimated in soil and forest floor using in situ incubations; fertilized soil mineralized 277 kg/ha/y in contrast to 18 kg/ha/y in control plots. Relative recovery of 15NH4-N applied to soil in laboratory incubations was principally in the form of NO3-N in the fertilized soils, while recovery was mostly in microbial biomass-N in the other treatments. Fertilization apparently added nitrogen that exceeded the heterotrophic microbial demand, resulting in higher rates of nitrate production and higher nitrous oxide fluxes. Despite the elevated nitrous oxide emission resulting from fertilization, we estimate that global inputs of nitrogen into forests are not currently contributing significantly to the increasing concentrations of nitrous oxide in the atmosphere.

Matson, Pamela A.↗

NASA NTRS2021

Aerosol Loading and Radiation Budget Perturbations in Densely Populated and Highly Polluted Indo-Gangetic Plain by COVID-19: Influences on Cloud Properties and Air Temperature

Aerosols emitted in densely populated and industrialized Indo-Gangetic Plain, one of the most polluted regions in the world, modulate regional climate, monsoon, and Himalayan glacier retreat. Thus, this region is important for understanding aerosol perturbations and their resulting impacts on atmospheric changes during COVID-19 lockdown period, a natural experimental condition created by the pandemic. By analyzing 5 years (2016–2020) data of aerosols and performing a radiative transfer calculation, we found that columnar and near-surface aerosol loadings decreased, leading to reductions in radiative cooling at the surface and top of the atmosphere and atmospheric warming during lockdown period. Further, satellite data analyses showed increases in cloud optical thickness and cloud-particle effective radius and decrease in lower tropospheric air temperature during lockdown period. These results indicate critical influences of COVID-19 lockdown on regional climate and water cycle over Indo-Gangetic Plain, emphasizing need for further studies from modeling perspectives.

P Khatri↗

NASA NTRS1985

An experimental data base for material selection and design of high-speed, high-pressure, oxygen turbomachinery

New technologies for space-based, reusable, throttleable, cryogenic, orbit transfer propulsion are being evaluated. A variable-thrust (200 to 3000 lbF), 2000 psi chamber pressure, LO2/LH2 engine has been selected to demonstrate the 20-hour, 500-restart life goal, and a specific impulse of 480 lbF-sec/lbM. The advanced design uses warm oxygen to power a fully integrated turbopump that delivers 4500 psi LO2. The selected engine cycle provides the following advantages over conventional expander cycle designs which use H2 to drive the LH2 and LO2 pumps; higher engine operating pressures and performance in a smaller envelope, lower turbine operating temperatures, elimination of interpropellant seals and purges, and an extended throttling range. The design approach and results of testing to characterize materials for use in high-pressure gaseous oxygen are discussed. Test methods include particle impact testing in a sonic-flow, hot GO2 streams and forced, high-speed friction rubbing testing. Materials are exposed to oxygen and nitrogen atmospheres at pressures of 100, 1000, and 3000 psi to identify separately the gas cooling effects from the metal oxidation effects at the rubbing surface. The selection of candidate design materials is based on an analytical parameter defined as the burn factor. Typical materials tested include carbon steel, stainless steel, nickel, copper, and monel alloys.

Schoenman, L.↗

NASA NTRS1988

Dynamics of exploding magma chambers: Implications for K-T volcanism and mass extinctions

Although it is well known that unconfined chemical explosives may yield pressures to several megabars on detonation in air, the explosive literature has yet to be accessed by some contributors to the volcanological literature who've indicated that pressures in excess of the overburden and/or tensile cannot be obtained. Idealized ballistic assessments of pressures internal to volcanoes yield pressures in the hundreds of kilobar range upon correction by addition of friction, etc. Previous assessments of exploding magma chamber pressure have been made from the characteristics of the Mt. St. Helens explosion. A variety of methods yield pressures of similar value: at least hundreds of kilobars. Such results are consistent with free energy requirements for quench supersaturation explosion, a process occurring in solidifying industrial melts. Several reviews of geochemical literature emphasize the carbon event at the Cretaceous-Tertiary (K-T) boundary as being an indicator of a massive dump of CO2 derived from the mantle and entering the atmosphere by extensive global volcanism. Oxygen isotope data indicates extreme warming at the end of the Cretaceous which is consistent with a greenhouse effect attending the CO2 event. Reaction rate equations for the quench supersaturation explosion mechanism indicated, are consistent with the rise in pressure to 30 kbar on solidification of magmatic melts, these pressures limited by the strength of the experimental apparatus.

Rice, A. R.↗

NASA NTRS1991

Computation of viscous blast wave flowfields

A method to determine unsteady solutions of the Navier-Stokes equations was developed and applied. The structural finite-volume, approximately factored implicit scheme uses Newton subiterations to obtain the spatially and temporally second-order accurate time history of the interaction of blast-waves with stationary targets. The inviscid flux is evaluated using MacCormack's modified Steger-Warming flux or Roe flux difference splittings with total variation diminishing limiters, while the viscous flux is computed using central differences. The use of implicit boundary conditions in conjunction with a telescoping in time and space method permitted solutions to this strongly unsteady class of problems. Comparisons of numerical, analytical, and experimental results were made in two and three dimensions. These comparisons revealed accurate wave speed resolution with nonoscillatory discontinuity capturing. The purpose of this effort was to address the three-dimensional, viscous blast-wave problem. Test cases were undertaken to reveal these methods' weaknesses in three regimes: (1) viscous-dominated flow; (2) complex unsteady flow; and (3) three-dimensional flow. Comparisons of these computations to analytic and experimental results provided initial validation of the resultant code. Addition details on the numerical method and on the validation can be found in the appendix. Presently, the code is capable of single zone computations with selection of any permutation of solid wall or flow-through boundaries.

Atwood, Christopher A.↗

NASA NTRSDate not supplied

Experimental and Theoretical Needs for the JWST Early Release Science Program on Radiative Feedback from Massive Stars (PDRs4ALL): III. A Quantum Chemistry Perspective

Massive stars disrupt their natal molecular cloud material by dissociating molecules, ionizing atoms and molecules, and heating the gas and dust. These processes drive the evolution of interstellar matter in our Galaxy and throughout the Universe from the era of vigorous star formation at z=1-3 to the present day. Much of this interaction occurs in Photo- Dissociation Regions (PDRs) where far-ultraviolet photons of these stars create a largely neutral, but warm region of gas and dust. PDR emission dominates the IR spectra of starforming galaxies and provides a unique tool to study the physical and chemical processes that are relevant for inter- and circumstellar media including diffuse clouds, molecular cloud and protoplanetary disk surfaces, and starburst galaxies. The ERS program ID1288 is dedicated to provide template data as well as data processing and analysis tools for PDRs. To this end, it will observe the Orion Bar, the proto-typical PDR situated in the nearby Orion Nebula, using NIRSpec IFU, MIRI IFU, and NIRCAM and MIRI imaging. These observations will, for the first time, spatially resolve and perform a tomography of the PDR, revealing the individual IR spectral signatures from the key zones and sub-regions within the ionized gas, the PDR, and the molecular cloud. Quantum chemistry can be used to determine molecular data such as ionization potentials, chemical reaction rates, electronic spectra, dissociation energies, channels, and branching ratios, etc. These are often used in synergy with experiment to take advantage of the strengths of each approach. An area of active research is modeling the infrared (IR) emission spectra produced by PAH molecules, including the effects of anharmonicity. This will be important in the interpretation of JWST data which will yield higher-resolution spectral data compared to Spitzer or ISO. Quantum chemistry methods can compute accurate anharmonic IR absorption spectra of PAH molecules up to about 25 C atoms, and the results have been benchmarked against high-resolution experimental spectra. These feed into a quantum Monte Carlo (QMC) approach to generate temperature-dependent anharmonic IR emission spectra and then used to generate fully anharmonic cascade emission IR spectra of PAH molecules -- the very type of spectra that JWST will observe. Work continues to extend these methods to larger PAH molecules. We will discuss the current state of this work, as well as

Timothy Lee↗

NASA NTRS1985

Computation of flow around a circular cylinder in a supercritical regime

Compressible flows around a circular cylinder in a supercritical regime at Mach number 0.3 have been calculated by using the Beam-Warming-Steger scheme based on the full Navier-Stokes equations with improved accuracy. The flow patterns are visualized extensively to observe the characteristics in this regime. The computations show that the flow at certain Reynolds numbers in a supercritical regime becomes rather steady and irregular with small drag coefficients. This may correspond to the experimental observations that the Strouhal number can not be measured clearly at a certain Reynolds number range in the supercritical regime.

Ishii, K.↗

NASA NTRS1994

The daytime course of total ozone content caused by cloud convection

Presented are the experimental data on the daytime course of the total O3 and SO2 content obtained by Brewer 044 spectrophotometer in the tropics (Thumba, India, 8.53 N, 76.87 W, March-May 1990) and at middle latitudes (Obninsk, Russia, 55.12 N, 36.6 W, May-October 1991) of the Northern Hemisphere. The analysis showed that under fine warm weather conditions without precipitation (air mass change and frontal passage were not observed during several days) in days with well-developed convective clouds (cloudless morning, convective clouds in the daytime, no clouds in the evening) there is a typical nearly symmetric (with respect to local noon) course of the total O3 (with the minimum at about local noon) and SO2 (with the maximum at about local noon) content. The minimum depth is about 2-5 percent of the average daytime values of the total ozone content. The synchronous measurements of pressure pulsations with microbarograph (they are the indicator of convective and turbulent motion development in the lower subcloud atmospheric layer) showed that during these days there is a nearly symmetric course of pressure pulsations with the maximum at about local noon.

Ishov, Alexander G.↗

NASA NTRS1989

Observation of organized structure in turbulent flow within and above a forest canopy

Data obtained with seven triaxial sonic anemometer/thermometers and three Lyman-alpha hygrometers at an experimental site in Ontario, Canada reveal the coherent occurrence of ramp patterns of temperature and humidity at several levels within and above the deciduous forest considered. The ramps appear most clearly in the middle and upper portion of the forest, and near the top of the forest they are composed of a weak ejecting motion transporting warm and/or moist air out of the forest, followed by strong sweeps of cool and/or dry air penetrating into the canopy. In the middle and upper parts of the canopy, the sweeps are found to conduct a large proportion of the overall transfer between the forest and the lower atmosphere, with a lesser contribution from ejections.

Gao, W.↗

NASA NTRS1988

Navier-Stokes simulation of transonic wing flow fields using a zonal grid approach

The transonic Navier-Stokes code was used to simulate flow fields about isolated wings for workshop wind-tunnel and free-air cases using the thin-layer Reynolds-averaged Navier-Stokes equations. An implicit finite-difference scheme based on a diagonal version of the Beam-Warming algorithm was used to integrate the governing equations. A zonal grid approach was used to allow efficient grid refinement near the wing surface. The flow field was sensitive to the turbulent transition model, and flow unsteadiness was observed for a wind-tunnel case but not for the corresponding free-air case. The specification of experimental pressure at the wind-tunnel exit plane is the primary reason for the difference of these two numerical solutions.

Chaderjian, Neal M.↗

NASA NTRS1988

Navier-Stokes simulation of transonic wing flow fields using a zonal grid approach

Chaderjian, Neal M.↗

NASA NTRS2009

The Effect of Electrolyte Additives upon the Lithium Kinetics of Li-Ion Cells Containing MCMB and LiNi(x)Co(1-x)O2 Electrodes and Exposed to High Temperatures

With the intent of improving the performance of lithium-ion cells at high temperatures, we have investigated the use of a number of electrolyte additives in experimental MCMB- Li(x)Ni(y)Co(1-y)O2 cells, which were exposed to temperatures as high as 80 C. In the present work, we have evaluated the use of a number of additives, namely vinylene carbonate (VC), dimethyl acetamide (DMAc), and mono-fluoroethylene carbonate (FEC), in an electrolyte solution anticipated to perform well at warm temperature (i.e., 1.0M LiPF6 in EC+EMC (50:50 v/v %). In addition, we have explored the use of novel electrolyte additives, namely lithium oxalate and lithium tetraborate. In addition to determining the capacity and power losses at various temperatures sustained as a result of high temperature cycling (cycling performed at 60 and 80 C), the three-electrode MCMB-Li(x)Ni(y)Co(1-y)O2 cells (lithium reference) enabled us to study the impact of high temperature storage upon the solid electrolyte interphase (SEI) film characteristics on carbon anodes (MCMB-based materials), metal oxide cathodes, and the subsequent impact upon electrode kinetics.

High Temperture Resilience↗

NASA NTRS2013

Experimental Evidence for Weathering and Martian Sulfate Formation Under Extremely Cold Weather-Limited Environments

High resolution photography and spectroscopy of the martian surface (MOC, HiRISE) from orbit has revolutionized our view of Mars with one of the most important discoveries being wide-spread layered sedimentary deposits associated with sulfate minerals across the low to mid latitude regions of Mars [1, 2]. The mechanism for sulfate formation on Mars has been frequently attributed to playa-like evaporative environments under prolonged warm conditions [3]. However, there are several problems with the presence of prolonged surface temperatures on Mars above 273 K during the Noachian including the faint young Sun [4] and the presence of suitable greenhouse gases [5]. The geomorphic evidence for early warm conditions may instead be explained by periodic episodes of warming rather than long term prolonged warm temperatures [6]. An alternate view of the ancient martian climate contends that prolonged warm temperatures were never present and that the atmosphere and climate has been similar to modern conditions throughout most of its history [6]. This view is more consistent with the climate models, but has had a difficult time explaining the sedimentary history of Mars and in particular the presence of sulfate minerals. We suggest here that mixtures of atmospheric aerosols, ice, and dust have the potential for creating small films of cryo-concentrated acidic solutions that may represent an important unexamined environment for understanding weathering processes on Mars [7, 8]. This study seeks to test whether sulfate formation may be possible at temperatures well below 0 C in water limited environments removing the need for prolonged warm periods to form sulfates on early Mars.

Niles, Paul B.↗