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Development and Application of Weld Track Thermal Analysis for the Exploration Extravehicular Mobility Unit

NASA is studying the next generation of space suit for safe operations in space, from the International Space Station to the lunar surface as part of the Exploration Extravehicular Mobility Unit project. The backplate structure of the portable life support system (PLSS) serves as the attachment point for assembly of the PLSS and contains embedded cooling channels. The thermal loop plumbing assembly and backplate are combined into a single component such that the fluid lines run through the midplane of the backplate. The manufacturing of the Ti-6Al-4V backplate consists of machining channels into a plate, welding cover plates on each channel using an electron beam, and additional machining for excess material removal and final detail. Careful control of the electron beam weld process is necessary to completely seal cover plates, produce consistent weld tracks, and produce channels with uniform cross sections free of debris and defects. The backplate contains multiple weld channels with unique geometries. The weld process parameters include choosing the beam current and focus, accelerating voltage, travel speed, pause times between weld tracks, and sequence of weld tracks. A transient finite element thermal analysis was developed to provide support for choosing and controlling the weld process parameters to maintain a consistent melt pool along each of the weld tracks. A moving distributed heat source is modeled to represent the heat input generated by the electron beam. The heat source model is a critical input to the analysis for accurate temperature predictions during the weld process. A modified conical heat source was developed to account for the change in working distance between the backplate and cover plates. The geometry of the material being welded must be accounted for by the heat source model to define the correct energy input. The weld process control is designed according to the predicted thermal history and melt pool dimensions for each of the weld channels. The analysis model, modified heat source, temperature and melt pool predictions, application of the thermal data to the weld parameters, and comparison with micrograph cross-sections from weld trials will be discussed in this presentation.

Electron Beam Welding↗

The new ITER baseline, research plan and open R&D issues

A new baseline (NB) has been proposed by the ITER Project to ensure a robust achievement of the Projects’ goals, in view of past challenges including delays incurred due to the Covid-19 pandemic, technical challenges in completing first-of-a-kind components and in nuclear licensing. The NB includes modifications to the configuration of the ITER device and its ancillaries (e.g. change from beryllium to tungsten as first wall material, modification of the heating and current drive mix, etc.) as well as additional testing of components (e.g. toroidal field coils) or phased installation (start with inertially cooled first wall before later installation of the final actively water-cooled components) to minimise operational risks. In the NB, the ITER research plan (IRP) will be divided into three main phases: (a) start of research operation, with 40 MW of ECH and 10 MW of ICH, which will focus on the demonstration of 15 MA operation in L-mode, commissioning of all required systems, including disruption mitigation, and the demonstration of H-mode plasma operation in deuterium; (b) DT-1, with 60–67 MW of ECH, 33 MW of neutral beam injection (NBI) and 10–20 MW of ICH, which will demonstrate robust operation in high confinement H-mode plasmas in DT up to Q ⩾ 10 and for burn durations of 300–500 s within an accumulated neutron fluence of ∼1% of the ITER machine’s lifetime total, and; (c) DT-2, with up to 67 MW of ECH, up to 49.5 MW of NBI and up to 20 MW of ICH, with the ITER tokamak and ancillaries in their final configuration to demonstrate routine operation in DT plasmas at high Q and the Q ⩾ 5 long-pulse and steady-state scenarios to the final neutron fluence and to perform R&D on nuclear fusion reactor issues. The logic, physics basis, modelling and experimental evaluations carried out to support the NB and the associated IRP are described. These include the impact of the tungsten wall on plasma scenarios and associated risk mitigation measures, as well as the optimisation of the tokamak components and ancillaries to minimise Project risks. Open R&D issues related to these evaluations and mitigation measures are also described together with experimental, modelling and validation activities required to address them.

ITER↗

Research in Neutrino Physics (Final Technical Report)

The goal of the experimental neutrino efforts at Louisiana State University is to measure the properties of neutrinos and to improve our understanding of neutrino interactions. In pursuit of this goal, the group will continue its Intensity Frontier work on the DUNE experiment at Fermilab and the T2K experiment at J-PARC, Japan. The current work is focused on understanding how neutrinos change flavor and on the possibility for asymmetry between neutrinos and anti-neutrinos. The effort on T2K includes physics measurements using the collected T2K data and preparation for the second phase T2K-II data with an increased beam power and the newly upgraded ND280 detector, featuring a novel 3D fine grained scintillation tracker with 4π acceptance and 3D readout. T2K is in a position to improve our understanding of neutrino nucleus interactions which continue to be one of the largest systematic uncertainties for neutrino oscillation measurements. On DUNE, the effort is on analyzing the data collected by the ProtoDUNE-SP prototype at CERN and on the design, installation, and commissioning of ProtoDUNE-II and later the DUNE Far Detector cold electronics. The final DUNE Module-1 components will be fully characterized by ProtoDUNE-II and the collected data will be used to improve and tune simulation and reconstruction algorithms, and to measure hadron scattering cross section, used to improve the modeling of neutrino final state interactions.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Magnets for a Muon Collider—Needs and Plans

We describe the magnet challenges for a Muon Collider, an exciting option considered for the future of particle physics at the energy frontier. Starting from the comprehensive work performed by the US Muon Accelerator Program, we have reviewed the performance specifications dictated by beam physics and the operating conditions to satisfy the accelerator needs. Among the many magnets that make up a muon collider, we have identified four systems that represent well the envelope of challenges: the target and capture solenoid, the final cooling solenoid, the accelerator dipoles and the collider dipoles. These systems provide focus for the development of novel concepts, largely based on HTS for reasons of performance, cost and sustainability. After giving a consolidated overview of the needs for the magnet systems, we describe here the basic technology options considered, and the plan for design and development activities.

43 PARTICLE ACCELERATORS↗

The Atacama Cosmology Telescope: Beam Measurements and the Microwave Brightness Temperatures of Uranus and Saturn

We describe the measurement of the beam profiles and window functions for the Atacama Cosmology Telescope (ACT), which operated from 2007 to 2010 with kilopixel bolometer arrays centered at 148, 218, and 277 GHz. Maps of Saturn are used to measure the beam shape in each array and for each season of observations. Radial profiles are transformed to Fourier space in a way that preserves the spatial correlations in the beam uncertainty to derive window functions relevant for angular power spectrum analysis. Several corrections are applied to the resulting beam transforms, including an empirical correction measured from the final cosmic microwave background (CMB) survey maps to account for the effects of mild pointing variation and alignment errors. Observations of Uranus made regularly throughout each observing season are used to measure the effects of atmospheric opacity and to monitor deviations in telescope focus over the season. Using the WMAP-based calibration of the ACT maps to the CMB blackbody, we obtain precise measurements of the brightness temperatures of the Uranus and Saturn disks at effective frequencies of 149 and 219 GHz. For Uranus we obtain thermodynamic brightness temperatures T(149/U) = 106.7 +/- 2.2 K and T(219/U) = 100.1 +/- 3.1 K. For Saturn, we model the effects of the ring opacity and emission using a simple model and obtain resulting (unobscured) disk temperatures of T(149/S) = 137.3 +/- 3.2 K and T(219/S) = 137.3 +/- 4.7 K.

Atacama Cosmology Telescope (ACT)↗

Collaborative R&D with REEL Solar Inc (REEL) to Understand and Overcome Performance Limitations in CdTe Solar Cells: Cooperative Research and Development (Final Report)

This CRADA will focus on processing, advanced characterization, and testing of photovoltaic materials and devices to understand and improve REEL CdTe solar technology. This will include examining process variations and different buffer, absorber, and contact layers from REEL and NLR to maximize performance. The unique and diverse advanced characterization tools at NLR, such as time-resolved photoluminescence, capacitance-voltage measurements, electron beam scattered diffraction, cathodoluminescence, electron microscopy, TOF-SIMS, and other measurements will be applied to characterize REEL processing to improve understanding and guide experimental directions. Accelerated stability and potential induced degradation tests will be used to analyze metastability, short-and-long term degradation, and improve bankability. A second and major thrust this period will be joint development of Si/CdTe tandem solar cells to overcome industry wide terrestrial solar efficiency limits with the two lowest cost and manufacturable solar materials today. This will include developing novel transparent back contacts that can be incorporated into tandem structures and other novel solar applications, detailed analysis of designs and configurations for CdTe/Si tandem modules, and prototyping REEL CdTe Technology with Si bottom cells in tandem structures.

14 SOLAR ENERGY↗

Microscopic and Metallurgical Aspects of the Space Shuttle Columbia Accident Investigation and Reconstruction

The Space Shuttle Columbia was descending for a landing at the Kennedy Space Center (KSC) on February 1, 2003. Approximately 20 minutes prior to touchdown, the Columbia began disintegrating over the western United States; the majority of debris eventually impacted in eastern Texas and western Louisiana. A monumental effort eventually recovered approximately 84,000 pieces of debris, approximately 38% of the Orbiter's original dry weight. The debris was transported to KSC, where the items were catalogued and evaluated. Critical areas of interest, such as the left and right leading edge surfaces and the underside of the ship, were placed upon a grid to aid in the reconstruction. Items of interest included metallic structures, reinforced carbon-carbon composites, and ceramic heat insulation tiles. Many of the leading edge elements had re-solidified metallic deposits spattered on them. These deposits became known as slag and were one of the main focuses of the investigation. In order to help determine the sequence of events inside the left wing during the accident, the slag's composition, layering order, and directionality of deposition were studied. A myriad of analytical tests were performed in an attempt to ascertain the compositional and depositional characteristics of selected slag deposits, including the ordering of deposited layers within each individual slag deposit harvested. Initially, Scanning Electron Microscopy and Energy Dispersive X-Ray Spectroscopy (SEM/EDX) were performed to quickly characterize the overall composition of individual slag deposits: SEM utilizes a narrowlyfocused high-energy electron beam impinging upon a specimen. The incident beam excites and liberates lower energy secondary electrons, which are detected and analyzed, providing a visual representation of the sample's surface topography. EDX also relies on an incident electron beam, except an EDX unit measures X-ray energies generated by the impinging beam. Each element generates a unique X-ray signature; the EDX detector measures these discreet energies. EDX actually penetrates approximately 2 microns into the bulk of the sample. However, random examination of various portions of slag, coupled with the semiquantitative nature of the SEM/EDX analysis, did not yield convincingly pertinent data. Therefore, X-ray dot mapping was conducted, which provided more understandable data, both in terms of slag layering and composition. An X-ray dot map is generated by performing numerous EDX scans for individual elements, then compiling the scans in a visual representation. Eventually, specimens consisting of not only the slag, but of the adjacent RCC substrate as well were cross-sectioned. X-Ray dot mapping of the materialographicallymounted and -polished cross- sections provided a visual representation of both the layering sequence and compositional characteristics of the slag. Contemporaneously, Electron Spectroscopy for Chemical Analysis/X-Ray Photoelectron Spectroscopy (ESCA/XPS) and powdered X-Ray Diffraction (XRD) were performed to further characterize the deposits and to attempt to identify what, if any, compounds were present. The ESCA/XPS analysis allowed the analyst to "sputter" into the sample with an electron gun, aiding in the identification of the layering sequence. XPS uses photons, rather than electrons, which impinge upon the surface of the sample. XPS measures the electrons emitted from within the first 5 nm of the sample's surface. The XRD measures the scatter angles of incident X-rays; the angle and intensity of scatter depend upon the crystalline structure of the pulverized sample. XRD is considered a qualitative rather than quantitative technique. ESCA/XPS revealed that the final layer to deposit was predominantly carbonaceous. XRD was successful in identifying specific compounds, such as Al 2O3, Al and/or Al3 21SiO47, mullite (3(Al2)O3 -SiO2), and nickel-aluminides. Eventually, Electron MicroProbe Analysis (EMPA) was conducted on the marialographically-prepared cross- sections of selected slag deposits. Microprobe combines SEM and Wavelength Dispersive X-Ray Spectroscopy (WDS), and, like EDX, uses a narrowly-focused high-energy electron beam impinging upon a specimen to elicit, in the case of EPMA, characteristic X-rays with specific wavelengths. This quantitative, analytical tool proved the most useful in determining depositional layering and composition of the slag deposits. This information was utilized in verifying the location of the breach in the left leading edge of the wing of the Columbia.

McDaniels, Steven J.↗

Investigating Interference Term in DUNE And SBND Neutrino Interactions with ACHILLES

Understanding neutrino-nucleus interactions is critical for conducting precise neutrino oscillation ex- periments. However, uncertainties in neutrino-nucleus cross section measurements and our incomplete understanding of nuclear effects remain a significant challenge in neutrino physics. In this paper, we investigate contributions from quantum interference between one-body and two-body interactions in charged-current quasi-elastic (CCQE) neutrino scattering amplitudes, using the ACHILLES event gen- erator. Simulations are performed using muon neutrino flux from Fermilab’s Booster Neutrino Beam (BNB), as well as Long-Baseline Neutrino Facility (LBNF) flux. We observe the neutrino flux interact- ing with Argon nuclei as detected by the Short Baseline Near Detector (SBND) and DUNE Near Detector (DUNE-ND), both Liquid Argon Time Projection Chambers (LArTPC). We focus on one muon and one proton final states with cascade interactions. We analyze multiple experimental observables including outgoing kinematic variables, energy-momentum transfer variables, and Transverse Kinematic Imbalance (TKI) variables. In this study, we also investigate the effects of PRISM (a method of sampling flux from multiple off-axis angles which creates different neutrino energy spectra). We find that the ratio of in- terference to quasi-elastic contributions gives a non-flat distribution across a 0-3.5 GeV energy range, indicating that effects of interference vary with the neutrino energy sampled. Our ultimate goal is to reduce systematic uncertainties from neutrino interactions when conducting oscillation experiments by working to disentangle the effects of quantum interference from the quasi-elastic signature.

Serumaga, Peera [Fermilab; UC, San Diego] (ORCID:0↗

Neutrinos and Dark Matter Across Energies and Epochs (Final Technical Report)

The opportunities afforded by upcoming next-generation neutrino experiments offer new physics potential that is complementary to high-energy collider searches. Although much lower in energy, the combination of large detectors and high intensity proton beams yields novel sensitivity to new physics. The types of new physics signals include both those which are terrestrially sourced as well as astrophysically produced. Within this project specific focuses include: (1) BSM searches at neutrino and dark matter experiments to look for axion-like particles, heavy neutrinos, and new force carriers; and (2) BSM signals from astrophysics.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Multibeam Electron Diffraction

One of the primary uses for transmission electron microscopy (TEM) is to measure diffraction pattern images in order to determine a crystal structure and orientation. In nanobeam electron diffraction (NBED), we scan a moderately converged electron probe over the sample to acquire thousands or even millions of sequential diffraction images, a technique that is especially appropriate for polycrystalline samples. However, due to the large Ewald sphere of TEM, excitation of Bragg peaks can be extremely sensitive to sample tilt, varying strongly for even a few degrees of sample tilt for crystalline samples. In this paper, we present multibeam electron diffraction (MBED), where multiple probe-forming apertures are used to create multiple scanning transmission electron microscopy (STEM) probes, all of which interact with the sample simultaneously. We detail designs for MBED experiments, and a method for using a focused ion beam to produce MBED apertures. We show the efficacy of the MBED technique for crystalline orientation mapping using both simulations and proof-of-principle experiments. We also show how the angular information in MBED can be used to perform 3D tomographic reconstruction of samples without needing to tilt or scan the sample multiple times. Finally, we also discuss future opportunities for the MBED method.

47 OTHER INSTRUMENTATION↗

Neutron Calibration Studies for the SuperCDMS SNOLAB Experiment

My time at Fermilab has been dedicated to advancing the field of dark matter detection through my contributions to the SuperCDMS collaboration. The first project involved the development and testing of a delivery system for a Cf-252 neutron source to calibrate the SuperCDMS silicon and germanium detectors. Subsequently, I focused on parametrizing the detectors' instrumental response by optimizing a plastic scintillator backing array to measure the scattering angle of a collimated neutron beam. The Monte Carlo simulation I designed provided insights into the detection efficiency of the array, and the best-fit design I arrived at for the scattering counters will be implemented into the final array. Additionally, I assembled a muon detector with legacy hardware to enhance the ability of the calibration experiment to reduce dark current and false signals. As my work nears completion, I am confident that these contributions will significantly enhance the precision and reliability of the SuperCDMS experiment, pushing the boundaries of our understanding of dark matter and contributing to the broader scientific community's quest to unravel the mysteries of the universe.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Theory and Simulation of Ultrafast Multidimensional Nonlinear X-ray Spectroscopy of Molecules (Final Report)

Emerging X-ray free electron laser (XFEL) beam sources offer new types of probes of matter with unprecedented spatial and temporal resolutions. These experimental advances must be met by robust theoretical and computational tools that provide predictive modeling capacity of the underlining electronic and structural dynamics. The latter will be essential for the design of sophisticated multi-pulse experiments and for their interpretation. The proposed research effort will focus on developing cutting- edge simulation tools for nonlinear multidimensional X-ray/optical spectroscopies and aims to address key questions in Priority Research Opportunities 1 (Probing and controlling electron motion within a molecule) and 3 (Capturing rare events and intermediate states in the transformation of matter) as mentioned in the BES Roundtable Report “Opportunities for Basic Research at the Frontiers of XFEL Ultrafast Science”. XFEL multidimensional nonlinear techniques, which combine sequences of X-ray and possibly optical pulses, provide a unique experimental toolbox for probing the dynamics of core and valence electronic excitations, as well as material structure. Predictive modeling of these dynamical processes requires the combination of analytical theory for nonlinear interactions of light and matter, robust quantum-chemical methodologies for the accurate description of electronic structure of various materials, and multiscale ab initio electron and nuclear dynamics techniques operating beyond Born-Oppenheimer approximation. These challenges will be addressed with three research thrusts (i) Develop and implement theoretical apparatus for modeling a broad range of multidimensional spectroscopic techniques enabled by present and upcoming XFEL facilities. This thrust also includes the incorporation of a computational module in the DOE supported open-source NWChem computational chemistry package as well as the development of other open-source codes ready for dissemination across a broad user base; (ii) Propose and design new multi-pulse experiments that make use of the capabilities of the incoming LCLS-II facility; (iii) Perform selected applications to specific molecular systems that can be carried out at LCLS-II and demonstrate how these X-ray sources may be used to study nonadiabatic dynamics through conical interactions, electronic correlations in multi-core excitons, and charge transfer/energy transfer processes. The proposed research will be carried out by a multi-disciplinary four-institution research team which combines academia and national laboratories and spans the broad and necessary expertise in theoretical spectroscopy, nonlinear optics, quantum chemistry, molecular non-adiabatic dynamics and code development. The work will be performed in a highly interactive team environment with junior researchers shared between institutions thus cementing cross- disciplinary interactions. The developed simulation tools will be immediately deployed for XFEL facility users, both experimentalists and theorists, via freely distributed codes and databases. Altogether, this project will facilitate establishing XFEL-based multidimensional spectroscopies as a novel diagnostic tool for monitoring electronic and structural dynamics in molecular materials.

74 ATOMIC AND MOLECULAR PHYSICS↗

Millimeter-wave beam scattering and induced broadening by plasma turbulence in the TCV tokamak

The scattering of millimeter-wave beams from electron density fluctuations and the associated beam broadening are experimentally demonstrated. Using a dedicated setup, instantaneous deflection and (de-)focusing of the beam due to density blobs on the beam path are shown to agree with full-wave simulations. The detected time-averaged wave power transmitted through the turbulent plasma is reproduced by the radiative-transfer model implemented in the WKBeam code, which predicts a ~50% turbulence-induced broadening of the beam cross-section. Finally, the role of core turbulence for the considered geometry is highlighted.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Tolerance Studies for the IMCC Rectilinear 6D Ionization Cooling Channel

As one of the main proposed future colliders that will enable us to reach energy scales capable of probing Beyond the Standard Model phenomena, muon colliders present unique challenges. To reach the desired luminosity, namely 1, 10, and 20 ab-1 for 3, 10, and 14 TeV, respectively, the six-dimensional emittance of the muon beam needs to be reduced significantly in a process described as muon cooling. The currently proposed system for muon cooling by the International Muon Collider Collaboration involves 6D initial cooling post-muon charge separation through rectilinear channels (A) before and rectilinear channels (B) after muon bunch merge, as well as a final 4D transverse cooling. This work focuses on the former stage of cooling with B rectilinear channels. First, we will compare its cooling performance against the rectilinear channel studied by the Muon Accelerator Program. Then, we do tolerance studies on all B stages, focusing on properties of the Radiofrequency (RF) cavities used in the channels and how they affect 6D emittance and transmission. We will evaluate the impact of these modifications on the overall performance of the rectilinear 6D cooling channel.

Karaaslan, Inci [Chicago U., EFI] (ORCID:000000033↗

Research in large adaptive antenna arrays

The feasibility of microwave holographic imaging of targets near the earth using a large random conformal array on the earth's surface and illumination by a CW source on a geostationary satellite is investigated. A geometrical formulation for the illuminator-target-array relationship is applied to the calculation of signal levels resulting from L-band illumination supplied by a satellite similar to ATS-6. The relations between direct and reflected signals are analyzed and the composite resultant signal seen at each antenna element is described. Processing techniques for developing directional beam formation as well as SNR enhancement are developed. The angular resolution and focusing characteristics of a large array covering an approximately circular area on the ground are determined. The necessary relations are developed between the achievable SNR and the size and number of elements in the array. Numerical results are presented for possible air traffic surveillance system. Finally, a simple phase correlation experiment is defined that can establish how large an array may be constructed.

Berkowitz, R. S.↗

Gas Stopper Developments for Improved Purity and Intensity of Low-Energy, Rare Isotope Ion Beams (Final Technical Report)

This final technical report summarizes the work of the Michigan State University (MSU) team supported by grant # DE-SC0021423 awarded by the Office of Nuclear Physics, Department of Energy. Objectives: The successful fulfillment of the FRIB science mission hinges on ensuring the availability of fast, stopped, and reaccelerated beams consisting of rare isotopes. This project's research and development focus was dedicated to supporting the advancement and creation of a cutting-edge linear gas stopper. The primary aim is to efficiently convert the high-intensity fast beams of rare isotopes provided by FRIB into high-quality, low-energy beams. These beams are essential for conducting stopped beam experiments or for subsequent reacceleration. The overarching goal is to advance technology, aiming to increase the beam rate capability of the linear gas stopper for medium-to-heavy-mass rare isotopes by more than tenfold compared to the currently most effective gas stopper in operation, and to improve the purity of the delivered beams. Project Description: The existing technology employed in gas stopping devices designed for low-energy, rare-isotope beams presents limitations in both the purity of extracted beams and the intensities of injected beams. These limitations are incompatible with the requirements of the recently commissioned rare isotope beam facility, FRIB. Our research and development efforts, aligned with the previously outlined objectives, focused on addressing the most critical aspects for enhancing beam-rate capability and purity. Specifically, advanced particle-in-cell simulations were developed and integrated into a simulation pipeline to explore the efficacy of multi-layer RF carpets on increasing ion transport efficiency with high incoming beam rates that generate space charge fields which can limit it. We also explored the possibility of using a collision-induced-dissociation (CID) gas cell to break up molecular contaminant ions that are generated during the stopping process. A prototype CID gas cell was constructed and tested with beams from an offline ion source, validating the concept with the successful demonstration of breaking of molecular ions. The outcome of this research enabled the formulation a conceptual design for a next-generation linear gas stopping device specifically tailored for FRIB. This device is envisioned to deliver rare-isotope-ion beams at a rate of 10 8 particles per second or higher, accompanied by advancements in purity. Methods employed: This project leverages advancements in technologies initially designed for the Advanced Cryogenic Gas Stopper (ACGS), the current state-of-the-art linear gas stopper, through the use of new simulations and beam purification via collision-induced-dissociation. The methods include: 1. Development of a prototype low-energy, low-pressure CID gas stopper. This prototype features a thin, approximately 20 nm, Si 3 N 4 entrance window designed for dissociating stable and rare-isotope molecular ions. The goal is to enhance beam purification and overall efficiency. 2. Creation of Particle-in-cell (PIC) simulations to assess the advantages of multi-layer RF carpets and multi-point extraction for ion transport efficiency. These simulations rely on the 3DCylPIC package, specifically designed for studying devices of this nature. The goal is to quantify and mitigate ion transport losses due to space charge generated in the stopping process of large numbers of ions. 3. Perform ion transport simulations across an RF carpet using an 8-phase travelling wave and evaluate its performance. Compared to the 4-phase RF carpets used in ACGS, the 8-phase carpets will double the wavelength of the generated traveling wave allowing for larger maximum RF amplitudes that could result in improved ion transport efficiency for high-intensity incoming beams when large space charge fields are present. Impact: Tackling the primary challenges associated with transforming high-energy projectile fragment beams into low-energy beams—specifically, addressing efficiency and purity—holds significant promise for advancing FRIB science. This advancement will particularly impact precision mass measurements, laser spectroscopy of short-lived nuclei, and studies in astrophysics and nuclear reactions using reaccelerated beams. These domains play a crucial role in addressing key questions outlined in the 2023 NSAC long-range plan, spanning nuclear structure, nuclear astrophysics, and fundamental symmetries. Additionally, they contribute to addressing 10 out of the 17 benchmarks identified by the NRC RISAC. The development of a next-generation gas stopping device capable of delivering low-energy, rare-isotope beams at a rate of 10 8 particles per second, or more, with high purity holds the potential to unlock experiments that would otherwise be unfeasible. Furthermore, it is expected to reduce the time required for experiments at FRIB, thereby maximizing scientific output. The research and development activities performed as part of this project bolstered essential competencies at FRIB in beam physics and ion source technologies, provided valuable training opportunities for junior scientists.

43 PARTICLE ACCELERATORS↗

Monolithic Spatial Heterodyne Raman Spectrometers (mSHRS): Toward highly miniature chemical sensors for deployment on moving platforms (Final Report, Phase I)

This report covers phase 1 (year 1) of the mSHRS project. Our ultimate long-term goal is to develop highly miniature Raman analyzers, known as spatial heterodyne Raman spectrometers (SHRS), that are deployable as in-situ chemical sensors on moving platforms. During Phase I (FY19/20) funding, our team focused our efforts solely on the key innovation needed toward realizing that goal: the development of the monolithic interferometer comprising the beam splitter and gratings with the appropriate design parameters and tolerances to enable Raman interferometry. We successfully developed and characterized the performance of the first monolithic SHRS devices including a monolithic version that incorporates field-widened optics. Our solid-state design approach integrated all optical components as a single monolithic unit for maintaining precise optical alignment during sensor operation, a requirement for operating in a vibration prone environment. This project has two principle activities: (1) Design and fabricate monolithic SHRS devices (i.e. monolithic device task) and (2) characterize the mSHRS devices in terms of performance (i.e. the Monolithic SHRS characterization task).

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Progress and Challenges of Additive Manufacturing of Tungsten and Alloys as Plasma-Facing Materials

Tungsten (W) and W alloys are considered as primary candidates for plasma-facing components (PFCs) that must perform in severe environments in terms of temperature, neutron fluxes, plasma effects, and irradiation bombardment. These materials are notoriously difficult to produce using additive manufacturing (AM) methods due to issues inherent to these techniques. The progress on applying AM techniques to W-based PFC applications is reviewed and the technical issues in selected manufacturing methods are discussed in this review. Specifically, we focus on the recent development and applications of laser powder bed fusion (LPBF), electron beam melting (EBM), and direct energy deposition (DED) in W materials due to their abilities to preserve the properties of W as potential PFCs. Additionally, the existing literature on irradiation effects on W and W alloys is surveyed, with possible solutions to those issues therein addressed. Finally, the gaps in possible future research on additively manufactured W are identified and outlined.

36 MATERIALS SCIENCE↗