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At least 109 records · Page 6

Deformation across the western United States: A local estimate of Pacific-North America transform deformation

We obtain a locally based estimate of Pacific-North America relative motion and an uncertainly in this estimate by integrating deformation rate along three different paths leading west across southwestern North America from east of the Rio Grande Rift to near the continental escarpment. Data are primarily Quatenary geologic slip rates estimates, and resulting deformation determinations therefore are 'instantaneous' in a geologic sense but 'long term' with respect to earthquake cycles. We deduce a rate of motion of the Pacific plane relative to North America that is 48 +/- 2 mm/yr, a rate indistinguishable from that predicted by the global kinematics models RM2 and NUVEL-1; however, we obtain an orientation that is 5-9 deg counterclockwise of these models. A more westerly motion of the Pacific plate, with respect to North America, is calculated from all three paths. The relatively westerly motion of the Pacific plate is accomodated by deformation in the North American continent that includes slip on relatively counterclockwise-oriented strike-slip faults (including the San Andreas fault), whic is especially relevant in and south of the Transverse Ranges, and a margin-normal component of net extension across the continent, which is especially relevant north of the Transverse Ranges. Deformation of the SW United States occurs in regionally coherent domains within the style of deformation is approximately uniform.

Humphreys, Eugene D.↗

Mechanisms for Diurnal Variability of Global Tropical Rainfall Observed from TRMM

The behavior and various controls of diurnal variability in tropical-subtropical rainfall are investigated using Tropical Rainfall Measuring Mission (TRMM) precipitation measurements retrieved from the three level-2 TRMM standard profile algorithms for the 1998 annual cycle. Results show that diurnal variability characteristics of precipitation are consistent for all three algorithms, providing assurance that TRMM retrievals are producing consistent estimates of rainfall variability. As anticipated, most ocean areas exhibit more rainfall at night, while over most land areas, rainfall peaks during daytime; however, important exceptions are noted. The dominant feature of the oceanic diurnal cycle is a rainfall maximum in late-evening-early-morning (LE-EM) hours, while over land the dominant maximum occurs in the mid- to late afternoon (MLA). In conjunction with these maxima are pronounced seasonal variations of the diurnal amplitudes. Amplitude analysis shows that the diurnal pattern and its seasonal evolution are closely related to the rainfall accumulation pattern and its seasonal evolution. In addition, the horizontal distribution of diurnal variability indicates that for oceanic rainfall, there is a secondary MLA maximum coexisting with the LE-EM maximum at latitudes dominated by large-scale convergence and deep convection. Analogously, there is a preponderancy for an LE EM maximum over land coexisting with the stronger MLA maximum, although it is not evident that this secondary continental feature is closely associated with the large-scale circulation. Neither of the secondary maxima exhibit phase behavior that can be considered semidiurnal in nature. Diurnal rainfall variability over the ocean associated with large-scale convection is clearly an integral component of the general circulation. Phase analysis reveals differences in regional and seasonal features of the diurnal cycle, indicating that underlying forcing mechanisms differ from place to place. This is underscored by the appearance of secondary ocean maxima in the presence of large-scale convection, along with other important features. Among these, there are clear-cut differences between the diurnal variability of seasonal rainfall over the mid-Pacific and Indian Ocean Basins. The mid-Pacific exhibits double maxima in spring and winter but only LE-EM maxima in summer and autumn, while the Indian Ocean exhibits double maxima in spring and summer and only an LE-EM maximum in autumn and winter. There are also evident daytime maxima within the major large-scale marine stratocumulus regions off the west coasts of continents. The study concludes with a discussion concerning how the observational evidence either supports or repudiates possible forcing mechanisms that have been suggested to explain diurnal rainfall variability.

Yang, Song↗

A typological framework of non-floodplain wetlands for global collaborative research and sustainable use

Non-floodplain wetlands (NFWs) are important but vulnerable inland freshwater systems that are receiving increased attention and protection worldwide. However, a lack of consistent terminology, incohesive research objectives, and inherent heterogeneity in existing knowledge hinder cross-regional information sharing and global collaboration. To address this challenge and facilitate future management decisions, we synthesized recent work to understand the state of NFW science and explore new opportunities for research and sustainable NFW use globally. Results from our synthesis show that although NFWs have been widely studied across all continents, regional biases exist in the literature. We hypothesize these biases in the literature stem from terminology rather than real geographical bias around existence and functionality. To confirm this observation, we explored a set of geographically representative NFW regions around the world and characteristics of research focal areas. We conclude that there is more that unites NFW research and management efforts than we might otherwise appreciate. Furthermore, opportunities for cross-regional information sharing and global collaboration exist, but a unified terminology will be needed, as will a focus on wetland functionality. Based on these findings, we discuss four pathways that aid in better collaboration, including improved cohesion in classification and terminology, and unified approaches to modeling and simulation. In turn, legislative objectives must be informed by science to drive conservation and management priorities. Finally, an educational pathway serves to integrate the measures and to promote new technologies that aid in our collective understanding of NFWs. Our resulting framework from NFW synthesis serves to encourage interdisciplinary collaboration and sustainable use and conservation of wetland systems globally.

54 ENVIRONMENTAL SCIENCES↗

Understanding Biases in Simulated Cloud Radiative Effects in E3SMv3

This study systematically investigates biases in cloud radiative effects (CREs) within the recently released Energy Exascale Earth System Model version 3 (E3SMv3). Compared to its previous version (E3SMv2), E3SMv3 shows excessively strong shortwave CRE over tropical and subtropical oceans, the Southern Ocean, and the Northern Hemisphere storm tracks, which is primarily caused by an overestimation of optically intermediate low clouds. The model also displays excessive longwave CRE over the Maritime Continent and other tropical deep convection regions, resulting from an overestimation of optically thick high clouds. Implementing the Predicted Particle Properties (P3) scheme for stratiform clouds played the most significant role in these cloud changes. In addition, using a double-moment scheme for convective clouds contributed to the increase in intermediate low clouds and optically thick clouds in tropical deep convection regions. Error metrics for total cloud amount (E TCA ), cloud properties (E ctp-τ ), and cloud properties weighted by their SW and LW radiative impacts (E SW and E LW ) indicate that E3SMv3's ability to reproduce observed cloud radiative effect of low, middle, and high clouds has not been improved compared to E3SMv2. Nevertheless, the performance of E3SMv3 remains well within the spread of CMIP6 models, with E SW and E LW values smaller than those in most CMIP6 models. This study underscores the importance of integrating diverse satellite observations for robust cloud evaluation and using cloud-radiation relationships as consistency check for model errors. It suggests that further model developments focus on improving cloud microphysics and their interactions with radiation.

Environmental sciences↗

MITR Low-Enriched Uranium Conversion Fluid-Structure Interaction Preliminary Design Verification

The U.S. National Nuclear Security Administration (NNSA) Office of Material Management and Minimization (M 3 ) has developed and is pursuing an integrated approach to address the persistent threat posed by unintentional proliferation of nuclear materials. The NNSA M 3 approach reduces the risk of highly enriched uranium (HEU) and plutonium falling into the hands of non-state actors by minimizing the use of and, when possible, eliminating weapons-usable nuclear material around the world. In this geopolitical context, most research and test reactors, both domestic and international, have completed or started a program of conversion from the use of HEU to low-enriched uranium (LEU) as fuel. Conversion of civilian research reactors from HEU to LEU, and the return of the HEU to the country of origin, are important components of the NNSA non-proliferation program. Worldwide, 71 reactors have been converted to the use of LEU fuel, and an additional 32 have been confirmed to be permanently shut down. The U.S., with 20 reactor conversions, is among the 39 countries on six continents where conversions have occurred. With recent conversions in Ghana and Nigeria, an important milestone was reached in completing conversion of all reactors on the continent of Africa to LEU fuel. Africa thus becomes the third continent to have completed conversion of all HEU reactors to LEU, following Australia and South America

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Cross-Disciplinarity in the Advance of Antarctic Ecosystem Research

The biodiversity, ecosystem services and climate variability of the Antarctic continent, and the Southern Ocean are major components of the whole Earth system. Antarctic ecosystems are driven more strongly by the physical environment than many other marine and terrestrial ecosystems. As a consequence, to understand ecological functioning, cross-disciplinary studies are especially important in Antarctic research. The conceptual study presented here is based on a workshop initiated by the Research Programme Antarctic Thresholds - Ecosystem Resilience and Adaption of the Scientific Committee on Antarctic Research, which focused on challenges in identifying and applying cross-disciplinary approaches in the Antarctic. Novel ideas, and first steps in their implementation, were clustered into eight themes, ranging from scale problems, risk maps, organism and ecosystem responses to multiple environmental changes, to evolutionary processes. Scaling models and data across different spatial and temporal scales were identified as an overarching challenge. Approaches to bridge gaps in the research programmes included multi-disciplinary monitoring, linking biomolecular findings and simulated physical environments, as well as integrative ecological modelling. New strategies in academic education are proposed. The results of advanced cross-disciplinary approaches can contribute significantly to our knowledge of ecosystem functioning, the consequences of climate change, and to global assessments that ultimately benefit humankind.

Scaling↗

Numerical Study of the Role of Shallow Convection in Moisture Transport and Climate

The objective of this investigation was to study the role of shallow convection on the regional water cycle of the Mississippi and Little Washita Basins of the Southern Great Plains (SGP) using a 3-D mesoscale model, the PSU/NCAR MM5. The underlying premise of the project was that current modeling of regional-scale climate and moisture cycles over the continents is deficient without adequate treatment of shallow convection. At the beginning of the study, it was hypothesized that an improved treatment of the regional water cycle can be achieved by using a 3-D mesoscale numerical model having high-quality parameterizations for the key physical processes controlling the water cycle. These included a detailed land-surface parameterization (the Parameterization for Land-Atmosphere-Cloud Exchange (PLACE) sub-model of Wetzel and Boone), an advanced boundary-layer parameterization (the 1.5-order turbulent kinetic energy (TKE) predictive scheme of Shafran et al.), and a more complete shallow convection parameterization (the hybrid-closure scheme of Deng et al.) than are available in most current models. PLACE is a product of researchers working at NASA's Goddard Space Flight Center in Greenbelt, MD. The TKE and shallow-convection schemes are the result of model development at Penn State. The long-range goal is to develop an integrated suite of physical sub-models that can be used for regional and perhaps global climate studies of the water budget. Therefore, the work plan focused on integrating, improving, and testing these parameterizations in the MM5 and applying them to study water-cycle processes over the SGP. These schemes have been tested extensively through the course of this study and the latter two have been improved significantly as a consequence.

Seaman, Nelson L.↗

Assessing Impact of Aerosol Intercontinental Transport on Regional Air Quality and Climate: What Satellites Can Help

Mounting evidence for intercontinental transport of aerosols suggests that aerosols from a region could significantly affect climate and air quality in downwind regions and continents. Current assessment of these impacts for the most part has been based on global model simulations that show large variability. The aerosol intercontinental transport and its influence on air quality and climate involve many processes at local, regional, and intercontinental scales. There is a pressing need to establish modeling systems that bridge the wide range of scales. The modeling systems need to be evaluated and constrained by observations, including satellite measurements. Columnar loadings of dust and combustion aerosols can be derived from the MODIS and MISR measurements of total aerosol optical depth and particle size and shape information. Characteristic transport heights of dust and combustion aerosols can be determined from the CALIPSO lidar and AIRS measurements. CALIPSO liar and OMI UV technique also have a unique capability of detecting aerosols above clouds, which could offer some insights into aerosol lofting processes and the importance of above-cloud transport pathway. In this presentation, I will discuss our efforts of integrating these satellite measurements and models to assess the significance of intercontinental transport of dust and combustion aerosols on regional air quality and climate.

Yu, Hongbin↗

Radiative Heating Rate Profiles over the Southeast Atlantic Ocean during the 2016 and 2017 Biomass Burning Seasons

Marine boundary layer clouds, including the transition from stratocumulus to cumulus, are poorly represented in numerical weather prediction and general circulation models. Further uncertainties in the cloud structure arise in the presence of biomass burning carbonaceous aerosol, as is the case over the southeast Atlantic Ocean where biomass burning aerosol is transported from the African continent. As the aerosol plume progresses across the southeast Atlantic Ocean, radiative heating within the aerosol layer has the potential to alter the thermodynamic environment and therefore the cloud structure; however, limited work has been done to quantify this along the trajectory of the aerosol plume in the region. The deployment of the First Atmospheric Radiation Measurement Mobile Facility in support of the Layered Atlantic Smoke Interactions with Clouds field campaign provided a unique opportunity to collect observations of cloud and aerosol properties during two consecutive biomass burning seasons during July through October of 2016 and 2017 over Ascension Island (7.96 °S, 14.35 °W). Using observed profiles of temperature, humidity, and clouds from the field campaign, alongside aerosol optical properties from MERRA-2 as input for the Rapid Radiation Transfer Model, profiles of the radiative heating rate due to aerosols and clouds were computed. Radiative heating is also assessed across the southeast Atlantic Ocean using an ensemble of back trajectories from the Hybrid Single Particle Lagrangian Integrated Trajectory Model. Idealized experiments using the Rapid Radiation Transfer Model with and without aerosols and a range of values for the single scattering albedo demonstrate that shortwave heating within the aerosol layer above Ascension Island can locally range between 2 and 8 K per day depending on the aerosol optical properties, though impacts of the aerosol can be felt elsewhere in the atmospheric column. When considered under clear conditions, the aerosol has a cooling effect at the TOA and based on the observed cloud properties at Ascension Island, the cloud albedo is not large enough to overcome this. Shortwave radiative heating due to biomass burning aerosol is not balanced by additional longwave cooling, and the net radiative impact results in a stabilization of the lower troposphere. However, these results are extremely sensitive to the single scattering albedo assumptions in models.

Allison B. Marquardt Collow↗

Continental Scale Aerosol Optical Properties Over East Asia as Measured by Aeronet and Comparison to Satellite and Modeled Results

The AERONET program has operated in E. Asia since 1995 providing time continuous and time averaged ground-based column-integrated aerosol optical properties in a variety of aerosol regimes In the last four years the distribution has greatly increased in Siberia, China, SE Asia and India in particular. Commensurate with that, significant improvement in data processing algorithms (Version 2.0) and access to ancillary data products through the WWW have become available to the scientific community. At this writing the following distribution represents E and S. Asia: 5 sites operate in Siberia (2 years), 1 in Mongolia (9 years), 3 in Korea (3 to 6 years), 3 in Japan (2 to 7 years), China 11 (6 to 0 years), Taiwan 4 (7 to 2 yrs), Viet Nam 2 (4 years), Thailand 2 to 5 (4 years), and Singapore 1 (4 months), India 1 to 3 (7 to 1 years), Pakistan 2 (1 year), and UAE 3 (3 years). An analysis of the aerosol optical depth at 500 nm using annual average quality assured AERONET data (pre 2006) was used to estimate the mean annual aerosol loading by continent, sub continent and ocean. The individual site data were assumed representative of regional aerosol loading and aggregated to the sub-continental, continental and oceanic areas and presented. This analysis will be updated with more recent data with particular emphasis on seasonal results for Asia and the addition of single scattering albedo retrievals. The ground based results will be compared to MODIS collection 5 results and model estimates for E. Asia using the AERONET Synergy Tool.

Holben, B. N.↗

DeepSAT: A Deep Learning Approach to Tree-Cover Delineation in 1-m NAIP Imagery for the Continental United States

High resolution tree cover classification maps are needed to increase the accuracy of current land ecosystem and climate model outputs. Limited studies are in place that demonstrates the state-of-the-art in deriving very high resolution (VHR) tree cover products. In addition, most methods heavily rely on commercial softwares that are difficult to scale given the region of study (e.g. continents to globe). Complexities in present approaches relate to (a) scalability of the algorithm, (b) large image data processing (compute and memory intensive), (c) computational cost, (d) massively parallel architecture, and (e) machine learning automation. In addition, VHR satellite datasets are of the order of terabytes and features extracted from these datasets are of the order of petabytes. In our present study, we have acquired the National Agriculture Imagery Program (NAIP) dataset for the Continental United States at a spatial resolution of 1-m. This data comes as image tiles (a total of quarter million image scenes with ~60 million pixels) and has a total size of ~65 terabytes for a single acquisition. Features extracted from the entire dataset would amount to ~8-10 petabytes. In our proposed approach, we have implemented a novel semi-automated machine learning algorithm rooted on the principles of "deep learning" to delineate the percentage of tree cover. Using the NASA Earth Exchange (NEX) initiative, we have developed an end-to-end architecture by integrating a segmentation module based on Statistical Region Merging, a classification algorithm using Deep Belief Network and a structured prediction algorithm using Conditional Random Fields to integrate the results from the segmentation and classification modules to create per-pixel class labels. The training process is scaled up using the power of GPUs and the prediction is scaled to quarter million NAIP tiles spanning the whole of Continental United States using the NEX HPC supercomputing cluster. An initial pilot over the state of California spanning a total of 11,095 NAIP tiles covering a total geographical area of 163,696 sq. miles has produced true positive rates of around 88 percent for fragmented forests and 74 percent for urban tree cover areas, with false positive rates lower than 2 percent for both landscapes.

Imagery↗

Exploring sustainable electricity system development pathways in South America’s MERCOSUR sub-region

South America has abundant natural water and energy resources, and exploiting these resources to achieve a clean energy future is central to the continent’s economic and sustainable development objectives for the next several decades. Designing pathways to achieving this clean energy future requires better understanding the structural, techno-economic, and policy forces that may influence the future development of the electricity sector in the region. Here, we focus on an interconnected electricity system of five South American countries – Argentina, Brazil, Chile, Paraguay, and Uruguay – which represent major electricity generation, consumption, and trade dynamics in the region. We explore the implications of various forces that could shape the future composition of the power sector in the sub-region, including: evolving renewable energy cost and performance, natural gas prices, cross-border interconnection facilities, early retirement of installed hydropower, and different decarbonization goals. We use a model framework based on a power system planning platform (GridPath) to co-optimize investment and operations of generation, storage, and transmission facilities out to 2050. Our results in a Reference scenario indicate that the electricity system can maintain a relatively clean energy portfolio by leveraging existing hydropower capacity and integrating increasingly cost-competitive wind and solar power. However, dependence on natural gas in the region is likely to remain high. A low-carbon electricity system can cost-effectively be achieved through policy interventions (e.g., renewable portfolio standards) and by diversifying investments in wind, solar, battery storage, and some new hydropower capacity. We also find that existing hydropower is critical for maintaining reliable future grid operations. Enhanced regional electricity trade, mostly based on existing interconnection capacities with nominal investment in new transmission, can significantly benefit the clean energy transition in the region.

29 ENERGY PLANNING, POLICY, AND ECONOMY↗

Radiative heating rate profiles over the southeast Atlantic Ocean during the 2016 and 2017 biomass burning seasons

Marine boundary layer clouds, including the transition from stratocumulus to cumulus, are poorly represented in numerical weather prediction and general circulation models. Further uncertainties in the cloud structure arise in the presence of biomass burning carbonaceous aerosol, as is the case over the southeast Atlantic Ocean, where biomass burning aerosol is transported from the African continent. As the aerosol plume progresses across the southeast Atlantic Ocean, radiative heating within the aerosol layer has the potential to alter the thermodynamic environment and therefore the cloud structure; however, limited work has been done to quantify this along the trajectory of the aerosol plume in the region. The deployment of the first Atmospheric Radiation Measurement (ARM) Mobile Facility (AMF1) in support of the Layered Atlantic Smoke Interactions with Clouds field campaign provided a unique opportunity to collect observations of cloud and aerosol properties during two consecutive biomass burning seasons during July through October of 2016 and 2017 over Ascension Island (7.96° S, 14.35° W). Using observed profiles of temperature, humidity, and clouds from the field campaign alongside aerosol optical properties from Modern-Era Retrospective analysis for Research and Applications, Version 2 (MERRA-2), as input for the Rapid Radiation Transfer Model (RRTM), profiles of the radiative heating rate due to aerosols and clouds were computed. Radiative heating is also assessed across the southeast Atlantic Ocean using an ensemble of back trajectories from the Hybrid Single Particle Lagrangian Integrated Trajectory (HYSPLIT) model. Idealized experiments using the RRTM with and without aerosols and a range of values for the single-scattering albedo (SSA) demonstrate that shortwave (SW) heating within the aerosol layer above Ascension Island can locally range between 2 and 8 K d -1 depending on the aerosol optical properties, though impacts of the aerosol can be felt elsewhere in the atmospheric column. When considered under clear conditions, the aerosol has a cooling effect at the TOA, and based on the observed cloud properties at Ascension Island, the cloud albedo is not large enough to overcome this. Shortwave radiative heating due to biomass burning aerosol is not balanced by additional longwave (LW) cooling, and the net radiative impact results in a stabilization of the lower troposphere. However, these results are extremely sensitive to the single-scattering albedo assumptions in models.

54 ENVIRONMENTAL SCIENCES↗

Air Mass Factor Formulation for Spectroscopic Measurements from Satellites: Application to Formaldehyde Retrievals from the Global Ozone Monitoring Experiment

We present a new formulation for the air mass factor (AMF) to convert slant column measurements of optically thin atmospheric species from space into total vertical columns. Because of atmospheric scattering, the AMF depends on the vertical distribution of the species. We formulate the AMF as the integral of the relative vertical distribution (shape factor) of the species over the depth of the atmosphere, weighted by altitude-dependent coefficients (scattering weights) computed independently from a radiative transfer model. The scattering weights are readily tabulated, and one can then obtain the AMF for any observation scene by using shape factors from a three dimensional (3-D) atmospheric chemistry model for the period of observation. This approach subsequently allows objective evaluation of the 3-D model with the observed vertical columns, since the shape factor and the vertical column in the model represent two independent pieces of information. We demonstrate the AMF method by using slant column measurements of formaldehyde at 346 nm from the Global Ozone Monitoring Experiment satellite instrument over North America during July 1996. Shape factors are cumputed with the Global Earth Observing System CHEMistry (GEOS-CHEM) global 3-D model and are checked for consistency with the few available aircraft measurements. Scattering weights increase by an order of magnitude from the surface to the upper troposphere. The AMFs are typically 20-40% less over continents than over the oceans and are approximately half the values calculated in the absence of scattering. Model-induced errors in the AMF are estimated to be approximately 10%. The GEOS-CHEM model captures 50% and 60% of the variances in the observed slant and vertical columns, respectively. Comparison of the simulated and observed vertical columns allows assessment of model bias.

Palmer, Paul I.↗

Quantifying the impacts of atmospheric rivers on the surface energy budget of the Arctic based on reanalysis

We present a comprehensive analysis of Arctic surface energy budget (SEB) components during atmospheric river (AR) events identified by integrated water vapor transport exceeding the monthly 85th-percentile climatological threshold in 3-hourly ERA5 reanalysis data from January 1980 to December 2019. Analysis of average anomalies in SEB components, net SEB, and the overall AR contribution to both the seasonal SEB components and net SEB climatology reveals clear seasonality and distinct land–sea–sea ice contrast patterns. Over the sea-ice-covered central Arctic Ocean, ARs significantly impact net SEB, inducing substantial surface warming in fall, winter, and spring. This warming is primarily driven by large anomalies in surface downward longwave radiation (LWD), which average 29–45 W m −2 during the cold seasons. In contrast, AR-related LWD anomalies are smaller in summer, averaging around 15 W m −2 , indicating a reduced impact during this season. Over sub-polar oceans, ARs have the most substantial positive impact on net SEB in cold seasons, mainly attributed to significant positive turbulent heat flux anomalies. AR-related turbulent heat anomalies reduce the upward turbulent flux, contributing up to −11 % relative to its seasonal climatology. In summer, ARs induce negative impacts on net SEB, primarily due to reduced shortwave radiation from increased cloud cover during AR events. Over continents, ARs generate smaller absolute impacts on net SEB because the large LWD anomalies are largely offset by corresponding increases in upward longwave radiation, particularly during cold seasons. Additionally, the seemingly large relative contributions of ARs to the net SEB over land primarily reflects the small magnitude of the climatological net SEB over continents. Greenland, especially western Greenland, exhibits significant downward longwave radiation anomalies associated with ARs, which drive large net SEB anomalies and contribute >54 % to mean SEB and induce amplified surface warming year-round. This holds significance for melt events, particularly during summer. Additionally, results of AR-related SEB impacts strongly depend on detection methods, as restrictive AR detection algorithms that emphasize extreme AR events, with large AR-related anomalies, do not necessarily indicate a large overall contribution to the SEB climatology due to the low occurrence frequency of these events. This study quantifies the role of ARs in the surface energy budget, contributing to our understanding of the Arctic warming and sea ice decline in ongoing Arctic amplification.

Arctic Sea ice change↗

Influence of Sea-Ice Anomalies on Antarctic Precipitation Using Source Attribution in the Community Earth System Model

We conduct sensitivity experiments using a general circulation model that has an explicit water source tagging capability forced by prescribed composites of pre-industrial sea-ice concentrations (SICs) and corresponding sea surface temperatures (SSTs) to understand the impact of sea-ice anomalies on regional evaporation, moisture transport and source–receptor relationships for Antarctic precipitation in the absence of anthropogenic forcing. Surface sensible heat fluxes, evaporation and column-integrated water vapor are larger over Southern Ocean (SO) areas with lower SICs. Changes in Antarctic precipitation and its source attribution with SICs have a strong spatial variability. Among the tagged source regions, the Southern Ocean (south of 50∘ S) contributes the most (40 %) to the Antarctic total precipitation, followed by more northerly ocean basins, most notably the South Pacific Ocean (27%), southern Indian Ocean (16 %) and South Atlantic Ocean (11 %). Comparing two experiments prescribed with high and low pre-industrial SICs, respectively, the annual mean Antarctic precipitation is about 150 Gt yr−1 (or 6 %) more in the lower SIC case than in the higher SIC case. This difference is larger than the model-simulated interannual variability in Antarctic precipitation (99 Gt yr−1). The contrast in contribution from the Southern Ocean, 102 Gt yr−1, is even more significant compared to the interannual variability of 35 Gt yr−1 in Antarctic precipitation that originates from the Southern Ocean. The horizontal transport pathways from individual vapor source regions to Antarctica are largely determined by large-scale atmospheric circulation patterns. Vapor from lower-latitude source regions takes elevated pathways to Antarctica. In contrast, vapor from the Southern Ocean moves southward within the lower troposphere to the Antarctic continent along moist isentropes that are largely shaped by local ambient conditions and coastal topography. This study also highlights the importance of atmospheric dynamics in affecting the thermodynamic impact of sea-ice anomalies associated with natural variability on Antarctic precipitation. Our analyses of the seasonal contrast in changes of basin-scale evaporation, moisture flux and precipitation suggest that the impact of SIC anomalies on regional Antarctic precipitation depends on dynamic changes that arise from SIC–SST perturbations along with internal variability. The latter appears to have a more significant effect on the moisture transport in austral winter than in summer.

Wang, Hailong↗

Airborne Measurements of Nitric Oxide, Nitrogen Dioxide, Ozone, and Total Reactive Nitrogen During the NASA Global Tropospheric Experiment

Fabrication of the University of Michigan Multichannel Chemiluminescence Instrument (UMMCI) was completed in early 1996 and the instrument participated in test flights on the NASA P3B at Wallops Island prior to integration and deployment for the PEM- Tropics A Mission. The UMMCI consists of 4 channels for simultaneous measurements of ozone and NO with the option for measurements of NO2 and NOy (total reactive nitrogen) when converters are placed upstream of the NO channels. Each NO channel consists of a zeroing volume and reaction vessel, while the ozone channel consists of an ozone catalyst (or scrubber) trap that is not in line with the reaction vessel. The detectors in all for channels are Hamamatsu photomultiplier tubes, which are followed by pulse amplifier discriminators on the NO channels and an electrometer on the ozone channel. Schematics of the Detector Module and NOx/03 Probe Insert and Diagrams of the Control and Data System, the Power and Ground System, the Gas Flow System, and the Calibration System Flow are attached. Intercomparisons were conducted with G. Gregory, NASA/Langley, during the test flights (following prior calibration of the ozone generator/calibrators at the Wallops Long-Path Absorption facility). Initial test results appeared to be reasonable, and instrument characterization studies proceeded for the ozone channel and the 3 NO channels until deployment for integration for the PEM-Tropics Mission. Ozone data was obtained for Flights #4, and 6-2 1, and finalized data was submitted to the PEM-Tropics Data Archive and to the Science Team during the April 1997 Data Workshop. Although it initially appeared that the instrument sensitivity varied, subsequent tests showed that this was the fault of a leak in the ozone calibrator. In fact; the instrument sensitivity has not been observed to vary in a large number of tests over the years since the PEM-Tropics mission. We have, therefore, a very high degree of confidence in the O3 data that we submitted. NO data was obtained for all flights except the mission out of Christmas Island and the subsequent return to Hawaii, during which time the NO channels were contaminated with back-flushing pure NO from the O3 channel. The NO channels were found to suffer from a varying artifact (7 - 22 pptv) which made the instrument's results unreliable for the marine boundary layer portions of the missions (where conditions were extremely clean with NO typically < 2 pptv and O3 only 8 ppbv). Nonetheless, the NO values were an upper limit and were quite useful in identifying pollution layers and outflow from the Latin American Continent. NO data was submitted to the archive for all flights during which data was obtained. Ozone data from the P3B was among the results presented in several peer-reviewed publications. Notably, the ozone data supported the first published finding of evidence for the occurrence of aerosol nucleation in the marine boundary layer. As well, the ozone data was utilized in a treatment of the wavenumber spectra of winds, temperature and trace gases and to demonstrate the occurrence of layering as observed by the P3B during PEM-Tropics A . O3 and NO data were used in an assessment of the impact of southern hemispheric biomass burning, and in the role of NOx and O3 in HOx photochemistry during the PEM Tropics A mission. These data, along with other species measured during PEM-Tropics A, have also been employed in the generation of climatologies for tropospheric ozone and its precursors by the PI's research group.

Carroll, Mary Anne↗

The Surface Longwave Downward Fluxes of the NASA GEWEX SRB Release 4.0 IP Products: Validation Against the Surface-Based BSRN and PMEL Observed Data

Since the NASA Global Energy Water Exchanges (GEWEX) Surface Radiation Budget (SRB) project released its 3rd version of products in 2010, the GEWEX Data Assessments Panel (GDAP) has been working on integrating various data products to address issues in the closing of the global energy and water cycles. The 4th version of the SRB products, Rel. 4.0-IP, has integrated data products from the cloud, aerosol, atmosphere, ocean surface, and land surface projects, coordinating within GDAP, to produce a long-term time series of TOA and surface radiative estimates. The Rel. 4-IP shortwave products span 34 years continuously from July 1983 to June 2017 on a quasi-equal-area 1degree longitude by 1degree latitude grid system. The longwave products are for land only from 1983-07 to 1987-12; for both land and ocean from 1988-01 to 2009-12; and ocean only from 2010-01 to 2017-06. The data are provided at 3 hourly, 3-hourly-monthly, daily and monthly means. The ISCCP HXS clouds and radiances are the key cloud input of the current GEWEX SRB algorithms. In addition, the longwave algorithm has also made changes in cloud microphysical property, surface skin temperature input, surface emissivity, atmospheric profile, adding longwave aerosol optical properties, revising cloud overlap procedure, and so on. Details of changes in both inputs and algorithms are documented in a NASA Algorithm Theoretical Basis Document (ATBD). We have validated the surface longwave downward fluxes against the surface-based Baseline Surface Radiation Network (BSRN) and the Pacific Marine Environmental Laboratory (PMEL) buoy data. As of 2020, the BSRN archive has 12,116 site-months of observed records from 73 stations on all seven continents, and as of 2017, PMEL archive has 4389 buoy months of observed records from 64 buoys deployed in the tropics of Pacific, Atlantic and Indian Oceans. This paper presents how the SRB Rel. 4.0-IP surface longwave downward fluxes compare with these surface-based measurements and how the comparison statistics differ from that of Rel. 3.0.

GEWEX SRB↗