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All sourcesNASA NTRSDOE OSTI
NASA NTRS1985

Seasonal simulations of the planetary boundary layer and boundary-layer stratocumulus clouds with a general circulation model

The formulation of the planetary boundary layer (PBL) and stratocumulus parametrizations in the UCLA general circulation model (GCM) are briefly summarized, and extensive new results are presented illustrating some aspects of the simulated seasonal changes of the global distributions of PBL depth, stratocumulus cloudiness, cloud-top entrainment instability, the cumulus mass flux, and related fields. Results from three experiments designed to reveal the sensitivity of the GCM results to aspects of the PBL and stratocumulus parametrizations are presented. The GCM results show that the layer cloud instability appears to limit the extent of the marine subtropical stratocumulus regimes, and that instability frequently occurs in association with cumulus convection over land. Cumulus convection acts as a very significant sink of PBL mass throughout the tropics and over the midlatitude continents in winter.

Randall, D. A.↗
NASA NTRS2015

Remote Sensing Measurements of the CO2 Mixing Ratio in the Planetary Boundary Layer Using Cloud Slicing with Airborne Lidar

We have measured the CO2 volume mixing ratio (VMR) within the planetary boundary layer (PBL) using cloud slicing with an airborne pulsed integrated path differential absorption (IPDA) lidar from flight altitudes of up to 13 km. During a flight over Iowa in summer 2011, simultaneous measurement of the optical range and CO2 absorption to clouds and the ground were made using time-resolved detection of pulse echoes from each scattering surface.We determined the CO2 absorption in the PBL by differencing the two lidar-measured absorption line shapes, one to a broken shallow cumulus cloud layer located at the top of the PBL and the other to the ground. Solving for the CO2 VMR in the PBL and that of the free troposphere, we measured a ≈15 ppm (4%) drawdown in the PBL. Both CO2 VMRs were within ≈3 ppm of in situ CO2 profile measurements. We have also demonstrated cloud slicing using scatter from thin, diffuse cirrus clouds and cumulus clouds, which allowed solving for the CO2 VMR for three vertical layers. The technique and retrieval algorithm are applicable to a space-based lidar instrument as well as to lidar IPDA measurements of other trace gases. Thus, lidar cloud slicing also offers promise toward space-based remote sensing of vertical trace gas profiles in the atmosphere using a variety of clouds.

VMR↗
NASA NTRS2018

Radiative Heating Profiles over Ascension Island during the 2016 and 2017 Biomass Burning Seasons

Marine boundary layer clouds, including the transition from stratocumulus to cumulus, are poorly represented in numerical weather prediction and general circulation models. In many cases, the complex physical relationships between cloud morphology and the environmental conditions in which marine boundary layer clouds exist are not well understood. Such uncertainties arise in the presence of biomass burning carbonaceous aerosol, as is the case over the southeast Atlantic Ocean, where it is likely that the absorbing and heating properties of these aerosols modify the microphysical composition and macrophysical arrangement of marine stratocumulus and trade cumulus. The deployment of the Atmospheric Radiation Measurement Mobile Facility #1 (AMF1) in support of LASIC (Layered Atlantic Smoke Interactions with Clouds) provided a unique opportunity to observe thermodynamic, cloud and aerosol properties during two consecutive biomass burning seasons from July through October of 2016 and 2017 over Ascension Island (7.96 S, 14.35 W). These observations in conjunction with radiation transfer modeling were used to assess the impact of biomass burning carbonaceous aerosol plumes as they passed over the site.Thermodynamic profiles were generated using a combination of radiosonde data and thermodynamic profilers to provide high temporal resolution profiles of quantities that are important for cloud development, such as CAPE and CIN. Coincident Ka-band radar and lidar profiles were used to characterize the cloud and sub-cloud structure. The resulting thermodynamic and cloud profiles are used as input forcing for the Rapid Radiative Transfer Model (RRTM) to compute radiative heating profiles over the observation site. Idealized experiments using RRTM, with and without aerosols present, are used to assess the impacts of the absorbing aerosol on the heating rate profiles.

Cumulus↗
NASA NTRS2020

Modeling the smoky troposphere of the southeast Atlantic: a comparison to ORACLES airborne observations from September of 2016

In the southeast Atlantic, well-defined smoke plumes from Africa advect over marine boundary layer cloud decks; both are most extensive around September, when most of the smoke resides in the free troposphere. A framework is put forth for evaluating the performance of a range of global and regional atmospheric composition models against observations made during the NASA ORACLES (ObseRvations of Aerosols above CLouds and their intEractionS) airborne mission in September 2016. A strength of the comparison is a focus on the spatial distribution of a wider range of aerosol composition and optical properties than has been done previously. The sparse airborne observations are aggregated into approximately 2° grid boxes and into three vertical layers: 3–6 km, the layer from cloud top to 3 km, and the cloud-topped marine boundary layer. Simulated aerosol extensive properties suggest that the flight-day observations are reasonably representative of the regional monthly average, with systematic deviations of 30 % or less. Evaluation against observations indicates that all models have strengths and weaknesses, and there is no single model that is superior to all the others in all metrics evaluated. Whereas all six models typically place the top of the smoke layer within 0–500 m of the airborne lidar observations, the models tend to place the smoke layer bottom 300–1400 m lower than the observations. A spatial pattern emerges, in which most models underestimate the mean of most smoke quantities (black carbon, extinction, carbon monoxide) on the diagonal corridor between 16° S, 6° E, and 10° S, 0° E, in the 3–6 km layer, and overestimate them further south, closer to the coast, where less aerosol is present. Model representations of the above-cloud aerosol optical depth differ more widely. Most models overestimate the organic aerosol mass concentrations relative to those of black carbon, and with less skill, indicating model uncertainties in secondary organic aerosol processes. Regional-mean free-tropospheric model ambient single scattering albedos vary widely, between 0.83 and 0.93 compared with in situ dry measurements centered at 0.86, despite minimal impact of humidification on particulate scattering. The modeled ratios of the particulate extinction to the sum of the black carbon and organic aerosol mass concentrations (a mass extinction efficiency proxy) are typically too low and vary too little spatially, with significant inter-model differences. Most models overestimate the carbonaceous mass within the offshore boundary layer. Overall, the diversity in the model biases suggests that different model processes are responsible. The wide range of model optical properties requires further scrutiny because of their importance for radiative effect estimates.

Yohei Shinozuka↗
DOE OSTI2022

Aircraft Observations of Turbulence in Cloudy and Cloud-Free Boundary Layers Over the Western North Atlantic Ocean From ACTIVATE and Implications for the Earth System Model Evaluation and Development

This study examines boundary layer turbulence derived from high temporal resolution meteorological measurements from 40 research flights over the western North Atlantic Ocean during the 2020 deployments of ACTIVATE. Frequency distributions of various turbulent quantities reveal stronger turbulence during the winter deployment than in summer and for cloud‐topped than in cloud‐free boundary layers during the summer deployment. Maximum turbulence kinetic energy (TKE) is most often within cloud from observations in winter and summer, whereas it is mostly below cloud in both seasons by a global model turbulence parameterization. Further, bivariate frequency distributions are consistent with the bivariate Gaussian probability distribution functions assumed for the closure of higher‐order turbulence/shallow convection parameterizations used by some global models. Turbulence simulated by the Community Atmosphere Model version 6 and the Energy Exascale Earth System Model Atmosphere Model version 2 using such parameterizations is not as strong as observed, with more TKE going into vertical wind perturbations rather than into zonal wind perturbations as observed, suggesting that the treatment of turbulence in Earth system models still needs to be further improved.

54 ENVIRONMENTAL SCIENCES↗
NASA NTRS1998

Design, Evaluation and GCM-Performance of a New Parameterization for Microphysics of Clouds with Relaxed Arakawa-Schubert Scheme (McRas)

A prognostic cloud scheme named McRAS (Microphysics of clouds with Relaxed Arakawa-Schubert Scheme) was developed with the aim of improving cloud-microphysics, and cloud-radiation interactions in GCMs. McRAS distinguishes convective, stratiform, and boundary-layer clouds. The convective clouds merge into stratiform clouds on an hourly time-scale, while the boundary-layer clouds do so instantly. The cloud condensate transforms into precipitation following the auto-conversion relations of Sundqvist that contain a parametric adaptation for the Bergeron-Findeisen process of ice crystal growth and collection of cloud condensate by precipitation. All clouds convect, advect, and diffuse both horizontally and vertically with a fully active cloud-microphysics throughout its life-cycle, while the optical properties of clouds are derived from the statistical distribution of hydrometeors and idealized cloud geometry. An evaluation of McRAS in a single column model (SCM) with the GATE Phase III data has shown that McRAS can simulate the observed temperature, humidity, and precipitation without discernible systematic errors. An evaluation with the ARM-CART SCM data in a cloud model intercomparison exercise shows reasonable but not an outstanding accurate simulation. Such a discrepancy is common to almost all models and is related, in part, to the input data quality. McRAS was implemented in the GEOS II GCM. A 50 month integration that was initialized with the ECMWF analysis of observations for January 1, 1987 and forced with the observed sea-surface temperatures and sea-ice distribution and vegetation properties (biomes, and soils), with prognostic soil moisture, snow-cover, and hydrology showed a very realistic simulation of cloud process, incloud water and ice, and cloud-radiative forcing (CRF). The simulated ITCZ showed a realistic time-mean structure and seasonal cycle, while the simulated CRF showed sensitivity to vertical distribution of cloud water which can be easily altered by the choice of time constant and incloud critical cloud water amount regulators for auto-conversion. The CRF and its feedbacks also have a profound effect on the ITCZ. Even though somewhat weaker than observed, the McRAS-GCM simulation produces robust 30-60 day oscillations in the 200 hPa velocity potential. Two ensembles of 4-summer (July, August, September) simulations, one each for 1987 and 1988 show that the McRAS-GCM simulates realistic and statistically significant precipitation differences over India, Central America, and tropical Africa. Several seasonal simulations were performed with McRAS-GEOS II GCM for the summer (June-July- August) and winter (December-January-February) periods to determine how the simulated clouds and CRFs would be affected by: i) advection of clouds; ii) cloud top entrainment instability, iii) cloud water inhomogeneity correction, and (iv) cloud production and dissipation in different cloud-processes. The results show that each of these processes contributes to the simulated cloud-fraction and CRF.

Sud, Y. C.↗
NASA NTRS1988

Coupling of the radiative, convective, and surface fluxes over the equatorial Pacific

An idealized energy-balance model for a closed tropical circulation is first presented to illustrate the coupling between the net tropospheric cooling, the surface fluxes, and the mean subsidence away from the precipitation zones. Then a one-dimensional diagnostic model and a radiation model with boundary layer clouds are combined to explore this coupling for a specific region, using mean sounding data over the tropical Pacific. The radiatively driven subsidence rate at the top of the convective boundary layer is approximately 35 mb/day and is largely independent of boundary layer cloud fraction. The sensitivity of the corresponding convective heat flux profiles to the mass divergence profile and cloud fraction within the boundary layer is explored. Reasonable assumptions give realistic surface sensible and latent heat fluxes for this region of approximately 10 and 130 W/sq m. The paper illustrates the important background climatic control of the radiation field on the tropical surface fluxes.

Ridgway, W.↗
NASA NTRS1990

Stratus: An interactive steady state mixed layer model for personal computers

A steady-state, horizontally homogeneous, cloud-topped marine boundary layer model based primarily on the work of Lilly (1968) and Schubert et al., (1979) is presented. The conservative thermodynamic variables are equivalent potential temperature, theta(sub e), and total water mixing ratio, q + l. Some of the differences between this and Lilly's (1968) model are: radiation is allowed to penetrate into the boundary layer; cloud top values of longwave radiation, equivalent potential temperature, and water vapor mixing ratio are linear functions of height derived from climatological data at California coastal stations; and the closure assumption assumes a weighted average of Lilly's (1968) maximum and minimum entrainment theories. This model was programmed in FORTRAN and will run interactively on an IBM-compatible personal computer. The program allows the user to specify the geographical location, the wind speed, the sea-surface temperature, the large scale horizontal divergence, and the initial guess for cloud top height. Output includes the steady state values of cloud top and cloud base height, mixed layer equivalent potential temperature and total water mixing ratio, and the associated convective and radiative fluxes.

Guinn, Thomas A.↗
DOE OSTI2026

Weak, shallow, dry convection over Angola increases offshore stratocumulus cloud droplet number concentrations

Boundary-layer cloud interactions involving shortwave-absorbing aerosols remain one of the least understood aerosol influences on climate. Here, we find the highest stratocumulus cloud droplet number concentrations over the southeast Atlantic occur when agricultural fires coincide with synoptically-weakened surface warming over Angola, occurring June-early August. Dry convection fills a shallow continental boundary layer with smoke, and a nighttime (local solar time 2-9) land breeze transports the aerosol into the marine boundary layer. Offshore aerosol transport is strengthened by low-level easterlies from a continental pressure high southeast of Angola. Simultaneously, the South Atlantic subtropical high is weaker, allowing extensive dispersal of aerosol offshore into the boundary layer, obscuring cloud brightening from shipping. Meteorological co-variation at synoptic scales compensates for cloud brightening by the smoke. Outgoing shortwave radiation increases by 15–20% of the monthly mean in June and July when offshore droplet numbers are less but the stratocumulus deck is more developed.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2025

Identifying synoptic controls on boundary layer thermodynamic and cloud properties in a regional forecast model

Although most of our understanding of boundary layer cloudiness is based on idealized, subtropical, barotropic marine environments, boundary layer clouds exist across a range of conditions. In this study, we use the Naval Research Laboratory's Coupled Ocean/Atmosphere Mesoscale Prediction System (COAMPS) and an automated cold-front-relative analysis framework to explore the boundary layer structure associated with low clouds across a transect through the cold front of a midlatitude synoptic cyclone. The model credibly captures boundary layer structure in line with conceptual models of midlatitude cyclones and ground-based observations at Graciosa Island in the Azores. The warm sector is conditionally unstable, with clouds that are too shallow and with too little liquid water, compared to cloud property retrievals from satellite and surface-based instruments. The cold-frontal region exhibits convection associated with weak stability and ascent. Northwest of the cold front, the boundary layer is well mixed, deeper, and capped by a strong inversion maintained by large-scale subsidence. Simulated clouds in frontal and post-frontal regions are mostly too thick, with too much liquid water and too little cloud base drizzle. The post-frontal clouds are associated with grid-scale updrafts, which appear to be the model's attempt to represent mesoscale organization of cellular convection typically observed in the cold sector of midlatitude cyclones. The deep, well-mixed post-frontal boundary layers and cloudiness are maintained by strong surface fluxes, as in cold air outbreaks. Our analysis framework serves as a unique approach to model verification, and our results offer insights into differences in boundary layer cloud behavior between subtropical and synoptic cold-sector regimes.

Eissner, Jordan M. [Univ. of Kansas, Lawrence, KS ↗
NASA NTRS2018

Characterizing Differences in the Aerosol Plume and Cloud Structure over Ascension Island During the 2016 and 2017 Biomass Burning Seasons

Marine boundary layer clouds, including the transition from stratocumulus to cumulus, are poorly represented in numerical weather prediction and general circulation models. In many cases, the complex physical relationships between marine boundary cloud morphology and the environmental conditions in which the clouds exist are not well understood. Such uncertainties arise in the presence of biomass burning carbonaceous aerosol, as is the case over the southeast Atlantic Ocean. It is likely that the absorbing and heating properties of these aerosols influence the microphysical composition and macrophysical arrangement of marine stratocumulus and trade cumulus in this region; however, this has yet to be quantified. The deployment of the Atmospheric Radiation Measurement Mobile Facility #1 (AMF1) in support of LASIC (Layered Atlantic Smoke Interactions with Clouds) provided a unique opportunity to collect observations of cloud and aerosol properties during two consecutive biomass burning seasons during July through October of 2016 and 2017 over Ascension Island (7.96 S, 14.35 W). Through the use of AMF1 observations, the Modern Era Retrospective Analysis for Research and Applications, version 2 (MERRA-2), and back trajectories from the Hybrid Single-Particle Lagrangian Integrated Trajectory model (HYSPLIT), it will be demonstrated that differences in the atmospheric circulation during the two years result in varying aerosol conditions over Ascension Island. When the aerosol plume is overhead, the aerosol loading is higher during the 2016 season as a result of a weaker subtropical high-pressure system. Furthermore, the aerosol plume originates from central Africa in 2016, but further south in 2017. Contrasts in the season-to-season and day-to-day aerosol loading are used to categorize boundary layer cloud and sub-cloud turbulence measurements above Ascension Island using the AMF1 Doppler lidar and cloud radar.

Collow, Allison B. Marquardt↗
NASA NTRS2023

A SmallSat Concept to Resolve Diurnal and Vertical Variations of Aerosols, Clouds, and Boundary Layer Height

A SmallSat mission concept is formulated here to carry out Time-varying Optical Measurements of Clouds and Aerosol Transport (TOMCAT) from space while embracing low-cost opportunities enabled by the revolution in Earth science observation technologies. TOMCAT’s “around-the-clock” measurements will provide needed insights and strong synergy with existing Earth observation satellites to 1) statistically resolve diurnal and vertical variation of cirrus cloud properties (key to Earth’s radiation budget), 2) determine the impacts of regional and seasonal planetary boundary layer (PBL) diurnal variation on surface air quality and low-level cloud distributions, and 3) characterize smoke and dust emission processes impacting their long-range transport on the subseasonal to seasonal time scales. Clouds, aerosol particles, and the PBL play critical roles in Earth’s climate system at multiple spatiotemporal scales. Yet their vertical variations as a function of local time are poorly measured from space. Active sensors for profiling the atmosphere typically utilize sun-synchronous low-Earth orbits (LEO) with rather limited temporal and spatial coverage, inhibiting the characterization of spatiotemporal variability. Pairing compact active lidar and passive multiangle remote sensing technologies from an inclined LEO platform enables measurements of the diurnal and vertical variability of aerosols, clouds, and aerosol-mixing-layer (or PBL) height in tropical-to-midlatitude regions where most of the world’s population resides. TOMCAT is conceived to bring potential societal benefits by delivering its data products in near–real time and offering on-demand hazard-monitoring capabilities to profile fire injection of smoke particles, the frontal lofting of dust particles, and the eruptive rise of volcanic plumes.

John E. Yorks↗
NASA NTRS1990

Cloud and boundary layer structure over San Nicolas Island during FIRE

The temporal evolution of the structure of the marine boundary layer and of the associated low-level clouds observed in the vicinity of the San Nicolas Island (SNI) is defined from data collected during the First ISCCP Regional Experiment (FIRE) Marine Stratocumulus Intense Field Observations (IFO) (July 1 to 19). Surface, radiosonde, and remote-sensing measurements are used for this analysis. Sounding from the Island and from the ship Point Sur, which was located approximately 100 km northwest of SNI, are used to define variations in the thermodynamic structure of the lower-troposphere on time scales of 12 hours and longer. Time-height sections of potential temperature and equivalent potential temperature clearly define large-scale variations in the height and the strength of the inversion and periods where the conditions for cloud-top entrainment instability (CTEI) are met. Well defined variations in the height and the strength of the inversion were associated with a Cataline Eddy that was present at various times during the experiment and with the passage of the remnants of a tropical cyclone on July 18. The large-scale variations in the mean thermodynamic structure at SNI correlate well with those observed from the Point Sur. Cloud characteristics are defined for 19 days of the experiment using data from a microwave radiometer, a cloud ceilometer, a sodar, and longwave and shortwave radiometers. The depth of the cloud layer is estimated by defining inversion heights from the sodar reflectivity and cloud-base heights from a laser ceilometer. The integrated liquid water obtained from NOAA's microwave radiometer is compared with the adiabatic liquid water content that is calculated by lifting a parcel adiabatically from cloud base. In addition, the cloud structure is characterized by the variability in cloud-base height and in the integrated liquid water.

Albrecht, Bruce A.↗
NASA NTRS2022

Analysis of the MODIS Above-Cloud Aerosol Retrieval Algorithm Using MCARS

The Multi-sensor Cloud and Aerosol Retrieval Simulator (MCARS) presently produces synthetic radiance data from Goddard Earth Observing System version 5 (GEOS-5) model output as if the Moderate Resolution Imaging Spectroradiometer (MODIS) was viewing a combination of atmospheric column inclusive of clouds, aerosols and a variety of gases and land/ocean surface at a specific location. In this paper we use MCARS to study the MODIS Above-Cloud AEROsol retrieval algorithm (MOD06ACAERO). MOD06ACAERO is presently a regional research algorithm able to retrieve aerosol optical thickness over clouds, in particular absorbing biomass burning aerosols overlying marine boundary layer clouds in the Southeastern Atlantic Ocean. The algorithm’s ability to provide aerosol information in cloudy conditions makes it a valuable source of information for modeling and climate studies n an area where current clear sky-only operational MODIS aerosol retrievals effectively have a data gap between the months of June and October. We use MCARS for a verification and closure study of the MOD06ACAERO algorithm. The purpose of this study is to develop a set of constraints a model developer might use during assimilation of MOD06ACAERO data. Our simulations indicate that the MOD06ACAERO algorithm performs well for marine boundary layer clouds in the SE Atlantic provided some specific screening rules are observed. For the present study, a combination of five simulated MODIS data granules was used for a dataset of 13.5 million samples with known input conditions. When pixel retrieval uncertainty was less than 30%, optical thickness of the underlying cloud layer was greater than 4 and scattering angle range within the cloud bow was excluded, MOD06ACAERO retrievals agreed with the underlying ground truth (GEOS-5 cloud and aerosol profiles used to generate the synthetic radiances) with a slope of 0.913, offset of 0.06, and RMSE=0.107. When only near-nadir pixels were considered (view zenith angle within +/-20 degrees) the agreement with source data further improved (0.977, 0.051 and 0.096 respectively). Algorithm closure was examined using a single case out of the five 38 used for verification. For closure, the MOD06ACAERO code was modified to use GEOS-5 temperature and moisture profiles as ancillary. Agreement of MOD06ACAERO retrievals with source data for the closure study had a slope of 0.996 with offset -0.007 and RMSE of 0.097 at pixel uncertainty level of less than 40%, illustrating the benefits of high-quality ancillary atmospheric data for such retrievals.

MODIS↗
NASA NTRS2003

Dynamic Turbulence Modelling in Large-eddy Simulations of the Cloud-topped Atmospheric Boundary Layer

The use of large eddy simulation, or LES, to study the atmospheric boundary layer dates back to the early 1970s when Deardor (1972) used a three-dimensional simulation to determine velocity and temperature scales in the convective boundary layer. In 1974 he applied LES to the problem of mixing layer entrainment (Deardor 1974) and in 1980 to the cloud-topped boundary layer (Deardor 1980b). Since that time the LES approach has been applied to atmospheric boundary layer problems by numerous authors. While LES has been shown to be relatively robust for simple cases such as a clear, convective boundary layer (Mason 1989), simulation of the cloud-topped boundary layer has proved more of a challenge. The combination of small length scales and anisotropic turbulence coupled with cloud microphysics and radiation effects places a heavy burden on the turbulence model, especially in the cloud-top region. Consequently, over the past few decades considerable effort has been devoted to developing turbulence models that are better able to parameterize these processes. Much of this work has involved taking parameterizations developed for neutral boundary layers and deriving corrections to account for buoyancy effects associated with the background stratification and local buoyancy sources due to radiative and latent heat transfer within the cloud (see Lilly 1962; Deardor 1980a; Mason 1989; MacVean & Mason 1990, for example). In this paper we hope to contribute to this effort by presenting a number of turbulence models in which the model coefficients are calculated dynamically during the simulation rather than being prescribed a priori.

Kirkpatrick, M. P.↗
DOE OSTI2023

Evaluation of four ground-based retrievals of cloud droplet number concentration in marine stratocumulus with aircraft in situ measurements

Abstract. Cloud droplet number concentration (Nd) is crucial for understanding aerosol–cloud interactions (ACI) and associated radiative effects. We present evaluations of four ground-based Nd retrievals based on comprehensive datasets from the Atmospheric Radiation Measurement (ARM) Aerosol and Cloud Experiments in the Eastern North Atlantic (ACE-ENA) field campaign. The Nd retrieval methods use ARM ENA observatory ground-based remote sensing observations from a micropulse lidar, Raman lidar, cloud radar, and the ARM NDROP (Droplet Number Concentration) value-added product (VAP), all of which also retrieve cloud effective radius (re). The retrievals are compared against aircraft measurements from the fast cloud droplet probe (FCDP) and the cloud and aerosol spectrometer (CAS) obtained from low-level marine boundary layer clouds on 12 flight days during summer and winter seasons. Additionally, the in situ measurements are used to validate the assumptions and characterizations used in the retrieval algorithms. Statistical comparisons of the probability distribution function (PDF) of the Nd and cloud re retrievals with aircraft measurements demonstrate that these retrievals align well with in situ measurements for overcast clouds, but they may substantially differ for broken clouds or clouds with low liquid water path (LWP). The retrievals are applied to 4 years of ground-based remote sensing measurements of overcast marine boundary layer clouds at the ARM ENA observatory to find that Nd (re) values exhibit seasonal variations, with higher (lower) values during the summer season and lower (higher) values during the winter season. The ensemble of various retrievals using different measurements and retrieval algorithms such as those in this paper can help to quantify Nd retrieval uncertainties and identify reliable Nd retrieval scenarios. Of the retrieval methods, we recommend using the micropulse lidar-based method. This method has good agreement with in situ measurements, less sensitivity to issues arising from precipitation and low cloud LWP and/or optical depth, and broad applicability by functioning for both daytime and nighttime conditions.

54 ENVIRONMENTAL SCIENCES↗