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At least 109 records · Page 6

Floquet dynamics of classical and quantum cavity fields

We show that the time-dependence of electromagnetic field in a periodically modulated cavity can be effectively analyzed using a Floquet map. The map relates the field states separated by one period of the drive; iterative application of the map allows to determine field configuration after arbitrary number of drive periods. For resonant and near-resonant drives, the map has stable and unstable fixed points, which are the loci of infinite energy concentration in the long time limit. The Floquet map method can be applied both to classical and quantum massless field problems, including the dynamical Casimir effect. The stroboscopic time evolution implemented by the map can be interpreted in terms of the wave propagation in a curved space, with the fixed points of the map corresponding to the black hole and white hole horizons. More practically, the map can be used to design protocols for signal compression/decompression, cooling, and sensing.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Godiva IV central cavity neutron environment characterization with threshold neutron detectors

Godiva IV is a cylindrical fast burst reactor comprised of approximately 65 kg of highly enriched uranium that is operated by Los Alamos National Laboratory and sited at the National Criticality Experiments Research Center at the Nevada National Security Site in Nevada in the United States. Godiva IV is typically operated at delayed critical and in the regime spanning from sub-prompt to super-prompt bursts. Godiva IV is used for sample irradiations, criticality safety demonstrations, dosimetry studies, and for studying super-prompt behavior. In preparation for both an upcoming experiment to reduce uncertainties in the prompt fission spectrum for 235U using threshold neutron detectors, and for future research using Godiva IV, it was desired to exercise the process of the selection of threshold neutron detectors/activation foils, radiation metrology, and the subsequent adjustment of the neutron spectrum. For this exercise, nine high purity threshold neutron detectors/activation foils were irradiated in a Godiva IV burst. The foils were then analyzed using a high-purity germanium detector in the NCERC counting laboratory to determine end of irradiation specific activities for available IRDFF-II reactions. This work summarizes the Godiva IV foil irradiation, radiation metrology results, and adjusted neutron spectrum. The results of this exercise ultimately characterized the neutron environment inside the sample irradiation cavity inside Godiva IV to a higher degree than previously performed, informed decisions for the upcoming larger scale experiment, and will inform future neutron spectrum characterizations at NCERC.

Whitman, Nicholas H.↗

Weighted-density functionals for cavity formation and dispersion energies in continuum solvation models

Continuum solvation models enable efficient first principles calculations of chemical reactions in solution, but require extensive parametrization and fitting for each solvent and class of solute systems. Here, we examine the assumptions of continuum solvation models in detail and replace empirical terms with physical models in order to construct a minimally-empirical solvation model. Specifically, we derive solvent radii from the nonlocal dielectric response of the solvent from ab initio calculations, construct a closed-form and parameter-free weighted-density approximation for the free energy of the cavity formation, and employ a pair-potential approximation for the dispersion energy. We show that the resulting model with a single solvent-independent parameter: the electron density threshold (n{sub c}), and a single solvent-dependent parameter: the dispersion scale factor (s{sub 6}), reproduces solvation energies of organic molecules in water, chloroform, and carbon tetrachloride with RMS errors of 1.1, 0.6 and 0.5 kcal/mol, respectively. We additionally show that fitting the solvent-dependent s{sub 6} parameter to the solvation energy of a single non-polar molecule does not substantially increase these errors. Parametrization of this model for other solvents, therefore, requires minimal effort and is possible without extensive databases of experimental solvation free energies.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Sub-gigahertz beam switching of vertical-cavity surface-emitting laser with transverse coupled cavity

We report a high-speed electrical beam switching of vertical cavity surface emitting laser with a transverse coupled cavity. A high speed (sub-gigahertz) and large deflection angle (>30°) beam switching is demonstrated by employing the transverse mode switching. The angular switching speed of 900 MHz is achieved with narrow beam divergence of below 4° and extinction ratio of 8 dB. We also measured the near- and far-field patterns to clarify the origin of the beam switching. We present a simple one-dimensional Bragg reflector waveguide model, which well predicts the beam switching characteristic.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Piezoelectrically Tuned, Multimode Cavity Search for Axion Dark Matter

The eV axion is a well-motivated extension to the standard model. The Axion Dark Matter 27 eXperiment (ADMX) collaboration seeks to discover this particle by looking for the resonant con28 version of dark-matter axions to microwave photons in a strong magnetic eld. In this paper we 29 report results from an ADMX pathnder experiment, the ADMX \Sidecar", which is designed to 30 pave the way for future, higher mass, searches. The Sidecar experiment excludes masses in three 31 widely spaced frequency ranges (4202-4249 MHz, 5086-5799 MHz and 7173-7203 MHz), correspond32 ing to masses favored by some cosmic string simulations. In addition, Sidecar demonstrates the 33 successful use of piezoelectric actuators for both cavity tuning and antenna coupling. Finally, this publication is the rst to report data taken on both the TM010 and TM020 modes.

Boutan, Christian R.↗

Analysis of Planar-Cavity Receiver Reactor for Solar Thermochemical Dry-Reforming

Concentrating solar thermal (CST) systems can be leveraged to provide not only heat for power generation, but also for energy storage and thermochemical fuel production. Such solar thermochemical processes have been studied conceptually, from solar thermochemical hydrogen production (STCH) and thermochemical energy storage (TCES), to gasification, reforming, and fuel upgrading by various means. The solar receiver and reactor are critical components in the conversion of solar energy into chemical energy in the form of 'solar fuels'. For effective conversion of solar energy within a coupled solar receiver-reactor, extremely high temperatures are required, thereby demanding a high solar concentration ratio (CR) for efficient operation. This creates a design challenge for the receiver-reactor, as many thermochemical processes involve gas or gas-solid systems that are limited by low heat transfer coefficients. A unique receiver design is proposed that has the potential to incorporate various high-temperature thermochemical processes such as TCES-assisted power generation, methane reforming, or STCH processes. Modeling this receiver and its potential applications requires a full three-dimensional model that accurately captures the interconnected effects of receiver geometry, spatial solar irradiance, complex radiation, reaction kinetics, fluid dynamics, and heat transfer. In this paper we analyze a CST system integrated with this unique planar-cavity receiver-reactor design using the developed model. The model presented in this paper showed where improved thermal management was needed to achieve suitable receiver performance when a dry-methane reforming process is implemented.

14 SOLAR ENERGY↗

Demonstration of a rapidly-swept external cavity quantum cascade laser for rapid and sensitive quantification of chemical mixtures

A rapidly-swept external cavity quantum cascade laser (ECQCL) system for fast open-path quantification of multiple chemicals and mixtures is presented. The ECQCL system is swept over its entire tuning range (>100 cm-1) at frequencies up to 200 Hz. At 200 Hz the wavelength tuning rate and spectral resolution are 2x104 cm-1/sec and < 0.2 cm-1, respectively. The capability of the current system to quantify changes in chemical concentrations on millesecond timescales is demonstrated at atmospheric pressure using an open-path multi-pass cell. The detection limits for chemicals ranged from ppb to ppm levels depending on the absorption cross-section.

Brumfield, Brian E.↗

Heating Issues in NSLS-II Storage Ring Cavity Coupler (Heating issues in coupler for the superconducting cavity)

The superconducting RF cavity that is being adopted for the NSLS-II storage ring is based on the CESR-B cavity designed by Cornell University. The external Quality Factor (Q ext ) for the original Cornell design is 225,000. NSLS-II design requires a Qext of 65,000. The coupler design has been modified to make the Q ext ≈ 65,000 using HFSS. Any possible issues with conductor heating in the coupler region was analyzed using ANSOFT thermal analysis. This document describes the procedure used to perform the analysis and discusses the results.

42 ENGINEERING↗

Impedance simulation for LEReC booster cavity transformed from ERL gun cavity

Wake impedance induced energy spread is a concern for the low energy cooling electron beam. The impedance simulation of the booster cavity for the LEReC projection is presented in this report. The simulation is done for both non-relativistic and ultra-relativistic cases. The space charge impedance in the first case is discussed. For impedance budget consideration of the electron machine, only simulation of the geometrical impedance in the latter case is necessary since space charge is considered separately.

43 PARTICLE ACCELERATORS↗

Design and characterization of an electromagnetic-resonant cavity microwave plasma reactor for atmospheric pressure carbon dioxide decomposition

Plasma processes are ideally suited for the conversion of renewable electricity into gas-phase reactivity, such as for the decomposition of carbon dioxide (CO 2 ). The design, development, and characterization of a microwave plasma reactor for atmospheric pressure undiluted carbon dioxide decomposition are presented. The reactor operates as an electromagnetic-resonant cavity in which the generated plasma forms a bulb attached to a converging-diverging nozzle and stabilized by streams of tangentially-injected processing gas. Electromagnetic wave confinement, residence time, and critical gas vorticity constitute fundamental reactor sizing and operation parameters. Experimental findings demonstrate that flow rate plays a dual role in plasma stabilization and process performance, whereas deposited power has a minor role in CO 2 decomposition.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Imaging of dark line defect growth in high-power diode laser cavities using broadband near infrared light emission from the laser cavity

An in situ and nondestructive technique is developed to image the formation and evolution of dark line defects in the cavity of a high-power diode laser. Here, the technique uses broadband near infrared emission that originates in the laser's core layers and enables defects to be imaged with high spatial resolution through the substrate. In particular, it enables defect imaging through the substrate of shorter wavelength lasers, even when the substrate is opaque near the lasing wavelength. The evolution of dark line defects during aging is studied in several devices, with correlations established between the observed characteristics of defect growth and changes in device parameters such as optical power, operating wavelength, threshold current, and slope efficiency. Gradual degradation is found to be associated with dark line defects that slowly propagate from dark spots that are present in the device interior in its fresh (unaged) condition, rather than propagating from spots that are formed during aging, suggesting a strategy to screen fresh devices for expected reliability. This defect growth phenomenon is found to be particularly evident in the dark spots near the output facet.

47 OTHER INSTRUMENTATION↗

Effect on cavity optomechanics of the interaction between a cavity field and a one-dimensional interacting bosonic gas

We investigate optomechanical coupling between one-dimensional interacting bosons and the electromagnetic field in a high-finesse optical cavity. We show that by tuning interatomic interactions, one can realize effective optomechanics with mechanical resonators ranging from side-mode excitations of a Bose-Einstein condensate (BEC) to particle-hole excitations of a Tonks-Girardeau (TG) gas. We propose that this unique feature can be formulated to detect the BEC-TG gas crossover and measure the sine-Gordon transition continuously and nondestructively.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Photon Antibunching from Few Quantum Dots in a Cavity

Single quantum dots (QDs) are frequently used as single-photon sources, taking advantage of the final exciton decay in a cascade that produces energetically detuned photons. We propose and analyze a new concept of single-photon source, namely, a few-QD microcavity system driven close to, but below the lasing threshold under strong excitation. Surprisingly, even for two or three QDs inside a cavity, antibunching is observed. To quantify the results, we find that a classification of single-photon emission in terms of antibunching in the autocorrelation function g (2) (0) is insufficient and more details of the photon statistics are required. Our investigations are based on a quantum-optical theory that we solve to obtain the density operator for the quantum-mechanical active medium and radiation field.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Starting dynamics of a linear-cavity femtosecond Mamyshev oscillator

Mamyshev oscillators can generate high-power femtosecond pulses, but starting a mode-locked state has remained a major challenge due to the suppression of continuous-wave lasing. Here, we study the starting dynamics of a linear Mamyshev oscillator designed to generate high-power femtosecond pulses while avoiding component damage. Reliable starting to stable mode-locking is achieved with a combination of modulation of the pump power and shifting of a filter passband. The starting process is automated, with full electronic control. The laser delivers 21-nJ pulses that are dechirped to 65 fs in duration outside the cavity.

Chen, Yi-Hao (ORCID:0000000244001983)↗

Real-time standoff detection of nitrogen isotopes in ammonia plumes using a swept external cavity quantum cascade laser

A swept-wavelength external cavity quantum cascade laser is used to measure time-resolved 15NH3 and 14NH3 concentrations and isotope ratios in a turbulent plume source located at 10 m standoff distance. Measurements show excellent agreement with expected values of isotope ratios for samples with natural and enriched 15N abundance. Detection sensitivity of 150 ppb*m is demonstrated for a 50 ms measurement interval, improving to 10 ppb*m with 10 s averaging, with isotopic precision as good as 0.8%.

Phillips, Mark C.↗