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At least 109 records · Page 6

Lean Premixed Combustion Stabilized by Low Swirl a Promising Concept for Practical Applications

Since its inception, the low-swirl burner (LSB) has shown to be a useful laboratory apparatus for fundamental studies of premixed turbulent flames. The LSB operates under wide ranges of equivalence ratios, flow rates, and turbulence intensities. Its flame is lifted and detached from the burner and allows easy access for laser diagnostics. The flame brush is axisymmetric and propagates normal to the incident reactants. Therefore, the LSB is well suited for investigating detailed flame structures and empirical coefficients such as flame speed, turbulence transport, and flame generated turbulence. Due to its capability to stabilize ultra-lean premixed turbulent flames (phi approx. = 0.55), the LSB has generated interest from the gas appliance industry for use as an economical low-NO(x) burner. Lean premixed combustion emits low levels of NO(x), due primarily to the low flame temperature. Therefore, it is a very effective NO(x) prevention method without involving selective catalytic reduction (SCR), fuel-air staging, or flue gas recirculation (FGR). En the gas turbine industry, substantial research efforts have already been undertaken and engines with lean premixed combustors are already in use. For commercial and residential applications, premixed pulsed combustors and premixed ceramic matrix burners are commercially available. These lean premixed combustion technologies, however, tend to be elaborate but have relatively limited operational flexibility, and higher capital, operating and maintenance costs. Consequently, these industries are continuing the development of lean premixed combustion technologies as well as exploring new concepts. This paper summarizes the research effects we have undertaken in the past few years to demonstrate the feasibility of applying the low-swirl flame stabilization method for a wide range of heating and power generation systems. The principle of flame stabilization by low-swirl is counter to the conventional high-swirl methods that rely on a recirculation zone to anchor the flame. In LSBS, flow recirculation is not promoted to allow the premixed turbulent flames to propagate freely. A LSB with an air-jet swirler is essentially an open tube with the swirler at its mid section. The small air-jets generate swirling motion only in the annular region and leaving the central core of the flow undisturbed, When this flow exits the burner tube, the angular momentum generates radial mean pressure gradient to diverge the non-swirling reactants stream. Consequently, the mean flow velocity decreases linearly. Propagating against this decelerating flow, the flame self-sustains at the position where the local flow velocity equals the flame speed, S(sub f). The LSB operates with a swirl number, S, between 0.02 to 0.1. This is much lower than the minimum S of 0.6 required for the high-swirl burners. We found that the swirl number needed for flame stabilization varies only slightly with fuel type, flow velocity, turbulent conditions and burner dimensions (i.e. throat diameter and swirl injection angle).

Cheng, R. K.↗

Large-Scale Flow Structure in Turbulent Nonpremixed Flames under Normal- And Low-Gravity Conditions

It is well known that buoyancy has a major influence on the flow structure of turbulent nonpremixed jet flames. Buoyancy acts by inducing baroclinic torques, which generate large-scale vortical structures that can significantly modify the flow field. Furthermore, some suggest that buoyancy can substantially influence the large-scale structure of even nominally momentum-dominated flames, since the low velocity flow outside of the flame will be more susceptible to buoyancy effects. Even subtle buoyancy effects may be important because changes in the large-scale structure affects the local entrainment and fluctuating strain rate, and hence the structure of the flame. Previous studies that have compared the structure of normal- and micro-gravity nonpremixed jet flames note that flames in microgravity are longer and wider than in normal-gravity. This trend was observed for jet flames ranging from laminar to turbulent regimes. Furthermore, imaging of the flames has shown possible evidence of helical instabilities and disturbances starting from the base of the flame in microgravity. In contrast, these characteristics were not observed in normal-gravity. The objective of the present study is to further advance our knowledge of the effects of weak levels of buoyancy on the structure of transitional and turbulent nonpremixed jet flames. In later studies we will utilize the drop tower facilities at NASA Glenn Research Center (GRC), but the preliminary work described in this paper was conducted using the 1.25-second drop tower located at the University of Texas at Austin. A more detailed description of these experiments can be found in Idicheria et al.

Clemens, N. T.↗

Buoyancy Effects in Strongly-pulsed, Turbulent Diffusion Flames

The objective of this experiment is to better understand the combustion behavior of pulsed, turbulent diffusion flames by conducting experiments in microgravity. The fuel jet is fully-modulated (i.e., completely shut off between pulses) by an externally controlled valve system leading to enhanced fuel/air mixing compared to acoustically excited or partially-modulated jets. Experiments are conducted both in laboratories at UW and WPI and in the GRC 2.2s Drop Tower. A single fuel nozzle with diameter d = 2 mm is centered in a combustor 20 x 20 cm in cross section and 67 cm in height. The gaseous fuel flow (ethylene or a 50/50 ethylene/nitrogen mixture by volume) is fully-modulated by a fast-response solenoid valve with injection times from tau = 4 to tau = 300 ms. The nominal Reynolds number based on the fuel velocity during injection, U(sub jet), is 5,000. A slow oxidizer co-flow properly ventilates the flame and an electrically heated wire loop serves as a continuous ignition source. Diagnostic techniques include video imaging, fine-wire thermocouples and thermopile radiometers, and gas sampling and standard emissions instruments (the last in the laboratory only).

Hermanson, J. C.↗

Buoyancy Effects in Strongly-Pulsed, Turbulent Diffusion Flames

The objective of this experiment is to better understand the combustion behavior of pulsed, turbulent diffusion flames by conducting experiments in microgravity. The fuel jet is fully-modulated (i.e., completely shut off between pulses) by an externally controlled valve system leading to enhanced fuel/air mixing compared to acoustically excited or partially-modulated jets. Experiments are conducted both in laboratories at UW and WPI and in the GRC 2.2s Drop Tower. A single fuel nozzle with diameter d = 2 mm is centered in a combustor 20 20 cm in cross section and 67 cm in height. The gaseous fuel flow (ethylene or a 50/50 ethylene/nitrogen mixture by volume) is fully-modulated by a fast-response solenoid valve with injection times from tau = 4 to tau = 300 ms. The nominal Reynolds number based on the fuel velocity during injection, U(sub jet), is 5,000. A slow oxidizer co-flow properly ventilates the flame and an electrically heated wire loop serves as a continuous ignition source. Diagnostic techniques include video imaging, fine-wire thermocouples and thermopile radiometers, and gas sampling and standard emissions instruments (the last in the laboratory only).

Hermanson, J. C.↗

The effects of turbulence on the flame structure and NO formation of ammonia turbulent premixed combustion at various equivalence ratios

Ammonia is carbon-free and is regarded as a potential fuel to address global warming issues. Here, in this work, three-dimensional direct numerical simulations (DNS) of ammonia/air turbulent premixed flames were performed to explore the influence of turbulence and equivalence ratio on the flame structure and NO formation characteristics. Two equivalence ratios were considered, i.e. Φ=0.9 and Φ=1.1. The general flame structures were presented and species distributions were examined. The NO mass fraction was found to be the highest in the product for the lean case and in the reaction zone for the rich case. The conditional mean values of species mass fractions and reaction rates were compared with those of the unstrained and strained laminar premixed flames to explore how well the laminar flame structures can approach those of the turbulent flame. The budget analysis of the species transport equations showed that turbulent diffusion plays an important role in species transport. The turbulent diffusivity D T was estimated using the gradient hypothesis based on the DNS data. Various laminar flame simulations with different diffusivities were carried out. It was shown that the conditional means of the DNS agree well with those of the laminar flames including D T in the transport property calculation. The global and local NO formation characteristics were investigated. It was found that the mean NO production conditioned on the progress variable is lower compared with the corresponding laminar flame in the rich case. However, the relative contributions from various NO pathways are rarely affected by turbulence. The NO mass fraction is higher in negative curvature regions compared with positive curvature regions of the flame surface for the rich case, which is due to the preferential diffusion of H 2 and other radicals and the enhanced NO pathways in negatively curved regions.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Extinction and Scattering Properties of Soot Emitted from Buoyant Turbulent Diffusion Flames

Extinction and scattering properties at wavelengths of 250-5200 nm were studied for soot emitted from buoyant turbulent diffusion flames in the long residence time regime where soot properties are independent of position in the overfire region and characteristic flame residence times. Flames burning in still air and fueled with gas (acetylene, ethylene, propane, and propylene) and liquid (benzene, toluene, cyclohexane, and n-heptane) hydrocarbon fuels were considered Measured scattering patterns and ratios of total scattering/absorption cross sections were in good agreement with predictions based on the Rayleigh-Debye-Gans (RDG) scattering approximation in the visible. Measured depolarization ratios were roughly correlated by primary particle size parameter, suggesting potential for completing RDG methodology needed to make soot scattering predictions as well as providing a nonintrusive way to measure primary soot particle diameters. Measurements of dimensionless extinction coefficients were in good agreement with earlier measurements for similar soot populations and were independent of fuel type and wavelength except for reduced values as the near ultraviolet was approached. The ratios of the scattering/absorption refractive index functions were independent of fuel type within experimental uncertainties and were in good agreement with earlier measurements. The refractive index function for absorption was similarly independent of fuel type but was larger than earlier reflectometry measurements in the infrared. Ratios of total scattering/absorption cross sections were relatively large in the visible and near infrared, with maximum values as large as 0.9 and with values as large as 0.2 at 2000 nm, suggesting greater potential for scattering from soot particles to affect flame radiation properties than previously thought.

Krishnan, S. S.↗

Extinction and Scattering Properties of Soot Emitted from Buoyant Turbulent Diffusion Flames

Extinction and scattering properties at wavelengths of 250-5200 nm were studied for soot emitted from buoyant turbulent diffusion flames in the long residence time regime where soot properties are independent of position in the overfire region and characteristic flame residence times. Flames burning in still air and fueled with gas (acetylene, ethylene, propane, and propylene) and liquid (benzene, toluene, cyclohexane, and n-heptane) hydrocarbon fuels were considered. Measured scattering patterns and ratios of total scattering/absorption cross sections were in good agreement with predictions based on the Rayleigh-Debye-Gans (RDG) scattering approximation in the visible. Measured depolarization ratios were roughly correlated by primary particle size parameter, suggesting potential for completing RDG methodology needed to make soot scattering predictions as well as providing a nonintrusive way to measure primary soot particle diameters. Measurements of dimensionless extinction coefficients were in good agreement with earlier measurements for similar soot populations and were independent of fuel type and wavelength except for reduced values as the near ultraviolet was approached. The ratios of the scattering/absorption refractive index functions were independent of fuel type within experimental uncertainties and were in good agreement with earlier measurements. The refractive index junction for absorption was similarly independent of fuel type but was larger than earlier reflectometry measurements in the infrared. Ratios of total scattering/absorption cross sections were relatively large in the visible and near infrared, with maximum values as large as 0.9 and with values as large as 0.2 at 2000 nm, suggesting greater potential for scattering from soot particles to affect flame radiation properties than previously thought.

Krishnan, S. S.↗

Acoustic diagnostics of the nonpremixed turbulent jet flame

The feasibility of inferring information regarding turbulence and combustion details in turbulent combustion zones through the acoustic field is explored. The well known theoretical formulation of Strahle is used. The real difficulty in prediction of the acoustic field is seen to be the unavailability of an expression for the local, instantaneous reaction rate in a turbulent field. A simplified expression is used to infer the nature of the acoustic field. Based on earlier photographic observations, a model is used as a working hypothesis to extract information regarding the acoustic field. These are seen to be substantiated by experiments as well. More importantly, it is found that changes in the operating conditions of various burners are almost instantly revealed in the acoustic spectra. Several experiments with a laboratory burner using several different gaseous reactants are reported to support this diagnostic information content of the acoustic fields of turbulent combustion zones.

Ramohalli, K.↗

An analysis of turbulent diffusion flame in axisymmetric jet

The kinetic theory of turbulent flow was employed to study the mixing limited combustion of hydrogen in axisymmetric jets. The integro-differential equations in two spatial and three velocity coordinates describing the combustion were reduced to a set of hyperbolic partial differential equations in the two spatial coordinates by a binodal approximation. The MacCormick's finite difference method was then employed for solution. The flame length was longer than that predicted by the flame-sheet analysis, and was found to be in general agreement with a recent experimental result. Increase of the turbulence energy and scale resulted in an enhancement of the combustion rate and, hence, in a shorter flame length. Details of the numerical method as well as of the physical findings are discussed.

Chung, P. M.↗

Segregation parameters and pair-exchange mixing models for turbulent nonpremixed flames

The progress of chemical reactions in nonpremixed turbulent flows depends on the coexistence of reactants, which are brought together by mixing. The degree of mixing can strongly influence the chemical reactions and it can be quantified by segregation parameters. In this paper, the relevance of segregation parameters to turbulent mixing and chemical reactions is explored. An analysis of the pair-exchange mixing models is performed and an explanation is given for the peculiar behavior of such models in homogeneous turbulence. The nature of segregation parameters in a H2/Ar-air nonpremixed jet flame is investigated. The results show that Monte Carlo simulation with the modified Curl's mixing model predicts segregation parameters in close agreement with the experimental values, providing an indirect validation for the theoretical model.

Chen, J.-Y.↗

Study of Turbulent Premixed Flame Propagation using a Laminar Flamelet Model

The laminar flamelet concept in turbulent reacting flows is considered applicable to many practical combustion systems (Linan & Williams 1993). For turbulent premixed combustion, the laminar flamelet regime is valid when turbulent Karlovitz number is less than unity, which is equivalent to stating that the characteristic thickness of the flame is less than that of a Kolmogorov eddy; this is known as the Klimov-Williams criterion (Williams 1985). In such a case, the flame maintains its laminar structure, and the effect of turbulent flow is merely to wrinkle and strain the flame front. The propagating wrinkled premixed flame can then be described as an infinitesimally thin surface dividing the unburnt fresh mixture and the burnt product.

Im, H. G.↗

Effects of gravity on sheared and nonsheared turbulent nonpremixed flames

The present numerical study is concerned with the fundamental physics of the multiway interaction between turbulence, chemical reaction, and buoyancy in a nonpremixed flame. The method of direct numerical simulation (DNS) is used to solve the instantaneous, three-dimensional governing equations. Because of the present supercomputer limitations, we consider two simple flow geometries, namely an initially uniform flow without shear (equivalent to grid-generated turbulence) and an initially uniform shear flow. In each flow, the fuel and oxidant initially exist as two separate streams. As the reactants mix, chemical reaction takes place and exothermic energy is released causing variations in density. In the presence of a gravity field, the spatial and temporal distributions of the induced buoyancy forces depend on the local density gradients and the direction of the gravitational acceleration. The effects of buoyancy include the generation of local shear, baroclinic production or destruction of vorticity, and countergradient heat and mass transport. Increased vorticity and small-scale turbulence promote further mixing and reaction. However, if the strain-rates become too high, local flame extinction can occur. Our objective is to gain an understanding of the complex interactions between the physical phenomena involved, with particular attention to the effects of buoyancy on the turbulence structure, flame behavior, and factors influencing flame extinction.

Elghobashi, Said↗

Direct numerical simulation of a turbulent methane/air flame impinged by a sub-breakdown electric field

Here, the effects of an external electric field on a turbulent methane/air diffusion flame are analyzed in this work using direct numerical simulations. The analyzed configuration consists of a temporally evolving mixing layer of air and a mixture of methane and nitrogen at 1 atm that is impinged by an electric field in the direction normal to the mean mixing plane. The combustion and chemi-ionization reactions involved in the flow are modeled using finite-rate chemistry and a reduced reaction scheme consisting of 26 species and 134 reactions. The mass diffusion and ion-wind effects are modeled using a detailed description of the diffusion coefficients and electric mobilities based on kinetic theory. The presented calculations show that the turbulence generated within the mixing layer is mostly unaffected by the applied electric field for the configuration under exam. In fact, the electric body force is developed away from the mixing region where the flow is uniform. Conversely, the turbulence is able to introduce very high intermittency in the electrically charged species concentration and, consequently, in the electric body force. Such intermittency will constitute a challenge in the future formulation of combustion models that take into account ion-wind effects.

09 BIOMASS FUELS↗

Measurements of superequilibrium hydroxyl concentrations in turbulent nonpremixed flames using saturated fluorescence

The first quantitative, time- and space-resolved measurements have been obtained for probability density functions of OH concentration in nonpremixed flames. Measurements using single-pulse, laser-saturated fluorescence in laminar, transitional, and turbulent nonpremixed H2-air flames provide unambiguous evidence for substantial OH superequilibrium concentrations, in qualitative agreement with predictions of laminar and turbulent combustion models. The average degree of superequilibrium, OH/OH(AE), is typically 4-5 near the jet exit and approaches unity far downstream. The maximum instantaneous OH concentration measured in transitional and turbulent H2-air flames is about 6 x 10 to the 16th molecules/cc, in accord with the maximum determined by partial equilibrium thermodynamic calculations and with the maximum OH concentrations measured in premixed H2-air flames.

Drake, M. C.↗

Comparison of spherical harmonics method and discrete ordinates method for radiative transfer in a turbulent jet flame

Here, in this study, we systematically compared the accuracy and computational cost of two popular solution methods for the radiative transfer equation (RTE): the spherical harmonics method (P N ) and the discrete ordinates method (DOM). We first investigated convergence characteristics of different orders of P N and DOM in a series of 1D homogeneous configurations with varying optical thicknesses. Both solvers perform better for optically thicker cases. The accuracy of P N methods increases with its order, , but the gain in accuracy reduces with the increase in , i.e., improvement of P 7 over P 5 is less than that of P 3 over P 1 . This decreasing trend becomes more prominent as the optical thickness decreases. On the other hand, DOM’s accuracy increases almost linearly with the increase in the number of ordinates (or polar angles in this study) in all cases. While comparing the directional profile of radiative intensity, both solvers perform better when the radiative intensity is more isotropic. These solvers were then connected with a full spectrum k-distribution (FSK) spectral model and used to perform radiation-coupled simulations of a turbulent jet flame in an axi-symmetric cylindrical domain. Results obtained from P 1 to P 7 approximations for P N , and 2 x 4, 4 x 4, 4 x 8, 8 x 8 finite angles for DOM are compared with that from an optically thin model, and a reference solution from line-by-line (LBL) photon Monte Carlo (PMC) method. The choice of radiation solver shows a noticeable impact on the temperature distribution of the flame. The P N solvers lead to slightly higher radiant fractions and the DOM solvers lead to slightly lower radiant fractions than the PMC benchmark solution. Finally, the computational costs of each of these solvers are also reported and an intermittent evaluation / time blending scheme to improve the computational efficiency of radiation solvers in radiation-coupled simulations are also demonstrated.

42 ENGINEERING↗

High-speed volumetric imaging of formaldehyde in a lifted turbulent jet flame using an acousto-optic deflector

The development of high-speed volumetric laser-induced fluorescence measurements of formaldehyde (CH 2 O-LIF) using a pulse-burst laser operated at a repetition rate of 100 kHz is presented here. A novel laser scanning system employing an acousto-optic deflector (AOD) enables quasi-4D CH 2 O-LIF imaging at a scan frequency of 10 kHz. The diagnostic capability of time-resolved volumetric imaging is demonstrated in a partially premixed DME/air lifted turbulent jet flame near the flame base. Simultaneous imaging of laser beam profiles is performed to account for the laser pulse energy fluctuation and laser sheet inhomogeneity. With the accurate registration of laser sheet positions, the volumetric reconstruction of CH 2 O-LIF signals is performed within a detection volume of 17.3 × 11.9 × 2.3 mm 3 with an average out-of-plane spatial resolution of 250μm. A surface detection algorithm with adaptive thresholding is used to determine the global maximum intensity gradient by calculating gradient percentiles. The flame topology characteristics are investigated by evaluating the 3D curvatures of CH 2 O surfaces. Curvatures calculated using 2D data systematically underestimate the full 3D curvature due to the lack of out-of-plane information. The inner surfaces near the turbulent fuel jet exhibit higher probabilities of large mean curvature than the outer surfaces. The saddle and cylindrical structures are dominant on both the inner and outer surfaces and the elliptic structures occur with lower probability. The results suggest that the damping of turbulent fluctuations by the temperature increase through the CH 2 O region reduces the curvature, but the local structure topology remains self-similar.

42 ENGINEERING↗