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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 109 records · Page 6
All sourcesNASA NTRSDOE OSTI
NASA NTRS1994

Bias properties of extragalactic distance indicators. 3: Analysis of Tully-Fisher distances for the Mathewson-Ford-Buchhorn sample of 1355 galaxies

The observational selection bias properties of the large Mathewson-Ford-Buchhorn (MFB) sample of axies are demonstrated by showing that the apparent Hubble constant incorrectly increases outward when determined using Tully-Fisher (TF) photometric distances that are uncorreted for bias. It is further shown that the value of H(sub 0) so determined is also multivlaued at a given redshift when it is calculated by the TF method using galaxies with differenct line widths. The method of removing this unphysical contradiction is developed following the model of the bias set out in Paper II. The model developed further here shows that the appropriate TF magnitude of a galaxy that is drawn from a flux-limited catalog not only is a function of line width but, even in the most idealistic cases, requires a triple-entry correction depending on line width, apparent magnitude, and catalog limit. Using the distance-limited subset of the data, it is shown that the mean intrinsic dispersion of a bias-free TF relation is high. The dispersion depends on line width, decreasing from sigma(M) = 0.7 mag for galaxies with rotational velocities less than 100 km s(exp-1) to sigma(M) = 0.4 mag for galaxies with rotational velocities greater than 250 km s(exp-1). These dispersions are so large that the random errors of the bias-free TF distances are too gross to detect any peculiar motions of individual galaxies, but taken together the data show again the offset of 500 km s(exp-1) fond both by Dressler & Faber and by MFB for galaxies in the direction of the putative Great Attractor but described now in a different way. The maximum amplitude of the bulk streaming motion at the Local Group is approximately 500 km s(exp-1) but the perturbation dies out, approaching the Machian frame defined by the CMB at a distance of approximately 80 Mpc (v is approximately 4000 km s(exp -1)). This decay to zero perturbation at v is approximately 4000 km s(exp -1) argues against existing models with a single attraction at approximately 4500 km s(exp -1) (the Great Attactor model) pulling the local region. Rather, the cause of the perturbation appears to be the well-known clumpy mass distribution within 4000 km s(exp -1) in the busy directions of Hydra, Centaurus, Antila and Dorado, as postulated earlier (Tammann & Sandage 1985).

Federspiel, Martin↗
NASA NTRS1988

The turbulent interstellar medium and pressure-bounded molecular clouds

The existence of turbulence throughout the interstellar medium suggests that an appropriate value for the average pressure may be P/K larger than about 10,000. Negative-index polytropic models of interstellar clouds in equilibrium with an external medium at these pressures are predicted to have sizes, line widths, masses, and size-line width and size-density relations in good agreement with those observed and inferred for dark clouds. Thus these observed features of interstellar clouds do not require that they be completely self-gravitating or 'virialized' in the commonly used sense.

Maloney, Philip↗
NASA NTRS2016

The Lick AGN Monitoring Project 2011: Spectroscopic Campaign and Emission-line Light Curves

In the Spring of 2011 we carried out a 2.5 month reverberation mapping campaign using the 3 m Shane telescope at Lick Observatory, monitoring 15 low-redshift Seyfert 1 galaxies. This paper describes the observations, reductions and measurements, and data products from the spectroscopic campaign. The reduced spectra were fitted with a multicomponent model in order to isolate the contributions of various continuum and emission-line components. We present light curves of broad emission lines and the active galactic nucleus (AGN) continuum, and measurements of the broad Hβ line widths in mean and rms spectra. For the most highly variable AGNs we also measured broad H beta line widths and velocity centroids from the nightly spectra. In four AGNs exhibiting the highest variability amplitudes, we detect anticorrelations between broad H beta width and luminosity, demonstrating that the broad-line region "breathes" on short timescales of days to weeks in response to continuum variations. We also find that broad H beta velocity centroids can undergo substantial changes in response to continuum variations; in NGC 4593, the broad H beta velocity shifted by approximately 250 km s(exp -1) over a 1 month period. This reverberation-induced velocity shift effect is likely to contribute a significant source of confusion noise to binary black hole searches that use multi-epoch quasar spectroscopy to detect binary orbital motion. We also present results from simulations that examine biases that can occur in measurement of broad-line widths from rms spectra due to the contributions of continuum variations and photon-counting noise.

galaxies: Seyfert↗
NASA NTRS2001

Calculated Half-widths and Line Shifts of Water Vapor Transitions in the 0.7- Micron Region and a Comparison with Published Data

Pressure-broadened half-widths and pressure-induced line shifts for the two most important bands of water vapor in the 0.7-micron region are determined using the complex Robert-Bonamy (CRB) formalism. The calculations are made with nitrogen and oxygen as the perturbing gas from which values for air as the perturbing gas are determined. The intermolecular potential is taken as a sum of electrostatic contributions and Lennard-Jones (6-12) atom-atom, and isotropic induction and dispersion components. The dynamics of the collision process are correct to second order in time. The calculated values are compared with published measurements and agreement is observed for both half-widths and line shifts. The temperature dependence of the half-width, which is necessary for reduction of remotely sensed data, is determined.

Gamache, Robert R.↗
NASA NTRS2004

Analysis of He I 1083 nm Imaging Spectroscopy Using a Spectral Standard

We develop a technique. for the analysis of He I 1083 nanometer spectra which addresses several difficulties through determination of a continuum background by comparison with a well calibrated standard and through removal of nearby solar and telluric blends by differential comparison to an average spectrum. The method is compared with earlier analysis of imaging spectroscopy obtained at the National Solar Observatory/Kitt Peak Vacuum Telescope (NSO/KPVT) with the NASA/NSO Spectromagnetograph (SPM). We examine distributions of Doppler velocity and line width as a function of central intensity for an active region, filament, quiet Sun, and coronal hole. For our example, we find that line widths and central intensity are oppositely correlated in a coronal hole and quiet Sun. Line widths are comparable to the quiet sun in the active region, are systematically lower in the filament, and extend to higher values in the coronal hole. Outward velocities of approximately equal to 2 to 4 kilometers per second are typically observed in the coronal hole. The sensitivity of these results to analysis technique is discussed.

Malanushenko, Elena V.↗
NASA NTRS1980

High density circuit technology

Acquisition of polyimide materials for inter-metal dielectrics was obtained from three vendors, with considerable evaluation conducted on the Dupont PI2550 material. Experimental results indicate this material can be patterned using contact printing to line width far below 0.1 mils. Optimum line width is acquired using plasma etch equipment. Metal lift-off experiments on thermal evaporated films were optimized for application to sputtered deposited films. Alternate metal-lift-off experiments are proposed for future investigation. Dry processing equipment studies and future trends in VLSI fabrication techniques are on-going.

Wade, T. E.↗
NASA NTRS1984

SMM/UVSP observations of the distribution of transition region oscillations and other properties in a sunspot

Observations of a sunspot in the C IV line at 1548 A formed in the transition region have been analyzed to obtain the time variations and/or mean values of the velocity, intensity, longitudinal magnetic field, and line width. Oscillations with periods between approximately 110 and 200 s are observed only over the umbra where the transition region magnetic field is highest and the line width is smallest. When periodic intensity variations occur at the same frequency as the velocity oscillations, the peak intensities occur slightly before the maximum upward motions. No periodic variations in the transition region magnetic field have been detected. Scatter diagrams are presented which show possible relationships between the flow velocity, emission line intensity, line width, and transition region magnetic field.

Henze, W.↗
DOE OSTI2025

Predicting multi-nodal in-nozzle particle interactions in high-viscosity fluid mediums for acoustophoretic direct-ink writing of line-patterned composites

Patterned functional materials offer improved properties (electrical, thermal, etc.) over their bulk counterparts in many applications, including energy storage, flexible electronics, and sensors. However, manufacturing approaches for patterning materials over large areas with features on the order of hundreds of microns or less are limited. Acoustophoresis, which uses acoustic forces to control particle arrangement in a fluid medium, is a pathway to address this challenge. This process is dependent on particle and fluid properties and enables patterning of a broad range of materials. Herein, a model with experimental validation is presented to demonstrate that acoustophoresis can be combined with direct-ink writing (DIW) to fabricate line patterns over large cm-scale areas. An in-nozzle particle interaction model was developed to investigate the impact of processing conditions on multi-nodal acoustophoretic DIW. The model predicts patterned line widths within a factor of two relative to experimental results for a high viscosity case study. Here, the model was used to investigate the impact of frequency, particle loading, particle radius, and acoustic pressure on line width and patterning time, providing critical feedback regarding the processing conditions suitable for a target application. Model results illustrate that frequency has the greatest impact on line patterns: increasing from 1 to 3 MHz resulted in a greater than 65% reduction in line width and a greater than 85% reduction in patterning time. Additionally, experiments were conducted with an alumina-epoxy ink and a ~21 cm 2 area pattern was rastered in ~5.5 minutes, demonstrating a path towards large-area line-patterned composite fabrication.

25 ENERGY STORAGE↗
NASA NTRS1988

Observation of Fe II (26.0 microns) in SN 1987A

The first observation of the 26-micron line from singly ionized iron in SN 1987A is reported. The total flux is 4.5 + or - 0.9 x 20 to the -18th W/sq cm. The line width (FWHM) is 4000 + or - 600 km/s. The minimum iron mass is found to be about 0.02 solar, indicating that the emission originates in the heavy element mantle and not in the hydrogen-rich envelope. Since this mass is less than estimates based on near-infrared measurements or the optical light curve, the emission is probably optically thick. In this case, the flux measurement together with the observed line width suggest a temperature of 3500 + or - 1500 K for the mantle. The broad line width suggests that mixing of the ejected iron with lighter elements in overlying layers has occurred.

Erickson, Edwin F.↗
DOE OSTI2024

Hyperspectral Detection of the Fluorescence Shift between Chirality-Sorted Empty and Water-Filled Single-Wall Carbon Nanotube Enantiomers

Single-wall carbon nanotubes (SWCNTs) have extraordinary electronic and optical properties that depend strongly on their exact chiral structure and their interaction with their inner and outer environment. The fluorescence (PL) of semiconducting SWCNTs, for instance, will shift depending on the molecules with which the SWCNT’s hollow core is filled. These interaction-induced shifts are challenging to resolve on the ensemble level in samples containing a mixture of different filling contents due to the relatively large inhomogeneous line width of the ensemble SWCNT PL compared to the size of these shifts. To circumvent this inhomogeneous broadening, single-tube spectroscopy and hyperspectral imaging are often applied, which until now required time-consuming statistical studies. Here, we present hyperspectral PL microscopy combined with automated SWCNT segmenting based on either principal component analysis or a convolutional neural network, capable of both spatially and spectrally resolving the PL along the length of many individual SWCNTs at the same time and automatically fitting peak positions and line widths of individual SWCNTs. The methodology is demonstrated by accurately determining the emission shifts and line widths of thousands of left- and right-handed empty and water-filled SWCNTs coated with a chiral surfactant, resulting in four statistical distributions which cannot be resolved in ensemble spectroscopy of unsorted samples. The results demonstrate a robust method to quickly probe ensemble properties with single-enantiomer spectral resolution. Moreover, it promises to be an absolute quantitative method to characterize the relative abundances of SWCNTs with different handedness or filling content in macroscopic samples, simply by counting individual species.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2020

High-resolution Near-infrared Spectroscopic Study of Galactic Supernova Remnants. I. Kinematic Distances

We have carried out high-resolution near-infrared spectroscopic observations toward 16 Galactic supernova remnants (SNRs) showing strong H 2 emission features. A dozen bright H 2 emission lines are clearly detected for individual SNRs, and we have measured their central velocities, line widths, and fluxes. For all SNRs except one (G9.9–0.8), the H 2 line ratios are well consistent with that of thermal excitation at T ~ 2000 K, indicating that the H 2 emission lines are most likely from shock-excited gas and therefore that they are physically associated with the remnants. The kinematic distances to the 15 SNRs are derived from the central velocities of the H 2 lines using a Galactic rotation model. We derive for the first time the kinematic distances to four SNRs: G13.5+0.2, G16.0–0.5, G32.1–0.9, and G33.2–0.6. Among the remaining 11 SNRs, the central velocities of the H 2 emission lines for six SNRs are well consistent (±5 km s -1 ) with those obtained in previous radio observations, while for the other five SNRs (G18.1–0.1, G18.9–1.1, Kes 69, 3C 396, W49B) they are significantly different. We discuss the velocity discrepancies in these five SNRs. In G9.9–0.8, the H 2 emission shows nonthermal line ratios and narrow line width (~4 km s -1 ), and we discuss its origin.

79 ASTRONOMY AND ASTROPHYSICS↗
NASA NTRS2010

Rocket-Plume Spectroscopy Simulation for Hydrocarbon-Fueled Rocket Engines

The UV-Vis spectroscopic system for plume diagnostics monitors rocket engine health by using several analytical tools developed at Stennis Space Center (SSC), including the rocket plume spectroscopy simulation code (RPSSC), to identify and quantify the alloys from the metallic elements observed in engine plumes. Because the hydrocarbon-fueled rocket engine is likely to contain C2, CO, CH, CN, and NO in addition to OH and H2O, the relevant electronic bands of these molecules in the spectral range of 300 to 850 nm in the RPSSC have been included. SSC incorporated several enhancements and modifications to the original line-by-line spectral simulation computer program implemented for plume spectral data analysis and quantification in 1994. These changes made the program applicable to the Space Shuttle Main Engine (SSME) and the Diagnostic Testbed Facility Thruster (DTFT) exhaust plume spectral data. Modifications included updating the molecular and spectral parameters for OH, adding spectral parameter input files optimized for the 10 elements of interest in the spectral range from 320 to 430 nm and linking the output to graphing and analysis packages. Additionally, the ability to handle the non-uniform wavelength interval at which the spectral computations are made was added. This allowed a precise superposition of wavelengths at which the spectral measurements have been made with the wavelengths at which the spectral computations are done by using the line-by-line (LBL) code. To account for hydrocarbon combustion products in the plume, which might interfere with detection and quantification of metallic elements in the spectral region of 300 to 850 nm, the spectroscopic code has been enhanced to include the carbon-based combustion species of C2, CO, and CH. In addition, CN and NO have spectral bands in 300 to 850 nm and, while these molecules are not direct products of hydrocarbon-oxygen combustion systems, they can show up if nitrogen or a nitrogen compound is present as an impurity in the propellants and/or these can form in the boundary layer as a result of interaction of the hot plume with the atmosphere during the ground testing of engines. Ten additional electronic band systems of these five molecules have been included into the code. A comprehensive literature search was conducted to obtain the most accurate values for the molecular and the spectral parameters, including Franck-Cordon factors and electronic transition moments for all ten band systems. For each elemental transition in the RPSSC, six spectral parameters - Doppler broadened line width at half-height, pressure-broadened line width at half-height, electronic multiplicity of the upper state, electronic term energy of the upper state, Einstein transition probability coefficient, and the atomic line center - are required. Input files have been created for ten elements of Ni, Fe, Cr, Co, Cu, Ca, Mn, Al, Ag, and Pd, which retain only relatively moderate to strong transitions in 300 to 430 nm spectral range for each element. The number of transitions in the input files is 68 for Ni; 148 for Fe; 6 for Cr; 87 for Co; 1 for Ca; 3 for Mn; 2 each for Cu, Al, and Ag; and 11 for Pd.

Tejwani, Gopal D.↗
NASA NTRS1990

NGC 1058: Gas motions in an extended, quiescent spiral disk

Researchers investigate in detail the motion of gas in the galaxy NGC 1058 using the very large array (VLA) to map the emission in the 21-cm line. This galaxy is so nearly face-on that the contribution to the line width due to the variation of the rotational velocity across the D-array beam is small compared with the random z-motion of the gas. Researchers confirm results of earlier studies (Lewis 1987, A. and A. Suppl., 63, 515; van der Kruit and Shostak 1984, A. and A., 134, 258) of the galaxy's total neutral hydrogen (HI) and kinematics, including the fact that the rotation curve drops faster than Keplerian at the outer edge of the disk, which is interpreted as a fortuitous twist of the plane of rotation in the outer disk. However, their very high velocity resolution (2.58 km s(exp -1) after Hanning smoothing) coupled with good spatial resolution, allows researchers to measure more accurately the line width, and even to some extent its shape, throughout the disk. One of the most interesting results of this study is the remarkable constancy of the line width in the outer disk. From radius 90 to 210 seconds the Gaussian velocity dispersion (sigma sub nu) of the 21-cm line has a mean value of 5.7 km s(exp -1) (after correcting for the spectral resolution) with a dispersion of less than 0.9 km s(exp -1) (after correcting for the spectral resolution) with a dispersion of less than 0.9 km s(exp -1). Translating this directly into a kinetic temperature (Doppler temperature): T sub Dopp equals 121K (sigma sub mu exp 2/(km s(exp -1) (exp 2) gives 4000 K, with a dispersion of less than 1500 K over the outer disk. This constancy is observed even when comparing the spiral arms versus inter-arm regions, which in the radius range from 100 to 150 seconds the surface density modulates (defined as the ratio N sub peak -N sub trough/N sub peak + N sub trough) from 0.5 to 0.25 in the range 150 to 200 seconds.

Hanson, Margaret Murray↗
DOE OSTI2024

Approaching Angstrom-Scale Resolution in Lithography Using Low-Molecular-Mass Resists (<500 Da)

Resists that enable high-throughput and high-resolution patterning are essential in driving the semiconductor technology forward. The ultimate patterning performance of a resist in lithography is limited because of the trade-off between resolution, line-width roughness, and sensitivity; improving one or two of these parameters typically leads to a loss in the third. As the patterned feature sizes approach angstrom scale, the trade-off between these three metrics becomes increasingly hard to resolve and calls for a fundamental rethinking of the resist chemistry. Low-molecular-mass monodispersed metal-containing resists of high atom economy can provide not only very high resolution but also very low line-width roughness without sacrificing sensitivity. Here we describe a modular metal-containing resist platform (molecular mass <500 Da) where a molecular resist consists of just two components: a metal and a radical initiator bonded to it. This simple system not only is amenable to high-resolution electron beam lithography (EBL) and extreme ultraviolet lithography (EUVL) but also unites them mechanistically, giving a consolidated perspective of molecular and chemical processes happening during exposure. Irradiation of the resist leads to the production of secondary electrons that generate radicals in the initiator bonded to metal. This brings about an intramolecular rearrangement and causes solubility switch in the exposed resist. We demonstrate record 1.9–2.0 nm isolated patterns and 7 nm half-pitch dense line-space features over a large area using EBL. With EUVL, 12 nm half-pitch line-space features are shown at a dose of 68 mJ/cm 2 . In both of these patterning techniques, the line-width roughness was found to be ≤2 nm, a record low value for any resist platform, also leading to a low-performance trade-off metric, Z factor, of 0.6 × 10 –8 mJ·nm 3 . With the ultimate resolution limited by instrumental factors, potential patterning at the level of a unit cell can be envisaged, making low-molecular-mass resists best poised for angstrom-scale lithography.

77 NANOSCIENCE AND NANOTECHNOLOGY↗
NASA NTRS2005

Coronal Structures in Cool Stars

We have extended our study of the structure of coronas in cool stars to very young stars still accreting from their surrounding disks. In addition we are pursing the connection between coronal X-rays and a powerful diagnostic line in the infrared, the He I 10830Angstrom transition of helium. Highlights of these are summarized below including publications during this reporting period and presentations. Spectroscopy of the infrared He I (lambda10830) line with KECK/NIRSPEC and IRTF/CSHELL and of the ultraviolet C III (lambda977) and O VI (lambda1032) emission with FUSE reveals that the classical T Tauri star TW Hydrae exhibits P Cygni profiles, line asymmetries, and absorption indicative of a continuous, fast (approximately 400 kilometers per second), hot (approximately 300,000 K) accelerating outflow with a mass loss rate approximately 10(exp -11)-10(exp -12) solar mass yr(sup -1) or larger. Spectra of T Tauri N appear consistent with such a wind. The source of the emission and outflow seems restricted to the stars themselves. Although the mass accretion rate is an order of magnitude less for TW Hya than for T Tau, the outflow reaches higher velocities at chromospheric temperatures in TW Hya. Winds from young stellar objects may be substantially hotter and faster than previously thought. The ultraviolet emission lines, when corrected for absorption are broad. Emission associated with the accretion flow and shock is likely to show turbulent broadening. We note that the UV line widths are significantly larger than the X-ray line widths. If the X-rays from TW Hya are generated at the accretion shock, the UV lines may not be directly associated with the shock. On the other hand, studies of X-ray emission in young star clusters, suggest that the strength of the X-ray emission is correlated with stellar rotation, thus casting doubt on an accretion origin for the X-rays. We are beginning to access the infrared spectral region where the He I 108308Angstroms transition occurs. This line is particularly useful as a diagnostic of coronal radiation since it is formed by recombination following photoionization of neutral helium by coronal X-rays. Because the lower level of the transition is metastable, infrared radiation from the stellar photosphere is absorbed which provides a diagnostic of atmospheric dynamics. This transition is useful both in young stars in the T Tauri phase and in active cool star binaries. We will investigate the influence of coronal x-rays on the strength of this transition.

Oliversen, Ronald↗
NASA NTRS1976

Components in interstellar molecular hydrogen

Results are reported for precise spectrophotometric measurements of the profiles of selected Lyman absorption lines produced by hydrogen molecules in various rotational levels along the line of sight to 13 stars which have shown some evidence for an increase in line width with increasing rotational quantum number (J). The line profiles were measured by multiple scans with the Copernicus satellite telescope. Based on analysis of the radial velocities, derivations of the column densities, and line-profile fitting, the following conclusions are made: (1) the increase in interstellar H2 line width with increasing J results from the presence of the most shortward component, which is relatively weak at low J but becomes more important at higher J; (2) the relative column densities found for the different J levels in each component may be fitted by a theoretical model in which rotational excitation is due to absorption of UV photons followed by radiative quadrupole spontaneous transitions or collisionally induced downward transitions between different J levels; (3) the atomic hydrogen density is between 300 and 1000 per cu cm in the most shortward component for each of three stars; (4) the approaching gas which produces each shortward component must be in the form of thin sheets; and (5) the sheets are the compressed gas behind a shock front moving through the interstellar medium.

Spitzer, L., Jr.↗
NASA NTRS1980

A study of the Jovian forbidden line S II nebula at high spectral resolution

Observations of forbidden line S II 6716-6731 A emissions from the Jovian magnetosphere have been carried out with a PEPSIOS spectrometer at the Hale 5 m telescope. Spectral resolving power was sufficient to resolve the forbidden line S II line widths. From measured 6716-6731 A doublet ratios and spectral line widths a thermal plasma is found characterized by temperatures about 2 x 10 to the 4th K and electron densities about 2000 cu cm. The source of forbidden line S II emissions was centered within a toroidal region of radius 5 Jupiter radii (inside the orbit of Io), with tight latitudinal confinement near the equilibrium equator for ions in the tilted corotating Jovian magnetic field, and significant long-lived longitudinal structure.

Trauger, J. T.↗