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At least 109 records · Page 6

Collisional Removal of OH (X (sup 2)Pi, nu=7) by O2, N2, CO2, and N2O

Collisional removal rate constants for the OH (X 2PI, nu = 7) radical are measured for the colliders O2, CO2, and N2O, and an upper limit is established for N2. OH(nu = 4) molecules, generated in a microwave discharge flow cell by the reaction of hydrogen atoms with ozone, are excited to v = 7 by the output of a pulsed infrared laser via direct vibrational overtone excitation. The temporal evolution of the P = 7 population is probed as a function of the collider gas partial pressure by a time-delayed pulsed ultraviolet laser. Fluorescence from the B 21 + state is detected in the visible spectral region.

Knutsen, Karen↗

The nu Andromedae System: Models and Stability

Radial velocity observations of the F8 V star nu Andromedae taken at Lick and at Whipple Observatories have revealed evidence of three periodicities in the line-of-sight velocity of the star. These periodicities have been interpreted as evidence for at least three low-mass companions (LMCs) revolving around nu Andromedae. The mass and orbital parameters inferred for these companions raise questions about the dynamical stability of the system. We report here results from our independent analysis of the published radial velocity data, as well as new unpublished data taken at Lick Observatory. Our results confirm the finding of three periods in the data. Our best fits to the data, on the assumption that these periods arise from the gravitational perturbations of companions in Keplerian orbits, are also generally in agreement but with some differences from the earlier findings. We find that the available data do not constrain well the orbital eccentricity of the middle companion in a three-companion model of the data. We also find that in order for our best-fit model to the Lick data to be dynamically stable over the lifetime of the star (approximately 2 billion years), the system must have a mean inclination to the plane of the sky greater than 13 deg. The corresponding minimum inclination for the best fit to the Whipple data set is 19 deg. These values imply that the maximum mass for the outer companion can be no greater than about 20 Jupiter masses. Our analysis of the stability of the putative systems also places constraints on the relative inclinations of the orbital planes of the companions. We comment on global versus local (i.e., method of steepest descent) means of finding best-fit orbits from radial velocity data sets.

Stepinski, Tomasz F.↗

Characterization of silicon-carbon clusters by infrared laser spectroscopy. The nu 1 band of SiC4

The nu 1 fundamental vibration of linear SiC4 has been observed by infrared diode laser spectroscopy of a supersonic cluster beam. Twenty-four rovibrational transitions were measured in the spectral region of 2094.6 to 2097.1 cm-1, the rotational temperature was 10 K. A combined least-squares fit of these transitions with previously reported microwave data yielded the following molecular constants: nu 1 = 2095.45806(37) cm-1, B" = 0.051161131(52) cm-1, and B' = 0.0509157(96) cm-1. These results are compared to vibrational spectroscopy measurements of SiC4 trapped in a solid Ar matrix and to ab initio calculations.

NASA Discipline Exobiology↗

Characterization of silicon-carbon clusters by infrared laser spectroscopy: the nu 3(sigma u) band of linear Si2C3

The nu 3(sigma u) fundamental vibration of 1 sigma g+ Si2C3 has been observed using a laser vaporization-supersonic cluster beam-diode laser spectrometer. Forty rovibrational transitions were measured in the range of 1965.8 to 1970.9 cm-1 with a rotational temperature of 10-15 K. A least-squares fit of these transitions yielded the following molecular constants: nu 3(sigma u)=1968.188 31(18) cm-1, B"=0.031 575 1(60) cm-1, and B'=0.031 437 4(57) cm-1. These results are in excellent agreement with recent Fourier transform infrared (FTIR) measurements of Si2C3 trapped in a solid Ar matrix [J. Chem. Phys. 100, 181(1994)] and with ab initio calculations [J. Chem. Phys. 100, 175 (1994)] which suggest cumulenic-like bonding for Si2C3, analogous to the isovalent C5 carbon cluster.

Non-NASA Center↗

Development of Lunar Highland REgolith Simulants, NU-LHT-1M,-2M

As part of a collaborative agreement between the U.S, Geological Survey (USGS) and NASA's Marshall Space Flight Center (MSFC) lunar highland simulants are being produced to support engineers and scientists in developing the technologies required to put a base on the moon by 2024. Two simulants have been produced to date: NU-LHT-1M and -2M (NASA/USGS-Lunar Highlands Type-l & 2 Medium-grained). Using starting material chiefly collected from the Stillwater Mine, Nye, MT, blending protocols were developed based on normative mineralogy calculated from average chemistry, for the Apollo 16 regolith. New technologies using a high temperature remotely coupled plasma melter were developed to generate both high quality and agglutinitic glasses that simulate the glassy components of the regolith. Detailed chemical, mineralogical and physical properties analysis of NU-LHT-1M indicate that it is overall a good surrogate for highlands lunar regolith (our new simulant LHT-2M has not be analyzed yet). The primary difference between 1M and 2M was the inclusion of trace mineralogy (phosphates and sulfide). Plans will also be presented on the future direction of the simulant project.

Stoeser, D. B.↗

Design and Impacts of Land-Biogenic-Atmosphere Coupling in the NASA-Unified WRF (NU-WRF) Modeling System

Land-Atmosphere coupling is typically designed and implemented independently for physical (e.g. water and energy) and chemical (e.g. biogenic emissions and surface depositions)-based models and applications. Differences in scale, data requirements, and physics thus limit the ability of Earth System models to be fully coupled in a consistent manner. In order for the physical-chemical-biological coupling to be complete, treatment of the land in terms of surface classification, condition, fluxes, and emissions must be considered simultaneously and coherently across all components. In this study, we investigate a coupling strategy for the NASA-Unified Weather Research and Forecasting (NU-WRF) model that incorporates the traditionally disparate fluxes of water and energy through NASA's LIS (Land Information System) and biogenic emissions through BEIS (Biogenic Emissions Inventory System) and MEGAN (Model of Emissions of Gases and Aerosols from Nature) into the atmosphere. In doing so, inconsistencies across model inputs and parameter data are resolved such that the emissions from a particular plant species are consistent with the heat and moisture fluxes calculated for that land cover type. In turn, the response of the atmospheric turbulence and mixing in the planetary boundary layer (PBL) acts on the identical surface type, fluxes, and emissions for each. In addition, the coupling of dust emission within the NU-WRF system is performed in order to ensure consistency and to maximize the benefit of high-resolution land representation in LIS. The impacts of those self-consistent components on' the simulation of atmospheric aerosols are then evaluated through the WRF-Chem-GOCART (Goddard Chemistry Aerosol Radiation and Transport) model. Overall, this ambitious project highlights the current difficulties and future potential of fully coupled. components. in Earth System models, and underscores the importance of the iLEAPS community in supporting improved knowledge of processes and innovative approaches for models and observations.

Tan, Qian↗

Air- and Self-Broadened Half Widths, Pressure-Induced Shifts, and Line Mixing in the Nu(sub 2) Band of (12)CH4

Lorentz self- and air-broadened half width and pressure-induced shift coefficients and their dependences on temperature have been measured from laboratory absorption spectra for nearly 130 transitions in the nu(sub 2) band of (12)CH4. In addition line mixing coefficients (using the relaxation matrix element formalism) for both self- and airbroadening were experimentally determined for the first time for a small number of transitions in this band. Accurate line positions and absolute line intensities were also determined. These parameters were obtained by analyzing high-resolution (approx. 0.003 to 0.01 per cm) laboratory spectra of high-purity natural CH4 and air-broadened CH4 recorded at temperatures between 226 and 297 K using the McMath-Pierce Fourier transform spectrometer (FTS) located at the National Solar Observatory on Kitt Peak, Arizona. A multispectrum nonlinear least squares technique was used to fit short (5-15 per cm) spectral intervals in 24-29 spectra simultaneously. Parameters were determined for nu(sub 2) transitions up to J" = 16. The variations of the measured broadening and shift parameters with the rotational quantum number index and tetrahedral symmetry species are examined. The present results are also compared with previous measurements available in the literature.

Smith, M. A. H.↗

High-Resolution NU-WRF Simulations of a Deep Convective-Precipitation System During MC3E: Comparisons Between Goddard Microphysics Schemes and Observations - Part 1

The Goddard microphysics scheme was recently improved by adding a 4th ice class (frozen dropshail). This new 4ICE scheme was implemented and tested in the Goddard Cumulus Ensemble model (GCE) for an intense continental squall line and a moderate,less-organized continental case. Simulated peak radar reflectivity profiles were improved both in intensity and shape for both cases as were the overall reflectivity probability distributions versus observations. In this study, the new Goddard 4ICE scheme is implemented into the regional-scale NASA Unified - Weather Research and Forecasting model (NU-WRF) and tested on an intense mesoscale convective system that occurred during the Midlatitude Continental Convective Clouds Experiment (MC3E). The NU42WRF simulated radar reflectivities, rainfall intensities, and vertical and horizontal structure using the new 4ICE scheme agree as well as or significantly better with observations than when using previous versions of the Goddard 3ICE (graupel or hail) schemes. In the 4ICE scheme, the bin microphysics-based rain evaporation correction produces more erect convective cores, while modification of the unrealistic collection of ice by dry hail produces narrow and intense cores, allowing more slow-falling snow to be transported rearward. Together with a revised snow size mapping, the 4ICE scheme produces a more horizontally stratified trailing stratiform region with a broad, more coherent light rain area. In addition, the NU-WRF 4ICE simulated radar reflectivity distributions are consistent with and generally superior to those using the GCE due to the less restrictive open lateral boundaries

Regional Scale Model↗

NU-WRF Development and Support at NASA GSFC

The NASA Unified WRF modeling system (NU-WRF) is an observation driven framework that combines WRF-ARW with Goddard developed radiation, microphysics, aerosols and land information system (LIS) packages. NU-WRF can be used for simulating aerosols and land use effects on a variety of weather events. This poster will present a description of the modeling system including updates and future plans.

Cruz, Carlos A.↗

Cold Season Performance of the NU-WRF Regional Climate Model in the Great Lakes Region

As Earth’s largest collection of freshwater, the Laurentian Great Lakes have enormous ecological and socio-economic value. Their basin has become a regional hotspot of climatic and limnological change, potentially threatening its vital natural resources. Consequentially, there is a need to assess the current state of climate models regarding their performance across the Great Lakes region and develop the next generation of high-resolution regional climate models to address complex limnological processes and lake-atmosphere interactions. In response to this need, the current paper focuses on the generation and analysis of a 20-member ensemble of 3-km National Aeronautics and Space Administration (NASA)-Unified Weather Research and Forecasting (NU-WRF) simulations for the 2014-2015 cold season. The study aims to identify the model’s strengths and weaknesses; optimal configuration for the region; and the impacts of different physics parameterizations, coupling to a 1D lake model, time-variant lake-surface temperatures, and spectral nudging. Several key biases are identified in the cold-season simulations for the Great Lakes region, including an atmospheric cold bias that is amplified by coupling to a 1D lake model but diminished by applying the Community Atmosphere Model radiation scheme and Morrison microphysics scheme; an excess precipitation bias; anomalously early initiation of fall lake turnover and subsequent cold lake bias; excessive and overly persistent lake ice cover; and insufficient evaporation over Lakes Superior and Huron. The research team is currently addressing these key limitations by coupling NU-WRF to a 3D lake model in support of the next generation of regional climate models for the critical Great Lakes Basin.

Michael Notaro↗

Measurement of $d^2 \sigma/d|\vec{q}|d E_{avail}$ and 2p2h contribution using charged current $\nu_\mu$ interactions in the NOvA Near Detector

This Thesis presents the analysis methods and measurement of the $d^2 \sigma/d|\vec{q}|d E_{avail}$-CC inclusive cross section that describes neutrino scattering in a predominantly hydrocarbon medium. Studies that are prerequisite for the analysis including, variable determinations, event selections, efficiency, purity determinations, and systematic uncertainty estimations, are summarized. Tests of the analysis are also detailed, and shown to reproduce the input distributions. The double-differential cross-section measurement provides the foundation for determination of the inclusive rate for the excess induced by 2p2h processes together with nuclear medium effects that are not described by the Fermi gas model. The methodology for the extraction of this rate, defined as the excess observed relative to the rate estimated for known single-nucleon interactions, is described in detail. The following new measurements are reported in this Thesis: (1) The $\nu_\mu-$CC inclusive double-differential cross section as a function of three-momentum transfer and available hadronic energy, for an average $E_\nu$ of 1.8 GeV, is obtained. The double-differential cross section value that obtains when the bin widths are taken to be the dimensions of the entire analysis domain, e.g. $0.2 \le |\vec{q}| \le 2.0 GeV/c$ and $0.0 \le E_{avail} \le 2.0$ GeV, is inclusive cross section is $(6.05 \pm 0.75)\times10^{-39}$ cm$^2$/GeV/GeV/$c$/nucleon. An event excess attributed to 2p2h-MEC processes is observed; most of the rate occurs in a contiguous phase space region $0.3 \le |\vec{q}| \le 1.0$ GeV$/c$ $0.0 \le E_{avail} \le 0.35$ GeV. This rate represents $12.0\pm 6.5\%$ of the observed CC inclusive cross section; its cross section ratio relative to CCQE scattering is estimated to be $44.3 \pm 23.9\%$.

Olson, Travis Grant↗

Nuclear Dependence of Charged Current Inclusive $\bar{\nu}_\mu -$A Cross Section Measurements at 6 GeV at MINERvA

The main advantage of the MINERvA detector is that it uses differently sized nuclear targets, in the same neutrino beam, allowing for a direct study of nuclear medium effects, with reduced flux and detector uncertainties. This thesis presents the first high statistics charged current antineutrino-nucleus inclusive two-dimensional cross section measurements using an antineutrino beam with $\langle E_{\bar\nu}\rangle\sim$ 6 GeV, on iron, lead, carbon and hydrocarbon targets, as a function of bjorken $x$ and four-momentum transfer squared $Q^2$, invariant mass $W$ and $Q^2$ and muon longitudinal and transverse momenta, $p_t$ and $p_z$. These nuclei of different sizes were utilized to measure the nuclear dependence of the cross section. The antineutrino interactions that were utilized for the analysis presented in this thesis, were having an antimuon in the final state with energy 2-20GeV and with an antimuon scattering angle less than $17^o$. This analysis represents one of the largest antineutrino datasets analyzed to date in the energy region of $\langle E_{\bar\nu} \rangle \sim$ 6 GeV. This direct evidence for the nuclear medium effects, can help benchmarking models, which can be used by future neutrino experiments like DUNE, by extrapolating these results to Argon target.

Gaur, Prameet Kumar↗

Single-Atom Metal Oxide Sites as Traps for Charge Separation in the Zirconium-Based Metal–Organic Framework NDC–NU-1000

Solvothermal deposition in metal–organic frameworks (MOFs) can be utilized to mount single-metal-atom catalytic species at chemically reactive sites on hexa-Zr(IV)-oxy(oxo,hydroxo,aqua) nodes in nanoscale crystallites of the MOF NDC-NU-1000 in a self-limiting fashion. Upon photoexcitation of the 1,3,6,8-tetrakis( p -benzoato)pyrene chromophores of the parent framework, charge transfer may occur between the chromophores and the installed heterometal sites. Extended X-ray absorption fine structure studies revealed the single-atom nature of the installed species. A combination of steady-state and ultrafast optical spectroscopy was utilized to uncover evidence of a charge-separated (CS) state arising in the metalated samples. The relevant dynamics were characterized with transient photoluminescence and femtosecond transient absorption spectroscopy. Here, we find that a titanium-oxy single atom site gives rise to the longest-lived CS species compared to cobalt and nickel in a similar arrangement. This study provides guidance in designing MOF-based catalytic systems for photocatalysis and solar-fuel production.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Semileptonic form factors for $$B\rightarrow D^*\ell \nu $$ at nonzero recoil from $$2+1$$-flavor lattice QCD: Fermilab Lattice and MILC Collaborations

Abstract We present the first unquenched lattice-QCD calculation of the form factors for the decay $$B\rightarrow D^*\ell \nu $$ B → D ∗ ℓ ν at nonzero recoil. Our analysis includes 15 MILC ensembles with $$N_f=2+1$$ N f = 2 + 1 flavors of asqtad sea quarks, with a strange quark mass close to its physical mass. The lattice spacings range from $$a\approx 0.15$$ a ≈ 0.15 fm down to 0.045 fm, while the ratio between the light- and the strange-quark masses ranges from 0.05 to 0.4. The valence b and c quarks are treated using the Wilson-clover action with the Fermilab interpretation, whereas the light sector employs asqtad staggered fermions. We extrapolate our results to the physical point in the continuum limit using rooted staggered heavy-light meson chiral perturbation theory. Then we apply a model-independent parametrization to extend the form factors to the full kinematic range. With this parametrization we perform a joint lattice-QCD/experiment fit using several experimental datasets to determine the CKM matrix element $$|V_{cb}|$$ | V cb | . We obtain $$\left| V_{cb}\right| = (38.40 \pm 0.68_{\text {th}} \pm 0.34_{\text {exp}} \pm 0.18_{\text {EM}})\times 10^{-3}$$ V cb = ( 38.40 ± 0 . 68 th ± 0 . 34 exp ± 0 . 18 EM ) × 10 - 3 . The first error is theoretical, the second comes from experiment and the last one includes electromagnetic and electroweak uncertainties, with an overall $$\chi ^2\text {/dof} = 126/84$$ χ 2 /dof = 126 / 84 , which illustrates the tensions between the experimental data sets, and between theory and experiment. This result is in agreement with previous exclusive determinations, but the tension with the inclusive determination remains. Finally, we integrate the differential decay rate obtained solely from lattice data to predict $$R(D^*) = 0.265 \pm 0.013$$ R ( D ∗ ) = 0.265 ± 0.013 , which confirms the current tension between theory and experiment.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

DIS physics at the EIC and LHeC and connections to the future LHC and $\nu$A programs

Deeply-inelastic scattering (DIS) stands to enter a golden age with the prospect of precision programs at the Electron-Ion Collider (EIC) and Large Hadron-electron Collider (LHeC). While these programs will be of considerable importance to resolving longstanding issues in (non)perturbative QCD as well as hadronic and nuclear structure, they will also have valuable implications for a wider range of physics at the Energy and Intensity Frontiers, including at the High-Luminosity LHC (HL-LHC) and future \nu A ν A facilities. In this plenary contribution, we highlight a number of salient examples of the potential HEP impact from the complementary EIC and LHeC programs drawn from their respective Yellow Report and Whitepaper. Interested readers are encouraged to consult the extensive studies and literature from which these examples are taken for more detail.

Hobbs, Timothy↗

First Measurement of Differential Charged Current Quasielastic–like $\nu_\mu$ -Argon Scattering Cross Sections with the MicroBooNE Detector

Current and future generation neutrino oscillation experiments aim towards a high-precision mea- surement of the oscillation parameters and that requires an unprecedented understanding of neutrino-nucleus scattering. Charged-current quasi-elastic (CCQE) scattering is the process in which the neutrino produces a charged lepton and removes a single intact nucleon from the nu- cleus without producing any additional particles. For existing and forthcoming accelerator–based neutrino experiments, CCQE interactions are either the dominant process or part of the signal.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Nu Tools: Exploring Practical Roles for Neutrinos in Nuclear Energy and Security

For decades, physicists have used neutrinos from nuclear reactors to advance basic science. These pursuits have inspired many ideas for application of neutrino detectors in nuclear energy and security. While developments in neutrino detectors are now making some of these ideas technically feasible, their value in the context of real needs and constraints has been unclear. This report seeks to help focus the picture of where neutrino technology may find practical roles in nuclear energy and security. This report is the final product of the Nu Tools study, commissioned in 2019 by the DOE National Nuclear Security Administration (NNSA) Office of Defense Nuclear Nonproliferation Research and Development (DNN R&D). The study was conducted over two years by a group of neutrino physicists and nuclear engineers. A central theme of the study and this report is that useful application of neutrinos will depend not only on advancing physics and technology but also on understanding the needs and constraints of potential end-users. The Study Approach emphasized broad end-user engagement. The major effort, undertaken from May to December 2020, was a series of engagements with the wider nuclear energy and security communities. Interviews with 41 experts revealed points of common understanding, which this report captures in three Cross-Cutting Findings, a Framework for Evaluating Utility, and seven Use Case Findings. The report concludes with two Recommendations. The findings and recommendations are summarized below. The respective ordering within each category does not represent a prioritization or implied value judgement.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗