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DOE OSTI2025

Observation of Orbital-Selective Dual Modulations in an Anisotropic Antiferromagnetic Kagome Metal TbTi 3 ⁢Bi 4

Orbital selectivity is pivotal in dictating the phase diagrams of multiorbital systems, with prominent examples including the orbital-selective Mott phase and superconductivity. The intercalation of anisotropic layers represents an effective method for enhancing orbital selectivity and thereby shaping the low-energy physics of multiorbital systems. Despite its potential, related experimental studies, especially those elucidating the correlation between orbital selectivity and magnetism, remain limited. In this work, we systematically examine the interplay between orbital selectivity and magnetism in the newly discovered anisotropic kagome TbTi 3 ⁢Bi 4 single crystal, and report the coexistence of orbital-selective dual-band modulations (𝑞 1 ∼ 1/3⁢𝑎*, 𝑞 2 ∼ 0.28⁢𝑏*) within the antiferromagnetic (AFM) state. By combining soft x-ray and vacuum ultraviolet angle-resolved photoemission spectroscopy measurements, neutron powder diffraction, scanning tunneling microscopy, and density-functional-theory calculations, we identify these dual-band reconstructions as manifestations of the AFM order driven by a (approximately 1/3, 0.28, 0) nesting instability of the intercalated Tb 5⁢𝑑 𝑥⁢𝑧 orbitals. These orbital-selective modulations induce unusual momentum-dependent band folding and lead to the emergence of Dirac cones only at the $\bar{M}$ 1 point, signaling a topological phase transition in the AFM state. Importantly, the discovery of orbital-selective (approximately 1/3, 0.28, 0) AFM order offers crucial insights into the mechanism underlying the fractional magnetization plateau in this kagome AFM metal. Our findings not only underscore the essential role of both conducting and localized electrons in determining the magnetic orders of Ln⁢Ti 3 ⁢Bi 4 (Ln = lanthanide) kagome metals but also offer a pathway for manipulating magnetism through selective control of anisotropic electronic structures.

Zhang, Renjie [Shanghai Jiao Tong University (Chin↗

DOE OSTI2025

Anisotropic Thermal Transport in Quasi-2D Ruddlesden-Popper Hybrid Perovskite Superlattices

Two-dimensional hybrid metal-halide perovskites (2D-MHPs) have emerged as important solution-processed semiconductors with favorable optical and electronic properties for diverse applications in photovoltaics, optoelectronics, and spintronics. The quasi-2D layered structures, featuring large acoustic impedance mismatches between the organic and inorganic sublattices, are expected to result in distinct and anisotropic thermal transport properties along the cross-plane and in-plane directions. Here, we introduce transducer-free vibrational-pump-visible-probe (VPVP) approaches that enable accurate quantification of anisotropic thermal transport properties in various archetypical single-crystalline 2D-MHPs. Specifically, using VPVP spectroscopy and VPVP microscopy, we measure the anisotropic thermal diffusivities of 2D-MHPs with systematically varied Pb-I octahedral layer thicknesses, as well as organic spacer types and lengths, revealing how these structural parameters alter the cross-plane and in-plane thermal transport properties in distinct ways. While diffuse interface scattering plays an important role in dictating cross-plane thermal transport, in-plane thermal transport is primarily determined by phonon transport within interconnected inorganic layers. Density functional theory incorporating four-phonon scatterings provides further insight into the low thermal conductivity and modest thermal conduction anisotropy in 2D-MHPs. Our work demonstrates a new all-optical and noncontact method, which requires minimal sample preparation and allows direct visualization of cross-plane and in-plane thermal transport, potentially compatible with sample environments. The demonstrated VPVP approaches can advance understanding of thermal transport in 2D-MHPs as well as wide-ranging hybrid and polymeric semiconductors beyond 2D-MHPs.

36 MATERIALS SCIENCE↗

DOE OSTI2021

Temperature dependence of London penetration depth anisotropy in superconductors with anisotropic order parameters

Here, we study the effects of anisotropic order parameters on the temperature dependence of London penetration depth anisotropy γ λ ( T ) . After MgB 2 , this dependence is commonly attributed to distinct gaps on multiband Fermi surfaces in superconductors. We have found, however, that the anisotropy parameter may depend on temperature also in one-band materials with anisotropic order parameters Δ ( T , k F ) ; a few such examples are given. We have also found that for different order parameters, the temperature dependence of Δ ( T ) / Δ ( 0 ) can be represented with good accuracy by the interpolation suggested by Einzel, which simplifies considerably the evaluation of γ λ ( T ) . Of particular interest are mixed order parameters of two symmetries for which γ λ ( T ) may go through a maximum for a certain relative weight of two phases. Also, for this case we find that the ratio Δ max ( 0 ) / T c may exceed substantially the weak-coupling limit of 1.76. It, however, does not imply strong coupling; rather, it is due to significantly anisotropic angular variation of Δ .

36 MATERIALS SCIENCE↗

DOE OSTI2021

Comprehensive anisotropic linear optical properties of the Weyl semimetals TaAs and NbAs

We report that TaAs and NbAs are two of the earliest identified Weyl semimetals that possess many intriguing optical properties, such as chirality-dependent optical excitations and giant second harmonic generation (SHG). Linear and nonlinear optics have been employed as tools to probe the Weyl physics in these crystals. Here, we extend these studies to address two important aspects: determining the complete anisotropic dielectric response and exploring if and how they can reveal essential Weyl physics. We determine the complete anisotropic dielectric functions of TaAs and NbAs by combining spectroscopic ellipsometry and density functional theory (DFT). Parameterized Lorentz oscillators are reported from 1.2 - 6 eV (experiment) and 0 - 6 eV (DFT), and good agreement is shown between them. Both linear and nonlinear optical properties have been previously reported to reveal Weyl physics. We suggest that strong optical resonances from trivial bands are the likely origin of the large optical SHG previously reported at these energies. Furthermore, by comparing the contribution of a small k -space centered around the Weyl cones with the total linear dielectric function, we find that these contributions are highly anisotropic and are < 25% of the total dielectric function below 0.5 eV; abov1 eV, these contributions are negligible. Thus, the study of Weyl physics using optical techniques requires very low energies, and even there, a careful assessment is required in distinguishing the much smaller contributions of the Weyl bands from the dominant contributions of the trivial bands and Drude response to the total dielectric function.

36 MATERIALS SCIENCE↗

DOE OSTI2024

Anisotropic weak antilocalization in thin films of the Weyl semimetal TaAs

Device applications of topological semimetals await the development of epitaxial films in the ultrathin limit. Weak antilocalization (WAL) has been extensively utilized in the understanding of surface states in topological insulators and shows promise for use in elucidating the properties of thin film topological semimetals. Here, we report insights from WAL in the surface state and interface transport properties of our recently synthesized single-crystal-like thin films of the Weyl semimetal TaAs(001) grown on GaAs(001). We observe robust, anisotropic WAL in the magnetoconductance from 2 to 20 K in films from 10 to 200 nm thick. We link the anisotropic WAL magnetoconductance to anisotropic mobility stemming from film topography. We conclude that WAL in the films likely originates from the antilocalization of topological surface states. The WAL magnetoconductance is impacted by the film thickness and topography, solidifying the useful role of WAL in the study of topological semimetal/semiconductor heterointerfaces. Published by the American Physical Society 2024

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

DOE OSTI2024

Topological edge conduction induced by strong anisotropic exchange interactions

Here, we predict that an interplay between isotropic and anisotropic exchange interactions in a honeycomb lattice structure can lead to topological edge conduction when the anisotropic interaction is at least twice the strength of the isotropic interaction. For materials like Na 2 ⁢IrO 3 , such a strong anisotropic exchange interaction simultaneously induces a zigzag type of antiferromagnetic order that breaks the time-reversal symmetry of the topological edge conductor. We show that the electronic transport in such topological conductors will exhibit a quantized Hall conductance without any external magnetic field when the Fermi energy lies within a particular energy range.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

DOE OSTI2023

3D structure of anisotropic flow in small collision systems at energies available at the BNL Relativistic Heavy Ion Collider

Here, we present (3 + 1)-dimensional [(3 + 1)D] dynamical simulations of asymmetric nuclear collisions at the BNL Relativistic Heavy Ion Collider (RHIC). Employing a dynamical initial state model coupled to (3 + 1)D viscous relativistic hydrodynamics, we explore the rapidity dependence of anisotropic flow in the RHIC small system scan at 200 GeV center-of-mass energy. We calibrate parameters to describe central 3 He + Au collisions and make extrapolations to d + Au and p + Au collisions. Our calculations demonstrate that approximately 50% of the v 3 (p T ) difference between the measurements by the STAR and PHENIX Collaborations can be explained by the use of reference flow vectors from different rapidity regions. This emphasizes the importance of longitudinal flow decorrelation for anisotropic flow measurements in asymmetric nuclear collisions, and the need for (3 + 1)D simulations. We also present results for the beam energy dependence of particle spectra and anisotropic flow in d + Au collisions.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

DOE OSTI2020

Shuffling mode competition leads to directionally anisotropic mobility of faceted Σ11 boundaries in fcc metals

Faceted grain boundaries can migrate in interesting and unexpected ways. For example, faceted Σ11 <110> tilt grain boundaries were observed to exhibit mobility values that could be strongly dependent on the direction of migration. In order to understand whether this directionally-anisotropic mobility is a general phenomenon and to isolate mechanistic explanations for this behavior, molecular dynamics simulations of bicrystals evolved under an artificial driving force are used to study interface migration for a range of boundary plane inclination angles and temperatures in multiple face centered cubic metals (Al, Ni, and Cu). We find that directionally anisotropic mobility is active in a large fraction of these boundaries in Ni and Cu and should therefore impact the coarsening of polycrystalline materials. On the other hand, no such anisotropy is observed in any of the Al boundaries, showing that this behavior is material-dependent. Migration of the faceted boundaries is accomplished through transformation events at facet nodes and incommensurate boundary plane facets, which are termed shuffling modes. Three major shuffling modes have been identified, namely Shockley shuffling, slip plane shuffling, and disordered shuffling. A shift from the first two ordered modes to the third disordered mode is found to be responsible for reducing or removing directionally-anisotropic mobility, especially at the highest temperatures studied.

36 MATERIALS SCIENCE↗

DOE OSTI2023

Anisotropic superconductivity at KTaO 3 (111) interfaces

A two-dimensional, anisotropic superconductivity was recently found at the KTaO 3 (111) interfaces. The nature of the anisotropic superconducting transition remains a subject of debate. To investigate the origins of the observed behavior, we grew epitaxial KTaO 3 (111)-based heterostructures. We show that the superconductivity is robust against the in-plane magnetic field and violates the Pauli limit. We also show that the Cooper pairs are more resilient when the bias is along [11$\bar{2}$] (I ∥ [11$\bar{2}$]) and the magnetic field is along [1$\bar{1}$0] (B ∥ [1$\bar{1}$0]). We discuss the anisotropic nature of superconductivity in the context of electronic structure, orbital character, and spin texture at the KTaO 3 (111) interfaces. The results point to future opportunities to enhance superconducting transition temperatures and critical fields in crystalline, two-dimensional superconductors with strong spin-orbit coupling.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

DOE OSTI2020

Exceptional coupling in photonic anisotropic metamaterials for extremely low waveguide crosstalk

Electromagnetic coupling is ubiquitous in photonic systems and transfers optical signals from one device to the other, creating crosstalk between devices. While this allows the functionality of some photonic components such as couplers, it limits the integration density of photonic chips, and many approaches have been proposed to reduce the crosstalk. However, due to the wave nature of light, complete elimination of crosstalk between closely spaced, identical waveguides is believed to be impossible and has not been observed experimentally. Here we show an exceptional coupling that can completely suppresses the crosstalk utilizing highly anisotropic photonic metamaterials. The anisotropic dielectric perturbations in the metamaterial mutually cancel the couplings from different field components, resulting in an infinitely long coupling length. We demonstrate the extreme suppression of crosstalk via exceptional coupling on a silicon-on-insulator platform, which is compatible with a complementary metal-oxide-semiconductor process. The idea of exceptional coupling with anisotropic metamaterials can be applied to many other electromagnetic devices, and it could drastically increase the integration density of photonic chips.

Mia, Md Borhan (ORCID:0000000320851331)↗

DOE OSTI2025

Probing Anisotropic Cosmic Birefringence with Foreground-Marginalised SPT B-mode Likelihoods

In this work, we construct foreground-marginalised versions of the SPT-3G D1 and SPTpol cosmic microwave background (CMB) B-mode polarisation likelihoods. The compression is performed using the CMB-lite framework and we use the resulting data sets to constrain anisotropic cosmic birefringence, parametrised by the amplitude of a scale-invariant anisotropic birefringence spectrum, A CB . Using the new SPT-3G data we report a upper limit on of 95% upper limit on A CB of 1.2 x 10 -4 , which tightens to 0.53 x 10 -4 when imposing a prior on the amplitude of gravitational lensing based on CMB lensing reconstruction analyses. These are the tightest constraints on anisotropic birefringence from BB power spectrum measurements to-date, demonstrating the constraining power of the South Pole Telescope. The likelihoods used in this work are made publicly available at https://github.com/lbalkenhol/candl_data

Balkenhol, Lennart [Sorbonne Université, Paris (Fr↗

DOE OSTI2025

Anisotropic Turbulent Flows Observed in Above-the-loop-top Regions during Solar Flares

Abstract Solar flare above-the-loop-top (ALT) regions are vital for understanding solar eruptions and fundamental processes in plasma physics. Recent advances in three-dimensional (3D) magnetohydrodynamic (MHD) simulations have revealed unprecedented details on turbulent flows and MHD instabilities in flare ALT regions. Here, for the first time, we examine the observable anisotropic properties of turbulent flows in ALT by applying a flow-tracking algorithm on narrow-band extreme-ultraviolet images that are observed from the face-on viewing perspective. First, the results quantitatively confirm the previous observation that vertical motions dominate and that the anisotropic flows are widely distributed in the entire ALT region with the contribution from both upflows and downflows. Second, the anisotropy shows height-dependent features, with the most substantial anisotropy appearing at a certain middle height in ALT, which agrees well with the MHD modeling results where turbulent flows are caused by Rayleigh–Taylor-type instabilities in the ALT region. Finally, our finding suggests that supra-arcade downflows (SADs), the most prominently visible dynamical structures in ALT regions, are only one aspect of turbulent flows. Among these turbulent flows, we also report the antisunward-moving underdense flows that might develop due to MHD instabilities, as suggested by previous 3D flare models. Our results indicate that the entire flare fan displays group behavior of turbulent flows where the observational bright spikes and relatively dark SADs exhibit similar anisotropic characteristics.

Xie, Xiaoyan (ORCID:0009000705827807)↗

NASA NTRS1979

Anisotropic friction, deformation, and fracture of single-crystal silicon carbide at room temperature

Anisotropic friction, deformation, and fracture studies were conducted with /0001/, /10(-1)0/, and /11(-2)0/ silicon carbide surfaces in sliding contact with diamond. The experiments were conducted with loads of 0.1, 0.2, and 0.3 N at a sliding velocity of 3 mm/min in mineral oil or in dry argon at room temperature. The 1010 direction on the basal /0001/ plane exhibits the lowest coefficient of friction and the greatest resistance to abrasion for silicon carbide. Anisotropic friction and deformation of the /0001/, /10(-1)0/, and /11(-2)0/ silicon carbide surfaces are primarily controlled by the slip system /10(-1)0/ 11(-2)0. The anisotropic fracture during sliding on the basal plane is due to surface cracking along /10(-1)0/ and subsurface cracking along /0001/. The fracture during sliding on the /11(-2)0/ or /10(-1)0/ surfaces is due to surface cracking along /0001/ and /11(-2)0/ or /10(-1)-1 and to subsurface cracking along /10(-1)0/.

Miyoshi, K.↗

NASA NTRS1980

A mixed-mode crack analysis of rectilinear anisotropic solids using conservation laws of elasticity

A very simple and convenient method of analysis for studying two-dimensional mixed-mode crack problems in rectilinear anisotropic solids is presented. The analysis is formulated on the basis of conservation laws of anisotropic elasticity and of fundamental relationships in anisotropic fracture mechanics. The problem is reduced to a system of linear algebraic equations in mixed-mode stress intensity factors. One of the salient features of the present approach is that it can determine directly the mixed-mode stress intensity solutions from the conservation integrals evaluated along a path removed from the crack-tip region without the need of solving the corresponding complex near-field boundary value problem. Several examples with solutions available in the literature are solved to ensure the accuracy of the current analysis. This method is further demonstrated to be superior to other approaches in its numerical simplicity and computational efficiency. Solutions of more complicated and practical engineering problems dealing with the crack emanating from a circular hole in composites are presented also to illustrate the capacity of this method.

Wang, S. S.↗

NASA NTRS1982

Comparison of transport equations based on Maxwellian and bi-Maxwellian distributions for anisotropic plasmas

A wide variety of plasma flow conditions is found in aeronomy and space plasma physics. Transport equations based on an isotropic Maxwellian vilecity distribution function can be used to describe plasma flows which contain 'small' temperature anisotropies. However, for plasma flows characterized by large temperature anisotropies, transport equations based on an anisotropic bi-Maxwellian (or two-temperature) velocity distribution function are expected to provide a much better description of the plasma transport properties. The present investigation is concerned with the extent to which transport equations based on both Maxwellian and bi-Maxwellian series expansions can describe plasma flows characterized by non-Maxwellian velocity distributions, giving particular attention to a modelling of the anisotropic character of the distribution function. The obtained results should provide clues as to the extent to which a given series expansion can account for the anisotropic character of a plasma.

Barakat, A. R.↗

NASA NTRS1985

The effects of anisotropic free-stream turbulence on turbulent boundary layer behavior

The effects of near-isotropic and highly anisotropic free-stream turbulence on mean flow properties of the turbulence structure of turbulent boundary layers in a near zero pressure gradient flow has been experimentally evaluated. Turbulence levels vary from 0.5% to 8.0% and the momentum thickness Reynolds number varies from 800 to 1100. The results indicate that the effects of free-stream turbulence on the classical boundary layer properties for near-isotropic turbulence which have been published by other investigators are similar to the case of highly anisotropic turbulence fields, while the effects of free-stream turbulence on the properties of the turbulent structure within the boundary layer for the case of near-isotropic turbulence are quite different compared to the highly anisotropic case.

Liang-Wei, F.↗

NASA NTRS1985

Model-size reduction technique for the analysis of symmetric anisotropic structures

A two-step computational procedure is presented for reducing the size of the analysis model for an anisotropic symmetric structure to that of the corresponding orthotropic structure. The key elements of the procedure are: (1) decomposition of the stiffness matrix into the sum of an orthotropic and nonorthotropic (anisotropic) parts; and (2) successive application of the finite element method and the classical Rayleigh-Ritz technique. The finite element method is first used to generate few global approximation vectors (or modes). Then the amplitudes of these modes are computed by using the Rayleigh-Ritz technique. The global approximation vectors are selected to be the solution corresponding to zero nonorthotropic matrix and its various-order derivatives with respect to an anisotropic tracing parameter (identifying the nonorthotropic material coefficients). The size of the analysis model used in generating the global approximation vectors is identical to that of the corresponding orthotropic structure. The effectiveness of the proposed technique is demonstrated by means of numerical examples and its potential for solving other quasi-symmetric problems is discussed.

Noor, A. K.↗

NASA NTRS1987

Anisotropic transport in modulation doped quantum well structures

The degree of anisotropy in the anisotropic electron transport that has been observed in GaAs modulation-doped quantum wells grown by MBE on Al(0.3)Ga(0.7)As is related to the thickness and growth parameters of this substrate, which is grown just prior to the inverted interface. It is presently observed that the inverted interface has an anisotropic roughness which affects the 77 K low field electron transport parallel to the interface, and gives rise to anisotropic electron scattering in the GaAs modulation-doped quantum well.

Radulescu, D. C.↗